FN Thomson Reuters Web of Knowledge™
VR 1.0
PT J
AU Yoo, E
   Kim, J
   Hosono, E
   Zhou, H
   Kudo, T
   Honma, I
AF Yoo, EunJoo
   Kim, Jedeok
   Hosono, Eiji
   Zhou, Hao-shen
   Kudo, Tetsuichi
   Honma, Itaru
TI Large reversible Li storage of graphene nanosheet families for use in
   rechargeable lithium ion batteries
SO NANO LETTERS
LA English
DT Article
ID WALLED CARBON NANOTUBES; P-N-JUNCTIONS; TRANSPORT; ANODE; INTERCALATION;
   GRAPHITE; BEHAVIOR; SHEETS; FIELD; SIZE
AB The lithium storage properties of graphene nanosheet (GNS) materials as high capacity anode materials for rechargeable lithium secondary batteries (LIB) were investigated. Graphite is a practical anode material used for LIB, because of its capability for reversible lithium ion intercalation in the layered crystals, and the structural similarities of GNS to graphite may provide another type of intercalation anode compound. While the accommodation of lithium in these layered compounds is influenced by the layer spacing between the graphene nanosheets, control of the intergraphene sheet distance through interacting molecules such as carbon nanotubes (CNT) or fullerenes (C(60)) might be crucial for enhancement of the storage capacity. The specific capacity of GNS was found to be 540 mAh/g, which is much larger than that of graphite, and this was increased up to 730 mAh/g and 784 mAh/g, respectively, by the incorporation of macromolecules of CNT and C(60) to the GNS.
C1 [Yoo, EunJoo; Hosono, Eiji; Honma, Itaru] Natl Inst Adv Ind Sci & Technol, Energy Technol Res Inst, Tsukuba, Ibaraki 3058568, Japan.
   [Kim, Jedeok] Natl Inst Mat Sci, Nanoion Mat Grp, Tsukuba, Ibaraki 3050044, Japan.
RP Honma, I (reprint author), Natl Inst Adv Ind Sci & Technol, Energy Technol Res Inst, Umezono 1-1-1,Cent 2, Tsukuba, Ibaraki 3058568, Japan.
EM i.homma@aist.go.jp
RI KIM, Jedeok/H-2802-2011; Hosono, Eiji/M-8402-2013
FU New Energy and Industrial Technology Development Organization Japan
FX This work was supported by the New Energy and Industrial Technology
   Development Organization Japan under a grant for Research and
   Development of Nanodevices for Practical Utilization of Nanotechnology
   (Nanotech Challenge Project).
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NR 29
TC 1330
Z9 1374
U1 269
U2 1641
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2008
VL 8
IS 8
BP 2277
EP 2282
DI 10.1021/nl800957b
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 337MR
UT WOS:000258440700028
PM 18651781
ER

PT J
AU Wu, ZS
   Ren, WC
   Wen, L
   Gao, LB
   Zhao, JP
   Chen, ZP
   Zhou, GM
   Li, F
   Cheng, HM
AF Wu, Zhong-Shuai
   Ren, Wencai
   Wen, Lei
   Gao, Libo
   Zhao, Jinping
   Chen, Zongping
   Zhou, Guangmin
   Li, Feng
   Cheng, Hui-Ming
TI Graphene Anchored with Co3O4 Nanoparticles as Anode of Lithium Ion
   Batteries with Enhanced Reversible Capacity and Cyclic Performance
SO ACS NANO
LA English
DT Article
DE graphene; cobalt oxide; nanomaterial; anode; lithium-ion batteries;
   cyclic performance
ID NEGATIVE ELECTRODE MATERIAL; COBALT OXIDE COMPOSITES; HIGH-QUALITY
   GRAPHENE; SN-C COMPOSITE; ELECTROCHEMICAL PERFORMANCE; STORAGE
   PROPERTIES; FACILE SYNTHESIS; GAS SENSORS; LI STORAGE; CARBON
AB We report a facile strategy to synthesize the nanocomposite of Co3O4 nanoparticles anchored on conducting graphene as an advanced anode material for high-performance lithium-ion batteries. The Co3O4 nanoparticles obtained are 10-30 nm in size and homogeneously anchor on graphene sheets as spacers to keep the neighboring sheets separated. This Co3O4/graphene nanocomposite displays superior Li-battery performance with large reversible capacity, excellent cyclic performance, and good rate capability, highlighting the importance of the anchoring of nanopartides on graphene sheets for maximum utilization of electrochemically active Co3O4 nanopartides and graphene for energy storage applications in high-performance lithium-ion batteries.
C1 [Wu, Zhong-Shuai; Ren, Wencai; Wen, Lei; Gao, Libo; Zhao, Jinping; Chen, Zongping; Zhou, Guangmin; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
RP Ren, WC (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM wcren@imr.ac.cn; cheng@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Chen, Zongping/G-6679-2012; Zhou,
   guangmin/J-6020-2013; Wu, Zhong-Shuai/F-1978-2014; Li, Feng/C-9991-2010;
   Gao, Libo/G-5928-2015
OI Gao, Libo/0000-0002-7822-9812
FU Ministry of Science and Technology of China [2006CB932703]; National
   Science Foundation of China [50872136, 50921004]; Chinese Academy of
   Sciences [KJCX2-YW-231]
FX This work was supported by Ministry of Science and Technology of China
   (No. 2006CB932703), National Science Foundation of China (Nos. 50872136
   and 50921004), and Chinese Academy of Sciences (No. KJCX2-YW-231).
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NR 57
TC 1118
Z9 1139
U1 317
U2 1413
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUN
PY 2010
VL 4
IS 6
BP 3187
EP 3194
DI 10.1021/nn100740x
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 612HU
UT WOS:000278888600030
PM 20455594
ER

PT J
AU Wang, HL
   Cui, LF
   Yang, YA
   Casalongue, HS
   Robinson, JT
   Liang, YY
   Cui, Y
   Dai, HJ
AF Wang, Hailiang
   Cui, Li-Feng
   Yang, Yuan
   Casalongue, Hernan Sanchez
   Robinson, Joshua Tucker
   Liang, Yongye
   Cui, Yi
   Dai, Hongjie
TI Mn3O4-Graphene Hybrid as a High-Capacity Anode Material for Lithium Ion
   Batteries
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID GRAPHENE SHEETS; PERFORMANCE; ELECTRODES; NANOTUBES; STORAGE; OXIDE
AB We developed two-step solution-phase reactions to form hybrid materials of Mn3O4 nanoparticles on reduced graphene oxide (RGO) sheets for lithium ion battery applications. Selective growth of Mn3O4 nanoparticles on RGO sheets, in contrast to free particle growth in solution, allowed for the electrically insulating Mn3O4 nanoparticles to be wired up to a current collector through the underlying conducting graphene network. The Mn3O4 nanoparticles formed on RGO show a high specific capacity up to similar to 900 mAh/g, near their theoretical capacity, with good rate capability and cycling stability, owing to the intimate interactions between the graphene substrates and the Mn3O4 nanoparticles grown atop. The Mn3O4/RGO hybrid could be a promising candidate material for a high-capacity, low-cost, and environmentally friendly anode for lithium ion batteries. Our growth-on-graphene approach should offer a new technique for the design and synthesis of battery electrodes based on highly insulating materials.
C1 [Cui, Li-Feng; Yang, Yuan; Cui, Yi] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA.
   [Wang, Hailiang; Casalongue, Hernan Sanchez; Robinson, Joshua Tucker; Liang, Yongye; Dai, Hongjie] Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
   [Wang, Hailiang; Casalongue, Hernan Sanchez; Robinson, Joshua Tucker; Liang, Yongye; Dai, Hongjie] Stanford Univ, Adv Mat Lab, Stanford, CA 94305 USA.
RP Cui, Y (reprint author), Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA.
EM yicui@stanford.edu; hdai@stanford.edu
RI Liang, Yongye/D-1099-2010; Liang, Yongye/D-9275-2012; Cui,
   Yi/L-5804-2013
OI Cui, Yi/0000-0002-6103-6352
FU Office of Naval Research; NSF [CHE-0639053]; KAUST; Stanford Graduate
   Fellowship
FX This work was supported in part by the Office of Naval Research, NSF
   award CHE-0639053 and a KAUST Investigator Award H. Wang and Y. Yang
   acknowledge financial support from Stanford Graduate Fellowship.
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NR 24
TC 975
Z9 989
U1 172
U2 1009
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD OCT 13
PY 2010
VL 132
IS 40
BP 13978
EP 13980
DI 10.1021/ja105296a
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 660RD
UT WOS:000282660100010
PM 20853844
ER

PT J
AU Zhou, GM
   Wang, DW
   Li, F
   Zhang, LL
   Li, N
   Wu, ZS
   Wen, L
   Lu, GQ
   Cheng, HM
AF Zhou, Guangmin
   Wang, Da-Wei
   Li, Feng
   Zhang, Lili
   Li, Na
   Wu, Zhong-Shuai
   Wen, Lei
   Lu, Gao Qing (Max)
   Cheng, Hui-Ming
TI Graphene-Wrapped Fe3O4 Anode Material with Improved Reversible Capacity
   and Cyclic Stability for Lithium Ion Batteries
SO CHEMISTRY OF MATERIALS
LA English
DT Article
ID ELECTRODE MATERIALS; STORAGE PROPERTIES; ENERGY-STORAGE; HOLLOW SPHERES;
   CARBON; PERFORMANCE; LI; COMPOSITE; NANOPARTICLES; OXIDE
AB A well-organized flexible interleaved composite of graphene nanosheets (GNSs) decorated with Fe3O4 particles was synthesized through in situ reduction of iron hydroxide between GNSs. The GNS/Fe3O4 composite shows a reversible specific capacity approaching 1026 mA h(-1) g(-1) after 30 cycles at 35 mA g(-1) 580 mAh g(-1) after 100 cycles at 700 mA g(-1) as well as improved cyclic stability and excellent rate capability. The multifunctional features of the GNS/Fe3O4 composite are considered as follows: (i) GNSs play a "flexible confinement" function to enwrap Fe3O4 particles, which can compensate for the volume change of Fe3O4 and prevent the detachment and agglomeration of pulverized Fe3O4, thus extending the cycling life of the electrode; (ii) GNSs provide a large contact surface for individual dispersion of well-adhered Fe3O4 particles and act as an excellent conductive agent to provide a highway for electron transport, improving the accessible capacity; (iii) Fe3O4 particles separate GNSs and prevent their restacking thus improving the adsorption and immersion of electrolyte on the surface of electroactive material; and (iv) the porosity formed by lateral GNSs and Fe3O4 particles facilitates ion transportation. As a result, this unique laterally confined GNS/Fe3O4 composite can dramatically improve the cycling stability and the rate capability of Fe3O4 as an anode material for lithium ion batteries.
C1 [Zhou, Guangmin; Li, Feng; Zhang, Lili; Li, Na; Wu, Zhong-Shuai; Wen, Lei; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
   [Wang, Da-Wei; Lu, Gao Qing (Max)] Univ Queensland, AIBN, ARC Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn; cheng@imr.ac.cn
RI WANG, DAWEI/E-5074-2010; Cheng, Hui-Ming/B-8682-2012; Lu, Gao
   Qing/A-2859-2008; Zhou, guangmin/J-6020-2013; Wu,
   Zhong-Shuai/F-1978-2014; Wei, Zhanhua/D-7544-2013; Li, Feng/C-9991-2010
OI WANG, DAWEI/0000-0002-6651-4261; Lu, Gao Qing/0000-0002-1456-6983; Wei,
   Zhanhua/0000-0003-2687-0293; 
FU National Science Foundation of China [50921004, 50632040]; K.C. Wong
   Education Foundation, Hong Kong; Chinese Academy of Sciences
   [KGCX2-YW-231]
FX This work was supported by National Science Foundation of China
   (Nos.50921004 and 50632040), K.C. Wong Education Foundation, Hong Kong,
   and Chinese Academy of Sciences (KGCX2-YW-231). We thank Mr. L. B. Gao,
   B. L. Liu, and S. F. Pei for helpful discussion.; Dr. D. M. Tang and Dr.
   C. B. Jiang for TEM support; and Prof. Peter Thrower for his
   constructive advice.
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NR 60
TC 897
Z9 914
U1 217
U2 1132
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0897-4756
J9 CHEM MATER
JI Chem. Mat.
PD SEP 28
PY 2010
VL 22
IS 18
BP 5306
EP 5313
DI 10.1021/cm101532x
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 650YX
UT WOS:000281891900022
ER

PT J
AU Sun, YQ
   Wu, QO
   Shi, GQ
AF Sun, Yiqing
   Wu, Qiong
   Shi, Gaoquan
TI Graphene based new energy materials
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID LITHIUM-ION BATTERIES; SENSITIZED SOLAR-CELLS; SOLUTION-PROCESSABLE
   GRAPHENE; PERFORMANCE ANODE MATERIALS; OXYGEN REDUCTION REACTION;
   LIQUID-PHASE EXFOLIATION; HIGH-RATE CAPABILITY; GRAPHITE OXIDE;
   ELECTROCHEMICAL PROPERTIES; FUEL-CELLS
AB Graphene, a one-atom layer of graphite, possesses a unique two-dimensional (2D) structure, high conductivity and charge carrier mobility, huge specific surface area, high transparency and great mechanical strength. Thus, it is expected to be an ideal material for energy storage and conversion. During the past several years, a variety of graphene based materials (GBMs) have been successfully prepared and applied in supercapacitors, lithium ion batteries, water splitting, electrocatalysts for fuel cells, and solar cells. In this review, we will summarize the recent advances in the synthesis and applications of GBMs in these energy related systems. The challenges and prospects of graphene based new energy materials are also discussed.
C1 [Sun, Yiqing; Wu, Qiong; Shi, Gaoquan] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
RP Sun, YQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM gshi@tsinghua.edu.cn
RI Wu, Qiong/F-1515-2015
OI Wu, Qiong/0000-0001-8768-7738
FU Natural Science Foundation of China [50873052, 20774056]
FX This work was supported by the Natural Science Foundation of China
   (50873052 and 20774056).
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NR 221
TC 822
Z9 834
U1 238
U2 1354
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD APR
PY 2011
VL 4
IS 4
BP 1113
EP 1132
DI 10.1039/c0ee00683a
PG 20
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 743EV
UT WOS:000289001400003
ER

PT J
AU Ji, LW
   Lin, Z
   Alcoutlabi, M
   Zhang, XW
AF Ji, Liwen
   Lin, Zhan
   Alcoutlabi, Mataz
   Zhang, Xiangwu
TI Recent developments in nanostructured anode materials for rechargeable
   lithium-ion batteries
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID WALLED CARBON NANOTUBES; ELECTROCHEMICAL ENERGY-STORAGE;
   NEGATIVE-ELECTRODE MATERIAL; CORE-SHELL NANOWIRES; ONE-POT SYNTHESIS;
   THIN-FILM ANODE; ALLOY-GRAPHITE COMPOSITE; HIGH-QUALITY GRAPHENE;
   HIGH-RATE CAPABILITY; HIGH-CAPACITY
AB In this paper, the use of nanostructured anode materials for rechargeable lithium-ion batteries (LIBs) is reviewed. Nanostructured materials such as nano-carbons, alloys, metal oxides, and metal sulfides/nitrides have been used as anodes for next-generation LIBs with high reversible capacity, fast power capability, good safety, and long cycle life. This is due to their relatively short mass and charge pathways, high transport rates of both lithium ions and electrons, and other extremely charming surface activities. In this review paper, the effect of the nanostructure on the electrochemical performance of these anodes is presented. Their synthesis processes, electrochemical properties, and electrode reaction mechanisms are also discussed. The major goals of this review are to give a broad overview of recent scientific researches and developments of anode materials using novel nanoscience and nanotechnology and to highlight new progresses in using these nanostructured materials to develop high-performance LIBs. Suggestions and outlooks on future research directions in this field are also given.
C1 [Ji, Liwen; Lin, Zhan; Alcoutlabi, Mataz; Zhang, Xiangwu] N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
RP Ji, LW (reprint author), N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
EM xiangwu_zhang@ncsu.edu
RI Lin, Zhan/C-6806-2011; Zhang, Xiangwu/F-1013-2011
OI Zhang, Xiangwu/0000-0002-6236-6281
FU Department of Energy [DE-EE0001177]; National Science Foundation
   [EEC-08212121]
FX We thank funding supports by the Department of Energy (NO. DE-EE0001177)
   and the ERC Program of the National Science Foundation Award (No.
   EEC-08212121). We also thank Mr Richard Padbury and Mr Yingfang Yao for
   helpful discussions and revisions.
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NR 331
TC 674
Z9 686
U1 277
U2 1262
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD AUG
PY 2011
VL 4
IS 8
BP 2682
EP 2699
DI 10.1039/c0ee00699h
PG 18
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 798NA
UT WOS:000293213600009
ER

PT J
AU Wang, GX
   Shen, XP
   Yao, J
   Park, J
AF Wang, Guoxiu
   Shen, Xiaoping
   Yao, Jane
   Park, Jinsoo
TI Graphene nanosheets for enhanced lithium storage in lithium ion
   batteries
SO CARBON
LA English
DT Article
ID GRAPHITE OXIDE; CARBON-FILMS; MECHANISM; INSERTION; CELLS
AB Graphene nanosheets were synthesized in large quantities using a chemical approach. Field emission electron microscope observation revealed that loose graphene nanosheets agglomerated and crumpled naturally into shapes resembling flower-petals. High resolution transmission electron microscope analysis, Raman spectroscopy and ultraviolet-visible spectroscopy measurements confirmed the graphitic crystalline structure of the graphene nanosheets. The nanosheets exhibited an enhanced lithium storage capacity as anodes in lithium-ion cells and good cyclic performance. (C) 2009 Elsevier Ltd. All rights reserved.
C1 [Wang, Guoxiu; Shen, Xiaoping; Yao, Jane; Park, Jinsoo] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
RP Wang, GX (reprint author), Univ Wollongong, Sch Mech Mat & Mechatron Engn, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM gwang@uow.edu.au
FU Australian Research Council (ARC) [D00772999]
FX Financial support from the Australian Research Council (ARC) through ARC
   Discovery Project D00772999 is gratefully acknowledged.
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NR 24
TC 591
Z9 611
U1 76
U2 424
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD JUL
PY 2009
VL 47
IS 8
BP 2049
EP 2053
DI 10.1016/j.carbon.2009.03.053
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 456OG
UT WOS:000266855800020
ER

PT J
AU Zhu, XJ
   Zhu, YW
   Murali, S
   Stollers, MD
   Ruoff, RS
AF Zhu, Xianjun
   Zhu, Yanwu
   Murali, Shanthi
   Stollers, Meryl D.
   Ruoff, Rodney S.
TI Nanostructured Reduced Graphene Oxide/Fe2O3 Composite As a
   High-Performance Anode Material for Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE reduced graphene oxide; Fe2O3; anode; lithium ion battery; homogeneous
   coprecipitation
ID IRREVERSIBLE CAPACITIES; STORAGE DEVICES; ALPHA-FE2O3; INSERTION; OXIDE;
   ELECTRODES; REDUCTION; NANOTUBES; GRAPHITE; HYBRID
AB Reduced graphene oxide/Fe2O3 composite was prepared using a facile two-step synthesis by homogeneous coprecipitation and subsequent reduction of the G-O with hydrazine under microwave irradiation to yield reduced graphene oxide (RG-O) platelets decorated with Fe2O3 nanoparticles. As an anode material for Li-ion batteries, the RG-O/Fe2O3 composite exhibited discharge and charge capacities of 1693 and 1227 mAh/g, respectively, normalized to the mass of Fe2O3 In the composite (and 1355 and 982 mAh/g, respectively, based on the total mass of the composite), with good cycling performance and rate capability. Characterization shows that the Fe2O3 nanoparticles are uniformly distributed on the surface of the RG-O platelet in the composite. The total specific capacity of RG-O/Fe2O3 is higher than the sum of pure RG-O and nanoparticle Fe2O3, indicating a positive synergistic effect of RG-O and Fe2O3 on the improvement of electrochemical performance. The synthesis approach presents a promising route for a large-scale production of RG-O platelet/metal oxide nanoparticle composites as electrode materials for Li-ion batteries.
C1 [Zhu, Xianjun; Zhu, Yanwu; Murali, Shanthi; Stollers, Meryl D.; Ruoff, Rodney S.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA.
   [Zhu, Xianjun; Zhu, Yanwu; Murali, Shanthi; Stollers, Meryl D.; Ruoff, Rodney S.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA.
   [Zhu, Xianjun] Cent China Normal Univ, Coll Chem, Wuhan 430079, Hubei, Peoples R China.
RP Ruoff, RS (reprint author), Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA.
EM r.ruoff@mail.utexas.edu
RI Wei, Zhanhua/D-7544-2013; Zhu, Yanwu/C-8979-2012; Ruoff,
   Rodney/K-3879-2015
OI Wei, Zhanhua/0000-0003-2687-0293; 
FU University of Texas at Austin; Texas Nanotechnology Research Superiority
   Initiative (TNRSI)/SWAN; Department of Energy Office of Science
   [DEFG02-07ER46377]; National Science Foundation [CBET-0553649]; China
   Scholarship Council; SRF for ROCS, SEM
FX This work was supported by The University of Texas at Austin, the Texas
   Nanotechnology Research Superiority Initiative (TNRSI)/SWAN, the
   Department of Energy Office of Science award DEFG02-07ER46377, the
   National Science Foundation award CBET-0553649, the China Scholarship
   Council Fellowship, and the Project sponsored by SRF for ROCS, SEM.
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NR 28
TC 575
Z9 584
U1 145
U2 789
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD APR
PY 2011
VL 5
IS 4
BP 3333
EP 3338
DI 10.1021/nn200493r
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 753CJ
UT WOS:000289742100107
PM 21443243
ER

PT J
AU Wu, ZS
   Ren, WC
   Xu, L
   Li, F
   Cheng, HM
AF Wu, Zhong-Shuai
   Ren, Wencai
   Xu, Li
   Li, Feng
   Cheng, Hui-Ming
TI Doped Graphene Sheets As Anode Materials with Superhigh Rate and Large
   Capacity for Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE doped graphene; anode; lithium ion batteries; high rate; nitrogen; boron
ID HIGH-RATE CAPABILITY; ELECTROCHEMICAL CAPACITORS; CARBON NANOTUBES; LI
   STORAGE; ELECTRODES; ENERGY; FILMS; PERFORMANCE; NANOSHEETS; DIFFUSION
AB One great challenge in the development of lithium ion batteries is to simultaneously achieve high power and large energy capacity at fast charge and discharge rates for several minutes to seconds. Here we show that nitrogen- or boron-doped graphene can be used as a promising anode for high-power and high-energy lithium ion batteries under high-rate charge and discharge conditions. The doped graphene shows a high reversible capacity of >1040 mAh g(-1) at a low rate of 50 mA g(-1). More importantly, it can be quickly charged and discharged in a very short time of 1 h to several tens of seconds together with high-rate capability and excellent long-term cyclability. For example, a very high capacity of similar to 199 and 235 mAh g(-1) was obtained for the N-doped graphene and B-doped graphene at 25 A g(-1) (about 30 s to full charge). We believe that the unique two-dimensional structure, disordered surface morphology, heteroatomic defects, better electrode/electrolyte wettability, increased intersheet distance, improved electrical conductivity, and thermal stability of the doped graphene are beneficial to rapid surface Li+ absorption and ultrafast Li+ diffusion and electron transport, and thus make the doped materials superior to those of pristine chemically derived graphene and other carbonaceous materials.
C1 [Wu, Zhong-Shuai; Ren, Wencai; Xu, Li; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China.
RP Ren, WC (reprint author), Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM wcren@imr.ac.cn; cheng@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Wu, Zhong-Shuai/F-1978-2014; Li,
   Feng/C-9991-2010
FU National Science Foundation of China [50872136, 50972147, 50921004,
   50632040]; Chinese Academy of Sciences [KJCX2-YW-231]
FX This work was supported by National Science Foundation of China (Nos.
   50872136, 50972147, 50921004, and 50632040) and Chinese Academy of
   Sciences (No. KJCX2-YW-231). We also thank Ms. X. H. Shao for the
   assistance with STEM measurements.
CR Wang B, 2010, J MATER CHEM, V20, P10661, DOI 10.1039/c0jm01941k
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NR 49
TC 564
Z9 569
U1 125
U2 632
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUL
PY 2011
VL 5
IS 7
BP 5463
EP 5471
DI 10.1021/nn2006249
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 796ES
UT WOS:000293035200022
PM 21696205
ER

PT J
AU Chang, K
   Chen, WX
AF Chang, Kun
   Chen, Weixiang
TI L-Cysteine-Assisted Synthesis of Layered MoS2/Graphene Composites with
   Excellent Electrochemical Performances for Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE L-cysteine-assisted; MoS2/graphene composites; anode material; lithium
   ion battery; ac impedance
ID ANODE MATERIAL; TUNGSTEN DISULFIDE; TUNABLE SYNTHESIS; MOS2; GRAPHENE;
   STORAGE; NANOSTRUCTURES; NANOPARTICLES; ELECTRODES; NANOSHEETS
AB A facile process was developed to synthesize layered MoS2/graphene (MoS2/G) composites by an L-cysteine-assisted solution-phase method, in which sodium molybdate, as-prepared graphene oxide (GO), and L-cysteine were used as starting materials. As-prepared MoS2/G was then fabricated into layered MoS2/G composites after annealing in a H-2/N-2 atmosphere at 800 degrees C for 2 h. The samples were systematically investigated by X-ray diffraction, field emission scanning electron microscopy, energy dispersive X-ray spectroscopy, and high-resolution transmission electron microscopy. Electrochemical performances were evaluated In two-electrode cells versus metallic lithium. It Is demonstrated that the obtained MoS2/G composites show three-dimensional architecture and excellent electrochemical performances as anode materials for U-ion batteries. The MoS2/G composite with a Mo:C molar ratio of 1:2 exhibits the highest specific capacity of similar to 1100 mAh/g at a current of 100 mA/g, as well as excellent cycling stability and high-rate capability. The superior electrochemical performances of MoS2/G composites as U-Ion battery anodes are attributed to their robust composite structure and the synergistic effects between layered MoS2 and graphene.
C1 [Chang, Kun; Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
EM weixiangchen@zju.edu.cn
RI Chang, Kun/I-1361-2012
FU Zhejiang Provincial Natural Science Foundation of China [Y407030,
   Y4100119]; Zhejiang Provincial Science and Technology Program for Public
   Interest [2011C31G2010027]; Ministry of Science and Technology of China
   [2010CB635116]
FX This work was supported by the Zhejiang Provincial Natural Science
   Foundation of China (Y407030, Y4100119), the Zhejiang Provincial Science
   and Technology Program for Public Interest (2011C31G2010027), and 973
   Fundamental Research Program from the Ministry of Science and Technology
   of China (2010CB635116).
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TC 496
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U1 178
U2 875
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUN
PY 2011
VL 5
IS 6
BP 4720
EP 4728
DI 10.1021/nn200659w
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 783AZ
UT WOS:000292055200055
PM 21574610
ER

PT J
AU Wu, ZS
   Zhou, GM
   Yin, LC
   Ren, W
   Li, F
   Cheng, HM
AF Wu, Zhong-Shuai
   Zhou, Guangmin
   Yin, Li-Chang
   Ren, Wencai
   Li, Feng
   Cheng, Hui-Ming
TI Graphene/metal oxide composite electrode materials for energy storage
SO NANO ENERGY
LA English
DT Review
DE Graphene; Metal oxide; Composite; Energy storage; Lithium ion battery;
   Supercapacitor
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIAL; EXFOLIATED GRAPHITE
   OXIDE; CHEMICAL-VAPOR-DEPOSITION; HIGH-QUALITY GRAPHENE; FUNCTIONALIZED
   GRAPHENE; ELECTROCHEMICAL CAPACITORS; REVERSIBLE CAPACITY; CYCLIC
   PERFORMANCE; FE3O4-GRAPHENE NANOCOMPOSITES
AB Recent progress on graphene/metal oxide composites as advanced electrode materials in lithium ion batteries (LIBs) and electrochemical capacitors (ECs) is described, highlighting the importance of synergistic effects between graphene and metal oxides and the beneficial role of graphene in composites for LIBs and ECs. It is demonstrated that, when the composites are used as electrode materials for LIBs and ECs, compared to their individual constituents, graphene/metal oxide composites with unique structural variables such as anchored, wrapped, encapsulated, sandwich, layered and mixed models have a significant improvement in their electrochemical properties such as high capacity, high rate capability and excellent cycling stability. First, an introduction on the properties, synthesis strategies and use of graphene is briefly given, followed by a state-of-the-art review on the preparation of graphene/metal oxide composites and their electrochemical properties in LIBs and ECs. Finally, the prospects and future challenges of graphene/metal oxide composites for energy storage are discussed. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Wu, Zhong-Shuai; Zhou, Guangmin; Yin, Li-Chang; Ren, Wencai; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
   [Wu, Zhong-Shuai] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Cheng, HM (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM cheng@imr.ac.cn
RI Zhou, guangmin/J-6020-2013; Wu, Zhong-Shuai/F-1978-2014; Cheng,
   Hui-Ming/B-8682-2012; Li, Feng/C-9991-2010
FU Key Research Program of Ministry of Science and Technology, China
   [2011CB932604]; National Natural Science Foundation of China [50921004];
   Chinese Academy Sciences [KGCX2-YW-231]; Jinlu Limited
FX This work was supported by the Key Research Program of Ministry of
   Science and Technology, China (no. 2011CB932604), the National Natural
   Science Foundation of China (no. 50921004), Chinese Academy Sciences
   (KGCX2-YW-231) and the Jinlu Limited.
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NR 196
TC 459
Z9 470
U1 271
U2 1276
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
EI 2211-3282
J9 NANO ENERGY
JI Nano Energy
PD JAN
PY 2012
VL 1
IS 1
BP 107
EP 131
DI 10.1016/j.nanoen.2011.11.001
PG 25
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 132EF
UT WOS:000318050000011
ER

PT J
AU Pan, DY
   Wang, S
   Zhao, B
   Wu, MH
   Zhang, HJ
   Wang, Y
   Jiao, Z
AF Pan, Dengyu
   Wang, Song
   Zhao, Bing
   Wu, Minghong
   Zhang, Haijiao
   Wang, Yong
   Jiao, Zheng
TI Li Storage Properties of Disordered Graphene Nanosheets
SO CHEMISTRY OF MATERIALS
LA English
DT Article
ID LITHIUM-ION BATTERIES; EXFOLIATED GRAPHITE OXIDE; CARBON; INSERTION;
   SHEETS; FILMS; ANODE; PERFORMANCE; MECHANISM; ELECTRODE
AB Graphene has aroused intensive interest because of its unique structure, superior properties, and various promising applications. Graphene nanostructures with significant disorder and defects have been considered to be poor materials because disorder and defects lower their electrical conductivity. In this paper, we report that highly disordered graphene nanosheets can find promising applications in high-capacity Li ion batteries because of their exceptionally high reversible capacities (794-1054 mA h/g) and good cyclic stability. To understand the Li storage mechanism of graphene nanosheets, we have prepared graphene nanosheets with structural parameters tunable via different reduction methods including hydrazine reduction, low-temperature pyrolysis, and electron beam irradiation. The effects of these parameters on Li storage properties were investigated systematically, A key structural parameter, Raman intensity ratio of D bands to G bands, has been identified to evaluate the reversible capacity. The greatly enhanced capacity in disordered graphene nanosheets is suggested to be mainly ascribed to additional reversible storage sites such as edges and other defects.
C1 [Pan, Dengyu; Zhang, Haijiao] Shanghai Univ, Inst Nanochem & Nanobiol, Shanghai 201800, Peoples R China.
   [Wang, Song; Zhao, Bing; Wu, Minghong; Wang, Yong; Jiao, Zheng] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 201800, Peoples R China.
RP Pan, DY (reprint author), Shanghai Univ, Inst Nanochem & Nanobiol, Shanghai 201800, Peoples R China.
EM dypan617@shu.edu.cn; bzhao@shu.edu.cn
RI WANG, Yong/B-1125-2012
FU Natural Science Foundation of China [10774118, 40830744, 50701029];
   Shanghai Pujiang Program [07pj14042]; Shanghai Leading Academic
   Discipline Project [S30109];  [NCET-05-0434]
FX This work is supported by Natural Science Foundation of China (10774118,
   40830744, 50701029). NCET-05-0434, Shanghai Pujiang Program (07pj14042
   the Shanghai Committee of Science and Technology (08520512200), and
   Shanghai Leading Academic Discipline Project (S30109).
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0897-4756
J9 CHEM MATER
JI Chem. Mat.
PD JUL 28
PY 2009
VL 21
IS 14
BP 3136
EP 3142
DI 10.1021/cm900395k
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 473AD
UT WOS:000268174400019
ER

PT J
AU Pumera, M
AF Pumera, Martin
TI Graphene-based nanomaterials for energy storage
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID LITHIUM ION BATTERIES; CARBON NANOTUBES; HYDROGEN STORAGE; GRAPHITE
   NANOFIBERS; COMPOSITE FILMS; ANODE MATERIALS; NITRIC-ACID; LI STORAGE;
   SUPERCAPACITORS; NANOSTRUCTURES
AB There is enormous interest in the use of graphene-based materials for energy storage. This article discusses the progress that has been accomplished in the development of chemical, electrochemical, and electrical energy storage systems using graphene. We summarize the theoretical and experimental work on graphene-based hydrogen storage systems, lithium batteries, and supercapacitors. Even though the research on the use of graphene for energy storage began very recently, the explosive growth of the research conducted in this area makes this minireview timely.
C1 Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore 637371, Singapore.
RP Pumera, M (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, 21 Nanyang Link, Singapore 637371, Singapore.
EM pumera@ntu.edu.sg
RI Pumera, Martin/F-2724-2010
OI Pumera, Martin/0000-0001-5846-2951
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NR 78
TC 420
Z9 430
U1 76
U2 492
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD MAR
PY 2011
VL 4
IS 3
BP 668
EP 674
DI 10.1039/c0ee00295j
PG 7
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 729CE
UT WOS:000287924700005
ER

PT J
AU Lian, PC
   Zhu, XF
   Liang, SZ
   Li, Z
   Yang, WS
   Wang, HH
AF Lian, Peichao
   Zhu, Xuefeng
   Liang, Shuzhao
   Li, Zhong
   Yang, Weishen
   Wang, Haihui
TI Large reversible capacity of high quality graphene sheets as an anode
   material for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Lithium-ion batteries; Graphite oxide; Thermal exfoliation; Graphene
   sheets
ID GRAPHITE OXIDE; ELECTROCHEMICAL PERFORMANCE; CARBON NANOTUBES; ELECTRODE
   MATERIALS; RAMAN-SPECTRA; LI STORAGE; NANOSHEETS; INSERTION; OXIDATION;
   COKES
AB High quality graphene sheets were prepared from graphite powder through oxidation followed by rapid thermal expansion in nitrogen atmosphere. The preparation process was systematically investigated by X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy and Brunauer-Emmett-Teller (BET) measurements. The morphology and structure of graphene sheets were characterized by scanning electron microscope (SEM) and high-resolution transmission electron microscopy (HRTEM). The electrochemical performances were evaluated in coin-type cells versus metallic lithium. It is found that the graphene sheets possess a curled morphology consisting of a thin wrinkled paper-like structure, fewer layers (similar to 4 layers) and large specific surface area (492.5 m(2) g(-1)). The first reversible specific capacity of the prepared graphene sheets was as high as 1264 mA h g(-1) at a current density of 100 mA g(-1). Even at a high current density of 500 mA g(-1), the reversible specific capacity remained at 718 mA h g(-1). After 40 cycles, the reversible capacity was still kept at 848 mA h g(-1) at the current density of 100 mA g(-1). These results indicate that the prepared high quality graphene sheets possess excellent electrochemical performances for lithium storage. (C) 2010 Elsevier Ltd. All rights reserved.
C1 [Lian, Peichao; Liang, Shuzhao; Li, Zhong; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Beijing 100864, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620
FU Program for New Century Excellent Talents in Chinese Ministry of
   Education [NECT-07-0307]; Natural Science Foundation of China [20936001]
FX This work was supported by Program for New Century Excellent Talents in
   Chinese Ministry of Education (no. NECT-07-0307) and by the Natural
   Science Foundation of China (no. 20936001).
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NR 41
TC 403
Z9 417
U1 67
U2 367
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD APR 30
PY 2010
VL 55
IS 12
BP 3909
EP 3914
DI 10.1016/j.electacta.2010.02.025
PG 6
WC Electrochemistry
SC Electrochemistry
GA 593YA
UT WOS:000277498000010
ER

PT J
AU Qie, L
   Chen, WM
   Wang, ZH
   Shao, QG
   Li, X
   Yuan, LX
   Hu, XL
   Zhang, WX
   Huang, YH
AF Qie, Long
   Chen, Wei-Min
   Wang, Zhao-Hui
   Shao, Qing-Guo
   Li, Xiang
   Yuan, Li-Xia
   Hu, Xian-Luo
   Zhang, Wu-Xing
   Huang, Yun-Hui
TI Nitrogen-Doped Porous Carbon Nanofiber Webs as Anodes for Lithium Ion
   Batteries with a Superhigh Capacity and Rate Capability
SO ADVANCED MATERIALS
LA English
DT Article
DE lithium ion battery; porous carbon; N-doping; polypyrrole templates;
   electrochemical performance
ID SECONDARY BATTERIES; GRAPHENE SHEETS; PERFORMANCE; STORAGE; ACTIVATION;
   ELECTRODES; NANOTUBES; TEMPLATE; CATHODE; KOH
C1 [Qie, Long; Chen, Wei-Min; Wang, Zhao-Hui; Shao, Qing-Guo; Li, Xiang; Yuan, Li-Xia; Hu, Xian-Luo; Zhang, Wu-Xing; Huang, Yun-Hui] Huazhong Univ Sci & Technol, State Key Lab Mat Proc & Die & Mould Technol, Sch Mat Sci & Engn, Wuhan 430074, Hubei, Peoples R China.
RP Huang, YH (reprint author), Huazhong Univ Sci & Technol, State Key Lab Mat Proc & Die & Mould Technol, Sch Mat Sci & Engn, Wuhan 430074, Hubei, Peoples R China.
EM huangyh@mail.hust.edu.cn
RI Shao, Qingguo/D-1598-2012; Wang, Zhaohui/D-5825-2013; Huang,
   Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010; Qie, Long/F-1488-2011
OI Shao, Qingguo/0000-0002-1459-1484; Hu, Xianluo/0000-0002-5769-167X; Qie,
   Long/0000-0003-1693-5911
FU Natural Science Foundation of China [50825203, 21175050]; 863 program
   [2009AA03Z225, 2011AA11290]; PCSIRT [IRT1014]
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 50825203 and 21175050), the 863 program (Grant Nos.
   2009AA03Z225 and 2011AA11290) and the PCSIRT (No. IRT1014). In addition,
   we thank the Analytical and Testing Center in Huazhong University of
   Science and Technology for SEM measurement.
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NR 32
TC 375
Z9 375
U1 131
U2 561
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD APR 17
PY 2012
VL 24
IS 15
BP 2047
EP 2050
DI 10.1002/adma.201104634
PG 4
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 923FN
UT WOS:000302604900020
PM 22422374
ER

PT J
AU Yao, J
   Shen, XP
   Wang, B
   Liu, HK
   Wang, GX
AF Yao, Jane
   Shen, Xiaoping
   Wang, Bei
   Liu, Huakun
   Wang, Guoxiu
TI In situ chemical synthesis of SnO2-graphene nanocomposite as anode
   materials for lithium-ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Graphene; SnO2 nanoparticles; Nanocomposite; Anode material; Lithium-ion
   batteries
ID GRAPHITE OXIDE; GRAPHENE; STORAGE; NANOPARTICLES; ELECTRODES;
   NANOSHEETS; CAPACITY; SHEETS; FILMS
AB An in situ chemical synthesis approach has been developed to prepare SnO2-graphene nanocomposite. Field emission scanning electron microscopy and transmission electron microscopy observation revealed the homogeneous distribution of SnO2 nanoparticles (4-6 nm in size) on graphene matrix. The electrochemical reactivities of the SnO2-graphene nanocomposite as anode material were measured by cyclic voltammetry and galvanostatic charge/discharge cycling. The as-synthesized SnO2-graphene nanocomposite exhibited a reversible lithium storage capacity of 765 mAh/g in the first cycle and an enhanced cyclability, which can be ascribed to 3D architecture of the SnO2-graphene nanocomposite. (C) 2009 Elsevier B.V. All rights reserved.
C1 [Yao, Jane; Shen, Xiaoping; Wang, Bei; Liu, Huakun; Wang, Guoxiu] Univ Wollongong, Sch Mechan Mat & Mechatron Engn, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
RP Wang, GX (reprint author), Univ Wollongong, Sch Mechan Mat & Mechatron Engn, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM gwang@uow.edu.au
RI Wang,  Bei/J-6550-2012; Liu, Hua/G-1349-2012
OI Wang,  Bei/0000-0002-3793-0629; Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP0772999]
FX We are grateful for financial support from the Australian Research
   Council (ARC) through the ARC Discovery Project (DP0772999).
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NR 19
TC 331
Z9 340
U1 46
U2 317
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD OCT
PY 2009
VL 11
IS 10
BP 1849
EP 1852
DI 10.1016/j.elecom.2009.07.035
PG 4
WC Electrochemistry
SC Electrochemistry
GA 516VL
UT WOS:000271571300001
ER

PT J
AU Brownson, DAC
   Kampouris, DK
   Banks, CE
AF Brownson, Dale A. C.
   Kampouris, Dimitrios K.
   Banks, Craig E.
TI An overview of graphene in energy production and storage applications
SO JOURNAL OF POWER SOURCES
LA English
DT Review
DE Graphene; Energy storage/generation; Electrochemistry; Super-capacitor;
   Battery; Fuel cell
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; FUEL-CELLS; ELECTROCHEMICAL
   PROPERTIES; REVERSIBLE CAPACITY; CATALYST SUPPORT; LI STORAGE;
   ELECTRODES; NANOSHEETS; PERFORMANCE
AB Energy production and storage are both critical research domains where increasing demands for the improved performance of energy devices and the requirement for greener energy resources constitute immense research interest. Graphene has incurred intense interest since its freestanding form was isolated in 2004, and with the vast array of unique and highly desirable electrochemical properties it offers, comes the most promising prospects when implementation within areas of energy research is sought. We present a review of the current literature concerning the electrochemical application of graphene in energy storage/generation devices, starting with its use as a super-capacitor through to applications in batteries and fuel cells, depicting graphene's utilisation in this technologically important field. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Brownson, Dale A. C.; Kampouris, Dimitrios K.; Banks, Craig E.] Manchester Metropolitan Univ, Fac Sci & Engn, Sch Environm Sci, Div Chem & Environm Sci, Manchester M1 5GD, Lancs, England.
RP Banks, CE (reprint author), Manchester Metropolitan Univ, Fac Sci & Engn, Sch Environm Sci, Div Chem & Environm Sci, Chester St, Manchester M1 5GD, Lancs, England.
EM c.banks@mmu.ac.uk
RI Kampouris, Dimitrios/E-6179-2012; Brownson, Dale/B-1949-2013; banks,
   craig/A-8889-2013
OI Kampouris, Dimitrios/0000-0002-4045-8775; banks,
   craig/0000-0002-0756-9764
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NR 77
TC 330
Z9 336
U1 66
U2 514
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 1
PY 2011
VL 196
IS 11
SI SI
BP 4873
EP 4885
DI 10.1016/j.jpowsour.2011.02.022
PG 13
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 751EI
UT WOS:000289599900001
ER

PT J
AU Zhou, GM
   Wang, DW
   Yin, LC
   Li, N
   Li, F
   Cheng, HM
AF Zhou, Guangmin
   Wang, Da-Wei
   Yin, Li-Chang
   Li, Na
   Li, Feng
   Cheng, Hui-Ming
TI Oxygen Bridges between NiO Nanosheets and Graphene for Improvement of
   Lithium Storage
SO ACS NANO
LA English
DT Article
DE graphene; NiO nanosheets; oxygen bridge; oxygen functional groups;
   density functional theory; lithium ion batteries
ID LI-ION BATTERIES; NEGATIVE-ELECTRODE MATERIALS; AUGMENTED-WAVE METHOD;
   MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; ANODE MATERIAL;
   NANOSTRUCTURED MATERIALS; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE;
   SADDLE-POINTS
AB Graphene has been widely used to dramatically improve the capacity, rate capability, and cycling performance of nearly any electrode material for batteries. However, the binding between graphene and these electrode materials has not been dearly elucidated. Here we report oxygen bridges between graphene with oxygen functional groups and NiO from analysis by X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy, and Raman spectroscopy and confirm the conformation of oxygen bridges by the first-principles calculations. We found that NiO nanosheets (NiO NSs) are bonded strongly to graphene through oxygen bridges. The oxygen bridges mainly originate from the pinning of hydroxyl/epoxy groups from graphene on the Ni atoms of NiO NSs. The calculated adsorption energies (137 and 1.84 eV for graphene with hydroxyl and epoxy) of a Ni adatom on oxygenated graphene by binding with oxygen are comparable with that on graphene (126 eV). However, the calculated diffusion barriers of the Ni adatom on the oxygenated graphene surface (223 and 1.69 eV for graphene with hydroxyl and epoxy) are much larger than that on the graphene (0.19 eV). Therefore, the NiO NS is anchored strongly on the graphene through a C-O-Ni bridge, which allows a high reversible capacity and excellent rate performance. The easy binding/difficult dissociating characteristic of Ni adatoms on the oxygenated graphene facilitates fast electron hopping from graphene to NiO and thus the reversible lithiation and delithiation of NiO. We believe that the understanding of this oxygen bridge between graphene and NiO will lead to the development of other high-performance electrode materials.
C1 [Zhou, Guangmin; Yin, Li-Chang; Li, Na; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
   [Wang, Da-Wei] Univ Queensland, Australian Inst Bioengn & Nanotethnol, ARC Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; WANG, DAWEI/E-5074-2010; Zhou,
   guangmin/J-6020-2013; Li, Feng/C-9991-2010
OI WANG, DAWEI/0000-0002-6651-4261; 
FU National Science Foundation of China [50921004, 51172239]; Chinese
   Academy of Sciences; GPU of MOF [ZDYZ2008-2-A12]; Informalization
   Construction Project [INFO-115-B01]; Supercomputing Center, CAS, China
FX This work was supported by National Science Foundation of China (Nos.
   50921004 and 51172239) and Chinese Academy of Sciences. We acknowledge
   the grant from the GPU project of MOF (No. ZDYZ2008-2-A12) and support
   from the Informalization Construction Project (No. INFO-115-B01) and the
   Supercomputing Center, CAS, China. We thank J. H. Luo for FTIR support.
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NR 63
TC 323
Z9 325
U1 73
U2 448
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD APR
PY 2012
VL 6
IS 4
BP 3214
EP 3223
DI 10.1021/nn300098m
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 929XP
UT WOS:000303099300041
PM 22424545
ER

PT J
AU Guo, P
   Song, HH
   Chen, XH
AF Guo, Peng
   Song, Huaihe
   Chen, Xiaohong
TI Electrochemical performance of graphene nanosheets as anode material for
   lithium-ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Lithium-ion batteries; Graphene nanosheets; Graphite; Cycle performance;
   AC impedance
ID IRREVERSIBLE CAPACITIES; MESOCARBON MICROBEADS; CARBON NANOTUBES;
   NATURAL GRAPHITE; INSERTION; STORAGE; CELLS
AB Graphene nanosheets (GNSs) were prepared from artificial graphite by oxidation, rapid expansion and ultrasonic treatment. The morphology, structure and electrochemical performance of GNSs as anode material for lithium-ion batteries were systematically investigated by high-resolution transmission electron microscope, scanning electron microscope, X-ray diffraction, Fourier transform infrared spectroscopy and a variety of electrochemical testing techniques. It was found that GNSs exhibited a relatively high reversible capacity of 672 mA h/g and fine cycle performance. The exchange current density of GNSs increased with the growth of cycle numbers exhibiting the peculiar electrochemical performance. (C) 2009 Elsevier B.V. All rights reserved.
C1 [Guo, Peng; Song, Huaihe; Chen, Xiaohong] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
RP Song, HH (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
EM songhh@mail.buct.edu.cn
RI Guo, Peng/F-8894-2010
OI Guo, Peng/0000-0003-1814-6780
FU Foundation of Excellent Doctoral Dissertation of Beijing City
   [YB20081001001]
FX This work was supported by the Foundation of Excellent Doctoral
   Dissertation of Beijing City (YB20081001001).
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NR 27
TC 318
Z9 330
U1 27
U2 193
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD JUN
PY 2009
VL 11
IS 6
BP 1320
EP 1324
DI 10.1016/j.elecom.2009.04.036
PG 5
WC Electrochemistry
SC Electrochemistry
GA 467LJ
UT WOS:000267740100058
ER

PT J
AU Chen, WF
   Li, SR
   Chen, CH
   Yan, LF
AF Chen, Wufeng
   Li, Sirong
   Chen, Chunhua
   Yan, Lifeng
TI Self-Assembly and Embedding of Nanoparticles by In Situ Reduced Graphene
   for Preparation of a 3D Graphene/Nanoparticle Aerogel
SO ADVANCED MATERIALS
LA English
DT Article
DE graphene; 3D architectures; nanoparticles; composite materials;
   lithium-ion batteries
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; SURFACE-AREA; OXIDE-FILMS;
   SHEETS; PERFORMANCE; FE3O4; ARCHITECTURES; REDUCTION; MONOLITHS
AB A 3D graphene architecture can be prepared via an in situ self-assembly of graphene prepared by a mild chemical reduction. Fe3O4 nanoparticles are homogeneously dispersed into a graphene oxide (GO) aqueous suspension, and a 3D magnetic graphene/Fe3O4 aerogel is prepared during the reduction of GO to graphene. This provides a general method to prepare 3D graphene/nanoparticle composites for a wide range of applications including catalysis and energy conversion.
C1 [Chen, Wufeng; Yan, Lifeng] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
   [Chen, Wufeng; Yan, Lifeng] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China.
   [Li, Sirong; Chen, Chunhua] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China.
RP Yan, LF (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
EM lfyan@ustc.edu.cn
RI Chen, Chunhua/F-5897-2010; Yan, Lifeng/D-5350-2009
FU National Natural Science Foundation of China [20874095, 51073147];
   National Basic Research Program of China [2010CB923302, 2011CB921403];
   Fundamental Research Funds for the Central Universities
FX This work is supported by the National Natural Science Foundation of
   China (No. 20874095 and No. 51073147), the National Basic Research
   Program of China (No. 2010CB923302 and 2011CB921403), and the
   Fundamental Research Funds for the Central Universities.
CR He L, 2009, SMALL, V5, P2802, DOI 10.1002/smll.200900911
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NR 44
TC 311
Z9 316
U1 164
U2 1014
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD DEC 15
PY 2011
VL 23
IS 47
BP 5679
EP +
DI 10.1002/adma.201102838
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 858ID
UT WOS:000297788600014
PM 22052602
ER

PT J
AU Machado, BF
   Serp, P
AF Machado, Bruno F.
   Serp, Philippe
TI Graphene-based materials for catalysis
SO CATALYSIS SCIENCE & TECHNOLOGY
LA English
DT Review
ID LITHIUM-ION BATTERIES; ENHANCED ELECTROCATALYTIC ACTIVITY; PERFORMANCE
   ANODE MATERIALS; SENSITIZED SOLAR-CELL; CHEMICALLY DERIVED GRAPHENE;
   VISIBLE-LIGHT IRRADIATION; ONE-STEP SYNTHESIS; IN-SITU SYNTHESIS;
   FUNCTIONALIZED GRAPHENE; GRAPHITE OXIDE
AB Graphene is one of the most promising materials in nanotechnology. From a theoretical point of view, it provides the ultimate two-dimensional model of a catalytic support. Its unique physical, chemical and mechanical properties are outstanding, and could allow the preparation of composite-materials with unprecedented characteristics. Even though the use of a single graphene sheet as a catalytic support has not yet been reported, some promising results have already been obtained with few-layer graphene. In this review, we will briefly discuss the most relevant synthetic routes to obtain graphene. Then, we will focus our attention on the properties and characterization techniques of graphene that are of relevance to catalysis, with emphasis on adsorption. After presenting an overview of the most common and effective preparation methods, we will discuss the catalytic application of graphene and graphene-based composites, with particular attention on energy conversion and photocatalysis.
C1 [Machado, Bruno F.; Serp, Philippe] Univ Toulouse UPS INP LCC, Composante ENSIACET, UPR CNRS 8241, Lab Chim Coordinat, F-31432 Toulouse 4, France.
   [Machado, Bruno F.] Univ Porto, LCM, Lab Associado LSRE LCM, Dept Engn Quim,Fac Engn, P-4200465 Oporto, Portugal.
RP Machado, BF (reprint author), Univ Toulouse UPS INP LCC, Composante ENSIACET, UPR CNRS 8241, Lab Chim Coordinat, 4 Allee Emile Monso,BP 44362, F-31432 Toulouse 4, France.
EM philippe.serp@ensiacet.fr
RI Machado, Bruno/A-9221-2010; 
OI Machado, Bruno/0000-0003-3183-7519
FU Fundacao para a Ciencia e a Tecnologia [SFRH/BPD/70299/2010]
FX The authors gratefully acknowledge Dr Revathi Bacsa for the selected
   area diffraction pattern, TEM and HRTEM micrographs used in this work.
   B.F.M. acknowledges Fundacao para a Ciencia e a Tecnologia for the grant
   SFRH/BPD/70299/2010.
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NR 391
TC 310
Z9 315
U1 92
U2 582
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2044-4753
EI 2044-4761
J9 CATAL SCI TECHNOL
JI Catal. Sci. Technol.
PY 2012
VL 2
IS 1
BP 54
EP 75
DI 10.1039/c1cy00361e
PG 22
WC Chemistry, Physical
SC Chemistry
GA 875DS
UT WOS:000299011200005
ER

PT J
AU Wang, GX
   Wang, B
   Wang, XL
   Park, J
   Dou, SX
   Ahn, H
   Kim, K
AF Wang, Guoxiu
   Wang, Bei
   Wang, Xianlong
   Park, Jinsoo
   Dou, Shixue
   Ahn, Hyojun
   Kim, Kiwon
TI Sn/graphene nanocomposite with 3D architecture for enhanced reversible
   lithium storage in lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID CARBONACEOUS MATERIALS; GRAPHITE OXIDE; ANODE MATERIAL; GRAPHENE;
   NANOPARTICLES; PERFORMANCE; ELECTRODES; CHEMISTRY; INSERTION; CAPACITY
AB A general strategy has been demonstrated to achieve optimum electrochemical performance by constructing 3D nanocomposite architecture with the combination of nanosize Sn particles and graphene nanosheets. In the first step, the lithium storage properties of graphene have been investigated by first principles calculations. The results show that lithium can be stably stored on both sides of graphene sheets (LiC(3)), inducing in a theoretical capacity of 744 mAh/g. In the second step, a synthetic approach has been designed to prepare Sn/graphene nanocomposite with 3D architecture, in which Sn nanoparticles act as a spacer to effectively separate graphene nanosheets. FESEM and TEM analysis revealed the homogeneous distribution of Sn nanoparticles (2-5 nm) in graphene nanosheet matrix. Cyclic voltammetry measurement has proved the highly reversible nature of the reaction between Li(+) and Sn/graphene nanocomposite. The 3D nanoarchitecture gives the Sn/graphene nanocomposite electrode an enhanced electrochemical performance. This strategy can be extended to prepare other anode and cathode materials for advanced energy storage and conversion devices such as lithium ion batteries, supercapacitors, and fuel cells.
C1 [Wang, Guoxiu; Wang, Bei; Wang, Xianlong; Park, Jinsoo; Dou, Shixue] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
   [Wang, Guoxiu; Wang, Bei; Wang, Xianlong; Park, Jinsoo; Dou, Shixue] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
   [Ahn, Hyojun; Kim, Kiwon] Gyeongsang Natl Univ, Sch Mat Sci & Engn, Jinju 660701, Gyeongnam, South Korea.
RP Wang, GX (reprint author), Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
EM gwang@uow.edu.au
RI Dou, Shi Xue/D-5179-2012; Wang,  Bei/J-6550-2012; Wang,
   Xiaolin/K-1481-2014
OI Dou, Shi Xue/0000-0003-3824-7693; Wang,  Bei/0000-0002-3793-0629; 
FU Australian Research Council (ARC); ARC Discovery Project [DP0559891];
   National Research Foundation of Korea through the WCU (World Class
   University) [R32-2008-000-20093-0]
FX We thank the Australian Research Council (ARC) for financial support
   through the ARC Discovery Project (DP0559891) and the National Research
   Foundation of Korea through the WCU (World Class University) Program
   (R32-2008-000-20093-0).
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NR 37
TC 309
Z9 315
U1 34
U2 292
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2009
VL 19
IS 44
BP 8378
EP 8384
DI 10.1039/b914650d
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 519DG
UT WOS:000271744600016
ER

PT J
AU Chang, K
   Chen, WX
AF Chang, Kun
   Chen, Weixiang
TI In situ synthesis of MoS2/graphene nanosheet composites with
   extraordinarily high electrochemical performance for lithium ion
   batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID ANODE MATERIAL; GRAPHENE; MOS2; CAPACITY; STORAGE; NANOPARTICLES;
   NANOTUBES; OXIDE
AB A facile process was developed to synthesize MoS2/graphene nanosheet (GNS) composites by a one-step in situ solution-phase method. These MoS2/GNS composites therefore exhibit extraordinary capacity, i.e., up to 1300 mA h g(-1), and excellent rate capability and cycling stability as an anode material for lithium ion batteries.
C1 [Chang, Kun; Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China.
EM weixiangchen@zju.edu.cn
RI Chang, Kun/I-1361-2012
FU Zhejiang Provincial Natural Science Foundation of China [Y407030,
   Y4100119]; Ministry of Science and Technology of China [2010CB635116]
FX This work was supported by the Zhejiang Provincial Natural Science
   Foundation of China (Y407030, Y4100119) and 973 Fundamental Research
   Program from the Ministry of Science and Technology of China
   (2010CB635116).
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NR 21
TC 303
Z9 311
U1 80
U2 507
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PY 2011
VL 47
IS 14
BP 4252
EP 4254
DI 10.1039/c1cc10631g
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 738AA
UT WOS:000288610500061
PM 21380470
ER

PT J
AU Zhang, SS
AF Zhang, Sheng S.
TI Liquid electrolyte lithium/sulfur battery: Fundamental chemistry,
   problems, and solutions
SO JOURNAL OF POWER SOURCES
LA English
DT Review
DE Lithium/sulfur battery; Polysulfide; Redox shuttle; Electrolyte;
   Carbon-sulfur composite; Li anode
ID COMPOSITE CATHODE MATERIALS; GLYCOL) DIMETHYL ETHER; HIGH-CAPACITY
   DENSITY; LI-S BATTERY; SULFUR BATTERIES; ELECTROCHEMICAL PROPERTIES;
   CARBON NANOTUBES; ENHANCED CYCLABILITY; GRAPHENE OXIDE; ION BATTERIES
AB Lithium/sulfur (Li/S) battery has a 3-5 fold higher theoretical energy density than state-of-art lithium-ion batteries, and research has been ongoing for more than three decades. However, the commercialization of Li/S battery still cannot be realized due to many problematic issues, including short cycle life, low cycling efficiency, poor safety and a high self-discharge rate. All these issues are related to the dissolution of lithium polysulfide (PS), the series of sulfur reduction intermediates, in liquid electrolyte and to resulting parasitic reactions with the lithium anode and electrolyte components. On the other hand, the dissolution of PS is essential for the performance of a Li/S cell. Without dissolution of PS, the Li/S cell cannot operate progressively due to the non-conductive nature of elemental sulfur and its reduction products. In this review article, we start with the fundamental chemistry of elemental sulfur in order to discuss the problems and solutions of liquid electrolyte Li/S battery. Published by Elsevier B.V.
C1 USA, Electrochem Branch, RDRL SED C, Sensors & Elect Devices Directorate,Res Lab, Adelphi, MD 20783 USA.
RP Zhang, SS (reprint author), USA, Electrochem Branch, RDRL SED C, Sensors & Elect Devices Directorate,Res Lab, Adelphi, MD 20783 USA.
EM shengshui.zhang.civ@mail.mil
RI Zhang, Sheng/A-4456-2012
OI Zhang, Sheng/0000-0002-2624-9248
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NR 106
TC 287
Z9 294
U1 150
U2 1207
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 1
PY 2013
VL 231
BP 153
EP 162
DI 10.1016/j.jpowsour.2012.12.102
PG 10
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 104ZZ
UT WOS:000316036700019
ER

PT J
AU Ishikawa, M
   Sugimoto, T
   Kikuta, M
   Ishiko, E
   Kono, M
AF Ishikawa, Masashi
   Sugimoto, Toshinori
   Kikuta, Manabu
   Ishiko, Eriko
   Kono, Michiyuki
TI Pure ionic liquid electrolytes compatible with a graphitized carbon
   negative electrode in rechargeable lithium-ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE ionic liquid; graphite negative electrode; Li-ion battery; cycleability
ID TEMPERATURE MOLTEN-SALT; ELECTROCHEMICAL INTERCALATION; CAPACITOR
   APPLICATIONS; NATURAL GRAPHITE; ANODE
AB Ambient temperature ionic liquids composed of bis(fluorosulfonyl)imide (FSI) as an anion and 1-ethyl-3-methylimidazolium (EMI) orN-methyl-N-propylpyrrolidinium (P-13) as a cation have the following desirable physicochemical properties, particularly for a battery electrolyte: a high ionic conductivity, low viscosity, and a low melting point. While an irreversible cationic intercalation into graphene interlayers at ca. 0.5 V versus Li/Li+ has been a significant and common problem with usual ionic liquids, we found that ionic liquids containing FSI with the Li cation can prevent such an irreversible reaction and provide reversible Li intercalation into graphene interlayers. Our experimental results found the reversible capacity of a graphite negative electrode, in a half-cell with EMI-FSI containing the Li cation as an electrolyte, to be a stable value of approximately 360 mAh g(--1) during 30 cycles at a charge/discharge rate of 0.2 C, The present paper may be the first report that a "pure" ionic liquid can provide a stable, reversible capacity for a graphitized negative electrode at an ambient temperature without any additives or solvents when an appropriate counter anion, e.g., FSI, is selected. (C) 2006 Elsevier B.V. All rights reserved.
C1 Kanagawa Univ, Fac Engn, Dept Appl Chem, Suita, Osaka 5648680, Japan.
   Kansai Univ, Res Ctr Business Acad Collaborat, Suita, Osaka 5648680, Japan.
   Daiichi Kogyo Seiyaku Co Ltd, Shimogyo Ku, Kyoto 6008873, Japan.
RP Ishikawa, M (reprint author), Kanagawa Univ, Fac Engn, Dept Appl Chem, 3-3-35 Yamate Cho, Suita, Osaka 5648680, Japan.
EM masaishi@ipcku.kansai-u.ac.jp
CR Fung YS, 2002, J ELECTROCHEM SOC, V149, pA319, DOI 10.1149/1.1448501
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   Ue M, 2003, J ELECTROCHEM SOC, V150, P499
NR 17
TC 274
Z9 276
U1 27
U2 156
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD NOV 8
PY 2006
VL 162
IS 1
BP 658
EP 662
DI 10.1016/j.jpowsour.2006.02.077
PG 5
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 105VF
UT WOS:000242059700080
ER

PT J
AU Liu, F
   Song, SY
   Xue, DF
   Zhang, HJ
AF Liu, Fei
   Song, Shuyan
   Xue, Dongfeng
   Zhang, Hongjie
TI Folded Structured Graphene Paper for High Performance Electrode
   Materials
SO ADVANCED MATERIALS
LA English
DT Article
DE graphene paper; flexible; folding; lithium-ion battery; supercapacitor
ID LITHIUM-ION BATTERIES; BINDER-FREE; DIRECT GROWTH; ANODE;
   SUPERCAPACITORS; NANOSHEETS; SHEETS; FILMS; OXIDE
C1 [Liu, Fei; Song, Shuyan; Xue, Dongfeng; Zhang, Hongjie] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
RP Xue, DF (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, 5625 Renmin St, Changchun 130022, Peoples R China.
EM dongfeng@ciac.jl.cn; hongjie@ciac.jl.cn
RI Xue, Dongfeng/E-5881-2011
OI Xue, Dongfeng/0000-0002-0748-0962
FU National Natural Science Foundation of China [50872016, 20973033,
   51125009]; National Natural Science Foundation for Creative Research
   Group [20921002]
FX Financial support from the National Natural Science Foundation of China
   (grant nos. 50872016, 20973033 and 51125009) and National Natural
   Science Foundation for Creative Research Group (grant no. 20921002) is
   acknowledged.
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NR 30
TC 273
Z9 277
U1 82
U2 446
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD FEB 21
PY 2012
VL 24
IS 8
BP 1089
EP 1094
DI 10.1002/adma.201104691
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 894ST
UT WOS:000300447900013
PM 22271320
ER

PT J
AU Bai, S
   Shen, XP
AF Bai, Song
   Shen, Xiaoping
TI Graphene-inorganic nanocomposites
SO RSC ADVANCES
LA English
DT Review
ID LITHIUM-ION BATTERIES; SENSITIZED SOLAR-CELLS; EXFOLIATED GRAPHITE
   OXIDE; IN-SITU SYNTHESIS; ENHANCED ELECTROCATALYTIC ACTIVITY;
   PERFORMANCE ANODE MATERIALS; VISIBLE-LIGHT IRRADIATION; FEW-LAYER
   GRAPHENE; ONE-STEP SYNTHESIS; NANOPARTICLE DECORATED GRAPHENE
AB Graphene (GN) has received intense interest in fields such as physics, chemistry, biology and materials science due to its exceptional electrical, mechanical, thermal and optical properties as well as its unique two-dimensional (2D) structure and large surface area. Recently, GN-inorganic nanocomposites have been opened up an exciting new field in the science and technology of GN. From the viewpoint of chemistry and materials, this account presents an overview of the synthesis and application of GN-inorganic nanocomposites. The challenges and perspective of these emerging nanocomposites are also discussed.
C1 [Bai, Song; Shen, Xiaoping] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.
RP Bai, S (reprint author), Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.
EM xiaopingshen@163.com
FU Natural Science Foundation of Jiangsu Province [BK2009196]; National
   Natural Science Foundation of China [51072071]
FX The authors are grateful for financial support from the Natural Science
   Foundation of Jiangsu Province (No. BK2009196) and the National Natural
   Science Foundation of China (No. 51072071).
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NR 545
TC 272
Z9 277
U1 115
U2 580
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 1
BP 64
EP 98
DI 10.1039/c1ra00260k
PG 35
WC Chemistry, Multidisciplinary
SC Chemistry
GA 876DD
UT WOS:000299086600003
ER

PT J
AU Zhou, XS
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Wan, Li-Jun
   Guo, Yu-Guo
TI Binding SnO2 Nanocrystals in Nitrogen-Doped Graphene Sheets as Anode
   Materials for Lithium-Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE anode materials; tin oxide nanocrystals; graphene sheets; lithium-ion
   batteries
ID OXYGEN REDUCTION REACTION; ONE-POT SYNTHESIS; HOLLOW NANOSPHERES;
   ELECTROCHEMICAL PROPERTIES; NANOSTRUCTURED MATERIALS; SNO2/GRAPHENE
   COMPOSITE; RECHARGEABLE BATTERIES; ELECTRODE MATERIALS; STORAGE
   CAPACITY; ENERGY-STORAGE
C1 [Zhou, Xiaosi; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Natural Science Foundation of China [51225204, 91127044,
   21121063]; National Basic Research Program of China [2011CB935700,
   2012CB932900, 2009CB930400]; Chinese Academy of Sciences
FX This work was supported by the National Natural Science Foundation of
   China (Grant Nos. 51225204, 91127044, and 21121063), the National Basic
   Research Program of China (Grant Nos. 2011CB935700, 2012CB932900, and
   2009CB930400), and the Chinese Academy of Sciences.
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PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
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PD APR 18
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EP 2157
DI 10.1002/adma.201300071
PG 6
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   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 127AD
UT WOS:000317664700006
PM 23427163
ER

PT J
AU Candelaria, SL
   Shao, YY
   Zhou, W
   Li, XL
   Xiao, J
   Zhang, JG
   Wang, Y
   Liu, J
   Li, JH
   Cao, GZ
AF Candelaria, Stephanie L.
   Shao, Yuyan
   Zhou, Wei
   Li, Xiaolin
   Xiao, Jie
   Zhang, Ji-Guang
   Wang, Yong
   Liu, Jun
   Li, Jinghong
   Cao, Guozhong
TI Nanostructured carbon for energy storage and conversion
SO NANO ENERGY
LA English
DT Review
DE Porous carbon; Carbon nanotubes; Graphene; Supercapacitor;
   Electrocatalyst; Lithium battery
ID LITHIUM-ION BATTERIES; METHANOL FUEL-CELLS; DOUBLE-LAYER CAPACITORS;
   HETEROJUNCTION SOLAR-CELLS; NATURAL-GAS STORAGE; AMMONIA BORANE
   NANOCOMPOSITES; PERFORMANCE ANODE MATERIAL; CHEMICAL-VAPOR-DEPOSITION;
   CARBIDE DERIVED CARBONS; PISTACHIO-NUT SHELLS
AB Carbon materials have been playing a significant role in the development of alternative clean and sustainable energy technologies. This review article summarizes the recent research progress on the synthesis of nanostructured carbon and its application in energy storage and conversion. In particular, we will systematically discuss the synthesis and applications of nanoporous carbon as electrodes for supercapacitors and electrodes in lithium-ion batteries, and the development of nanoporous media for methane gas storage, coherent nanocomposites for hydrogen storage, electrocatalysts and catalyst supports for fuel cells, new porous carbon for lithium-sulfur batteries, and porous carbon for lithium-oxygen batteries. The common challenges in developing simple, scalable, and environmentally friendly synthetic and manufacturing processes, in controlling the nanoscale and high level structures and functions, and in integrating such materials with suitable device architectures are reviewed. Possible new directions to overcome the current limitations on the performance are discussed. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Candelaria, Stephanie L.; Cao, Guozhong] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.
   [Shao, Yuyan; Li, Xiaolin; Xiao, Jie; Zhang, Ji-Guang; Wang, Yong; Liu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA.
   [Zhou, Wei; Li, Jinghong] Tsinghua Univ, Dept Chem, Beijing Key Lab Microanalyt Methods & Instrumenta, Beijing 100084, Peoples R China.
   [Zhou, Wei; Li, Jinghong] Tsinghua Univ, Key Lab Bioorgan Phosphorus Chem & Chem Biol, Beijing 100084, Peoples R China.
RP Liu, J (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA.
EM jun.liu@pnnl.gov; jhli@mail.tsinghua.edu.cn; gzcao@u.washington.edu
RI Shao, Yuyan/A-9911-2008; Cao, Guozhong/E-4799-2011; Li, Jinghong
   /D-4283-2012
OI Shao, Yuyan/0000-0001-5735-2670; 
FU National Science Foundation [DMI-0455994, DMR-0605159, CMMI-1030048];
   Air Force Office of Scientific Research (AFOSR-MURI) [FA9550-06-1-0326];
   Washington Technology Center; Pacific Northwest National Laboratory
   (PNNL); Intel Labs; EnerG2; University of Washington Bioenergy IGERT
   fellowship [DGE-0654252]; U.S. Department of Energy (DOE), Office of
   Basic Energy Sciences, Division of Materials Sciences and Engineering
   [KC020105-FWP12152]; DOE by Battelle [DE-AC05-76RL01830]; National Basic
   Research Program of China [2011CB935704]; National Natural Science
   Foundation of China [11079002]
FX This work has been supported in part by National Science Foundation
   (DMI-0455994, DMR-0605159, and CMMI-1030048) and Air Force Office of
   Scientific Research (AFOSR-MURI, FA9550-06-1-0326). This work has also
   been supported by Washington Technology Center, Pacific Northwest
   National Laboratory (PNNL), Intel Labs, and EnerG2. SLC acknowledges the
   University of Washington Bioenergy IGERT fellowship (DGE-0654252) and
   the GO-MAP fellowship. PNNL researchers would like to acknowledge
   support from the U.S. Department of Energy (DOE), Office of Basic Energy
   Sciences, Division of Materials Sciences and Engineering, under Award
   KC020105-FWP12152. PNNL is a multi-program national laboratory operated
   for DOE by Battelle under Contract DE-AC05-76RL01830. Tsinghua
   University researchers acknowledge financial support from National Basic
   Research Program of China (No. 2011CB935704) and National Natural
   Science Foundation of China (No. 11079002).
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NR 344
TC 252
Z9 254
U1 159
U2 763
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAR
PY 2012
VL 1
IS 2
BP 195
EP 220
DI 10.1016/j.nanoen.2011.11.006
PG 26
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 132EG
UT WOS:000318050100004
ER

PT J
AU Wang, JZ
   Zhong, C
   Wexler, D
   Idris, NH
   Wang, ZX
   Chen, LQ
   Liu, HK
AF Wang, Jia-Zhao
   Zhong, Chao
   Wexler, David
   Idris, Nurul Hayati
   Wang, Zhao-Xiang
   Chen, Li-Quan
   Liu, Hua-Kun
TI Graphene-Encapsulated Fe3O4 Nanoparticles with 3D Laminated Structure as
   Superior Anode in Lithium Ion Batteries
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE electrochemistry; graphene; iron oxide; lithium ion batteries;
   nanoparticles
ID ELECTROCHEMICAL PROPERTIES; HYDROTHERMAL SYNTHESIS; ELECTRODE MATERIALS;
   CYCLIC PERFORMANCE; COMPOSITE; CAPACITY; STORAGE; FILMS; NANOSHEETS;
   SHEETS
AB Fe3O4-graphene composites with three-dimensional laminated structures have been synthesised by a simple in situ hydrothermal method. From field-emission and transmission electron microscopy results, the Fe3O4 nanoparticles, around 3-15 nm in size, are highly encapsulated in a graphene nanosheet matrix. The reversible Li-cycling properties of Fe3O4-graphene have been evaluated by galvanostatic discharge-charge cycling, cyclic voltammetry and impedance spectroscopy. Results show that the Fe3O4-graphene nanocomposite with a graphene content of 38.0 wt% exhibits a stable capacity of about 650 mAh g(-1) with no noticeable fading for up to 100 cycles in the voltage range of 0.0-3.0 V. The superior performance of Fe3O4-graphene is clearly established by comparison of the results with those from bare Fe3O4. The graphene nanosheets in the composite materials could act not only as lithium storage active materials, but also as an electronically conductive matrix to improve the electrochemical performance of Fe3O4.
C1 [Wang, Jia-Zhao; Zhong, Chao; Idris, Nurul Hayati; Liu, Hua-Kun] Univ Wollongong, Inst Superconducting & Elect Mat, Meadow, NSW 2519, Australia.
   [Wang, Jia-Zhao; Zhong, Chao; Idris, Nurul Hayati; Liu, Hua-Kun] Univ Wollongong, ARC Ctr Excellence Electromat Sci, Meadow, NSW 2519, Australia.
   [Wexler, David] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
   [Wang, Zhao-Xiang; Chen, Li-Quan] Chinese Acad Sci, Lab Solid State Ion, Inst Phys, Beijing 100190, Peoples R China.
RP Wang, JZ (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Squires Way, Meadow, NSW 2519, Australia.
EM jiazhao@uow.edu.au
RI Wang, Jiazhao/G-4972-2011; Wei, Zhanhua/D-7544-2013; Liu,
   Hua/G-1349-2012; Idris, Nurul Hayati /K-4915-2012
OI Wei, Zhanhua/0000-0003-2687-0293; Liu, Hua/0000-0002-0253-647X; 
FU Australian Research Council (ARC) [DP 0987805]; ARC Centre of
   Excellence; International Linkage Project [CH090014]
FX Financial support provided by an Australian Research Council (ARC)
   Discovery Project (DP 0987805), ARC Centre of Excellence funding, and an
   International Linkage Project (CH090014) are gratefully acknowledged.
   Technical assistance on the FESEM by Darren Attard is highly
   appreciated. Many thanks also go to Dr. Tania Silver for critical
   reading of the manuscript.
CR Zhang YL, 2010, NANO TODAY, V5, P15, DOI 10.1016/j.nantod.2009.12.009
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NR 36
TC 251
Z9 253
U1 43
U2 385
PU WILEY-BLACKWELL
PI MALDEN
PA COMMERCE PLACE, 350 MAIN ST, MALDEN 02148, MA USA
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PY 2011
VL 17
IS 2
BP 661
EP 667
DI 10.1002/chem.201001348
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA 716FM
UT WOS:000286954500035
PM 21207587
ER

PT J
AU Liu, R
   Duay, J
   Lee, SB
AF Liu, Ran
   Duay, Jonathon
   Lee, Sang Bok
TI Heterogeneous nanostructured electrode materials for electrochemical
   energy storage
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIAL; CORE-SHELL NANOWIRES;
   LI-ION; HIGH-CAPACITY; CARBON NANOTUBE; HIGH-POWER; SECONDARY BATTERIES;
   TEMPLATE SYNTHESIS; CATHODE MATERIALS
AB In order to fulfil the future requirements of electrochemical energy storage, such as high energy density at high power demands, heterogeneous nanostructured materials are currently studied as promising electrode materials due to their synergic properties, which arise from integrating multi-nanocomponents, each tailored to address a different demand (e. g., high energy density, high conductivity, and excellent mechanical stability). In this article, we discuss these heterogeneous nanomaterials based on their structural complexity: zero-dimensional (0-D) (e. g. core-shell nanoparticles), one-dimensional (1-D) (e. g. coaxial nanowires), two-dimensional (2-D) (e. g. graphene based composites), three-dimensional (3-D) (e. g. mesoporous carbon based composites) and the even more complex hierarchical 3-D nanostructured networks. This review tends to focus more on ordered arrays of 1-D heterogeneous nanomaterials due to their unique merits. Examples of different types of structures are listed and their advantages and disadvantages are compared. Finally a future 3-D heterogeneous nanostructure is proposed, which may set a goal toward developing ideal nano-architectured electrodes for future electrochemical energy storage devices.
C1 [Liu, Ran; Duay, Jonathon; Lee, Sang Bok] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA.
   [Lee, Sang Bok] Korea Adv Inst Sci & Technol, Grad Sch Nanosci & Technol WCU, Taejon 305701, South Korea.
RP Lee, SB (reprint author), Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA.
EM slee@umd.edu
RI Liu, Ran/B-3785-2011; Duay, Jonathon /A-2108-2012; Lee, Sang
   Bok/B-4421-2009
FU Laboratory for Physical Sciences; US Department of Energy, Office of
   Science, Office of Basic Energy Sciences [DESC0001160]; KOSEF under the
   MEST [R31-2008-000-10071-0]
FX The work was supported by Laboratory for Physical Sciences and also
   supported as part of the Science of Precision Multifunctional
   Nanostructures for Electrical Energy Storage, an Energy Frontier
   Research Centre funded by the US Department of Energy, Office of
   Science, Office of Basic Energy Sciences under Award Number DESC0001160
   (J.D., S.B.L.). S.B.L. thanks the WCU program funded by the KOSEF under
   the MEST (grant number: R31-2008-000-10071-0).
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NR 149
TC 247
Z9 250
U1 43
U2 265
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
EI 1364-548X
J9 CHEM COMMUN
JI Chem. Commun.
PY 2011
VL 47
IS 5
BP 1384
EP 1404
DI 10.1039/c0cc03158e
PG 21
WC Chemistry, Multidisciplinary
SC Chemistry
GA 708UJ
UT WOS:000286389500002
PM 21109866
ER

PT J
AU Wang, HL
   Dai, HJ
AF Wang, Hailiang
   Dai, Hongjie
TI Strongly coupled inorganic-nano-carbon hybrid materials for energy
   storage
SO CHEMICAL SOCIETY REVIEWS
LA English
DT Review
ID LITHIUM-ION BATTERIES; REDUCED GRAPHENE OXIDE; OXYGEN-REDUCTION
   REACTION; PERFORMANCE ANODE MATERIALS; POSITIVE-ELECTRODE MATERIALS;
   IMPROVED REVERSIBLE CAPACITY; METAL-FREE ELECTROCATALYSTS; ONE-STEP
   SYNTHESIS; PEM FUEL-CELLS; LI-ION
AB The global shift of energy production from fossil fuels to renewable energy sources requires more efficient and reliable electrochemical energy storage devices. In particular, the development of electric or hydrogen powered vehicles calls for much-higher-performance batteries, supercapacitors and fuel cells than are currently available. In this review, we present an approach to synthesize electrochemical energy storage materials to form strongly coupled hybrids (SC-hybrids) of inorganic nanomaterials and novel graphitic nano-carbon materials such as carbon nanotubes and graphene, through nucleation and growth of nanoparticles at the functional groups of oxidized graphitic nano-carbon. We show that the inorganic-nano-carbon hybrid materials represent a new approach to synthesize electrode materials with higher electrochemical performance than traditional counterparts made by simple physical mixtures of electrochemically active inorganic particles and conducting carbon materials. The inorganic-nano-carbon hybrid materials are novel due to possible chemical bonding between inorganic nanoparticles and oxidized carbon, affording enhanced charge transport and increased rate capability of electrochemical materials without sacrificing specific capacity. Nano-carbon with various degrees of oxidation provides a novel substrate for nanoparticle nucleation and growth. The interactions between inorganic precursors and oxidized-carbon substrates provide a degree of control over the morphology, size and structure of the resulting inorganic nanoparticles. This paper reviews the recent development of inorganic-nano-carbon hybrid materials for electrochemical energy storage and conversion, including the preparation and functionalization of graphene sheets and carbon nanotubes to impart oxygen containing groups and defects, and methods of synthesis of nanoparticles of various morphologies on oxidized graphene and carbon nanotubes. We then review the applications of the SC-hybrid materials for high performance lithium ion batteries, rechargeable Li-S and Li-O-2 batteries, supercapacitors and ultrafast Ni-Fe batteries, and new electrocatalysts for oxygen reduction, oxygen evolution and hydrogen evolution reactions.
C1 [Wang, Hailiang; Dai, Hongjie] Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
RP Dai, HJ (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
EM hdai1@stanford.edu
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NR 289
TC 240
Z9 240
U1 193
U2 989
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0306-0012
J9 CHEM SOC REV
JI Chem. Soc. Rev.
PY 2013
VL 42
IS 7
BP 3088
EP 3113
DI 10.1039/c2cs35307e
PG 26
WC Chemistry, Multidisciplinary
SC Chemistry
GA 116FX
UT WOS:000316869500026
PM 23361617
ER

PT J
AU Chou, SL
   Wang, JZ
   Choucair, M
   Liu, HK
   Stride, JA
   Dou, SX
AF Chou, Shu-Lei
   Wang, Jia-Zhao
   Choucair, Mohammad
   Liu, Hua-Kun
   Stride, John A.
   Dou, Shi-Xue
TI Enhanced reversible lithium storage in a nanosize silicon/graphene
   composite
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Silicon; Graphene; Nano; Lithium-ion battery; Composite
ID LI-ION BATTERIES; ANODE MATERIAL; RECHARGEABLE BATTERIES; GRAPHENE
   NANOSHEETS; NEGATIVE ELECTRODES; SILICON; SI; PERFORMANCE; INSERTION;
   CAPACITY
AB Si/graphene composite was prepared by simply mixing of commercially available nanosize Si and graphene. Electrochemical tests show that the Si/graphene composite maintains a capacity of 1168 mAh g(-1) and an average coulombic efficiency of 93% up to 30 cycles. EIS indicates that the Si/graphene composite electrode has less than 50% of the charge-transfer resistance compared with nanosize Si electrode, evidencing the enhanced ionic conductivity of Si/graphene composite. The enhanced cycling stability is attributed to the fact that the Si/graphene composite can accommodate large volume charge of Si and maintain good electronic contact. (C) 2009 Elsevier B.V. All rights reserved.
C1 [Chou, Shu-Lei; Wang, Jia-Zhao; Liu, Hua-Kun; Dou, Shi-Xue] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
   [Chou, Shu-Lei; Wang, Jia-Zhao; Liu, Hua-Kun] Univ Wollongong, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2522, Australia.
   [Choucair, Mohammad; Stride, John A.] Univ New S Wales, Sch Chem, Sydney, NSW 2052, Australia.
   [Stride, John A.] Australian Nucl Sci & Technol Org, Bragg Inst, Menai, NSW 2234, Australia.
RP Chou, SL (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM sc478@uow.edu.au; jiazhao@uow.edu.au
RI Chou, Shulei/D-9895-2011; Wang, Jiazhao/G-4972-2011; Dou, Shi
   Xue/D-5179-2012; Choucair, Mohammad/I-8196-2012; Liu, Hua/G-1349-2012
OI Chou, Shulei/0000-0003-1155-6082; Dou, Shi Xue/0000-0003-3824-7693; Liu,
   Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP0987805]; ARC Centre of Excellence
   [CE0561616]
FX Financial support provided by the Australian Research Council (ARC)
   through DP0987805 and ARC Centre of Excellence funding (CE0561616) is
   gratefully acknowledged. The authors also want to thank Dr. T. Silver
   for the critical reading of the manuscript.
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NR 31
TC 231
Z9 245
U1 44
U2 321
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD FEB
PY 2010
VL 12
IS 2
BP 303
EP 306
DI 10.1016/j.elecom.2009.12.024
PG 4
WC Electrochemistry
SC Electrochemistry
GA 560CC
UT WOS:000274878400034
ER

PT J
AU Su, LW
   Jing, Y
   Zhou, Z
AF Su, Liwei
   Jing, Yu
   Zhou, Zhen
TI Li ion battery materials with core-shell nanostructures
SO NANOSCALE
LA English
DT Review
ID RECHARGEABLE LITHIUM BATTERIES; LICOO2 CATHODE MATERIAL; COATED SILICON
   NANOCOMPOSITES; NEGATIVE-ELECTRODE MATERIALS; TRANSITION-METAL
   PHOSPHATES; ATOMIC LAYER DEPOSITION; HIGH-VOLTAGE REGION; SOL-GEL
   METHOD; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE
AB Nanomaterials have some disadvantages in application as Li ion battery materials, such as low density, poor electronic conductivity and high risk of surface side reactions. In recent years, materials with core-shell nanostructures, which was initially a common concept in semiconductors, have been introduced to the field of Li ion batteries in order to overcome the disadvantages of nanomaterials, and increase their general performances in Li ion batteries. Many efforts have been made to exploit core-shell Li ion battery materials, including cathode materials, such as lithium transition metal oxides with varied core and shell compositions, and lithium transition metal phosphates with carbon shells; and anode materials, such as metals, alloys, Si and transition metal oxides with carbon shells. More recently, graphene has also been proposed as a shell material. All these core-shell nanostructured materials presented enhanced electrochemical capacity and cyclic stability. In this review, we summarize the preparation, electrochemical performances, and structural stability of core-shell nanostructured materials for lithium ion batteries, and we also discuss the problems and prospects of this kind of materials.
C1 [Su, Liwei; Jing, Yu; Zhou, Zhen] Nankai Univ, Inst New Energy Mat Chem, Key Lab Adv Energy Mat Chem, Minist Educ, Tianjin 300071, Peoples R China.
RP Zhou, Z (reprint author), Nankai Univ, Inst New Energy Mat Chem, Key Lab Adv Energy Mat Chem, Minist Educ, Tianjin 300071, Peoples R China.
EM zhouzhen@nankai.edu.cn
RI Zhou, Zhen/C-4517-2008; Su, Liwei/G-2295-2011; Jing, Yu/C-9280-2015
OI Zhou, Zhen/0000-0003-3232-9903; Su, Liwei/0000-0002-9791-3476; 
FU 973 Program [2009CB220100]; MOE NCET [08-0293]; Innovation Research Team
   in China [IRT0927]
FX This work was supported by the 973 Program (2009CB220100) and MOE NCET
   (08-0293) as well as Innovation Research Team (IRT0927) in China.
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NR 251
TC 230
Z9 235
U1 95
U2 537
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2011
VL 3
IS 10
BP 3967
EP 3983
DI 10.1039/c1nr10550g
PG 17
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 829XB
UT WOS:000295618200001
PM 21879116
ER

PT J
AU Wang, XY
   Zhou, XF
   Yao, K
   Zhang, JG
   Liu, ZP
AF Wang, Xuyang
   Zhou, Xufeng
   Yao, Ke
   Zhang, Jiangang
   Liu, Zhaoping
TI A SnO2/graphene composite as a high stability electrode for lithium ion
   batteries
SO CARBON
LA English
DT Article
ID STORAGE CAPACITY; ELECTROCHEMICAL PERFORMANCE; CO3O4 NANOPARTICLES;
   CYCLIC PERFORMANCE; GRAPHENE; ANODE; NANOSTRUCTURES; NANOSHEETS; FILMS
AB A simple solution based synthesis route, based on an oxidation-reduction reaction between graphene oxide and SnCl2 center dot 2H(2)O, has been developed to produce a SnO2/graphene composite In the prepared composite, crystalline SnO2 nanoparticles with sizes of 3-5 nm uniformly clung to the graphene matrix When used as an electrode material for lithium ion batteries, the composite presented excellent rate performance and high cyclic stability The effect of SnO2/graphene ratio on electrochemical performance has been investigated It was found that the optimum molar ratio of SnO2/graphene was about 3 2 1, corresponding to 2 4 wt % of graphene The composite could deliver a charge capacity of 840 mAh/g (with capacity retention of 86%) after 30 charge/discharge cycles at a current density of 67 mA/g, and it could retain a charge capacity of about 590 and 270 mAh/g after 50 cycles at the current density of 400 and 1000 mA/g, respectively (C) 2010 Elsevier Ltd All rights reserved
C1 [Wang, Xuyang; Zhou, Xufeng; Yao, Ke; Zhang, Jiangang; Liu, Zhaoping] Chinese Acad Sci, NIMTE, Ningbo 315201, Zhejiang, Peoples R China.
RP Liu, ZP (reprint author), Chinese Acad Sci, NIMTE, Ningbo 315201, Zhejiang, Peoples R China.
FU Chinese Academy of Sciences [KGCX2-YW-231-4, KGCX2-YW 365]; Natural
   Science Foundation of Ningbo [2009A610046, 2009A610029]; Zhejiang
   Provincial Natural Science Foundation
FX We are grateful for financial support from the Chinese Academy of
   Sciences (Program of Knowledge Innovation, Grant No KGCX2-YW-231-4 and
   KGCX2-YW 365), the Natural Science Foundation of Ningbo (Grant No
   2009A610046 and 2009A610029) and Zhejiang Provincial Natural Science
   Foundation
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NR 34
TC 229
Z9 237
U1 27
U2 212
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
EI 1873-3891
J9 CARBON
JI Carbon
PD JAN
PY 2011
VL 49
IS 1
BP 133
EP 139
DI 10.1016/j.carbon.2010.08.052
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 690CJ
UT WOS:000284977500019
ER

PT J
AU Lian, PC
   Zhu, XF
   Xiang, HF
   Li, Z
   Yang, WS
   Wang, HH
AF Lian, Peichao
   Zhu, Xuefeng
   Xiang, Hongfa
   Li, Zhong
   Yang, Weishen
   Wang, Haihui
TI Enhanced cycling performance of Fe3O4-graphene nanocomposite as an anode
   material for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene sheets; Fe3O4 nanoparticles; Nanocomposite; Anode material;
   Lithium-ion batteries
ID REVERSIBLE CAPACITY; GRAPHENE NANOSHEETS; AMORPHOUS OXIDE; LI STORAGE;
   COMPOSITE; FABRICATION; ELECTRODES; SHEETS
AB Fe3O4-graphene nanocomposite was prepared by a gas/liquid interface reaction. The structure and morphology of the Fe3O4-graphene nanocomposite were characterized by X-ray diffraction, scanning electron microscopy and high-resolution transmission electron microscopy. The electrochemical performances were evaluated in coin-type cells. Electrochemical tests show that the Fe3O4-22.7 wt.% graphene nanocomposite exhibits much higher capacity retention with a large reversible specific capacity of 1048 mAh g(-1) (99% of the initial reversible specific capacity) at the 90th cycle in comparison with that of the bare Fe3O4 nanoparticles (only 226 mAh g(-1) at the 34th cycle). The enhanced cycling performance can be attributed to the facts that the graphene sheets distributed between the Fe3O4 nanoparticles can prevent the aggregation of the Fe3O4 nanoparticles, and the Fe3O4-graphene nanocomposite can provide buffering spaces against the volume changes of Fe3O4 nanoparticles during electrochemical cycling. (C) 2010 Elsevier Ltd. All rights reserved.
C1 [Lian, Peichao; Xiang, Hongfa; Li, Zhong; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou 510640, Peoples R China.
EM hhwang@scut.edu.cn
RI Xiang, Hongfa/I-5126-2012; Yang, Weishen/P-1623-2014; Zhu,
   Xuefeng/G-8809-2013
OI Xiang, Hongfa/0000-0002-6182-1932; Yang, Weishen/0000-0001-9615-7421;
   Zhu, Xuefeng/0000-0001-5932-7620
FU National Natural Science Foundation of China [20936001]; SCUT
   [2009220038]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 20936001) and the Fundamental Research Funds
   for the Central Universities, SCUT (2009220038).
CR Wang SQ, 2010, J POWER SOURCES, V195, P5379, DOI 10.1016/j.jpowsour.2010.03.035
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NR 35
TC 229
Z9 238
U1 40
U2 273
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD DEC 30
PY 2010
VL 56
IS 2
BP 834
EP 840
DI 10.1016/j.electacta.2010.09.086
PG 7
WC Electrochemistry
SC Electrochemistry
GA 692TL
UT WOS:000285177900029
ER

PT J
AU Chen, JS
   Lou, XW
AF Chen, Jun Song
   Lou, Xiong Wen (David)
TI SnO2-Based Nanomaterials: Synthesis and Application in Lithium-Ion
   Batteries
SO SMALL
LA English
DT Review
ID ONE-POT SYNTHESIS; POLYCRYSTALLINE SNO2 NANOTUBES; LARGE-SCALE
   SYNTHESIS; MULTIWALLED CARBON NANOTUBES; CAPACITY ANODE MATERIAL;
   GAS-SENSING PROPERTIES; AT-CNT NANOSTRUCTURES; HYBRID HOLLOW SPHERES;
   CORE-SHELL; STORAGE PROPERTIES
AB The development of new electrode materials for lithium-ion batteries (LIBs) has always been a focal area of materials science, as the current technology may not be able to meet the high energy demands for electronic devices with better performance. Among all the metal oxides, tin dioxide (SnO2) is regarded as a promising candidate to serve as the anode material for LIBs due to its high theoretical capacity. Here, a thorough survey is provided of the synthesis of SnO2-based nanomaterials with various structures and chemical compositions, and their application as negative electrodes for LIBs. It covers SnO2 with different morphologies ranging from 1D nanorods/nanowires/nanotubes, to 2D nanosheets, to 3D hollow nanostructures. Nanocomposites consisting of SnO2 and different carbonaceous supports, e.g., amorphous carbon, carbon nanotubes, graphene, are also investigated. The use of Sn-based nanomaterials as the anode material for LIBs will be briefly discussed as well. The aim of this review is to provide an in-depth and rational understanding such that the electrochemical properties of SnO2-based anodes can be effectively enhanced by making proper nanostructures with optimized chemical composition. By focusing on SnO2, the hope is that such concepts and strategies can be extended to other potential metal oxides, such as titanium dioxide or iron oxides, thus shedding some light on the future development of high-performance metal-oxide based negative electrodes for LIBs.
C1 [Chen, Jun Song; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
   [Chen, Jun Song; Lou, Xiong Wen (David)] Nanyang Technol Univ, Energy Res Inst NTU, Singapore 637553, Singapore.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM xwlou@ntu.edu.sg
RI Lou , Xiong Wen (David)/D-2648-2009
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NR 216
TC 227
Z9 228
U1 153
U2 1009
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
J9 SMALL
JI Small
PD JUN 10
PY 2013
VL 9
IS 11
BP 1877
EP 1893
DI 10.1002/smll.201202601
PG 17
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 156PC
UT WOS:000319833700002
PM 23386368
ER

PT J
AU Su, J
   Cao, MH
   Ren, L
   Hu, CW
AF Su, Jing
   Cao, Minhua
   Ren, Ling
   Hu, Changwen
TI Fe3O4-Graphene Nanocomposites with Improved Lithium Storage and
   Magnetism Properties
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID GRAPHITE OXIDE SHEETS; ION BATTERIES; ELECTROCHEMICAL PROPERTIES;
   REVERSIBLE CAPACITY; GRAPHENE NANOSHEETS; CO3O4 NANOPARTICLES;
   NEGATIVE-ELECTRODE; CYCLIC PERFORMANCE; ANODE MATERIAL; CARBON
AB In this paper, we proposed a facile one-step strategy to prepare graphene-Fe3O4 (GN-Fe3O4) nanocomposites under hydrothermal conditions, where the reduction process of graphite oxide (GO) sheets into GN was accompanied by the generation of Fe3O4 nanoparticles. The reduction extent of GO by this process could be comparable to that by conventional methods. A transmission electron microscopy image has shown that the as-formed Fe3O4 nanoparticles with a diameter as small as 7 nm were densely and uniformly deposited on GN sheets, and, as a result, the aggregating of the Fe3O4 nanoparticles was effectively prevented. The GN Fe3O4 nanocomposites exhibit improved cycling stability and rate performances as a potential anode material for high-performance lithium ion batteries. In addition, the GN-Fe3O4 nanocomposites exhibit a superparamagnetic behavior, making them promising candidates for practical applications in the fields of bionanotechnology/controlled targeted drug delivery.
C1 [Su, Jing; Cao, Minhua; Ren, Ling; Hu, Changwen] Beijing Inst Technol, Key Lab Cluster Sci, Minist Educ China, Dept Chem, Beijing 100081, Peoples R China.
RP Cao, MH (reprint author), Beijing Inst Technol, Key Lab Cluster Sci, Minist Educ China, Dept Chem, Beijing 100081, Peoples R China.
EM caomh@bit.edu.cn
FU Natural Science Foundation of China (NSFC) [20731002, 10876002,
   20871016, 91022006, 20973023]; 111 Project [B07012]; Program for New
   Century Excellent Talents in University; State Key Laboratory of
   Explosion Science and Technology; Beijing Institute of Technology
   [ZDKT08-01, YBKT09-13]; Specialized Research Fund for the Doctoral
   Program of Higher Education (SRFDP) [200800070015, 20101101110031];
   Beijing Municipal Commission [Z09010300820902]
FX This work was supported by the Natural Science Foundation of China
   (NSFC, Nos. 20731002, 10876002, 20871016, 91022006, and 20973023), the
   111 Project (B07012), the Program for New Century Excellent Talents in
   University, Open Fund of State Key Laboratory of Explosion Science and
   Technology and Beijing Institute of Technology (No. ZDKT08-01 and
   YBKT09-13), the Specialized Research Fund for the Doctoral Program of
   Higher Education (SRFDP, No. 200800070015 and 20101101110031), and the
   Funding Project for Science and Technology Program of Beijing Municipal
   Commission (No. Z09010300820902).
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NR 42
TC 224
Z9 229
U1 38
U2 266
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD AUG 4
PY 2011
VL 115
IS 30
BP 14469
EP 14477
DI 10.1021/jp201666s
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 798HB
UT WOS:000293192100004
ER

PT J
AU Wang, HB
   Zhang, CJ
   Liu, ZH
   Wang, L
   Han, PX
   Xu, HX
   Zhang, KJ
   Dong, SM
   Yao, JH
   Cui, GL
AF Wang, Haibo
   Zhang, Chuanjian
   Liu, Zhihong
   Wang, Li
   Han, Pengxian
   Xu, Hongxia
   Zhang, Kejun
   Dong, Shanmu
   Yao, Jianhua
   Cui, Guanglei
TI Nitrogen-doped graphene nanosheets with excellent lithium storage
   properties
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; CARBON NANOTUBES; ELECTROCHEMICAL IMPEDANCE;
   ION BATTERIES; OXIDE; GRAPHITE; SHEETS; GROWTH; SPECTROSCOPY; INSERTION
AB In this work, nitrogen-doped graphene nanosheets serving as lithium storage materials are presented. The nitrogen-doped graphene nanosheets were prepared by heat treatment of graphite oxide under an ammonia atmosphere at 800 degrees C for 2 h. Scanning electron microscopy, transmission electron microscopy, Raman spectroscopy, and X-ray photoelectron spectroscopy were employed to characterize the prepared product as nitrogen-doped graphene nanosheets with a doping level of ca. 2% nitrogen, where the N binding configuration of the graphene includes 57.4% pyridinic, 35.0% pyrrolic and 7.6% graphitic N atoms. Galvanostatic charge/discharge experiments revealed that these nitrogen-doped graphene nanosheets exhibited a high reversible capacity (900 mA h g(-1) at 42 mA g(-1) (1/20 C)), excellent rate performance (250 mA h g(-1) at a current density of 2.1 A g(-1) (2.5 C)), and significantly enhanced cycling stability, which demonstrated nitrogen-doped graphene nanosheets to be a promising candidate for anode materials in high rate lithium-ion batteries.
C1 [Wang, Haibo; Zhang, Chuanjian; Liu, Zhihong; Wang, Li; Han, Pengxian; Xu, Hongxia; Zhang, Kejun; Dong, Shanmu; Yao, Jianhua; Cui, Guanglei] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
   [Wang, Li] Ocean Univ China, Qingdao 266003, Peoples R China.
RP Cui, GL (reprint author), Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
EM cuigl@qibebt.ac.cn
RI Han, Pengxian/D-6159-2011; Cui, Guanglei/D-4816-2011
FU Chinese Academy of Sciences; National Program on Key Basic Research
   Project of China (973 Program) [MOST2011CB935700]; Shangdong Province
   Fund for Distinguished Young Scientist; National Natural Science
   Foundation of China [20901077]
FX We appreciate the support of "100 Talents" program of the Chinese
   Academy of Sciences, National Program on Key Basic Research Project of
   China (973 Program) (No. MOST2011CB935700), Shangdong Province Fund for
   Distinguished Young Scientist and National Natural Science Foundation of
   China (Grant No. 20901077).
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NR 49
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U1 39
U2 209
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 14
BP 5430
EP 5434
DI 10.1039/c1jm00049g
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 738RJ
UT WOS:000288659500034
ER

PT J
AU Fu, LJ
   Liu, H
   Li, C
   Wu, YP
   Rahm, E
   Holze, R
   Wu, HQ
AF Fu, LJ
   Liu, H
   Li, C
   Wu, YP
   Rahm, E
   Holze, R
   Wu, HQ
TI Surface modifications of electrode materials for lithium ion batteries
SO SOLID STATE SCIENCES
LA English
DT Review
DE surface modification; anode materials; carbon; cathode materials;
   lithium cobalt oxide (LiCoO(2)); lithium nickel oxide (LiNiO(2));
   lithium manganese oxide (LiMn(2)O(4)); lithium ion battery; mild
   oxidation; coating
ID COMPOSITE MICROENCAPSULATED GRAPHITE; ELEVATED-TEMPERATURE PERFORMANCE;
   INITIAL IRREVERSIBLE CAPACITY; CHARGE-DISCHARGE PROPERTIES; LICOO2
   CATHODE MATERIALS; COMMON NATURAL GRAPHITE; MODIFIED SPINEL LIMN2O4;
   IMPROVED CARBON ANODE; SOL-GEL METHODS; ELECTROCHEMICAL PERFORMANCE
AB Since the birth of the lithium ion battery in the early 1990s, its development has been very rapid and it has been widely applied as power source for a lot of light and high value electronics due to its significant advantages over traditional rechargeable battery systems. Recent research demonstrates the importance of surface structural features of electrode materials for their electrochemical performance, and in this paper the latest progress on this aspect is reviewed. Electrode materials are either anodic or cathodic ones. The former mainly include graphitic carbons, whose surfaces can be modified by mild oxidation, deposition of metals and metal oxides, coating with polymers and other kinds of carbons. P, Through these modifications, the surface structures of the graphitic carbon anodes are improved, and these improvements include: (1) smoothing the active edge surfaces by removing some reactive sites and/or defects on the graphite surface, (2) forming a dense oxide layer on the graphite surface, and (3) covering active edge structures on the graphite surface. Meanwhile, other accompanying changes occur: (1) production of nanochannels/micropores, (2) an increase in the electronic conductivity, (3) an inhibition of structural changes during cycling, (4) a reduction of the thickness of the SEI (solid-electrolyte-interface) layer, and (5) an increase in the number of host sites for lithium storage. As a result, the direct contact of graphite with the electrolyte solution is prevented, its surface reactivity with electrolytes, the decomposition of electrolytes, the co-intercalation of the solvated lithium ions and the charge-transfer resistance ire decreased, and the movement of graphene sheets is inhibited. When the surfaces of cathode materials, mainly including LiCoO(2), LiNiO(2) and LiMn(2)O(4), are coated with oxides such as MgO, Al(2)O(3), ZnO, SnO(2), ZrO(2), Li(2)O(.)2B(2)O(3) glass and other electroactive oxides, the coating can prevent their direct contact with the electrolyte Solution, suppress the phase transitions, improve the structural stability, and decrease the disorder of cations in the crystal sites. As a result, side reactions and the amount of the heat production during cycling are decreased. Simultaneously, other effects are observed such as: (1) suppression of the dissolution of Mn(2+), (2) higher conductivity, and (3) removal of HF from the electrolyte solution. Consequently, after the above-mentioned effective coating, marked improvements in the electrochemical performance of the electrode materials including the reversible capacity, the coulombic efficiency in the first cycle, the cycling behavior, and the high rate capability have been achieved. However, many surface science issues are still remaining open, e.g., mechanisms of these coatings and different actions of different coatings, and some further directions are suggested for the Surface modification of the electrode materials. (c) 2005 Elsevier SAS. All rights reserved.
C1 Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.
   Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
   Tech Univ Chemnitz, Inst Chem AG Elektrochem, D-09107 Chemnitz, Germany.
RP Holze, R (reprint author), Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.
EM rudolf.holze@chemie.tu-chemnitz.de
RI Liu, Hao/B-7522-2009; Wu, Yuping/H-1593-2011
OI Liu, Hao/0000-0003-0266-9472; Wu, Yuping/0000-0002-0833-1205
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   ZHANG T, UNPUB
NR 131
TC 222
Z9 231
U1 122
U2 752
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1293-2558
J9 SOLID STATE SCI
JI Solid State Sci.
PD FEB
PY 2006
VL 8
IS 2
BP 113
EP 128
DI 10.1016/j.solidstatesciences.2005.10.019
PG 16
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical; Physics, Condensed
   Matter
SC Chemistry; Physics
GA 015ZW
UT WOS:000235591300001
ER

PT J
AU Wang, X
   Cao, XQ
   Bourgeois, L
   Guan, H
   Chen, SM
   Zhong, YT
   Tang, DM
   Li, HQ
   Zhai, TY
   Li, L
   Bando, Y
   Golberg, D
AF Wang, Xi
   Cao, Xinqiang
   Bourgeois, Laure
   Guan, Hasigaowa
   Chen, Shimou
   Zhong, Yeteng
   Tang, Dai-Ming
   Li, Huiqiao
   Zhai, Tianyou
   Li, Liang
   Bando, Yoshio
   Golberg, Dmitri
TI N-Doped Graphene-SnO2 Sandwich Paper for High-Performance Lithium-Ion
   Batteries
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE graphene; batteries; doping; charge transport
ID CHEMICAL-VAPOR-DEPOSITION; ENERGY-STORAGE; ANODE MATERIAL; CYCLIC
   PERFORMANCE; CAPACITY; OXIDE; NANOSHEETS; NANOPARTICLES; GROWTH; ARRAYS
AB A new facile route to fabricate N-doped graphene-SnO2 sandwich papers is developed. The 7,7,8,8-tetracyanoquinodimethane anion (TCNQ-) plays a key role for the formation of such structures as it acts as both the nitrogen source and complexing agent. If used in lithium-ion batteries (LIBs), the material exhibits a large capacity, high rate capability, and excellent cycling stability. The superior electrochemical performance of this novel material is the result from its unique features: excellent electronic conductivity related to the sandwich structure, short transportation length for both lithium ions and electrons, and elastomeric space to accommodate volume changes upon Li insertion/extraction.
C1 [Wang, Xi; Chen, Shimou; Tang, Dai-Ming; Zhai, Tianyou; Li, Liang; Bando, Yoshio; Golberg, Dmitri] Natl Inst Mat Sci, ICYS, Tsukuba, Ibaraki 3050044, Japan.
   [Wang, Xi; Chen, Shimou; Tang, Dai-Ming; Zhai, Tianyou; Li, Liang; Bando, Yoshio; Golberg, Dmitri] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton MANA, Tsukuba, Ibaraki 3050044, Japan.
   [Cao, Xinqiang; Zhong, Yeteng] Chinese Acad Sci, Beijing Natl Lab Mol Sci, Key Lab Photochem, Inst Chem, Beijing 100190, Peoples R China.
   [Bourgeois, Laure] Monash Univ, Monash Ctr Elect Microscopy, Clayton, Vic 3800, Australia.
   [Bourgeois, Laure] Monash Univ, Dept Mat Engn, Clayton, Vic 3800, Australia.
   [Guan, Hasigaowa] Ocean Univ China, Key Lab Marine Chem Theory & Technol, Minist Educ, Qingdao 266100, Peoples R China.
   [Li, Huiqiao] Natl Inst Adv Ind & Technol AIST, Energy Technol Res Inst, Tsukuba, Ibaraki 3058568, Japan.
RP Wang, X (reprint author), Natl Inst Mat Sci, ICYS, Namiki 1-1, Tsukuba, Ibaraki 3050044, Japan.
EM Wang.Xi2@nims.go.jp; Huiqiaoli@gmail.com; zhai.tianyou@gmail.com
RI Chen, Shimou/G-4451-2010; Li, Liang/D-2920-2009; Guan,
   Hasigaowa/A-1795-2013; Tang, Dai-Ming/B-6641-2011; Li,
   Huiqiao/D-3536-2009; Wang, Xi/E-7277-2012; Zhai, Tianyou /D-2882-2009
OI Tang, Dai-Ming/0000-0001-7136-7481; Zhai, Tianyou /0000-0003-0985-4806
FU Japan Society for Promotion of Science (JSPS); International Center for
   Materials Nanoarchitectonics (MANA) tenable at the National Institute
   for Materials Science (NIMS)
FX This work was supported by the Japan Society for Promotion of Science
   (JSPS) and the International Center for Materials Nanoarchitectonics
   (MANA) tenable at the National Institute for Materials Science (NIMS).
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NR 53
TC 220
Z9 222
U1 74
U2 481
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD JUL 10
PY 2012
VL 22
IS 13
BP 2682
EP 2690
DI 10.1002/adfm.201103110
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 967YV
UT WOS:000305945000003
ER

PT J
AU Sun, YM
   Hu, XL
   Luo, W
   Huang, YH
AF Sun, Yongming
   Hu, Xianluo
   Luo, Wei
   Huang, Yunhui
TI Self-Assembled Hierarchical MoO2/Graphene Nanoarchitectures and Their
   Application as a High-Performance Anode Material for Lithium-Ion
   Batteries
SO ACS NANO
LA English
DT Article
DE nanohybrid; lithium ion battery; self-assembly; hierarchical
   nanostructures
ID ALPHA-FE2O3 NANOTUBES; REVERSIBLE CAPACITY; RATE CAPABILITY; GRAPHITE
   OXIDE; NANOWIRES; ELECTRODE; STORAGE; HYBRID; NANOPARTICLES; REDUCTION
AB Self-assembled hierarchical MoO2/graphene nanoarchitectures have been fabricated on a large scale through a facile solution-phase process and subsequent reduction of the Moprecursor/graphene composite. The as-formed MoO2/graphene nanohybrid as an anode material for lithium-ion batteries exhibits not only a highly reversible capacity but also an excellent cycling performance as well as good rate capability. Results show that the hierarchical rods made of primary MoO2 nanocrystals are uniformly encapsulated within the graphene sheets. The synergistic effect of the hierarchical nanoarchitecture and the conducting graphene support may contribute to the enhanced electrochemical performances of the hybrid MoO2/graphene electrode. This work presents a facile synthetic strategy that is potentially competitive for scaling-up industrial production.. Besides, the MoO2/graphene hybrids with a well-defined hierarchical topology not only provide flexible building blocks for advanced functional devices, but are also ideal candidates for studying their nanoarchitecture-dependent performances In catalytic and electronic applications.
C1 [Sun, Yongming; Hu, Xianluo; Luo, Wei; Huang, Yunhui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China.
RP Hu, XL (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China.
EM huxl@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Luo, Wei/E-1582-2011; Sun, Yongming/G-7799-2012; Huang,
   Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU Natural Science Foundation of China [50825203, 51002057]; 863 program
   [2009AA03Z225]; Natural Science Foundation of Hubei Province
   [2008CDA026]; Fundamental Research Funds for the Central Universities
   [2010QN007]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 50825203 and 51002057), the 863 program (Grant No.
   2009AA03Z225), the Natural Science Foundation of Hubei Province (Grant
   No. 2008CDA026), the Fundamental Research Funds for the Central
   Universities (HUST: 2010QN007), and the PCSIRT (Program for Changjiang
   Scholars and Innovative Research Team in University). The authors thank
   Analytical and Testing Center of HUST for SEM measurements.
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NR 42
TC 220
Z9 222
U1 60
U2 236
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD SEP
PY 2011
VL 5
IS 9
BP 7100
EP 7107
DI 10.1021/nn201802c
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 824FI
UT WOS:000295187400038
PM 21823572
ER

PT J
AU He, CN
   Wu, S
   Zhao, NQ
   Shi, CS
   Liu, EZ
   Li, JJ
AF He, Chunnian
   Wu, Shan
   Zhao, Naiqin
   Shi, Chunsheng
   Liu, Enzuo
   Li, Jiajun
TI Carbon-Encapsulated Fe3O4 Nanoparticles as a High-Rate Lithium Ion
   Battery Anode Material
SO ACS NANO
LA English
DT Article
DE high rate; core-shell; nanohybrid; carbon-encapsulated Fe3O4
   nanoparticles; 2D nanosheet; in situ synthesis; energy storage
ID ONE-POT SYNTHESIS; HIGH-RATE PERFORMANCE; REDUCED GRAPHENE;
   ENERGY-STORAGE; NANOSTRUCTURED MATERIALS; NANOSHEET COMPOSITES;
   CAPACITY; NANOCOMPOSITES; NANOCRYSTALS; NANOSPHERES
AB A facile and scalable in situ synthesis strategy is developed to fabricate carbon-encapsulated Fe3O4 nanoparticles homogeneously embedded in two-dimensional (2D) porous graphitic carbon nanosheets (Fe3O4@C@PGC nanosheets) as a durable high-rate lithium ion battery anode material. With assistance of the surface of NaCl particles, 20 Fe@C@PGC nanosheets can be in situ synthesized by using the Fe(NO3)(3) center dot 9H(2)O and C6H12O6 as the metal and carbon precursor, respectively. After annealing under air, the Fe@C@PGC nanosheets can be converted to Fe3O4@C@PGC nanosheets, in which Fe3O4 nanoparticles (similar to 18.2 nm) coated with conformal and thin onion-like carbon shells are homogeneously embedded in 2D high-conducting carbon nanosheets with a thickness of less than 30 nm. In the constructed architecture, the thin carbon shells can avoid the direct exposure of encapsulated Fe3O4 to the electrolyte and preserve the structural and Interfacial stabilization of Fe3O4 nanoparticles. Meanwhile, the flexible and conductive PGC nanosheets can accommodate the mechanical stress induced by the volume change of embedded Fe3O4@C nanoparticles as well as inhibit the aggregation of Fe3O4 nanoparticles and thus maintain the structural and electrical integrity of the Fe3O4@C@PGC electrode during the lithiation/delithiation processes. As a result, this Fe3O4@C@PGC electrode exhibits superhigh rate capability (858, 587, and 311 mAh/g at 5, 10, and 20 C, respectively, 1 C = 1 A/g) and extremely excellent cyding performance at high rates (only 3.47% capacity loss after 350 cycles at a high rate of 10 C), which is the best one ever reported for an Fe3O4-based electrode including various nanostructured Fe3O4 anode materials, composite electrodes, etc.
C1 [Zhao, Naiqin] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
   Tianjin Univ, Tianjin Key Lab Composites & Funct Mat, Tianjin 300072, Peoples R China.
RP Zhao, NQ (reprint author), Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
EM nqzhao@tju.edu.cn
FU National Natural Science Foundation of China [51002188, 51272173];
   National Excellent Doctoral Dissertation of China [201145]; Program for
   New Century Excellent Talents in University [NCET-12-0408]; Natural
   Science Foundation of Tianjin City [12JCYBJC11700]; Elite Scholar
   Program of Tianjin University; Innovation Foundation of Tianjin
   University; National Basic Research Program of China [2010CB934700];
   Projects for the Science & Technology Pillar Program of Tianjin City
   [12ZCZDGX00800]
FX The authors acknowledge the financial support by the National Natural
   Science Foundation of China (Nos. 51002188, and 51272173) and Foundation
   for the Author of National Excellent Doctoral Dissertation of China (No.
   201145), Program for New Century Excellent Talents in University
   (NCET-12-0408), Natural Science Foundation of Tianjin City (No.
   12JCYBJC11700), Elite Scholar Program of Tianjin University, Innovation
   Foundation of Tianjin University, National Basic Research Program of
   China (2010CB934700) and Key Projects for the Science & Technology
   Pillar Program of Tianjin City (No. 12ZCZDGX00800).
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NR 42
TC 218
Z9 220
U1 97
U2 607
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD MAY
PY 2013
VL 7
IS 5
BP 4459
EP 4469
DI 10.1021/nn401059h
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 156XD
UT WOS:000319856300085
PM 23614734
ER

PT J
AU Xue, DJ
   Xin, S
   Yan, Y
   Jiang, KC
   Yin, YX
   Guo, YG
   Wan, LJ
AF Xue, Ding-Jiang
   Xin, Sen
   Yan, Yang
   Jiang, Ke-Cheng
   Yin, Ya-Xia
   Guo, Yu-Guo
   Wan, Li-Jun
TI Improving the Electrode Performance of Ge through Ge@C Core-Shell
   Nanoparticles and Graphene Networks
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; FACILE SYNTHESIS; CATHODE
   MATERIAL; STORAGE DEVICES; CARBON MATRIX; CAPACITY; NANOWIRES; HOLLOW;
   NANOCOMPOSITE
AB Germanium is a promising high-capacity anode material for lithium ion batteries, but it usually exhibits poor cycling stability because of its huge volume variation during the lithium uptake and release process. A double protection strategy to improve the electrode performance of Ge through the use of Ge@C core-shell nanostructures and reduced graphene oxide (RGO) networks has been developed. The as-synthesized Ge@C/RGO nanocomposite showed excellent cycling performance and rate capability in comparison with Ge@C nanoparticles when used as an anode material for Li ion batteries, which can be attributed to the electronically conductive and elastic RGO networks in addition to the carbon shells and small particle sizes of Ge. The strategy is simple yet very effective, and because of its versatility, it may be extended to other high-capacity electrode materials with large volume variations and low electrical conductivities.
C1 [Guo, Yu-Guo] Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Beijing 100190, Peoples R China.
   Chinese Acad Sci, Beijing Natl Lab Mol Sci, Inst Chem, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Inst Chem, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn; wanlijun@iccas.ac.cn
RI xue, dingjiang/A-1776-2012; Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2009CB930400,
   2012CB932900]; National Natural Science Foundation of China [91127044,
   21121063, 50730005]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grants 2011CB935700, 2009CB930400, and 2012CB932900), the National
   Natural Science Foundation of China (Grants 91127044, 21121063, and
   50730005), and the Chinese Academy of Sciences.
CR Zhang LS, 2010, J MATER CHEM, V20, P5462, DOI 10.1039/c0jm00672f
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NR 36
TC 214
Z9 218
U1 52
U2 364
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD FEB 8
PY 2012
VL 134
IS 5
BP 2512
EP 2515
DI 10.1021/ja211266m
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA 894XK
UT WOS:000300460600017
PM 22260540
ER

PT J
AU Li, N
   Chen, ZP
   Ren, WC
   Li, F
   Cheng, HM
AF Li, Na
   Chen, Zongping
   Ren, Wencai
   Li, Feng
   Cheng, Hui-Ming
TI Flexible graphene-based lithium ion batteries with ultrafast charge and
   discharge rates
SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF
   AMERICA
LA English
DT Article
DE flexible device; full battery
ID HIGH-POWER; STORAGE DEVICES; ELECTRODES; PERFORMANCE; INSERTION; PAPER;
   CELL
AB There is growing interest in thin, lightweight, and flexible energy storage devices to meet the special needs for next-generation, high-performance, flexible electronics. Here we report a thin, lightweight, and flexible lithium ion battery made from graphene foam, a three-dimensional, flexible, and conductive interconnected network, as a current collector, loaded with Li4Ti5O12 and LiFePO4, for use as anode and cathode, respectively. No metal current collectors, conducting additives, or binders are used. The excellent electrical conductivity and pore structure of the hybrid electrodes enable rapid electron and ion transport. For example, the Li4Ti5O12/graphene foam electrode shows a high rate up to 200 C, equivalent to a full discharge in 18 s. Using them, we demonstrate a thin, lightweight, and flexible full lithium ion battery with a high-rate performance and energy density that can be repeatedly bent to a radius of 5 mm without structural failure and performance loss.
C1 [Li, Na; Chen, Zongping; Ren, Wencai; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China.
   [Li, Na] Univ Sci & Technol China, Sch Chem & Mat Sci, Dept Mat Sci & Engn, Hefei 230026, Peoples R China.
RP Cheng, HM (reprint author), Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, Shenyang 110016, Peoples R China.
EM cheng@imr.ac.cn
RI Chen, Zongping/G-6679-2012; Cheng, Hui-Ming/B-8682-2012; Li,
   Feng/C-9991-2010
FU Ministry of Science and Technology of China [2012AA030303]; National
   Natural Science Foundation of China [51172240, 50921004, 50972147];
   Chinese Academy of Sciences [KGZD-EW-303]
FX This work was supported by Ministry of Science and Technology of China
   Grant 2012AA030303, National Natural Science Foundation of China Grants
   51172240, 50921004, and 50972147, and Chinese Academy of Sciences Grant
   KGZD-EW-303.
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NR 33
TC 213
Z9 226
U1 75
U2 434
PU NATL ACAD SCIENCES
PI WASHINGTON
PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA
SN 0027-8424
J9 P NATL ACAD SCI USA
JI Proc. Natl. Acad. Sci. U. S. A.
PD OCT 23
PY 2012
VL 109
IS 43
BP 17360
EP 17365
DI 10.1073/pnas.1210072109
PG 6
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 038AO
UT WOS:000311147800019
PM 23045691
ER

PT J
AU Yin, SY
   Zhang, YY
   Kong, JH
   Zou, CJ
   Li, CM
   Lu, XH
   Ma, J
   Boey, FYC
   Chen, XD
AF Yin, Shengyan
   Zhang, Yanyan
   Kong, Junhua
   Zou, Changji
   Li, Chang Ming
   Lu, Xuehong
   Ma, Jan
   Boey, Freddy Yin Chiang
   Chen, Xiaodong
TI Assembly of Graphene Sheets into Hierarchical Structures for
   High-Performance Energy Storage
SO ACS NANO
LA English
DT Article
DE bioinspiration; hierarchical structures; graphene; self-assembly;
   lithium-ion battery
ID LITHIUM ION BATTERIES; ORGANIZED HONEYCOMB MORPHOLOGY; NANOSTRUCTURED
   MATERIALS; GRAPHITE OXIDE; ANODE MATERIAL; LI STORAGE; NANOSHEETS;
   SYSTEMS; FILMS; CAPABILITY
AB The electrodes with the hierarchical nanoarchitectures could offer a huge increase in energy storage capacity. However, the ability to achieve such hierarchical architectures on a multiple scale still has remained a great challenge. In this paper, we report a scalable self-assembly strategy to create bioinspired hierarchical structures composed of functionalized graphene sheets to work as anodes of lithium-ion batteries. The resulting electrodes with novel multilevel architectures simultaneously optimize ion transport and capacity, leading to a high performance of reversible capacity of up to 1 600 mAh/g, and 1150 mAh/g after 50 cycles. Importantly, the process to fabricate such hierarchical structures is facile, low-cost, green, and scalable, providing a universal approach for the rational design and engineering of electrode materials with enhanced performance, and it may have utility in various applications, including biological scaffold, catalysis, and sensors.
C1 [Yin, Shengyan; Zhang, Yanyan; Kong, Junhua; Zou, Changji; Lu, Xuehong; Ma, Jan; Boey, Freddy Yin Chiang; Chen, Xiaodong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Li, Chang Ming] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637457, Singapore.
RP Chen, XD (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM chenxd@ntu.edu.sg
RI Li, Chang Ming/G-6192-2010; Chen, Xiaodong/A-4537-2009; Lu,
   Xuehong/A-2232-2011; yin, shengyan/H-4549-2012
OI Chen, Xiaodong/0000-0002-3312-1664; 
FU National Research Foundation of Singapore [NRF-RF2009-04, CREATE]
FX This work was supported by National Research Foundation of Singapore
   (NRF-RF2009-04 and CREATE).
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NR 49
TC 213
Z9 220
U1 44
U2 252
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD MAY
PY 2011
VL 5
IS 5
BP 3831
EP 3838
DI 10.1021/nn2001728
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 767AD
UT WOS:000290826800050
PM 21510618
ER

PT J
AU Brownson, DAC
   Kampouris, DK
   Banks, CE
AF Brownson, Dale A. C.
   Kampouris, Dimitrios K.
   Banks, Craig E.
TI Graphene electrochemistry: fundamental concepts through to prominent
   applications
SO CHEMICAL SOCIETY REVIEWS
LA English
DT Review
ID LITHIUM-ION BATTERIES; CHEMICAL-VAPOR-DEPOSITION; PLANE
   PYROLYTIC-GRAPHITE; NANOTUBE-MODIFIED ELECTRODES; GLASSY-CARBON
   ELECTRODE; SURFACTANT-FREE GRAPHENE; MULTILAYER GRAPHENE; CYCLIC
   VOLTAMMETRY; ANODE MATERIAL; ASCORBIC-ACID
AB The use of graphene, a one atom thick individual planar carbon layer, has exploded in a plethora of scientific disciplines since it was reported to possess a range of unique and exclusive properties. Despite graphene being explored theoretically since the 1940s and known to exist since the 1960s, the recent burst of interest from a large proportion of scientists globally can be correlated with work by Geim and Novoselov in 2004/5, who reported the so-called "scotch tape method" for the production of graphene in addition to identifying its unique electronic properties which has escalated into graphene being reported to be superior in a superfluity of areas. Consequently, many are involved in the pursuit of producing new methodologies to fabricate pristine graphene on an industrial scale in order to meet the current world-wide appetite for graphene. One area which receives considerable interest is the field of electrochemistry, where graphene has been reported to be beneficial in various applications ranging from sensing through to energy storage and generation and carbon based molecular electronics. Electrochemistry is an interfacial technique which is dominated by processes that occur at the solid-liquid interface and thus with the correct understanding can be beneficially utilised to characterise the surface under investigation. In this tutorial review we overview fundamental concepts of Graphene Electrochemistry, making electrochemical characterisation accessible to those who are working on new methodologies to fabricate graphene, bridging the gap between materials scientists and electrochemists and also assisting those exploring graphene in electrochemical areas, or that wish to start to. An overview of the recent understanding of graphene modified electrodes is also provided, highlighting prominent applications reported in the current literature.
C1 [Brownson, Dale A. C.; Kampouris, Dimitrios K.; Banks, Craig E.] Manchester Metropolitan Univ, Fac Sci & Engn, Sch Sci & Environm, Div Chem & Environm Sci, Manchester M1 5GD, Lancs, England.
RP Banks, CE (reprint author), Manchester Metropolitan Univ, Fac Sci & Engn, Sch Sci & Environm, Div Chem & Environm Sci, Chester St, Manchester M1 5GD, Lancs, England.
EM c.banks@mmu.ac.uk
RI Brownson, Dale/B-1949-2013; Kampouris, Dimitrios/E-6179-2012; banks,
   craig/A-8889-2013
OI Kampouris, Dimitrios/0000-0002-4045-8775; banks,
   craig/0000-0002-0756-9764
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NR 172
TC 205
Z9 205
U1 54
U2 413
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0306-0012
J9 CHEM SOC REV
JI Chem. Soc. Rev.
PY 2012
VL 41
IS 21
BP 6944
EP 6976
DI 10.1039/c2cs35105f
PG 33
WC Chemistry, Multidisciplinary
SC Chemistry
GA 016UJ
UT WOS:000309544700007
PM 22850696
ER

PT J
AU Li, BJ
   Cao, HQ
   Shao, J
   Li, GQ
   Qu, MZ
   Yin, G
AF Li, Baojun
   Cao, Huaqiang
   Shao, Jin
   Li, Guoqiang
   Qu, Meizhen
   Yin, Gui
TI Co3O4@graphene Composites as Anode Materials for High-Performance
   Lithium Ion Batteries
SO INORGANIC CHEMISTRY
LA English
DT Article
ID SN-C COMPOSITE; HIGH-CAPACITY; REVERSIBLE CAPACITY; GRAPHENE NANOSHEETS;
   CO3O4 NANOTUBES; HOLLOW; NANOPARTICLES; ELECTRODES; OXIDE; LI
AB This paper reports on the synthesis of Co3O4@graphene composites (CGC) and their applications as anode materials in lithium ion batteries (LIBs). Through a chemical deposition method, Co3O4 nanoparticles (NPs) with sizes in the range of 10-30 nm were homogeneously dispersed onto graphene sheets. Due to their high electrical conductivity, the graphene sheets in the CGC improved the electrical conductivity and the structure stability of CGC. CGC displayed a superior performance in LIBs with a large reversible capacity value of 941 mA hg(-1) in the initial cycle with a large current density and an excellent cyclic performance of 740 mA hg(-1) after 60 cycles, corresponding to 88.3% of the theoretical value of CGC, owing to the interactions between graphene sheets and Co3O4 NPs anchored on the graphene sheets. This synthesis approach may find its application in the design and synthesis of novel electrode materials used in LIBs.
C1 [Li, Baojun; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Shao, Jin; Li, Guoqiang; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
   [Yin, Gui] Nanjing Univ, Dept Chem, Nanjing 210093, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn; mzhqu@cioc.ac.cn
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]; Jiangsu
   Province Foundation of Natural Science [BK2006717]; China Post-doctoral
   Science Foundation [20100470302]
FX Financial support from the National Natural Science Foundation of China
   (no. 20921001 and 20535020), the Innovation Method Fund of China (no.
   20081885189), the National High Technology Research and Development
   Program of China (no. 2009AA03Z321), the Jiangsu Province Foundation of
   Natural Science (no. BK2006717), and the China Post-doctoral Science
   Foundation (no. 20100470302) is acknowledged.
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NR 41
TC 202
Z9 207
U1 30
U2 190
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD MAR 7
PY 2011
VL 50
IS 5
BP 1628
EP 1632
DI 10.1021/ic1023086
PG 5
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 725ZO
UT WOS:000287685600006
PM 21244033
ER

PT J
AU Zhao, X
   Hayner, CM
   Kung, MC
   Kung, HH
AF Zhao, Xin
   Hayner, Cary M.
   Kung, Mayfair C.
   Kung, Harold H.
TI In-Plane Vacancy-Enabled High-Power Si-Graphene Composite Electrode for
   Lithium-Ion Batteries
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE energy storage; graphene; graphenic scaffold; Li-ion batteries; silicon
ID GRAPHITE OXIDE; PERFORMANCE; SILICON; ANODES; CAPACITY; STORAGE; CARBON;
   SUPERCAPACITORS; REDUCTION; FILMS
C1 [Zhao, Xin; Hayner, Cary M.; Kung, Mayfair C.; Kung, Harold H.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA.
RP Kung, HH (reprint author), Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA.
EM hkung@northwestern.edu
RI Kung, Harold/B-7647-2009; Kung, Mayfair/B-7648-2009
FU U.S. Department of Energy, Basic Energy Sciences through the Center for
   Electrical Energy Storage, an Energy Frontier Research Center
   [DE-AC02-06CH11357]
FX This research was supported by the U.S. Department of Energy, Basic
   Energy Sciences, grant DE-AC02-06CH11357 through the Center for
   Electrical Energy Storage, an Energy Frontier Research Center. We thank
   Dr. Shuyou Li (EPIC, NU), Dr. Xinqi Chen (KECK, NU), and Mr. Yuki
   Kusachi (Nissan) for helpful discussions.
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NR 38
TC 201
Z9 209
U1 47
U2 328
PU WILEY PERIODICALS, INC
PI MALDEN
PA COMMERCE PLACE, 350 MAIN STREET, MALDEN, MA 02148-529 USA
SN 1614-6832
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD NOV
PY 2011
VL 1
IS 6
BP 1079
EP 1084
DI 10.1002/aenm.201100426
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 848MU
UT WOS:000297056500017
ER

PT J
AU Shi, WH
   Zhu, JX
   Sim, DH
   Tay, YY
   Lu, ZY
   Zhang, XJ
   Sharma, Y
   Srinivasan, M
   Zhang, H
   Hng, HH
   Yan, QY
AF Shi, Wenhui
   Zhu, Jixin
   Sim, Dao Hao
   Tay, Yee Yan
   Lu, Ziyang
   Zhang, Xiaojun
   Sharma, Yogesh
   Srinivasan, Madhavi
   Zhang, Hua
   Hng, Huey Hoon
   Yan, Qingyu
TI Achieving high specific charge capacitances in Fe3O4/reduced graphene
   oxide nanocomposites
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; SUPERCAPACITOR ELECTRODES; ELECTROCHEMICAL
   CAPACITOR; CARBON NANOTUBES; GRAPHITE OXIDE; ANODE MATERIAL;
   BINDER-FREE; COMPOSITES; REDUCTION; HYBRID
AB We report a facile approach to synthesize nanocomposites with Fe3O4 nanopaticles (NPs) attached to reduced graphene oxide (rGO) sheets by a solvothermal process, which combines the growth of Fe3O4 NPs and the reduction of GOs in one single step. These Fe3O4/rGO nanocomposites were further used to fabricate thin film supercapacitor electrodes by using a spray deposition technique without the addition of insulating binders. It was found that the Fe3O4/rGO nanocomposites showed much higher specific capacitances than that of either pure rGO or pure Fe3O4 NPs. We further carried out electrochemical characterization of the Fe3O4/rGO nanocomposites with different Fe3O4 : rGO weight ratios (e.g. I-Fe3O4 : rGO) and showed that Fe3O4/rGO nanocomposites with I-Fe3O4 : rGO 2.8 exhibited the highest specific capacitance of 480 F g(-1) at a discharge current density of 5 A g(-1) with the corresponding energy density of 67 W h kg(-1) at a power density of 5506 W kg(-1). These Fe3O4/rGO nanocomposites also showed stable cycling performance without any decrease in the specific capacitance after 1000 charge/discharge cycles.
C1 [Shi, Wenhui; Zhu, Jixin; Sim, Dao Hao; Tay, Yee Yan; Lu, Ziyang; Zhang, Xiaojun; Srinivasan, Madhavi; Zhang, Hua; Hng, Huey Hoon; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Sharma, Yogesh; Srinivasan, Madhavi; Yan, Qingyu] Nanyang Technol Univ, Energy Res Inst NTU, Singapore 639798, Singapore.
RP Yan, QY (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
EM alexyan@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; Hng, Huey Hoon/A-2246-2011; zhu,
   Jixin/F-8763-2011; Lu, Ziyang /L-7857-2014; Srinivasan,
   Madhavi/A-2247-2011; Zhang, Hua/A-1302-2009
OI Hng, Huey Hoon/0000-0002-8950-025X; 
FU MOE (Singapore) [AcRF Tier 1 RG 31/08, MOE2010-T2-1-060]; Singapore
   Ministry of Education [MOE2010-T2-1-017];  [NRF2009EWT-CERP001-026]; 
   [NRF-CRP4-2008-03]
FX The authors gratefully acknowledge AcRF Tier 1 RG 31/08 of MOE
   (Singapore), NRF2009EWT-CERP001-026 (Singapore) and Singapore Ministry
   of Education (MOE2010-T2-1-017). H.Z. thanks the support of AcRF Tier 2
   (ARC 10/10, No. MOE2010-T2-1-060) from MOE in Singapore. M.S. thanks the
   support of NRF-CRP4-2008-03 (Singapore).
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NR 53
TC 200
Z9 204
U1 42
U2 369
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 10
BP 3422
EP 3427
DI 10.1039/c0jm03175e
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 724OE
UT WOS:000287585300023
ER

PT J
AU Zhou, GM
   Li, F
   Cheng, HM
AF Zhou, Guangmin
   Li, Feng
   Cheng, Hui-Ming
TI Progress in flexible lithium batteries and future prospects
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID LI-ION BATTERIES; CARBON NANOTUBE ELECTRODES; HIGH-PERFORMANCE ANODES;
   ENERGY-STORAGE ARCHITECTURES; CHEMICAL-VAPOR-DEPOSITION; GRAPHENE PAPER
   ELECTRODES; SOLID-STATE BATTERIES; BINDER-FREE ANODES; SULFUR BATTERIES;
   POLYMER ELECTROLYTES
AB With the advent of flexible electronics, flexible lithium-ion batteries have attracted great attention as a promising power source in the emerging field of flexible and wearable electronic devices such as roll-up displays, touch screens, conformable active radio-frequency identification tags, wearable sensors and implantable medical devices. In this review, we summarize the recent research progress of flexible lithium-ion batteries, with special emphasis on electrode material selectivity and battery structural design. We begin with a brief introduction of flexible lithium-ion batteries and the current development of flexible solid-state electrolytes for applications in this field. This is followed by a detailed overview of the recent progress on flexible electrode materials based on carbon nanotubes, graphene, carbon cloth, conductive paper (cellulose), textiles and some other low-dimensional nanostructured materials. Then recently proposed prototypes of flexible cable/wire type, transparent and stretchable lithium-ion batteries are highlighted. The latest advances in the exploration of other flexible battery systems such as lithium-sulfur, Zn-C (MnO2) and sodium-ion batteries, as well as related electrode materials are included. Finally, the prospects and challenges toward the practical uses of flexible lithium-ion batteries in electronic devices are discussed.
C1 [Zhou, Guangmin; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
RP Zhou, GM (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM cheng@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Li, Feng/C-9991-2010
FU Key Research Program of Ministry of Science and Technology, China
   [2011CB932604, 2014CB932402]; National Science Foundation of China
   [51221264, 51172239, 51372253]
FX This work was supported by the Key Research Program of Ministry of
   Science and Technology, China (nos. 2011CB932604, 2014CB932402) and the
   National Science Foundation of China (nos. 51221264, 51172239 and
   51372253).
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NR 216
TC 199
Z9 203
U1 362
U2 1347
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD APR
PY 2014
VL 7
IS 4
BP 1307
EP 1338
DI 10.1039/c3ee43182g
PG 32
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AD4GI
UT WOS:000333205800006
ER

PT J
AU Li, BJ
   Cao, HQ
   Shao, J
   Qu, MZ
   Warner, JH
AF Li, Baojun
   Cao, Huaqiang
   Shao, Jin
   Qu, Meizhen
   Warner, Jamie H.
TI Superparamagnetic Fe3O4 nanocrystals@graphene composites for energy
   storage devices
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM ION BATTERIES; IRON-OXIDE NANOPARTICLES; PHOTOVOLTAIC DEVICES;
   REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; ANODE MATERIAL; ELECTRODES;
   CARBON; FILMS; SUPERCAPACITORS
AB In this paper, a Fe3O4 nanocrystals@graphene composite (FGC) was synthesized via a chemical deposition method by using graphene oxide as a precursor. We also investigate the structures, physicochemical properties and applications of FGCs, involving superparamagnetic performance, and use as supercapacitors and lithium ion battery (LIBs). The results showed that the Fe3O4 NCs were formed and incorporated onto the surface of the graphene sheets. The composite material FGC with a micrometre scale structure possessed similar size as the graphene sheets and exhibited superparamagnetic behavior at room temperature. The supercapacitance values of the FGC composites were enlarged compared with those of the graphene sheets or Fe3O4 NCs, which is attributed to the interaction between the Fe3O4 NCs and the graphene sheets. Meanwhile, a superior rechargeable stability of FGCs used as an anode material in LIBs can be observed.
C1 [Li, Baojun; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Shao, Jin; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
   [Warner, Jamie H.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
RI Wei, Zhanhua/D-7544-2013
OI Wei, Zhanhua/0000-0003-2687-0293
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]; China
   Postdoctoral Science Foundation [20100470302]
FX Financial supports from the National Natural Science Foundation of China
   (No. 20921001 and 20535020), the Innovation Method Fund of China (No.
   20081885189), the National High Technology Research and Development
   Program of China (No. 2009AA03Z321), and the China Postdoctoral Science
   Foundation (No. 20100470302) are acknowledged.
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NR 79
TC 199
Z9 202
U1 31
U2 269
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 13
BP 5069
EP 5075
DI 10.1039/c0jm03717f
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 735WB
UT WOS:000288450200046
ER

PT J
AU Luo, JS
   Liu, JL
   Zeng, ZY
   Ng, CF
   Ma, LJ
   Zhang, H
   Lin, JY
   Shen, ZX
   Fan, HJ
AF Luo, Jingshan
   Liu, Jilei
   Zeng, Zhiyuan
   Ng, Chi Fan
   Ma, Lingjie
   Zhang, Hua
   Lin, Jianyi
   Shen, Zexiang
   Fan, Hong Jin
TI Three-Dimensional Graphene Foam Supported Fe3O4 Lithium Battery Anodes
   with Long Cycle Life and High Rate Capability
SO NANO LETTERS
LA English
DT Article
DE 3D graphene foam; iron oxide; lithium ion battery; atomic layer
   deposition; high rate capability; Li ion storage
ID ATOMIC LAYER DEPOSITION; HIGH-PERFORMANCE ANODE; ION BATTERIES; REDUCED
   GRAPHENE; NANOSTRUCTURED MATERIALS; ENERGY-CONVERSION; ULTRAFAST-CHARGE;
   COMPOSITE ANODE; OXIDE FILMS; CARBON
AB Fe3O4 has long been regarded as a promising anode material for lithium ion battery due to its high theoretical capacity, earth abundance, low cost, and nontoxic properties. However, up to now no effective and scalable method has been realized to overcome the bottleneck of poor cyclability and low rate capability. In this article, we report a bottom-up strategy assisted by atomic layer deposition to graft bicontinuous mesoporous nanostructure Fe3O4 onto three-dimensional graphene foams and directly use the composite as the lithium ion battery anode. This electrode exhibits high reversible capacity and fast charging and discharging capability. A high capacity of 785 mAh/g is achieved at 1C rate and is maintained without decay up to 500 cycles. Moreover, the rate of up to 60C is also demonstrated, rendering a fast discharge potential. To our knowledge, this is the best reported rate performance for Fe3O4 in lithium ion battery to date.
C1 [Luo, Jingshan; Liu, Jilei; Ng, Chi Fan; Ma, Lingjie; Lin, Jianyi; Shen, Zexiang; Fan, Hong Jin] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
   [Zeng, Zhiyuan; Zhang, Hua; Shen, Zexiang] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Shen, Zexiang; Fan, Hong Jin] Nanyang Technol Univ, Ctr Disrupt Photon Technol, Singapore 637371, Singapore.
   [Lin, Jianyi] ASTAR, Inst Chem Engn & Sci, Jurong Isl 627833, Singapore.
RP Fan, HJ (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
EM fanhj@ntu.edu.sg
RI Fan, Hongjin/A-2662-2010; Shen, Zexiang/B-6988-2011; zeng,
   zhiyuan/G-7571-2015; Zhang, Hua/A-1302-2009; 
OI Fan, Hongjin/0000-0003-1237-4555; zeng, zhiyuan/0000-0001-7483-1438;
   Luo, Jingshan/0000-0002-1770-7681
FU SERC Public Sector Research Funding, Agency for Science, Technology, and
   Research (A*STAR) [1121202012]; Singapore Ministry of Education Academic
   Research Fund [MOE2011-T3-1-005]; Singapore MOE under AcRF [ARC 26/13,
   MOE2013-T2-1-034]; AcRF [RG 61/12]; NTU Start-Up Grant [M4080865];
   Singapore National Research Foundation; Energy Research Institute @NTU
FX H.J.F. thanks the financial support by SERC Public Sector Research
   Funding (Grant 1121202012), Agency for Science, Technology, and Research
   (A*STAR). H.J.F. and Z.X.S. appreciate the support by Singapore Ministry
   of Education Academic Research Fund Tier 3 (MOE2011-T3-1-005). H.Z.
   acknowledges the support by Singapore MOE under AcRF Tier 2 (ARC 26/13,
   No. MOE2013-T2-1-034), AcRF Tier 1 (RG 61/12), and NTU Start-Up Grant
   (M4080865). This research is also funded by the Singapore National
   Research Foundation and the publication is supported under the Campus
   for Research Excellence And Technological Enterprise (CREATE) programme
   (Nanomaterials for Energy and Water Management). The authors also
   acknowledge partial financial support from the Energy Research Institute
   @NTU and the help from Ting Yu and his group members with the usage of
   glovebox and oxygen plasma etcher.
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NR 55
TC 198
Z9 203
U1 104
U2 522
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD DEC
PY 2013
VL 13
IS 12
BP 6136
EP 6143
DI 10.1021/nl403461n
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 272CZ
UT WOS:000328439200058
PM 24219630
ER

PT J
AU Liu, H
   Wang, GX
   Liu, J
   Qiao, SZ
   Ahn, HJ
AF Liu, Hao
   Wang, Guoxiu
   Liu, Jian
   Qiao, Shizhang
   Ahn, Hyojun
TI Highly ordered mesoporous NiO anode material for lithium ion batteries
   with an excellent electrochemical performance
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID HIGH-POWER; GRAPHENE NANOSHEETS; NEGATIVE ELECTRODES; STORAGE
   PROPERTIES; NANOWIRE; NANOTUBES; OXIDE; CO3O4; SNO2; CATHODE
AB In this work, we have synthesized highly ordered mesoporous NiO materials by a nanocasting method using mesoporous silica KIT-6 as the hard templates. Mesoporous NiO particles were characterized by small angle X-ray diffraction (XRD), nitrogen adsorption/desorption, and transmission electron microscopy (TEM). The results demonstrated that the as-prepared mesoporous NiO had an ordered Ia3d symmetric mesostructure, with a high surface area of 96 m(2)/g. Mesoporous NiO materials were tested as an anode material for lithium ion batteries, exhibiting much lower activation energy (20.75 kJ mol(-1)) compared to the bulk NiO (45.02 kJ mol(-1)). We found that the mesoporous NiO electrode has higher lithium intercalation kinetics than its bulk counterpart. The specific capacity of mesoporous NiO after 50 cycles was maintained 680 mAh/g at 0.1 C, which was much higher than that of the commercial bulk NiO (188 mAh/g). Furthermore, at a high rate of 2C, the discharge capacity of mesoporous NiO was as high as 515 mAh/g, demonstrating the potential to be used for high power lithium ion batteries.
C1 [Wang, Guoxiu] Univ Technol Sydney, Dept Chem & Forens Sci, Sydney, NSW 2007, Australia.
   [Ahn, Hyojun] Gyeongsang Natl Univ, Sch Mat Sci & Engn, Jinju 660701, Gyeongnam, South Korea.
   [Liu, Hao; Liu, Jian; Qiao, Shizhang] Univ Queensland, Australian Inst Bioengn & Nanotechnol, ARC Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia.
RP Wang, GX (reprint author), Univ Technol Sydney, Dept Chem & Forens Sci, Sydney, NSW 2007, Australia.
EM Guoxiu.Wang@uts.edu.au; s.qiao@uq.edu.au
RI Liu, Hao/B-7522-2009; Liu, Jian/C-5665-2009; Qiao, Shizhang /A-6057-2010
OI Liu, Hao/0000-0003-0266-9472; Liu, Jian/0000-0002-5114-0404; Qiao,
   Shizhang /0000-0002-4568-8422
FU Australian Research Council (ARC) [DP0772999, LP0989134]; National
   Foundation of Korea (NRF) through the WCU (World Class University)
   [R32-2008-000-20093-0]
FX We thank the Australian Research Council (ARC) for financial support
   through the ARC Discovery Project (DP0772999) and the ARC Linkage
   Project (LP0989134). We also would like to acknowledge the support from
   the National Foundation of Korea (NRF) through the WCU (World Class
   University) Program (R32-2008-000-20093-0).
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NR 41
TC 198
Z9 200
U1 47
U2 301
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 9
BP 3046
EP 3052
DI 10.1039/c0jm03132a
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 721QI
UT WOS:000287369300037
ER

PT J
AU Chang, K
   Chen, WX
   Ma, L
   Li, H
   Li, H
   Huang, FH
   Xu, ZD
   Zhang, QB
   Lee, JY
AF Chang, Kun
   Chen, Weixiang
   Ma, Lin
   Li, Hui
   Li, He
   Huang, Feihe
   Xu, Zhude
   Zhang, Qingbo
   Lee, Jim-Yang
TI Graphene-like MoS2/amorphous carbon composites with high capacity and
   excellent stability as anode materials for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID TUNGSTEN DISULFIDE; MOLYBDENUM-DISULFIDE; MOS2; NANOTUBES; STORAGE;
   NANOSHEETS
AB A facile process to synthesize graphene-like MoS2/amorphous carbon (a-C) composites was developed. MoS2/C composites were firstly prepared by hydrothermal method employing sodium molybdate, sulfocarbamide and glucose as starting materials. The graphene-like MoS2/a-C composites were obtained after annealing at 800 degrees C in H-2/N-2. The samples were characterized by XRD, SEM, EDS and HRTEM. It was confirmed that in the composites MoS2 has a structure of single-layer, which is named graphene-like nanostructure. The graphene-like MoS2 nanosheets were uniformly dispersed in amorphous carbon. The interlaminar distance of the adjacent graphene-like MoS2 nanosheets in the composites measured was similar to 1.0 nm. The mechanism of the formation of the graphene-like MoS2/a-C composites was investigated. The graphene-like MoS2/a-C composites exhibited high capacity and excellent cyclic stability used as anode materials for Li-ion batteries. The composite prepared by adding 1.0 g of glucose in hydrothermal solution exhibited the highest reversible capacity (962 mAh g(-1)) and excellent cyclic stability. After 100 cycles, it still retained 912 mAh g(-1). The significant improvements in the electrochemical properties of the graphene-like MoS2/a-C composites could be attributed to the graphene-like structure of the MoS2 nanosheets and the synergistic effects of graphene-like MoS2 and amorphous carbon.
C1 [Chang, Kun; Chen, Weixiang; Li, Hui; Huang, Feihe; Xu, Zhude] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
   [Ma, Lin] Zhanjiang Normal Univ, Chem Sci & Technol Sch, Zhanjiang 524048, Peoples R China.
   [Li, He] Zhejiang Shuren Univ, Coll Biol & Environm Engn, Hangzhou 310015, Zhejiang, Peoples R China.
   [Zhang, Qingbo; Lee, Jim-Yang] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 119260, Singapore.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
EM weixiangchen@zju.edu.cn
RI LEE, Jim Yang/E-5904-2010; Huang, Feihe/A-1020-2012; Chang,
   Kun/I-1361-2012; yang, dong/J-1427-2012; Zhang, Qingbo/B-7070-2015
OI Zhang, Qingbo/0000-0001-8289-0227
FU Zhejiang Provincial Natural Science Foundation of China [Y407030,
   Y4100119]; Ministry of Science and Technology of China [2010CB635116];
   Guangdong Natural Science Foundation [10452404801004521]
FX This work was supported by the Zhejiang Provincial Natural Science
   Foundation of China (Y407030, Y4100119), 973 Fundamental Research
   Program from the Ministry of Science and Technology of China
   (2010CB635116) and Ph.D Start-up Research Program of Guangdong Natural
   Science Foundation (10452404801004521).
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NR 28
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Z9 197
U1 88
U2 503
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 17
BP 6251
EP 6257
DI 10.1039/c1jm10174a
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 750DG
UT WOS:000289524300021
ER

PT J
AU Wang, B
   Wu, XL
   Shu, CY
   Guo, YG
   Wang, CR
AF Wang, Bao
   Wu, Xing-Long
   Shu, Chun-Ying
   Guo, Yu-Guo
   Wang, Chun-Ru
TI Synthesis of CuO/graphene nanocomposite as a high-performance anode
   material for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ELECTRODE MATERIALS; ELECTROCHEMICAL PERFORMANCE; SPRAY-PYROLYSIS; LI
   STORAGE; CUO; MICROSPHERES; NETWORKS; CELLS
AB An optimized nanostructure design for electrode materials for high-performance lithium-ion batteries was realized by introducing three-dimensional (3D) graphene networks into transition metal oxide nanomicrostructures. A CuO/graphene composite was selected as a typical example of the optimized design. Self-assembled CuO and CuO/graphene urchin-like structures have been successfully synthesized by a simple solution method and investigated with SEM, TEM, XRD, and electrochemical measurements. The CuO/graphene nanocomposite exhibits a remarkably enhanced cycling performance and rate performance compared with pure CuO urchin-like structure when being used as anode materials in lithium-ion batteries. During all the 100 discharge-charge cycles under a current density of 65 mA g(-1), the CuO/graphene electrode can stably deliver a reversible capacity of ca. 600 mA h g(-1). At a high current density of 6400 mA g(-1), the specific charge capacity of the CuO/graphene nanocomposite is still as high as 150 mA h g(-1), which is three times larger than that of graphene (48 mA h g(-1)), while that of CuO is nearly null under the same current density. The enhancement of the electrochemical performance could be attributed to the 3D electrically conductive networks of graphene as well as the unique nanomicrostructure of the CuO/graphene nanocomposite in which the CuO nanomicroflowers are enwrapped by a thin layer of graphene as an elastic buffer.
C1 [Wang, Bao; Wu, Xing-Long; Shu, Chun-Ying; Guo, Yu-Guo; Wang, Chun-Ru] Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing Natl Lab Mol Sci, Inst Chem, Beijing 100190, Peoples R China.
   [Wang, Bao; Wu, Xing-Long] Chinese Acad Sci, Grad Sch, Beijing 100064, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing Natl Lab Mol Sci, Inst Chem, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn; crwang@iccas.ac.cn
RI Wu, Xing-Long/J-8388-2012; Guo, Yu-Guo/A-1223-2009; Wang,
   Bao/G-9032-2015
OI Wu, Xing-Long/0000-0003-1069-9145; Guo, Yu-Guo/0000-0003-0322-8476; 
FU National Natural Science Foundation of China [20821003, 20702053,
   50730005]; National Key Project on Basic Research [2009CB930400]; 973
   Program [2006CB300402]; Ministry of Science and Technology
   [2008ZX05013-004]; Chinese Academy of Sciences
FX This work is supported by the National Natural Science Foundation of
   China (Grant Nos., 20821003, 20702053 and 50730005), National Key
   Project on Basic Research (Grant No. 2009CB930400), the 973 Program
   (2006CB300402), Ministry of Science and Technology (2008ZX05013-004),
   and the Chinese Academy of Sciences.
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NR 23
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PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2010
VL 20
IS 47
BP 10661
EP 10664
DI 10.1039/c0jm01941k
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 684IC
UT WOS:000284542600014
ER

PT J
AU Su, YZ
   Li, S
   Wu, DQ
   Zhang, F
   Liang, HW
   Gao, PF
   Cheng, C
   Feng, XL
AF Su, Yuezeng
   Li, Shuang
   Wu, Dongqing
   Zhang, Fan
   Liang, Haiwei
   Gao, Pengfei
   Cheng, Chong
   Feng, Xinliang
TI Two-Dimensional Carbon-Coated Graphene/Metal Oxide Hybrids for Enhanced
   Lithium Storage
SO ACS NANO
LA English
DT Article
DE lithium-ion battery; metal oxide; 2D nanosheet; graphene; core-shell
ID PERFORMANCE ANODE MATERIAL; ION BATTERIES; REVERSIBLE CAPACITY; REDUCED
   GRAPHENE; AMORPHOUS OXIDE; SNO2 NANOWIRE; SANDWICH-LIKE; NANOPARTICLES;
   NANOSHEETS; COMPOSITE
AB Metal oxides (MOs) have been widely investigated as promising high-capacity anode material for lithium ion batteries, but they usually exhibit poor cycling stability and rate performance due to the huge volume change induced by the alloying reaction with lithium. In this article, we present a double protection strategy by fabricating a two-dimensional (2D) core-shell nanostructure to improve the electrochemical performance of metal oxides in lithium storage. The 2D core-shell architecture is constructed by confining the well-defined graphene based metal oxides nanosheets (G@MO) within carbon layers. The resulting 2D carbon-coated graphene/metal oxides nanosheets (G@MO@C) inherit the advantages of graphene, which possesses high electrical conductivity, large aspect ratio, and thin feature. Furthermore, the carbon shells can tackle the deformation of MO nanoparticles while keeping the overall electrode highly conductive and active in lithium storage. As the result, the produced G@MO@C hybrids exhibit outstanding reversible capacity and excellent rate performance for lithium storage (G@SnO2@C, 800 mAh g(-1) at the rate of 200 mA g(-1) after 100 cycles; G@Fe3O4@C, 920 mAh g(-1) at the rate of 200 mA g(-1) after 100 cycles).
C1 [Wu, Dongqing; Zhang, Fan; Liang, Haiwei; Gao, Pengfei; Cheng, Chong; Feng, Xinliang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Su, Yuezeng; Li, Shuang] Shanghai Jiao Tong Univ, Sch Aeronaut & Astronaut, Shanghai 200240, Peoples R China.
   [Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Wu, DQ (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Dongchuan Rd 800, Shanghai 200240, Peoples R China.
EM wudongqing@sjtu.edu.cn; feng@mpip-mainz.mpg.de
RI Liang, Hai-Wei/B-7292-2011
FU 973 Program of China [2012CB933404]; Natural Science Foundation of China
   [21174083, 21102091]; BASF; Ph.D. Programs Foundation of Ministry of
   Education of China for Young Scholars [20110073120039]; Shanghai Pujiang
   Program [11PJ1405400]
FX This work was financially supported by 973 Program of China
   (2012CB933404), Natural Science Foundation of China (21174083 and
   21102091), BASF, Shanghai Pujiang Program (11PJ1405400), and the Ph.D.
   Programs Foundation of Ministry of Education of China for Young Scholars
   (20110073120039).
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NR 41
TC 193
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U1 87
U2 512
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD SEP
PY 2012
VL 6
IS 9
BP 8349
EP 8356
DI 10.1021/nn303091t
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 009QP
UT WOS:000309040600089
PM 22931096
ER

PT J
AU Li, XF
   Meng, XB
   Liu, J
   Geng, DS
   Zhang, Y
   Banis, MN
   Li, YL
   Yang, JL
   Li, RY
   Sun, XL
   Cai, M
   Verbrugge, MW
AF Li, Xifei
   Meng, Xiangbo
   Liu, Jian
   Geng, Dongsheng
   Zhang, Yong
   Banis, Mohammad Norouzi
   Li, Yongliang
   Yang, Jinli
   Li, Ruying
   Sun, Xueliang
   Cai, Mei
   Verbrugge, Mark W.
TI Tin Oxide with Controlled Morphology and Crystallinity by Atomic Layer
   Deposition onto Graphene Nanosheets for Enhanced Lithium Storage
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE SnO2 anodes; amorphous; crystalline; graphene; lithium-ion batteries
ID BATTERY ANODE MATERIALS; THIN-FILM ELECTRODES; IN-SITU SYNTHESIS; LI-ION
   BATTERIES; HIGH-CAPACITY; ELECTROCHEMICAL PROPERTIES; RECHARGEABLE
   BATTERIES; SNO2 NANOPARTICLES; SNO2/GRAPHENE COMPOSITE; SECONDARY
   BATTERIES
AB As one of the most promising negative electrode materials in lithium-ion batteries (LIBs), SnO2 experiences intense investigation due to its high specific capacity and energy density, relative to conventional graphite anodes. In this study, for the first time, atomic layer deposition (ALD) is used to deposit SnO2, containing both amorphous and crystalline phases, onto graphene nanosheets (GNS) as anodes for LIBs. The resultant SnO2-graphene nanocomposites exhibit a sandwich structure, and, when cycled against a lithium counter electrode, demonstrate a promising electrochemical performance. It is demonstrated that the introduction of GNS into the nanocomposites is beneficial for the anodes by increasing their electrical conductivity and releasing strain energy: thus, the nanocomposite electrode materials maintain a high electrical conductivity and flexibility. It is found that the amorphous SnO2-GNS is more effective than the crystalline SnO2-GNS in overcoming electrochemical and mechanical degradation; this observation is consistent with the intrinsically isotropic nature of the amorphous SnO2, which can mitigate the large volume changes associated with charge/discharge processes. It is observed that after 150 charge/discharge cycles, 793 mA h g-1 is achieved. Moreover, a higher coulombic efficiency is obtained for the amorphous SnO2-GNS composite anode. This study provides an approach to fabricate novel anode materials and clarifies the influence of SnO2 phases on the electrochemical performance of LIBs.
C1 [Li, Xifei; Meng, Xiangbo; Liu, Jian; Geng, Dongsheng; Zhang, Yong; Banis, Mohammad Norouzi; Li, Yongliang; Yang, Jinli; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
   [Cai, Mei; Verbrugge, Mark W.] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Li, XF (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Li, Yongliang/H-3179-2011; Li, Xifei/A-1966-2012; Sun, Andy
   (Xueliang)/I-4535-2013; Liu, Jian/I-5571-2014; Geng,
   Dongsheng/G-7124-2011; Sun, Xueliang/C-7257-2012; Meng,
   Xiangbo/H-3264-2012
OI Li, Yongliang/0000-0002-5008-0868; Li, Xifei/0000-0002-4828-4183; Liu,
   Jian/0000-0003-0756-2260; Meng, Xiangbo/0000-0002-4631-7260
FU Natural Science and Engineering Research Council of Canada (NSERC);
   General Motors; Canada Research Chair (CRC) Program; Canadian Foundation
   for Innovation (CFI); Ontario Research Fund (ORF); Early Researcher
   Award (ERA); University of Western Ontario
FX This research was supported by the Natural Science and Engineering
   Research Council of Canada (NSERC), General Motors, the Canada Research
   Chair (CRC) Program, the Canadian Foundation for Innovation (CFI), the
   Ontario Research Fund (ORF), the Early Researcher Award (ERA) and the
   University of Western Ontario. X. L. is grateful to the Ontario PDF
   Program.
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NR 86
TC 193
Z9 194
U1 44
U2 332
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 1616-301X
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD APR 24
PY 2012
VL 22
IS 8
BP 1647
EP 1654
DI 10.1002/adfm.201101068
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 925XC
UT WOS:000302794400011
ER

PT J
AU Yang, SB
   Cui, GL
   Pang, SP
   Cao, Q
   Kolb, U
   Feng, XL
   Maier, J
   Mullen, K
AF Yang, Shubin
   Cui, Guanglei
   Pang, Shuping
   Cao, Qian
   Kolb, Ute
   Feng, Xinliang
   Maier, Joachim
   Mullen, Klaus
TI Fabrication of Cobalt and Cobalt Oxide/Graphene Composites: Towards
   High-Performance Anode Materials for Lithium Ion Batteries
SO CHEMSUSCHEM
LA English
DT Article
DE cobalt; composites; electrochemistry; graphene; nanoparticles
ID EXFOLIATED GRAPHITE OXIDE; NEGATIVE-ELECTRODE; GRAPHENE; STORAGE;
   NANOPLATELETS; TIN
C1 [Yang, Shubin; Pang, Shuping; Feng, Xinliang; Mullen, Klaus] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
   [Cui, Guanglei; Cao, Qian; Maier, Joachim] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany.
   [Kolb, Ute] Johannes Gutenberg Univ Mainz, Inst Phys Chem, D-55128 Mainz, Germany.
RP Yang, SB (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany.
RI Kolb, Ute/A-2642-2011; Cui, Guanglei/D-4816-2011; Yang,
   Shubin/B-4840-2015; Mainz, EMZ-M/E-3619-2016
OI Yang, Shubin/0000-0001-9973-9785; 
FU Max Planck Society; German Science Foundation (Korean-German IRTG); DFG
   [SPP 1355]
FX This work was financially supported by the Max Planck Society through
   the program ENERCHEM, the German Science Foundation (Korean-German IRTG)
   and DFG Priority Program SPP 1355.
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NR 24
TC 191
Z9 198
U1 24
U2 163
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 1864-5631
J9 CHEMSUSCHEM
JI ChemSusChem
PY 2010
VL 3
IS 2
BP 236
EP 239
DI 10.1002/cssc.200900106
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA 566EJ
UT WOS:000275352600022
PM 19816895
ER

PT J
AU Mai, YJ
   Wang, XL
   Xiang, JY
   Qiao, YQ
   Zhang, D
   Gu, CD
   Tu, JP
AF Mai, Y. J.
   Wang, X. L.
   Xiang, J. Y.
   Qiao, Y. Q.
   Zhang, D.
   Gu, C. D.
   Tu, J. P.
TI CuO/graphene composite as anode materials for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; Cupric oxide; Lithium-ion battery; Coulombic efficiency
ID REDUCED GRAPHENE OXIDE; ELECTROCHEMICAL PERFORMANCE; REVERSIBLE
   CAPACITY; LI STORAGE; CU2O FILM; CUO; SUPERCAPACITORS; NANOSHEETS;
   OXIDATION; NANOSTRUCTURES
AB CuO/graphene composite is synthesized from CuO and graphene oxide sheets following reduced by hydrazine vapor. As the electrode material for lithium-ion batteries, CuO nanoparticles with sizes of about 30 nm homogeneously locate on graphene sheets, and act as spacers to effectively prevent the agglomeration of graphene sheets, keeping their high active surface. In turn, the graphene sheets with good electrical conductivity server as a conducting network for fast electron transfer between the active materials and charge collector, as well as buffered spaces to accommodate the volume expansion/contraction during discharge/charge process. The synergetic effect is beneficial for the electrochemical performances of CuO/graphene composite, such as improved initial coulombic efficiency (68.7%) and reversible capacity of 583.5 mAh g(-1) with 75.5% retention of the reversible capacity after 50 cycles. (C) 2010 Elsevier Ltd. All rights reserved.
C1 [Tu, J. P.] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
RP Tu, JP (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
EM tujp@zju.edu.cn
RI Qiao, Yanqiang/E-8159-2012
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NR 48
TC 189
Z9 193
U1 45
U2 264
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 1
PY 2011
VL 56
IS 5
BP 2306
EP 2311
DI 10.1016/j.electacta.2010.11.036
PG 6
WC Electrochemistry
SC Electrochemistry
GA 732YZ
UT WOS:000288227800057
ER

PT J
AU Zhang, M
   Lei, DN
   Yin, XM
   Chen, LB
   Li, QH
   Wang, YG
   Wang, TH
AF Zhang, Ming
   Lei, Danni
   Yin, Xiaoming
   Chen, Libao
   Li, Qiuhong
   Wang, Yanguo
   Wang, Taihong
TI Magnetite/graphene composites: microwave irradiation synthesis and
   enhanced cycling and rate performances for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ANODE MATERIALS; FE3O4; ELECTRODES; GRAPHENE; NANOPARTICLES;
   TEMPERATURE; INSERTION; GROWTH; GAS
AB By employing microwave irradiation as a heat source, magnetite/graphene composites were synthesized by depositing Fe(3+) in the interspaces of graphene sheets. The Fe(3)O(4) nanoparticles were dispersed on graphene sheets. As anode materials for lithium ion batteries, they showed high reversible capacities, as well as significantly enhanced cycling performances (about 650 mA h g(-1) after 50 cycles) and high rate capabilities (350 mA h g(-1) at 5 C). The enhancement could be attributed to graphene sheets, which served as electron conductors and buffers. Our results opened a new doorway for the application of graphene sheets to prepare anode materials of lithium ion batteries with superior performances.
C1 [Chen, Libao] Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
RP Chen, LB (reprint author), Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM lbchen@hnu.edu.cn; thwang@hnu.cn
RI Wang, Taihong/K-8968-2012; Wei, Zhanhua/D-7544-2013; Zhang,
   Ming/F-1456-2014
OI Wei, Zhanhua/0000-0003-2687-0293; Zhang, Ming/0000-0003-4307-2058
FU National Key Basic Research Program of China [2007CB310500]; Chinese
   Ministry of Education [705040]; National Natural Science Foundation of
   China [90606009]
FX This work was partly supported by the "973'' National Key Basic Research
   Program of China (Grant No. 2007CB310500), Chinese Ministry of Education
   (Grant No. 705040), and National Natural Science Foundation of China
   (Grant No. 90606009).
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NR 35
TC 189
Z9 193
U1 35
U2 162
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2010
VL 20
IS 26
BP 5538
EP 5543
DI 10.1039/c0jm00638f
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 614HM
UT WOS:000279046200024
ER

PT J
AU Lian, PC
   Zhu, XF
   Liang, SZ
   Li, Z
   Yang, WS
   Wang, HH
AF Lian, Peichao
   Zhu, Xuefeng
   Liang, Shuzhao
   Li, Zhong
   Yang, Weishen
   Wang, Haihui
TI High reversible capacity of SnO2/graphene nanocomposite as an anode
   material for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene sheets; SnO2 nanoparticles; Nanocomposite; Anode material;
   Lithium-ion batteries
ID ONE-POT SYNTHESIS; IN-SITU SYNTHESIS; STORAGE PROPERTIES; HOLLOW
   NANOSPHERES; NEGATIVE-ELECTRODE; OXIDE COMPOSITE; AMORPHOUS OXIDE; SNO2
   NANOTUBES; THIN-FILMS; TIN
AB A gas-liquid interfacial synthesis approach has been developed to prepare SnO2/graphene nanocomposite. The as-prepared nanocomposite was characterized by X-ray diffraction, field emission scanning electron microscopy, transmission electron microscopy, and Brunauer-Emmett-Teller measurements. Field emission scanning electron microscopy and transmission electron microscopy observation revealed the homogeneous distribution of SnO2 nanoparticles (2-6 nm in size) on graphene matrix. The electrochemical performances were evaluated by using coin-type cells versus metallic lithium. The SnO2/graphene nanocomposite prepared by the gas-liquid interface reaction exhibits a high reversible specific capacity of 1304 mAh g(-1) at a current density of 100 mA g(-1) and excellent rate capability, even at a high current density of 1000 mA g(-1), the reversible capacity was still as high as 748 mAh g(-1). The electrochemical test results show that the SnO2/graphene nanocomposite prepared by the gas-liquid interfacial synthesis approach is a promising anode material for lithium-ion batteries. (c) 2011 Elsevier Ltd. All rights reserved.
C1 [Lian, Peichao; Liang, Shuzhao; Li, Zhong; Wang, Haihui] S China Univ Technol, Sch Chem &Chem Engn, Guangzhou 510640, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem &Chem Engn, 381 Wushan Rd, Guangzhou 510640, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620
FU National Natural Science Foundation of China [20936001]; SCUT
   [2009220038]
FX This work was financially supported by the National Natural Science
   Foundation of China (no. 20936001) and the Fundamental Research Funds
   for the Central Universities, SCUT (2009220038).
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NR 50
TC 188
Z9 194
U1 20
U2 167
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD APR 30
PY 2011
VL 56
IS 12
BP 4532
EP 4539
DI 10.1016/j.electacta.2011.01.126
PG 8
WC Electrochemistry
SC Electrochemistry
GA 765JL
UT WOS:000290701500016
ER

PT J
AU Luo, B
   Liu, SM
   Zhi, LJ
AF Luo, Bin
   Liu, Shaomin
   Zhi, Linjie
TI Chemical Approaches toward Graphene-Based Nanomaterials and their
   Applications in Energy-Related Areas
SO SMALL
LA English
DT Review
DE graphene; solar cells; lithium ion batteries; supercapacitors; catalysis
ID LITHIUM-ION BATTERIES; EXFOLIATED GRAPHITE OXIDE; ENHANCED
   ELECTROCATALYTIC ACTIVITY; SOLUTION-PROCESSABLE GRAPHENE; PERFORMANCE
   ANODE MATERIALS; CARBON NANOTUBE ELECTRODES; MIYAURA COUPLING REACTION;
   SENSITIZED SOLAR-CELLS; HIGH-QUALITY GRAPHENE; FEW-LAYER GRAPHENE
AB A gold rush has been triggered all over the world for exploiting the possible applications of graphene-based nanomaterials. For this purpose, two important problems have to be solved; one is the preparation of graphene-based nanomaterials with well-defined structures, and the other is the controllable fabrication of these materials into functional devices. This review gives a brief overview of the recent research concerning chemical and thermal approaches toward the production of well-defined graphene-based nanomaterials and their applications in energy-related areas, including solar cells, lithium ion secondary batteries, supercapacitors, and catalysis.
C1 [Luo, Bin; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
   [Liu, Shaomin] Curtin Univ, Dept Chem Engn, Perth, WA 6845, Australia.
RP Zhi, LJ (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Liu , Shaomin /E-3669-2010; Luo, Bin/P-7836-2015
OI Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [20973044]; Ministry of
   Science and Technology of China [2009AA03Z328, 2009DPA41220]; Chinese
   Academy of Sciences [KJCX2-YW-H21]; Guangdong-CAS [2009B091300007]
FX Financial support from the National Natural Science Foundation of China
   (Grant No. 20973044), the Ministry of Science and Technology of China
   (No. 2009AA03Z328 and No. 2009DPA41220), the Chinese Academy of Sciences
   (No. KJCX2-YW-H21), and the Guangdong-CAS strategic cooperation Program
   (2009B091300007) is acknowledged.
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NR 311
TC 185
Z9 191
U1 65
U2 387
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
J9 SMALL
JI Small
PD MAR 12
PY 2012
VL 8
IS 5
BP 630
EP 646
DI 10.1002/smll.201101396
PG 17
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 903ND
UT WOS:000301122400002
PM 22121112
ER

PT J
AU Peng, CX
   Chen, BD
   Qin, Y
   Yang, SH
   Li, CZ
   Zuo, YH
   Liu, SY
   Yang, JH
AF Peng, Chengxin
   Chen, Bingdi
   Qin, Yao
   Yang, Shihe
   Li, Chunzhong
   Zuo, Yuanhui
   Liu, Siyang
   Yang, Jinhu
TI Facile Ultrasonic Synthesis of CoO Quantum Dot/Graphene Nanosheet
   Composites with High Lithium Storage Capacity
SO ACS NANO
LA English
DT Article
DE ultrasonic synthesis; CoO quantum dots; graphene; composites;
   lithium-ion batteries; anode materials; lithium storage capacity
ID COBALT OXIDE COMPOSITES; ION BATTERY ELECTRODES; ANODE MATERIAL;
   ELECTROCHEMICAL PERFORMANCE; NANOSTRUCTURED MATERIALS; REVERSIBLE
   CAPACITY; CYCLIC PERFORMANCE; ENERGY-CONVERSION; NANOWIRE ARRAYS; LI
   STORAGE
AB In this paper, we report a facile ultrasonic method to synthesize well-dispersed CoO quantum dots (3-8 nm) on graphene nanosheets at room temperature by employing Co-4(CO)(12) as cobalt precursor. The prepared CoO/graphene composites displayed high performance as an anode material for lithium-ion battery, such as high reversible lithium storage capacity (1592 mAh g(-1) after 50 cycles), high Coulombic efficiency (over 95%), excellent cycling stability, and high rate capability (1008 mAh g(-1) with a total retention of 77.6% after 50 cycles at a current density of 1000 mA g(-1), dramatically increased from the initial 50 mA g(-1)). The extraordinary performance arises from the structure advantages of the composites: the nanosized CoO quantum dots with high dispersity on conductive graphene substrates supply not only large quantity of accessible active sites for lithium-ion insertion but also good conductivity and short diffusion length for lithium ions, which are beneficial for high capacity and rate capability. Meanwhile, the isolated CoO quantum dots anchored tightly on the graphene nanosheets can effectively circumvent the volume expansion/contraction associated with lithium insertion/extraction during discharge/charge processes, which is good for high capacity as well as cycling stability. Moreover, regarding the anomalous behavior of capacity increase with cycles (activation effect) observed, we proposed a tentative hypothesis stressing the competition between the conductivity increase and the amorphorization of the composite electrodes during cycling in determining the trends of the capacity, in the hope to gain a fuller understanding of the inner working of the novel nanostructured electrode-based lithium-ion batteries.
C1 [Peng, Chengxin; Chen, Bingdi; Qin, Yao; Zuo, Yuanhui; Liu, Siyang; Yang, Jinhu] Tongji Univ, Inst Adv Mat & Nano Biomed, Shanghai 200092, Peoples R China.
   [Peng, Chengxin; Chen, Bingdi; Qin, Yao; Zuo, Yuanhui; Liu, Siyang; Yang, Jinhu] Tongji Univ, Dept Chem, Shanghai 200092, Peoples R China.
   [Yang, Shihe] Hong Kong Univ Sci & Technol, William Mong Inst Nano Sci & Technol, Dept Chem, Nano Sci & Technol Program, Kowloon, Hong Kong, Peoples R China.
   [Li, Chunzhong] E China Univ Sci & Technol, Sch Mat Sci & Engn, Key Lab Ultrafine Mat, Minist Educ, Shanghai 200237, Peoples R China.
RP Yang, JH (reprint author), Tongji Univ, Inst Adv Mat & Nano Biomed, Chifeng Rd 67, Shanghai 200092, Peoples R China.
EM yangjinhu2010@gmail.com
RI Chen, Bingdi/I-5857-2012; Qin, Yao/K-6003-2012; Li,
   Chunzhong/B-1103-2015; 
OI Li, Chunzhong/0000-0001-7897-5850; Yang, Shihe/0000-0002-6469-8415
FU National Natural Science Foundation [21001082, 20925621]; Shanghai
   Pujiang Program [10PJ1410400]; Research Fund for the Doctoral Program of
   Higher Education of China [20090072120013]; Key Laboratory for Ultrafine
   Materials of Ministry of Education; East China University of Science,
   and Technology; Tongji University [2008KJ046, 2009KJ075]
FX We thank the National Natural Science Foundation (21001082, 20925621),
   Shanghai Pujiang Program (10PJ1410400), Research Fund for the Doctoral
   Program of Higher Education of China (20090072120013), Visiting scholar
   fund of the Key Laboratory for Ultrafine Materials of Ministry of
   Education, East China University of Science, and Technology and the
   Program for Young Excellent Talents in Tongji University (2008KJ046 and
   2009KJ075) for financial support.
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NR 52
TC 185
Z9 186
U1 58
U2 349
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD FEB
PY 2012
VL 6
IS 2
BP 1074
EP 1081
DI 10.1021/nn202888d
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
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SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 898QW
UT WOS:000300757900011
PM 22224549
ER

PT J
AU Sun, YM
   Hu, XL
   Luo, W
   Xia, FF
   Huang, YH
AF Sun, Yongming
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   Xia, Fangfang
   Huang, Yunhui
TI Reconstruction of Conformal Nanoscale MnO on Graphene as a High-Capacity
   and Long-Life Anode Material for Lithium Ion Batteries
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE anodes; cycling behavior; manganese oxide; graphene; lithium ion
   batteries
ID STORAGE PROPERTIES; REVERSIBLE CAPACITY; ELECTRODE MATERIALS; GRAPHITE
   OXIDE; PERFORMANCE; HYBRID; COO; NANOSTRUCTURES; NANOCOMPOSITES;
   NANOPARTICLES
AB To tackle the issue of inferior cycle stability and rate capability for MnO anode materials in lithium ion batteries, a facile strategy is explored to prepare a hybrid material consisting of MnO nanocrystals grown on conductive graphene nanosheets. The prepared MnO/graphene hybrid anode exhibits a reversible capacity as high as 2014.1 mAh g1 after 150 discharge/charge cycles at 200 mA g1, excellent rate capability (625.8 mAh g1 at 3000 mA g1), and superior cyclability (843.3 mAh g1 even after 400 discharge/charge cycles at 2000 mA g1 with only 0.01% capacity loss per cycle). The results suggest that the reconstruction of the MnO/graphene electrodes is intrinsic due to conversion reactions. A long-term stable nanoarchitecture of graphene-supported ultrafine manganese oxide nanoparticles is formed upon cycling, which yields a long-life anode material for lithium ion batteries. The lithiation and delithiation behavior suggests that the further oxidation of Mn(II) to Mn(IV) and the interfacial lithium storage upon cycling contribute to the enhanced specific capacity. The excellent rate capability benefits from the presence of conductive graphene and a short transportation length for both lithium ions and electrons. Moreover, the as-formed hybrid nanostructure of MnO on graphene may help achieve faster kinetics of conversion reactions.
C1 [Sun, Yongming; Hu, Xianluo; Luo, Wei; Xia, Fangfang; Huang, Yunhui] Huazhong Univ Sci & Technol, Coll Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
RP Hu, XL (reprint author), Huazhong Univ Sci & Technol, Coll Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
EM huxl@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Huang, Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010; Luo, Wei/E-1582-2011
OI Hu, Xianluo/0000-0002-5769-167X; 
FU Natural Science Foundation of China [51002057, 21271078, 50825203]; 863
   program [2009AA03Z225]; Natural Science Foundation of Hubei Province
   [2008CDA026]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 51002057, 21271078 and 50825203), the 863 program (Grant No.
   2009AA03Z225), the Natural Science Foundation of Hubei Province (Grant
   No. 2008CDA026), and the PCSIRT (Program for Changjiang Scholars and
   Innovative Research Team in University). The authors thank the
   Analytical and Testing Center of HUST for XRD, FESEM, TEM, and TG-DTA
   measurements.
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NR 57
TC 184
Z9 186
U1 53
U2 336
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD MAY 20
PY 2013
VL 23
IS 19
BP 2436
EP 2444
DI 10.1002/adfm.201202623
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 142PF
UT WOS:000318808800010
ER

PT J
AU Li, Z
   Xu, ZW
   Tan, XH
   Wang, HL
   Holt, CMB
   Stephenson, T
   Olsen, BC
   Mitlin, D
AF Li, Zhi
   Xu, Zhanwei
   Tan, Xuehai
   Wang, Huanlei
   Holt, Chris M. B.
   Stephenson, Tyler
   Olsen, Brian C.
   Mitlin, David
TI Mesoporous nitrogen-rich carbons derived from protein for ultra-high
   capacity battery anodes and supercapacitors
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID LITHIUM-ION BATTERIES; ENERGY-STORAGE; CARBONACEOUS MATERIALS; SUPERIOR
   PERFORMANCE; CATHODE MATERIALS; GRAPHITIC CARBON; GRAPHENE OXIDE; DOPED
   CARBON; ELECTRODES; ARCHITECTURE
AB In this work we demonstrate that biomass-derived proteins serve as an ideal precursor for synthesizing carbon materials for energy applications. The unique composition and structure of the carbons resulted in very promising electrochemical energy storage performance. We obtained a reversible lithium storage capacity of 1780 mA h g(-1), which is among the highest ever reported for any carbon-based electrode. Tested as a supercapacitor, the carbons exhibited a capacitance of 390 F g(-1), with an excellent cycle life (7% loss after 10 000 cycles). Such exquisite properties may be attributed to a unique combination of a high specific surface area, partial graphitization and very high bulk nitrogen content. It is a major challenge to derive carbons possessing all three attributes. By templating the structure of mesoporous cellular foam with egg white-derived proteins, we were able to obtain hierarchically mesoporous (pores centered at similar to 4 nm and at 20-30 nm) partially graphitized carbons with a surface area of 805.7 m(2) g(-1) and a bulk N-content of 10.1 wt%. When the best performing sample was heated in Ar to eliminate most of the nitrogen, the Li storage capacity and the specific capacitance dropped to 716 mA h g(-1) and 80 F g(-1), respectively.
C1 [Li, Zhi; Xu, Zhanwei; Tan, Xuehai; Wang, Huanlei; Holt, Chris M. B.; Stephenson, Tyler; Olsen, Brian C.; Mitlin, David] Univ Alberta, Edmonton, AB T6G 2V4, Canada.
   [Li, Zhi; Xu, Zhanwei; Tan, Xuehai; Wang, Huanlei; Holt, Chris M. B.; Stephenson, Tyler; Olsen, Brian C.; Mitlin, David] NRC, Natl Inst Nanotechnol NINT, Edmonton, AB T6G 2M9, Canada.
RP Li, Z (reprint author), Univ Alberta, 9107-116 St, Edmonton, AB T6G 2V4, Canada.
EM huanleiwang@gmail.com; dmitlin@ualberta.ca
RI Wang, Huanlei/F-2061-2013; Li, Zhi/H-3377-2011; 
OI Li, Zhi/0000-0003-1668-4948; Olsen, Brian/0000-0001-9758-3641
FU Alberta Innovates Bio Solutions; Alberta Egg Farmers; Alberta Livestock
   and Meat Agency (ALMA); NINT NRC
FX Funding by Alberta Innovates Bio Solutions, Alberta Egg Farmers, Alberta
   Livestock and Meat Agency (ALMA) and NINT NRC.
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NR 58
TC 181
Z9 181
U1 73
U2 491
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD MAR
PY 2013
VL 6
IS 3
BP 871
EP 878
DI 10.1039/c2ee23599d
PG 8
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 093BC
UT WOS:000315165700022
ER

PT J
AU Zhou, XS
   Yin, YX
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Yin, Ya-Xia
   Wan, Li-Jun
   Guo, Yu-Guo
TI Facile synthesis of silicon nanoparticles inserted into graphene sheets
   as improved anode materials for lithium-ion batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID STORAGE DEVICES; HIGH-CAPACITY; NANOSTRUCTURED MATERIALS;
   ENERGY-CONVERSION; CATHODE MATERIAL; SI; NANOCOMPOSITES; NANOSPHERES;
   PERFORMANCE; LI
AB Silicon nanoparticles have been successfully inserted into graphene sheets via a novel method combining freeze-drying and thermal reduction. The as-obtained Si/graphene nanocomposite exhibits remarkably enhanced cycling performance and rate performance compared with bare Si nanoparticles for lithium-ion batteries.
C1 [Zhou, Xiaosi; Yin, Ya-Xia; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Key Project on Basic Research [2011CB935700, 2009CB930400,
   2012CB932900]; National Natural Science Foundation of China [91127044,
   2112106]; CAS
FX This work was supported by the National Key Project on Basic Research
   (Grants 2011CB935700, 2009CB930400 and 2012CB932900), the National
   Natural Science Foundation of China (Grants 91127044 and 2112106), and
   the CAS.
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NR 35
TC 177
Z9 181
U1 37
U2 317
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PD FEB 21
PY 2012
VL 48
IS 16
BP 2198
EP 2200
DI 10.1039/c2cc17061b
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 895YV
UT WOS:000300533500008
PM 22252533
ER

PT J
AU Zhang, CZ
   Mahmood, N
   Yin, H
   Liu, F
   Hou, YL
AF Zhang, Chenzhen
   Mahmood, Nasir
   Yin, Han
   Liu, Fei
   Hou, Yanglong
TI Synthesis of Phosphorus-Doped Graphene and its Multifunctional
   Applications for Oxygen Reduction Reaction and Lithium Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE phosphorus-doped graphene; synthesis; oxygen reduction reaction; lithium
   ion batteries
ID METAL-FREE ELECTROCATALYSTS; CARBON NANOTUBES; ANODE MATERIALS; GRAPHITE
   OXIDE; HIGH-YIELD; NITROGEN; SHEETS; FILMS; PERFORMANCE; SULFUR
C1 [Zhang, Chenzhen; Mahmood, Nasir; Yin, Han; Liu, Fei; Hou, Yanglong] Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China.
RP Hou, YL (reprint author), Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China.
EM hou@pku.edu.cn
RI Yin, Han/G-1745-2012; Hou, Yanglong/B-8688-2012
FU NSFC [51125001, 51172005, 90922033]; National Basic Research Program of
   China [2010CB934601]; Natural Science Foundation of Beijing [2122022];
   New Century Talent of the Education Ministry of China [NCET-09-0177];
   Yok Ying Tung Foundation [122043];  [20120001110078]
FX This work was supported in part by the NSFC (51125001, 51172005,
   90922033), the National Basic Research Program of China (2010CB934601),
   the Natural Science Foundation of Beijing (2122022), the Doctoral
   Program (20120001110078) and New Century Talent of the Education
   Ministry of China (NCET-09-0177), and Yok Ying Tung Foundation (122043).
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NR 49
TC 176
Z9 179
U1 80
U2 433
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD SEP 20
PY 2013
VL 25
IS 35
BP 4932
EP 4937
DI 10.1002/adma.201301870
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 261VN
UT WOS:000327692800015
PM 23864555
ER

PT J
AU Luo, JY
   Zhao, X
   Wu, JS
   Jang, HD
   Kung, HH
   Huang, JX
AF Luo, Jiayan
   Zhao, Xin
   Wu, Jinsong
   Jang, Hee Dong
   Kung, Harold H.
   Huang, Jiaxing
TI Crumpled Graphene-Encapsulated Si Nanoparticles for Lithium Ion Battery
   Anodes
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID POROUS SILICON PARTICLES; CARBON-COATED SILICON; HIGH-CAPACITY;
   ELECTRODE MATERIALS; OXIDE; STORAGE; COMPOSITE; NANOCOMPOSITES;
   CHALLENGES; NANOWIRES
AB Submicrometer-sized capsules made of Si nanoparticles wrapped by crumpled graphene shells were made by a rapid, one-step capillary-driven assembly route in aerosol droplets. Aqueous dispersion of micrometer-sized graphene oxide (GO) sheets and Si nanoparticles were nebulized to form aerosol droplets, which were passed through a preheated tube furnace. Evaporation-induced capillary force wrapped graphene (a.k.a., reduced GO) sheets around the Si particles, and heavily crumpled the shell. The folds and wrinkles in the crumpled graphene coating can accommodate the volume expansion of Si upon lithiation without fracture, and thus help to protect Si nanoparticles from excessive deposition of the insulating solid electrolyte interphase. Compared to the native Si particles, the composite capsules have greatly improved performance as Li ion battery anodes in terms of capacity, cycling stability, and Coulombic efficiency.
C1 [Luo, Jiayan; Wu, Jinsong; Huang, Jiaxing] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.
   [Zhao, Xin; Kung, Harold H.] Northwestern Univ, Dept Chem Engn, Evanston, IL 60208 USA.
   [Jang, Hee Dong] Korea Inst Geosci & Mineral Resources, Rare Met Res Ctr, Taejon 305350, South Korea.
RP Huang, JX (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.
EM Jiaxing-huang@northwestern.edu
RI Huang, Jiaxing/A-9417-2012; Huang, Jiaxing/B-7521-2009; Luo,
   Jiayan/A-9927-2011
FU Initiative for Sustainability and Energy at Northwestern (ISEN); 3M
   graduate fellowship; Ryan Fellowship; Northwestern University
   International Institute for Nanotechnology; Ministry of Knowledge
   Economy of Korea; U.S. Department of Energy, Basic Energy Sciences
   through the Center for Electrical Energy Storage, an Energy Frontier
   Research Center [DE-AC02-06CH11357]
FX J.H. thanks the Initiative for Sustainability and Energy at Northwestern
   (ISEN) for an Early Career Investigator Award, a Sloan Research
   Fellowship, and the Sony Corporation for an unrestricted gift donation.
   J.L. gratefully acknowledges support from the 3M graduate fellowship,
   the Ryan Fellowship, and the Northwestern University International
   Institute for Nanotechnology. H.D.J. thanks the General Research Project
   of the Korea Institute of Geoscience and Mineral Resources (KIGAM)
   funded by the Ministry of Knowledge Economy of Korea. X.Z. and H.H.K.
   were supported by the U.S. Department of Energy, Basic Energy Sciences,
   Grant DE-AC02-06CH11357 through the Center for Electrical Energy
   Storage, an Energy Frontier Research Center.
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NR 39
TC 168
Z9 170
U1 47
U2 359
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD JUL 5
PY 2012
VL 3
IS 13
BP 1824
EP 1829
DI 10.1021/jz3006892
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 972BQ
UT WOS:000306251900018
PM 26291867
ER

PT J
AU Zhao, X
   Hayner, CM
   Kung, MC
   Kung, HH
AF Zhao, Xin
   Hayner, Cary M.
   Kung, Mayfair C.
   Kung, Harold H.
TI Flexible Holey Graphene Paper Electrodes with Enhanced Rate Capability
   for Energy Storage Applications
SO ACS NANO
LA English
DT Article
DE holey; graphene; defects; electrode; Li-ion battery
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIALS; ELECTROCHEMICAL
   CAPACITORS; RECHARGEABLE BATTERIES; CARBONACEOUS MATERIALS; REVERSIBLE
   CAPACITY; CYCLIC PERFORMANCE; GRAPHITE OXIDE; LI STORAGE; SHEETS
AB The unique combination of high surface area, high electrical conductivity and robust mechanical integrity has attracted great interest in the use of graphene sheets for future electronics applications. Their potential applications for high-power energy storage devices, however, are restricted by the accessible volume, which may be only a fraction of the physical volume, a consequence of the compact geometry of the stack and the ion mobility. Here we demonstrated that remarkably enhanced power delivery can be realized in graphene papers for the use in Li-ion batteries by controlled generation of in-plane porosity via a mechanical cavitation-chemical oxidation approach. These flexible,, holey graphene papers, created via facile microscopic engineering, possess abundant ion binding sites, enhanced Ion diffusion kinetics, and excellent high-rate lithium-ion storage capabilities, and are suitable for high-performance energy storage devices.
C1 [Zhao, Xin; Hayner, Cary M.; Kung, Mayfair C.; Kung, Harold H.] Northwestern Univ, Chem & Biol Engn Dept, Evanston, IL 60208 USA.
RP Kung, HH (reprint author), Northwestern Univ, Chem & Biol Engn Dept, Evanston, IL 60208 USA.
EM hkung@northwestern.edu
RI Kung, Harold/B-7647-2009; Kung, Mayfair/B-7648-2009
FU Center for Electrical Energy Storage, an Energy Frontier Research
   Center; U.S. Department of Energy, Office of Science and Office of Basic
   Energy Sciences [DE-ACO2-06CH11357]
FX This research was supported by the Center for Electrical Energy Storage,
   an Energy Frontier Research Center funded by the U.S. Department of
   Energy, Office of Science and Office of Basic Energy Sciences, grant no.
   DE-ACO2-06CH11357.
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TC 168
Z9 170
U1 69
U2 330
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2011
VL 5
IS 11
BP 8739
EP 8749
DI 10.1021/nn202710s
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 849RR
UT WOS:000297143300032
PM 21980979
ER

PT J
AU Huang, X
   Tan, CL
   Yin, ZY
   Zhang, H
AF Huang, Xiao
   Tan, Chaoliang
   Yin, Zongyou
   Zhang, Hua
TI 25th Anniversary Article: Hybrid Nanostructures Based on Two-Dimensional
   Nanomaterials
SO ADVANCED MATERIALS
LA English
DT Review
DE two-dimensional nanomaterials; graphene; transition metal
   dichalcogenides; hybrid nanostructures; heterostructures
ID LITHIUM-ION BATTERIES; REDUCED GRAPHENE OXIDE; OXYGEN REDUCTION
   REACTION; HYDROGEN EVOLUTION REACTION; PERFORMANCE ANODE MATERIAL;
   CARBON NANOTUBE AEROGELS; HEXAGONAL BORON-NITRIDE; NITROGEN-DOPED
   GRAPHENE; DER-WAALS EPITAXY; CDSE QUANTUM DOTS
AB Two-dimensional (2D) nanomaterials, such as graphene and transition metal dichalcogenides (TMDs), receive a lot of attention, because of their intriguing properties and wide applications in catalysis, energy-storage devices, electronics, optoelectronics, and so on. To further enhance the performance of their application, these 2D nanomaterials are hybridized with other functional nanostructures. In this review, the latest studies of 2D nanomaterial-based hybrid nanostructures are discussed, focusing on their preparation methods, properties, and applications.
C1 [Huang, Xiao; Tan, Chaoliang; Yin, Zongyou; Zhang, Hua] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
RP Zhang, H (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM hzhang@ntu.edu.sg
RI Huang, Xiao/B-7720-2014; Zhang, Hua/A-1302-2009
FU MOE under AcRF in Singapore [ARC 26/13, MOE2013-T2-1-034, RG 61/12,
   RGT18/13, RG5/13]; Singapore National Research Foundation; Campus for
   Research Excellence And Technological Enterprise (CREATE) programme
   (Nanomaterials for Energy and Water Management)
FX This article is part of a series celebrating the 25th anniversary of
   Advanced Materials. This work was supported by MOE under AcRF Tier 2
   (ARC 26/13, No. MOE2013-T2-1-034), AcRF Tier 1 (RG 61/12, RGT18/13 and
   RG5/13), and Start-Up Grant (M4080865.070.706022) in Singapore. This
   research is also funded by the Singapore National Research Foundation
   and the publication is supported under the Campus for Research
   Excellence And Technological Enterprise (CREATE) programme
   (Nanomaterials for Energy and Water Management).
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NR 268
TC 165
Z9 165
U1 302
U2 1032
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA POSTFACH 101161, 69451 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD APR
PY 2014
VL 26
IS 14
BP 2185
EP 2204
DI 10.1002/adma.201304964
PG 20
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AF0IV
UT WOS:000334398400004
PM 24615947
ER

PT J
AU Shin, WH
   Jeong, HM
   Kim, BG
   Kang, JK
   Choi, JW
AF Shin, Weon Ho
   Jeong, Hyung Mo
   Kim, Byung Gon
   Kang, Jeung Ku
   Choi, Jang Wook
TI Nitrogen-Doped Multiwall Carbon Nanotubes for Lithium Storage with
   Extremely High Capacity
SO NANO LETTERS
LA English
DT Article
DE Carbon nanotubes; nitrogen-doping; lithium ion capacitor; metal oxide;
   high capacity; long lifetime
ID ELECTROCHEMICAL REACTIVITY; BATTERY APPLICATION; ION BATTERIES;
   GRAPHENE; ULTRACAPACITORS; PERFORMANCE; CHALLENGES; ELECTRODES; ANODES;
   ATOMS
AB The increasing demands on high performance energy storage systems have raised a new class of devices, so-called lithium ion capacitors (LICs). As its name says, LIC is an intermediate system between lithium ion batteries and supercapacitors, designed for taking advantages of both types of energy storage systems. Herein, as a quest to improve the Li storage capability compared to that of other existing carbon nanomaterials, we have developed extrinsically defective multiwall carbon nanotubes by nitrogen-doping. Nitrogen-doped carbon nanotubes contain wall defects through which lithium ions can diffuse so as to occupy a large portion of the interwall space as storage regions. Furthermore, when integrated with 3 nm nickel oxide nanoparticles for a further capacity boost, nitrogen doping enables unprecedented cell performance by engaging anomalous electrochemical phenomena such as nanoparticles division into even smaller ones, their agglomeration-free diffusion between nitrogen-doped sites as well as capacity rise with cycles. The final cells exhibit a capacity as high as 3500 mAh/g, a cycle life of greater than 10 000 times, and a discharge rate capability of 1.5 min while retaining a capacity of 350 mAh/g.
C1 [Shin, Weon Ho; Kim, Byung Gon; Kang, Jeung Ku; Choi, Jang Wook] Korea Adv Inst Sci & Technol, Grad Sch EEWS WCU, Taejon 305701, South Korea.
   [Jeong, Hyung Mo; Kang, Jeung Ku] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea.
   [Kang, Jeung Ku] Korea Adv Inst Sci & Technol, KAIST Inst Nanocentury, Taejon 305701, South Korea.
RP Kang, JK (reprint author), Korea Adv Inst Sci & Technol, Grad Sch EEWS WCU, 373-1 Guseong Dong, Taejon 305701, South Korea.
EM jeung@kaistackr.ac.kr; jangwookchoi@kaist.ac.kr
RI Choi, Jang Wook/C-1821-2011; Kang, Jeung ku/C-1610-2011
OI Choi, Jang Wook/0000-0001-8783-0901; 
FU National Research Foundation of Korea; Korean Government (MEST)
   [NRF-2010-0029031]; Korea Basic Science Institute [T32413]; World Class
   University [R-31-2008-000-10055-0]
FX We are pleased to acknowledge the National Research Foundation of Korea
   Grant funded by the Korean Government (MEST) for the financial support
   through the Secondary Battery Program (NRF-2010-0029031), Korea Basic
   Science Institute Grant (T32413), and the World Class University Program
   (R-31-2008-000-10055-0) for the financial support.
CR Jiang KY, 2003, NANO LETT, V3, P275, DOI 10.1021/nl025914t
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NR 31
TC 159
Z9 159
U1 37
U2 232
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD MAY
PY 2012
VL 12
IS 5
BP 2283
EP 2288
DI 10.1021/nl3000908
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 937XE
UT WOS:000303696400019
PM 22452675
ER

PT J
AU Chen, DY
   Ji, G
   Ma, Y
   Lee, JY
   Lu, JM
AF Chen, Dongyun
   Ji, Ge
   Ma, Yue
   Lee, Jim Yang
   Lu, Jianmei
TI Graphene-Encapsulated Hollow Fe3O4 Nanoparticle Aggregates As a
   High-Performance Anode Material for Lithium Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE Fe3O4; graphene; anode material; lithium ion batteries
ID HIGH-CAPACITY; CYCLING PERFORMANCE; REVERSIBLE CAPACITY; STORAGE;
   FABRICATION; NANOTUBES; NANOCOMPOSITES; ELECTRODES; ANATASE; FILMS
AB Graphene-encapsulated ordered aggregates of Fe3O4 nanoparticles with nearly spherical geometry and hollow interior were synthesized by a simple self-assembly process. The open interior structure adapts well to the volume change in repetitive Li+ insertion and extraction reactions; and the encapsulating graphene connects the Fe3O4 nanoparticles electrically. The structure and morphology of the grapheneFe(3)O(4) composite were confirmed by X-ray diffraction, scanning electron microscopy, and high-resolution transmission microscopy. The electrochemical performance of the composite for reversible Li+ storage was evaluated by cyclic voltammetry and constant current charging and discharging. The results showed a high and nearly unvarying specific capacity for 50 cycles. Furthermore, even after 90 cycles of charge and discharge at different current densities, about 92% of the initial capacity at 100 mA g(-1) was still recoverable, indicating excellent cycle stability. The graphene Fe3O4 composite is therefore a capable Li+ host with high capacity that can be cycled at high rates with good cycle life. The unique combination of graphene encapsulation and a hollow porous structure definitely contributed to this versatile electrochemical performance.
C1 [Chen, Dongyun; Ji, Ge; Ma, Yue; Lee, Jim Yang] Natl Univ Singapore, Dept Chem & Biomol Engn, Fac Engn, Singapore 119260, Singapore.
   [Chen, Dongyun; Lu, Jianmei] Soochow Univ, Key Lab Organ Synth Jiangsu Prov, Key Lab Funct Mat Environm Protect, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China.
RP Lee, JY (reprint author), Natl Univ Singapore, Dept Chem & Biomol Engn, Fac Engn, 10 Kent Ridge Crescent, Singapore 119260, Singapore.
EM cheleejy@nus.edu.sg; lujm@suda.edu.cn
RI LEE, Jim Yang/E-5904-2010; Lu, Jian-Mei/H-1186-2012
OI Lu, Jian-Mei/0000-0003-2302-3275
FU China Scholarship Council (CSC)
FX The attachment of D.C. to the National University of Singapore is
   partially financially supported by the China Scholarship Council (CSC).
CR Wang B, 2010, J MATER CHEM, V20, P10661, DOI 10.1039/c0jm01941k
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NR 40
TC 158
Z9 160
U1 28
U2 221
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD AUG
PY 2011
VL 3
IS 8
BP 3078
EP 3083
DI 10.1021/am200592r
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 810SH
UT WOS:000294146900037
PM 21749101
ER

PT J
AU Cao, XH
   Shi, YM
   Shi, WH
   Rui, XH
   Yan, QY
   Kong, J
   Zhang, H
AF Cao, Xiehong
   Shi, Yumeng
   Shi, Wenhui
   Rui, Xianhong
   Yan, Qingyu
   Kong, Jing
   Zhang, Hua
TI Preparation of MoS2-Coated Three-Dimensional Graphene Networks for
   High-Performance Anode Material in Lithium-Ion Batteries
SO SMALL
LA English
DT Article
DE MoS2; graphene networks; chemical vapor deposition; lithium-ion
   batteries; binder-free materials
ID METAL DICHALCOGENIDE NANOSHEETS; LI-ION; STORAGE PROPERTIES; MOS2;
   CARBON; OXIDE; NANOSTRUCTURES; ELECTRODES; GROWTH; SUPERCAPACITOR
AB A novel composite, MoS2-coated three-dimensional graphene network (3DGN), referred to as MoS2/3DGN, is synthesized by a facile CVD method. The 3DGN, composed of interconnected graphene sheets, not only serves as template for the deposition of MoS2, but also provides good electrical contact between the current collector and deposited MoS2. As a proof of concept, the MoS2/3DGN composite, used as an anode material for lithium-ion batteries, shows excellent electrochemical performance, which exhibits reversible capacities of 877 and 665 mAh g(-1) during the 50(th) cycle at current densities of 100 and 500 mA g(-1), respectively, indicating its good cycling performance. Furthermore, the MoS2/3DGN composite also shows excellent high-current-density performance, e.g., depicts a 10(th)-cycle capacity of 466 mAh g(-1) at a high current density of 4 A g(-1).
C1 [Cao, Xiehong; Shi, Wenhui; Rui, Xianhong; Yan, Qingyu; Zhang, Hua] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Shi, Yumeng; Kong, Jing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA.
RP Zhang, H (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM hzhang@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; Rui, Xianhong/D-2604-2015; Cao,
   Xiehong/I-9665-2014; Zhang, Hua/A-1302-2009; Shi, Yumeng/A-7349-2012
OI Rui, Xianhong/0000-0003-1125-0905; Cao, Xiehong/0000-0002-3004-7518;
   Shi, Yumeng/0000-0002-9623-3778
FU MOE under AcRF [ARC 10/10, MOE2010-T2-1-060]; Singapore National
   Research Foundation under CREATE programme: Nanomaterials for Energy and
   Water Management; NTU under the Start-Up Grant in Singapore
   [M4080865.070.706022]; A*STAR SERC [1021700144]; Singapore National
   Research Foundation under CREATE program: EMobility in Megacities
FX X. Cao and Y. Shi contributed equally to this work. This work was
   supported by MOE under AcRF Tier 2 (ARC 10/10, No. MOE2010-T2-1-060),
   Singapore National Research Foundation under CREATE programme:
   Nanomaterials for Energy and Water Management, and NTU under the
   Start-Up Grant (M4080865.070.706022) in Singapore. Q. Yan thanks A*STAR
   SERC grant 1021700144 and Singapore National Research Foundation under
   CREATE program: EMobility in Megacities.
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NR 48
TC 156
Z9 158
U1 112
U2 711
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD OCT 25
PY 2013
VL 9
IS 20
BP 3433
EP 3438
DI 10.1002/smll.201202697
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 239JB
UT WOS:000326017700012
PM 23637090
ER

PT J
AU Qiu, YC
   Yan, KY
   Yang, SH
   Jin, LM
   Deng, H
   Li, WS
AF Qiu, Yongcai
   Yan, Keyou
   Yang, Shihe
   Jin, Limin
   Deng, Hong
   Li, Weishan
TI Synthesis of Size-Tunable Anatase TiO2 Nanospindles and Their Assembly
   into Anatase@Titanium Oxynitride/Titanium Nitride-Graphene
   Nanocomposites for Rechargeable Lithium Ion Batteries with High Cycling
   Performance
SO ACS NANO
LA English
DT Article
DE anatase nanospindles; TiO2@TiOxNy/TiN-graphene; nanocomposite; anode;
   lithium ion batteries
ID NANOCRYSTALLINE TIO2; VISIBLE-LIGHT; PARTICLE-SIZE; LI-STORAGE; OXIDE;
   NANOWIRES; NANOSTRUCTURES; NANOTUBES; ELECTRODES; EFFICIENCY
AB This paper embarks upon three levels of undertaking ranging from nanomaterials synthesis to assembly and functionalization. First, we have prepared size-tunable anatase TiO2 nanospindles via a hydrothermal process by using tubular titanates as self sacrificing precursors. Second, we have densely dispersed the TiO2 nanospindles onto functional graphene oxides (GO) via a spontaneous self assembly process. After annealing of the TiO2/GO hybrid nanocomposite in an NH3 gas flow, the TiO2 surface was effectively nitridated and the GO was reduced to graphene sheets (GS) in order to further fortify the electronic functionality of the nanocomposite. Third, the anatase@oxynitride/titanium nitride GS(TiO2@TiOxNy/TiN-GS) hybrid nanocomposite was studied as an anode material for lithium ion batteries (LIBS). showing excellent rate capability and cycling performance compared to the pure TiO2 nanospindles. Our systematic studies have revealed that the TiO2@TiOxNy/TiN-GS nanocomposite with graphene nanosheets covered with the TiO2@TiOxNy/TiN nanospindles on both sides provide a promising solutions to the problems of poor electron transport and severe aggregation of TiO2 nanoparticles by enhancing both electron transport through the conductive matrix and Li ion accessibility to the active material from the liquid electrolyte. More generally, the size-tunable TiO2 nanospindles with their unique (101) outer surface planes provide an archetype for the in depth investigation of their surface-specific and size dependent phsicochemical properties.
C1 [Qiu, Yongcai; Yan, Keyou; Yang, Shihe] Hong Kong Univ Sci & Technol, Dept Chem, Nano Sci & Technol Program, William Mong Inst Nano Sci & Technol, Kowloon, Hong Kong, Peoples R China.
   [Jin, Limin; Deng, Hong; Li, Weishan] S China Normal Univ, Sch Chem & Environm, Guangzhou 510006, Guangdong, Peoples R China.
   [Jin, Limin; Deng, Hong; Li, Weishan] S China Normal Univ, Guangdong Higher Educ Inst, Key Lab Electrochem Technol Energy Storage & Powe, Guangzhou 510006, Guangdong, Peoples R China.
RP Yang, SH (reprint author), Hong Kong Univ Sci & Technol, Dept Chem, Nano Sci & Technol Program, William Mong Inst Nano Sci & Technol, Kowloon, Hong Kong, Peoples R China.
RI Qiu, Yongcai/J-6562-2012; Yan, Keyou/N-1991-2013
OI Qiu, Yongcai/0000-0002-7843-6811; 
FU NSFC/HK RGC [N_HKUST609/09]; HK RGC (GRF) [HKUST 604809]
FX This work was supported by the NSFC/HK RGC Joint Research Scheme
   (N_HKUST609/09) and the HK RGC General Research Funds (GRF No HKUST
   604809)
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PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2010
VL 4
IS 11
BP 6515
EP 6526
DI 10.1021/nn101603g
PG 12
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 682YD
UT WOS:000284438000027
PM 21038869
ER

PT J
AU Xu, YH
   Liu, Q
   Zhu, YJ
   Liu, YH
   Langrock, A
   Zachariah, MR
   Wang, CS
AF Xu, Yunhua
   Liu, Qing
   Zhu, Yujie
   Liu, Yihang
   Langrock, Alex
   Zachariah, Michael R.
   Wang, Chunsheng
TI Uniform Nano-Sn/C Composite Anodes for Lithium Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Tin nanoparticle; aerosol spray pyrolysis; anode; energy storage;
   lithium-ion battery
ID HOLLOW CARBON; SECONDARY BATTERIES; ALLOY ANODE; C COMPOSITE; TIN;
   PERFORMANCE; NANOPARTICLES; INSERTION; GRAPHITE; GRAPHENE
AB Nano-Sn/C composites are ideal anode materials for high energy and power density Li-ion batteries. However, because of the low melting point of Sn and the tendency of grain growth, especially during high temperature carbonization, it has been a significant challenge to create well-dispersed ultrasmall Sn nanoparticles within a carbon matrix. In this paper, we demonstrate an aerosol spray pyrolysis technique, as a facile and scalable method, to synthesize a nano-Sn/C composite with uniformly dispersed 10 nm nano-Sn within a spherical carbon matrix. The discharge capacity of nano-Sn/C composite sphere anodes maintains the initial capacity of 710 mAh/g after 130 cycles at 0.25 C. The nano-Sn/C composite sphere anodes can provide similar to 600 mAh/g even at a high rate of 20 C. To the best of our knowledge, such high rate performance for Sn anodes has not been reported previously. The exceptional performance of the nano-Sn/C composite is attributed to the unique nano-Sn/C structure: (1) carbon matrix offers mechanical support to accommodate the stress associated with the large volume change of nano-Sn, thus alleviating pulverization; (2) the carbon matrix prevents Sn nanoparticle agglomeration upon prolonged cycling; and (3) carbon network provides continuous path for Li ions and electrons inside the nano-Sn/C composite spheres.
C1 [Xu, Yunhua; Zhu, Yujie; Liu, Yihang; Langrock, Alex; Wang, Chunsheng] Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA.
   [Liu, Qing; Zachariah, Michael R.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA.
RP Zachariah, MR (reprint author), Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA.
EM mrz@umd.edu; cswang@umd.edu
RI Wang, Chunsheng/H-5767-2011; Xu, Yunhua/D-7751-2012; Langrock,
   Alex/E-8567-2015; Liu, Yihang/E-6958-2013
OI Wang, Chunsheng/0000-0002-8626-6381; Liu, Yihang/0000-0002-2491-9439
FU Army Research Office [W911NF1110231]; Ellen Williams Distinguished
   Postdoctoral Fellowship
FX The authors gratefully acknowledge the support of the Army Research
   Office under Contract No.: W911NF1110231 (Dr. Robert Mantz, Program
   Manager) and Ellen Williams Distinguished Postdoctoral Fellowship.
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PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
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JI Nano Lett.
PD FEB
PY 2013
VL 13
IS 2
BP 470
EP 474
DI 10.1021/nl303823k
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 091WC
UT WOS:000315079500023
PM 23282084
ER

PT J
AU Fang, Y
   Lv, YY
   Che, RC
   Wu, HY
   Zhang, XH
   Gu, D
   Zheng, GF
   Zhao, DY
AF Fang, Yin
   Lv, Yingying
   Che, Renchao
   Wu, Haoyu
   Zhang, Xuehua
   Gu, Dong
   Zheng, Gengfeng
   Zhao, Dongyuan
TI Two-Dimensional Mesoporous Carbon Nanosheets and Their Derived Graphene
   Nanosheets: Synthesis and Efficient Lithium Ion Storage
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID OXYGEN REDUCTION; ENERGY-STORAGE; PERFORMANCE; FILMS; OXIDE;
   NANOCOMPOSITES; NANOSPHERES; FABRICATION; NANOTUBES; BATTERIES
AB We report a new solution deposition method to synthesize an unprecedented type of two-dimensional ordered mesoporous carbon nanosheets via a controlled low-concentration monomicelle close-packing assembly approach. These obtained carbon nanosheets possess only one layer of ordered mesopores on the surface of a substrate, typically the inner walls of anodic aluminum oxide pore channels, and can be further converted into mesoporous graphene nanosheets by carbonization. The atomically flat graphene layers with mesopores provide high surface area for lithium ion adsorption and intercalation, while the ordered mesopores perpendicular to the graphene layer enable efficient ion transport as well as volume expansion flexibility, thus representing a unique orthogonal architecture for excellent lithium ion storage capacity and cycling performance. Lithium ion battery anodes made of the mesoporous graphene nanosheets have exhibited an excellent reversible capacity of 1040 mAh/g at 100 mA/g, and they can retain at 833 mAh/g even after numerous cycles at varied current densities. Even at a large current density of 5 A/g, the reversible capacity is retained around 255 mAh/g, larger than for most other porous carbon-based anodes previously reported, suggesting a remarkably promising candidate for energy storage.
C1 [Fang, Yin; Lv, Yingying; Che, Renchao; Wu, Haoyu; Gu, Dong; Zheng, Gengfeng; Zhao, Dongyuan] Fudan Univ, Dept Chem, Adv Mat Lab, Shanghai 200433, Peoples R China.
   [Fang, Yin; Lv, Yingying; Che, Renchao; Wu, Haoyu; Gu, Dong; Zheng, Gengfeng; Zhao, Dongyuan] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
   [Zhang, Xuehua] Univ Melbourne, Dept Chem & Biomol Engn, Melbourne, Vic 3010, Australia.
RP Zhao, DY (reprint author), Fudan Univ, Dept Chem, Adv Mat Lab, Shanghai 200433, Peoples R China.
EM dyzhao@fudan.edu.cn
RI zhang, xuehua/G-1085-2010; Zheng, Gengfeng/G-7023-2011; Zhao,
   Dongyuan/E-5796-2010; Gu, Dong/D-1940-2009
OI Zheng, Gengfeng/0000-0002-1803-6955; Gu, Dong/0000-0003-4600-4499
FU State Key Basic Research Program of the PRC [2012CB224805,
   2013CB934104]; NSF of China [20890123, 429 21200004]; Shanghai Leading
   Academic Discipline Project [B108]; Science and Technology Commission of
   Shanghai Municipality [08DZ2270500]; Delta Company Foundation;
   Scholarship Award for Excellent Doctoral Student granted by Ministry of
   Education
FX This work was supported by the State Key Basic Research Program of the
   PRC (2012CB224805, 2013CB934104), the NSF of China (20890123 and 429
   21200004), the Shanghai Leading Academic Discipline Project (B108), the
   Science and Technology Commission of Shanghai Municipality
   (08DZ2270500), Delta Company Foundation, and the Scholarship Award for
   Excellent Doctoral Student granted by Ministry of Education.
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TC 150
Z9 153
U1 93
U2 743
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD JAN 30
PY 2013
VL 135
IS 4
BP 1524
EP 1530
DI 10.1021/ja310849c
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA 083VE
UT WOS:000314492500056
PM 23282081
ER

PT J
AU Zhou, XS
   Yin, YX
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Yin, Ya-Xia
   Wan, Li-Jun
   Guo, Yu-Guo
TI Self-Assembled Nanocomposite of Silicon Nanoparticles Encapsulated in
   Graphene through Electrostatic Attraction for Lithium-Ion Batteries
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE electrostatic attraction; graphene; lithium-ion batteries;
   self-assembly; silicon nanoparticles
ID ANODE MATERIALS; HOLLOW NANOSPHERES; STORAGE DEVICES; ENERGY-STORAGE;
   SI; LI; PERFORMANCE; NANOWIRES; ELECTRODE; FABRICATION
C1 [Zhou, Xiaosi; Yin, Ya-Xia; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2012CB932900,
   2009CB930400]; National Natural Science Foundation of China [91127044,
   21121063]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2011CB935700, 2012CB932900 and 2009CB930400), the National
   Natural Science Foundation of China (Grant Nos. 91127044 and 21121063),
   and the Chinese Academy of Sciences.
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Z9 150
U1 29
U2 240
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD SEP
PY 2012
VL 2
IS 9
BP 1086
EP 1090
DI 10.1002/aenm.201200158
PG 5
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 003SU
UT WOS:000308632400003
ER

PT J
AU Luo, B
   Fang, Y
   Wang, B
   Zhou, JS
   Song, HH
   Zhi, LJ
AF Luo, Bin
   Fang, Yan
   Wang, Bin
   Zhou, Jisheng
   Song, Huaihe
   Zhi, Linjie
TI Two dimensional graphene-SnS2 hybrids with superior rate capability for
   lithium ion storage
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID PERFORMANCE ANODE MATERIALS; PARTICLE-SIZE; BATTERIES; SNS2; NANOSHEETS;
   CAPACITY; SANDWICH; OXIDE; NANOPARTICLES; FABRICATION
AB A novel porous nanoarchitecture composed of 2D graphene-SnS2 (G-SnS2) units is developed via a two-step approach in this work. The special structure endows the high-rate transportation of electrolyte ions and electrons throughout the electrode matrix, resulting in remarkable electrochemical performance when it was used as anode in lithium ion batteries.
C1 [Luo, Bin; Fang, Yan; Wang, Bin; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
   [Zhou, Jisheng; Song, Huaihe] Beijing Univ Chem Technol, State key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
RP Luo, B (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Luo, Bin/P-7836-2015
OI Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [20973044]; Ministry of
   Science and Technology of China [2009AA03Z328, 2009DPA41220]; Chinese
   Academy of Sciences [KJCX2-YW-H21]; Guangdong-CAS [2009B091300007]
FX Financial supported from the National Natural Science Foundation of
   China (Grant No. 20973044), the Ministry of Science and Technology of
   China (No. 2009AA03Z328 andNo. 2009DPA41220), the Chinese Academy of
   Sciences (No. KJCX2-YW-H21), and the Guangdong-CAS strategic cooperation
   Program (2009B091300007) is acknowledged.
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U1 50
U2 235
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD JAN
PY 2012
VL 5
IS 1
BP 5226
EP 5230
DI 10.1039/c1ee02800f
PG 5
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 875PX
UT WOS:000299046100009
ER

PT J
AU Lin, J
   Peng, ZW
   Xiang, CS
   Ruan, GD
   Yan, Z
   Natelson, D
   Tour, JM
AF Lin, Jian
   Peng, Zhiwei
   Xiang, Changsheng
   Ruan, Gedeng
   Yan, Zheng
   Natelson, Douglas
   Tour, James M.
TI Graphene Nanoribbon and Nanostructured SnO2 Composite Anodes for Lithium
   Ion Batteries
SO ACS NANO
LA English
DT Article
DE graphene nanoribbons; GNRs; SnO2; lithium ion batteries; capacity
ID RECHARGEABLE BATTERIES; NEGATIVE ELECTRODES; CARBON NANOTUBES;
   MESOPOROUS SNO2; C COMPOSITE; STORAGE; PERFORMANCE; CAPABILITY; GROWTH;
   BINDER
AB A composite made from graphene nanoribbons (GNRs) and tin oxide (SnO2) nanoparticles (NPs) is synthesized and used as the anode material for lithium ion batteries (LIBs). The conductive GNRs, prepared using sodium/potassium unzipping of multiwall carbon nanotubes, can boost the lithium storage performance of SnO2 NPs. The composite, as an anode material for LIBs, exhibits reversible capacities of over 1520 and 1130 mAh/g for the first discharge and charge, respectively, which is more than the theoretical capacity of SnO2. The reversible capacity retains similar to 825 mAh/g at a current density of 100 mA/g with a Coulombic efficiency of 98% after 50 cycles. Further, the composite shows good power performance with a reversible capacity of similar to 580 mAh/g at the current density of 2 A/g. The high capacity, good power performance and retention can be attributed to uniformly distributed SnO2 NPs along the high-aspect-ratio GNRs. The GNRs act as conductive additives that buffer the volume changes of SnO2 during cycling. This work provides a starting point for exploring the composites made from GNRs and other transition metal oxides for lithium storage applications.
C1 [Lin, Jian; Tour, James M.] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
   [Lin, Jian; Tour, James M.] Rice Univ, Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA.
   [Peng, Zhiwei; Xiang, Changsheng; Ruan, Gedeng; Yan, Zheng; Tour, James M.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
   [Natelson, Douglas] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA.
   [Natelson, Douglas] Rice Univ, Dept Elect & Comp Engn, Houston, TX 77005 USA.
   [Tour, James M.] Rice Univ, Dept Comp Sci, Houston, TX 77005 USA.
RP Natelson, D (reprint author), Rice Univ, Dept Phys & Astron, 6100 Main St, Houston, TX 77005 USA.
EM natelson@rice.edu; tour@rice.edu
RI LIN, JIAN/D-2235-2013; Ruan, Gedeng/G-8225-2014; Xiang,
   Changsheng/G-2046-2014
OI LIN, JIAN/0000-0002-4675-2529; Ruan, Gedeng/0000-0002-7530-8013; 
FU Boeing; AFOSR [FA9550-09-1-0581]; Sandia National Laboratory [1100745];
   AFOSR MURI [FA9550-12-1-0035]; ONR MURI program [00006766,
   N00014-09-1-1066]
FX Funding for this research was provided by Boeing, the AFOSR
   (FA9550-09-1-0581), Sandia National Laboratory (1100745), the AFOSR MURI
   (FA9550-12-1-0035) and the ONR MURI program (#00006766,
   N00014-09-1-1066).
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U1 64
U2 421
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUL
PY 2013
VL 7
IS 7
BP 6001
EP 6006
DI 10.1021/nn4016899
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 191MO
UT WOS:000322417400041
PM 23758123
ER

PT J
AU Chen, YJ
   Xiao, G
   Wang, TS
   Ouyang, QY
   Qi, LH
   Ma, Y
   Gao, P
   Zhu, CL
   Cao, MS
   Jin, HB
AF Chen, Yu-Jin
   Xiao, Gang
   Wang, Tie-Shi
   Ouyang, Qiu-Yun
   Qi, Li-Hong
   Ma, Yang
   Gao, Peng
   Zhu, Chun-Ling
   Cao, Mao-Sheng
   Jin, Hai-Bo
TI Porous Fe3O4/Carbon Core/Shell Nanorods: Synthesis and Electromagnetic
   Properties
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID LITHIUM-ION BATTERIES; MAGNETIC-RESONANCE DETECTION; CARBON NANOTUBES;
   MICROWAVE-ABSORPTION; FE3O4 NANOPARTICLES; ANODE MATERIAL; NANOCRYSTALS;
   GRAPHENE; CANCER; SPECTROSCOPY
AB The porous Fe3O4/carbon core/shell nanorods were fabricated via a three-step process. alpha-Fe2O3 nanorods were first obtained, and alpha-Fe2O3/carbon core/shell nanorods were subsequently fabricated using glucose as a carbon source by a hydrothermal method, in which the thickness of the carbon coating was about 3.5 nm. Fe3O4/carbon core/shell nanorods were synthesized after an annealing treatment of the product above under a mixture of Ar/H-2 flow. After the H-2 deoxidation process, the Fe3O4 core exhibited a character of porosity; the thickness of the carbon shell was decreased to about 2.5 nm, and its degree of graphitization was enhanced. The interesting core/shell nanostructures are ferromagnetic at room temperature, and the Verwey temperature was about 120 K. Electromagnetic properties of the core/shell nanorod-wax composite were investigated in detail. The maximum reflection loss was about -27.9 dB at 14.96 GHz for the composite with a thickness of 2.0 mm, and the absorption bandwidth with the reflection loss below -18 dB was up to 10.5 GHz for the absorber with the thickness of 2-5 mm. The excellent electromagnetic wave absorption properties of the porous Fe3O4/carbon core/shell nanorods were attributed to effective complementarities between the dielectric loss and the magnetic loss.
C1 [Chen, Yu-Jin; Xiao, Gang; Wang, Tie-Shi; Ouyang, Qiu-Yun; Qi, Li-Hong; Ma, Yang] Harbin Engn Univ, Coll Sci, Harbin 15001, Peoples R China.
   [Gao, Peng; Zhu, Chun-Ling] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 15001, Peoples R China.
   [Cao, Mao-Sheng; Jin, Hai-Bo] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
RP Chen, YJ (reprint author), Harbin Engn Univ, Coll Sci, Harbin 15001, Peoples R China.
EM chenyujin@hrbeu.edu.cn; gaopeng@hrbeu.edu.cn; zhuchunling@hrbeu.edu.cn
OI Cao, Mao-Sheng/0000-0001-6810-9422
FU National Natural Science Foundation of China [51072038, 21001035]; NECT;
   Outstanding Youth Foundation of Heilongjiang Province [JC201008];
   Natural Science Foundation of Heilongjiang Province, China [F200828,
   E200839]; Ministry of Science and Technology of China [2008DFR20420];
   Fundamental Research Funds for the Central Universities [HEUCFT1010,
   HEUCF20111127, HEUCF20111124, HEUCF101016]; Harbin Key Sci-tech Project
   [2010AA4BG004]
FX The authors acknowledge the support from the National Natural Science
   Foundation of China (Grants 51072038 and 21001035), NECT, Outstanding
   Youth Foundation of Heilongjiang Province (Grant JC201008), Natural
   Science Foundation of Heilongjiang Province, China (Grants F200828 and
   E200839), Project supported by the Ministry of Science and Technology of
   China (Grant 2008DFR20420), the Fundamental Research Funds for the
   Central Universities (Grants HEUCFT1010, HEUCF20111127, HEUCF20111124,
   and HEUCF101016), and also Harbin Key Sci-tech Project (Grant
   2010AA4BG004).
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NR 59
TC 145
Z9 145
U1 65
U2 331
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD JUL 21
PY 2011
VL 115
IS 28
BP 13603
EP 13608
DI 10.1021/jp202473y
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 794JQ
UT WOS:000292892600010
ER

PT J
AU Chang, K
   Chen, WX
AF Chang, Kun
   Chen, Weixiang
TI Single-layer MoS2/graphene dispersed in amorphous carbon: towards high
   electrochemical performances in rechargeable lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ANODE MATERIAL; HIGH-CAPACITY; EXFOLIATED MOS2; LI STORAGE; GRAPHENE;
   NANOPARTICLES; COMPOSITES; NANOSHEETS; OXIDE; WS2
AB Here we report a facile process to synthesize the novel nanocomposites comprised of single-layer MoS2, graphene and amorphous carbon (SL-MoS2/G@a-C) by a hydrothermal route employing sodium molybdate, sulfocarbamide, as-prepared graphene oxide and glucose as starting materials and then annealing in H-2/N-2 atmosphere at 800 degrees C. The samples were systematically investigated using X-ray diffraction, field emission scanning electron microscopy, and high-resolution transmission electron microscopy. It was demonstrated that the single-layer MoS2 and graphene in the composites dispersed highly uniformly in the amorphous carbon. The mechanism of the formation of SL-MoS2/G@a-C nanocomposites was investigated. It was found that the SL-MoS2/G@a-C nanocomposites exhibited very high reversible capacity with excellent cyclic stability and high-rate capability as anode materials of Li-ion batteries. Among three SL-MoS2/G@a-C samples, the SL-MoS2/G@a-C (1 : 1) nanocomposite delivered the largest reversible capacity (1116 mAh g(-1)) with negligible fading of the capacity after 250 cycles, and still retained a high specific capacity of 850 mAh g(-1) and good cyclic stability at a high current density of 1000 mA g(-1).
C1 [Chang, Kun; Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China.
EM weixiangchen@zju.edu.cn
RI Chang, Kun/I-1361-2012
FU Natural Science Foundation of China [21173190]; Zhejiang Provincial
   Natural Science Foundation of China [Y4100119]; Public Interest Program
   from the Zhejiang Provincial Science and Technology [2011C21024];
   Ministry of Science and Technology of China [2010CB635116]
FX This work was supported by the Natural Science Foundation of China
   (21173190), the Zhejiang Provincial Natural Science Foundation of China
   (Y4100119), the Public Interest Program from the Zhejiang Provincial
   Science and Technology (2011C21024) and 973 Fundamental Research Program
   from the Ministry of Science and Technology of China (2010CB635116).
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NR 47
TC 144
Z9 146
U1 43
U2 324
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 43
BP 17175
EP 17184
DI 10.1039/c1jm12942b
PG 10
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 837MG
UT WOS:000296207300023
ER

PT J
AU Li, XF
   Geng, DS
   Zhang, Y
   Meng, XB
   Li, RY
   Sun, XL
AF Li, Xifei
   Geng, Dongsheng
   Zhang, Yong
   Meng, Xiangbo
   Li, Ruying
   Sun, Xueliang
TI Superior cycle stability of nitrogen-doped graphene nanosheets as anodes
   for lithium ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Graphene; Nitrogen doping; Anode; Cycle stability; Lithium ion batteries
ID CARBON NANOTUBE BUNDLES; STORAGE; CAPACITY; ENERGY; REDUCTION; FILMS;
   OXIDE
AB The specific capacity of nitrogen-doped graphene nanosheet (N-GNS) evidently increases with charge/discharge cycles, exhibiting superior electrochemical performance. N-GNS presented a specific capacity of 684 mAh g(-1) in the 501st cycles while only 452 mAh g(-1) in the 100th cycle, accounting for higher cycling stability and larger specific capacity in comparison to a pristine graphene and a commercialized graphite anode. The obtained significant improvement is attributed to the incorporated nitrogen to graphene planes with a result of more structural defects during cycling. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Li, Xifei; Geng, Dongsheng; Zhang, Yong; Meng, Xiangbo; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Geng, Dongsheng/G-7124-2011; Li, Xifei/A-1966-2012; Sun, Andy
   (Xueliang)/I-4535-2013; Meng, Xiangbo/H-3264-2012; Sun,
   Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; Meng, Xiangbo/0000-0002-4631-7260; 
FU NSERC; SpringPower International; CRC Program; CFI; ORF; ERA; UWO
FX This research was supported by NSERC, SpringPower International, CRC
   Program, CFI, ORF, ERA and UWO. X. Li is grateful to the Ontario PDF
   Program.
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NR 30
TC 140
Z9 148
U1 18
U2 161
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD AUG
PY 2011
VL 13
IS 8
BP 822
EP 825
DI 10.1016/j.elecom.2011.05.012
PG 4
WC Electrochemistry
SC Electrochemistry
GA 816EU
UT WOS:000294582300020
ER

PT J
AU Xu, C
   Wang, X
   Yang, LC
   Wu, YP
AF Xu, Chao
   Wang, Xin
   Yang, Lichun
   Wu, Yuping
TI Fabrication of a graphene-cuprous oxide composite
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Graphene; Cu(2)O cubes; Adsorption; Reduction; Composite
ID EXFOLIATED GRAPHITE OXIDE; LITHIUM-ION BATTERIES; FUNCTIONALIZED
   GRAPHENE; POLYOL PROCESS; AQUEOUS DISPERSIONS; CU2O NANOPARTICLES;
   CARBON NANOTUBES; ORGANIC-SOLVENTS; ANODE MATERIAL; SHEETS
AB A composite of graphene-cuprous oxide (Cu(2)O) was prepared using copper acetate-adsorbed graphene oxide (GO) sheets as precursors. In this composite, in-situ formed Cu(2)O particles were derived from the adsorbed copper acetate which attached to graphene sheets and prevented the aggregation of the reduced graphene oxide sheets. The as-synthesized Cu(2)O crystals were cube-like particles distributed randomly on the sheets due to the template effect of GO, consequently forming a graphene-Cu(2)O cubes composite. A preliminary study on the electrochemical behavior of the graphene-Cu(2)O composite used as anode material for lithium ion batteries was carried out. (C) 2009 Elsevier Inc. All rights reserved.
C1 [Xu, Chao; Wang, Xin] Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Peoples R China.
   [Yang, Lichun; Wu, Yuping] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.
   [Yang, Lichun; Wu, Yuping] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
RP Wang, X (reprint author), Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Peoples R China.
EM wxin@public1.ptt.js.cn
RI Wu, Yuping/H-1593-2011; Yang, Lichun/J-9841-2015
OI Wu, Yuping/0000-0002-0833-1205; 
FU National Natural Science Foundation of China [10776014]; High Technology
   Foundation of Jiangsu Province [BG(2007)047]
FX Financial support from the National Natural Science Foundation of China
   (No. 10776014) and the High Technology Foundation of Jiangsu Province
   (No. BG(2007)047) is greatly appreciated.
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NR 39
TC 140
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U1 25
U2 159
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD SEP
PY 2009
VL 182
IS 9
BP 2486
EP 2490
DI 10.1016/j.jssc.2009.07.001
PG 5
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 557AD
UT WOS:000274638600022
ER

PT J
AU Wang, JZ
   Zhong, C
   Chou, SL
   Liu, HK
AF Wang, Jia-Zhao
   Zhong, Chao
   Chou, Shu-Lei
   Liu, Hua-Kun
TI Flexible free-standing graphene-silicon composite film for lithium-ion
   batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Graphene-silicon composite; Free-standing electrode; In-situ filtration
   method; Lithium-ion battery
ID CARBON NANOTUBE PAPER; ELECTROCHEMICAL PROPERTIES; ELECTRODES; STORAGE;
   LAYER; ANODE; OXIDE; SUPERCAPACITORS; NANOCOMPOSITE; PERFORMANCE
AB Flexible, free-standing, paper-like, graphene-silicon composite materials have been synthesized by a simple, one-step, in-situ filtration method. The Si nanoparticles are highly encapsulated in a graphene nanosheet matrix. The electrochemical results show that graphene-Si composite film has much higher discharge capacity beyond 100 cycles (708 mAh g(-1)) than that of the cell with pure graphene (304 mAh g(-1)). The graphene functions as a flexible mechanical support for strain release, offering an efficient electrically conducting channel, while the nanosized silicon provides the high capacity. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Wang, Jia-Zhao] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2519, Australia.
   Univ Wollongong, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2519, Australia.
RP Wang, JZ (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2519, Australia.
EM jiazhao@uow.edu.au
RI Chou, Shulei/D-9895-2011; Wang, Jiazhao/G-4972-2011; Liu,
   Hua/G-1349-2012
OI Chou, Shulei/0000-0003-1155-6082; Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP 0987805]
FX Financial support provided by the Australian Research Council (ARC)
   through a Discovery Project (DP 0987805) is gratefully acknowledged.
   Many thanks also go to Dr. Tania Silver for critical reading of the
   manuscript.
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NR 30
TC 139
Z9 142
U1 32
U2 248
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD NOV
PY 2010
VL 12
IS 11
BP 1467
EP 1470
DI 10.1016/j.elecom.2010.08.008
PG 4
WC Electrochemistry
SC Electrochemistry
GA 682FF
UT WOS:000284386100003
ER

PT J
AU Zhao, B
   Song, JS
   Liu, P
   Xu, WW
   Fang, T
   Jiao, Z
   Zhang, HJ
   Jiang, Y
AF Zhao, Bing
   Song, Jinsong
   Liu, Peng
   Xu, Weiwen
   Fang, Tao
   Jiao, Zheng
   Zhang, Haijiao
   Jiang, Yong
TI Monolayer graphene/NiO nanosheets with two-dimension structure for
   supercapacitors
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM ION BATTERIES; CARBON NANOTUBES; ELECTROCHEMICAL CAPACITORS;
   REVERSIBLE CAPACITY; ENERGY-STORAGE; ANODE MATERIAL; NICKEL-OXIDE;
   COMPOSITE; PERFORMANCE; ELECTRODES
AB In this paper, graphene oxide (GO) synthesized from the modified Hummer method is used directly to fabricate unique two-dimension graphene/NiO composite material. Nickel ions are adsorbed on both sides of GO based on self-assembly by the electrostatic interactions of two species, forming the monolayer graphene/NiO sheet. The as-prepared composite is characterized using X-ray diffraction (XRD), Raman, SEM, TEM, Energy Dispersive Spectrometer (EDS) analysis and nitrogen adsorption/desorption. The results demonstrate that the NiO nanoparticles (5-7 nm) is uniformly dispersed on the surface of graphene, which greatly increases the surface area of the composite (134.5 m(2) g(-1)). This two-dimensional structure enhances supercapacitive performance with a high specific capacitance of 525 F g(-1) at a current density of 200 mA g(-1). A capacity retention of 95.4% can be maintained after 1000 cycles, suggesting its promising potential in supercapacitors.
C1 [Zhao, Bing; Song, Jinsong; Liu, Peng; Xu, Weiwen; Fang, Tao; Jiao, Zheng; Zhang, Haijiao; Jiang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
RP Jiang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
EM jiangyong@shu.edu.cn
FU Shanghai Municipal Education Commission [10YZ03, 10YZ05]; Natural
   Science Foundation of Shanghai [09ZR1411800, 10ZR1411300]; Shanghai Key
   Laboratory of Green Chemistry and Chemical Processes (ECNU); Laboratory
   of Chemical Engineering (ECUST); Shanghai Leading Academic Discipline
   Project [S30109]
FX This work is supported by the Innovation Program of Shanghai Municipal
   Education Commission (10YZ03 and 10YZ05), Natural Science Foundation of
   Shanghai (09ZR1411800 and 10ZR1411300), Shanghai Key Laboratory of Green
   Chemistry and Chemical Processes (ECNU), Laboratory of Chemical
   Engineering (ECUST), and Shanghai Leading Academic Discipline Project
   (No. S30109).
CR Cheng MY, 2010, J POWER SOURCES, V195, P4977, DOI 10.1016/j.jpowsour.2010.02.059
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NR 34
TC 136
Z9 137
U1 27
U2 131
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 46
BP 18792
EP 18798
DI 10.1039/c1jm13016a
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 848RR
UT WOS:000297072000043
ER

PT J
AU Zhang, KJ
   Han, PX
   Gu, L
   Zhang, LX
   Liu, ZH
   Kong, QS
   Zhang, CJ
   Dong, SM
   Zhang, ZY
   Yao, JH
   Xu, HX
   Cui, GL
   Chen, LQ
AF Zhang, Kejun
   Han, Pengxian
   Gu, Lin
   Zhang, Lixue
   Liu, Zhihong
   Kong, Qingshan
   Zhang, Chuanjian
   Dong, Shanmu
   Zhang, Zhongyi
   Yao, Jianhua
   Xu, Hongxia
   Cui, Guanglei
   Chen, Liquan
TI Synthesis of Nitrogen-Doped MnO/Graphene Nanosheets Hybrid Material for
   Lithium Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE nitrogen-doped MnO; nitrogen-doped graphene nanosheets; surface defects;
   anode material; lithium ion batteries
ID ANODE MATERIAL; OXIDE NANOPARTICLES; VANADIUM NITRIDE; GRAPHENE;
   STORAGE; CARBON; LI; ELECTRODES; CAPACITY; FABRICATION
AB Nitrogen-doped MnO/graphene nanosheets (N-MnO/GNS) hybrid material was synthesized by a simple. hydrothermal method followed by ammonia annealing. The samples were systematically investigated by X-ray diffraction analysis, Raman spectroscopy, X-ray photoelectron spectroscopy, transmission electron microscopy, and atomic force microscopy. N-doped MnO (N-MnO) nanoparticles were homogenously anchored on the thin layers of N-doped GNS (N-GNS) to form an efficient electronic/ionic mixed conducting network. This nanostructured hybrid exhibited a reversible electrochemical lithium storage capacity as high as 772 mAh g(-1) at 100 mA g(-1) after 90 cycles, and an excellent rate capability of 202 mA h g(-1) at a high current density of 5 A g(-1). It is expected that N-MnO/GNS hybrid could be a promising candidate material as a high capacity. anode for lithium ion batteries.
C1 [Zhang, Kejun; Han, Pengxian; Zhang, Lixue; Liu, Zhihong; Kong, Qingshan; Zhang, Chuanjian; Dong, Shanmu; Zhang, Zhongyi; Yao, Jianhua; Xu, Hongxia; Cui, Guanglei; Chen, Liquan] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
   [Gu, Lin; Chen, Liquan] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China.
RP Cui, GL (reprint author), Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
EM cuigl@qibebt.ac.cn
RI Zhang, Lixue/G-2721-2010; zheng, yonghong/H-3700-2012; Cui,
   Guanglei/D-4816-2011; Han, Pengxian/D-6159-2011; Gu, Lin/D-9631-2011
OI Gu, Lin/0000-0002-7504-031X
FU Chinese Academy of Sciences; National Program on Key Basic Research
   Project of China (973 Program) [MOST2011CB935700]; Shandong Province
   Fund for Distinguished Young Scientist [BS2009NJ013]; National Natural
   Science Foundation of China [20971077]
FX We appreciate the support of "100 Talents" program of the Chinese
   Academy of Sciences, National Program on Key Basic Research Project of
   China (973 Program) (MOST2011CB935700), Shandong Province Fund for
   Distinguished Young Scientist (BS2009NJ013), and National Natural
   Science Foundation of China (Grant 20971077).
CR Wehling TO, 2008, NANO LETT, V8, P173, DOI [10.1021/nl072364w, 10.1021/nL072364w]
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NR 41
TC 135
Z9 135
U1 31
U2 202
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD FEB
PY 2012
VL 4
IS 2
BP 658
EP 664
DI 10.1021/am201173z
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 897IW
UT WOS:000300644500024
PM 22211424
ER

PT J
AU Wang, B
   Li, XL
   Zhang, XF
   Luo, B
   Jin, MH
   Liang, MH
   Dayeh, SA
   Picraux, ST
   Zhi, LJ
AF Wang, Bin
   Li, Xianglong
   Zhang, Xianfeng
   Luo, Bin
   Jin, Meihua
   Liang, Minghui
   Dayeh, Shadi A.
   Picraux, S. T.
   Zhi, Linjie
TI Adaptable Silicon-Carbon Nanocables Sandwiched between Reduced Graphene
   Oxide Sheets as Lithium Ion Battery Anodes
SO ACS NANO
LA English
DT Article
DE silicon nanowire; graphene; adapting; lithium ion battery
ID NANOSTRUCTURED SILICON; CRYSTALLINE SILICON; NANOWIRE ANODES;
   LITHIATION; CAPACITY; NANOCOMPOSITES; NANOPARTICLES; INSERTION;
   FRACTURE; STORAGE
AB Silicon has been touted as one of the most promising anode materials for next generation lithium ion batteries. Yet, how to build energetic silicon-based electrode architectures by addressing the structural and interfacial stability issues facing silicon anodes still remains a big challenge. Here, we develop a novel kind of self-supporting binder-free silicon-based anodes via the encapsulation of silicon nanowires (SiNWs) with dual adaptable apparels (overlapped graphene (G) sheaths and reduced graphene oxide (RGO) overcoats). In the resulted architecture (namely, SiNW@G@RGO), the overlapped graphene sheets, as adaptable but sealed sheaths, prevent the direct exposure of encapsulated silicon to the electrolyte and enable the structural and interfacial stabilization of silicon nanowires. Meanwhile, the flexible and conductive RGO overcoats accommodate the volume change of embedded SiNW@G nanocables and thus maintain the structural and electrical integrity of the SiNW@G@RGO. As a result, the SiNW@G@RGO electrodes exhibit high reversible specific capacity of 1600 mAh g(-1) at 2.1 A g(-1), 80% capacity retention after 100 cycles, and superior rate capability (500 mAh g(-1) at 8.4 A g(-1)) on the basis of the total electrode weight.
C1 [Wang, Bin; Li, Xianglong; Zhang, Xianfeng; Luo, Bin; Jin, Meihua; Liang, Minghui; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
   [Dayeh, Shadi A.] Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92093 USA.
   [Picraux, S. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
RP Li, XL (reprint author), Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
EM lixl@nanoctr.cn; zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [20973044, 21173057,
   21273054]; Ministry of Science and Technology of China [2012CB933400,
   2012CB933403]; Chinese Academy of Sciences; Beijing Municipal Science
   and Technology Commission; Nanostructures for Electrical Energy Storage,
   an Energy Frontier Research Center; U.S. Department of Energy, Office of
   Science, Office of Basic Energy Sciences [DESC0001160]
FX Financial support from the National Natural Science Foundation of China
   (Grant Nos. 20973044, 21173057, 21273054), the Ministry of Science and
   Technology of China (No. 2012CB933400 and No. 2012CB933403), the Chinese
   Academy of Sciences, and Beijing Municipal Science and Technology
   Commission is acknowledged. S.T.P. also acknowledges support from
   Nanostructures for Electrical Energy Storage, an Energy Frontier
   Research Center funded by the U.S. Department of Energy, Office of
   Science, Office of Basic Energy Sciences under Award Number DESC0001160.
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NR 47
TC 134
Z9 137
U1 49
U2 451
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD FEB
PY 2013
VL 7
IS 2
BP 1437
EP 1445
DI 10.1021/nn3052023
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 099KA
UT WOS:000315618700063
PM 23281801
ER

PT J
AU Abouimrane, A
   Compton, OC
   Amine, K
   Nguyen, ST
AF Abouimrane, Ali
   Compton, Owen C.
   Amine, Khalil
   Nguyen, SonBinh T.
TI Non-Annealed Graphene Paper as a Binder-Free Anode for Lithium-Ion
   Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID EXFOLIATED GRAPHITE OXIDE; AQUEOUS DISPERSIONS; NANOSHEETS; FILMS;
   ELECTRODES; REDUCTION; STORAGE
AB Non-annealed graphene paper, prepared via reduction of prefabricated graphene oxide paper with hydrazine hydrate, was employed as the sole component of a binder-free lithium-ion battery anode, circumventing the polymer binders and other additives required for the fabrication of conventional electrodes. The binder-free anode fabricated from this non-annealed paper possessed excellent cyclability, while exhibiting a voltage versus capacity profile similar to that of a polymer-bound graphene powder anode. Kinetic barriers may exist for Li ion diffusion through the layered paper structure as decreasing the current rate from 50 to 10 mA.g(-1) increased the reversible capacity by over 150%.
C1 [Abouimrane, Ali; Amine, Khalil] Argonne Natl Lab, Mat Sci & Engn Div, Argonne, IL 60439 USA.
   [Compton, Owen C.; Nguyen, SonBinh T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
   [Compton, Owen C.; Nguyen, SonBinh T.] Northwestern Univ, Int Inst Nanotechnol, Evanston, IL 60208 USA.
RP Amine, K (reprint author), Argonne Natl Lab, Mat Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM amine@anl.gov; stn@northwestern.edu
RI Amine, Khalil/K-9344-2013; Nguyen, SonBinh/C-1682-2014
OI Nguyen, SonBinh/0000-0002-6977-3445
FU U.S. Department of Energy (FreedomCar, Vehicle Technology Office); NSF
   through the Materials Research Science and Engineering Center at
   Northwestern University [DMR-0520513]; ARO [W991NF-09-1-0541]; Argonne,
   a U.S. Department of Energy Office of Science laboratory
   [DE-AC02-06CH11357];  [CHE-0936924]
FX This work was supported by the U.S. Department of Energy (FreedomCar,
   Vehicle Technology Office), the NSF (Award No. DMR-0520513 through the
   Materials Research Science and Engineering Center at Northwestern
   University), and ARO (Award No. W991NF-09-1-0541). O.C.C. is an NSF-ACC
   fellow (Award No. CHE-0936924). We thank Prof. Mark Ratner for helpful
   discussions. The authors also thank UChicago Argonne, LLC, Operator of
   Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of
   Energy Office of Science laboratory, is operated under Contract No.
   DE-AC02-06CH11357.
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NR 24
TC 134
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U2 101
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD JUL 29
PY 2010
VL 114
IS 29
BP 12800
EP 12804
DI 10.1021/jp103704y
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 627VE
UT WOS:000280070900058
ER

PT J
AU Wang, ZL
   Xu, D
   Wang, HG
   Wu, Z
   Zhang, XB
AF Wang, Zhong-Li
   Xu, Dan
   Wang, Heng-Guo
   Wu, Zhong
   Zhang, Xin-Bo
TI In Situ Fabrication of Porous Graphene Electrodes for High-Performance
   Energy Storage
SO ACS NANO
LA English
DT Article
DE energy storage high power; in situ synthesis; synergistic effect;
   graphene
ID LITHIUM-ION BATTERIES; NITROGEN-DOPED GRAPHENE; HOLLOW CARBON
   NANOSPHERES; HIGH-RATE CAPABILITY; PAPER ELECTRODES; ULTRAFAST-CHARGE;
   ANODE MATERIALS; LI STORAGE; CAPACITY; OXIDE
AB In the development of energy-storage devices, simultaneously achieving high power and large energy capacity at fast rate is still a great challenge. In this paper, the synergistic effect of structure and doping in the graphene is demonstrated for high-performance lithium storage with ulftrafast and long-cycling capabilities. By an in situ constructing strategy, hierarchically porous structure, highly conductive network, and heteroatom doping are ideally combined in one graphene electrode. Compared to pristine graphene, it is found that the degree of improvement with both structure and doping effects is much larger than the sum of that with only structure effect or doping effect. Benefitting from the synergistic effect of structure and doping, the novel electrodes can deliver a high-power density of 116 kW kg(-1) while the energy density remains as high as 322 Wh kg(-1) at 80 A g(-1) (only 10 s to full charge), which provides an electrochemical storage level with the power density of a supercapacitor and the energy density of a battery, bridging the gap between them. Furthermore, the optimized electrodes exhibit long-cycling capability with nearly no capacity loss for 3000 cycles and wide temperature features with high capacities ranging from -20 to 55 degrees C.
C1 [Wang, Zhong-Li; Xu, Dan; Wang, Heng-Guo; Wu, Zhong; Zhang, Xin-Bo] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Wu, Zhong] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
RP Zhang, XB (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
EM xbzhang@clac.jl.cn
RI ZHANG, Xinbo/G-8698-2011
OI ZHANG, Xinbo/0000-0002-5806-159X
FU The Chinese Academy of Sciences; Foundation for Innovative Research
   Groups of the National Natural Science Foundation of China [20921002];
   National Natural Science Foundation of China [21101147, 21203176]
FX The authors greatly appreciated the editor and referees for their
   constructive comments and insightful suggestions on this manuscript.
   This work is financially supported by 100 Talents Programme of The
   Chinese Academy of Sciences, Foundation for Innovative Research Groups
   of the National Natural Science Foundation of China (Grant No. 20921002)
   and National Natural Science Foundation of China (Grant No. 21101147 and
   21203176).
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U2 579
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD MAR
PY 2013
VL 7
IS 3
BP 2422
EP 2430
DI 10.1021/nn3057388
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 115YB
UT WOS:000316846700060
PM 23383862
ER

PT J
AU Zhang, F
   Zhang, TF
   Yang, X
   Zhang, L
   Leng, K
   Huang, Y
   Chen, YS
AF Zhang, Fan
   Zhang, Tengfei
   Yang, Xi
   Zhang, Long
   Leng, Kai
   Huang, Yi
   Chen, Yongsheng
TI A high-performance supercapacitor-battery hybrid energy storage device
   based on graphene-enhanced electrode materials with ultrahigh energy
   density
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID LITHIUM-ION BATTERIES; ANODE MATERIALS; NANOCOMPOSITES; CAPACITORS;
   CATHODE; FILMS
AB In pursuing higher energy density with no sacrifice of power density, a supercapacitor-battery hybrid energy storage device-combining an electrochemical double layer capacitance (EDLC) type positive electrode with a Li-ion battery type negative electrode-has been designed and fabricated. Graphene is introduced to both electrodes: an Fe3O4/graphene (Fe3O4/G) nanocomposite with high specific capacity as negative electrode material, and a graphene-based three-dimensional porous carbon material (3DGraphene) with high surface area (similar to 3355 m(2) g(-1)) as positive electrode material. The Fe3O4/G nanocomposite shows a high reversible specific capacity exceeding 1000 mA h g(-1) at 90 mA g(-1) and remaining at 704 mA h g(-1) at 2700 mA g(-1), as well as excellent rate capability and improved cycle stability. Meanwhile the 3DGraphene positive electrode also displays great electrochemical performance. With these two graphene-enhanced electrode materials and using the best recommended industry evaluation method, the hybrid supercapacitor Fe3O4/G//3DGraphene demonstrates an ultrahigh energy density of 147 W h kg(-1) (power density of 150 W kg(-1)), which also remains of 86 W h kg(-1) even at high power density of 2587 W kg(-1), so far the highest value of the reported hybrid supercapacitors. Furthermore, the energy density of the hybrid supercapacitor is comparable to lithium ion batteries, and the power density also reaches that of symmetric supercapacitors, indicating that the hybrid supercapacitor could be a very promising novel energy storage system for fast and efficient energy storage in the future.
C1 [Zhang, Fan] Nankai Univ, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China.
   Nankai Univ, Ctr Nanoscale Sci & Technol, Inst Polymer Chem, Coll Chem, Tianjin 300071, Peoples R China.
RP Zhang, F (reprint author), Nankai Univ, Key Lab Funct Polymer Mat, Tianjin 300071, Peoples R China.
EM yschen99@nankai.edu.cn
RI Chen, Yongsheng/D-3256-2011; huang, yi/B-9867-2015
OI Chen, Yongsheng/0000-0003-1448-8177; 
FU MoST [2012CB933401, 2011DFB50300]; NSFC [50933003, 51273093]
FX The authors gratefully acknowledge financial support from MoST (Grants
   2012CB933401 and 2011DFB50300), NSFC (Grants 50933003 and 51273093).
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U1 83
U2 539
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD MAY
PY 2013
VL 6
IS 5
BP 1623
EP 1632
DI 10.1039/c3ee40509e
PG 10
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
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SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 131HX
UT WOS:000317984700029
ER

PT J
AU Zhu, JY
   He, JH
AF Zhu, Jiayi
   He, Junhui
TI Facile Synthesis of Graphene-Wrapped Honeycomb MnO2 Nanospheres and
   Their Application in Supercapacitors
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE monodisperse MnO2 nanospheres; graphene sheets; nanocomposites;
   electrostatic interaction; honeycomb-like "opened" structure;
   supercapacitors
ID MANGANESE OXIDE NANOSTRUCTURES; LITHIUM ION BATTERIES; ELECTROCHEMICAL
   CAPACITORS; FUNCTIONALIZED GRAPHENE; WATER-TREATMENT; ENERGY-STORAGE;
   ANODE MATERIAL; NANOSHEETS; POLY(O-PHENYLENEDIAMINE); NANOARCHITECTURES
AB Graphene-wrapped MnO2 nanocomposites were first fabricated by coassembly between honeycomb MnO2 nanospheres and graphene sheets via electrostatic interaction. The materials were characterized by means of X-ray diffraction, scanning electron microscopy, transmission electron microscopy, atomic force microscopy, and thermogravimetric analysis. The novel MnO2/graphene hybrid materials were used for investigation of electrochemical capacitive behaviors. The hybrid materials displayed enhanced capacitive performance (210 F/g at 0.5 A/g). Additionally, over 82.4% of the initial capacitance was retained after repeating the cyclic voltammetry test for 1000 cycles. The improved electrochemical performance might be attributed to the combination of the pesudocapacitance of MnO2 nanospheres with the honeycomb-like "opened" structure and good electrical conductivity of graphene sheets.
C1 [Zhu, Jiayi; He, Junhui] Chinese Acad Sci, Funct Nanomat Lab, Beijing 100190, Peoples R China.
   [Zhu, Jiayi; He, Junhui] Chinese Acad Sci, Key Lab Photochem Convers & Optoelect Mat, Beijing 100190, Peoples R China.
   [Zhu, Jiayi] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China.
RP He, JH (reprint author), Chinese Acad Sci, Funct Nanomat Lab, Zhongguancundonglu 29, Beijing 100190, Peoples R China.
EM jhhe@mail.ipc.ac.cn
FU National Natural Science Foundation of China [20871118]; Knowledge
   Innovation Program of Chinese Academy of Sciences (CAS)
   [timetinKGCX2-YW-370, KGCX2-EW-304-2]; Key Laboratory of Photochemical
   Conversion and Optoelectronic Materials, Technical Institute of Physics
   and Chemistry (TIPC), CAS
FX We thank Dr. X. Zhang and Prof. Y. W. Ma (Institute of Electrical
   Engineering, Chinese Academy of Sciences, Beijing, P. R. China) for
   helpful discussions. This work was supported by the National Natural
   Science Foundation of China (Grant 20871118) and the Knowledge
   Innovation Program of Chinese Academy of Sciences (CAS) (Grant
   timetinKGCX2-YW-370, KGCX2-EW-304-2). It was also partially supported by
   Key Laboratory of Photochemical Conversion and Optoelectronic Materials,
   Technical Institute of Physics and Chemistry (TIPC), CAS.
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NR 47
TC 130
Z9 133
U1 35
U2 212
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAR
PY 2012
VL 4
IS 3
BP 1770
EP 1776
DI 10.1021/am3000165
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 981BR
UT WOS:000306941000001
PM 22329919
ER

PT J
AU Xiang, HF
   Zhang, K
   Ji, G
   Lee, JY
   Zou, CJ
   Chen, XD
   Wu, JS
AF Xiang, Hongfa
   Zhang, Kai
   Ji, Ge
   Lee, Jim Yang
   Zou, Changji
   Chen, Xiaodong
   Wu, Jishan
TI Graphene/nanosized silicon composites for lithium battery anodes with
   improved cycling stability
SO CARBON
LA English
DT Article
ID GRAPHENE SHEETS; ION BATTERIES; SOLVOTHERMAL REDUCTION; EPITAXIAL
   GRAPHENE; HIGH-CAPACITY; LI STORAGE; ELECTRODES; GRAPHITE; FILMS;
   PERFORMANCE
AB Graphene/nanosized silicon composites were prepared and used for lithium battery anodes. Two types of graphene samples were used and their composites with nanosized silicon were prepared in different ways. In the first method, graphene oxide (GO) and nanosized silicon particles were homogeneously mixed in aqueous solution and then the dry samples were annealed at 500 degrees C to give thermally reduced GO and nanosized silicon composites. In the second method, the graphene sample was prepared by fast heat treatment of expandable graphite at 1050 degrees C and the graphene/nanosized silicon composites were then prepared by mechanical blending. In both cases, homogeneous composites were formed and the presence of graphene in the composites has been proved to effectively enhance the cycling stability of silicon anode in the lithium-ion batteries. The significant enhancement on cycling stability could be ascribed to the high conductivity of the graphene materials and absorption of volume changes of silicon by graphene sheets during the lithiadon/delithiation process. In particular, the composites using thermally expanded graphite exhibited not only more excellent cycling performance, but also higher specific capacity of 2753 mAh/g because the graphene sheets prepared by this method have fewer structural defects than thermally reduced GO. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Xiang, Hongfa; Zhang, Kai; Wu, Jishan] Natl Univ Singapore, Dept Chem, Singapore 117543, Singapore.
   [Ji, Ge; Lee, Jim Yang] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 117576, Singapore.
   [Zou, Changji; Chen, Xiaodong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
RP Wu, JS (reprint author), Natl Univ Singapore, Dept Chem, 3 Sci Dr 3, Singapore 117543, Singapore.
EM chmwuj@nus.edu.sg
RI Chen, Xiaodong/A-4537-2009; LEE, Jim Yang/E-5904-2010; Wu,
   Jishan/J-5898-2013; 
OI Chen, Xiaodong/0000-0002-3312-1664; Wu, Jishan/0000-0002-8231-0437;
   Xiang, Hongfa/0000-0002-6182-1932
FU A*Star SERC [R-143-000-401-305]
FX This work was financially supported by A*Star SERC Thematic Strategic
   Research Programme - Sustainable Materials: Composites & Lightweights
   (R-143-000-401-305).
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NR 43
TC 129
Z9 135
U1 23
U2 189
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD APR
PY 2011
VL 49
IS 5
BP 1787
EP 1796
DI 10.1016/j.carbon.2011.01.002
PG 10
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 729MA
UT WOS:000287952700033
ER

PT J
AU Zhu, JX
   Yang, D
   Yin, ZY
   Yan, QY
   Zhang, H
AF Zhu, Jixin
   Yang, Dan
   Yin, Zongyou
   Yan, Qingyu
   Zhang, Hua
TI Graphene and Graphene-Based Materials for Energy Storage Applications
SO SMALL
LA English
DT Review
ID LITHIUM-ION BATTERIES; NITROGEN-DOPED GRAPHENE; HIGH-PERFORMANCE ANODE;
   LI-S BATTERIES; THERMAL INTERFACE MATERIALS; SULFUR BATTERIES;
   ELECTROCHEMICAL CAPACITORS; CATHODE MATERIAL; AIR BATTERIES;
   MICRO-SUPERCAPACITORS
AB With the increased demand in energy resources, great efforts have been devoted to developing advanced energy storage and conversion systems. Graphene and graphene-based materials have attracted great attention owing to their unique properties of high mechanical flexibility, large surface area, chemical stability, superior electric and thermal conductivities that render them great choices as alternative electrode materials for electrochemical energy storage systems. This Review summarizes the recent progress in graphene and graphene-based materials for four energy storage systems, i.e., lithium-ion batteries, supercapacitors, lithium-sulfur batteries and lithium-air batteries.
C1 [Zhu, Jixin; Yang, Dan; Yin, Zongyou; Yan, Qingyu; Zhang, Hua] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Zhu, Jixin; Yang, Dan; Yan, Qingyu] TUM CREATE, Singapore 138602, Singapore.
RP Yan, QY (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM AlexYan@ntu.edu.sg; hzhang@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; zhu, Jixin/F-8763-2011; Zhang, Hua/A-1302-2009
FU Singapore A*STAR SERC [1021700144]; Singapore MPA [23/04.15.03];
   Singapore National Research Foundation under CREATE; MOE in Singapore
   [ARC 26/13, MOE2013-T2-1-034, RG 61/12, RGT18/13, M4080865.070.706022];
   Singapore National Research Foundation; Campus for Research Excellence
   And Technological Enterprise (CREATE) programme (Nanomaterials for
   Energy and Water Management)
FX Dr. Jixin Zhu, Dan Yang contributed equally to this work. This work was
   financially supported Singapore A*STAR SERC grant 1021700144 and
   Singapore MPA 23/04.15.03 grant, and Singapore National Research
   Foundation under CREATE program: EMobility in Megacities. This work was
   also supported by MOE under AcRF Tier 2 (ARC 26/13, No.
   MOE2013-T2-1-034), AcRF Tier 1 (RG 61/12, RGT18/13) and Start-Up Grant
   (M4080865.070.706022) in Singapore. This research is also funded by the
   Singapore National Research Foundation and the publication is supported
   under the Campus for Research Excellence And Technological Enterprise
   (CREATE) programme (Nanomaterials for Energy and Water Management).
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NR 157
TC 127
Z9 129
U1 155
U2 746
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD SEP 10
PY 2014
VL 10
IS 17
SI SI
BP 3480
EP 3498
DI 10.1002/smll.201303202
PG 19
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AO9XJ
UT WOS:000341713500005
PM 24431122
ER

PT J
AU Zhou, WW
   Zhu, JX
   Cheng, CW
   Liu, JP
   Yang, HP
   Cong, CX
   Guan, C
   Jia, XT
   Fan, HJ
   Yan, QY
   Li, CM
   Yu, T
AF Zhou, Weiwei
   Zhu, Jixin
   Cheng, Chuanwei
   Liu, Jinping
   Yang, Huanping
   Cong, Chunxiao
   Guan, Cao
   Jia, Xingtao
   Fan, Hong Jin
   Yan, Qingyu
   Li, Chang Ming
   Yu, Ting
TI A general strategy toward graphene@metal oxide core-shell nanostructures
   for high-performance lithium storage
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID ION BATTERIES; ANODE MATERIAL; ELECTROCHEMICAL CAPACITORS;
   FIELD-EMISSION; COMPOSITE; SHEETS; FILMS; NANOCOMPOSITES; NANOPARTICLES;
   FABRICATION
AB We demonstrate a simple, efficient, yet versatile method for the realization of core-shell assembly of graphene around various metal oxide (MO) nanostructures, including nanowires (NWs) and nanoparticles (NPs). The process is driven by (i) the ring-opening reaction between the epoxy groups and amine groups in graphene oxide (GO) platelets and amine-modified MO nanostructures, respectively, and (ii) electrostatic interaction between these two components. Nearly every single NW or NP is observed to be wrapped by graphene. To the best of our knowledge, this is the first report that substrate-supported MO NWs are fully coated with a graphene shell. As an example of the functional properties of these compound materials, the graphene@alpha-Fe(2)O(3) core shell NPs are investigated as the lithium-ion battery (LIB) electrode, which show a high reversible capacity, improved cycling stability, and excellent rate capability with respect to the pristine alpha-Fe(2)O(3). The superior performance of the composite electrode is presumably attributed to the effectiveness of the graphene shell in preventing the aggregation, buffering the volume change, maintaining the integrity of NPs, as well as improving the conductivity of the electrode.
C1 [Zhou, Weiwei; Cheng, Chuanwei; Liu, Jinping; Yang, Huanping; Cong, Chunxiao; Guan, Cao; Jia, Xingtao; Fan, Hong Jin; Yu, Ting] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
   [Zhu, Jixin; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Liu, Jinping] Cent China Normal Univ, Dept Phys, Inst Nanosci & Nanotechnol, Wuhan 430079, Peoples R China.
   [Li, Chang Ming] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637457, Singapore.
   [Yu, Ting] Natl Univ Singapore, Fac Sci, Dept Phys, Singapore 117542, Singapore.
RP Zhou, WW (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link, Singapore 637371, Singapore.
EM yuting@ntu.edu.sg
RI zhu, Jixin/F-8763-2011; Yan , Qingyu/A-2237-2011; Liu,
   Jinping/A-9285-2008; Fan, Hongjin/A-2662-2010; guan, cao/M-4391-2013;
   Cheng, Chuanwei/C-8646-2009; 
OI Fan, Hongjin/0000-0003-1237-4555; cong, chunxiao/0000-0001-9786-825X;
   Yu, Ting/0000-0002-0113-2895
FU Singapore National Research Foundation [NRF-RF2010-07]; MOE Tier 2 [MOE
   2009-T2-1-037]
FX This work is supported by the Singapore National Research Foundation
   under NRF RF Award No. NRF-RF2010-07 and MOE Tier 2 MOE 2009-T2-1-037.
CR Hwang JO, 2011, J MATER CHEM, V21, P3432, DOI 10.1039/c0jm01495h
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NR 47
TC 127
Z9 128
U1 34
U2 201
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD DEC
PY 2011
VL 4
IS 12
BP 4954
EP 4961
DI 10.1039/c1ee02168k
PG 8
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 855KF
UT WOS:000297562300020
ER

PT J
AU Zhu, N
   Liu, W
   Xue, MQ
   Xie, ZA
   Zhao, D
   Zhang, MN
   Chen, JT
   Cao, TB
AF Zhu, Nan
   Liu, Wen
   Xue, Mianqi
   Xie, Zhuang
   Zhao, Dan
   Zhang, Meining
   Chen, Jitao
   Cao, Tingbing
TI Graphene as a conductive additive to enhance the high-rate capabilities
   of electrospun Li4Ti5O12 for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Electrospinning; Graphene; Lithium-ion battery; High-rate
   charging/discharging
ID EXFOLIATED GRAPHITE OXIDE; ANODE MATERIAL; NANOFIBERS; PERFORMANCE;
   FABRICATION; STORAGE; NANOPARTICLES; REDUCTION; NANOWIRES; INSERTION
AB Spinel Li4Ti5O12 (LTO) is a promising candidate anode material for Li-ion batteries due to its well-known zero-strain merits. To improve the electronic properties of spinel LTO. which are intrinsically poor, we processed the material into a nanosized architecture to shorten the distance for Li-ion and electron transport using the versatile electrospinning method. Graphene was chosen as an effective carbon coating to improve the surface conductivity of the nanocomposites. The as-prepared graphene-embedded LTO anode material showed improved discharging/charging and cycling properties, particularly at high rates, such as 22 C, which makes the nanocomposite an attractive anode material for applications in electric vehicles. (C) 2010 Elsevier Ltd. All rights reserved.
C1 [Liu, Wen; Chen, Jitao] Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, Beijing 100871, Peoples R China.
   [Zhu, Nan; Xue, Mianqi; Xie, Zhuang; Zhao, Dan; Zhang, Meining; Cao, Tingbing] Renmin Univ China, Dept Chem, Beijing 100872, Peoples R China.
RP Chen, JT (reprint author), Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, Beijing 100871, Peoples R China.
EM chenjitao@pku.edu.cn; tcao@chem.ruc.edu.cn
RI XIE, Zhuang/F-4236-2010; Chen, Jitao/G-2995-2011; ruc, chem/E-4160-2012;
   Xue, Mianqi/A-7647-2012
OI Chen, Jitao/0000-0002-2620-5587; 
FU NSF of China [20674096, 20733001, 50773092]
FX This research was supported by the NSF of China under grant nos.
   20674096, 20733001 and 50773092.
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NR 33
TC 126
Z9 134
U1 26
U2 243
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD AUG 1
PY 2010
VL 55
IS 20
BP 5813
EP 5818
DI 10.1016/j.electacta.2010.05.029
PG 6
WC Electrochemistry
SC Electrochemistry
GA 632KO
UT WOS:000280422800042
ER

PT J
AU Shi, Y
   Wen, L
   Li, F
   Cheng, HM
AF Shi, Ying
   Wen, Lei
   Li, Feng
   Cheng, Hui-Ming
TI Nanosized Li4Ti5O12/graphene hybrid materials with low polarization for
   high rate lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Lithium titanate; Graphene; High rate anode materials; Lithium-ion
   batteries
ID ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE; NANOCRYSTALLINE LI4TI5O12;
   REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; SPINEL LI4TI5O12; RATE
   CAPABILITY; GRAPHENE; COMPOSITE; INSERTION
AB We report a simple strategy to prepare a hybrid of lithium titanate (Li4Ti5O12, LTO) nanoparticles well-dispersed on electrical conductive graphene nanosheets as an anode material for high rate lithium ion batteries. Lithium ion transport is facilitated by making pure phase Li4Ti5O12 particles in a nanosize to shorten the ion transport path. Electron transport is improved by forming a conductive graphene network throughout the insulating Li4Ti5O12 nanoparticles. The charge transfer resistance at the particle/electrolyte interface is reduced from 53.9 Omega to 36.2 Omega and the peak currents measured by a cyclic voltammogram are increased at each scan rate. The difference between charge and discharge plateau potentials becomes much smaller at all discharge rates because of lowered polarization. With 5 wt.% graphene, the hybrid materials deliver a specific capacity of 122 mAh g(-1) even at a very high charge/discharge rate of 30C and exhibit an excellent cycling performance, with the first discharge capacity of 132.2 mAh g(-1) and less than 6% discharge capacity loss over 300 cycles at 20C. The outstanding electrochemical performance and acceptable initial columbic efficiency of the nano-Li4Ti5O12/graphene hybrid with 5 wt.% graphene make it a promising anode material for high rate lithium ion batteries. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Shi, Ying; Wen, Lei; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Li, Feng/C-9991-2010
FU Ministry of Science and Technology of China [2009AA03Z337]; National
   Science Foundation of China [50921004, 50632040]; Chinese Academy of
   Sciences [KJCX2-YW-231]
FX This work was supported by Ministry of Science and Technology of China
   (No. 2009AA03Z337), National Science Foundation of China (Nos. 50921004
   and 50632040), and Chinese Academy of Sciences (No. KJCX2-YW-231). The
   authors thank Dr. G. Liu and Mr. G.M. Zhou and Miss N. Li for helpful
   discussion and Dr. D.M. Tang for his help in TEM characterization.
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NR 34
TC 124
Z9 127
U1 22
U2 190
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD OCT 15
PY 2011
VL 196
IS 20
BP 8610
EP 8617
DI 10.1016/j.jpowsour.2011.06.002
PG 8
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 818GF
UT WOS:000294739000058
ER

PT J
AU Compton, OC
   Jain, B
   Dikin, DA
   Abouimrane, A
   Amine, K
   Nguyen, ST
AF Compton, Owen C.
   Jain, Bonny
   Dikin, Dmitriy A.
   Abouimrane, Ali
   Amine, Khalil
   Nguyen, SonBinh T.
TI Chemically Active Reduced Graphene Oxide with Tunable C/O Ratios
SO ACS NANO
LA English
DT Article
DE graphene; graphene oxide; surface functionalization; thermal reduction;
   lithium-ion battery
ID EXFOLIATED GRAPHITE OXIDE; LITHIUM-ION BATTERIES; FUNCTIONALIZED
   GRAPHENE; AQUEOUS DISPERSIONS; VITAMIN-C; REDUCTION; PAPER; SHEETS;
   NANOSHEETS; NANOPLATELETS
AB Organic dispersions of graphene oxide can be thermally reduced in polar organic solvents under reflux conditions to afford electrically conductive, chemically active reduced graphene oxide (CARGO) with tunable C/O ratios, dependent on the boiling point of the solvent. The reductions are achieved after only 1 h of reflux, and the corresponding C/O ratios do not change upon further thermal treatment. Hydroxyl and carboxyl groups can be removed when the reflux Is carried out above 155 degrees C, while epoxides are removable only when the temperature is higher than 200 degrees C. The increasing hydrophobic nature of CARGO, as its C/O ratio increases, Improves the dispersibility of the nanosheets In a polystyrene matrix, in contrast to the aggregates formed with CARGO having lower C/O ratios. The excellent processability of the obtained CARGO dispersions is demonstrated via freestanding CARGO papers that exhibit tunable electrical conductivity/chemical activity and can be used as lithium-ion battery anodes with enhanced Coulombic efficiency.
C1 [Compton, Owen C.; Jain, Bonny; Nguyen, SonBinh T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.
   [Compton, Owen C.; Abouimrane, Ali; Amine, Khalil; Nguyen, SonBinh T.] Argonne Natl Lab, Div Engn & Mat Sci, Argonne, IL 60439 USA.
   [Dikin, Dmitriy A.] Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA.
RP Nguyen, ST (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.
EM stn@northwestern.edu
RI Dikin, Dmitriy/B-7592-2009; Dikin, Dmitriy/A-1086-2010; Amine,
   Khalil/K-9344-2013; Dikin, Dmitriy/B-4649-2014; Nguyen,
   SonBinh/C-1682-2014
OI Dikin, Dmitriy/0000-0001-8100-4502; Nguyen, SonBinh/0000-0002-6977-3445
FU NSF [DMR-0520513]; Materials Research Science and Engineering Center at
   Northwestern University; ARO [W991NF-09-1-0541]; U.S. Department of
   Energy (FreedomCar, Vehicle Technology Office); NSF-ACC [CHE-0936924];
   U.S. Department of Energy Office of Science laboratory
   [DE-AC02-06CH11357]
FX This work was supported by the NSF (Award No. DMR-0520513 through the
   Materials Research Science and Engineering Center at Northwestern
   University), ARO (Award No. W991NF-09-1-0541), and the U.S. Department
   of Energy (FreedomCar, Vehicle Technology Office). O.C.C. is an NSF-ACC
   fellow (Award No. CHE-0936924). Argonne National Laboratory is a U.S.
   Department of Energy Office of Science laboratory operated under
   Contract No. DE-AC02-06CH11357. We thank the Initiative for
   Sustainability and Energy (ISEN) at Northwestern for funding the
   purchase of some of the equipments used in this work. We are grateful to
   the reviewers of this manuscript for their suggestions, which greatly
   strengthen the final paper.
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NR 56
TC 124
Z9 126
U1 26
U2 137
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUN
PY 2011
VL 5
IS 6
BP 4380
EP 4391
DI 10.1021/nn1030725
PG 12
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 783AZ
UT WOS:000292055200019
PM 21473647
ER

PT J
AU Zhou, JS
   Song, HH
   Ma, LL
   Chen, XH
AF Zhou, Jisheng
   Song, Huaihe
   Ma, Lulu
   Chen, Xiaohong
TI Magnetite/graphene nanosheet composites: interfacial interaction and its
   impact on the durable high-rate performance in lithium-ion batteries
SO RSC ADVANCES
LA English
DT Article
ID ANODE MATERIAL; CARBON NANOTUBES; ELECTROCHEMICAL PERFORMANCE; GRAPHENE
   OXIDE; FUNCTIONALIZED GRAPHENE; HOLLOW NANOPARTICLES; ARYLDIAZONIUM
   SALTS; CYCLING PERFORMANCE; IRON SURFACES; METAL
AB We explore in-depth the interfacial interaction between Fe(3)O(4) nanoparticles and graphene nanosheets as well as its impact on the electrochemical performance of Fe(3)O(4)/graphene anode materials for lithium-ion batteries. Fe(3)O(4)/graphene hybrid materials are prepared by direct pyrolysis of Fe(NO(3))(3)center dot 9H(2)O on graphene sheets. The interfacial interaction between Fe(3)O(4) and graphene nanosheets is investigated in detail by thermogravimetric and differential scanning calorimetry analysis, Raman spectrum, X-ray photoelectron energy spectrum and Fourier transform infrared spectroscopy. It was found that Fe(3)O(4) nanoparticles disperse homogeneously on graphene sheets, and form strong covalent bond interactions (Fe-O-C bond) with graphene basal plane. The strong covalent links ensure the high specific capacity and long-period cyclic stability of Fe(3)O(4)/graphene hybrid electrodes for lithium-ion batteries at high current density. The capacity keeps as high as 796 mAhg(-1) after 200 cycles without any fading in comparison with the first reversible capacity at the current density of 500 mAg(-1) (ca. 0.6 C). At 1 Ag(-1) (ca. 1.3 C), the reversible capacity attains ca. 550 mAhg(-1) and 97% of initial capacity is maintained after 300 cycles. This work reveals an important factor affecting the high-rate and cyclic stability of metal oxide anode, and provides an effective way to the design of new anode materials for lithium-ion batteries.
C1 [Zhou, Jisheng; Song, Huaihe; Ma, Lulu; Chen, Xiaohong] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Key Lab Carbon Fiber & Funct Polymers, Minist Educ, Beijing, Peoples R China.
   [Ma, Lulu] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
RP Zhou, JS (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Key Lab Carbon Fiber & Funct Polymers, Minist Educ, Beijing, Peoples R China.
EM songhh@mail.buct.edu.cn
FU National Natural Science Foundation of China [50572003, 50972004];
   Xinjiang Key Laboratory of Electronic Information Materials and Devices
   [XJYS0901-2010-03]; Foundation of Excellent Doctoral Dissertation of
   Beijing City [YB20081001001]
FX This work was supported by the National Natural Science Foundation of
   China (50572003 and 50972004), the Opening Project of Xinjiang Key
   Laboratory of Electronic Information Materials and Devices
   (XJYS0901-2010-03), and Foundation of Excellent Doctoral Dissertation of
   Beijing City (YB20081001001).
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NR 78
TC 123
Z9 124
U1 29
U2 126
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2011
VL 1
IS 5
BP 782
EP 791
DI 10.1039/c1ra00402f
PG 10
WC Chemistry, Multidisciplinary
SC Chemistry
GA 833GH
UT WOS:000295870100009
ER

PT J
AU Liu, XH
   Liu, Y
   Kushima, A
   Zhang, SL
   Zhu, T
   Li, J
   Huang, JY
AF Liu, Xiao Hua
   Liu, Yang
   Kushima, Akihiro
   Zhang, Sulin
   Zhu, Ting
   Li, Ju
   Huang, Jian Yu
TI In Situ TEM Experiments of Electrochemical Lithiation and Delithiation
   of Individual Nanostructures
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE lithium embrittlement; degradation; nanobatteries; coatings; anisotropy
ID LITHIUM-ION BATTERIES; WALLED CARBON NANOTUBES; TRANSMISSION
   ELECTRON-MICROSCOPY; LINI0.8CO0.2O2 CATHODE MATERIALS; LIQUID-METAL
   EMBRITTLEMENT; SOLID-STATE AMORPHIZATION; SIZE-DEPENDENT FRACTURE;
   ATOMIC LAYER DEPOSITION; FILM LICOO2 CATHODES; SECONDARY BATTERIES
AB Understanding the microscopic mechanisms of electrochemical reaction and material degradation is crucial for the rational design of high-performance lithium ion batteries (LIBs). A novel nanobattery assembly and testing platform inside a transmission electron microscope (TEM) has been designed, which allows a direct study of the structural evolution of individual nanowire or nanoparticle electrodes with near-atomic resolution in real time. In this review, recent progresses in the study of several important anode materials are summarized. The consistency between in situ and ex situ results is shown, thereby validating the new in situ testing paradigm. Comparisons between a variety of nanostructures lead to the conclusion that electrochemical reaction and mechanical degradation are material specific, size dependent, and geometrically and compositionally sensitive. For example, a highly anisotropic lithiation in Si is observed, in contrast to the nearly isotropic response in Ge. The Ge nanowires can develop a spongy network, a unique mechanism for mitigating the large volume changes during cycling. The Si nanoparticles show a critical size of similar to 150 nm below which fracture is averted during lithiation, and above which surface cracking, rather than central cracking, is observed. In carbonaceous nanomaterials, the lithiated multi-walled carbon nanotubes (MWCNTs) are drastically embrittled, while few-layer graphene nanoribbons remain mechanically robust after lithiation. This distinct contrast manifests a strong geometrical embrittlement effect as compared to a relatively weak chemical embrittlement effect. In oxide nanowires, discrete cracks in ZnO nanowires are generated near the lithiation reaction front, leading to leapfrog cracking, while a mobile dislocation cloud at the reaction front is observed in SnO2 nanowires. This contrast is corroborated by ab initio calculations that indicate a strong chemical embrittlement of ZnO, but not of SnO2, after a small amount of lithium insertion. In metallic nanowires such as Al, delithiation causes pulverization, and the product nanoparticles are held in place by the surface Li-Al-O glass tube, suggesting possible strategies for improving electrode cyclability by coatings. In addition, a new in situ chemical lithiation method is introduced for fast screening of battery materials by conventional TEM. Evidently, in situ nanobattery experiments inside TEM are a powerful approach for advancing the fundamental understanding of electrochemical reactions and materials degradation and therefore pave the way toward rational design of high-performance LIBs.
C1 [Zhu, Ting] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA.
   [Kushima, Akihiro; Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA.
   [Kushima, Akihiro; Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.
   [Zhang, Sulin] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16802 USA.
   [Liu, Xiao Hua; Liu, Yang; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA.
RP Zhu, T (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA.
EM ting.zhu@me.gatech.edu; liju@mit.edu; jhuang@sandia.gov
RI Li, Ju/A-2993-2008; Kushima, Akihiro/H-2347-2011; Liu, Yang/C-9576-2012;
   Zhu, Ting/A-2206-2009; Liu, Xiaohua/A-8752-2011; Zhang, Sulin
   /E-6457-2010
OI Li, Ju/0000-0002-7841-8058; Liu, Xiaohua/0000-0002-7300-7145; 
FU Laboratory Directed Research and Development (LDRD) project at Sandia
   National Laboratories (SNL); Nanostructures for Electrical Energy
   Storage (NEES), an Energy Frontier Research Center (EFRC); US Department
   of Energy, Office of Science, Office of Basic Energy Sciences
   [DESC0001160]; Sandia-Los Alamos Center for Integrated Nanotechnologies
   (CINT); US Department of Energy's National Nuclear Security
   Administration [DE-AC04-94AL85000]; NSF [CMMI-0900692, CMMI-0758554,
   1100205, DMR-1008104, DMR-1120901]; AFOSR [FA9550-08-1-0325]
FX X. H. Liu, Y. Liu, and A. Kushima contributed equally to this work.
   Portions of this work were supported by a Laboratory Directed Research
   and Development (LDRD) project at Sandia National Laboratories (SNL) and
   partly by Nanostructures for Electrical Energy Storage (NEES), an Energy
   Frontier Research Center (EFRC) funded by the US Department of Energy,
   Office of Science, Office of Basic Energy Sciences under Award Number
   DESC0001160. The LDRD supported the development and fabrication of
   platforms. The NEES center supported the development of TEM techniques.
   The Sandia-Los Alamos Center for Integrated Nanotechnologies (CINT)
   supported the TEM capability. Sandia National Laboratories is a
   multiprogram laboratory managed and operated by Sandia Corporation, a
   wholly owned subsidiary of Lockheed Martin Company, for the US
   Department of Energy's National Nuclear Security Administration under
   Contract DE-AC04-94AL85000. S. Zhang acknowledges support by NSF
   CMMI-0900692. T. Zhu acknowledges support by NSF CMMI-0758554 and
   1100205. A. Kushima and J. Li acknowledge the support of NSF DMR-1008104
   and DMR-1120901, and AFOSR FA9550-08-1-0325. We also would like to
   acknowledge the collaborative work with Li Zhong, Jiangwei Wang, Liqiang
   Zhang, Wentao Liang, Shan Huang, Jeong-Hyun Cho, Jinkyoung Yoo, Shadi A.
   Dayeh, S. Tom Picraux, Scott X. Mao, John Sullivan, Nicholas Hudak, and
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NR 150
TC 122
Z9 122
U1 79
U2 420
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD JUL
PY 2012
VL 2
IS 7
SI SI
BP 722
EP 741
DI 10.1002/aenm.201200024
PG 20
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 972WE
UT WOS:000306311100003
ER

PT J
AU Zhang, CF
   Peng, X
   Guo, ZP
   Cai, CB
   Chen, ZX
   Wexler, D
   Li, S
   Liu, HK
AF Zhang, Chaofeng
   Peng, Xing
   Guo, Zaiping
   Cai, Chuanbin
   Chen, Zhixin
   Wexler, David
   Li, Sean
   Liu, Huakun
TI Carbon-coated SnO2/graphene nanosheets as highly reversible anode
   materials for lithium ion batteries
SO CARBON
LA English
DT Article
ID STORAGE CAPACITY; SNO2; GRAPHENE; OXIDE; PERFORMANCE; COMPOSITE;
   ELECTRODE
AB A simple approach is reported to prepare carbon-coated SnO2 nanoparticle-graphene nanosheets (Gr-SnO2-C) as an anode material for lithium ion batteries. The material exhibits excellent electrochemical performance with high capacity and good cycling stability (757 mA h g(-1) after 150 cycles at 200 mA g(-1)). The likely contributing factors to the outstanding charge/discharge performance of Gr-SnO2-C could be related to the synergism between the excellent conductivity and large area of graphene, the nanosized particles of SnO2, and the effects of the coating layer of carbon, which could alleviate the effects of volume changes, keep the structure stable, and increase the conductivity. This work suggests a strategy to prepare carbon-coated graphene-metal oxide which could be used to improve the electrochemical performance of lithium ion batteries. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Zhang, Chaofeng; Guo, Zaiping; Liu, Huakun] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
   [Zhang, Chaofeng; Peng, Xing; Guo, Zaiping; Chen, Zhixin; Wexler, David] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2522, Australia.
   [Cai, Chuanbin] Shanghai Univ, Res Ctr Superconductors & Appl Technol, Dept Phys, Shanghai 200444, Peoples R China.
   [Li, Sean] Univ New S Wales, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia.
RP Guo, ZP (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM zguo@uow.edu.au
RI Li, Sean/E-8910-2010; Liu, Hua/G-1349-2012
OI Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP1094261]
FX Financial support provided by the Australian Research Council (ARC)
   through an ARC Discovery Project (DP1094261) is gratefully acknowledged.
   The authors would like to thank Mr. Zhongwei Wang, Dr. Guodong Du, and
   Dr. Peng Zhang for their help, and also thank Dr. T. Silver for critical
   reading of the manuscript.
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PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD APR
PY 2012
VL 50
IS 5
BP 1897
EP 1903
DI 10.1016/j.carbon.2011.12.040
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 910YU
UT WOS:000301685300023
ER

PT J
AU Yu, AP
   Park, HW
   Davies, A
   Higgins, DC
   Chen, ZW
   Xiao, XC
AF Yu, Aiping
   Park, Hey Woong
   Davies, Aaron
   Higgins, Drew C.
   Chen, Zhongwei
   Xiao, Xingcheng
TI Free-Standing Layer-By-Layer Hybrid Thin Film of Graphene-MnO2 Nanotube
   as Anode for Lithium Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID NEGATIVE-ELECTRODE MATERIALS; COBALT OXIDE COMPOSITES; REVERSIBLE
   CAPACITY; LI STORAGE; PERFORMANCE; REDUCTION
AB Free-standing layer-by-layer assembled hybrid graphene-MnO2 nanotube (NT) thin films were prepared by an ultrafiltration technique and studied as anodes for lithium ion batteries. Each thin layer of graphene provides not only conductive pathways accelerating a conversion reaction of MnO2 but also buffer layers to maintain electrical contact with MnO2 NT during lithium insertion/extraction. In addition, the unique structures of the thin film provide porous structures that enhance Li ion diffusion into the structure. The graphene-MnO2 NT films as anode present excellent cycle and rate capabilities with a reversible specific capacity based on electrode composite mass of 495 mAh/g at 100 mA/g after 40 cycles with various current rates from 100 to 1600 mA/g. On the contrary, graphene-free MnO2 NT electrodes demonstrate only 140 mAh/g at 80 mA/g after 10 cycles. Furthermore, at a high current rate of 1600 mA/g, the charge capacity of graphene-MnO2 NT film reached 208 mAh/g.
C1 [Yu, Aiping; Park, Hey Woong; Davies, Aaron; Chen, Zhongwei] Univ Waterloo, Dept Chem Engn, Waterloo, ON N2L 3G1, Canada.
   [Xiao, Xingcheng] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
RP Chen, ZW (reprint author), Univ Waterloo, Dept Chem Engn, 200 Univ Ave W, Waterloo, ON N2L 3G1, Canada.
EM zhwchen@uwaterloo.ca; xingcheng.xiao@gm.com
RI chen, zhongwei/A-5605-2015
FU Natural Sciences and Engineering Research Council of Canada (NSERC)
FX The University of Waterloo and the Natural Sciences and Engineering
   Research Council of Canada (NSERC) are gratefully acknowledged for their
   financial support for this work.
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NR 24
TC 122
Z9 124
U1 25
U2 181
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD AUG 4
PY 2011
VL 2
IS 15
BP 1855
EP 1860
DI 10.1021/jz200836h
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 801EL
UT WOS:000293419600003
ER

PT J
AU Xiao, XL
   Liu, XF
   Zhao, H
   Chen, DF
   Liu, FZ
   Xiang, JH
   Hu, ZB
   Li, YD
AF Xiao, Xiaoling
   Liu, Xiangfeng
   Zhao, Hu
   Chen, Dongfeng
   Liu, Fengzhen
   Xiang, Junhui
   Hu, Zhongbo
   Li, Yadong
TI Facile Shape Control of Co3O4 and the Effect of the Crystal Plane on
   Electrochemical Performance
SO ADVANCED MATERIALS
LA English
DT Article
DE Co3O4; crystal plane effect; electrochemical performance; electrodes;
   lithium ion batteries
ID LITHIUM-ION BATTERIES; REVERSIBLE CAPACITY; ELECTRODE MATERIALS;
   NANOWIRE ARRAYS; ANODE MATERIAL; STORAGE; GRAPHENE; NANOPARTICLES;
   CHALLENGES; NANOSHEETS
AB Co3O4 with three different crystal plane structures - cubes bounded by {001} planes, truncated octahedra enclosed by {111} and {001} planes, and octahedra with exposed {111} planes - is synthesized using a very simple one-step hydrothermal method. The three kinds of Co3O4 exhibit significantly different electrochemical performances and the effect of different exposed crystal planes on the electrochemical performance of Co3O4 is comprehensively studied.
C1 [Xiao, Xiaoling; Liu, Xiangfeng; Zhao, Hu; Liu, Fengzhen; Hu, Zhongbo] Chinese Acad Sci, Grad Univ, Coll Mat Sci & Optoelect Technol, Beijing 100049, Peoples R China.
   [Chen, Dongfeng] China Inst Atom Energy, Inst Nucl Phys, Beijing 102413, Peoples R China.
   [Xiang, Junhui] Chinese Acad Sci, Grad Univ, Coll Chem & Chem Engn, Beijing 100049, Peoples R China.
   [Li, Yadong] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
RP Xiao, XL (reprint author), Chinese Acad Sci, Grad Univ, Coll Mat Sci & Optoelect Technol, Beijing 100049, Peoples R China.
EM xlxiao@gucas.ac.cn; ydli@mail.tsinghua.edu.cn
FU State Key Project of Fundamental Research [2010CB833101, 2012CB932504];
   China Postdoctoral Science Foundation [20100480512]; Chinese Academy of
   Sciences
FX This work was supported by the State Key Project of Fundamental Research
   (2010CB833101 and 2012CB932504), the China Postdoctoral Science
   Foundation (20100480512), and the Chinese Academy of Sciences ("Hundred
   Talents Project"). Thanks go to Prof. K. B. Zhou of the Graduate
   University of the Chinese Academy of Sciences for helpful discussion.
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NR 40
TC 121
Z9 122
U1 62
U2 503
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD NOV 8
PY 2012
VL 24
IS 42
BP 5762
EP 5766
DI 10.1002/adma.201202271
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 030XA
UT WOS:000310602200016
PM 22911458
ER

PT J
AU Shah, MSAS
   Park, AR
   Zhang, K
   Park, JH
   Yoo, PJ
AF Shah, Md. Selim Arif Sher
   Park, A. Reum
   Zhang, Kan
   Park, Jong Hyeok
   Yoo, Pil J.
TI Green Synthesis of Biphasic TiO2-Reduced Graphene Oxide Nanocomposites
   with Highly Enhanced Photocatalytic Activity
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE titania; graphene; nanocomposites; green synthesis; hydrothermal;
   photocatalysis
ID GRAPHITE OXIDE; TIO2 NANOPARTICLES; TIO2-GRAPHENE NANOCOMPOSITES;
   COMPOSITE-MATERIALS; RAMAN-SPECTRA; SOLAR-CELLS; GAS-PHASE; SHEETS;
   NANOCRYSTALS; REDUCTION
AB A series of TiO2-reduced graphene oxide (RGO) nanocomposites were prepared by simple one-step hydrothermal reactions using the titania precursor, TiCl4 and graphene oxide (GO) without reducing agents. Hydrolysis of TiCl4 and mild reduction of GO were simultaneously carried Out under hydrothermal conditions. While conventional approaches mostly utilize multistep chemical methods wherein strong reducing agents, such as hydrazine, hydroquinone, and sodium borohydride are employed, our method provides the notable advantages of a single step reaction without employing toxic solvents or reducing agents, thereby providing a novel green synthetic route to produce the nanocomposites of RGO and TiO2. The as-synthesized nanocomposites were characterized by several crystallographic, microscopic, and spectroscopic characterization methods, which enabled confrimation of the robustness of the suggested reaction scheme. Notably, X-ray diffraction and transmission electron micrograph proved that TiO2 contained both anatase and rutile phase's. In addition, the photocatalytic activities of the synthesized composites were measured for the degradation of rhodamine B dye. The catalyst also can degrade a colorless dye such as benzoic acid under visible light. The synthesized nanocomposites of biphasic TiO2 with RGO showed enhanced catalytic activity compared to conventional TiO2 photocatalyst, P25. The photocatalytic activity is strongly affected by the concentration of RGO in the nanocomposites, with the best photocatalytic activity observed for the composite of 2.0 wt % RGO. Since the synthesized biphasic TiO2-RGO nanocomposites have been shown to effectively reduce the electron-hole recombination rate, it is anticipated that they will be utilized as anode materials in lithium ion batteries.
C1 [Shah, Md. Selim Arif Sher; Park, A. Reum; Park, Jong Hyeok; Yoo, Pil J.] Sungkyunkwan Univ, Sch Chem Engn, Suwon 440746, South Korea.
   [Zhang, Kan; Park, Jong Hyeok; Yoo, Pil J.] Sungkyunkwan Univ, SKKU Adv Inst Nanotechnol SAINT, Suwon 440746, South Korea.
RP Yoo, PJ (reprint author), Sungkyunkwan Univ, Sch Chem Engn, Suwon 440746, South Korea.
EM pjyoo@skku.edu
RI Park, Jong Hyeok/A-7778-2012; Yoo, Pil J./A-1069-2012
OI Park, Jong Hyeok/0000-0002-6629-3147; Yoo, Pil J./0000-0002-5499-6566
FU National Research Foundation of Korea (NRF) [2010-0009877,
   2010-0029409]; Korea Government (MEST);  [NRF-C1AAA001-2010-0028962]
FX This work was supported by research Grant NRF-C1AAA001-2010-0028962 and
   Basic Science Research Program Grants 2010-0009877, 2010-0029409 through
   the National Research Foundation of Korea (NRF) funded by the Korea
   Government (MEST).
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NR 60
TC 121
Z9 122
U1 40
U2 249
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD AUG
PY 2012
VL 4
IS 8
BP 3893
EP 3901
DI 10.1021/am301287m
PG 9
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 991JZ
UT WOS:000307698600019
ER

PT J
AU Fan, ZJ
   Yan, J
   Wei, T
   Ning, GQ
   Zhi, LJ
   Liu, JC
   Cao, DX
   Wang, GL
   Wei, F
AF Fan, Zhuang-Jun
   Yan, Jun
   Wei, Tong
   Ning, Guo-Qing
   Zhi, Lin-Jie
   Liu, Jin-Cheng
   Cao, Dian-Xue
   Wang, Gui-Ling
   Wei, Fei
TI Nanographene-Constructed Carbon Nanofibers Grown on Graphene Sheets by
   Chemical Vapor Deposition: High-Performance Anode Materials for Lithium
   Ion Batteries
SO ACS NANO
LA English
DT Article
DE graphene nanosheets; carbon nanofibers; lithium ion battery
ID ELECTROCHEMICAL ENERGY-STORAGE; HYBRID FILMS; MESOPHASE PITCH; GRAPHITE
   OXIDE; HIGH-CAPACITY; LI STORAGE; COMPOSITES; NANOTUBES; HOLLOW;
   ELECTRODES
AB We report on the fabrication of 3D carbonaceous material composed of 1D carbon nanofibers (CNF) grown on 2D graphene sheets (GNS) via a CVD approach in a fluidized bed reactor. Nanographene-constructed carbon nanofibers contain many cavities, open tips, and graphene platelets with edges exposed, providing more extra space for Li(+) storage. More interestingly, nanochannels consisting of graphene platelets arrange almost perpendicularly to the fiber axis, which is favorable for lithium Ion diffusion from different orientation In addition, 3D interconnected architectures facilitate the collection and transport of electrons during the cycling process. As a result, the CNF/GNS hybrid material shows high reversible capacity (667 mAh/g), high-rate performance, and cycling,stability, which is superior to those of purE graphene, natural graphite, and carbon nanotubes. The simple,CVD approach offers a new pathway for large-scale production of novel hybrid carbon materials for energy storage.
C1 [Fan, Zhuang-Jun; Yan, Jun; Wei, Tong; Liu, Jin-Cheng; Cao, Dian-Xue; Wang, Gui-Ling] Harbin Engn Univ, Minist Educ, Coll Mat Sci & Chem Engn, Key Lab Superlight Mat & Surface Technol, Harbin 150001, Peoples R China.
   [Ning, Guo-Qing] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China.
   [Zhi, Lin-Jie] Natl Ctr Nanosci & Technol China, Beijing 100190, Peoples R China.
   [Wei, Fei] Tsinghua Univ, Dept Chem Engn, Beijing Key Lab Green Chem React Engn & Technol, Beijing 100084, Peoples R China.
RP Fan, ZJ (reprint author), Harbin Engn Univ, Minist Educ, Coll Mat Sci & Chem Engn, Key Lab Superlight Mat & Surface Technol, Harbin 150001, Peoples R China.
EM fanzhj666@163.com; zhilj@nanoctr.cn; weifei@flotu.org
RI Wei, Fei/H-4674-2012; Wei, Fei/H-4809-2012; Yan, Jun/D-4360-2011
OI Yan, Jun/0000-0002-9967-3912
FU National Science Foundation of China [51077014, 21003028]; Fundamental
   Research Funds for the Central Universities [HEUCF101006]
FX The authors acknowledge financial support from the National Science
   Foundation of China (Nos. 51077014, 21003028) and Fundamental Research
   Funds for the Central Universities (HEUCF101006).
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NR 54
TC 120
Z9 122
U1 32
U2 180
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD APR
PY 2011
VL 5
IS 4
BP 2787
EP 2794
DI 10.1021/nn200195k
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 753CJ
UT WOS:000289742100043
PM 21425865
ER

PT J
AU Wu, DQ
   Zhang, F
   Liang, HW
   Feng, XL
AF Wu, Dongqing
   Zhang, Fan
   Liang, Haiwei
   Feng, Xinliang
TI Nanocomposites and macroscopic materials: assembly of chemically
   modified graphene sheets
SO CHEMICAL SOCIETY REVIEWS
LA English
DT Review
ID ONE-STEP SYNTHESIS; LITHIUM ION BATTERIES; REDUCED GRAPHENE;
   FUNCTIONALIZED GRAPHENE; COMPOSITE HYDROGELS; GOLD NANOPARTICLES; CARBON
   NANOTUBES; FULLERENE C-60; GRAPHITE OXIDE; ANODE MATERIAL
AB Self-assembly of chemically modified graphenes (CMGs), including graphene oxide (GO), reduced graphene oxide (RGO) and their derivatives, has emerged as one of the most appealing strategies to develop unprecedented graphene-based functional materials. With the assistance of various non-covalent forces such as hydrogen bonding, ionic, amphiphilic and pi-pi interactions, CMGs decorated with multiple functional groups are favorable for assembly with different organic and inorganic components which can result in hierarchical composites possessing unique structures and functions. In this review, we will summarize the state-of-the-art self-assembly strategies that have been established to construct CMG based nanomaterials, including nanoparticles, nanospheres, nanofibers, nanorods, nanosheets, and macroscopic thin films, fibers and porous networks. The driving forces involved in the self-assembly process will be elucidated in the context. Further, we will also highlight several representative examples of applications regarding the self-assembled CMG based materials.
C1 [Wu, Dongqing; Zhang, Fan; Liang, Haiwei; Feng, Xinliang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Liang, Haiwei; Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Feng, XL (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
EM feng@mpip-mainz.mpg.de
RI Liang, Hai-Wei/B-7292-2011
FU 973 Program of China [2012CB933404]; Natural Science Foundation of China
   [21174083, 21102091]; BASF; Shanghai Pujiang Program [11PJ1405400]; PhD
   Programs Foundation of Ministry of Education of China for Young Scholars
   [20110073120039]
FX This work was financially supported by 973 Program of China
   (2012CB933404), Natural Science Foundation of China (21174083 and
   21102091), BASF, Shanghai Pujiang Program (11PJ1405400), PhD Programs
   Foundation of Ministry of Education of China for Young Scholars
   (20110073120039).
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NR 229
TC 119
Z9 121
U1 80
U2 527
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0306-0012
J9 CHEM SOC REV
JI Chem. Soc. Rev.
PY 2012
VL 41
IS 18
BP 6160
EP 6177
DI 10.1039/c2cs35179j
PG 18
WC Chemistry, Multidisciplinary
SC Chemistry
GA 992MD
UT WOS:000307779600019
PM 22875044
ER

PT J
AU Zou, YQ
   Wang, Y
AF Zou, Yuqin
   Wang, Yong
TI Sn@CNT Nanostructures Rooted in Graphene with High and Fast Li-Storage
   Capacities
SO ACS NANO
LA English
DT Article
DE carbon nanotube; graphene; lithium ion batteries; Sn; SnS(2)
ID LITHIUM-ION BATTERIES; CARBON NANOTUBES; ANODE MATERIAL; NANOPARTICLES;
   COMPOSITE; PERFORMANCE; ELECTRODES; NANOSHEETS
AB Development of materials with carefully crafted nanostructures has been an important strategy for the next-generation lithium-Ion batteries to achieve higher capacity, longer cycle life, and better rate capability. Graphene-based and Sn-based anode materials are promising anodes with higher capacities than graphite; however, most of them exhibit fast capacity fading at prolonged cycling and poor rate capability. This paper reports a hierarchical Sn@CNT nanostructure rooted in graphene, which exhibits larger than theoretical reversible capacities of 1160-982 mAh/g in 100 cycles at 100 mA/g and excellent rate capability (828 mAh/g at 1000 mA/g and 594 mAh/g at 5000 mA/g). The excellent electrochemical performances compared to graphene/Sn-based anodes have been attributed to the efficient prevention of graphene agglomeration by Sn@CNT decoration and the increased electrochemical activities of Sn by CNT shell protection and GNS support.
C1 [Zou, Yuqin; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shanghai 200444, Peoples R China.
RP Wang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012
FU National Natural Science Foundation of China [50971085]; Shanghai
   Municipal Government [09JC140-6100, S30109]
FX The authors gratefully acknowledge the Instrumental and Analysis and
   Research Center, Shanghai University, for materials characterizations
   and the financial support from the Program for Professor of Special
   Appointment (Eastern Scholar), National Natural Science Foundation of
   China (50971085), and Shanghai Municipal Government (09JC140-6100,
   S30109).
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NR 38
TC 119
Z9 122
U1 23
U2 189
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD OCT
PY 2011
VL 5
IS 10
BP 8108
EP 8114
DI 10.1021/nn2027159
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 837MU
UT WOS:000296208700063
PM 21939228
ER

PT J
AU Yao, YJ
   Miao, SD
   Liu, SZ
   Ma, LP
   Sun, HQ
   Wang, SB
AF Yao, Yunjin
   Miao, Shiding
   Liu, Shizhen
   Ma, Li Ping
   Sun, Hongqi
   Wang, Shaobin
TI Synthesis, characterization, and adsorption properties of magnetic
   Fe3O4@graphene nanocomposite
SO CHEMICAL ENGINEERING JOURNAL
LA English
DT Article
DE Graphene; Adsorption; Magnetic nanoparticle; Dyes
ID LITHIUM-ION BATTERIES; METHYLENE-BLUE ADSORPTION; CONGO-RED; CO3O4
   NANOPARTICLES; CARBON NANOTUBES; POLYACRYLIC-ACID; ANODE MATERIAL;
   WASTE-WATER; DYE REMOVAL; EQUILIBRIUM
AB This paper reports the synthesis of magnetic Fe3O4@graphene composite (FGC) and utilization in dye removal from aqueous media. The structural, surface, and magnetic characteristics of the nanosized composite were investigated by field emission scanning electron microscopy, transmission electron microscopy, energy-dispersive X-ray spectrometer, powder X-ray diffraction, Fourier transform infrared, and thermogravimetric analysis. Through a chemical deposition method, Fe3O4 nanoparticles in size of 30 nm were homogeneously dispersed onto graphene sheets. Adsorption isotherm and kinetics of methylene blue (MB) and Congo red (CR) onto FGC were studied in a batch system. The maximum adsorption capacities of MB and CR on FGC were found to be 45.27 and 33.66 mg/g, respectively. The second-order kinetic equation could best describe the sorption kinetics. The findings of the present work highlight the facile fabrication of magnetic FGC and application in adsorption and separation. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Yao, Yunjin; Miao, Shiding] Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China.
   [Yao, Yunjin; Liu, Shizhen; Ma, Li Ping; Sun, Hongqi; Wang, Shaobin] Curtin Univ Technol, Dept Chem Engn, Perth, WA 6845, Australia.
RP Yao, YJ (reprint author), Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China.
EM yaoyunjin@gmail.com; shaobin.wang@curtin.edu.au
RI Wang, Shaobin/C-5507-2008; yao, yunjin/C-9615-2012
OI Wang, Shaobin/0000-0002-1751-9162; yao, yunjin/0000-0002-5462-4973
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NR 38
TC 118
Z9 124
U1 38
U2 246
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 1385-8947
J9 CHEM ENG J
JI Chem. Eng. J.
PD MAR 1
PY 2012
VL 184
BP 326
EP 332
DI 10.1016/j.cej.2011.12.017
PG 7
WC Engineering, Environmental; Engineering, Chemical
SC Engineering
GA 913WM
UT WOS:000301908100041
ER

PT J
AU Li, BJ
   Cao, HQ
   Shao, J
   Qu, MZ
AF Li, Baojun
   Cao, Huaqiang
   Shao, Jin
   Qu, Meizhen
TI Enhanced anode performances of the Fe3O4-Carbon-rGO three dimensional
   composite in lithium ion batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID HIGH-CAPACITY; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE;
   TIN-NANOPARTICLES; ELECTRODES; STORAGE; NANOWIRES; FABRICATION; SPHERES
AB A three dimensional composite was constructed by anchoring Fe3O4 nanoparticles encapsulated within carbon shells onto reduced graphene oxide sheets, which exhibited enhanced anode performances in lithium ion batteries with a specific capacity of 842.7 mAh g(-1) and superior recycle stability after 100 cycles.
C1 [Li, Baojun; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Shao, Jin; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]; China
   Postdoctoral Science Foundation [20100470302]
FX Financial support from the National Natural Science Foundation of China
   (No. 20921001 and 20535020), the Innovation Method Fund of China (No.
   20081885189), the National High Technology Research and Development
   Program of China (No. 2009AA03Z321), and the China Postdoctoral Science
   Foundation (No. 20100470302) is acknowledged.
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NR 41
TC 118
Z9 120
U1 13
U2 119
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PY 2011
VL 47
IS 37
BP 10374
EP 10376
DI 10.1039/c1cc13462k
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 815BH
UT WOS:000294500600054
PM 21847467
ER

PT J
AU Zhang, M
   Lei, D
   Du, ZF
   Yin, XM
   Chen, LB
   Li, QH
   Wang, YG
   Wang, TH
AF Zhang, Ming
   Lei, Danni
   Du, Zhifeng
   Yin, Xiaoming
   Chen, Libao
   Li, Qiuhong
   Wang, Yangguo
   Wang, Taihong
TI Fast synthesis of SnO2/graphene composites by reducing graphene oxide
   with stannous ions
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ELECTROCHEMICAL PROPERTIES; LITHIUM STORAGE; ANODE MATERIAL; SHEETS;
   PERFORMANCE; HYBRID; ELECTRODES; NANOSHEETS; BATTERIES; CAPACITY
AB This article propounds a new strategy of preparing graphene by reducing GO with stannous ions for the synthesis of SnO2/graphene composites. As anode materials for lithium ion batteries, the composites showed good performance. This opens a new approach for the synthesis of graphene/metal-oxide composites with excellent properties.
C1 [Zhang, Ming; Lei, Danni; Du, Zhifeng; Yin, Xiaoming; Chen, Libao; Li, Qiuhong; Wang, Yangguo; Wang, Taihong] Hunan Univ, Minist Educ, Key Lab Micronano Optoelectron Devices, State Key Lab Chemobiosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
RP Wang, TH (reprint author), Hunan Univ, Minist Educ, Key Lab Micronano Optoelectron Devices, State Key Lab Chemobiosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
EM liqiuhong2004@hotmail.com; thwang@hnu.cn
RI Wang, Taihong/K-8968-2012; Zhang, Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU "973" National Key Basic Research Program of China [2007CB310500]; Hunan
   Provincial Natural Science Foundation of China [10JJ1011]; National
   Natural Science Foundation of China [21003041]
FX This work was partly supported from "973" National Key Basic Research
   Program of China (Grant No. 2007CB310500), Hunan Provincial Natural
   Science Foundation of China (Grant No. 10JJ1011), and National Natural
   Science Foundation of China (Grant No. 21003041).
CR Zhang JL, 2010, CHEM COMMUN, V46, P1112, DOI 10.1039/b917705a
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   Wang HL, 2009, J AM CHEM SOC, V131, P9910, DOI 10.1021/ja904251p
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NR 34
TC 117
Z9 120
U1 23
U2 125
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 6
BP 1673
EP 1676
DI 10.1039/c0jm03410j
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 711TK
UT WOS:000286614100004
ER

PT J
AU Mukherjee, R
   Thomas, AV
   Krishnamurthy, A
   Koratkar, N
AF Mukherjee, Rahul
   Thomas, Abhay Varghese
   Krishnamurthy, Ajay
   Koratkar, Nikhil
TI Photothermally Reduced Graphene as High-Power Anodes for Lithium-Ion
   Batteries
SO ACS NANO
LA English
DT Article
DE graphene; lithium-ion battery; high rower; rate capability; cycle life
ID GRAPHITE OXIDE; ELECTROCHEMICAL PERFORMANCE; RATE CAPABILITY; STORAGE;
   CAPACITY; PAPER; ELECTRODES; NANOSHEETS; COMPOSITE; SYSTEM
AB Conventional graphitic anodes in lithium-ion batteries cannot provide high-power densities due to slow diffusivity of lithium ions in the bulk electrode material. Here we report photoflash and laser-reduced free-standing graphene paper as high-rate capable anodes for lithium-Ion batteries. Photothermal reduction of graphene oxide yields an expanded structure with micrometer-scale pores, cracks, and intersheet voids. This open-pore structure enables access to the underlying sheets of graphene for lithium ions and facilitates efficient intercalation kinetics even at ultrafast charge/discharge rates of >100 C. Importantly, photothermally reduced graphene anodes are structurally robust and display outstanding stability and cycling ability. At charge/discharge rates of similar to 40 C, photoreduced graphene anodes delivered a steady capacity of similar to 156 mAh/g(anode) continuously over 1000 charge/discharge cycles, providing a stable power density of similar to 10 kW/ka(anode). Such electrodes are envisioned to be mass scalable with relatively simple and low-cost fabrication procedures, thereby providing a clear pathway toward commercialization.
C1 [Mukherjee, Rahul; Thomas, Abhay Varghese; Krishnamurthy, Ajay; Koratkar, Nikhil] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
   [Koratkar, Nikhil] Rensselaer Polytech Inst, Dept Mat Sci & Engn, Troy, NY 12180 USA.
RP Koratkar, N (reprint author), Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
EM koratn@rpi.edu
RI Mukherjee, Rahul/H-8174-2013
OI Mukherjee, Rahul/0000-0002-2358-9247
FU USA National Science Foundation [0969895]
FX N.K. acknowledges funding support from the USA National Science
   Foundation (Award 0969895) and the John A. Clark and Edward T. Crossan
   Chair Professorship from the Rensselaer Polytechnic Institute. We would
   also like to thank David Guglielmo for help with operating the laser
   cutting machine and Dr. Xiang Sun for helping with BET characterization.
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NR 38
TC 115
Z9 117
U1 22
U2 165
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD SEP
PY 2012
VL 6
IS 9
BP 7867
EP 7878
DI 10.1021/nn303145j
PG 12
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 009QP
UT WOS:000309040600034
PM 22881216
ER

PT J
AU Shen, LF
   Yuan, CZ
   Luo, HJ
   Zhang, XG
   Yang, SD
   Lu, XJ
AF Shen, Laifa
   Yuan, Changzhou
   Luo, Hongjun
   Zhang, Xiaogang
   Yang, Sudong
   Lu, Xiangjun
TI In situ synthesis of high-loading Li4Ti5O12-graphene hybrid
   nanostructures for high rate lithium ion batteries
SO NANOSCALE
LA English
DT Article
ID GRAPHENE NANOSHEETS; ANODE MATERIAL; LI STORAGE; PERFORMANCE; INSERTION
AB Nanocrystalline Li4Ti5O12 grown on conducting graphene nanosheets (GNS) with good crystallinity was investigated as an advanced lithium-ion battery anode material for potential large-scale applications. This hybrid anode nanostructure material showed ultrahigh rate capability and good cycling properties at high rates.
C1 [Shen, Laifa; Luo, Hongjun; Zhang, Xiaogang; Yang, Sudong; Lu, Xiangjun] Nanjing Univ Aeronaut & Astronaut, Coll Mat Sci & Engn, Nanjing 210016, Peoples R China.
   [Yuan, Changzhou] Anhui Univ Technol, Sch Mat Sci & Engn, Maanshan 243002, Peoples R China.
RP Zhang, XG (reprint author), Nanjing Univ Aeronaut & Astronaut, Coll Mat Sci & Engn, Nanjing 210016, Peoples R China.
EM azhangxg@163.com
RI Lv, Henry/C-9692-2011; Zhang, Xiaogang/J-9565-2012; Shen,
   Laifa/J-7312-2012; Zhang, Xiao/G-8896-2013; Yuan, Changzhou/B-8757-2014
FU National Basic Research Program of China (973 Program) [2007CB209703];
   National Natural Science Foundation of China [206033040, 20873064]
FX This work was supported by the National Basic Research Program of China
   (973 Program) (No. 2007CB209703), and the National Natural Science
   Foundation of China (No. 206033040, No. 20873064).
CR Shen LF, 2010, J MATER CHEM, V20, P6998, DOI 10.1039/c0jm00348d
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NR 26
TC 114
Z9 119
U1 24
U2 125
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2011
VL 3
IS 2
BP 572
EP 574
DI 10.1039/c0nr00639d
PG 3
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 721OE
UT WOS:000287363500021
PM 21076732
ER

PT J
AU Guo, JC
   Yang, ZC
   Yu, YC
   Abruna, HD
   Archer, LA
AF Guo, Juchen
   Yang, Zichao
   Yu, Yingchao
   Abruna, Hector D.
   Archer, Lynden A.
TI Lithium-Sulfur Battery Cathode Enabled by Lithium-Nitrile Interaction
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID HIGH-CAPACITY; GRAPHENE OXIDE; ION BATTERIES; PERFORMANCE; COMPOSITE;
   CYCLE; PARTICLES; NANOTUBES
AB Lithium sulfide is a promising cathode material for high-energy lithium ion batteries because, unlike elemental sulfur, it obviates the need for metallic lithium anodes. Like elemental sulfur, however, a successful lithium sulfide cathode requires an inherent mechanism for preventing lithium polysulfide dissolution and shuttling during electrochemical cycling. A new scheme is proposed to create composites based on lithium sulfide uniformly dispersed in a carbon host, which serve to sequester polysulfides. The synthesis methodology makes use of interactions between lithium ions in solution and nitrile groups uniformly distributed along the chain backbone of a polymer precursor (e.g., polyacrylonitrile), to control the distribution of lithium sulfide in the host material. The Li2S-carbon composites obtained by carbonizing the precursor are evaluated as cathode materials in a half-cell lithium battery, and are shown to yield high galvanic charge/discharge capacities and excellent Coulombic efficiency, demonstrating the effectiveness of the architecture in homogeneously distributing Li2S and in sequestering lithium polysulfides.
C1 [Guo, Juchen; Yang, Zichao; Archer, Lynden A.] Cornell Univ, Sch Chem & Biomol Engn, Ithaca, NY 14853 USA.
   [Yu, Yingchao; Abruna, Hector D.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA.
RP Guo, JC (reprint author), Univ Calif Riverside, Dept Environm Chem & Engn, Riverside, CA 92521 USA.
EM jguo@engr.ucr.edu; laa25@cornell.edu
RI Yu, Yingchao/C-4769-2012
FU Energy Materials Center at Cornell, an Energy Frontier Research Center;
   U.S. Department of Energy, Office of Science, Office of Basic Energy
   Sciences [DESC0001086]; National Science Foundation, Partnerships for
   Innovation Program [IIP-1237622]; ACS Division of Analytical Chemistry;
   Eastman Chemical Co.; NSF [DMR-1120296]
FX This material is based on work supported in part by the Energy Materials
   Center at Cornell, an Energy Frontier Research Center funded by the U.S.
   Department of Energy, Office of Science, Office of Basic Energy Sciences
   under Award Number DESC0001086. We also acknowledge the National Science
   Foundation, Partnerships for Innovation Program (Grant no. IIP-1237622)
   for partial support of the study. Y.Y. acknowledges the fellowship from
   ACS Division of Analytical Chemistry and support from Eastman Chemical
   Co. This work made use of the electron microscopy facility at the
   Cornell Center for Materials Research, a NSF supported MRSEC through
   Grant DMR-1120296.
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
J9 J AM CHEM SOC
JI J. Am. Chem. Soc.
PD JAN 16
PY 2013
VL 135
IS 2
BP 763
EP 767
DI 10.1021/ja309435f
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA 075XP
UT WOS:000313920800045
PM 23234561
ER

PT J
AU Xing, WB
   Wilson, AM
   Eguchi, K
   Zank, G
   Dahn, JR
AF Xing, WB
   Wilson, AM
   Eguchi, K
   Zank, G
   Dahn, JR
TI Pyrolyzed polysiloxanes for use as anode materials in lithium-ion
   batteries
SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY
LA English
DT Article
ID NANODISPERSED SILICON; CARBONS
AB More than sixty siloxane polymers containing various organofunctional siloxane units were synthesized. The synthesized siloxane polymers were pyrolyzed in inert gas at 1000 degrees C. Chemical analysis showed that the products of pyrolysis were distributed over a well-defined region in the Si-C-O Gibbs phase diagram. The electrochemical and structural properties of these materials were measured using coin-type test cells and x-rap powder diffraction, respectively. The most interesting materials are found near the line in the Si-C-O Gibbs triangle connecting carbon to SiO1.3. Materials with the largest reversible specific capacity for lithium (about 900 mAh/g) are on this line and were at about 43% carbon, 32% oxygen, and 25% silicon (atomic percent). Materials which were almost pure carbon showed diffraction patterns characteristic of disordered carbons. Along the line from carbon to SiO1.3 the sample structure can be described as a mixture of single or small groups of graphene sheets mixed with regions of Si-C-O amorphous glass. The amount and composition of the glass changed according to the overall sample composition. Moving from carbon to SiO1.3, the reversible capacity first rises from about 340 mAh/g for pure carbon, to a maximum of 900 mAh/g near 50% carbon, and then falls to near zero mAh/g at 0% carbon. This suggests that the amorphous glass can reversibly react with lithium, provided the carbon is present to provide a path for electrons and Li ions. However, the hysteresis in the voltage profile(difference between charge and discharge voltages) and the irreversible capacity increase almost linearly along this line. There is a clear correlation between both the irreversible capacity and hysteresis in these materials with their oxygen content. Along the line connecting carbon to silicon, the reversible capacity rises from 340 mAh/g for pure carbon to about 600 mAh/g for samples with about 15 atomic percent Si. It then decreases to near zero as the composition nears SiC. Along the C-SiC line, the irreversible capacities remain below about 200 mAh/g. We are quite convinced that optimized silicon-containing carbons can be good alternatives to pure carbons as anode materials in lithium-ion batteries.
C1 SIMON FRASER UNIV,DEPT PHYS,BURNABY,BC V5A 1S6,CANADA.
   DOW CORNING ASIA LTD,KANAGAWA,JAPAN.
RP Xing, WB (reprint author), DALHOUSIE UNIV,DEPT PHYS,HALIFAX,NS B3H 3J5,CANADA.
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J9 J ELECTROCHEM SOC
JI J. Electrochem. Soc.
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PY 1997
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BP 2410
EP 2416
DI 10.1149/1.1837828
PG 7
WC Electrochemistry; Materials Science, Coatings & Films
SC Electrochemistry; Materials Science
GA XM567
UT WOS:A1997XM56700038
ER

PT J
AU Peng, X
   Peng, LL
   Wu, CZ
   Xie, Y
AF Peng, Xu
   Peng, Lele
   Wu, Changzheng
   Xie, Yi
TI Two dimensional nanomaterials for flexible supercapacitors
SO CHEMICAL SOCIETY REVIEWS
LA English
DT Review
ID REDUCED GRAPHENE OXIDE; HIGH-ENERGY DENSITY; LITHIUM-ION BATTERIES;
   PERFORMANCE ELECTROCHEMICAL CAPACITORS; SOLID-STATE SUPERCAPACITORS;
   MICRO-SUPERCAPACITORS; ULTRATHIN NANOSHEETS; CARBON-FILMS; HYBRID
   STRUCTURE; ANODE MATERIAL
AB Flexible supercapacitors, as one of most promising emerging energy storage devices, are of great interest owing to their high power density with great mechanical compliance, making them very suitable as power back-ups for future stretchable electronics. Two-dimensional (2D) nanomaterials, including the quasi-2D graphene and inorganic graphene-like materials (IGMs), have been greatly explored to providing huge potential for the development of flexible supercapacitors with higher electrochemical performance. This review article is devoted to recent progresses in engineering 2D nanomaterials for flexible supercapacitors, which survey the evolution of electrode materials, recent developments in 2D nanomaterials and their hybrid nanostructures with regulated electrical properties, and the new planar configurations of flexible supercapacitors. Furthermore, a brief discussion on future directions, challenges and opportunities in this fascinating area is also provided.
C1 [Wu, Changzheng] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.
   Univ Sci & Technol China, Collaborat Innovat Ctr Chem Energy Mat, Hefei 230026, Anhui, Peoples R China.
RP Wu, CZ (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.
EM czwu@ustc.edu.cn
RI Wu, Changzheng/F-1784-2010; China, iChEM/F-2855-2015
OI Wu, Changzheng/0000-0002-4416-6358; 
FU National Natural Science Foundation of China [21222101, 11132009,
   21331005, 11321503, J1030412]; Chinese Academy of Science [XDB01010300];
   Program for New Century Excellent Talents in University; Fundamental
   Research Funds for the Central Universities [WK2060190027, WK2310000024]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 21222101, 11132009, 21331005, 11321503,
   J1030412), the Chinese Academy of Science (XDB01010300), the Program for
   New Century Excellent Talents in University, and the Fundamental
   Research Funds for the Central Universities (No. WK2060190027 and
   WK2310000024).
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NR 110
TC 110
Z9 111
U1 138
U2 515
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0306-0012
EI 1460-4744
J9 CHEM SOC REV
JI Chem. Soc. Rev.
PY 2014
VL 43
IS 10
BP 3303
EP 3323
DI 10.1039/c3cs60407a
PG 21
WC Chemistry, Multidisciplinary
SC Chemistry
GA AF9CX
UT WOS:000335014000005
PM 24614864
ER

PT J
AU Qin, J
   He, CN
   Zhao, NQ
   Wang, ZY
   Shi, CS
   Liu, EZ
   Li, JJ
AF Qin, Jian
   He, Chunnian
   Zhao, Naiqin
   Wang, Zhiyuan
   Shi, Chunsheng
   Liu, En-Zuo
   Li, Jiajun
TI Graphene Networks Anchored with Sn@Graphene as Lithium Ion Battery Anode
SO ACS NANO
LA English
DT Article
DE Sn; graphene; high-rate; core-shell; nanohybrid; 3D network; in situ
   synthesis; chemical vapor deposition; lithium storage
ID CHEMICAL-VAPOR-DEPOSITION; COMPOSITE ANODES; REDUCED GRAPHENE; HOLLOW
   CARBON; CNT NANOSTRUCTURES; C COMPOSITE; STORAGE; PERFORMANCE;
   NANOPARTICLES; NANOSHEETS
AB A facile and scalable in situ chemical vapor deposition (CVD) technique using metal precursors as a catalyst and a three-dimensional (3D) self-assembly of NaCl particles as a template is developed for one-step fabrication of 3D porous graphene networks anchored with Sn nanoparticles (5-30 nm) encapsulated with graphene shells of about 1 nm (Sn@G-PGNWs) as a superior lithium ion battery anode. In the constructed architecture, the CVD-synthesized graphene shells with excellent elasticity can effectively not only avoid the direct exposure of encapsulated Sn to the electrolyte and preserve the structural and interfacial stabilization of Sn nanoparticles but also suppress the aggregation of Sn nanoparticles and buffer the volume expansion, while the interconnected 3D porous graphene networks with high electrical conductivity, large surface area, and high mechanical flexibility tightly pin the core-shell structure of Sn@G and thus lead to remarkably enhanced electrical conductivity and structural integrity of the overall electrode. As a consequence, this 3D hybrid anode exhibits very high rate performance (1022 mAh/g at 0.2 C, 865 mAh/g at 03 C, 780 mAh/g at 1 C, 652 mAh/g at 2 C, 459 mAh/g at 5 C, and 270 mAh/g at 10 C, 1 C = 1 A/g) and extremely long cycling stability even at high rates (a high capacity of 682 mAh/g is achieved at 2 A/g and is maintained approximately 96.3% after 1000 cycles). As far as we know, this is the best rate capacity and longest cycle life ever reported for a Sn-based lithium ion battery anode.
C1 [Qin, Jian; He, Chunnian; Zhao, Naiqin; Wang, Zhiyuan; Shi, Chunsheng; Liu, En-Zuo; Li, Jiajun] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
   [Qin, Jian; He, Chunnian; Zhao, Naiqin; Wang, Zhiyuan; Shi, Chunsheng; Liu, En-Zuo; Li, Jiajun] Tianjin Univ, Tianjin Key Lab Composites & Funct Mat, Tianjin 300072, Peoples R China.
   [He, Chunnian; Zhao, Naiqin] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300072, Peoples R China.
RP He, CN (reprint author), Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
EM cnhe08@tju.edu.cn; nqzhao@tju.edu.cn
FU National Natural Science Foundation of China [51071107, 51002188,
   51272173]; Foundation for the Author of National Excellent Doctoral
   Dissertation of China [201145]; Program for New Century Excellent
   Talents in University [NCET-12-0408]; Natural Science Foundation of
   Tianjin City [12JCYBJC11700]; Elite Scholar Program of Tianjin
   University; Innovation Foundation of Tianjin University; National Basic
   Research Program of China [2010CB934700]
FX The authors acknowledge the financial support by the National Natural
   Science Foundation of China (No. 51071107, No. 51002188, and No.
   51272173), Foundation for the Author of National Excellent Doctoral
   Dissertation of China (No. 201145), Program for New Century Excellent
   Talents in University (NCET-12-0408), Natural Science Foundation of
   Tianjin City (No. 12JCYBJC11700), Elite Scholar Program of Tianjin
   University, Innovation Foundation of Tianjin University, and National
   Basic Research Program of China (2010CB934700).
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NR 55
TC 109
Z9 110
U1 86
U2 375
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD FEB
PY 2014
VL 8
IS 2
BP 1728
EP 1738
DI 10.1021/nn406105n
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AB8SB
UT WOS:000332059200070
PM 24400945
ER

PT J
AU Chang, HX
   Wu, HK
AF Chang, Haixin
   Wu, Hongkai
TI Graphene-based nanocomposites: preparation, functionalization, and
   energy and environmental applications
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID LITHIUM-ION BATTERIES; SENSITIZED SOLAR-CELLS; OXYGEN REDUCTION
   REACTION; VISIBLE-LIGHT IRRADIATION; SINGLE-LAYER GRAPHENE; PERFORMANCE
   ELECTROCHEMICAL CAPACITORS; PHOTOCATALYTIC HYDROGEN EVOLUTION; METHANOL
   FUEL-CELLS; ANODE MATERIAL; HYDROTHERMAL SYNTHESIS
AB Graphene, a two-dimensional carbon sheet with one atom thickness and one of the thinnest materials in universe, has inspired huge interest in physics, materials science, chemistry and biology. However, pure graphene sheets are limited for many applications despite their excellent characteristics and scientists face challenges to induce more and controlled functionality. Therefore graphene nanocomposites or hybrids are attracting increasing efforts for real applications in energy and environmental areas by introducing controlled functional building blocks to graphene. In this Review, we first give a brief introduction of graphene's unique physical and chemical properties followed by various preparation and functionalization methods for graphene nanocomposites in the second section. We focus on recent energy-related progress of graphene nanocomposites in solar energy conversion (e.g., photovoltaic and photoelectrochemical devices, artificial photosynthesis) and electrochemical energy devices (e.g., lithium ion battery, supercapacitor, fuel cell) in the third section. We then review the advances in environmental applications of functionalized graphene nanocomposites for the detection and removal of heavy metal ions, organic pollutants, gas and bacteria in the fourth section. Finally a conclusion and perspective is given to discuss the remaining challenges for graphene nanocomposites in energy and environmental science.
C1 [Chang, Haixin; Wu, Hongkai] Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan.
   [Wu, Hongkai] Hong Kong Univ Sci & Technol, Dept Chem, Hong Kong, Hong Kong, Peoples R China.
   [Chang, Haixin] Huazhong Univ Sci & Technol, State Key Lab Mat Proc & Die & Mould Technol, Sch Mat Sci & Engn, Wuhan 430074, Peoples R China.
RP Chang, HX (reprint author), Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan.
EM hxchang@wpi-aimr.tohoku.ac.jp; chhkwu@ust.hk
RI Chang, Haixin/A-1753-2012
FU World Premier International Research Center Initiative (WPI), MEXT,
   Japan; MEXT; JSPS, Japan [25870057]
FX This work is supported by World Premier International Research Center
   Initiative (WPI), MEXT, Japan. H.X.C. acknowledges the WPI-AIMR fusion
   research funding from MEXT and a Grant-in-Aid for Young Scientists B
   from JSPS (no. 25870057), Japan.
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NR 292
TC 108
Z9 110
U1 181
U2 829
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD DEC
PY 2013
VL 6
IS 12
BP 3483
EP 3507
DI 10.1039/c3ee42518e
PG 25
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 255OS
UT WOS:000327250300006
ER

PT J
AU Ma, CC
   Shao, XH
   Cao, DP
AF Ma, Congcong
   Shao, Xiaohong
   Cao, Dapeng
TI Nitrogen-doped graphene nanosheets as anode materials for lithium ion
   batteries: a first-principles study
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID WALLED CARBON NANOTUBES; BORON; ABSORPTION
AB First-principles calculations are performed to investigate the effects of the electron-deficiency of N-doped graphenes on their application in lithium ion batteries (LIBs), where three different defect models, graphitic, pyridinic, and pyrrolic graphenes are used. First, we investigate adsorption of a single Li atom on various graphenes and explore the change of the electronic properties in order to understand the adsorption mechanism. Then, adsorption of multiple Li atoms is also performed to consider the lithium storage properties of N-doped graphene nanosheets. The results show that the pyridinic graphene is the most suitable for Li storage with a high storage capacity, while the graphitic structure is the weakest of the three types. Moreover, the average potential of Li intercalation in the graphene materials was also calculated, and results indicate that the reversible capacity of the pyridinic structure can reach 1262 mAh g(-1), which is higher than the experimental data (1043 mAh g(-1)). Therefore, we recommend pyridinic graphene in the N-doped structures as anode materials of lithium ion batteries and the corresponding reversible capacity of LIBs would be improved significantly. It is expected that this work could provide helpful information for the design and fabrication of anode materials of LIBs.
C1 [Ma, Congcong; Cao, Dapeng] Beijing Univ Chem Technol, State Key Lab Organicinorgan Composites, Div Mol & Mat Simulat, Beijing 100029, Peoples R China.
   [Shao, Xiaohong] Beijing Univ Chem Technol, Coll Sci, Beijing 100029, Peoples R China.
RP Cao, DP (reprint author), Beijing Univ Chem Technol, State Key Lab Organicinorgan Composites, Div Mol & Mat Simulat, Beijing 100029, Peoples R China.
EM caodp@mail.buct.edu.cn
FU Huo Yingdong Fundamental Research Foundation [121070]; National Basic
   Research Program of China [2011CB706900]; NSF of China [21121064];
   Ministry of Education [20100010110001]; BUCT
FX This work is supported by Huo Yingdong Fundamental Research Foundation
   (121070), National Basic Research Program of China (2011CB706900), NSF
   of China (21121064), Doctoral Programs of Ministry of Education
   (20100010110001) and Chemical Grid Program from BUCT.
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NR 29
TC 107
Z9 107
U1 22
U2 196
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 18
BP 8911
EP 8915
DI 10.1039/c2jm00166g
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 923QW
UT WOS:000302634800026
ER

PT J
AU Zhang, BA
   Zheng, QB
   Huang, ZD
   Oh, SW
   Kim, JK
AF Zhang, Biao
   Zheng, Qing Bin
   Huang, Zhen Dong
   Oh, Sei Woon
   Kim, Jong Kyo
TI SnO2-graphene-carbon nanotube mixture for anode material with improved
   rate capacities
SO CARBON
LA English
DT Article
ID LITHIUM-ION BATTERIES; CARBON NANOTUBES; REVERSIBLE CAPACITY; GRAPHENE
   NANOSHEETS; CYCLIC PERFORMANCE; STORAGE; NANOPARTICLES; PAPER;
   ELECTRODES; OXIDE
AB SnO2-graphene-carbon nanotube (SnO2-G-CNT) mixture is synthesized using graphene oxide as precursor for application as anode material in rechargeable Li ion batteries. It is shown that the SnO2 nanoparticles of 3-6 nm in diameter are not only attached onto the surface of graphene sheets by anchoring with surface functional groups, but they also are encapsulated in pore channels formed by entangled graphene sheets. The incorporation of carbon nanotubes reduces the charge transfer resistance of the anode made from the mixture through the formation of 3D electronic conductive networks. The SnO2-GCNT anodes deliver remarkable capacities of 345 and 635 mAh g(-1) at 1.5 and 0.25 A g(-1), respectively. Flexible electrodes consisting of highly-aligned SnO2-G-CNT papers are also prepared using a simple vacuum filtration technique. They present a stable capacity of 387 mAh g(-1) at 0.1 A g(-1) after 50 cycles through the synergy of the high specific capacity of SnO2 nanoparticles and the excellent cycleability of G-CNT paper. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Zhang, Biao; Zheng, Qing Bin; Huang, Zhen Dong; Oh, Sei Woon; Kim, Jong Kyo] Hong Kong Univ Sci & Technol, Dept Mech Engn, Kowloon, Hong Kong, Peoples R China.
RP Kim, JK (reprint author), Hong Kong Univ Sci & Technol, Dept Mech Engn, Kowloon, Hong Kong, Peoples R China.
EM mejkkim@ust.hk
RI Kim, Jang Kyo /B-3099-2010; zheng, qingbin/F-9323-2011; Zhendong,
   Huang/E-5269-2011; Zhang, Biao/A-8662-2013
OI Kim, Jang Kyo /0000-0002-5390-8763; 
FU Research Grant Council of Hong Kong [614010, 613811]; Hong Kong SAR
   [GHP/028/08SZ]; Finetex-HKUST RD Center [FTG001-MECH.07/08]; School of
   Engineering, HKUST
FX This project was supported by the Research Grant Council of Hong Kong
   (Project Codes: 614010 and 613811), the Innovation and Technology Fund
   of Hong Kong SAR (Project Code: GHP/028/08SZ) and the Finetex-HKUST R&D
   Center (Project Code: FTG001-MECH.07/08). The authors also appreciate
   the technical assistance from the Materials Characterization and
   Preparation Facilities (MCPF) of HKUST. B.Z. is supported partly by the
   Postgraduate Scholarship through the Nanoscience and Technology Program
   of the School of Engineering, HKUST.
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NR 40
TC 107
Z9 108
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U2 166
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD NOV
PY 2011
VL 49
IS 13
BP 4524
EP 4534
DI 10.1016/j.carbon.2011.06.059
PG 11
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 817BL
UT WOS:000294645700050
ER

PT J
AU Ji, LW
   Tan, ZK
   Kuykendall, T
   An, EJ
   Fu, YB
   Battaglia, V
   Zhang, YG
AF Ji, Liwen
   Tan, Zhongkui
   Kuykendall, Tevye
   An, Eun Ji
   Fu, Yanbao
   Battaglia, Vincent
   Zhang, Yuegang
TI Multilayer nanoassembly of Sn-nanopillar arrays sandwiched between
   graphene layers for high-capacity lithium storage
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID ION BATTERIES; ANODE MATERIAL; HOLLOW CARBON; SECONDARY BATTERIES;
   TIN-NANOPARTICLES; FILM FORMATION; PERFORMANCE; NANOFIBERS; ELECTRODE;
   ENCAPSULATION
AB Sn nanopillar arrays embedded between graphene sheets were assembled using a conventional film deposition and annealing process. The as-formed three-dimensional (3D) multilayered nanostructure was directly used as an anode material for rechargeable lithium-ion batteries without adding any polymer binder and carbon black. Electrochemical measurements showed very high reversible capacity and excellent cycling performance at a current density as high as 5 A g(-1). These results demonstrated that nanocomposite materials with highly functional 1D and 2D components can be synthesized by employing conventional top-down manufacturing methods and self-assembly principles.
C1 [Ji, Liwen; Tan, Zhongkui; Kuykendall, Tevye; An, Eun Ji; Zhang, Yuegang] Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, Berkeley, CA 94720 USA.
   [Fu, Yanbao; Battaglia, Vincent] Univ Calif Berkeley, Lawrence Berkeley Lab, Adv Energy Technol Dept, Berkeley, CA 94720 USA.
RP Ji, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA.
EM yzhang5@lbl.gov
RI Zhang, Y/E-6600-2011; Fu, Yanbao/F-9583-2011
OI Zhang, Y/0000-0003-0344-8399; Fu, Yanbao/0000-0001-7752-680X
FU Office of Science, Office of Basic Energy Sciences, of the U. S.
   Department of Energy [DE-AC02-05CH11231]
FX This work was supported by the Office of Science, Office of Basic Energy
   Sciences, of the U. S. Department of Energy under contract No.
   DE-AC02-05CH11231.
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NR 51
TC 107
Z9 107
U1 15
U2 116
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD SEP
PY 2011
VL 4
IS 9
BP 3611
EP 3616
DI 10.1039/c1ee01592c
PG 6
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 812QB
UT WOS:000294306900058
ER

PT J
AU Li, BJ
   Cao, HQ
   Yin, G
   Lu, YX
   Yin, JF
AF Li, Baojun
   Cao, Huaqiang
   Yin, Gui
   Lu, Yuexiang
   Yin, Jiefu
TI Cu2O@reduced graphene oxide composite for removal of contaminants from
   water and supercapacitors
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM ION BATTERIES; CU2O NANOPARTICLES; ROOM-TEMPERATURE; NANOSHEETS;
   CAPACITY; EXCITONS; SCIENCE; SHEETS; ROUTE; ANODE
AB Cu2O@reduced graphene oxide composite displays a good ability to remove dyes from water and high stability in supercapacitors, highlighting potential applications in environmental and energy storage issues.
C1 [Li, Baojun; Cao, Huaqiang; Lu, Yuexiang; Yin, Jiefu] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Yin, Gui] Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210093, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
RI Lu, Yuexiang/B-4742-2011
OI Lu, Yuexiang/0000-0003-2755-7733
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]; Jiangsu
   Province Foundation of Natural Science [BK2006717]; China Postdoctoral
   Science Foundation [20100470302]
FX Financial support from the National Natural Science Foundation of China
   (No. 20921001 and 20535020), the Innovation Method Fund of China (No.
   20081885189), the National High Technology Research and Development
   Program of China (No. 2009AA03Z321), the Jiangsu Province Foundation of
   Natural Science (No. BK2006717), and the China Postdoctoral Science
   Foundation (No. 20100470302) are acknowledged.
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NR 42
TC 106
Z9 110
U1 18
U2 158
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 29
BP 10645
EP 10648
DI 10.1039/c1jm12135a
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 795MP
UT WOS:000292978600010
ER

PT J
AU Mai, YJ
   Shi, SJ
   Zhang, D
   Lu, Y
   Gu, CD
   Tu, JP
AF Mai, Y. J.
   Shi, S. J.
   Zhang, D.
   Lu, Y.
   Gu, C. D.
   Tu, J. P.
TI NiO-graphene hybrid as an anode material for lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Nickel oxide; Graphene; Thermodynamics; Kinetics; Voltage hysteresis
ID NEGATIVE-ELECTRODE MATERIALS; CONVERSION REACTIONS; REVERSIBLE CAPACITY;
   LI-STORAGE; NANOCOMPOSITE; PERFORMANCE; INSERTION; FILM; HYSTERESIS;
   STABILITY
AB A NiO-graphene hybrid is synthesized by a liquid phase deposition method. As an anode material for lithium ion batteries, the cyclic stability and rate capability of NiO is significantly improved after the incorporation of graphene sheets. The NiO-graphene hybrid electrode delivers a capacity of 646.1 mA h g(-1) after 35 cycles at a current density of 100 mA g(-1), corresponding to 86.3% capacity retention. When the current density is increased to 400 and 800 mA g(-1), it still maintains a capacity of 509 and 368.5 mA h g(-1), respectively. The thermodynamic and kinetic properties of NiO electrodes with and without graphene are investigated by galvanostatic intermittent titration technique. The relationship between the rate and voltage hysteresis is also discussed. The polarization of both the electrodes in all cases obeys ohmic rule in the present rate range. The incorporation of graphene sheets can partly reduce the voltage polarization thereby the voltage hysteresis with increasing the current density. However, the extrapolation to zero current ends up in an approximate residual voltage for both the NiO electrodes. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Tu, J. P.] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
   Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
RP Tu, JP (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
EM tujplab@zju.edu.cn
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NR 47
TC 105
Z9 105
U1 22
U2 190
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD APR 15
PY 2012
VL 204
BP 155
EP 161
DI 10.1016/j.jpowsour.2011.12.038
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 904TM
UT WOS:000301220800023
ER

PT J
AU Zhang, L
   Wu, HB
   Lou, XW
AF Zhang, Lei
   Wu, Hao Bin
   Lou, Xiong Wen (David)
TI Iron-Oxide- Based Advanced Anode Materials for LithiumIon Batteries
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE iron oxide; Fe2O3; Fe3O4; lithium-ion batteries; anode materials
ID HIGH-PERFORMANCE ANODE; LI-ION BATTERIES; METAL-ORGANIC-FRAMEWORKS;
   ONE-POT SYNTHESIS; STORAGE PROPERTIES; HOLLOW SPHERES; ENERGY-STORAGE;
   NANOSTRUCTURED MATERIALS; HYBRID NANOSTRUCTURES; ALPHA-FE2O3 NANOTUBES
AB Iron oxides, such as Fe2O3 and Fe3O4, have recently received increased attention as very promising anode materials for rechargeable lithium-ion batteries (LIBs) because of their high theoretical capacity, non-toxicity, low cost, and improved safety. Nanostructure engineering has been demonstrated as an effective approach to improve the electrochemical performance of electrode materials. Here, recent research progress in the rational design and synthesis of diverse iron oxide-based nanomaterials and their lithium storage performance for LIBs, including 1D nanowires/rods, 2D nanosheets/flakes, 3D porous/hierarchical architectures, various hollow structures, and hybrid nanostructures of iron oxides and carbon (including amorphous carbon, carbon nanotubes, and graphene). By focusing on synthesis strategies for various iron-oxide-based nanostructures and the impacts of nanostructuring on their electrochemical performance, novel approaches to the construction of iron-oxide-based nanostructures are highlighted and the importance of proper structural and compositional engineering that leads to improved physical/chemical properties of iron oxides for efficient electrochemical energy storage is stressed. Iron-oxide-based nanomaterials stand a good chance as negative electrodes for next generation LIBs.
C1 [Zhang, Lei; Wu, Hao Bin; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM xwlou@ntu.edu.sg
RI Zhang, Lei/A-4182-2013; Wu, Haobin/D-1572-2014; Lou , Xiong Wen
   (David)/D-2648-2009
OI Zhang, Lei/0000-0002-6385-5773; Wu, Haobin/0000-0002-0725-6442; 
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NR 83
TC 103
Z9 103
U1 108
U2 568
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD MAR
PY 2014
VL 4
IS 4
AR 1300958
DI 10.1002/aenm.201300958
PG 11
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AD0LE
UT WOS:000332924700009
ER

PT J
AU Xu, C
   Zeng, Y
   Rui, XH
   Xiao, N
   Zhu, JX
   Zhang, WY
   Chen, J
   Liu, WL
   Tan, HT
   Hng, HH
   Yan, QY
AF Xu, Chen
   Zeng, Yi
   Rui, Xianhong
   Xiao, Ni
   Zhu, Jixin
   Zhang, Wenyu
   Chen, Jing
   Liu, Weiling
   Tan, Huiteng
   Hng, Huey Hoon
   Yan, Qingyu
TI Controlled Soft-Template Synthesis of Ultrathin C@FeS Nanosheets with
   High-Li-Storage Performance
SO ACS NANO
LA English
DT Article
DE soft-template; 2D nanostructures; metal sulfides; iron; lithium ion
   battery
ID LITHIUM-ION BATTERIES; METAL SULFIDE NANOCRYSTALS; ELECTROCHEMICAL
   PERFORMANCE; ALPHA-FE2O3/C NANOCOMPOSITE; ORIENTED ATTACHMENT; SULFUR
   BATTERIES; ANODE MATERIAL; GRAPHENE; CATHODE; SHEETS
AB We report a facile approach to prepare carbon-coated troilite FeS (C@FeS) nanosheets via surfactant-assisted solution-based synthesis. 1-Dodecanethiol is used as both the sulfur source and the surfactant, which may form different-shaped micelles to direct the growth of nanostructures. Under appropriate growth conditions, the iron and sulfur atoms react to form thin layers of FeS while the hydrocarbon tails of 1-dodecanethiol separate the thin FeS layers, which turn to carbon after annealing in Ar. Such an approach can be extended to grow C@FeS nanospheres and nanoplates by modifying the synthesis parameters. The C@FeS nanosheets display excellent Li storage properties with high specific capacities and stable charge/discharge cyclability, especially at fast charge/discharge rates.
C1 [Xu, Chen; Zeng, Yi; Rui, Xianhong; Xiao, Ni; Zhu, Jixin; Zhang, Wenyu; Liu, Weiling; Tan, Huiteng; Hng, Huey Hoon; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Xu, Chen; Zeng, Yi; Zhu, Jixin; Zhang, Wenyu; Tan, Huiteng; Yan, Qingyu] Nanyang Technol Univ, TUM CREATE Res Ctr, Singapore 637459, Singapore.
   [Xu, Chen; Zhang, Wenyu; Tan, Huiteng; Yan, Qingyu] Nanyang Technol Univ, Energy Res Inst, Singapore 637553, Singapore.
RP Yan, QY (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
EM alexyan@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; zhu, Jixin/F-8763-2011; Hng, Huey
   Hoon/A-2246-2011; Rui, Xianhong/D-2604-2015
OI Hng, Huey Hoon/0000-0002-8950-025X; Rui, Xianhong/0000-0003-1125-0905
FU AcRF Tier 1 of MOE (Singapore) [RG 31/08]; Singapore Ministry of
   Education [M0E2010-12-1-017]; A*STAR SERC [1021700144]; Singapore [MPA
   23/04.15.03 RDP 009/10/102, MPA 23/04.15.03 RDP 020/10/113]; 
   [NRF2009EWT-CERP001-026]
FX The authors gratefully acknowledge AcRF Tier 1 RG 31/08 of MOE
   (Singapore), NRF2009EWT-CERP001-026 (Singapore), Singapore Ministry of
   Education (MOE2010-T2-1-017), A*STAR SERC Grant 1021700144, and
   Singapore MPA 23/04.15.03 RDP 009/10/102 and MPA 23/04.15.03 RDP
   020/10/113 grants.
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TC 102
Z9 103
U1 69
U2 391
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUN
PY 2012
VL 6
IS 6
BP 4713
EP 4721
DI 10.1021/nn2045714
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 963YQ
UT WOS:000305661300019
PM 22568936
ER

PT J
AU Zhou, WW
   Liu, JP
   Chen, T
   Tan, KS
   Jia, XT
   Luo, ZQ
   Cong, CX
   Yang, HP
   Li, CM
   Yu, T
AF Zhou, Weiwei
   Liu, Jinping
   Chen, Tao
   Tan, Kim Seng
   Jia, Xingtao
   Luo, Zhiqiang
   Cong, Chunxiao
   Yang, Huanping
   Li, Chang Ming
   Yu, Ting
TI Fabrication of Co3O4-reduced graphene oxide scrolls for high-performance
   supercapacitor electrodes
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID LITHIUM ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; EXFOLIATED
   GRAPHITE OXIDE; REVERSIBLE CAPACITY; CO3O4 NANOPARTICLES; CARBON
   NANOSCROLLS; CYCLIC PERFORMANCE; ROOM-TEMPERATURE; ANODE MATERIAL;
   HYDROUS RUO2
AB A new type of scrolled structure of Co3O4/reduced graphene oxide (r-GO) is facilely prepared through a two-step surfactant-assisted method. This assembly enables almost every single Co3O4 scroll to connect with the r-GO platelets, thus leading to remarkable electrochemical performances in terms of high specific capacitance and good rate capability.
C1 [Zhou, Weiwei; Liu, Jinping; Tan, Kim Seng; Jia, Xingtao; Luo, Zhiqiang; Cong, Chunxiao; Yang, Huanping; Yu, Ting] Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore.
   [Liu, Jinping] Cent China Normal Univ, Inst Nanosci & Nanotechnol, Dept Phys, Wuhan 430079, Peoples R China.
   [Chen, Tao; Li, Chang Ming] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637457, Singapore.
   [Yu, Ting] Natl Univ Singapore, Dept Phys, Fac Sci, Singapore 117542, Singapore.
RP Yu, T (reprint author), Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, 21 Nanyang Link, Singapore 637371, Singapore.
EM yuting@ntu.edu.sg
RI Liu, Jinping/A-9285-2008; Chen, Tao/H-3501-2011; LUO,
   ZHIQIANG/G-8410-2015; Chen, Tao/C-3448-2016
OI cong, chunxiao/0000-0001-9786-825X; Yu, Ting/0000-0002-0113-2895; 
FU Singapore National Research Foundation under NRF RF [NRF-RF2010-07, MOE
   Tier 2 MOE2009-T2-1-037]
FX This work is supported by the Singapore National Research Foundation
   under NRF RF Award No. NRF-RF2010-07 and MOE Tier 2 MOE2009-T2-1-037.
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   Zhu W, 2006, CRYST GROWTH DES, V6, P2804, DOI 10.1021/cg060439o
NR 38
TC 102
Z9 103
U1 30
U2 164
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2011
VL 13
IS 32
BP 14462
EP 14465
DI 10.1039/c1cp21917k
PG 4
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 802MR
UT WOS:000293516200023
PM 21735027
ER

PT J
AU Chang, K
   Geng, DS
   Li, XF
   Yang, JL
   Tang, YJ
   Cai, M
   Li, RY
   Sun, XL
AF Chang, Kun
   Geng, Dongsheng
   Li, Xifei
   Yang, Jinli
   Tang, Yongji
   Cai, Mei
   Li, Ruying
   Sun, Xueliang
TI Ultrathin MoS2/Nitrogen-Doped Graphene Nanosheets with Highly Reversible
   Lithium Storage
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE MoS2; Nitrogen-doped graphene; Nanosheet; Lithium ion batteries
ID ION BATTERIES; DOPED GRAPHENE; ELECTROCHEMICAL PERFORMANCES; CARBON;
   MOS2; ANODE; NANOSTRUCTURES; NANOPARTICLES; COMPOSITES; CAPACITY
C1 [Chang, Kun; Geng, Dongsheng; Li, Xifei; Yang, Jinli; Tang, Yongji; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
   [Cai, Mei] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Li, Xifei/A-1966-2012; Geng, Dongsheng/G-7124-2011; Sun,
   Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; 
FU Natural Sciences and Engineering Research Council of Canada (NSERC);
   General Motors of Canada; Canada Research Chair (CRC) Program;
   University of Western Ontario
FX This work is supported by Natural Sciences and Engineering Research
   Council of Canada (NSERC), General Motors of Canada, Canada Research
   Chair (CRC) Program, and the University of Western Ontario.
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NR 30
TC 101
Z9 103
U1 49
U2 250
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD JUL
PY 2013
VL 3
IS 7
BP 839
EP 844
DI 10.1002/aenm.201201108
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 261XO
UT WOS:000327698200004
ER

PT J
AU Xin, X
   Zhou, XF
   Wu, JH
   Yao, XY
   Liu, ZP
AF Xin, Xing
   Zhou, Xufeng
   Wu, Jinghua
   Yao, Xiayin
   Liu, Zhaoping
TI Scalable Synthesis of TiO2/Graphene Nanostructured Composite with
   High-Rate Performance for Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE Li-ion battery; titania; graphene; anode; nanocomposite
ID ANATASE TIO2 NANOSHEETS; ANODE MATERIALS; ELECTROCHEMICAL PERFORMANCE;
   STORAGE; NANOTUBES; CAPACITY; NANOCOMPOSITE; NANOFIBERS; INSERTION;
   NANOMATERIALS
AB A simple and scalable method is developed to synthesize TiO2/graphene nanostructured composites as high-performance anode materials for Li-ion batteries using hydroxyl titanium oxalate (HTO) as the intermediate for TiO2. With assistance of a surfactant, amorphous HTO can condense as a flower-like nanostructure on graphene oxide (GO) sheets. By calcination, the HTO/GO nanocomposite can be converted to TiO2/graphene nanocomposite with well preserved flower-like nanostructure. In the composite, TiO2 nanoparticles with an ultrasmall size of several nanometers construct the porous flower-like nanostructure which strongly attached onto conductive graphene nanosheets. The TiO2/graphene nanocomposite is able to deliver a capacity of 230 mA h g(-1) at 0.1 C (corresponding to a current density of 17 mA g(-1)), and demonstrates superior high-rate charge-discharge capability and cycling stability at charge/discharge rates up to 50 C in a half cell configuration. Full cell measurement using the TiO2/graphene as the anode material and spinel LiMnO2 as the cathode material exhibit good high-rate performance and cycling stability, indicating that the TiO2/graphene nanocomposite has a practical application potential in advanced Li-ion batteries.
C1 [Xin, Xing; Zhou, Xufeng; Wu, Jinghua; Yao, Xiayin; Liu, Zhaoping] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
RP Zhou, XF (reprint author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
EM zhouxf@nimte.ac.cn; liuzp@nimte.ac.cn
RI Yao, Xiayin/P-3690-2014
FU Zhejiang Provincial Natural Science Foundation of China [R4100194];
   National Natural Science Foundation of China [21201173]; Key Research
   Program of the Chinese Academy of Sciences [KGZD-EW-202-4]; 973 program
   [2011CB935900]
FX We are grateful for financial support from Zhejiang Provincial Natural
   Science Foundation of China (Grant No. R4100194), National Natural
   Science Foundation of China (Grant No. 21201173), the Key Research
   Program of the Chinese Academy of Sciences (Grant No. KGZD-EW-202-4),
   and the 973 program (Grant No. 2011CB935900). We thank Mr. Saixi Yaletu
   for synthesizing the LiMn<INF>2</INF>O<INF>4</INF> cathode material and
   Mr. Huasheng Hu and Mr. Yongfeng Zeng for their helps in the fabrication
   and testing of the 18650-type full cells.
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NR 53
TC 101
Z9 102
U1 57
U2 523
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD DEC
PY 2012
VL 6
IS 12
BP 11035
EP 11043
DI 10.1021/nn304725m
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 057LA
UT WOS:000312563600068
PM 23185962
ER

PT J
AU Luo, B
   Wang, B
   Liang, MH
   Ning, J
   Li, XL
   Zhi, LJ
AF Luo, Bin
   Wang, Bin
   Liang, Minghui
   Ning, Jing
   Li, Xianglong
   Zhi, Linjie
TI Reduced Graphene Oxide-Mediated Growth of Uniform Tin-Core/Carbon-Sheath
   Coaxial Nanocables with Enhanced Lithium Ion Storage Properties
SO ADVANCED MATERIALS
LA English
DT Article
DE graphene oxide; hybrid materials; nanocables; lithium-ion batteries
ID PERFORMANCE ANODE MATERIALS; SENSITIZED SOLAR-CELLS; AT-CNT
   NANOSTRUCTURES; SN-C COMPOSITE; CARBON NANOTUBES; IN-SITU; CYCLIC
   PERFORMANCE; ONE-STEP; BATTERIES; NANOPARTICLES
AB Tin-core/carbon-sheath coaxial nanocables directly integrated into a reduced graphene oxide (RGO) surface are constructed by a new strategy involving a RGO-mediated procedure. The as-synthesized nanocables (see figure), with uniform diameter and high aspect ratio, are versatile and exhibit excellent lithium storage properties, as revealed by electrochemical evaluation.
C1 [Luo, Bin; Wang, Bin; Liang, Minghui; Ning, Jing; Li, Xianglong; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Zhi, LJ (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [20973044, 21173057];
   Ministry of Science and Technology of China [2009AA03Z328, 2009DPA41220,
   2012CB933403]; Chinese Academy of Sciences [KJCX2-YW-H21]; Guangdong-CAS
   [2009B091300007]
FX Financial support from the National Natural Science Foundation of China
   (Grant nos. 20973044, 21173057), the Ministry of Science and Technology
   of China (nos. 2009AA03Z328, 2009DPA41220, and 2012CB933403), the
   Chinese Academy of Sciences (No. KJCX2-YW-H21), and the Guangdong-CAS
   strategic cooperation Program (2009B091300007) is acknowledged.
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NR 46
TC 101
Z9 103
U1 28
U2 182
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD MAR 15
PY 2012
VL 24
IS 11
BP 1405
EP 1409
DI 10.1002/adma.201104362
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 906HT
UT WOS:000301336500004
PM 22302438
ER

PT J
AU Zhu, ZQ
   Wang, SW
   Du, J
   Jin, Q
   Zhang, TR
   Cheng, FY
   Chen, J
AF Zhu, Zhiqiang
   Wang, Shiwen
   Du, Jing
   Jin, Qi
   Zhang, Tianran
   Cheng, Fangyi
   Chen, Jun
TI Ultrasmall Sn Nanoparticles Embedded in Nitrogen-Doped Porous Carbon As
   High-Performance Anode for Lithium-Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Tin nanoparticles; nitrogen-doped porous carbon network; Sn (Salen);
   anode; Li-ion battery
ID OXYGEN-REDUCTION; ELECTROCHEMICAL PERFORMANCE; STORAGE CAPABILITY;
   COMPOSITE ANODES; GRAPHENE SHEETS; C COMPOSITE; CAPACITY; LI;
   NANOCRYSTALS; SILICON
AB In this Letter, we reported on the preparation and Li-ion battery anode application of ultrasmall Sn nanoparticles (similar to 5 nm) embedded in nitrogen-doped porous carbon network (denoted as 5-Sn/C). Pyrolysis of Sn(Salen) at 650 degrees C under Ar atmosphere was carried out to prepare N-doped porous 5-Sn/C with the BET specific surface area of 286.3 m(2) g(-1). The 5-Sn/C showed an initial discharge capacity of 1014 mAh g(-1) and a capacity retention of 722 mAh g(-1) after 200 cycles at the current density of 0.2 A g(-1). Furthermore, a reversible capacity of similar to 480 mAh was obtained at much higher current density of 5 A g(-1). The remarkable electrochemical performance of 5-Sn/C was attributed to the effective combination of ultrasmall Sn nanoparticles, uniform distribution, and porous carbon network structure, which simultaneously solved the major problems of pulverization, loss of electrical contact, and particle aggregation facing Sn anode.
C1 [Chen, Jun] Nankai Univ, Key Lab Adv Energy Mat Chem, Minist Educ, Coll Chem, Tianjin 300071, Peoples R China.
   Nankai Univ, Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300071, Peoples R China.
RP Chen, J (reprint author), Nankai Univ, Key Lab Adv Energy Mat Chem, Minist Educ, Coll Chem, Tianjin 300071, Peoples R China.
EM chenabc@nankai.edu.cn
RI Chen, Jun/D-4873-2016
FU Programs of National 973 [2011CB935900]; NSFC [51231003, 21322101]; MOE
   [B12015, 113016A]
FX This work was supported by the Programs of National 973 (2011CB935900),
   NSFC (51231003 and 21322101), and MOE (B12015 and 113016A).
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NR 46
TC 99
Z9 99
U1 86
U2 463
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD JAN
PY 2014
VL 14
IS 1
BP 153
EP 157
DI 10.1021/nl403631h
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 288BJ
UT WOS:000329586700025
PM 24328829
ER

PT J
AU Ren, YL
   Wu, HY
   Lu, MM
   Chen, YJ
   Zhu, CL
   Gao, P
   Cao, MS
   Li, CY
   Ouyang, QY
AF Ren, Yu-Lan
   Wu, Hong-Yu
   Lu, Ming-Ming
   Chen, Yu-Jin
   Zhu, Chun-Ling
   Gao, Peng
   Cao, Mao-Sheng
   Li, Chun-Yan
   Ouyang, Qiu-Yun
TI Quaternary Nanocomposites Consisting of Graphene, Fe3O4@Fe Core@Shell,
   and ZnO Nanoparticles: Synthesis and Excellent Electromagnetic
   Absorption Properties
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE graphene; Fe3O4; Fe; ZnO; quaternary nanocomposites; electromagnetic
   absorption
ID LITHIUM ION BATTERIES; CORE/SHELL NANORODS SYNTHESIS;
   MICROWAVE-ABSORPTION; CARBON NANOTUBES; ANODE MATERIAL; REVERSIBLE
   CAPACITY; TERNARY COMPOSITES; X-BAND; PERFORMANCE; OXIDE
AB This paper presents for the first time a successful synthesis of quaternary nanocomposites consisting of graphene, Fe3O4@Fe core/shell nanopariticles, and ZnO nanoparticles. Transmission electron microscopy measurements show that the diameter of the Fe3O4@Fe core/shell nanoparitcles is about 18 nm, the Fe3O4 shell's thickness is about 5 nm, and the diameter of ZnO nanoparticles is in range of 2-10 nm. The measured electromagnetic parameters show that the absorption bandwidth with reflection loss less than 20 dB is up to 7.3 GHz, and in the band range more than 99% of electromagnetic wave energy is attenuated. Moreover, the addition amount of the nanocomposites in the matrix is only 20 wt %. Therefore, the excellent electromagnetic absorption properties with lightweight and wide absorption frequency band are realized by the nanocomposites.
C1 [Ren, Yu-Lan; Wu, Hong-Yu; Chen, Yu-Jin; Li, Chun-Yan; Ouyang, Qiu-Yun] Harbin Engn Univ, Coll Sci, Harbin, Peoples R China.
   [Zhu, Chun-Ling; Gao, Peng] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin, Peoples R China.
   [Lu, Ming-Ming; Cao, Mao-Sheng] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
RP Chen, YJ (reprint author), Harbin Engn Univ, Coll Sci, Harbin, Peoples R China.
EM chenyujin@hrbeu.edu.cn; gaopeng@mail.neu.edu.cn
OI Cao, Mao-Sheng/0000-0001-6810-9422
FU National Natural Science Foundation of China [51072038, 51272050,
   61205113, 51172275, 21001035]; Program for New Century Excellent Talents
   in University [NECT-10-0049]; Outstanding Youth Foundation of
   Heilongjiang Province [JC201008]
FX We thank the National Natural Science Foundation of China (Grants
   51072038, 51272050, 61205113, 51172275, and 21001035), Program for New
   Century Excellent Talents in University (NECT-10-0049), and Outstanding
   Youth Foundation of Heilongjiang Province (Grant JC201008) for the
   financial support of this research.
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NR 55
TC 99
Z9 100
U1 56
U2 302
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD DEC
PY 2012
VL 4
IS 12
BP 6436
EP 6442
DI 10.1021/am3021697
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 065LM
UT WOS:000313149800007
PM 23176086
ER

PT J
AU Huang, XL
   Wang, RZ
   Xu, D
   Wang, ZL
   Wang, HG
   Xu, JJ
   Wu, Z
   Liu, QC
   Zhang, Y
   Zhang, XB
AF Huang, Xiao-lei
   Wang, Ru-zhi
   Xu, Dan
   Wang, Zhong-li
   Wang, Heng-guo
   Xu, Ji-jing
   Wu, Zhong
   Liu, Qing-chao
   Zhang, Yu
   Zhang, Xin-bo
TI Homogeneous CoO on Graphene for Binder-Free and Ultralong-Life Lithium
   Ion Batteries
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE Li-ion batteries; anodes; binder-free electrodes; graphene
ID HIGH-CAPACITY; ELECTROCHEMICAL LITHIATION; ANODE MATERIAL; PERFORMANCE;
   OXIDE; NANOWIRES; ELECTRODE; STORAGE
AB Ultralong cycle life, high energy, and power density rechargeable lithium-ion batteries are crucial to the ever-increasing large-scale electric energy storage for renewable energy and sustainable road transport. However, the commercial graphite anode cannot perform this challenging task due to its low theoretical capacity and poor rate-capability performance. Metal oxides hold much higher capacity but still are plagued by low rate capability and serious capacity degradation. Here, a novel strategy is developed to prepare binder-free and mechanically robust CoO/graphene electrodes, wherein homogenous and full coating of -Co(OH)(2) nanosheets on graphene, through a novel electrostatic induced spread growth method, plays a key role. The combined advantages of large 2D surface and moderate inflexibility of the as-obtained -Co(OH)(2)/graphene hybrid enables its easy coating on Cu foil by a simple layer-by-layer stacking process. Devices made with these electrodes exhibit high rate capability over a temperature range from 0 to 55 degrees C and, most importantly, maintain excellent cycle stability up to 5000 cycles even at a high current density.
C1 [Huang, Xiao-lei; Xu, Dan; Wang, Zhong-li; Wang, Heng-guo; Xu, Ji-jing; Wu, Zhong; Liu, Qing-chao; Zhang, Xin-bo] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Huang, Xiao-lei; Wu, Zhong] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
   [Wang, Ru-zhi] Beijing Univ Technol, Coll Mat Sci & Engn, Beijing 100124, Peoples R China.
   [Zhang, Yu] Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China.
RP Huang, XL (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
EM jade@buaa.edu.cn; xbzhang@ciac.jl.cn
RI Zhang, Yu/A-5935-2010; ZHANG, Xinbo/G-8698-2011; XiaoLei,
   Huang/I-3210-2014
OI ZHANG, Xinbo/0000-0002-5806-159X; XiaoLei, Huang/0000-0002-2211-4813
FU Chinese Academy of Sciences; National Program on Key Basic Research
   Project of China (973 Program) [2012CB215500]; National Natural Science
   Foundation of China [21101147, 21203176]; China Postdoctoral Science
   Foundation [2011M500624]; Special Foundation of China Postdoctoral
   Science [2012T50293]
FX This work was financially supported by 100 Talents Programme of The
   Chinese Academy of Sciences, National Program on Key Basic Research
   Project of China (973 Program, Grant No. 2012CB215500), National Natural
   Science Foundation of China (Grant No. 21101147 and 21203176), China
   Postdoctoral Science Foundation (2011M500624), and Special Foundation of
   China Postdoctoral Science (2012T50293).
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NR 45
TC 98
Z9 102
U1 42
U2 213
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD SEP 20
PY 2013
VL 23
IS 35
BP 4345
EP 4353
DI 10.1002/adfm.201203777
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 258XU
UT WOS:000327492800013
ER

PT J
AU Ji, LW
   Zhang, XW
AF Ji, Liwen
   Zhang, Xiangwu
TI Fabrication of porous carbon nanofibers and their application as anode
   materials for rechargeable lithium-ion batteries
SO NANOTECHNOLOGY
LA English
DT Article
ID SECONDARY BATTERIES; FIBERS; PERFORMANCE; MORPHOLOGIES; INSERTION;
   SURFACES; POLYMER; BLENDS; WEBS
AB Porous carbon nanofibers were prepared by the electrospinning of a bicomponent polymer solution, followed by thermal treatments under different atmospheres. The surface morphology, thermal properties, and crystalline features of these nanofibers were characterized using various analytic techniques, and it was found that they were formed with turbostratically disordered graphene sheets and had small pores and large surface areas. The unique structure of these porous carbon nanofibers resulted in good electrochemical performance such as high reversible capacity and good cycle stability when they were used as anodes for rechargeable lithium-ion batteries.
C1 [Ji, Liwen; Zhang, Xiangwu] N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
RP Zhang, XW (reprint author), N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
EM xiangwu_zhang@ncsu.edu
RI Zhang, Xiangwu/F-1013-2011
OI Zhang, Xiangwu/0000-0002-6236-6281
FU US National Science Foundation [0555959]; National Science Foundation
   under Award [EEC-08212121]; ACS Petroleum Research Fund [47863-G10]
FX This work was supported by the US National Science Foundation (No.
   0555959), the ERC Program of the National Science Foundation under Award
   Number EEC-08212121, and ACS Petroleum Research Fund 47863-G10. The
   authors also thank Mr Andrew J Medford for his help in sample
   characterizations.
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NR 26
TC 98
Z9 101
U1 22
U2 92
PU IOP PUBLISHING LTD
PI BRISTOL
PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND
SN 0957-4484
J9 NANOTECHNOLOGY
JI Nanotechnology
PD APR 15
PY 2009
VL 20
IS 15
AR 155705
DI 10.1088/0957-4484/20/15/155705
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
   Physics, Applied
SC Science & Technology - Other Topics; Materials Science; Physics
GA 424BD
UT WOS:000264539600019
PM 19420557
ER

PT J
AU Mahmood, N
   Zhang, CZ
   Hou, YL
AF Mahmood, Nasir
   Zhang, Chenzhen
   Hou, Yanglong
TI Nickel Sulfide/Nitrogen-Doped Graphene Composites: Phase-Controlled
   Synthesis and High Performance Anode Materials for Lithium Ion Batteries
SO SMALL
LA English
DT Article
DE phase-controlled synthesis; Ni3S4; NiS1; 03; nitrogen-doped graphene;
   lithium ion batteries
ID OXYGEN REDUCTION REACTION; SULFIDE NANOSTRUCTURES; ENERGY-CONVERSION;
   STORAGE; NANOPARTICLES; CAPACITY; NI3S4; OXIDE; NANOWIRES; CATALYST
C1 [Mahmood, Nasir; Zhang, Chenzhen; Hou, Yanglong] Peking Univ, Dept Mat Sci & Engn, Coll Engn, Beijing 100871, Peoples R China.
RP Hou, YL (reprint author), Peking Univ, Dept Mat Sci & Engn, Coll Engn, Beijing 100871, Peoples R China.
EM hou@pku.edu.cn
RI Hou, Yanglong/B-8688-2012
FU NSFC [51125001, 51172005]; Beijing Natural Science Foundation [2122022];
   Aerostatic Science Foundation [2010ZF71003]; New Century Excellent
   Talent of the Ministry of Education of China [NCET-09-0177]; Fok Ying
   Tong Foundation [122043]
FX This work was supported by the NSFC (51125001, 51172005), Beijing
   Natural Science Foundation (2122022), Aerostatic Science Foundation
   (2010ZF71003), New Century Excellent Talent of the Ministry of Education
   of China (NCET-09-0177) and Fok Ying Tong Foundation (122043).
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NR 48
TC 97
Z9 97
U1 40
U2 306
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
J9 SMALL
JI Small
PD APR 22
PY 2013
VL 9
IS 8
SI SI
BP 1321
EP 1328
DI 10.1002/smll.201203032
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 127HS
UT WOS:000317689600015
PM 23494938
ER

PT J
AU Chen, ZX
   Zhou, M
   Cao, YL
   Ai, XP
   Yang, HX
   Liu, J
AF Chen, Zhongxue
   Zhou, Min
   Cao, Yuliang
   Ai, Xinping
   Yang, Hanxi
   Liu, Jun
TI In Situ Generation of Few-Layer Graphene Coatings on SnO2-SiC Core-Shell
   Nanoparticles for High-Performance Lithium-Ion Storage
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
DE tin oxide; few-layer graphene; conversion reactions; core-shell
   nanostructures; lithium-ion batteries
ID ELECTROCHEMICAL LITHIATION; ELECTRODE MATERIALS; AMORPHOUS OXIDE; ANODE
   MATERIAL; BATTERIES; CAPACITY; CARBON; TIN; COMPOSITE; NANOSTRUCTURES
AB A simple ball-milling method is used to synthesize a tin oxide-silicon carbide/few-layer graphene core-shell structure in which nanometer-sized SnO2 particles are uniformly dispersed on a supporting SiC core and encapsulated with few-layer graphene coatings by in situ mechanical peeling. The SnO2-SiC/G nanocomposite material delivers a high reversible capacity of 810 mA h g-1 and 83% capacity retention over 150 charge/discharge cycles between 1.5 and 0.01 V at a rate of 0.1 A g-1. A high reversible capacity of 425 mA h g-1 also can be obtained at a rate of 2 A g-1. When discharged (Li extraction) to a higher potential at 3.0 V (vs. Li/Li+), the SnO2-SiC/G nanocomposite material delivers a reversible capacity of 1451 mA h g-1 (based on the SnO2 mass), which corresponds to 97% of the expected theoretical capacity (1494 mA h g-1, 8.4 equivalent of lithium per SnO2), and exhibits good cyclability. This result suggests that the core-shell nanostructure can achieve a completely reversible transformation from Li4.4Sn to SnO2 during discharging (i.e., Li extraction by dealloying and a reversible conversion reaction, generating 8.4 electrons). This suggests that simple mechanical milling can be a powerful approach to improve the stability of high-performance electrode materials involving structural conversion and transformation.
C1 [Chen, Zhongxue; Zhou, Min; Cao, Yuliang; Ai, Xinping; Yang, Hanxi] Wuhan Univ, Coll Chem & Mol Sci, Hubei Key Lab Electrochem Power Sources, Wuhan 430072, Peoples R China.
   [Cao, Yuliang; Liu, Jun] Pacific NW Natl Lab, Richland, WA 99352 USA.
RP Cao, YL (reprint author), Wuhan Univ, Coll Chem & Mol Sci, Hubei Key Lab Electrochem Power Sources, Wuhan 430072, Peoples R China.
EM ylcao@whu.edu.cn; Jun.Liu@pnl.gov
RI Chen, Zhongxue/J-9070-2014
FU National Basic Research Program of China [2009CB220100]; National
   Science Foundation of China [21173160]; National High Technology
   Development Program of China (863) [2011AA11A254]; U.S. Department of
   Energy (DOE), Office of Basic Energy Sciences, Division of Materials
   Sciences and Engineering [KC020105-FWP12152]; DOE by Battelle
   [DE-AC05-76RL01830]
FX The authors are grateful for the financial support provided by the
   National Basic Research Program of China (2009CB220100) the National
   Science Foundation of China (No. 21173160), and the National High
   Technology Development Program of China (863, No. 2011AA11A254), and
   also the support from the U.S. Department of Energy (DOE), Office of
   Basic Energy Sciences, Division of Materials Sciences and Engineering,
   under Award KC020105-FWP12152. The authors also thank Dr. B. Schwenzer
   for her helpful suggestions. Pacific Northwest National Laboratory is a
   multiprogram national laboratory operated for DOE by Battelle under
   Contract DE-AC05-76RL01830.
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NR 53
TC 97
Z9 101
U1 33
U2 169
PU WILEY PERIODICALS, INC
PI MALDEN
PA COMMERCE PLACE, 350 MAIN STREET, MALDEN, MA 02148-529 USA
SN 1614-6832
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD JAN
PY 2012
VL 2
IS 1
BP 95
EP 102
DI 10.1002/aenm.201100464
PG 8
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA 874UB
UT WOS:000298982500014
ER

PT J
AU Liao, JY
   Higgins, D
   Lui, G
   Chabot, V
   Xiao, XC
   Chen, ZW
AF Liao, Jin-Yun
   Higgins, Drew
   Lui, Gregory
   Chabot, Victor
   Xiao, Xingcheng
   Chen, Zhongwei
TI Multifunctional TiO2-C/MnO2 Core-Double-Shell Nanowire Arrays as
   High-Performance 3D Electrodes for Lithium Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Li-ion batteries; core-shell; TiO2; MnO2; nanowire; 3D
ID ELECTROCHEMICAL ENERGY-STORAGE; COMPOSITE ELECTRODES; CATHODE MATERIALS;
   HIGH-CAPACITY; HIGH-POWER; ANODE; TIO2; NANOTUBE; NANOSTRUCTURES;
   GRAPHENE/MNO2
AB The unique TiO2-C/MnO2 core-double-shell nanowires are synthesized for the first time using as anode materials for lithium ion batteries (LIBs). They combine both advantages from TiO2 such as excellent cycle stability and MnO2 with high capacity (1230 mA h g(-1)). The additional C interlayer intends to improve the electrical conductivity. The self-supported nanowire arrays grown directly on current-collecting substrates greatly simplify the fabrication processing of electrodes without applying binder and conductive additives. Each nanowire is anchored to the current collector, leading to fast charge transfer. The unique one-dimensional core-double-shell nanowires exhibit enhanced electrochemical performance with a higher discharge/charge capacity, superior rate capability, and longer cycling lifetime.
C1 [Liao, Jin-Yun; Higgins, Drew; Lui, Gregory; Chabot, Victor; Chen, Zhongwei] Univ Waterloo, Waterloo Inst Nanotechnol, Dept Chem Engn, Waterloo, ON N2L 3G1, Canada.
   [Xiao, Xingcheng] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
RP Xiao, XC (reprint author), Gen Motors Global Res & Dev Ctr, 30500 Mound Rd, Warren, MI 48090 USA.
EM xingcheng.xiao@gm.com; zhwchen@uwaterloo.ca
RI chen, zhongwei/A-5605-2015; Liao, Jin-Yun/E-3798-2013
FU Natural Sciences and Engineering Research Council of Canada (NSERC);
   University of Waterloo; Waterloo Institute for Nanotechnology
FX This work was financially supported by the Natural Sciences and
   Engineering Research Council of Canada (NSERC), the University of
   Waterloo and the Waterloo Institute for Nanotechnology. The authors
   thank Mr. Hey Woong Park, Mr. Drew Higgins, Mr. Victor Chabot, and Mr.
   Gregory Lui at the University of Waterloo for their help in editing the
   manuscript.
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NR 42
TC 96
Z9 96
U1 59
U2 337
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5467
EP 5473
DI 10.1021/nl4030159
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 253TH
UT WOS:000327111700075
PM 24079359
ER

PT J
AU Xu, CH
   Sun, J
   Gao, L
AF Xu, Chaohe
   Sun, Jing
   Gao, Lian
TI Direct growth of monodisperse SnO2 nanorods on graphene as high capacity
   anode materials for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID GRAPHITE OXIDE SHEETS; ONE-POT SYNTHESIS; STORAGE PROPERTIES; HOLLOW
   SPHERES; NANOPARTICLES; PERFORMANCE; COMPOSITE; ELECTRODES; REDUCTION;
   FABRICATION
AB We developed a facile one-step hydrothermal procedure to prepare hybrid materials of SnO2 nanorods on graphene sheets (GS). Composites with individual SnO2 nanorods of 10-20 nm in diameter and 100-200 nm in length show a high reversible specific capacity and outstanding cycling stability (710 mAh g(-1)) as anode materials for lithium ion batteries. Owing to the enhanced lithium storage properties, the SnO2/GS hybrid could be a promising candidate material for a high-capacity, low cost and environmentally friendly anode for lithium ion batteries (LIBs). This one-step hydrothermal procedure provides a facile technique for the design and morphology control of nanocrystals on GS and will be a versatile route in producing metal oxide/GS composites.
C1 [Xu, Chaohe; Sun, Jing; Gao, Lian] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
RP Sun, J (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, 1295 Dingxi Rd, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn; liagao@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU National Natural Science Foundation of China [50972153, 509721157,
   51072215]; Shanghai Municipal Committee of science and technology
   [10DZ0505000]
FX This work is supported by the National Natural Science Foundation of
   China (Grant No. 50972153, 509721157 and 51072215) and Shanghai
   Municipal Committee of science and technology (Grant No. 10DZ0505000).
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   Xu CH, 2009, J PHYS CHEM C, V113, P20509, DOI 10.1021/jp909740h
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NR 52
TC 96
Z9 98
U1 16
U2 110
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 3
BP 975
EP 979
DI 10.1039/c1jm14099j
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 877WF
UT WOS:000299212700028
ER

PT J
AU Chang, K
   Wang, Z
   Huang, GC
   Li, H
   Chen, WX
   Lee, JY
AF Chang, Kun
   Wang, Zhen
   Huang, Guochuang
   Li, He
   Chen, Weixiang
   Lee, Jim Yang
TI Few-layer SnS2/graphene hybrid with exceptional electrochemical
   performance as lithium-ion battery anode
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Few-layer; Solution-phase; Tin disulfide/graphene hybrid; Defect sites;
   Lithium ion battery; Anode material
ID GRAPHENE; STORAGE; SNS2; CAPACITY; OXIDE
AB Here we develop a facile process for preparing few-layer SnS2/graphene (FL-SnS2/G) hybrid by solution-phase method employing L-cysteine as a complexing, sulfide source and reducing agent. The FL-SnS2/G hybrid is characterized by XRD, SEM and HRTEM. It is demonstrated that the few-layer SnS2 with defects or disorder structure supports on graphene surface. Electrochemical tests show the FL-SnS2/G hybrid exhibits an extraordinary capacity of up to 920 mAh g(-1) with excellent cycling stability and high-rate capability. The significant improvement in the electrochemical performances is attributed to the robust composite structure and some synergistic interactions between few-layer SnS2 and graphene. Electrochemical impedance spectra confirm that the incorporation of graphene considerably improved the electric conductivity and electron rapid transfer of the FL-SnS2/G hybrid. Therefore, this new kind of FL-SnS2/G hybrid can be used as a promising anode material for lithium ion batteries. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Chang, Kun; Wang, Zhen; Huang, Guochuang; Li, He; Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
   [Lee, Jim Yang] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 119260, Singapore.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
EM weixiangchen@zju.edu.cn
RI LEE, Jim Yang/E-5904-2010; Chang, Kun/I-1361-2012
FU Natural Science Foundation of China [21173190]; Program for
   International Science and Technology Cooperation Projects of China (the
   8th Science and Technology Cooperation Projects of China-Singapore)
   [S2012GR0025]; Program from Science and Technology Department of
   Zhejiang Province [2011G210024]; Research Fund for the Doctoral Program
   of Higher Education of China [20050335086]; Zhejiang Provincial Natural
   Science Foundation of China [Y4100119]; Ministry of Science and
   Technology of China [2010CB635116]
FX This work was supported by the Natural Science Foundation of China
   (21173190), the Program for International Science and Technology
   Cooperation Projects of China (the 8th Science and Technology
   Cooperation Projects of China-Singapore, S2012GR0025), the Program from
   Science and Technology Department of Zhejiang Province (2011G210024),
   the Research Fund for the Doctoral Program of Higher Education of China
   (20050335086). the Zhejiang Provincial Natural Science Foundation of
   China (Y4100119), and 973 Fundamental Research Program from the Ministry
   of Science and Technology of China (2010CB635116).
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NR 35
TC 95
Z9 96
U1 29
U2 196
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD MAR 1
PY 2012
VL 201
BP 259
EP 266
DI 10.1016/j.jpowsour.2011.10.132
PG 8
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 892CN
UT WOS:000300264400035
ER

PT J
AU Zhao, GX
   Wen, T
   Chen, CL
   Wang, XK
AF Zhao, Guixia
   Wen, Tao
   Chen, Changlun
   Wang, Xiangke
TI Synthesis of graphene-based nanomaterials and their application in
   energy-related and environmental-related areas
SO RSC ADVANCES
LA English
DT Review
ID LITHIUM-ION BATTERIES; CHEMICAL-VAPOR-DEPOSITION; SOLUTION-PROCESSABLE
   GRAPHENE; PERFORMANCE ANODE MATERIALS; ORGANIC SOLAR-CELLS; ONE-STEP
   SYNTHESIS; ONE-POT SYNTHESIS; CARBON NANOTUBES; GRAPHITE OXIDE;
   LOW-TEMPERATURE
AB As a fascinating two-dimensional carbon allotrope, graphene has triggered a 'gold rush' all over scientific research areas especially since the Nobel Prize for Physics in 2010. To exploit the prominent properties of graphene-based nanomaterials, two important problems are focused in this review: one is the synthesis of these graphene-based nanomaterials with different kinds of well-defined structures, and the other is the effective application of them as active nanomaterials in functional devices or processes. In this critical review, from the viewpoint of chemistry and materials, we give a brief overview of the recent significant advances in the synthesis of graphene-based nanomaterials and their applications in energy-related areas and environmental pollution remediation areas, including supercapacitors, lithium ion batteries, solar cells, adsorption, and degradation of organic/inorganic pollutants from large volumes of aqueous solutions in environmental pollution cleanup. The main challenges and perspectives of the materials for future research are also discussed.
C1 [Zhao, Guixia; Wen, Tao; Chen, Changlun; Wang, Xiangke] Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China.
RP Zhao, GX (reprint author), Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China.
EM xkwang@ipp.ac.cn
RI Chen, Changlun/H-9177-2012; ZHAO, GUIXIA/J-3036-2014; Wang,
   Xiangke/I-5806-2012
OI Wang, Xiangke/0000-0002-3352-1617
FU MOST [2011CB933700]; NSFC [20971126, 21071147, 21071107, 91126020]; open
   foundation of State Key Lab of Pollution Control and Resource Reuse
FX Financial support from 973 projects of MOST (2011CB933700), NSFC
   (20971126, 21071147, 21071107, 91126020), and open foundation of State
   Key Lab of Pollution Control and Resource Reuse are acknowledged.
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NR 204
TC 95
Z9 97
U1 35
U2 254
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 25
BP 9286
EP 9303
DI 10.1039/c2ra20990j
PG 18
WC Chemistry, Multidisciplinary
SC Chemistry
GA 050NS
UT WOS:000312061000002
ER

PT J
AU Du, ZF
   Yin, XM
   Zhang, M
   Hao, QY
   Wang, YG
   Wang, TH
AF Du, Zhifeng
   Yin, Xiaoming
   Zhang, Ming
   Hao, Quanyi
   Wang, Yanguo
   Wang, Taihong
TI In situ synthesis of SnO2/graphene nanocomposite and their application
   as anode material for lithium ion battery
SO MATERIALS LETTERS
LA English
DT Article
DE SnO2; Nanomaterials; Graphene; Nanocomposite; Lithium ion battery
ID STORAGE CAPACITY; FILMS; OXIDE
AB SnO2/graphene nanocomposite was prepared via an in situ chemical synthesis method. The nanocomposite was characterized by X-ray diffraction, filed emission scanning electron microscope and transmission electron microscope, which revealed that tiny SnO2 nanoparticles could be homogeneously distributed on the graphene matrix. The electrochemical performance of the SnO2/graphene nanocomposite as anode material was measured by galvanostatic charge/discharge cycling. The SnO2/graphene nanocomposite showed a reversible capacity of 665 mAh/g after 50 cycles and an excellent cycling performance for lithium ion battery, which was ascribed to the three-dimensional architecture of SnO2/graphene nanocomposite. These results suggest that SnO2/graphene nanocomposite would be a promising anode material for lithium ion battery. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Wang, Taihong] Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
RP Wang, TH (reprint author), Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM thwang@hnu.cn
RI Wang, Taihong/K-8968-2012; Zhang, Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU "973" National Key Basic Research Program of China [2007CB310500];
   Chinese Ministry of Education [705040]; National Natural Science
   Foundation of China [90606009]
FX This work was partly supported from "973" National Key Basic Research
   Program of China (Grant No. 2007CB310500), Chinese Ministry of Education
   (Grant No. 705040), and National Natural Science Foundation of China
   (Grant No. 90606009).
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NR 13
TC 95
Z9 100
U1 6
U2 80
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0167-577X
J9 MATER LETT
JI Mater. Lett.
PD OCT 15
PY 2010
VL 64
IS 19
BP 2076
EP 2079
DI 10.1016/j.matlet.2010.06.039
PG 4
WC Materials Science, Multidisciplinary; Physics, Applied
SC Materials Science; Physics
GA 647DB
UT WOS:000281595100013
ER

PT J
AU Shi, YM
   Wang, Y
   Wong, JI
   Tan, AYS
   Hsu, CL
   Li, LJ
   Lu, YC
   Yang, HY
AF Shi, Yumeng
   Wang, Ye
   Wong, Jen It
   Tan, Alex Yuan Sheng
   Hsu, Chang-Lung
   Li, Lain-Jong
   Lu, Yi-Chun
   Yang, Hui Ying
TI Self-assembly of hierarchical MoSx/CNT nanocomposites (2 < x < 3):
   towards high performance anode materials for lithium ion batteries
SO SCIENTIFIC REPORTS
LA English
DT Article
ID MOS2 THIN-LAYERS; HYDROGEN EVOLUTION; ELECTROCHEMICAL PERFORMANCES;
   ASSISTED SYNTHESIS; CARBON NANOTUBES; LARGE-AREA; GRAPHENE; STORAGE;
   COMPOSITES; NANOPARTICLES
AB Two dimension (2D) layered molybdenum disulfide (MoS2) has emerged as a promising candidate for the anode material in lithium ion batteries (LIBs). Herein, 2D MoSx (2 <= x <= 3) nanosheet-coated 1D multiwall carbon nanotubes (MWNTs) nanocomposites with hierarchical architecture were synthesized via a high-throughput solvent thermal method under low temperature at 2006 degrees C. The unique hierarchical nanostructures with MWNTs backbone and nanosheets of MoSx have significantly promoted the electrode performance in LIBs. Every single MoSx nanosheet interconnect to MWNTs centers with maximized exposed electrochemical active sites, which significantly enhance ion diffusion efficiency and accommodate volume expansion during the electrochemical reaction. A remarkably high specific capacity (i.e., >1000 mAh/g) was achieved at the current density of 50 mA g(-1), which is much higher than theoretical numbers for either MWNTs or MoS2 along (similar to 372 and similar to 670 mAh/g, respectively). We anticipate 2D nanosheets/1D MWNTs nanocomposites will be promising materials in new generation practical LIBs.
C1 [Shi, Yumeng; Wang, Ye; Wong, Jen It; Tan, Alex Yuan Sheng; Yang, Hui Ying] Singapore Univ Technol & Design, Singapore 138682, Singapore.
   [Hsu, Chang-Lung; Li, Lain-Jong] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan.
   [Hsu, Chang-Lung] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 300, Taiwan.
   [Li, Lain-Jong] Natonal Tsing Hua Univ, Dept Phys, Hsinchu 300, Taiwan.
   [Lu, Yi-Chun] Chinese Univ Hong Kong, Dept Mech & Automat Engn, Hong Kong, Hong Kong, Peoples R China.
RP Yang, HY (reprint author), Singapore Univ Technol & Design, Singapore 138682, Singapore.
EM yanghuiying@sutd.edu.sg
RI Li, Lain-Jong/D-5244-2011; Lu, Yi-Chun/J-1841-2015; Shi,
   Yumeng/A-7349-2012
OI Li, Lain-Jong/0000-0002-4059-7783; Lu, Yi-Chun/0000-0003-1607-1615; Shi,
   Yumeng/0000-0002-9623-3778
FU SMART innovation grant; SUTD-ZJU research grant [ZJURP1100104]
FX This work is supported by SMART innovation grant and SUTD-ZJU research
   grant ZJURP1100104.
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   BAKER MA, APPL SURF SCI, V150, P255
NR 52
TC 93
Z9 93
U1 40
U2 319
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2045-2322
J9 SCI REP-UK
JI Sci Rep
PD JUL 9
PY 2013
VL 3
AR UNSP 2169
DI 10.1038/srep02169
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 179AJ
UT WOS:000321488600005
PM 23835645
ER

PT J
AU Lei, C
   Han, F
   Li, D
   Li, WC
   Sun, Q
   Zhang, XQ
   Lu, AH
AF Lei, Cheng
   Han, Fei
   Li, Duo
   Li, Wen-Cui
   Sun, Qiang
   Zhang, Xiang-Qian
   Lu, An-Hui
TI Dopamine as the coating agent and carbon precursor for the fabrication
   of N-doped carbon coated Fe3O4 composites as superior lithium ion anodes
SO NANOSCALE
LA English
DT Article
ID CONTROLLED ALPHA-FE2O3 NANOPARTICLES; HIGH ELECTROCHEMICAL PERFORMANCE;
   ONE-POT SYNTHESIS; STORAGE CAPABILITY; BATTERIES; NANOCRYSTALS;
   GRAPHENE; NITROGEN; PYROLYSIS; STABILITY
AB Dopamine is an excellent and flexible agent for surface coating of inorganic nanoparticles and contains unusually high concentrations of amine groups. In this study, we demonstrate that through a controlled coating of a thin layer of polydopamine on the surface of alpha-Fe2O3 in the dopamine aqueous solution, followed by subsequent carbonization, N-doped carbon-encapsulated magnetite has been synthesized and shows excellent electrochemical performance as anode material for lithium-ion batteries. Due to the strong binding affinity to iron oxide and excellent coating capability of this new carbon precursor, the conformal polydopamine derived carbon is continuous and uniform, and its thickness can be tailored. Moreover, due to the high percentage of nitrogen content in the precursor, the resulting carbon layer contains a moderate amount of N species, which can substantially improve the electrochemical performance. The composites synthesized by this facile method exhibit superior electrochemical performance, including remarkably high specific capacity (>800 mA h g(-1) at a current of 500 mA g(-1)), high rate capability (595 and 396 mA h g(-1) at a current of 1000 and 2000 mA g(-1), respectively) and excellent cycle performance (200 cycles with 99% capacity retention), which adds to the potential as promising anodes for the application in lithium-ion batteries.
C1 [Lei, Cheng; Han, Fei; Li, Duo; Li, Wen-Cui; Sun, Qiang; Zhang, Xiang-Qian; Lu, An-Hui] Dalian Univ Technol, Fac Chem Environm & Biol Sci & Technol, Sch Chem Engn, State Key Lab Fine Chem, Dalian 116024, Peoples R China.
RP Lu, AH (reprint author), Dalian Univ Technol, Fac Chem Environm & Biol Sci & Technol, Sch Chem Engn, State Key Lab Fine Chem, Dalian 116024, Peoples R China.
EM anhuilu@dlut.edu.cn
FU Fundamental Research Funds for the Central Universities [DUT12ZD218];
   Program for New Century Excellent Talents in University of China
   [NCET-08-0075]; PhD Programs Foundation of the Ministry of Education of
   China [20100041110017]
FX The project was supported by the Fundamental Research Funds for the
   Central Universities (DUT12ZD218), the Program for New Century Excellent
   Talents in University of China (NCET-08-0075), and the PhD Programs
   Foundation (20100041110017) of the Ministry of Education of China.
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NR 54
TC 93
Z9 94
U1 55
U2 420
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 3
BP 1168
EP 1175
DI 10.1039/c2nr33043a
PG 8
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 074HH
UT WOS:000313803000046
PM 23292140
ER

PT J
AU Zhou, XS
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Wan, Li-Jun
   Guo, Yu-Guo
TI Facile synthesis of MoS2@CMK-3 nanocomposite as an improved anode
   material for lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID STORAGE PROPERTIES; INTERCALATION CHEMISTRY; MOLYBDENUM-DISULFIDE;
   SUPERIOR-PERFORMANCE; MESOPOROUS CARBON; MOS2; NANOPARTICLES; GRAPHENE;
   NANOSHEETS; NANOSTRUCTURES
AB MoS2@CMK-3 nanocomposite consisting of confined nanosized MoS2 in CMK-3 carbon matrix exhibits much improved cycling performance and rate capability due to the enlarged interlayer distance and favorable conductivity.
C1 [Zhou, Xiaosi; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, BNLMS, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, BNLMS, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2009CB930400,
   2012CB932900]; National Natural Science Foundation of China [91127044,
   21127901, 21121063]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant no. 2011CB935700, 2009CB930400 and 2012CB932900), the National
   Natural Science Foundation of China (Grant no. 91127044, 21127901 and
   21121063), and the Chinese Academy of Sciences.
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NR 40
TC 93
Z9 94
U1 35
U2 188
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 19
BP 5868
EP 5871
DI 10.1039/c2nr31822a
PG 4
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 004UF
UT WOS:000308705900013
PM 22948608
ER

PT J
AU Rui, XH
   Zhu, JX
   Sim, D
   Xu, C
   Zeng, Y
   Hng, HH
   Lim, TM
   Yan, QY
AF Rui, Xianhong
   Zhu, Jixin
   Sim, Daohao
   Xu, Chen
   Zeng, Yi
   Hng, Huey Hoon
   Lim, Tuti Mariana
   Yan, Qingyu
TI Reduced graphene oxide supported highly porous V2O5 spheres as a
   high-power cathode material for lithium ion batteries
SO NANOSCALE
LA English
DT Article
ID HIGH-PERFORMANCE; ELECTRODE MATERIALS; CYCLIC PERFORMANCE; ANODE
   MATERIAL; CAPACITY; INTERCALATION; STORAGE; SHEETS; NANOPARTICLES;
   NANOWIRES
AB Reduced graphene oxide (rGO) supported highly porous polycrystalline V2O5 spheres (V2O5/rGO) were prepared by using a solvothermal approach followed by an annealing process. Initially, reduced vanadium oxide (rVO) nanoparticles with sizes in the range of 10-50 nm were formed through heterogeneous nucleation on rGO sheets during the solvothermal process. These rVO nanoparticles were oxidized to V2O5 after the annealing process in air at 350 degrees C and assembled into polycrystalline porous spheres with sizes of 200-800 nm. The weight ratio between the rGO and V2O5 is tunable by changing the weight ratio of the precursors, which in turn affects the morphology of V2O5/rGO composites. The V2O5/rGO composites display superior cathode performances with highly reversible specific capacities, good cycling stabilities and excellent rate capabilities (e.g. 102 mA h g(-1) at 19 degrees C).
C1 [Rui, Xianhong; Lim, Tuti Mariana] Nanyang Technol Univ, Sch Civil & Environm Engn, Singapore 639798, Singapore.
   [Rui, Xianhong; Zhu, Jixin; Sim, Daohao; Xu, Chen; Zeng, Yi; Hng, Huey Hoon; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Lim, Tuti Mariana] Ngee Ann Polytech, Sch Life Sci & Chem Technol, Singapore 599489, Singapore.
   [Yan, Qingyu] Nanyang Technol Univ, Energy Res Inst, Singapore 637459, Singapore.
   [Yan, Qingyu] Nanyang Technol Univ, TUM CREATE Ctr Electromobil, Singapore 637459, Singapore.
RP Lim, TM (reprint author), Nanyang Technol Univ, Sch Civil & Environm Engn, Singapore 639798, Singapore.
EM tmlim@ntu.edu.sg; alexyan@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; zhu, Jixin/F-8763-2011; Lim, Tuti/F-8875-2012;
   Hng, Huey Hoon/A-2246-2011; Rui, Xianhong/D-2604-2015
OI Hng, Huey Hoon/0000-0002-8950-025X; Rui, Xianhong/0000-0003-1125-0905
FU AcRF of MOE (Singapore) [RG 31/08]; Singapore Ministry of Education
   [MOE2010-T2-1-017]; A*STAR SERC [1021700144];  [NRF2009EWT-CERP001-026];
    [MPA 23/04.15.03 RDP 009/10/102];  [MPA 23/04.15.03 RDP 020/10/113]
FX The authors gratefully acknowledge AcRF Tier 1 RG 31/08 of MOE
   (Singapore), NRF2009EWT-CERP001-026 (Singapore), Singapore Ministry of
   Education (MOE2010-T2-1-017), A*STAR SERC grant 1021700144 and Singapore
   MPA 23/04.15.03 RDP 009/10/102 and MPA 23/04.15.03 RDP 020/10/113 grant.
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NR 40
TC 89
Z9 92
U1 22
U2 188
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2011
VL 3
IS 11
BP 4752
EP 4758
DI 10.1039/c1nr10879d
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 843FZ
UT WOS:000296659000039
PM 21989744
ER

PT J
AU Shi, Y
   Wang, JZ
   Chou, SL
   Wexler, D
   Li, HJ
   Ozawa, K
   Liu, HK
   Wu, YP
AF Shi, Yi
   Wang, Jia-Zhao
   Chou, Shu-Lei
   Wexler, David
   Li, Hui-Jun
   Ozawa, Kiyoshi
   Liu, Hua-Kun
   Wu, Yu-Ping
TI Hollow Structured Li3VO4 Wrapped with Graphene Nanosheets in Situ
   Prepared by a One-Pot Template-Free Method as an Anode for Lithium-Ion
   Batteries
SO NANO LETTERS
LA English
DT Article
DE Lithium vanadium oxide; graphene; nanosheet; hollow structure; anode;
   lithium ion battery
ID CATHODE MATERIAL; RATE CAPABILITY; CARBON; CAPACITY; STORAGE; LI4TI5O12;
   NANOSTRUCTURES; NANOPARTICLES; LI1+XV1-XO2; PERFORMANCE
AB To explore good anode materials Of high safety, high reversible capacity, good cycling, and excellent rate capability, a Li3VO4 microbox with wall thickness of 40 nrn was prepared by a one-pot and template-free in situ hydro [thermal method. In addition, its composite with graphene nanosheets of about six layers of graphene was achieved. Both of them, especially the Li3VO4/graphene nanosheets composite, show superior electrochemical performance to the formerly reported vanadium-based anode materials. The composite: shows a reversible capacity of 223 mAh even at 20C (1C = 400 mAh g(-1)). After 500 cycles at 10C there is no evident capacity fading.
C1 [Shi, Yi; Wu, Yu-Ping] Fudan Univ, Dept Chem, New Energy & Mat Lab NEML, Shanghai 200433, Peoples R China.
   [Shi, Yi; Wu, Yu-Ping] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
   [Shi, Yi; Wang, Jia-Zhao; Chou, Shu-Lei; Liu, Hua-Kun] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
   [Wexler, David] Univ Wollongong, Electron Microscopy Ctr, Wollongong, NSW 2522, Australia.
   [Li, Hui-Jun] Univ Wollongong, Fac Engn, Wollongong, NSW 2522, Australia.
   [Ozawa, Kiyoshi] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050047, Japan.
RP Wang, JZ (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM wuyp@fudan.edu.cn
RI Wang, Jiazhao/G-4972-2011; Wu, Yuping/H-1593-2011; Chou,
   Shulei/D-9895-2011; Liu, Hua/G-1349-2012
OI Wu, Yuping/0000-0002-0833-1205; Chou, Shulei/0000-0003-1155-6082; Liu,
   Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP100103909]; National Natural
   Science Foundation of China (NSFC) [21073046]
FX Financial support from an Australian Research Council (ARC) Discovery
   Project (DP100103909) and the National Natural Science Foundation of
   China (NSFC) (21073046) is greatly appreciated. Many thanks also go to
   Dr. Tania Silver for critical reading of the manuscript.
CR Sun YQ, 2011, ENERG ENVIRON SCI, V4, P1113, DOI 10.1039/c0ee00683a
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NR 39
TC 88
Z9 89
U1 30
U2 202
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD OCT
PY 2013
VL 13
IS 10
BP 4715
EP 4720
DI 10.1021/nl402237u
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 243ZG
UT WOS:000326356300022
PM 24024651
ER

PT J
AU Mao, S
   Wen, ZH
   Kim, H
   Lu, GH
   Hurley, P
   Chen, JH
AF Mao, Shun
   Wen, Zhenhai
   Kim, Haejune
   Lu, Ganhua
   Hurley, Patrick
   Chen, Junhong
TI A General Approach to One-Pot Fabrication of Crumpled Graphene-Based
   Nanohybrids for Energy Applications
SO ACS NANO
LA English
DT Article
DE crumpled graphene; nanocrystal; nanohybrid; aerosolization;
   electrochemical supercapacitor; lithium-ion battery
ID ELECTROCHEMICAL CAPACITORS; OXIDE; PERFORMANCE; SUPERCAPACITORS;
   COMPOSITES; ELECTRODES; BATTERIES; SHEETS; ANODE; MNO2
AB Crumpled graphene oxide (GO)/graphene Is a new type of carbon nanostructure that has drawn growing attention due to its three-dimensional open structure and excellent stability in an aqueous solution. Here we report a general and one-step approach to produce crumpled graphene (CG) nanocrystal hybrids, which are produced by direct aerosolization of a GO suspension mixed with precursor ions. Nanocrystals spontaneously grow from precursor ions and assemble on both external and internal surfaces of CG balls during the solvent evaporation and GO crumpling process. More importantly, CG nanocrystal hybrids can be directly deposited onto various current-collecting substrates, enabling their tremendous potential for energy applications. As a proof of concept, we demonstrate the use of hybrid electrodes of CG-Mn3O4 and CG SnO2 in an electrochemical supercapacitor and a lithium-ion battery, respectively. The performance of the resulting capacitor/battery is attractive and outperforms conventional flat graphene-based hybrid devices. This study provides a new and facile route to fabricating high-performance hybrid CG nanocrystal electrodes for various energy systems.
C1 [Mao, Shun; Wen, Zhenhai; Kim, Haejune; Lu, Ganhua; Chen, Junhong] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA.
   [Hurley, Patrick] Johnson Controls Inc, Power Solut, Global Technol & Innovat, Milwaukee, WI 53209 USA.
RP Chen, JH (reprint author), Univ Wisconsin, Dept Mech Engn, 3200 N Cramer St, Milwaukee, WI 53211 USA.
EM jhchen@uwm.edu
RI Lu, Ganhua/B-4643-2010; wen, zhenhai/D-7165-2011; MAO, SHUN/G-9966-2015
OI Lu, Ganhua/0000-0003-3279-8427; wen, zhenhai/0000-0002-0397-4156; 
FU U.S. National Science Foundation [CMMI-0900509]; U.S. Department of
   Energy [DE-EE0003208]
FX Financial support for this work was provided by the U.S. National
   Science Foundation (CMMI-0900509) and the U.S. Department of Energy
   (DE-EE0003208). The authors thank Prof. M. Gajdardziska-Josifovska for
   TEM access at the HRTEM Laboratory of UWM, Dr. H. A. Owen for technical
   support with SEM analyses, and Dr. S. E. Hardcastle for technical
   support with XRD analyses. The SEM imaging was conducted at the Electron
   Microscope Laboratory of UWM. The XRD was conducted at the Advanced
   Analysis Facility of UWM.
CR Sun YQ, 2011, ENERG ENVIRON SCI, V4, P1113, DOI 10.1039/c0ee00683a
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NR 37
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Z9 90
U1 44
U2 334
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2012
VL 6
IS 8
BP 7505
EP 7513
DI 10.1021/nn302818J
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 995DU
UT WOS:000307988900113
PM 22838735
ER

PT J
AU Qiu, JX
   Zhang, P
   Ling, M
   Li, S
   Liu, PR
   Zhao, HJ
   Zhang, SQ
AF Qiu, Jingxia
   Zhang, Peng
   Ling, Min
   Li, Sheng
   Liu, Porun
   Zhao, Huijun
   Zhang, Shanqing
TI Photocatalytic Synthesis of TiO2 and Reduced Graphene Oxide
   Nanocomposite for Lithium Ion Battery
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium ion batteries; UV photocatalysis; TiO2; reduced graphene oxide
ID ANATASE TIO2; ANODE MATERIAL; PERFORMANCE; STORAGE; INSERTION;
   NANOPARTICLES; COMPOSITES; ELECTRODES; NANOSHEETS; REDUCTION
AB In this work, we synthesized graphene oxide (GO) using the improved Hummers oxidation method. TiO2 nanoparticles can be anchored on the GO sheets via the abundant oxygen containing functional groups such as epoxy, hydroxyl, carbonyl, and carboxyl groups on the GO sheets. Using the TiO2 photocatalyst, the GO was photocatalytically reduced under UV illumination, leading to the production of TiO2-reduced graphene oxide (TiO2-RGO) nanocomposite. The as prepared TiO2, TiO2-GO, and TiO2-RGO nanocomposite were used to fabricate lithium ion batteries (LIBs) as the active anode materials and their corresponding lithium ion insertion/extraction performance was evaluated The resultant LIBs of the TiO2-RGO nanocomposite possesses more stable cyclic performance, larger reversible capacity, and better rate capability, compared with that of the pure TiO2 and TiO2-GO samples. The electrochemical and materials characterization suggest that the graphene network provides efficient pathways for electron transfer, and the TiO2 nanoparticles prevent the restacking of the graphene nanosheets, resulting in the improvement in both electric conductivity and specific capacity, respectively. This work suggests that the TiO2 based photocatalytic method could be a simple, low-cost, and efficient approach for large-scale production of anode materials for lithium ion batteries.
C1 [Zhang, Shanqing] Griffith Univ, Environm Futures Ctr, Ctr Clean Environm & Energy, Griffith, Qld 4222, Australia.
   Griffith Univ, Griffith Sch Environm, Griffith, Qld 4222, Australia.
RP Zhang, SQ (reprint author), Griffith Univ, Environm Futures Ctr, Ctr Clean Environm & Energy, Gold Coast Campus, Griffith, Qld 4222, Australia.
EM s.zhang@griffith.edu.au
RI Li, Sheng/H-6569-2015; Zhao, Huijun/H-5882-2015; Zhang,
   Shanqing/C-2590-2008
OI Li, Sheng/0000-0003-1645-6865; Zhao, Huijun/0000-0002-3028-0459; 
FU Australian Research Council
FX The authors acknowledge the financial support of the ARC Discovery
   Grants from the Australian Research Council.
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NR 44
TC 88
Z9 90
U1 28
U2 184
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD JUL
PY 2012
VL 4
IS 7
BP 3636
EP 3642
DI 10.1021/am300722d
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 978EC
UT WOS:000306722400041
PM 22738305
ER

PT J
AU Yang, SB
   Gong, YJ
   Liu, Z
   Zhan, L
   Hashim, DP
   Ma, LL
   Vajtai, R
   Ajayan, PM
AF Yang, Shubin
   Gong, Yongji
   Liu, Zheng
   Zhan, Liang
   Hashim, Daniel P.
   Ma, Lulu
   Vajtai, Robert
   Ajayan, Pulickel M.
TI Bottom-up Approach toward Single-Crystalline VO2-Graphene Ribbons as
   Cathodes for Ultrafast Lithium Storage
SO NANO LETTERS
LA English
DT Article
DE Nanoribbons; graphene; ultrafast; electrode; lithium ion batteries
ID ION BATTERIES; HIGH-CAPACITY; HIGH-POWER; LONG-LIFE; ELECTRODES;
   GRAPHENE; ANODES; NANOBELTS
AB Although lithium ion batteries have gained commercial success owing to their high energy density, they lack suitable electrodes capable of rapid charging and discharging to enable a high power density critical for broad applications. Here, we demonstrate a simple bottom-up approach toward single crystalline vanadium oxide (VO2) ribbons with graphene layers. The unique structure of VO2-graphene ribbons thus provides the right combination of electrode properties and could enable the design of high-power lithium ion batteries. As a consequence, a high reversible capacity and ultrafast charging and discharging capability is achieved with these ribbons as cathodes for lithium storage. A full charge or discharge is capable in 20 s. More remarkably, the resulting electrodes retain more than 90% of the initial capacity after cycling more than 1000 times at an ultrahigh rate of 190C, providing the best reported rate performance for cathodes in lithium ion batteries to date.
C1 [Yang, Shubin; Liu, Zheng; Zhan, Liang; Hashim, Daniel P.; Ma, Lulu; Vajtai, Robert; Ajayan, Pulickel M.] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
   [Gong, Yongji; Ajayan, Pulickel M.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
RP Yang, SB (reprint author), Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
EM sy13@rice.edu; ajayan@rice.edu
RI Hashim, Daniel/H-1694-2013; Liu, Zheng/C-1813-2014; Yang,
   Shubin/B-4840-2015
OI Liu, Zheng/0000-0002-8825-7198; Yang, Shubin/0000-0001-9973-9785
FU U.S. Army Research Office through a MURI grant on Novel Free-Standing 2D
   Crystalline Materials focusing on Atomic Layers of Nitrides, Oxides, and
   Sulfides [W911NF-11-1-0362]; NSF [0940902]; U.S. Office of Naval
   Research MURI grant [N000014-09-1-1066]
FX This work was financially supported by U.S. Army Research Office through
   a MURI grant (W911NF-11-1-0362) on Novel Free-Standing 2D Crystalline
   Materials focusing on Atomic Layers of Nitrides, Oxides, and Sulfides.
   D.P.H. is grateful to the NSF for the Graduate Research Fellowship award
   grant no. 0940902. L.M. acknowledges the financial support provided by
   U.S. Office of Naval Research MURI grant (N000014-09-1-1066).
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NR 28
TC 87
Z9 89
U1 30
U2 296
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD APR
PY 2013
VL 13
IS 4
BP 1596
EP 1601
DI 10.1021/nl400001u
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 125OO
UT WOS:000317549300037
PM 23477543
ER

PT J
AU Mai, YJ
   Zhang, D
   Qiao, YQ
   Gu, CD
   Wang, XL
   Tu, JP
AF Mai, Y. J.
   Zhang, D.
   Qiao, Y. Q.
   Gu, C. D.
   Wang, X. L.
   Tu, J. P.
TI MnO/reduced graphene oxide sheet hybrid as an anode for Li-ion batteries
   with enhanced lithium storage performance
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Manganese monoxide; Graphene; Hybrid; Lithium ion battery
ID REVERSIBLE CAPACITY; ELECTRODE MATERIALS; CARBON NANOTUBES; METAL
   FLUORIDES; NANOPARTICLES; NANORIBBONS; CONVERSION; STABILITY; COMPOSITE
AB Relatively small hysteresis in voltage, appropriate electromotive force and low average delithiation voltage make MnO, among many transition metal oxides. MnO/reduced graphene oxide sheet (MnO/RGOS) hybrid is synthesized by a two-step electrode design consisting of liquid phase deposition of MnCO3 nanoparticles on the surface of graphene oxide sheets followed by heat treatment in flowing nitrogen. As an anode for Li-ion batteries, the MnO/RGOS hybrid electrode shows a reversible capacity of 665.5 mA h g(-1) after 50 cycles at a current density of 100 mA g(-1) and delivers 454.2 mA h g(-1) at a rate of 400 mA g(-1), which is obviously better than that of bare MnO electrode. Those reasons for such enhanced electrochemical properties are investigated by galvanostatic intermittent titration technique (GITT) as well as electrochemical impedance spectroscopy (EIS). The probable origins, in the term of thermodynamic and kinetic factors, for the marked hysteresis in voltage observed between charge and discharge are also discussed. (C) 2012 Elsevier BM. All rights reserved.
C1 [Tu, J. P.] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
RP Tu, JP (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
EM tujp@zju.edu.cn
FU Fundamental Research Funds for the Central Universities [2011QNA4006];
   Key Science and Technology Innovation Team of Zhejiang Province
   [2010R50013]
FX This work was supported by the Fundamental Research Funds for the
   Central Universities (2011QNA4006) and Key Science and Technology
   Innovation Team of Zhejiang Province (2010R50013).
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NR 50
TC 87
Z9 93
U1 26
U2 242
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD OCT 15
PY 2012
VL 216
BP 201
EP 207
DI 10.1016/j.jpowsour.2012.05.084
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 999SO
UT WOS:000308335500028
ER

PT J
AU Vinayan, BP
   Nagar, R
   Raman, V
   Rajalakshmi, N
   Dhathathreyan, KS
   Ramaprabhu, S
AF Vinayan, B. P.
   Nagar, Rupali
   Raman, V.
   Rajalakshmi, N.
   Dhathathreyan, K. S.
   Ramaprabhu, S.
TI Synthesis of graphene-multiwalled carbon nanotubes hybrid nanostructure
   by strengthened electrostatic interaction and its lithium ion battery
   application
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID FUNCTIONALIZED GRAPHENE; OXYGEN REDUCTION; ANODE MATERIAL; COMPOSITES;
   SUPERCAPACITORS; INSERTION; STORAGE
AB We report a novel way of synthesizing graphene-carbon nanotube hybrid nanostructure as an anode for lithium (Li) ion batteries. For this, graphene was prepared by the solar exfoliation of graphite oxide, while multiwalled carbon nanotubes (MWNTs) were prepared by the chemical vapor deposition method. The graphene-MWNT hybrid nanostructure was synthesized by first modifying graphene surface using a cationic polyelectrolyte and MWNT surface with acid functionalization. The hybrid structure was obtained by homogeneous mixing of chemically modified graphene and MWNT constituents. This hybrid nanostructure exhibits higher specific capacity and cyclic stability. The strengthened electrostatic interaction between the positively charged surface of graphene sheets and the negatively charged surface of MWNTs prevents the restacking of graphene sheets that provides a highly accessible area and short diffusion path length for Li-ions. The higher electrical conductivity of MWNTs promotes an easier movement of the electrons within the electrode. The present synthesis scheme recommends a new pathway for large-scale production of novel hybrid carbon nanomaterials for energy storage applications and underlines the importance of preparation routes followed for synthesizing nanomaterials.
C1 [Vinayan, B. P.; Nagar, Rupali; Ramaprabhu, S.] Indian Inst Technol, Dept Phys, AENL, Nanofunct Mat Technol Ctr NFMTC, Madras 600036, Tamil Nadu, India.
   [Raman, V.; Rajalakshmi, N.; Dhathathreyan, K. S.] Ctr Fuel Cell Technol ARCI, Madras 600113, Tamil Nadu, India.
RP Ramaprabhu, S (reprint author), Indian Inst Technol, Dept Phys, AENL, Nanofunct Mat Technol Ctr NFMTC, Madras 600036, Tamil Nadu, India.
EM ramp@iitm.ac.in
RI S, Ramaprabhu/A-1071-2014; Vedarajan, Raman/E-7267-2016; 
OI Vedarajan, Raman/0000-0002-0178-6987; Natarajan,
   Rajalakshmi/0000-0001-7926-8111
FU Indian Institute of Technology Madras, DST- Government of India; US- Air
   force
FX The authors are grateful to Indian Institute of Technology Madras, DST-
   Government of India and US- Air force for supporting this work.
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NR 31
TC 86
Z9 86
U1 19
U2 77
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 19
BP 9949
EP 9956
DI 10.1039/c2jm16294f
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 931HN
UT WOS:000303207100074
ER

PT J
AU Chen, SQ
   Chen, P
   Wu, MH
   Pan, DY
   Wang, Y
AF Chen, Shuangqiang
   Chen, Peng
   Wu, Minghong
   Pan, Dengyu
   Wang, Yong
TI Graphene supported Sn-Sb@carbon core-shell particles as a superior anode
   for lithium ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Core-shell nanostructure; Graphene nanosheets; Lithium-ion battery;
   Sn-Sb
ID COMPOSITE ANODE; LI STORAGE; PERFORMANCE; NANOSHEETS; FABRICATION;
   ELECTRODES; CAPACITY
AB This paper reports the preparation and Li-storage properties of graphene nanosheets(GNS), GNS supported Sn-Sb@carbon (50-150 nm) and Sn-Sb nanoparticles (5-10 nm). The best cycling performance and excellent high rate capabilities were observed for GNS-supported Sn-Sb@carbon core-shell particles, which exhibited initial capacities of 978, 850 and 668 mAh/g respectively at 0.1C, 2C and 5C (1C = 800 mA/g) with good cyclability. Besides the GNS support, the carbon skin around Sn-Sb particles is believed to be a key factor to improve electrochemical properties of Sn-Sb. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Wu, Minghong; Pan, Dengyu] Shanghai Univ, Inst Nanochem & Nanobiol, Shanghai 200041, Peoples R China.
   [Chen, Shuangqiang; Chen, Peng; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shanghai 200444, Peoples R China.
RP Pan, DY (reprint author), Shanghai Univ, Inst Nanochem & Nanobiol, Shanghai 200041, Peoples R China.
EM dypan617@shu.edu.cn; yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012; Chen, Shuangqiang/F-5289-2013
FU National Natural Science Foundation of China [50971085, 50701029,
   10774118]; Shanghai Science & Technology Committee [09JC1406100,
   09530501200, 09ZR1411800]; Shanghai Municipal Education Commission
   [09zz96, 10YZ03, S30109]
FX The authors gratefully acknowledge the Program for Professor of Special
   Appointment (Eastern Scholar), National Natural Science Foundation of
   China (50971085, 50701029, 10774118), Shanghai Science & Technology
   Committee (09JC1406100, 09530501200, 09ZR1411800) and Shanghai Municipal
   Education Commission (09zz96, 10YZ03, S30109) for the financial support.
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NR 28
TC 86
Z9 92
U1 14
U2 122
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD OCT
PY 2010
VL 12
IS 10
BP 1302
EP 1306
DI 10.1016/j.elecom.2010.07.005
PG 5
WC Electrochemistry
SC Electrochemistry
GA 683AQ
UT WOS:000284444500011
ER

PT J
AU Tang, YX
   Zhang, YY
   Deng, JY
   Wei, JQ
   Tam, HL
   Chandran, BK
   Dong, ZL
   Chen, Z
   Chen, XD
AF Tang, Yuxin
   Zhang, Yanyan
   Deng, Jiyang
   Wei, Jiaqi
   Hong Le Tam
   Chandran, Bevita Kallupalathinkal
   Dong, Zhili
   Chen, Zhong
   Chen, Xiaodong
TI Mechanical Force-Driven Growth of Elongated Bending TiO2-based
   Nanotubular Materials for Ultrafast Rechargeable Lithium Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
ID RATE LI-ION; NANOSTRUCTURED MATERIALS; TITANATE NANOTUBES;
   ENERGY-STORAGE; GRAPHENE SHEETS; ANODE MATERIALS; CRYSTAL-GROWTH;
   BOUNDARY-LAYER; HIGH-CAPACITY; HIGH-POWER
AB A stirring hydrothermal process that enables the formation of elongated bending TiO2-based nanotubes is presented. By making use of its bending nature, the elongated TiO2 (B) nanotubular crosslinked-network anode electrode can cycle over 10 000 times in half cells while retaining a relatively high capacity (114 mA h g(-1)) at an ultra-high rate of 25 C (8.4 A g(-1)).
C1 [Tang, Yuxin; Zhang, Yanyan; Deng, Jiyang; Wei, Jiaqi; Hong Le Tam; Chandran, Bevita Kallupalathinkal; Dong, Zhili; Chen, Zhong; Chen, Xiaodong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
RP Chen, XD (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM chenxd@ntu.edu.sg
RI Dong, Zhili/A-2249-2011; Chen, Xiaodong/A-4537-2009; Chen,
   Zhong/A-2244-2011
OI Chen, Xiaodong/0000-0002-3312-1664; Chen, Zhong/0000-0001-7518-1414
FU National Research Foundation (NRF); Prime Minister's Office, Singapore
   under its Campus for Research Excellence and Technological Enterprise
   (CREATE); NRF Fellowship scheme [NRF-RF2009-04]
FX This work was supported by the National Research Foundation (NRF), Prime
   Minister's Office, Singapore under its Campus for Research Excellence
   and Technological Enterprise (CREATE) programme (Nanomaterials for
   Energy and Water management and Singapore-Berkeley Research Initiative
   for Sustainable Energy (SinBeRISE)) and NRF Fellowship scheme
   (NRF-RF2009-04).
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NR 70
TC 85
Z9 85
U1 92
U2 387
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD SEP 17
PY 2014
VL 26
IS 35
BP 6111
EP +
DI 10.1002/adma.201402000
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AP5WE
UT WOS:000342148600009
PM 25043343
ER

PT J
AU Wang, H
   Feng, HB
   Li, JH
AF Wang, Hua
   Feng, Hongbin
   Li, Jinghong
TI Graphene and Graphene-like Layered Transition Metal Dichalcogenides in
   Energy Conversion and Storage
SO SMALL
LA English
DT Review
ID LITHIUM ION BATTERIES; SENSITIZED SOLAR-CELLS; HIGH-PERFORMANCE
   SUPERCAPACITOR; SOLUTION-PROCESSABLE GRAPHENE; ENHANCED HYDROGEN
   EVOLUTION; MOS2 ULTRATHIN NANOSHEETS; OXYGEN REDUCTION; DOPED GRAPHENE;
   ELECTROCHEMICAL CAPACITORS; ANODE MATERIAL
AB Being confronted with the energy crisis and environmental problems, the exploration of clean and renewable energy materials as well as their devices are urgently demanded. Two-dimensional (2D) atomically-thick materials, graphene and graphene-like layered transition metal dichalcogenides (TMDs), have showed vast potential as novel energy materials due to their unique physicochemical properties. In this Review, we outline the typical application of graphene and grpahene-like TMDs in energy conversion and storage fields, and hope to promote the development of 2D TMDs in this field through the analysis and comparisons with the relatively natural graphene. First, a brief introduction of electronic structures and basic properties of graphene and TMDs are presented. Then, we summarize the exciting progress of these materials made in both energy conversion and storage field including solar cells, electrocatalysis, supercapacitors and lithium ions batteries. Finally, the prospects and further developments in these exciting fields of graphene and graphene-like TMDs materials are also suggested.
C1 [Wang, Hua; Feng, Hongbin; Li, Jinghong] Tsinghua Univ, Beijing Key Lab Analyt Methods & Instrumentat, Dept Chem, Beijing 100084, Peoples R China.
   [Wang, Hua] Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China.
RP Li, JH (reprint author), Tsinghua Univ, Beijing Key Lab Analyt Methods & Instrumentat, Dept Chem, Beijing 100084, Peoples R China.
EM jhli@mail.tsinghua.edu.cn
RI Li, Jinghong /D-4283-2012
FU National Basic Research Program of China [2011CB935704, 2013CB934004];
   National Natural Science Foundation of China [21235004]; Research Fund
   of Ministry of Education of China [20110002130007]
FX This work was financially supported by National Basic Research Program
   of China (no. 2011CB935704, no. 2013CB934004), the National Natural
   Science Foundation of China (no. 21235004), and Research Fund of
   Ministry of Education of China (no. 20110002130007).
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U2 740
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD JUN 12
PY 2014
VL 10
IS 11
SI SI
BP 2165
EP 2181
DI 10.1002/smll.201303711
PG 17
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AJ6JO
UT WOS:000337799300005
PM 24577755
ER

PT J
AU Tao, LQ
   Zai, JT
   Wang, KX
   Zhang, HJ
   Xu, M
   Shen, J
   Su, YZ
   Qian, XF
AF Tao, Liqi
   Zai, Jiantao
   Wang, Kaixue
   Zhang, Haojie
   Xu, Miao
   Shen, Jie
   Su, Yuezeng
   Qian, Xuefeng
TI Co3O4 nanorods/graphene nanosheets nanocomposites for lithium ion
   batteries with improved reversible capacity and cycle stability
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Cobalt oxide; Graphene nanosheets; Nanocomposite; Lithium ion batteries;
   Anode materials
ID GRAPHENE NANOSHEETS; FACILE SYNTHESIS; ANODE MATERIALS; HYBRID ANODE;
   GAS SENSORS; PERFORMANCE; CARBON; OXIDE; NANOMATERIALS; ELECTRODES
AB Co3O4 nanorods/GNS (graphene nanosheets) nanocomposites have been synthesized through a one-spot solvothermal method, and characterized by X-ray diffraction, field emission scanning electron microscopy and transmission electron microscopy. Electrochemical performances reveal that the obtained Co3O4 nanorods/GNS nanocomposites exhibit improved cycling stability, remarkably high reversible lithium storage capacity and superior rate capability, e.g. approximate 1310 mAh g(-1) and 1090 mAh g(-1) of capacity are retained even after 40 cycles at a current density of 100 mA g(-1) and 1000 mA g(-1), respectively. The high electrochemical performances can be attributed to the unique structure of Co3O4 nanorods/GNS nanocomposites, in which the 1D structure of Co3O4 can prevent the aggregation of Co3O4 and reduce the stacking degree of GNS, providing an excellent ion diffusion and electronic conduction pathway. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Tao, Liqi; Zai, Jiantao; Wang, Kaixue; Zhang, Haojie; Xu, Miao; Shen, Jie; Qian, Xuefeng] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Tao, Liqi; Zai, Jiantao; Wang, Kaixue; Zhang, Haojie; Xu, Miao; Shen, Jie; Qian, Xuefeng] Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China.
   [Su, Yuezeng] Shanghai Jiao Tong Univ, Sch Aeronaut & Astronaut, Shanghai 200240, Peoples R China.
RP Qian, XF (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
EM xfqian@sjtu.edu.cn
RI Wang, Kai-Xue/A-4852-2009; 宰(Zai), 建陶(Jiantao)/I-8703-2012; Qian,
   Xuefeng/G-5749-2011; Zhang, Haojie/C-6586-2016
OI Wang, Kai-Xue/0000-0002-2076-5487; 宰(Zai),
   建陶(Jiantao)/0000-0001-7562-6233; Qian, Xuefeng/0000-0002-8199-6502; 
FU National Basic Research Program of China [2009CB930400, 2007CB209705];
   National Natural Science Foundation of China [21071097, 20901050];
   Shanghai Pujiang Program [09PJ1405700]; State Key Laboratory of High
   Performance Ceramics and Superfine Microstructure [SKL200901SIC]
FX The work was supported by National Basic Research Program of China
   (2009CB930400 and 2007CB209705), National Natural Science Foundation of
   China (21071097 and 20901050), Shanghai Pujiang Program (09PJ1405700)
   and the key project of State Key Laboratory of High Performance Ceramics
   and Superfine Microstructure (SKL200901SIC).
CR Wang KX, 2007, ADV MATER, V19, P3016, DOI 10.1002/adma.200602189
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   Zhang J, 2008, APPL PHYS LETT, V93, DOI 10.1063/1.3044453
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NR 36
TC 85
Z9 88
U1 24
U2 146
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD MAR 15
PY 2012
VL 202
BP 230
EP 235
DI 10.1016/j.jpowsour.2011.10.131
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 890IU
UT WOS:000300139100030
ER

PT J
AU Zhong, C
   Wang, JZ
   Chen, ZX
   Liu, HK
AF Zhong, Chao
   Wang, Jiazhao
   Chen, Zhixin
   Liu, Huakun
TI SnO2-Graphene Composite Synthesized via an Ultrafast and Environmentally
   Friendly Microwave Autoclave Method and Its Use as a Superior Anode for
   Lithium-Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID RECHARGEABLE BATTERIES; REVERSIBLE CAPACITY; STORAGE CAPABILITY; CYCLIC
   PERFORMANCE; RAMAN-SPECTRUM; SNO2; NANOPARTICLES; CHALLENGES; SHEETS
AB SnO2-graphene composites have been synthesized by an ultrafast and environmentally friendly microwave autoclave method. From field emission scanning electron microscopy and transmission electron microscopy, it can be determined that the SnO2 nanoparticles, around 4-S nm in diameter, are uniformly sandwiched between graphene nanosheets containing only a few layers. The successful synthesis demonstrates that in situ loading of SnO2 nanoparticles can be an effective way to prevent graphene nanosheets from being restacked during the reduction. The Li-cycling properties of the materials have been evaluated by galvanostatic discharge-charge cycling and impedance spectroscopy. Results show that the SnO2-graphene composite with a graphene content of 33.3 wt % exhibits a very stable capacity of about 590 mAh g(-1) without noticeable fading for up to 200 cycles.
C1 [Zhong, Chao; Wang, Jiazhao; Liu, Huakun] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2500, Australia.
   [Wang, Jiazhao; Liu, Huakun] Univ Wollongong, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2500, Australia.
   [Chen, Zhixin] Univ Wollongong, Sch Mech Mat & Mechatron Engn, Wollongong, NSW 2500, Australia.
RP Zhong, C (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2500, Australia.
EM cz527@uowmail.edu.au; jiazhao@uow.edu.au
RI Wang, Jiazhao/G-4972-2011; Liu, Hua/G-1349-2012
OI Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP 0987805]
FX Financial support provided by an Australian Research Council (ARC)
   Discovery Project (DP 0987805) is gratefully acknowledged. Technical
   assistance on AFM by Mr. Darren Attard is highly appreciated. Many
   thanks also go to Dr. Tania Silver for critical reading of the
   manuscript.
CR Zhang LS, 2010, J MATER CHEM, V20, P5462, DOI 10.1039/c0jm00672f
   Xu YX, 2008, J AM CHEM SOC, V130, P5856, DOI 10.1021/ja800745y
   Chou SL, 2009, ELECTROCHIM ACTA, V54, P7519, DOI 10.1016/j.electacta.2009.08.006
   Dieguez A, 2001, J APPL PHYS, V90, P1550, DOI 10.1063/1.1385573
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   Yoo E, 2008, NANO LETT, V8, P2277, DOI 10.1021/nl800957b
   Bruce PG, 2008, ANGEW CHEM INT EDIT, V47, P2930, DOI 10.1002/anie.200702505
   Wu ZS, 2010, ACS NANO, V4, P3187, DOI 10.1021/nn100740x
   TUINSTRA F, 1970, J CHEM PHYS, V53, P1126, DOI 10.1063/1.1674108
   Kim H, 2011, J ELECTROCHEM SOC, V158, pA930, DOI 10.1149/1.3599632
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NR 33
TC 85
Z9 86
U1 7
U2 91
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD DEC 22
PY 2011
VL 115
IS 50
BP 25115
EP 25120
DI 10.1021/jp2061128
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 860KR
UT WOS:000297947700085
ER

PT J
AU Zhang, X
   Kumar, PS
   Aravindan, V
   Liu, HH
   Sundaramurthy, J
   Mhaisalkar, SG
   Duong, HM
   Ramakrishna, S
   Madhavi, S
AF Zhang, Xiang
   Kumar, Palaniswamy Suresh
   Aravindan, Vanchiappan
   Liu, Hui Hui
   Sundaramurthy, Jayaraman
   Mhaisalkar, Subodh G.
   Duong, Hai Minh
   Ramakrishna, Seeram
   Madhavi, Srinivasan
TI Electrospun TiO2-Graphene Composite Nanofibers as a Highly Durable
   Insertion Anode for Lithium Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID TIO2 NANOFIBERS; ENERGY-STORAGE; ANATASE TIO2; GRAPHENE; PERFORMANCE;
   CARBON; ELECTROCHEMISTRY; NANOSTRUCTURES; NANOCOMPOSITES; NANOPARTICLES
AB We report the synthesis and electrochemical performance of one-dimensional TiO2-graphene composite nanofibers (TiO2-G nanofibers) by a simple electrospinning technique for the first time. Structural and morphological properties were characterized by various techniques, such as X-ray diffraction, scanning electron microscopy (SEM), transmission electron microscopy (TEM) Raman spectroscopy, and BET surface area analysis. Lithium insertion properties were evaluated by both galvanostatic and potentiostatic mocks in half-cell configurations. Cyclic voltammetric study reveals the Li-insertion/extraction by a two-phase reaction mechanism that is supported by galvanostatic charge-discharge profiles. Li/TiO2-G half-cells showed an initial discharge capacity of 260 mA h g(-1) at current density of 33 mA g(-1). Further, Li/TiO2-G cell retained 84% of reversible capacity after 300 cycles at a current density of 150 mA g(-1), which is 25% higher than bare TiO2 nanofibers under the same test conditions. The cell also exhibits promising high rate behavior with a discharge capacity of 71 mA h g(-1) at a current density of 1.8 A g(-1).
C1 [Zhang, Xiang; Kumar, Palaniswamy Suresh; Sundaramurthy, Jayaraman; Madhavi, Srinivasan] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Zhang, Xiang; Duong, Hai Minh; Ramakrishna, Seeram] Natl Univ Singapore, Dept Mech Engn, Singapore 117576, Singapore.
   [Liu, Hui Hui] Natl Univ Singapore, Dept Chem, Singapore 117576, Singapore.
   [Kumar, Palaniswamy Suresh; Sundaramurthy, Jayaraman; Ramakrishna, Seeram] Natl Univ Singapore, Ctr Nanofibers & Nanotechnol, Singapore 117576, Singapore.
   [Aravindan, Vanchiappan; Mhaisalkar, Subodh G.; Madhavi, Srinivasan] Nanyang Technol Univ, ERI N, Singapore 637553, Singapore.
RP Madhavi, S (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
EM seeram@nus.edu.sg; Madhavi@ntu.edu.sg
RI Mhaisalkar, Subodh/A-2231-2011; Zhang, Xiang/O-2394-2013; Jayaraman,
   Sundaramurthy/F-8237-2012; Srinivasan, Madhavi/A-2247-2011; 
OI Mhaisalkar, Subodh/0000-0002-9895-2426; Jayaraman,
   Sundaramurthy/0000-0003-1522-6240; Aravindan,
   Vanchiappan/0000-0003-1357-7717
FU Singapore NRF-CRP grant on "Nanonets for Harnessing Solar Energy and
   Storage"; FRC Startup grant, National University of Singapore, Singapore
   [R-265-000-361-133]; National Research Foundation, Singapore through
   Clean Energy Research Project [NRF2009EWT-CERP001-036]
FX This work was supported by Singapore NRF-CRP grant on "Nanonets for
   Harnessing Solar Energy and Storage" and the FRC Startup grant
   R-265-000-361-133, National University of Singapore, Singapore. V.A. and
   S.M. wish to thank the National Research Foundation, Singapore, for the
   financial support through Clean Energy Research Project
   (NRF2009EWT-CERP001-036).
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NR 45
TC 84
Z9 85
U1 42
U2 230
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD JUL 19
PY 2012
VL 116
IS 28
BP 14780
EP 14788
DI 10.1021/jp302574g
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 975IF
UT WOS:000306503200006
ER

PT J
AU Zhu, XJ
   Zhu, YW
   Murali, S
   Stoller, MD
   Ruoff, RS
AF Zhu, Xianjun
   Zhu, Yanwu
   Murali, Shanthi
   Stoller, Meryl D.
   Ruoff, Rodney S.
TI Reduced graphene oxide/tin oxide composite as an enhanced anode material
   for lithium ion batteries prepared by homogenous coprecipitation
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Reducul graphene oxide; Tin oxide; Homogeneous coprecipitation; Lithium
   ion battery; Anode
ID SN-C COMPOSITE; IRREVERSIBLE CAPACITIES; PERFORMANCE; TIN; ELECTRODE;
   STABILITY; INSERTION; GRAPHITE; HYBRID
AB Reduced graphene oxide/tin oxide composite is prepared by homogenous coprecipitation. Characterizations show that tin oxide particles are anchored uniformly on the surface of reduced graphene oxide platelets. As an anode material for Li ion batteries, it has 2140 mAh g(-1) and 1080 mAh g(-1) capacities for the first discharge and charge, respectively, which is more than the theoretical capacity of tin oxide, and has good capacity retention with a capacity of 649 mAh g(-1) after 30 cycles. The simple synthesis method can be readily adapted to prepare other composites containing reduced graphene oxide as a conducting additive that, in addition to supporting metal oxide nanoparticles, can also provide additional Li binding sites to, perhaps, further enhance capacity. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Zhu, Xianjun; Zhu, Yanwu; Murali, Shanthi; Stoller, Meryl D.; Ruoff, Rodney S.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA.
   [Zhu, Xianjun; Zhu, Yanwu; Murali, Shanthi; Stoller, Meryl D.; Ruoff, Rodney S.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA.
   [Zhu, Xianjun] Cent China Normal Univ, Coll Chem, Wuhan 430079, Hubei, Peoples R China.
RP Ruoff, RS (reprint author), Univ Texas Austin, Dept Mech Engn, 1 Univ Stn C2200, Austin, TX 78712 USA.
EM r.ruoff@mail.utexas.edu
RI Zhu, Yanwu/C-8979-2012; Ruoff, Rodney/K-3879-2015
FU University of Texas at Austin; U.S. Department of Energy, Office of
   Basic Energy Sciences, Division of Materials Sciences and Engineering
   [DE-SC001951]; National Science Foundation [DMR-0907324]; China
   Scholarship Council; SRF for ROCS, SEM
FX This work was supported by the University of Texas at Austin, the U.S.
   Department of Energy, Office of Basic Energy Sciences, Division of
   Materials Sciences and Engineering under Award DE-SC001951, the National
   Science Foundation (DMR-0907324), the China Scholarship Council
   Fellowship, and the Project-sponsored by SRF for ROCS, SEM.
CR Zhou GM, 2010, CHEM MATER, V22, P5306, DOI 10.1021/cm101532x
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NR 24
TC 84
Z9 84
U1 10
U2 80
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD AUG 1
PY 2011
VL 196
IS 15
BP 6473
EP 6477
DI 10.1016/j.jpowsour.2011.04.015
PG 5
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 783GA
UT WOS:000292068300066
ER

PT J
AU Guo, P
   Song, HH
   Chen, XH
AF Guo, Peng
   Song, Huaihe
   Chen, Xiaohong
TI Hollow graphene oxide spheres self-assembled by W/O emulsion
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; GRAPHITE OXIDE; ANODE MATERIALS; FUNCTIONALIZED
   GRAPHENE; GOLD NANOPARTICLES; CARBON NANOSPHERES; LI STORAGE; SHEETS;
   PERFORMANCE; NANOSHEETS
AB Hollow graphene oxide spheres (HGOSs) were fabricated from graphene oxide nanosheets (GONs) utilizing a water-in-oil (W/O) emulsion technique without surfactant. Effects of oxidation treatment and water removal on the formation and morphology of HGOSs are investigated. The oxidation time for preparing GONs is a crucial factor for the formation and morphology of HGOSs. We found that with increasing oxidation time, the morphology and surface topography of HGOSs vary from irregular and rough to uniform and smooth shape with decreasing diameter. Moreover, the electrochemical performance of HGOSs as anode materials in lithium-ion batteries was evaluated. The heat-treated HGOSs exhibit a 485 mAh g(-1) reversible capacity and high rate performance thanks to the hollow structure, thin and porous shells consisting of graphene.
C1 [Guo, Peng; Song, Huaihe; Chen, Xiaohong] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing, Peoples R China.
RP Song, HH (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing, Peoples R China.
EM songhh@mail.buct.edu.cn
RI Guo, Peng/F-8894-2010
OI Guo, Peng/0000-0003-1814-6780
FU Foundation of Excellent Doctoral Dissertation of Beijing City
   [YB20081001001]
FX This work was supported by the Foundation of Excellent Doctoral
   Dissertation of Beijing City (YB20081001001).
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NR 61
TC 84
Z9 85
U1 19
U2 139
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2010
VL 20
IS 23
BP 4867
EP 4874
DI 10.1039/b927302f
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 604JO
UT WOS:000278275500017
ER

PT J
AU Xiao, L
   Wu, DQ
   Han, S
   Huang, YS
   Li, S
   He, MZ
   Zhang, F
   Feng, XL
AF Xiao, Li
   Wu, Dongqing
   Han, Sheng
   Huang, Yanshan
   Li, Shuang
   He, Mingzhong
   Zhang, Fan
   Feng, Xinliang
TI Self-Assembled Fe2O3/Graphene Aerogel with High Lithium Storage
   Performance
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE Fe2O3/GAs; 3D interconnected graphene; self-assembly; anode material;
   lithium-ion batteries
ID CHEMICALLY-MODIFIED GRAPHENE; ION BATTERIES; REDUCED GRAPHENE;
   ENERGY-STORAGE; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE; OXIDE;
   ALPHA-FE2O3; CAPACITY; METAL
AB In this study, graphene aerogel (GA)-supported Fe2O3 particles with three-dimensional (3D) architecture was prepared by a one-pot hydrothermal process. Fe2O3 particles were dispersed uniformly on the graphene sheets, and the resulting composites self-assembled into a 3D network via hydrothermal treatment. This strategy provides a facile and environmentally friendly method for the large-scale synthesis of Fe2O3/GAs without any additional reductant. As the anode material for lithium ion batteries, the Fe2O3/GAs in this study manifested an excellent reversible capacity of 995 mA h g(-1) after 50 cycles at a charge-discharge rate of 100 mA g(-1) and even delivered reversible capacity as high as 372 mA h g(-1) at a high rate of 5000 mA g(-1). The outstanding electrochemical performance of Fe2O3/GAs can be attributed to the synergistic interaction between uniformly dispersed Fe2O3 particles and graphene aerogel, in which a robust 3D framework of graphene provided highly conductive networks with a large surface area and short diffusion path length for the transport of lithium ions.
C1 [Xiao, Li; He, Mingzhong] China Univ Geosci, Fac Mat Sci & Chem, Wuhan 430074, Peoples R China.
   [Wu, Dongqing; Han, Sheng; Huang, Yanshan; Li, Shuang; Zhang, Fan; Feng, Xinliang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Zhang, F (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
EM fan-zhang@sjtu.edu.cn; feng@mpip-mainz.mpg.de
FU 973 Program of China [2012CB933404]; Natural Science Foundation of China
   [21174083, 21102091]; Shanghai Pujiang Program [11PJ1405400]; BASF;
   Ph.D. Programs Foundation of Ministry of Education of China
   [20110073120039]
FX We acknowledge funding support from 973 Program of China (2012CB933404),
   Natural Science Foundation of China (21174083 and 21102091), BASF,
   Shanghai Pujiang Program (11PJ1405400), and the Ph.D. Programs
   Foundation of Ministry of Education of China for Young Scholars
   (20110073120039).
CR Zou YQ, 2011, J PHYS CHEM C, V115, P20747, DOI 10.1021/jp206876t
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NR 43
TC 83
Z9 83
U1 62
U2 390
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY 8
PY 2013
VL 5
IS 9
BP 3764
EP 3769
DI 10.1021/am400387t
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 143AQ
UT WOS:000318839100039
PM 23551107
ER

PT J
AU Choi, BG
   Chang, SJ
   Lee, YB
   Bae, JS
   Kim, HJ
   Huh, YS
AF Choi, Bong Gill
   Chang, Sung-Jin
   Lee, Young Boo
   Bae, Jong Seong
   Kim, Hae Jin
   Huh, Yun Suk
TI 3D heterostructured architectures of Co3O4 nanoparticles deposited on
   porous graphene surfaces for high performance of lithium ion batteries
SO NANOSCALE
LA English
DT Article
ID ENERGY-STORAGE; NANOSTRUCTURED MATERIALS; CYCLIC PERFORMANCE; REDUCED
   GRAPHENE; ANODE MATERIAL; CONVERSION; CAPACITY; COMPOSITES; ELECTRODES;
   COBALT
AB Control of structure and morphology in electrode design is crucial for creating efficient transport pathways of ions and electrons in high-performance energy storage devices. Here we report the fabrication of high-performance anode materials for lithium-ion batteries based on a 3D heterostructured architecture consisting of Co3O4 nanoparticles deposited onto porous graphene surfaces. A combination of replication and filtration processes - a simple and general method - allows a direct assembly of 2D graphene sheets into 3D porous films with large surface area, porosity, and mechanical stability. The polystyrene spheres are employed as sacrificial templates for an embossing technique that yields porous structures with tunable pore sizes ranging from 100 nm to 2 mm. Co3O4 nanoparticles with high-energy storage capacity can be easily incorporated into the pore surfaces by a simple deposition strategy, thereby creating a 3D heterogeneous Co3O4/graphene film. In particular, we exploit the 3D Co3O4/graphene composite films as anode materials for lithium ion batteries in order to resolve the current issues of rate capability and cycling life. This unique heterogeneous 3D structure is capable of delivering excellent Li+ ion storage/release and displays the following characteristics: a high rate capability of 71% retention even at a high current rate of 1000 mA g(-1) and a good cycling performance with 90.6% retention during 50 cycles. The versatile and simple nature of preparing 3D heterogeneous graphene films with various functional nanoparticles can be extended to overcome the major challenges that exist for many electrochemical devices.
C1 [Choi, Bong Gill; Chang, Sung-Jin; Kim, Hae Jin; Huh, Yun Suk] Korea Basic Sci Inst, Div Mat Sci, Taejon 305333, South Korea.
   [Lee, Young Boo] Korea Basic Sci Inst, Jeonju Ctr, Jeonju 561756, South Korea.
   [Bae, Jong Seong] Korea Basic Sci Inst, Res Lab, Pusan 609735, South Korea.
RP Huh, YS (reprint author), Korea Basic Sci Inst, Div Mat Sci, Taejon 305333, South Korea.
EM yshuh@kbsi.re.kr
FU National Research Foundation of Korea; Korean Government (MEST)
   [NRF-2010-C1AAA001-0029018]; KBSI [T3209B]
FX We acknowledge the financial support by the National Research Foundation
   of Korea Grant funded by the Korean Government (MEST,
   NRF-2010-C1AAA001-0029018) and by KBSI grant T3209B to Y. S. Huh.
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NR 37
TC 83
Z9 83
U1 22
U2 169
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 19
BP 5924
EP 5930
DI 10.1039/c2nr31438j
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 004UF
UT WOS:000308705900021
PM 22899185
ER

PT J
AU Liu, WW
   Yan, XB
   Lang, JW
   Peng, C
   Xue, QJ
AF Liu, Wen-wen
   Yan, Xing-bin
   Lang, Jun-wei
   Peng, Chao
   Xue, Qun-ji
TI Flexible and conductive nanocomposite electrode based on graphene sheets
   and cotton cloth for supercapacitor
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; WALLED CARBON NANOTUBES; SENSITIZED SOLAR-CELLS;
   ELECTROCHEMICAL CAPACITORS; FUNCTIONALIZED GRAPHENE; ENERGY-STORAGE;
   ANODE MATERIAL; NICKEL-OXIDE; THIN-FILM; COMPOSITES
AB There is currently a strong demand for energy storage devices which are cheap, light weight, flexible, and possess high power and energy densities to meet the various requirements of modern gadgets. Herein, we prepare a flexible and easily processed electrode via a simple "brush-coating and drying" process using everyday cotton cloth as the platform and a stable graphene oxide (GO) suspension as the ink. After such a simple manufacturing operation followed by annealing at 300 degrees C in argon atmosphere, the as-obtained graphene sheets (GNSs)-cotton cloth (CC) composite fabric exhibits good electrical conductivity, outstanding flexibility, and strong adhesion between GNSs and cotton fibers. Using this GNSs-CC composite fabric as the electrode material and pure CC as the separator, a home-made supercapacitor was fabricated. The supercapacitor shows the specific capacitance of 81.7 F g(-1) (two-electrode system) in aqueous electrolyte, which is one of the highest values for GNSs-based supercapacitors. Moreover, the supercapacitor also exhibits satisfactory capacitance in ionic-liquid/organic electrolyte. An all-fabric supercapacitor was also fabricated using pure CC as separator and GNSs-CC composite fabric as electrode and current collector. Such a conductive GNSs-CC composite fabric may provide new design opportunities for wearable electronics and energy storage applications.
C1 [Liu, Wen-wen; Yan, Xing-bin; Lang, Jun-wei; Peng, Chao; Xue, Qun-ji] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China.
   [Liu, Wen-wen] Chinese Acad Sci, Grad Univ, Beijing 100080, Peoples R China.
RP Yan, XB (reprint author), Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China.
EM xbyan@licp.cas.cn
RI Yan, Xingbin/B-2408-2014
FU Top Hundred Talents Program of the Chinese Academy of Sciences; National
   Nature Science Foundations of China [51005225]; Youth Science
   Foundations of Gansu Province [1107RJYA274]
FX This work was supported by the Top Hundred Talents Program of the
   Chinese Academy of Sciences, the National Nature Science Foundations of
   China (51005225), and the Youth Science Foundations of Gansu Province
   (1107RJYA274).
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U2 325
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 33
BP 17245
EP 17253
DI 10.1039/c2jm32659k
PG 9
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 981MR
UT WOS:000306972900078
ER

PT J
AU Lotfabad, EM
   Ding, J
   Cui, K
   Kohandehghan, A
   Kalisvaart, WP
   Hazelton, M
   Mitlin, D
AF Lotfabad, Elmira Memarzadeh
   Ding, Jia
   Cui, Kai
   Kohandehghan, Alireza
   Kalisvaart, W. Peter
   Hazelton, Michael
   Mitlin, David
TI High-Density Sodium and Lithium Ion Battery Anodes from Banana Peels
SO ACS NANO
LA English
DT Article
DE carbon; graphite; graphene; anode; battery; capacitor; SIB; NIB; NAB
ID ELECTROCHEMICAL ENERGY-STORAGE; POROUS CARBON NANOFIBERS; HIGH-CAPACITY;
   RATE CAPABILITY; GRAPHENE SHEETS; NEGATIVE ELECTRODE; ULTRAFAST CHARGE;
   REDUCED GRAPHENE; RATE PERFORMANCE; DISCHARGE RATES
AB Banana peel pseudographite (BPPG) offers superb dual functionality for sodium ion battery (NIB) and lithium ion battery (LIB) anodes. The materials possess low surface areas (19-217 m(2) g(-1)) and a relatively high electrode packing density (0.75 g cm(-3) vs similar to 1 g cm(-3) for graphite). Tested against Na, BPPG delivers a gravimetric (and volumetric) capacity of 355 mAh g(-1) (by active material similar to 700 mAh cm(-3), by electrode volume similar to 270 mAh cm(-3)) after 10 cycles at 50 mA g(-1). A nearly flat similar to 200 mAh g(-1) plateau that is below 0.1 V and a minimal charge/discharge voltage hysteresis make BPPG a direct electrochemical analogue to graphite but with Na. A charge capacity of 221 mAh g(-1) at 500 mA g(-1) degraded by 7% after 600 cycles, while a capacity of 336 mAh g(-1) 100 mAg(-1) is degraded by 11% after 300 cycles, in both cases with similar to 100% cycling Coulombic efficiency. For LIB applications BPPG offers a gravimetric (volumetric) capacity of 1090 mAh g(-1) (by material similar to 2200 mAh cm(-3), by electrode similar to 900 mAh cm(-3)) at 50 mA g(-1). The reason that BPPG works so well for both NIBs and LIBs is that it uniquely contains three essential features: (a) dilated intergraphene spacing for Na intercalation at low voltages; (b) highly accessible near-surface nanopores for Li metal filling at low voltages; and (c) substantial defect content in the graphene planes for U adsorption at higher voltages. The <0.1 V charge storage mechanism is fundamentally different for Na versus for Li. A combination of XRD and XPS demonstrates highly reversible Na intercalation rather than metal underpotential deposition. By contrast, the same analysis proves the presence of metallic Li in the pores, with intercalation being much less pronounced.
C1 [Lotfabad, Elmira Memarzadeh; Ding, Jia; Kohandehghan, Alireza; Kalisvaart, W. Peter; Hazelton, Michael; Mitlin, David] Univ Alberta, Dept Chem & Mat Engn, Edmonton, AB T6G 2V4, Canada.
   [Lotfabad, Elmira Memarzadeh; Ding, Jia; Cui, Kai; Kohandehghan, Alireza; Kalisvaart, W. Peter; Hazelton, Michael; Mitlin, David] Natl Res Council Canada, Natl Inst Nanotechnol NINT, Edmonton, AB T6G 2M9, Canada.
RP Lotfabad, EM (reprint author), Univ Alberta, Dept Chem & Mat Engn, 9107 116th St, Edmonton, AB T6G 2V4, Canada.
EM memarzad@ualberta.ca; dmitlin@ualberta.ca
FU NSERC; NINT NRC
FX This work was supported by NSERC Discovery and by NINT NRC.
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NR 108
TC 82
Z9 82
U1 56
U2 272
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD JUL
PY 2014
VL 8
IS 7
BP 7115
EP 7129
DI 10.1021/nn502045y
PG 15
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AL9LR
UT WOS:000339463100067
PM 24897543
ER

PT J
AU Yu, DYW
   Prikhodchenko, PV
   Mason, CW
   Batabyal, SK
   Gun, J
   Sladkevich, S
   Medvedev, AG
   Lev, O
AF Yu, Denis Y. W.
   Prikhodchenko, Petr V.
   Mason, Chad W.
   Batabyal, Sudip K.
   Gun, Jenny
   Sladkevich, Sergey
   Medvedev, Alexander G.
   Lev, Ovadia
TI High-capacity antimony sulphide nanoparticle-decorated graphene
   composite as anode for sodium-ion batteries
SO NATURE COMMUNICATIONS
LA English
DT Article
ID ELECTRODES; NANOCOMPOSITES; PERFORMANCE; STABILITY; INSERTION; CATHODE;
   STORAGE; CELL; SB
AB Sodium-ion batteries are an alternative to lithium-ion batteries for large-scale applications. However, low capacity and poor rate capability of existing anodes are the main bottlenecks to future developments. Here we report a uniform coating of antimony sulphide (stibnite) on graphene, fabricated by a solution-based synthesis technique, as the anode material for sodium-ion batteries. It gives a high capacity of 730mAhg(-1) at 50mAg(-1), an excellent rate capability up to 6C and a good cycle performance. The promising performance is attributed to fast sodium ion diffusion from the small nanoparticles, and good electrical transport from the intimate contact between the active material and graphene, which also provides a template for anchoring the nanoparticles. We also demonstrate a battery with the stibnite-graphene composite that is free from sodium metal, having energy density up to 80Whkg(-1). The energy density could exceed that of some lithium-ion batteries with further optimization.
C1 [Yu, Denis Y. W.] City Univ Hong Kong, Sch Energy & Environm, Kowloon, Hong Kong, Peoples R China.
   [Yu, Denis Y. W.; Batabyal, Sudip K.] Nanyang Technol Univ, Energy Res Inst NTU, Singapore 639798, Singapore.
   [Yu, Denis Y. W.; Mason, Chad W.] TUM CREATE, Ctr Electromobil, Singapore 138602, Singapore.
   [Prikhodchenko, Petr V.; Medvedev, Alexander G.] Russian Acad Sci, Kurnakov Inst Gen & Inorgan Chem, Moscow 119991, Russia.
   [Gun, Jenny; Sladkevich, Sergey; Medvedev, Alexander G.; Lev, Ovadia] Hebrew Univ Jerusalem, Casali Inst, IL-91904 Jerusalem, Israel.
   [Gun, Jenny; Sladkevich, Sergey; Medvedev, Alexander G.; Lev, Ovadia] Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel.
   [Gun, Jenny; Sladkevich, Sergey; Medvedev, Alexander G.; Lev, Ovadia] Hebrew Univ Jerusalem, Harvey M Krueger Family Ctr Nanosci & Nanotechnol, IL-91904 Jerusalem, Israel.
RP Yu, DYW (reprint author), City Univ Hong Kong, Sch Energy & Environm, Tat Chee Ave, Kowloon, Hong Kong, Peoples R China.
EM denisyu@cityu.edu.hk; prikhman@gmail.com
RI Medvedev, Alexander/H-8470-2013; Prikhodchenko, Petr/M-4915-2015; 
OI Medvedev, Alexander/0000-0002-6762-004X; Batabyal, Sudip
   Kumar/0000-0003-0615-9576; Yu, Denis/0000-0002-5883-7087
FU National Research Foundation of Singapore under the TUM CREATE Centre
   for Electromobility; CREATE Center for Nanotechnology for Water and
   Energy Management; Energy Research Institute at Nanyang Technological
   University, Singapore; I-SAEF, Israel Strategic Alternative Energy
   Foundation; Russian Foundation for Basic Research [11-03-00551,
   14-03-00279]
FX This study was supported by the National Research Foundation of
   Singapore under the TUM CREATE Centre for Electromobility and the CREATE
   Center for Nanotechnology for Water and Energy Management and the Energy
   Research Institute at Nanyang Technological University, Singapore. The
   financial assistance of I-SAEF, Israel Strategic Alternative Energy
   Foundation is gratefully acknowledged. We thank Russian Foundation for
   Basic Research (grants 11-03-00551 and 14-03-00279).
CR Xiao LF, 2012, CHEM COMMUN, V48, P3321, DOI 10.1039/c2cc17129e
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NR 30
TC 82
Z9 83
U1 67
U2 328
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD DEC
PY 2013
VL 4
AR 2922
DI 10.1038/ncomms3922
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 285LW
UT WOS:000329396500008
PM 24322450
ER

PT J
AU Li, L
   Raji, ARO
   Tour, JM
AF Li, Lei
   Raji, Abdul-Rahman O.
   Tour, James M.
TI Graphene-Wrapped MnO2-Graphene Nanoribbons as Anode Materials for
   High-Performance Lithium Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
ID CARBON; OXIDE; NANOTUBES; STORAGE; CHALLENGES; ELECTRODES; SHEETS
AB A facile and cost-effective approach for the fabrication of a hierarchical nanocomposite material of graphene-wrapped MnO2-graphene nanoribbons (GMG) is developed. The resulting composite has a high specific capacity and an excellent cycling stability owing to the synergistic combination of the electrically conductive graphene, graphene nanoribbons, and MnO2.
   [GRAPHICS]
   .
C1 [Li, Lei; Raji, Abdul-Rahman O.; Tour, James M.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
   [Tour, James M.] Rice Univ, Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA.
   [Tour, James M.] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
RP Tour, JM (reprint author), Rice Univ, Dept Chem, 6100 Main St MS 60, Houston, TX 77005 USA.
EM tour@rice.edu
FU ONR MURI program [00006766, N00014-09-1-1066]; AFOSR MURI program
   [FA9550-12-1-0035]; AFOSR [FA9550-09-1-0581]; Chinese Scholarship
   Council
FX The ONR MURI program (#00006766, N00014-09-1-1066), the AFOSR MURI
   program (FA9550-12-1-0035), the AFOSR (FA9550-09-1-0581), and the
   Chinese Scholarship Council provided funding.
CR Ang WA, 2012, ACS APPL MATER INTER, V4, P7010, DOI 10.1021/am3022653
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NR 36
TC 81
Z9 82
U1 47
U2 243
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD NOV 20
PY 2013
VL 25
IS 43
BP 6298
EP 6302
DI 10.1002/adma.201302915
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AA3BL
UT WOS:000330967800020
PM 23996876
ER

PT J
AU Han, S
   Wu, DQ
   Li, S
   Zhang, F
   Feng, XL
AF Han, Sheng
   Wu, Dongqing
   Li, Shuang
   Zhang, Fan
   Feng, Xinliang
TI Graphene: A Two-Dimensional Platform for Lithium Storage
SO SMALL
LA English
DT Review
DE graphene; lithium storage; electrode materials; metal oxides; carbon
ID LI-ION BATTERIES; PERFORMANCE ANODE MATERIALS; NITROGEN-DOPED GRAPHENE;
   IMPROVED REVERSIBLE CAPACITY; CHEMICALLY-MODIFIED GRAPHENE; ENHANCED
   RATE CAPABILITY; IN-SITU SYNTHESIS; REDUCED GRAPHENE; CATHODE MATERIAL;
   ELECTROCHEMICAL PERFORMANCES
AB Lithium ion batteries (LIBs) have attracted great attention due to their high energy density, low maintenance requirements, and relatively low self-discharge. Since the electrode materials hold the key for the electrochemical performance of LIBs, the design and synthesis of unconventional electrode materials with high lithium-storage capacities are the current focus in LIB research. In the last few years, a great deal of effort has been directed toward graphene as the electrode material for LIBs owing to its high intrinsic surface area, high electrical conductivity, and good compatibility with other electrochemically active components. This review paper outlines the componential and structural design for graphene-based hybrids in LIBs with enhanced electrochemical performance. The typical fabrication methods and structureproperty relationships of these hybrids are discussed.
C1 [Han, Sheng; Wu, Dongqing; Li, Shuang; Zhang, Fan; Feng, Xinliang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
   [Han, Sheng] Shanghai Inst Technol, New Energy Mat Lab, Shanghai 201418, Peoples R China.
RP Zhang, F (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Dongchuan Rd 800, Shanghai 200240, Peoples R China.
EM fan-zhang@sjtu.edu.cn; feng@mpip-mainz.mpg.de
FU 973 Program of China [2012CB933404]; ERC; Natural Science Foundation of
   China [21174083, 21102091]; BASF; Shanghai Pujiang Program
   [11PJ1405400]; PhD Programs Foundation of Ministry of Education of China
   for Young Scholars [20110073120039]
FX This work was financially supported by 973 Program of China
   (2012CB933404), ERC Grant on 2DMATER, Natural Science Foundation of
   China (21174083 and 21102091), BASF, Shanghai Pujiang Program
   (11PJ1405400), PhD Programs Foundation of Ministry of Education of China
   for Young Scholars (20110073120039).
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NR 167
TC 81
Z9 81
U1 46
U2 617
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD APR 22
PY 2013
VL 9
IS 8
SI SI
BP 1173
EP 1187
DI 10.1002/smll.201203155
PG 15
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 127HS
UT WOS:000317689600005
PM 23495008
ER

PT J
AU Wang, B
   Wang, Y
   Park, J
   Ahn, H
   Wang, GX
AF Wang, Bei
   Wang, Ying
   Park, Jinsoo
   Ahn, Hyojun
   Wang, Guoxiu
TI In situ synthesis of Co3O4/graphene nanocomposite material for
   lithium-ion batteries and supercapacitors with high capacity and
   supercapacitance
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Co3O4; Graphene; Lithium-ion batteries; Supercapacitors
ID HYDROTHERMAL SYNTHESIS; GRAPHENE NANOSHEETS; CYCLIC PERFORMANCE;
   GRAPHITE OXIDE; CARBON; CO3O4; ELECTRODES; NANOPARTICLES; COMPOSITE;
   STORAGE
AB Co3O4/graphene nanocomposite material was prepared by an in situ solution-based method under reflux conditions. In this reaction progress, Co2+ salts were converted to Co3O4 nanoparticles which were simultaneously inserted into the graphene layers, upon the reduction of graphite oxide to graphene. The prepared material consists of uniform Co3O4 nanoparticles (15-25 nm), which are well dispersed on the surfaces of graphene nanosheets. This has been confirmed through observations by field emission scanning electron microscopy, transmission electron microscopy and atomic force microscopy. The prepared composite material exhibits an initial reversible lithium storage capacity of 722 mAh g(-1) in lithium-ion cells and a specific supercapacitance of 478 F g(-1) in 2 M KOH electrolyte for supercapacitors, which were higher than that of the previously reported pure graphene nanosheets and Co3O4 nanoparticles. Co3O4/graphene nanocomposite material demonstrated an excellent electrochemical performance as an anode material for reversible lithium storage in lithium ion cells and as an electrode material in supercapacitors. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Wang, Bei; Wang, Ying; Wang, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Sydney, NSW 2007, Australia.
   [Park, Jinsoo; Ahn, Hyojun] Gyeongsang Natl Univ, Sch Mat Sci & Engn, Gyeongnam 660701, South Korea.
RP Wang, B (reprint author), Univ Technol Sydney, Sch Chem & Forens Sci, Sydney, NSW 2007, Australia.
EM Bei.Wang-1@student.uts.edu.au; Guoxiu.Wang@uts.edu.au
RI Wang,  Bei/J-6550-2012
OI Wang,  Bei/0000-0002-3793-0629
FU Australian Research Council (ARC) [DP1093855, LP0989134]; National
   Foundation of Korea through a World Class University (WCU)
   [R32-2008-000-20093-0]
FX We thank the Australian Research Council (ARC) for financial support
   through the ARC Discovery Project (DP1093855) and the ARC Linkage
   Project (LP0989134). We would also like to acknowledge the support from
   the National Foundation of Korea through a World Class University (WCU)
   Program (R32-2008-000-20093-0). Assoc. Prof. Alison Ung is highly
   appreciated for proofreading of the manuscript.
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NR 48
TC 81
Z9 86
U1 15
U2 116
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD JUL 21
PY 2011
VL 509
IS 29
BP 7778
EP 7783
DI 10.1016/j.jallcom.2011.04.152
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 775PJ
UT WOS:000291473500025
ER

PT J
AU Ding, ZJ
   Zhao, L
   Suo, LM
   Jiao, Y
   Meng, S
   Hu, YS
   Wang, ZX
   Chen, LQ
AF Ding, Zijing
   Zhao, Liang
   Suo, Liumin
   Jiao, Yang
   Meng, Sheng
   Hu, Yong-Sheng
   Wang, Zhaoxiang
   Chen, Liquan
TI Towards understanding the effects of carbon and nitrogen-doped carbon
   coating on the electrochemical performance of Li4Ti5O12 in lithium ion
   batteries: a combined experimental and theoretical study
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID AB-INITIO; ELECTRONIC-PROPERTIES; STORAGE DEVICES; LIFEPO4; SPINEL;
   ANODE; GROWTH
AB We investigate the effects of carbon coating, with and without nitrogen-dopants, on the electrochemical performance of a promising anode material Li4Ti5O12 (LTO) in lithium ion battery applications. The comparative experimental results show that LTO samples coated with nitrogen-doped carbon derived from pyridine and an ionic liquid exhibit significant improvements in rate capability and cycling performance compared with a LTO sample coated by carbon derived from toluene and the pristine LTO sample. For the first time, we construct an atomistic model for the interface between the lithium transition metal oxide and carbon coating layers. Our first-principles calculations based on density functional theory reveal that at this interface there is strong binding between the graphene coating layer and the Ti-terminated LTO surface, which significantly reduces the chemical activity of LTO surfaces and stabilizes the electrode/electrolyte interface, providing a clue to solve the swelling problem for LTO-based batteries. More importantly, electron transfer from the LTO surface to graphene greatly improves the electric conductivity of the interface. Nitrogen-dopants in graphene coatings further increase the interfacial stability and electric conductivity, which is beneficial to the electrochemical performance in energy storage applications.
C1 [Ding, Zijing; Zhao, Liang; Suo, Liumin; Jiao, Yang; Meng, Sheng; Hu, Yong-Sheng; Wang, Zhaoxiang; Chen, Liquan] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
RP Meng, S (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
EM smeng@aphy.iphy.ac.cn; yshu@aphy.iphy.ac.cn
RI ZHAO, LIANG/G-6059-2011; Meng, Sheng/A-7171-2010; Hu,
   Yong-Sheng/H-1177-2011
OI Hu, Yong-Sheng/0000-0002-8430-6474
FU Chinese Academy of Sciences [KJCX2-YW-W26]; "863" Project
   [2009AA033101]; "973" Projects [2007CB936500, 2010CB833102]; NSFC
   [50972164]
FX We acknowledge helpful discussions with Drs Hong Li, Chuying Ouyang and
   Hong Wei. This work was supported by funding from the 100 Talent Project
   of the Chinese Academy of Sciences, "863" Project (2009AA033101), "973"
   Projects (2007CB936500, 2010CB833102), NSFC (50972164) and CAS project
   (KJCX2-YW-W26).
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NR 35
TC 81
Z9 84
U1 22
U2 139
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2011
VL 13
IS 33
BP 15127
EP 15133
DI 10.1039/c1cp21513b
PG 7
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 807AK
UT WOS:000293860500034
PM 21789334
ER

PT J
AU Lv, W
   Sun, F
   Tang, DM
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   Liu, C
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   Cheng, HM
AF Lv, Wei
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   Tang, Dai-Ming
   Fang, Hai-Tao
   Liu, Chang
   Yang, Quan-Hong
   Cheng, Hui-Ming
TI A sandwich structure of graphene and nickel oxide with excellent
   supercapacitive performance
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM ION BATTERIES; ELECTROCHEMICAL PROPERTIES; REVERSIBLE CAPACITY;
   NANOCOMPOSITE; ANODE; RUO2
AB Hybrid structures combining graphene nanosheets (GNSs) and metal oxide nanoparticles (NPs) are increasingly attracting researchers due to their potential applications in electrochemical energy storage. Such hybrid structures reported thus far are mostly in random organizations of nanosheets anchored with NPs and macroscopically exist in powder aggregates. In this work, a sandwich structure of GNSs and oxide NPs that are macroscopically a free-standing membrane is reported, and a multi-step strategy conducted under "homogenous" and "mild" conditions is developed to ensure the successful fabrication of the membrane-like structure. Both components, tightly fixed NPs and planar GNSs as the skeleton of such sandwich structures, can avoid aggregation or stacking during electrochemical charge-discharge cycling, which effectively maintains the active surface and leaves stable and open channels for ion transport. Such a layered sandwich structure also acts as an ideal strain buffer to accommodate volume changes of the NPs in a fixed direction, and thus has a better resilience and structural stability in the electrochemical charge/discharge process. Hence, such a GNS/NP sandwich structure represents an ideal structure for electrochemical energy storage and a solution for easy manipulation for various applications due to the membrane morphology.
C1 [Lv, Wei; Sun, Feng; Yang, Quan-Hong] Tianjin Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Green Chem Technol, Tianjin 300072, Peoples R China.
   [Tang, Dai-Ming; Liu, Chang; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
   [Fang, Hai-Tao] Harbin Inst Technol, Sch Mat Sci & Engn, Harbin 150001, Peoples R China.
RP Yang, QH (reprint author), Tianjin Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Green Chem Technol, Tianjin 300072, Peoples R China.
EM qhyangcn@tju.edu.cn
RI Tang, Dai-Ming/B-6641-2011; Cheng, Hui-Ming/B-8682-2012; Liu,
   Chang/G-4667-2012; Lv, Wei/M-1964-2013
OI Tang, Dai-Ming/0000-0001-7136-7481; Lv, Wei/0000-0003-0874-3477
FU National Natural Science Foundation of China [50972101, 51072131];
   Specialized Research Fund for the Doctoral Program of Higher Education
   [20090032110014]; SRF for ROCS (SEM); Foundation of State Key Laboratory
   of Coal Conversion [10-11-913]; Program of Introducing Talents of
   Discipline to Universities, China [B06006]
FX We appreciate the support from the National Natural Science Foundation
   of China (no. 50972101 and 51072131), the Specialized Research Fund for
   the Doctoral Program of Higher Education (no. 20090032110014), the
   Project sponsored by SRF for ROCS (SEM), the Foundation of State Key
   Laboratory of Coal Conversion (Grant no. 10-11-913) and the Program of
   Introducing Talents of Discipline to Universities (no. B06006), China.
CR Geim AK, 2007, NAT MATER, V6, P183, DOI 10.1038/nmat1849
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NR 27
TC 81
Z9 85
U1 9
U2 86
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 25
BP 9014
EP 9019
DI 10.1039/c1jm10400d
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 777JK
UT WOS:000291611600014
ER

PT J
AU Zhong, HX
   Yang, GZ
   Song, HW
   Liao, QY
   Cui, H
   Shen, PK
   Wang, CX
AF Zhong, Haoxiang
   Yang, Gongzheng
   Song, Huawei
   Liao, Qingyu
   Cui, Hao
   Shen, Peikang
   Wang, Cheng-Xin
TI Vertically Aligned Graphene-Like SnS2 Ultrathin Nanosheet Arrays:
   Excellent Energy Storage, Catalysis, Photoconduction, and Field-Emitting
   Performances
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID LITHIUM-ION BATTERIES; THIN-FILM ANODE; FLOWERLIKE SNS2; NANOSTRUCTURES;
   NANOPARTICLES; NANOTUBES; PROPERTY; CAPACITY
AB New layered SnS2 nanosheet arrays consisting of 1-5 atomic layers were synthesized directly on Sn foil as both the tin source and the metal current collector substrates by a simple biomolecule-assisted method. It is found that SnS2 nanosheets synthesized have excellent photoelectric applications, such as on lithium ion batteries, and photocatalytic, field emission, and photoconductive properties. Cyclic voltammetry and discharge and charge behaviors of the atomic SnS2 nanosheets were examined, and it shows that the average discharge capacity in 1050 mAh/g is much larger than the theoretical capacity at the 1C rate. The photocatalytic action driven by solar light is quite quick, and the degradation rate of RhB is 90%, only irradiated for 20 min when the content of SnS2 nanosheets is 0.4 g/L. The response of the SnS2 device to the incidence UV light is very fast and shows excellent photosensitivity and stability. In addition, field emission properties of SnS2 nanosheets were also researched, and we found that the turn-on field for SnS2 is 6.9 V/mu m, which lowered ever reported values. The enhanced photoelectric properties are likely to originate in a graphene-like structure. Thus, graphene-like SnS2 materials are promising candidates in the photoelectric field.
C1 [Zhong, Haoxiang; Yang, Gongzheng; Song, Huawei; Liao, Qingyu; Cui, Hao; Shen, Peikang; Wang, Cheng-Xin] Sun Yat Sen Zhongshan Univ, State Key Lab Optoelect Mat & Technol, Sch Phys Sci & Engn, Guangzhou 510275, Guangdong, Peoples R China.
   [Shen, Peikang; Wang, Cheng-Xin] Sun Yat Sen Zhongshan Univ, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China.
RP Shen, PK (reprint author), Sun Yat Sen Zhongshan Univ, State Key Lab Optoelect Mat & Technol, Sch Phys Sci & Engn, Guangzhou 510275, Guangdong, Peoples R China.
EM stsspk@mail.sysu.edu.cn; wchengx@mail.sysu.edu.cn
RI Shen, Pei Kang/O-2004-2013; Song, Huawei/K-7097-2014
FU National Nature Science Foundation of China [51125008, 50772135];
   Doctoral Foundation [200805580018]; China Postdoctoral Science
   Foundation [20100470946]
FX The National Nature Science Foundation of China (51125008 and 50772135)
   and Doctoral Foundation (200805580018) and China Postdoctoral Science
   Foundation (20100470946) supported this work.
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NR 41
TC 80
Z9 80
U1 34
U2 284
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD APR 26
PY 2012
VL 116
IS 16
BP 9319
EP 9326
DI 10.1021/jp301024d
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 930VY
UT WOS:000303173900056
ER

PT J
AU Ji, JY
   Ji, HX
   Zhang, LL
   Zhao, X
   Bai, X
   Fan, XB
   Zhang, FB
   Ruoff, RS
AF Ji, Junyi
   Ji, Hengxing
   Zhang, Li Li
   Zhao, Xin
   Bai, Xin
   Fan, Xiaobin
   Zhang, Fengbao
   Ruoff, Rodney S.
TI Graphene-Encapsulated Si on Ultrathin-Graphite Foam as Anode for High
   Capacity Lithium-Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE Si; ultrathin-graphite foam; three-dimensional electrode; conductive
   network; lithium ion battery
ID SILICON NANOPARTICLES; ENERGY-STORAGE; ELECTRODES; CATHODE; NANOSPHERES;
   PERFORMANCE
C1 [Ji, Junyi; Ji, Hengxing; Zhang, Li Li; Zhao, Xin; Bai, Xin; Ruoff, Rodney S.] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA.
   [Ji, Junyi; Ji, Hengxing; Zhang, Li Li; Zhao, Xin; Bai, Xin; Ruoff, Rodney S.] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA.
   [Ji, Junyi; Fan, Xiaobin; Zhang, Fengbao] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
RP Ji, HX (reprint author), Univ Texas Austin, Dept Mech Engn, 1 Univ Stn C2200, Austin, TX 78712 USA.
EM jihengx@mail.utexas.edu; r.ruoff@mail.utexas.edu
RI Ji, Hengxing/B-5041-2009; Zhang, lili/J-4905-2015; Ruoff,
   Rodney/K-3879-2015
OI Ji, Hengxing/0000-0003-2851-9878; 
FU U.S. Department of Energy (DOE) [DE-AR0000178]; China Scholarship
   Council
FX We appreciate support from the U.S. Department of Energy (DOE) under
   award ARPA-E contract DE-AR0000178. Junyi Ji is supported by the China
   Scholarship Council Fellowship. We also appreciate comments by Prof.
   Guihua Yu.
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NR 38
TC 79
Z9 79
U1 48
U2 298
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD SEP 6
PY 2013
VL 25
IS 33
BP 4673
EP 4677
DI 10.1002/adma.201301530
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 261VM
UT WOS:000327692700024
PM 23847098
ER

PT J
AU Zhou, XS
   Dai, ZH
   Liu, SH
   Bao, JC
   Guo, YG
AF Zhou, Xiaosi
   Dai, Zhihui
   Liu, Shuhu
   Bao, Jianchun
   Guo, Yu-Guo
TI Ultra-Uniform SnOx/Carbon Nanohybrids toward Advanced Lithium-Ion
   Battery Anodes
SO ADVANCED MATERIALS
LA English
DT Article
ID CORE-SHELL NANOPARTICLES; HOLLOW NANOSPHERES; ELECTROCHEMICAL IMPEDANCE;
   RECHARGEABLE BATTERIES; TIN-NANOPARTICLES; COMPOSITE ANODES; GRAPHENE
   SHEETS; STORAGE; SILICON; PERFORMANCE
AB Ultra-uniform SnOx/carbon nanohybrids for lithium-ion batteries are successfully prepared by solvent replacement and subsequent electrospinning. The resulting 1D nanostructure with Sn-N bonding between the SnOx and N-containing carbon nanofiber matrix can not only tolerate the substantial volume change and suppress the aggregation of SnOx, but also enhances the transport of both electrons and ions for the embedded SnOx, thus leading to high cycling performance and rate capability.
C1 [Zhou, Xiaosi; Dai, Zhihui; Bao, Jianchun] Nanjing Normal Univ, Jiangsu Key Lab Biofunct Mat, Sch Chem & Mat Sci, Nanjing 210023, Jiangsu, Peoples R China.
   [Guo, Yu-Guo] Chinese Acad Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, BNLMS, Inst Chem, Beijing 100190, Peoples R China.
   [Liu, Shuhu] Chinese Acad Sci, BSRF, IHEP, Beijing 100049, Peoples R China.
RP Zhou, XS (reprint author), Nanjing Normal Univ, Jiangsu Key Lab Biofunct Mat, Sch Chem & Mat Sci, Nanjing 210023, Jiangsu, Peoples R China.
EM zhouxiaosi@njnu.edu.cn; ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2012CB932900];
   National Natural Science Foundation of China [51225204, 91127044,
   21121063, 21127901]; "Strategic Priority Research Program" of the
   Chinese Academy of Sciences [XDA09010102]; Priority Academic Program
   Development of Jiangsu Higher Education Institutions; Program for
   Jiangsu Collaborative Innovation Center of Biomedical Functional
   Materials
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2011CB935700 and 2012CB932900), the National Natural Science
   Foundation of China (Grant Nos. 51225204, 91127044, 21121063, and
   21127901), and the "Strategic Priority Research Program" of the Chinese
   Academy of Sciences (Grant No. XDA09010102). We also appreciate the
   financial support from the Priority Academic Program Development of
   Jiangsu Higher Education Institutions and the Program for Jiangsu
   Collaborative Innovation Center of Biomedical Functional Materials.
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NR 60
TC 78
Z9 78
U1 65
U2 300
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD JUN 18
PY 2014
VL 26
IS 23
BP 3943
EP 3949
DI 10.1002/adma.201400173
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AJ4CS
UT WOS:000337618600021
PM 24664966
ER

PT J
AU Chang, JB
   Huang, XK
   Zhou, GH
   Cui, SM
   Hallac, PB
   Jiang, JW
   Hurley, PT
   Chen, JH
AF Chang, Jingbo
   Huang, Xingkang
   Zhou, Guihua
   Cui, Shumao
   Hallac, Peter B.
   Jiang, Junwei
   Hurley, Patrick T.
   Chen, Junhong
TI Multilayered Si Nanoparticle/Reduced Graphene Oxide Hybrid as a
   High-Performance Lithium-Ion Battery Anode
SO ADVANCED MATERIALS
LA English
DT Article
ID LONG CYCLE LIFE; SILICON NANOPARTICLES; RATE CAPABILITY; NANOCOMPOSITE;
   ELECTRODE; SPECTROSCOPY; CHALLENGES; NANOWIRES; STORAGE; SHEETS
AB Multilayered Si/RGO anode nanostructures, featuring alternating Si nanoparticle (NP) and RGO layers, good mechanical stability, and high electrical conductivity, allow Si NPs to easily expand between RGO layers, thereby leading to high reversible capacity up to 2300 mAh g(-1) at 0.05 C (120 mA g(-1)) and 87% capacity retention (up to 630 mAh g(-1)) at 10 C after 152 cycles.
C1 [Chang, Jingbo; Huang, Xingkang; Zhou, Guihua; Cui, Shumao; Chen, Junhong] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA.
   [Hallac, Peter B.; Jiang, Junwei; Hurley, Patrick T.] Johnson Controls, Power Solut, Global Technol & Innovat, Milwaukee, WI 53209 USA.
RP Chen, JH (reprint author), Univ Wisconsin, Dept Mech Engn, 3200 North Cramer St, Milwaukee, WI 53211 USA.
EM jhchen@uwm.edu
RI Cui, Shumao/O-2987-2013; Chang, Jingbo/F-8088-2014
FU U.S. Department of Energy [DE-EE0003208]; Johnson Controls, Inc.
FX Financial support for this work was provided by the U.S. Department of
   Energy (DE-EE0003208) and Johnson Controls, Inc. The SEM imaging was
   conducted at the UWM Bioscience Electron Microscope Facility. The
   authors thank Dr. H. A. Owen for technical support with SEM analysis.
CR Zhou XS, 2012, ADV ENERGY MATER, V2, P1086, DOI 10.1002/aenm.201200158
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NR 50
TC 78
Z9 79
U1 52
U2 258
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD FEB 5
PY 2014
VL 26
IS 5
BP 758
EP 764
DI 10.1002/adma.201302757
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AH3RT
UT WOS:000336043500013
PM 24115353
ER

PT J
AU Yang, S
   Yue, WB
   Zhu, J
   Ren, Y
   Yang, XJ
AF Yang, Sheng
   Yue, Wenbo
   Zhu, Jia
   Ren, Yu
   Yang, Xiaojing
TI Graphene-Based Mesoporous SnO2 with Enhanced Electrochemical Performance
   for Lithium-Ion Batteries
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE composite materials; electrodes; hierarchical structures; porous
   materials; batteries
ID HIGH-CAPACITY; ANODE MATERIALS; STORAGE; OXIDE; NANOPARTICLES;
   MICROSPHERES; ELECTRODES; DEPOSITION; NANOWIRES; COMPOSITE
AB Graphene-based metal oxides generally show outstanding electrochemical performance due to the superior properties of graphene. However, the aggregation of active metal oxide nanoparticles on the graphene surface may result in a capacity fading and poor cycle performance. Here, a mesostructured graphene-based SnO2 composite is prepared through in situ growth of SnO2 particles on the graphene surface using cetyltrimethylammonium bromide as the structure-directing agent. This novel mesoporous composite inherits the advantages of graphene nanosheets and mesoporous materials and exhibits higher reversible capacity, better cycle performance, and better rate capability compared to pure mesoporous SnO2 and graphene-based nonporous SnO2. It is concluded that the synergetic effect between graphene and mesostructure benefits the improvement of the electrochemical properties of the hybrid composites. This facile method may offer an attractive alternative approach for preparation of the graphene-based mesoporous composites as high- performance electrodes for lithium-ion batteries.
C1 [Yang, Sheng; Yue, Wenbo; Zhu, Jia; Yang, Xiaojing] Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China.
   [Ren, Yu] Natl Inst Clean & Low Carbon Energy, Beijing 102209, Peoples R China.
RP Yang, S (reprint author), Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China.
EM wbyue@bnu.edu.cn; yang.xiaojing@bnu.edu.cn
FU National Natural Science Foundation of China [20903013, 21101014,
   21273022, 51272030]; Beijing Municipal Natural Science Foundation
   [2112022]
FX This work is financially supported by National Natural Science
   Foundation of China (20903013, 21101014, 21273022 and 51272030) and
   Beijing Municipal Natural Science Foundation (2112022).
CR Yang S, 2012, RSC ADV, V2, P8827, DOI 10.1039/c2ra20746j
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NR 33
TC 78
Z9 80
U1 27
U2 162
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD JUL 26
PY 2013
VL 23
IS 28
BP 3570
EP 3576
DI 10.1002/adfm.201203286
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 258WS
UT WOS:000327490000011
ER

PT J
AU Gu, Y
   Xu, Y
   Wang, Y
AF Gu, Yan
   Xu, Yi
   Wang, Yong
TI Graphene-Wrapped CoS Nanoparticles for High-Capacity Lithium-Ion Storage
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE CoS; graphene nanosheets; nanocomposite; anode; lithium-ion battery
ID ANODE MATERIAL; ELECTROCHEMICAL PROPERTIES; BATTERIES; SULFIDE;
   NANOSTRUCTURES; REACTIVITY; NANOSHEETS; OXIDE
AB Graphene-wrapped CoS nanoparticles are synthesized by a solvothermal approach. The product is significantly different from porous CoS microspheres prepared in the absence of graphene under similar preparation conditions. The CoS microspheres and CoS/graphene composite are fabricated as anode materials for lithium-ion batteries. The CoS/graphene composite is found to be better suitable as an anode in terms of higher capacity and better cycling performances. The nanocomposite exhibits an unprecedented high reversible capacity of 1056 mA h/g among all cobalt sulfide-based anode materials, Good cycling performances are also observed at both small and high current rates.
C1 [Gu, Yan; Xu, Yi; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shanghai 200444, Peoples R China.
RP Wang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012
FU Program of Professor Special Appointment (Eastern Scholar); National
   Natural Science Foundation of China [51271105]; Shanghai Municipal
   Government [11JC1403900, 11SG38, S30109]
FX The authors gratefully acknowledge the Program of Professor Special
   Appointment (Eastern Scholar), the National Natural Science Foundation
   of China (51271105), Shanghai Municipal Government (11JC1403900, 11SG38,
   S30109) for financial support.
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NR 32
TC 78
Z9 78
U1 41
U2 298
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD FEB 13
PY 2013
VL 5
IS 3
BP 801
EP 806
DI 10.1021/am3023652
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 091WE
UT WOS:000315079700045
PM 23317533
ER

PT J
AU Wang, JJ
   Li, YL
   Sun, XL
AF Wang, Jiajun
   Li, Yongliang
   Sun, Xueliang
TI Challenges and opportunities of nanostructured materials for aprotic
   rechargeable lithium-air batteries
SO NANO ENERGY
LA English
DT Review
DE Lithium-air batteries; Nanomaterials; Catalysis; Electrochemistry;
   Cathode
ID OXYGEN REDUCTION REACTION; HIGH ELECTROCATALYTIC ACTIVITY; MULTIWALLED
   CARBON NANOTUBES; ORGANIC ELECTROLYTE BATTERY; DOPED GRAPHENE
   NANOSHEETS; ETHER-BASED ELECTROLYTES; MEMBRANE FUEL-CELLS; LI-AIR;
   LI-O-2 BATTERIES; POLYMER ELECTROLYTE
AB Rechargeable lithium-air (O-2) batteries have received much attention due to their extremely high theoretical energy densities, which far exceeds that of current lithium-ion batteries. The considerable high energy densities come from (i) pure metal lithium as anode and (ii) the cathode oxidant, oxygen, which comes from the surrounding air. However, there are still many scientific and technical challenges especially nanomaterial challenges to overcome before it turns into reality. In this review, the fundamental principles and understanding of the electrochemical reaction in the aprotic lithium-air batteries are first presented. We emphasized on the discussion of the nanomaterial's issues which prevent their practical implementation, including the material status and challenges from cathode, electrolyte, anode and other components. These problems will be discussed in detail and possible solutions are also suggested. Finally, we explore future research directions in the field of aprotic rechargeable lithium-air batteries. (c) 2012 Elsevier Ltd. All rights reserved.
C1 [Wang, Jiajun; Li, Yongliang; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Li, Yongliang/H-3179-2011; Sun, Xueliang/C-7257-2012; wang,
   jiajun/H-3315-2012
OI Li, Yongliang/0000-0002-5008-0868; 
FU Natural Sciences and Engineering Research Council of Canada; Canada
   Research Chair Program; Canada Foundation for Innovation; University of
   Western Ontario
FX This research was supported by the Natural Sciences and Engineering
   Research Council of Canada, the Canada Research Chair Program, the
   Canada Foundation for Innovation and the University of Western Ontario.
   The authors are also in debt to Linda Zhang and Ruijie Wang for their
   kind help and discussion.
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NR 197
TC 77
Z9 78
U1 73
U2 426
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD JUL
PY 2013
VL 2
IS 4
BP 443
EP 467
DI 10.1016/j.nanoen.2012.11.014
PG 25
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 198QI
UT WOS:000322937000006
ER

PT J
AU Su, LW
   Zhou, Z
   Qin, X
   Tang, QW
   Wu, DH
   Shen, PW
AF Su, Liwei
   Zhou, Zhen
   Qin, Xue
   Tang, Qiwei
   Wu, Dihua
   Shen, Panwen
TI CoCO3 submicrocube/graphene composites with high lithium storage
   capability
SO NANO ENERGY
LA English
DT Article
DE Anodes; Cobalt carbonate; Energy storage; Graphene; Lithium ion
   batteries
ID ION BATTERIES; ELECTROCHEMICAL REDUCTION; ELECTRODE MATERIALS;
   NEGATIVE-ELECTRODE; CARBON-DIOXIDE; CO2 REDUCTION; CAPACITY; SURFACES;
   GRAPHENE; ORIGIN
AB The composites of CoCO3 submicrocubes and graphene nanosheets (GNSs) were prepared through a solvothermal route and were tested as anode materials for lithium ion batteries. Profiting from the advantages of GNSs, CoCO3/GNS composites delivered high capacities of over 1000 mAh g(-1), much higher than theoretical values based on available lithium storage mechanisms. Instead, we propose an electrochemical catalytic conversion mechanism for lithium storage, in which not only cations (Co2+) but also anions (CO32-) are involved in the electron transfer. C4+ in CO32- is reduced to C-0 or other low-valence C under the electrochemical catalysis of newly-generated Co nanoparticles. This new mechanism may provide more clues for exploiting advanced materials for Li ion batteries and other energy storage devices. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Su, Liwei; Zhou, Zhen; Wu, Dihua; Shen, Panwen] Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Key Lab Adv Energy Mat Chem,Minist Educ, Tianjin 300071, Peoples R China.
   [Qin, Xue; Tang, Qiwei] Tianjin Univ, Dept Chem, Tianjin 300072, Peoples R China.
RP Zhou, Z (reprint author), Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Key Lab Adv Energy Mat Chem,Minist Educ, Tianjin 300071, Peoples R China.
EM zhouzhen@nankai.edu.cn
RI Zhou, Zhen/C-4517-2008; Su, Liwei/G-2295-2011
OI Zhou, Zhen/0000-0003-3232-9903; Su, Liwei/0000-0002-9791-3476
FU 973 Program [2009CB220100]; NSFC [21073096]; Fundamental Research Funds
   for the Central Universities in China
FX This work was supported by the 973 Program (2009CB220100), the NSFC
   (21073096), and the Fundamental Research Funds for the Central
   Universities in China.
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NR 27
TC 77
Z9 78
U1 36
U2 175
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAR
PY 2013
VL 2
IS 2
BP 276
EP 282
DI 10.1016/j.nanoen.2012.09.012
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 135VV
UT WOS:000318319700015
ER

PT J
AU Wang, RH
   Xu, CH
   Sun, J
   Gao, L
   Lin, CC
AF Wang, Ronghua
   Xu, Chaohe
   Sun, Jing
   Gao, Lian
   Lin, Chucheng
TI Flexible free-standing hollow Fe3O4/graphene hybrid films for
   lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-PERFORMANCE ANODE; REDUCED GRAPHENE; RATE CAPABILITY; STORAGE
   CAPACITY; FE3O4; OXIDE; NANOPARTICLES; ELECTRODE; COMPOSITE; PAPER
AB Flexible free-standing hollow Fe3O4/graphene (H-Fe3O4/GS) films were fabricated through vacuum filtration and thermal reduction processes, in which graphene formed a three-dimensional conductive network, with hollow and porous Fe3O4 spindles being captured and distributed homogeneously. Using the films as binder-free and free-standing electrodes for lithium-ion batteries, H-Fe3O4/GS with 39.6 wt % graphene exhibited a high specific capacity (1555 mA h g(-1) at 100 mA g(-1)), enhanced rate capability and excellent cyclic stability (940 and 660 mA h g(-1) at 200 and 500 mA g(-1) after 50 cycles, respectively). The superior electrochemical performance of this novel material can be attributed to two factors. One is that the three dimensional (3D) graphene network formed is very helpful for keeping H-Fe3O4 in good electrical contact. Another is the short transport length for both lithium ions and electrons due to the porous nature which accommodates volume change and favors electrolyte penetration. It is believed that the strategy for preparing free-standing H-Fe3O4/GS films presented in this work will provide new insight into the design and synthesis of other metal oxide/GS electrodes for flexible energy storage devices.
C1 [Wang, Ronghua; Xu, Chaohe; Sun, Jing; Gao, Lian; Lin, Chucheng] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
RP Wang, RH (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, 1295 Dingxi Rd, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU 973 Project [2012CB932303]; National Natural Science Foundation of China
   [50972153, 51072215, 51172261]
FX This work is supported by the 973 Project (2012CB932303), the National
   Natural Science Foundation of China (Grant no. 50972153, 51072215 and
   51172261).
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NR 52
TC 77
Z9 77
U1 35
U2 297
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 5
BP 1794
EP 1800
DI 10.1039/c2ta00753c
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085UP
UT WOS:000314640100037
ER

PT J
AU Wang, HL
   Liang, YY
   Gong, M
   Li, YG
   Chang, W
   Mefford, T
   Zhou, JG
   Wang, J
   Regier, T
   Wei, F
   Dai, HJ
AF Wang, Hailiang
   Liang, Yongye
   Gong, Ming
   Li, Yanguang
   Chang, Wesley
   Mefford, Tyler
   Zhou, Jigang
   Wang, Jian
   Regier, Tom
   Wei, Fei
   Dai, Hongjie
TI An ultrafast nickel-iron battery from strongly coupled inorganic
   nanoparticle/nanocarbon hybrid materials
SO NATURE COMMUNICATIONS
LA English
DT Article
ID LITHIUM ION BATTERIES; FLUIDIZED-BED REACTOR; OXYGEN REDUCTION; CARBON
   NANOTUBES; MASS-PRODUCTION; GRAPHENE; CHALLENGES; ELECTRODES; FUTURE;
   ANODE
AB Ultrafast rechargeable batteries made from low-cost and abundant electrode materials operating in safe aqueous electrolytes could be attractive for electrochemical energy storage. If both high specific power and energy are achieved, such batteries would be useful for power quality applications such as to assist propelling electric vehicles that require fast acceleration and intense braking. Here we develop a new type of Ni-Fe battery by employing novel inorganic nanoparticle/graphitic nanocarbon (carbon nanotubes and graphene) hybrid materials as electrode materials. We successfully increase the charging and discharging rates by nearly 1,000-fold over traditional Ni-Fe batteries while attaining high energy density. The ultrafast Ni-Fe battery can be charged in similar to 2 min and discharged within 30 s to deliver a specific energy of 120 Wh kg(-1) and a specific power of 15 kW kg(-1). These features suggest a new generation of Ni-Fe batteries as novel devices for electrochemical energy storage.
C1 [Wang, Hailiang; Liang, Yongye; Gong, Ming; Li, Yanguang; Chang, Wesley; Mefford, Tyler; Dai, Hongjie] Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
   [Zhou, Jigang; Wang, Jian; Regier, Tom] Canadian Light Source Inc, Saskatoon, SK S7N 0X4, Canada.
   [Wei, Fei] Tsinghua Univ, Dept Chem Engn, Beijing 100084, Peoples R China.
RP Dai, HJ (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
EM hdai@stanford.edu
RI Liang, Yongye/D-9275-2012; Wang, Jian/M-1805-2013; Li,
   Yanguang/A-2319-2014; Zhou, Jigang/N-6831-2014; Wei, Fei/H-4809-2012
OI Li, Yanguang/0000-0003-0506-0451; Zhou, Jigang/0000-0001-6644-2862; 
FU Intel; Stanford Precourt Institute for Energy; Stanford Graduate
   Fellowship; NSERC; NRC; CIHR of Canada; University of Saskatchewan
FX This work is supported by Intel, a Stinehart/Reed Award for Energy
   Research at Stanford from the Stanford Precourt Institute for Energy,
   and a Stanford Graduate Fellowship. CLS is supported by the NSERC, NRC,
   CIHR of Canada, and the University of Saskatchewan.
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NR 34
TC 77
Z9 78
U1 22
U2 264
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD JUN
PY 2012
VL 3
AR 917
DI 10.1038/ncomms1921
PG 8
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 970AG
UT WOS:000306099900044
PM 22735445
ER

PT J
AU Zou, F
   Hu, XL
   Li, Z
   Qie, L
   Hu, CC
   Zeng, R
   Jiang, Y
   Huang, YH
AF Zou, Feng
   Hu, Xianluo
   Li, Zhen
   Qie, Long
   Hu, Chenchen
   Zeng, Rui
   Jiang, Yan
   Huang, Yunhui
TI MOF-Derived Porous ZnO/ZnFe2O4/C Octahedra with Hollow Interiors for
   High-Rate Lithium-Ion Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE hollow structures; porous nanostructures; batteries; metal-organic
   frameworks
ID METAL-ORGANIC FRAMEWORKS; HIGH-PERFORMANCE ANODE; STORAGE CAPACITY;
   ENERGY-STORAGE; CARBON; NANOPARTICLES; GRAPHENE; MICROSPHERES;
   COMPOSITES; OXIDES
C1 [Zou, Feng; Hu, Xianluo; Li, Zhen; Qie, Long; Hu, Chenchen; Zeng, Rui; Jiang, Yan; Huang, Yunhui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
RP Hu, XL (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
EM huxl@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU Natural Science Foundation of China [21271078, 51002057]; NCET (Program
   for New Century Excellent Talents in University) [NECT-12-0223]
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 21271078 and 51002057) and NCET (Program for New Century
   Excellent Talents in University, No. NECT-12-0223).
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NR 39
TC 76
Z9 76
U1 143
U2 439
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD OCT 15
PY 2014
VL 26
IS 38
BP 6622
EP 6628
DI 10.1002/adma.201402322
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AR7MG
UT WOS:000343763200015
PM 25124234
ER

PT J
AU Li, L
   Wu, Z
   Yuan, S
   Zhang, XB
AF Li, Lin
   Wu, Zhong
   Yuan, Shuang
   Zhang, Xin-Bo
TI Advances and challenges for flexible energy storage and conversion
   devices and systems
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID LITHIUM-ION BATTERIES; SENSITIZED SOLAR-CELLS; ALL-SOLID-STATE; WALLED
   CARBON NANOTUBES; NANOSTRUCTURED CATHODE MATERIALS; RECHARGEABLE LI-O-2
   BATTERIES; PERFORMANCE ANODE MATERIAL; CHEMICAL-VAPOR-DEPOSITION;
   REDUCED GRAPHENE OXIDE; CARBIDE-DERIVED CARBON
AB To meet the rapid development of flexible, portable, and wearable electronic devices, extensive efforts have been devoted to develop matchable energy storage and conversion systems as power sources, such as flexible lithium-ion batteries (LIBs), supercapacitors (SCs), solar cells, fuel cells, etc. Particularly, during recent years, exciting works have been done to explore more suitable and effective electrode/electrolyte materials as well as more preferable cell configuration and structural designs to develop flexible power sources with better electrochemical performance for integration into flexible electronics. An overview is given for these remarkable contributions made by the leading scientists in this important and promising research area. Some perspectives for the future and impacts of flexible energy storage and conversion systems are also proposed.
C1 [Li, Lin; Wu, Zhong; Yuan, Shuang; Zhang, Xin-Bo] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Li, Lin; Yuan, Shuang] Jilin Univ, Minist Educ, Key Lab Automobile Mat, Changchun 130012, Peoples R China.
   [Li, Lin; Yuan, Shuang] Jilin Univ, Coll Mat Sci & Engn, Changchun 130012, Peoples R China.
   [Wu, Zhong] Univ Chinese Acad Sci, Beijing 100124, Peoples R China.
RP Li, L (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
EM xbzhang@ciac.ac.cn
RI ZHANG, Xinbo/G-8698-2011
OI ZHANG, Xinbo/0000-0002-5806-159X
FU Chinese Academy of Sciences, National Program on Key Basic Research
   Project of China (973 Program) [2014CB932300, 2012CB215500]; Foundation
   for Innovative Research Groups of the National Natural Science
   Foundation of China [20921002]; National Natural Science Foundation of
   China [21101147, 21203176]
FX This work is financially supported by 100 Talents Programme of The
   Chinese Academy of Sciences, National Program on Key Basic Research
   Project of China (973 Program, Grant no. 2014CB932300, 2012CB215500),
   Foundation for Innovative Research Groups of the National Natural
   Science Foundation of China (Grant no. 20921002), National Natural
   Science Foundation of China (Grant no. 21101147 and 21203176).
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NR 255
TC 76
Z9 77
U1 113
U2 492
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD JUL
PY 2014
VL 7
IS 7
BP 2101
EP 2122
DI 10.1039/c4ee00318g
PG 22
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AJ8SL
UT WOS:000337977600003
ER

PT J
AU Prabakar, SJR
   Hwang, YH
   Bae, EG
   Shim, S
   Kim, D
   Lah, MS
   Sohn, KS
   Pyo, M
AF Prabakar, S. J. Richard
   Hwang, Yun-Hwa
   Bae, Eun-Gyoung
   Shim, Sangdeok
   Kim, Dongwook
   Lah, Myoung Soo
   Sohn, Kee-Sun
   Pyo, Myoungho
TI SnO2/Graphene Composites with Self-Assembled Alternating Oxide and Amine
   Layers for High Li-Storage and Excellent Stability
SO ADVANCED MATERIALS
LA English
DT Article
DE tin dioxide; graphene; self assembly; anode; lithium ion batteries
ID LITHIUM-ION BATTERIES; GRAPHENE NANOSHEETS; HOLLOW SPHERES; PERFORMANCE;
   CAPACITY; ANODE; INSERTION; NANOSTRUCTURES; NANOCOMPOSITES; ADSORPTION
C1 [Prabakar, S. J. Richard; Hwang, Yun-Hwa; Bae, Eun-Gyoung; Pyo, Myoungho] Sunchon Natl Univ, Dept Printed Elect Engn, World Class Univ WCU Program, Sunchon 540742, Chonnam, South Korea.
   [Shim, Sangdeok] Sunchon Natl Univ, Dept Chem & Premed, Sunchon 540742, Chonnam, South Korea.
   [Kim, Dongwook; Lah, Myoung Soo] Ulsan Natl Inst Sci & Technol, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea.
   [Sohn, Kee-Sun] Sejong Univ, Fac Nanotechnol & Adv Mat Engn, Seoul 143747, South Korea.
RP Sohn, KS (reprint author), Sejong Univ, Fac Nanotechnol & Adv Mat Engn, Seoul 143747, South Korea.
EM sksohn@sejong.ac.kr; mho@sunchon.ac.kr
RI Lah, Myoung Soo/E-5885-2010
FU WCU program through the Korea Science and Engineering Foundation;
   Ministry of Education, Science and Technology [R31-10022]
FX This research was supported by the WCU program through the Korea Science
   and Engineering Foundation funded by the Ministry of Education, Science
   and Technology (R31-10022).
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NR 41
TC 76
Z9 76
U1 30
U2 386
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD JUN 25
PY 2013
VL 25
IS 24
BP 3307
EP 3312
DI 10.1002/adma.201301264
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 168UT
UT WOS:000320732000004
PM 23670979
ER

PT J
AU Poh, HL
   Simek, P
   Sofer, Z
   Pumera, M
AF Poh, Hwee Ling
   Simek, Petr
   Sofer, Zdenek
   Pumera, Martin
TI Sulfur-Doped Graphene via Thermal Exfoliation of Graphite Oxide in H2S,
   SO2, or CS2 Gas
SO ACS NANO
LA English
DT Article
DE graphene; doping; sulfur; gas phase; electrochemistry
ID LITHIUM-ION BATTERIES; ANODE MATERIALS; SHEETS; COMPOSITE; FILMS
AB Doping of graphene with heteroatoms is an effective way to tailor its properties. Here we describe a simple and scalable method of doping graphene lattice with sulfur atoms during the thermal exfoliation process of graphite oxides. The graphite oxides were first prepared by Staudenmaler, Hofmann, and Hummers methods followed by treatments in hydrogen sulfide, sulfur dioxide, or carbon disulfide. The doped materials were characterized by scanning electron microscopy, high-resolution X-ray photoelectron spectroscopy, combustible elemental analysis, and Raman spectroscopy. The zeta-potential and conductivity of sulfur-doped graphenes were also investigated in this paper. It was found that the level of doping is more dramatically Influenced by the type of graphite oxide used rather than the type of sulfur-containing gas used during exfoliation. Resulting sulfur-doped graphenes act as metal-free electrocatalysts for oxygen reduction reaction.
C1 [Poh, Hwee Ling; Pumera, Martin] Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore 637371, Singapore.
   [Simek, Petr; Sofer, Zdenek] Inst Chem Technol, Dept Inorgan Chem, CR-16628 Prague 6, Czech Republic.
RP Pumera, M (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Chem & Biol Chem, Singapore 637371, Singapore.
EM pumera@ntu.edu.sg
RI Pumera, Martin/F-2724-2010; Sofer, Zdenek/A-9690-2010
OI Pumera, Martin/0000-0001-5846-2951; 
FU MINDEF/NTU fund [JPP 11/02/06]; Ministry of Education of the Czech
   Republic [MSM6046137302]; Specific University Research grant (MSMT)
   [20/2013]
FX M.P. thanks MINDEF/NTU fund JPP 11/02/06 and JSPS-NTU fund. Z.S. and
   P.S. thank the Ministry of Education of the Czech Republic (Project No.
   MSM6046137302) and the Specific University Research grant (MSMT No.
   20/2013).
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NR 32
TC 76
Z9 76
U1 47
U2 318
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD JUN
PY 2013
VL 7
IS 6
BP 5262
EP 5272
DI 10.1021/nn401296b
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 173QK
UT WOS:000321093800062
PM 23656223
ER

PT J
AU Wang, B
   Li, XL
   Zhang, XF
   Luo, B
   Zhang, YB
   Zhi, LJ
AF Wang, Bin
   Li, Xianglong
   Zhang, Xianfeng
   Luo, Bin
   Zhang, Yunbo
   Zhi, Linjie
TI Contact-Engineered and Void-Involved Silicon/Carbon Nanohybrids as
   Lithium-Ion-Battery Anodes
SO ADVANCED MATERIALS
LA English
DT Article
DE nanohybrids; nanostructured silicon; graphitic tubes; line-to-line
   contact; lithium-ion batteries
ID SI NANOPARTICLES; GRAPHENE SHEETS; NANOWIRES; NANOCOMPOSITES; STORAGE;
   FABRICATION; ELECTRODES; PARTICLES; SPACE
C1 [Wang, Bin; Li, Xianglong; Zhang, Xianfeng; Luo, Bin; Zhang, Yunbo; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Li, XL (reprint author), Natl Ctr Nanosci & Technol, 11 Beiyitiao Zhongguancun, Beijing 100190, Peoples R China.
EM lixl@nanoctr.cn; zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [21173057, 21273054];
   Ministry of Science and Technology of China [2012CB933400,
   2012CB933403]; Beijing Municipal Science and Technology Commission
   [Z121100006812003]; Chinese Academy of Sciences
FX Financial support from the National Natural Science Foundation of China
   (Grant No. 21173057, 21273054), the Ministry of Science and Technology
   of China (No. 2012CB933400 and No. 2012CB933403), the Beijing Municipal
   Science and Technology Commission (No. Z121100006812003), and the
   Chinese Academy of Sciences is acknowledged. The authors also
   acknowledge kind help of Dr. S. T. Picraux at Los Alamos National
   Laboratory.
CR Zhou XS, 2012, ADV ENERGY MATER, V2, P1086, DOI 10.1002/aenm.201200158
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NR 37
TC 75
Z9 75
U1 25
U2 179
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD JUL 12
PY 2013
VL 25
IS 26
BP 3560
EP 3565
DI 10.1002/adma.201300844
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 262PN
UT WOS:000327749300007
PM 23712858
ER

PT J
AU Xia, H
   Zhu, DD
   Fu, YS
   Wang, X
AF Xia, Hui
   Zhu, Dongdong
   Fu, Yongsheng
   Wang, Xin
TI CoFe2O4-graphene nanocomposite as a high-capacity anode material for
   lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Cobalt ferrite; Graphene; Anode material; Lithium-ion batteries;
   Nanocomposite
ID GRAPHENE; PERFORMANCE; HYBRID; CARBON; OXIDE; COMPOSITE; ELECTRODE;
   NANOPARTICLES; COFE2O4; STORAGE
AB A straightforward hydrothermal strategy is designed for the fabrication of CoFe2O4-graphene nanocomposites with different graphene contents. Due to the synergetic effect between the conducting graphene nanosheets and CoFe2O4 nanoparticles, the nanocomposites exhibit promising electrochemical performance as anode material for lithium-ion batteries. It is found that the graphene content plays an important role in tuning the electrochemical performance of the nanocomposite. With 20 wt% graphene, the CoFe2O4-graphene nanocomposite electrode can deliver a high reversible specific capacity up to 1082 mAh g(-1) as well as excellent cycling stability and rate capability. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Xia, Hui; Zhu, Dongdong] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China.
   [Xia, Hui; Fu, Yongsheng; Wang, Xin] Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Jiangsu, Peoples R China.
RP Xia, H (reprint author), Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Xiaolingwei 200, Nanjing 210094, Jiangsu, Peoples R China.
EM xiahui@njust.edu.cn; wxin@public1.ptt.js.cn
RI Zhu, Dongdong/F-2929-2014; 
OI Xia, Hui/0000-0002-2517-2410
FU National Natural Science Foundation of China [21171094, 51102134];
   Priority Academic Program Development of Jiangsu Higher Education
   Institutions; NUST [2011PYXM03, 2011ZDJH21]; Department of Education of
   Jiangsu Province [CXZZ11_0245]
FX This investigation was supported by the National Natural Science
   Foundation of China (No. 21171094, 51102134), A Project Funded by the
   Priority Academic Program Development of Jiangsu Higher Education
   Institutions, NUST Research Funding (2011PYXM03, 2011ZDJH21) and the
   Department of Education of Jiangsu Province (CXZZ11_0245).
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NR 44
TC 75
Z9 75
U1 19
U2 176
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD NOV 30
PY 2012
VL 83
BP 166
EP 174
DI 10.1016/j.electacta.2012.08.027
PG 9
WC Electrochemistry
SC Electrochemistry
GA 040MN
UT WOS:000311327100022
ER

PT J
AU Kottegoda, IRM
   Idris, NH
   Lu, L
   Wang, JZ
   Liu, HK
AF Kottegoda, Iresha R. M.
   Idris, Nurul Hayati
   Lu, Lin
   Wang, Jia-Zhao
   Liu, Hua-Kun
TI Synthesis and characterization of graphene-nickel oxide nanostructures
   for fast charge-discharge application
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE NiO nanoparticles; Graphene; Nickel oxide-graphene composites; Lithium
   batteries
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; REVERSIBLE CAPACITY; ELECTRODE
   MATERIALS; CYCLIC PERFORMANCE; ENERGY-STORAGE; GRAPHITE OXIDE; LI
   STORAGE; COMPOSITE; NIO
AB Graphene-metal oxide composites as anode materials for Li-ion batteries have been investigated extensively, but these attempts are mostly limited to moderate rate charge-discharge applications. Here, graphene-nickel oxide nanostructures have been synthesised using a controlled hydrothermal method, which enabled in situ formation of NiO with a coralloid nanostructure on graphene. Graphene/NiO (20%), graphene/NiO (50%) and pure NiO show stable discharge capacities of 185 mAh/g at 20 C (1 C = 300 mA/g), 450 mAh/g at 1 C, and 400 mAh/g at 1 C, respectively. High rate capability and good stability in prolonged charge-discharge cycling permit the application of the material in fast charging batteries for upcoming electric vehicles. To the best of our knowledge such fast rate performance of graphene/metal oxide composite as anode and such stability for pure NiO as anode have not been reported previously. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Kottegoda, Iresha R. M.; Idris, Nurul Hayati; Lu, Lin; Wang, Jia-Zhao; Liu, Hua-Kun] Univ Wollongong, Inst Superconducting & Elect Mat, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2519, Australia.
   [Idris, Nurul Hayati] Univ Malaysia Terengganu, Fac Sci, Dept Phys Sci, Kuala Terengganu 21030, Malaysia.
RP Kottegoda, IRM (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2519, Australia.
EM iresha@iti.lk; jiazhao@uow.edu.au
RI Wang, Jiazhao/G-4972-2011; Liu, Hua/G-1349-2012; Idris, Nurul Hayati
   /K-4915-2012
OI Liu, Hua/0000-0002-0253-647X; 
FU Australian Government; Australian Research Council (ARC) [DP 0987805];
   Ministry of Higher Education of the Government of Malaysia
FX The first author is grateful for fellowship support from the Australian
   Government funded Endeavour Research Award. Financial support was also
   provided by the Australian Research Council (ARC) through a Discovery
   Project (DP 0987805). Nurul Hayati Idris is grateful to the Ministry of
   Higher Education of the Government of Malaysia for SLAB/SLAI scholarship
   support. We thank Darren Attard for his invaluable support for field
   emission scanning electron microscopy and Raman spectroscopy. The
   authors would also like to thank Dr. Tania Silver for critical reading
   and correction of this manuscript.
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NR 48
TC 75
Z9 76
U1 14
U2 108
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JUN 30
PY 2011
VL 56
IS 16
BP 5815
EP 5822
DI 10.1016/j.electacta.2011.03.143
PG 8
WC Electrochemistry
SC Electrochemistry
GA 788EK
UT WOS:000292428000052
ER

PT J
AU Kim, HK
   Bak, SM
   Kim, KB
AF Kim, Hyun-Kyung
   Bak, Seong-Min
   Kim, Kwang-Bum
TI Li4Ti5O12/reduced graphite oxide nano-hybrid material for high rate
   lithium-ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Li4Ti5O12; Reduced graphite oxide; Li4Ti5O12/reduced graphite oxide
   nano-hybrid; Microwave-assisted solvothermal reaction; Li-ion battery
ID ANODE MATERIAL; DISPERSION; GRAPHENE; TIO2
AB A spinel Li4Ti5O12 nanoplatelet/reduced graphite oxide nano-hybrid was successfully synthesized by a two-step microwave-assisted solvothermal reaction and heat treatment. The Li4Ti5O12 in the hybrid could deliver a discharge capacity of 154 mAhg(-1) of Li4Ti5O12 at 1 C-rate, 128 mAhg(-1) of Li4Ti5O12 at 50 C-rate and 101 mAhg(-1) of Li4Ti5O12 at 100 C-rate. It demonstrated promising potential as an anode material in a Li-ion battery with excellent rate capability and good cycling. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Kim, Hyun-Kyung; Bak, Seong-Min; Kim, Kwang-Bum] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea.
RP Kim, KB (reprint author), Yonsei Univ, Dept Mat Sci & Engn, 134 Shinchon Dong, Seoul 120749, South Korea.
EM kbkim@yonsei.ac.kr
RI Bak, Seong Min/J-4597-2013
FU Ministry of Science and Technology [R0A- 2007-000-10042-0]; GS Caltex
   Corporation
FX This work was supported by Korea Science and Engineering Foundation
   (KOSEF) through the National Research Lab. Program funded by the
   Ministry of Science and Technology (No. R0A- 2007-000-10042-0). The
   authors would like to thank GS Caltex Corporation for financial support
   of this research.
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NR 19
TC 75
Z9 76
U1 10
U2 94
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD DEC
PY 2010
VL 12
IS 12
BP 1768
EP 1771
DI 10.1016/j.elecom.2010.10.018
PG 4
WC Electrochemistry
SC Electrochemistry
GA 702OT
UT WOS:000285904700026
ER

PT J
AU Wang, TS
   Liu, ZH
   Lu, MM
   Wen, B
   Ouyang, QY
   Chen, YJ
   Zhu, CL
   Gao, P
   Li, CY
   Cao, MS
   Qi, LH
AF Wang, Tieshi
   Liu, Zhaohong
   Lu, Mingming
   Wen, Bo
   Ouyang, Qiuyun
   Chen, Yujin
   Zhu, Chunling
   Gao, Peng
   Li, Chunyan
   Cao, Maosheng
   Qi, Lihong
TI Graphene-Fe3O4 nanohybrids: Synthesis and excellent electromagnetic
   absorption properties
SO JOURNAL OF APPLIED PHYSICS
LA English
DT Article
ID LITHIUM ION BATTERIES; CORE/SHELL NANORODS SYNTHESIS;
   MICROWAVE-ABSORPTION; CARBON NANOTUBES; REVERSIBLE CAPACITY; FE3O4
   NANOPARTICLES; ANODE MATERIAL; NANOCOMPOSITES; COMPOSITES; PERMITTIVITY
AB Graphene (G)-Fe3O4 nanohybrids were fabricated by first depositing beta-FeOOH crystals with diameter of 3-5 nm on the surface of the graphene sheets. After annealing under Ar flow, beta-FeOOH nanocrystals were reduced to Fe3O4 nanoparticles by the graphene sheets, and thus G-Fe3O4 nanohybrids were obtained. The Fe3O4 nanoparticles with a diameter of about 25 nm were uniformly dispersed over the surface of the graphene sheets. Moreover, compared with other magnetic materials and the graphene, the nanohybrids exhibited significantly increased electromagnetic absorption properties owing to high surface areas, interfacial polarizations, and good separation of magnetic nanoparticles. The maximum reflection loss was up to -40.36 dB for G-Fe3O4 nanohybrids with a thickness of 5.0mm. The nanohybrids are very promising for lightweight and strong electromagnetic attenuation materials. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774243]
C1 [Wang, Tieshi; Liu, Zhaohong; Ouyang, Qiuyun; Chen, Yujin; Li, Chunyan; Qi, Lihong] Harbin Engn Univ, Coll Sci, Harbin 150001, Peoples R China.
   [Lu, Mingming; Wen, Bo; Cao, Maosheng] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
   [Zhu, Chunling; Gao, Peng] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China.
RP Chen, YJ (reprint author), Harbin Engn Univ, Coll Sci, Harbin 150001, Peoples R China.
EM chenyujin@hrbeu.edu.cn; gaopeng@hrbeu.edu.cn; caomaosheng@bit.edu.cn
OI Cao, Mao-Sheng/0000-0001-6810-9422
FU National Natural Science Foundation of China [51072038, 51272050,
   61205113, 51172275, 21001035]; Program for New Century Excellent Talents
   in University [NECT-10-0049]; Outstanding Youth Foundation of
   Heilongjiang Province [JC201008]
FX We thank the National Natural Science Foundation of China (Grant Nos.
   51072038, 51272050, 61205113, 51172275, and 21001035), Program for New
   Century Excellent Talents in University (NECT-10-0049), and also
   Outstanding Youth Foundation of Heilongjiang Province (Grant No
   JC201008) for the financial support of this research.
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NR 50
TC 74
Z9 74
U1 42
U2 294
PU AMER INST PHYSICS
PI MELVILLE
PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1,
   MELVILLE, NY 11747-4501 USA
SN 0021-8979
J9 J APPL PHYS
JI J. Appl. Phys.
PD JAN 14
PY 2013
VL 113
IS 2
AR 024314
DI 10.1063/1.4774243
PG 8
WC Physics, Applied
SC Physics
GA 072BY
UT WOS:000313644500080
ER

PT J
AU Su, LW
   Zhou, Z
   Shen, PW
AF Su, Liwei
   Zhou, Zhen
   Shen, Panwen
TI Ni/C Hierarchical Nanostructures with Ni Nanoparticles Highly Dispersed
   in N-Containing Carbon Nanosheets: Origin of Li Storage Capacity
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID LITHIUM-ION BATTERIES; SOLID-ELECTROLYTE INTERFACE; SOLVOTHERMAL
   SYNTHESIS; NICKEL NANOPARTICLES; GRAPHITE-ELECTRODES; REVERSIBLE
   CAPACITY; MAGNETIC-PROPERTIES; DOPED GRAPHENE; ANODE; PERFORMANCE
AB Ni/C hierarchical composites, which consist of Ni nanoparticles highly dispersed in N-containing carbon nanosheets, were prepared via a facile, economical, and green route, and the electrochemical Li storage performance was investigated. On the basis of the available lithium storage mechanisms, Ni nanoparticles are inert to react with Li+ and contribute nothing to electrochemical Li storage. However, the composites exhibited an unexpected reversible capacity of 1051 mAh g(-1) after 30 cycles and 635 mAh g(-1) after 100 cycles at the current density of 200 mA g(-1). Such high reversible capacity cannot be simply ascribed to the Li insertion/extraction in carbon nanosheets. Instead, we proposed a possible origin of the reversible capacity, the electrochemical catalysis of Ni nanoparticles on the reversible formation/decomposition of some components in solid electrolyte interface films. These findings can further understand the role of transition-metal nanoparticles in lithium storage and open new doors for exploiting advanced materials for Li ion batteries and other energy-storage devices.
C1 [Su, Liwei; Zhou, Zhen; Shen, Panwen] Nankai Univ, Tianjin Key Lab Met & Mol Based Mat Chem, Key Lab Adv Energy Mat Chem, Minist Educ,Inst New Energy Mat Chem, Tianjin 300071, Peoples R China.
RP Zhou, Z (reprint author), Nankai Univ, Tianjin Key Lab Met & Mol Based Mat Chem, Key Lab Adv Energy Mat Chem, Minist Educ,Inst New Energy Mat Chem, Tianjin 300071, Peoples R China.
EM zhouzhen@nankai.edu.cn
RI Zhou, Zhen/C-4517-2008; Su, Liwei/G-2295-2011
OI Zhou, Zhen/0000-0003-3232-9903; Su, Liwei/0000-0002-9791-3476
FU 973 Program [2009CB220100]; NSFC [21073096]; Fundamental Research Funds
   for the Central Universities in China
FX This work was supported by the 973 Program (2009CB220100), NSFC
   (21073096), and the Fundamental Research Funds for the Central
   Universities in China.
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NR 56
TC 74
Z9 74
U1 18
U2 95
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD NOV 15
PY 2012
VL 116
IS 45
BP 23974
EP 23980
DI 10.1021/jp310054b
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 038RC
UT WOS:000311190800017
ER

PT J
AU Ji, LW
   Toprakci, O
   Alcoutlabi, M
   Yao, YF
   Li, Y
   Zhang, S
   Guo, BK
   Lin, Z
   Zhang, XW
AF Ji, Liwen
   Toprakci, Ozan
   Alcoutlabi, Mataz
   Yao, Yingfang
   Li, Ying
   Zhang, Shu
   Guo, Bingkun
   Lin, Zhan
   Zhang, Xiangwu
TI alpha-Fe2O3 Nanoparticle-Loaded Carbon Nanofibers as Stable and
   High-Capacity Anodes for Rechargeable Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium-ion batteries; anodes; nanofibers; carbon; alpha-Fe2O3
ID ENERGY-STORAGE; ELECTROCHEMICAL PROPERTIES; ELECTRODE MATERIALS;
   IRON-OXIDES; CONVERSION; PERFORMANCE; FABRICATION; COMPOSITE; CELLS;
   GRAPHENE
AB alpha-Fe2O3 nanoparticle-loaded carbon nanofiber composites were fabricated via electrospinning FeCl3.6H(2)O salt-polyacrylonitrile precursors in N,N-dimethylformamide solvent and the subsequent carbonization in inert gas. Scanning electron microscopy, transmission electron microscopy, energy dispersive X-ray spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and elemental analysis were used to study the morphology and composition of alpha-Fe2O3-carbon nanofiber composites. It was indicated that alpha-Fe2O3 nanoparticles with an average size of about 20 nm have a homogeneous dispersion along the carbon nanofiber surface. The resultant alpha-Fe2O3-carbon nanofiber composites were used directly as the anode material in rechargeable lithium half cells, and their electrochemical performance was evaluated. The results indicated that these alpha-Fe2O3-carbon nanofiber composites have high reversible capacity, good capacity retention, and acceptable rate capability when used as anode materials for rechargeable lithium-ion batteries.
C1 [Ji, Liwen; Toprakci, Ozan; Alcoutlabi, Mataz; Yao, Yingfang; Li, Ying; Zhang, Shu; Guo, Bingkun; Lin, Zhan; Zhang, Xiangwu] N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
RP Zhang, XW (reprint author), N Carolina State Univ, Dept Text Engn Chem & Sci, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA.
EM xiangwu_zhang@ncsu.edu
RI Lin, Zhan/C-6806-2011; Zhang, Xiangwu/F-1013-2011; Li, Ying/N-3918-2013;
   Guo, Bingkun/J-5774-2014
OI Zhang, Xiangwu/0000-0002-6236-6281; 
FU U.S. Department of Energy [DE-EE0001177]; ERC of the National Science
   Foundation [EEC-08212121]; Advanced Transportation Energy Center at
   North Carolina State University
FX This work was supported by the U.S. Department of Energy (No.
   DE-EE0001177), the ERC Program of the National Science Foundation under
   Award Number EEC-08212121, and the Advanced Transportation Energy Center
   at North Carolina State University.
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NR 50
TC 74
Z9 74
U1 30
U2 185
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY
PY 2012
VL 4
IS 5
BP 2672
EP 2679
DI 10.1021/am300333s
PG 8
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 945OF
UT WOS:000304285200049
PM 22524417
ER

PT J
AU Zhou, XS
   Yin, YX
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Yin, Ya-Xia
   Wan, Li-Jun
   Guo, Yu-Guo
TI A robust composite of SnO2 hollow nanospheres enwrapped by graphene as a
   high-capacity anode material for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ONE-POT SYNTHESIS; STORAGE PROPERTIES; ELECTROCHEMICAL PROPERTIES;
   SNO2/GRAPHENE COMPOSITE; RECHARGEABLE BATTERIES; CYCLIC PERFORMANCE;
   TIN-NANOPARTICLES; MESOPOROUS SNO2; CAVITY SIZE; CARBON
AB Graphene enwrapped SnO2 hollow nanospheres have been developed with combination of two desirable components: hollow nanostructures and graphene coating. The as-obtained SnO2-HNS/G becomes robust and exhibits stable cyclability and superior high-rate capability.
C1 [Zhou, Xiaosi; Yin, Ya-Xia; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, BNLMS, Inst Chem, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, BNLMS, Inst Chem, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2009CB930400,
   2012CB932900]; National Natural Science Foundation of China [91127044,
   21121063]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant nos. 2011CB935700, 2009CB930400 and 2012CB932900), the National
   Natural Science Foundation of China (Grant nos. 91127044 and 21121063),
   and the Chinese Academy of Sciences.
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NR 54
TC 74
Z9 74
U1 10
U2 122
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 34
BP 17456
EP 17459
DI 10.1039/c2jm32984k
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 985YF
UT WOS:000307305700013
ER

PT J
AU Sethuraman, VA
   Hardwick, LJ
   Srinivasan, V
   Kostecki, R
AF Sethuraman, Vijay A.
   Hardwick, Laurence J.
   Srinivasan, Venkat
   Kostecki, Robert
TI Surface structural disordering in graphite upon lithium
   intercalation/deintercalation
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Lithium-ion battery; Graphite anode; Structural disordering; Capacity
   fade; Raman spectroscopy
ID IN-SITU RAMAN; ION BATTERIES; AMORPHOUS-CARBON; ELECTRODES;
   SPECTROSCOPY; INSERTION; INTERCALATION; CELLS; MECHANISMS; CAPACITY
AB We report on the origin of the Surface structural disordering in graphite anodes induced by lithium intercalation and deintercalation processes. Average Raman spectra of graphitic anodes reveal that cycling at potentials that correspond to low lithium concentrations in Li(x)C (0 <= x<0.16) is responsible for most of the structural damage observed at the graphite surface. The extent of surface structural disorder in graphite is significantly reduced for the anodes that were cycled at potentials where stage-1 and stage-2 compounds (x > 0.33) are present. Electrochemical impedance spectra show larger interfacial impedance for the electrodes that were fully delithiated during cycling as compared to electrodes that were cycled at lower potentials (U < 0. 15 V vs. Li/Li(+)). Steep Li(+) surface-bulk concentration gradients at the surface of graphite during early stages of intercalation processes, and the inherent increase of the Li(x)C d-spacing tend to induce local stresses at the edges of graphene layers, and lead to the breakage of C-C bonds. The exposed graphite edge sites react with the electrolyte to (re)form the SEI layer, which leads to gradual degradation of the graphite anode, and causes reversible capacity loss in a lithium-ion battery. Published by Elsevier B.V.
C1 [Sethuraman, Vijay A.; Hardwick, Laurence J.; Srinivasan, Venkat; Kostecki, Robert] Univ Calif Berkeley, Lawrence Berkeley Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
RP Kostecki, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Lab, Environm Energy Technol Div, 1 Cyclotron Rd,MS 70-108B, Berkeley, CA 94720 USA.
EM R_Kostecki@lbl.gov
RI Sethuraman, Vijay/E-5702-2010
OI Sethuraman, Vijay/0000-0003-4624-1355
FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office
   of Vehicle Technologies; United States Department of Energy
   [DE-AC02-05CH11231]
FX The authors gratefully acknowledge the financial support from the
   Assistant Secretary for Energy Efficiency and Renewable Energy, Office
   of Vehicle Technologies, the United States Department of Energy, under
   contract no. DE-AC02-05CH11231. The authors thank Dr. Vincent Battaglia
   and Dr. Gao Liu for the provision of the electrode material and Dr. Paul
   Berdahl for helpful discussions.
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NR 32
TC 74
Z9 78
U1 11
U2 70
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 1
PY 2010
VL 195
IS 11
SI SI
BP 3655
EP 3660
DI 10.1016/j.jpowsour.2009.12.034
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 566PW
UT WOS:000275386100042
ER

PT J
AU Zhang, M
   Qu, BH
   Lei, DN
   Chen, YJ
   Yu, XZ
   Chen, LB
   Li, QH
   Wang, YG
   Wang, TH
AF Zhang, Ming
   Qu, Baihua
   Lei, Danni
   Chen, Yuejiao
   Yu, Xinzhi
   Chen, Libao
   Li, Qiuhong
   Wang, Yanguo
   Wang, Taihong
TI A green and fast strategy for the scalable synthesis of Fe2O3/graphene
   with significantly enhanced Li-ion storage properties
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID RECHARGEABLE LITHIUM BATTERIES; ANODE MATERIAL; GRAPHENE SHEETS;
   ELECTROCHEMICAL PERFORMANCE; SOLVOTHERMAL SYNTHESIS; ALPHA-FE2O3
   NANOTUBES; ELECTRODE MATERIALS; NEGATIVE-ELECTRODE; THERMAL-STABILITY;
   COMPOSITE
AB In this study, we proposed and demonstrated an environmentally friendly and effective methodology to prepare Fe2O3/graphene composites. The essence of this method was that ferrous ions could serve as both reductant and the iron source for Fe2O3, which is greener and more facile than the preparation methods for other iron oxide/graphene composites. As anode materials for lithium ion batteries, Fe2O3/graphene composites achieved high reversible capacities of about 800 mA h g(-1) after 100 cycles at a charge-discharge rate of 0.2 C. Moreover, they delivered rate capacities as high as 420 mA h g(-1) at a rate of 5 C. Both the cycling performance and rate capacities of Fe2O3/graphene composites were better than those of commercial Fe2O3 and its graphene composites. The improved performance toward the storage of Li+ was ascribed to graphene sheets, which acted as volume buffers and electron conductors. We believe that the strategy of preparing Fe2O3/graphene composites proposed by us may open a new way for the synthesis of metal oxide/graphene for various potential purposes.
C1 [Wang, Taihong] Hunan Univ, Key Lab Micro Nano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
RP Wang, TH (reprint author), Hunan Univ, Key Lab Micro Nano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM thwang@iphy.ac.cn
RI Qu, Baihua/H-9594-2012; Wang, Taihong/K-8968-2012; Zhang,
   Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU "973'' National Key Basic Research Program of China [2007CB310500];
   Hunan Provincial Natural Science Foundation of China [10JJ1011];
   National Natural Science Foundation of China [21003041, 21103046]; China
   Scholarship Council
FX This work was partly supported from the "973'' National Key Basic
   Research Program of China (Grant No. 2007CB310500), Hunan Provincial
   Natural Science Foundation of China (Grant No. 10JJ1011), National
   Natural Science Foundation of China (Grant No. 21003041, 21103046) and
   China Scholarship Council.
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NR 58
TC 73
Z9 76
U1 23
U2 162
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 9
BP 3868
EP 3874
DI 10.1039/c2jm15927a
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 890ZX
UT WOS:000300187000028
ER

PT J
AU Zheng, XL
   Xu, JB
   Yan, KY
   Wang, H
   Wang, ZL
   Yang, SH
AF Zheng, Xiaoli
   Xu, Jianbo
   Yan, Keyou
   Wang, Hong
   Wang, Zilong
   Yang, Shihe
TI Space-Confined Growth of MoS2 Nanosheets within Graphite: The Layered
   Hybrid of MoS2 and Graphene as an Active Catalyst for Hydrogen Evolution
   Reaction
SO CHEMISTRY OF MATERIALS
LA English
DT Article
ID LITHIUM-ION BATTERIES; METAL DICHALCOGENIDE NANOSHEETS; EDGE SITES;
   REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; H-2 PRODUCTION; ANODE MATERIAL;
   NANOPARTICLES; ELECTROCATALYST; COMPOSITE
AB Since the electrocatalytic activity of layered molybdenum disulfide (MoS2) for hydrogen evolution reaction (HER) closely depends on its exposed edges, the morphology and size of the material are critically important. Herein, we introduce a novel solvent-evaporation-assisted intercalation method to fabricate the hybrid of alternating MoS2 sheets and reduced graphene oxide layers, in which the nanosize of the MoS2 nanosheets can be effectively controlled by leveraging the confinement effect within the two-dimensional graphene layers. Significantly, the resulting MoS2/reduced graphene oxide (RGO) composite shows excellent catalytic activity for HER characterized by higher current densities and lower onset potentials than the conventional pre-exfoliated RGO supported MoS2 nanosheets. Further experiments on the effect of oxidation degree of graphene, the crystallinity of MoS2, and the exposed active site density on the HER performance of the MoS2/RGO composites show that there is an optimum condition for the catalytic activity of HER due to a balance between the numbers of exposed active sites of MoS2 and the internal conductive channels provided by graphene.
C1 [Zheng, Xiaoli; Xu, Jianbo; Yan, Keyou; Wang, Hong; Wang, Zilong; Yang, Shihe] Hong Kong Univ Sci & Technol, William Mong Inst Nano Sci & Technol, Dept Chem, Kowloon, Hong Kong, Peoples R China.
RP Yang, SH (reprint author), Hong Kong Univ Sci & Technol, William Mong Inst Nano Sci & Technol, Dept Chem, Kowloon, Hong Kong, Peoples R China.
EM chsyang@ust.hk
RI Yan, Keyou/N-1991-2013; 
OI Yang, Shihe/0000-0002-6469-8415
FU HK-RGC General Research Funds (GRF) [HKUST 605710, 606511]
FX This work was supported by the HK-RGC General Research Funds (GRF No.
   HKUST 605710 and 606511).
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NR 71
TC 72
Z9 72
U1 78
U2 336
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0897-4756
EI 1520-5002
J9 CHEM MATER
JI Chem. Mat.
PD APR 8
PY 2014
VL 26
IS 7
BP 2344
EP 2353
DI 10.1021/cm500347r
PG 10
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA AF2WD
UT WOS:000334572300019
ER

PT J
AU Gwon, H
   Hong, J
   Kim, H
   Seo, DH
   Jeon, S
   Kang, K
AF Gwon, Hyeokjo
   Hong, Jihyun
   Kim, Haegyeom
   Seo, Dong-Hwa
   Jeon, Seokwoo
   Kang, Kisuk
TI Recent progress on flexible lithium rechargeable batteries
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID CARBON-NANOTUBE ELECTRODES; GRAPHENE-PAPER ELECTRODES; ENERGY-STORAGE
   DEVICES; LI-ION BATTERY; POLYMER ELECTROLYTES; BINDER-FREE; CURRENT
   COLLECTOR; ANODE MATERIALS; DIRECT GROWTH; FILMS
AB Flexible lithium ion batteries (LIBs) have received considerable attention as a key component to enable future flexible electronic devices. A number of designs for flexible LIBs have been reported in recent years; in this article, we review recent progress. We focus on how flexibility can be introduced into each component of the LIB, including the active materials, electrolytes, separators, and current collectors. Approaches to integrating each component into a single device are described and the corresponding changes in the electrochemical and mechanical properties are discussed. Finally, the key challenges in the development of flexible LIBs are summarized.
C1 [Gwon, Hyeokjo; Hong, Jihyun; Kim, Haegyeom; Seo, Dong-Hwa; Kang, Kisuk] Seoul Natl Univ, Dept Mat Sci & Engn, RIAM, Seoul 151742, South Korea.
   [Gwon, Hyeokjo; Jeon, Seokwoo] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea.
   [Hong, Jihyun; Kim, Haegyeom; Seo, Dong-Hwa; Kang, Kisuk] Seoul Natl Univ, Ctr Nanoparticle Res, IBS, Seoul 151742, South Korea.
RP Gwon, H (reprint author), Seoul Natl Univ, Dept Mat Sci & Engn, RIAM, 1 Gwanak Ro, Seoul 151742, South Korea.
EM matlgen1@snu.ac.kr
RI Seo, Dong-Hwa/D-1446-2011; Kang, Kisuk/B-5776-2011; Hong,
   Jihyun/G-5146-2012; Kim, Haegyeom/E-4448-2011; JEON,
   SEOKWOO/C-1701-2011; 
OI Seo, Dong-Hwa/0000-0002-7200-7186; Hong, Jihyun/0000-0001-7210-2901;
   Kim, Haegyeom/0000-0002-5962-8244
FU Korea Institute of Energy Technology Evaluation and Planning (KETEP)
   [20124010203320]; Korea government Ministry of Trade, Industry and
   Energy; National Research Foundation of Korea; Korean Government (MEST)
   [NRF-2009-0094219]; Research Center Program of IBS (Institute for Basic
   Science) in Korea; Power Generation & Electricity Delivery of the KETEP;
   Korea government Ministry of Trade, industry Energy [2012T100201680]
FX This work was supported by the Human Resources Development program
   (20124010203320) of the Korea Institute of Energy Technology Evaluation
   and Planning (KETEP) grant funded by the Korea government Ministry of
   Trade, Industry and Energy and supported by a National Research
   Foundation of Korea Grant funded by the Korean Government (MEST)
   (NRF-2009-0094219). This work was supported by the Research Center
   Program of IBS (Institute for Basic Science) in Korea and supported by
   the Power Generation & Electricity Delivery of the KETEP grant funded by
   the Korea government Ministry of Trade, industry & Energy
   (2012T100201680).
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NR 118
TC 72
Z9 74
U1 77
U2 461
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD FEB
PY 2014
VL 7
IS 2
BP 538
EP 551
DI 10.1039/c3ee42927j
PG 14
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AA9KZ
UT WOS:000331413700004
ER

PT J
AU Yao, YJ
   Miao, SD
   Yu, SM
   Ma, LP
   Sun, HQ
   Wang, SB
AF Yao, Yunjin
   Miao, Shiding
   Yu, Shaoming
   Ma, Li Ping
   Sun, Hongqi
   Wang, Shaobin
TI Fabrication of Fe3O4/SiO2 core/shell nanoparticles attached to graphene
   oxide and its use as an adsorbent
SO JOURNAL OF COLLOID AND INTERFACE SCIENCE
LA English
DT Article
DE Fe3O4/SiO2 core/shell nanoparticle; Graphene; Adsorption; Methylene blue
ID LITHIUM-ION BATTERIES; MULTIWALLED CARBON NANOTUBES; METHYLENE-BLUE
   ADSORPTION; EXFOLIATED GRAPHITE OXIDE; IN-SITU SYNTHESIS; CO3O4
   NANOPARTICLES; MAGNETIC-PROPERTIES; ANODE MATERIAL; MICROSPHERES;
   PERFORMANCE
AB Amino-functionalized Fe3O4/SiO2 core/shell nanoparticles were synthesized by reacting Fe3O4 nanoparticles with tetraethyl orthosilicate and (3-aminopropyl) triethoxysilane to introduce amino groups on the surface. The amino groups on the Fe3O4/SiO2 were reacted with the carboxylic groups of graphene oxide (GO) with the aid of 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide and N-hydroxysuccinnimide to form Fe3O4/SiO2-GO nanoparticles. The structural, surface, and magnetic characteristics of the material were investigated by scanning and transmission electron microscopy, energy-dispersive X-ray spectrometry, powder X-ray diffraction, Fourier transform infrared spectroscopy, and thermogravimetric analysis. Adsorption equilibrium and kinetics of methylene blue on the Fe3O4/SiO2-GO were studied in a batch system. The maximum adsorption capacities were found to be 97.0, 102.6, and 111.1 mg g(-1) at 25, 45, and 60 degrees C, respectively. A second-order kinetic equation could best describe the sorption kinetics. Thermodynamic parameters indicated that the adsorption of methylene blue onto the material was thermodynamically feasible and could occur spontaneously. (C) 2012 Elsevier Inc. All rights reserved.
C1 [Yao, Yunjin; Miao, Shiding; Yu, Shaoming] Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China.
   [Yao, Yunjin; Ma, Li Ping; Sun, Hongqi; Wang, Shaobin] Curtin Univ Technol, Dept Chem Engn, Perth, WA 6845, Australia.
RP Yao, YJ (reprint author), Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China.
EM yaoyunjin@gmail.com; shaobin.wang@curtin.edu.au
RI Wang, Shaobin/C-5507-2008; yao, yunjin/C-9615-2012
OI Wang, Shaobin/0000-0002-1751-9162; yao, yunjin/0000-0002-5462-4973
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NR 33
TC 72
Z9 75
U1 28
U2 299
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0021-9797
J9 J COLLOID INTERF SCI
JI J. Colloid Interface Sci.
PD AUG 1
PY 2012
VL 379
BP 20
EP 26
DI 10.1016/j.jcis.2012.04.030
PG 7
WC Chemistry, Physical
SC Chemistry
GA 963AH
UT WOS:000305592000004
PM 22625432
ER

PT J
AU Choi, J
   Jin, J
   Jung, IG
   Kim, JM
   Kim, HJ
   Son, SU
AF Choi, Jaewon
   Jin, Jaewon
   Jung, Il Gu
   Kim, Jung Min
   Kim, Hae Jin
   Son, Seung Uk
TI SnSe2 nanoplate-graphene composites as anode materials for lithium ion
   batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; OXIDE; NANOPARTICLES; CELLS;
   NANOMATERIALS; NANOCRYSTALS; ELECTRODES; NANOTUBES; NANODISKS
AB Through a solution approach, SnSe2 nanoplate-graphene composites were prepared and applied as anode materials in lithium ion batteries, showing promising storage performance superior to SnSe2 nanoplates or graphene alone.
C1 [Kim, Jung Min; Kim, Hae Jin] Korea Basic Sci Inst, Taejon 350333, South Korea.
   [Choi, Jaewon; Jin, Jaewon; Jung, Il Gu; Son, Seung Uk] Sungkyunkwan Univ, Dept Chem, Suwon 440746, South Korea.
   [Choi, Jaewon; Jin, Jaewon; Jung, Il Gu; Son, Seung Uk] Sungkyunkwan Univ, Dept Energy Sci, Suwon 440746, South Korea.
RP Kim, HJ (reprint author), Korea Basic Sci Inst, Taejon 350333, South Korea.
EM sson@skku.edu
FU Ministry of Education, Science and Technology [P30402,
   R31-2008-000-10029-0]; Priority Research Centers [NRF-2010-0029698]
FX This work was supported by KBSI grants P30402 and R31-2008-000-10029-0
   (WCU program) through the National Research Foundation of Korea funded
   by the Ministry of Education, Science and Technology. I. G. J.
   acknowledges the grant NRF-2010-0029698 (Priority Research Centers
   Program).
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PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PY 2011
VL 47
IS 18
BP 5241
EP 5243
DI 10.1039/c1cc10317b
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 752KH
UT WOS:000289689600037
PM 21445446
ER

PT J
AU Liang, MH
   Luo, B
   Zhi, LJ
AF Liang, Minghui
   Luo, Bin
   Zhi, Linjie
TI Application of graphene and graphene-based materials in clean
   energy-related devices
SO INTERNATIONAL JOURNAL OF ENERGY RESEARCH
LA English
DT Article
DE graphene; solar cell; lithium ion batteries; supercapacitors
ID LITHIUM-ION BATTERIES; SENSITIZED SOLAR-CELLS; DOUBLE-LAYER CAPACITORS;
   ANODE MATERIAL; TRANSPARENT CONDUCTORS; MESOPOROUS CARBON;
   TIN-NANOPARTICLES; PERFORMANCE; FILMS; ELECTRODES
AB The unique properties of graphene render it as a versatile material applying in various energy-related devices. Solar cells with transparent and conductive graphene film as window electrode have exhibited considerable power conversion efficiency. The graphene-based materials used as anode in lithium ion secondary batteries displayed excellent cycling performance and high capacities. Supercapacitors with great potential for practical application have been fabricated as well using graphene-based materials as electrode. Graphene has emerged as a promising two-dimensional nanomaterial for developing economic and efficient energy-related devices. In this review, the recent progress concerning the application of graphene and graphene-based materials in clean energy-related devices has been summarized briefly. Copyright (C) 2009 John Wiley & Sons, Ltd.
C1 [Liang, Minghui; Luo, Bin; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Zhi, LJ (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Luo, Bin/P-7836-2015
OI Luo, Bin/0000-0003-2088-6403
FU National Center for Nanoscience and Technology of China; Chinese Academy
   of Sciences [KJCX2-YW-MI1]; Ministry of Science and Technology of China
   [2009AA03Z328, 2009DPA41220]
FX Contract/grant sponsor: National Center for Nanoscience and Technology
   of China Contract/grant sponsor: Chinese Academy of Sciences;
   contract/grant number: KJCX2-YW-MI1 Contract/grant sponsor: Ministry of
   Science and Technology of China; contract/grant numbers: 2009AA03Z328,
   2009DPA41220
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NR 50
TC 72
Z9 77
U1 9
U2 62
PU WILEY-BLACKWELL
PI HOBOKEN
PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA
SN 0363-907X
J9 INT J ENERG RES
JI Int. J. Energy Res.
PD OCT 25
PY 2009
VL 33
IS 13
SI SI
BP 1161
EP 1170
DI 10.1002/er.1598
PG 10
WC Energy & Fuels; Nuclear Science & Technology
SC Energy & Fuels; Nuclear Science & Technology
GA 510CW
UT WOS:000271066600007
ER

PT J
AU Liang, SZ
   Zhu, XF
   Lian, PC
   Yang, WS
   Wang, HH
AF Liang, Shuzhao
   Zhu, Xuefeng
   Lian, Peichao
   Yang, Weishen
   Wang, Haihui
TI Superior cycle performance of Sn@C/graphene nanocomposite as an anode
   material for lithium-ion batteries
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Tin; Carbon coating; Graphene; Anode material; Lithium-ion batteries
ID CARBON SPHERES; HOLLOW CARBON; ALLOY ANODE; CAPACITY; STORAGE;
   NANOPARTICLES; PARTICLES; NANOTUBES; ELECTRODE; OXIDE
AB A novel anode material for lithium-ion batteries, tin nanoparticles coated with carbon embedded in graphene (Sn@C/graphene), was fabricated by hydrothermal synthesis and subsequent annealing. The structure and morphology of the nanocomposite were characterized by X-ray diffraction, scanning electron microscopy, and transmission electron microscopy. The size of the Sn@C nanoparticles is about 50-200 nm. The reversible specific capacity of the nanocomposite is similar to 662 mAh g(-1) at a specific current of 100 mA g(-1) after 100 cycles, even similar to 417 mAh g(-1) at the high current of 1000 mA g(-1). These results indicate that Sn@C/graphene possesses superior cycle performance and high rate capability. The enhanced electrochemical performances can be ascribed to the characteristic structure of the nanocomposite with both of the graphene and carbon shells, which buffer the volume change of the metallic tin and prevent the detachment and agglomeration of pulverized tin. (C) 2011 Elsevier Inc. All rights reserved.
C1 [Liang, Shuzhao; Lian, Peichao; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou 510640, Peoples R China.
EM sz.liang02@mail.edu.cn; hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620
FU National Natural Science Foundation of China [20936001]; SCUT
   [2009220038]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 20936001) and the Fundamental Research Funds
   for the Central Universities, SCUT (2009220038).
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U2 92
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD JUN
PY 2011
VL 184
IS 6
BP 1400
EP 1404
DI 10.1016/j.jssc.2011.03.052
PG 5
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 773TB
UT WOS:000291332300008
ER

PT J
AU Mahmood, N
   Zhang, CZ
   Jiang, J
   Liu, F
   Hou, YL
AF Mahmood, Nasir
   Zhang, Chenzhen
   Jiang, Jie
   Liu, Fei
   Hou, Yanglong
TI Multifunctional Co3S4/Graphene Composites for Lithium Ion Batteries and
   Oxygen Reduction Reaction
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE cobalt; electrochemistry; lithium ion batteries; nanotubes; oxygen
   reduction reaction
ID STORAGE DEVICES; HOLLOW SPHERES; NANOSTRUCTURED MATERIALS; ELECTRODE
   PERFORMANCE; COSE2 NANOPARTICLES; ENERGY-CONVERSION; CATHODE CATALYST;
   ANODE MATERIALS; FUEL-CELLS; GRAPHENE
AB Cobalt sulfide is a good candidate for both lithium ion batteries (LIBs) and cathodic oxygen reduction reaction (ORR), but low conductivity, poor cyclability, capacity fading, and structural changes hinder its applications. The incorporation of graphene into Co3S4 makes it a promising electrode by providing better electrochemical coupling, enhanced conductivity, fast mobility of ions and electrons, and a stabilized structure due to its elastic nature. With the objective of achieving high-performance composites, herein we report a facile hydrothermal process for growing Co3S4 nanotubes (NTs) on graphene (G) sheets. Electrochemical impedance spectroscopy (EIS) verified that graphene dramatically increases the conductivity of the composites to almost twice that of pristine Co3S4. Electrochemical measurements indicated that the as-synthesized Co3S4/G composites exhibit good cyclic stability and a high discharge capacity of 720mAhg1 up to 100 cycles with 99.9% coulombic efficiency. Furthermore, the composites react with dissolved oxygen in the ORR by four- and two-electron mechanisms in both acidic and basic media with an onset potential close to that of commercial Pt/C. The stability of the composites is much higher than that of Pt/C, and exhibit high methanol tolerance. Thus, these properties endorse Co3S4/G composites as auspicious candidates for both LIBs and ORR.
C1 [Mahmood, Nasir; Zhang, Chenzhen; Jiang, Jie; Liu, Fei; Hou, Yanglong] Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China.
RP Hou, YL (reprint author), Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China.
EM hou@pku.edu.cn
RI Hou, Yanglong/B-8688-2012
FU National Natural Science Foundation of China [51125001, 51172005,
   90922033]; National Basic Research Program of China [2010CB934601];
   Natural Science Foundation of Beijing [2122022]; New Century Excellent
   Talents Program [NCET-09-0177]; Ministry of Education of China
   [20120001110078]; Yok Ying Tung Foundation [122043]; New Star Program of
   Beijing Municipal Science & Technology Committee [2008B02]
FX This work was supported in part by the National Natural Science
   Foundation of China (51125001, 51172005, and 90922033), the National
   Basic Research Program of China (2010CB934601), the Natural Science
   Foundation of Beijing (2122022), the New Century Excellent Talents
   Program (NCET-09-0177), the Doctoral Program (20120001110078) of the
   Ministry of Education of China, the Yok Ying Tung Foundation (122043),
   and the New Star Program of Beijing Municipal Science & Technology
   Committee (2008B02).
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NR 54
TC 70
Z9 70
U1 44
U2 332
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD APR
PY 2013
VL 19
IS 16
BP 5183
EP 5190
DI 10.1002/chem.201204549
PG 8
WC Chemistry, Multidisciplinary
SC Chemistry
GA 123OL
UT WOS:000317399600031
PM 23447515
ER

PT J
AU Fan, W
   Gao, W
   Zhang, C
   Tjiu, WW
   Pan, JS
   Liu, TX
AF Fan, Wei
   Gao, Wei
   Zhang, Chao
   Tjiu, Weng Weei
   Pan, Jisheng
   Liu, Tianxi
TI Hybridization of graphene sheets and carbon-coated Fe3O4 nanoparticles
   as a synergistic adsorbent of organic dyes
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM ION BATTERIES; ONE-STEP SYNTHESIS; HYDROTHERMAL CARBONIZATION;
   ANODE MATERIAL; OXIDE; COMPOSITE; NANOSHEETS; REMOVAL; WATER; ADSORPTION
AB Magnetic graphene-Fe3O4@carbon (GFC)hybrids with hierarchical nanostructures have been synthesized and their application as an adsorbent for the removal of organic dyes has been investigated. Graphene-Fe3O4 hybrids were first prepared via a facile one-pot solvothermal process, then carbonaceous coatings on Fe3O4 nanoparticles of nanometer thickness were synthesized by a hydrothermal carbonization process using eco-friendly glucose as a carbon source. Graphene sheets acting as two-dimensional (2D)substrates can effectively prevent the Fe3O4 nanoparticles from aggregating and enable a good dispersion of these magnetic nanoparticles. The carbonaceous layer protects the Fe3O4 nanoparticles in acidic environments and greatly enhances the specific surface area of the hybrids which is beneficial for the removal of organic dyes, such as methylene blue (MB). The resultant GFC hybrids exhibit great adsorption properties not only in water but also in acidic environments, and about 86% and 77% of the dye removal efficiency can be retained after five adsorption-desorption cycles in water and 1 MHCl, respectively. The rapid and efficient adsorption of organic dyes from water as well as acid suggests that the GFC hybrids have potential environmental applications as alternatives to commercial materials in wastewater treatment for the removal of organic dyes.
C1 [Fan, Wei; Gao, Wei; Zhang, Chao; Liu, Tianxi] Fudan Univ, State Key Lab Mol Engn Polymers, Dept Macromol Sci, Shanghai 200433, Peoples R China.
   [Tjiu, Weng Weei; Pan, Jisheng] ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore.
RP Liu, TX (reprint author), Fudan Univ, State Key Lab Mol Engn Polymers, Dept Macromol Sci, 220 Handan Rd, Shanghai 200433, Peoples R China.
EM txliu@fudan.edu.cn
RI Liu, Tianxi/E-6628-2011; Zhang, Chao/M-6454-2013
OI Liu, Tianxi/0000-0002-5592-7386; 
FU National Natural Science Foundation of China [51125011]; "Shu Guang"
   project [09SG02]; Shanghai Municipal Education Commission; Shanghai
   Education Development Foundation
FX The authors are grateful for the financial support from the National
   Natural Science Foundation of China (51125011), and "Shu Guang" project
   (09SG02) supported by Shanghai Municipal Education Commission and
   Shanghai Education Development Foundation.
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NR 46
TC 70
Z9 73
U1 22
U2 206
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 48
BP 25108
EP 25115
DI 10.1039/c2jm35609k
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 049GN
UT WOS:000311970800017
ER

PT J
AU Xiao, Z
   Xia, Y
   Ren, ZH
   Liu, ZY
   Xu, G
   Chao, CY
   Li, X
   Shen, G
   Han, GR
AF Xiao, Zhen
   Xia, Yang
   Ren, Zhaohui
   Liu, Zhenya
   Xu, Gang
   Chao, Chunying
   Li, Xiang
   Shen, Ge
   Han, Gaorong
TI Facile synthesis of single-crystalline mesoporous alpha-Fe2O3 and Fe3O4
   nanorods as anode materials for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID REVERSIBLE CAPACITY; STORAGE PROPERTIES; GRAPHENE; HEMATITE; OXIDE;
   PERFORMANCE; FABRICATION; NANOCRYSTALS; CAPABILITY; NANOSHEETS
AB In this work, single-crystalline alpha-FeOOH nanorods with a length of 400-700 nm and a diameter of 20-80 nm were successfully synthesized via a facile template-free hydrothermal method. Single-crystalline mesoporous alpha-Fe2O3 and Fe3O4 nanorods could be obtained from these a-FeOOH precursors after calcining at 350 degrees C in air and 500 degrees C in nitrogen, respectively. The as-prepared single-crystalline mesoporous alpha-Fe2O3 and Fe3O4 nanorods exhibited a large specific surface area and porosity, effectively enhancing the electrochemical reaction area and accommodate the strain during the charge-discharge cycling process.
C1 [Xiao, Zhen; Ren, Zhaohui; Liu, Zhenya; Xu, Gang; Chao, Chunying; Li, Xiang; Shen, Ge; Han, Gaorong] Zhejiang Univ, State Key Lab Silicon Mat, Dept Mat Sci & Engn, Cyrus Tang Ctr Sensor Mat & Applicat, Hangzhou 310027, Peoples R China.
   [Xia, Yang] Zhejiang Univ Technol, Coll Chem Engn & Mat Sci, Hangzhou 310014, Zhejiang, Peoples R China.
RP Ren, ZH (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Dept Mat Sci & Engn, Cyrus Tang Ctr Sensor Mat & Applicat, Hangzhou 310027, Peoples R China.
EM renzh@zju.edu.cn; hgr@zju.edu.cn
RI LI, Xiang/F-3717-2011
OI LI, Xiang/0000-0002-4675-5367
FU National Natural Science Foundation of China [51102212]; Cyrus Tang
   Center for Sensor Materials and Applications [112205-M11201/005];
   Fundamental Research Funds for the Central Universities [588040*
   172210221/014]; Opening Foundation of Zhejing Provincial Top Key
   Discipline
FX This work was financially supported by the National Natural Science
   Foundation of China (Grant no. 51102212), Cyrus Tang Center for Sensor
   Materials and Applications (112205-M11201/005), the Fundamental Research
   Funds for the Central Universities (no. 588040* 172210221/014) and the
   Opening Foundation of Zhejing Provincial Top Key Discipline.
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NR 38
TC 70
Z9 75
U1 32
U2 195
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 38
BP 20566
EP 20573
DI 10.1039/c2jm34083f
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 004CV
UT WOS:000308658600067
ER

PT J
AU Wang, SW
   Wang, LJ
   Zhang, K
   Zhu, ZQ
   Tao, ZL
   Chen, J
AF Wang, Shiwen
   Wang, Lijiang
   Zhang, Kai
   Zhu, Zhiqiang
   Tao, Zhanliang
   Chen, Jun
TI Organic Li4C8H2O6 Nanosheets for Lithium-Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Lithium-ion batteries; organic electrode materials; nanosheets;
   spectroscopy; energy level diagram
ID ELECTRODE MATERIALS; CATHODE MATERIALS; STORAGE MATERIALS; POLYMER;
   ANODES; HYDROGEL; GRAPHENE; CHARGE; SALT
AB Organic tetralithium salts of 2,5-dihydroxyterephthalic acid (Li4C8H2O6) with the morphologies of bulk, nanoparticles, and nanosheets have been investigated as the active materials of either positive or negative electrode of rechargeable lithium-ion batteries. It is demonstrated that, in the electrolyte of LiPF6 dissolved in ethylene carbonate (EC) and dimethyl carbonate (DMC), reversible two-Li-ion electrochemical reactions are taking place with redox Li4C8H2O6/Li2C8H2O6 at similar to 2.6 V for a positive electrode and Li4C8H2O6/Li6C8H2O6 at similar to 0.8 V for a negative electrode, respectively. In the observed system, the electrochemical performance of high to low order is nanosheets > nanoparticles > bulk. Remarkably, Li4C8H2O6 nanosheets show the discharge capacities of 223 and 145 mAh g(-1) at 0.1 and 5 C rates, respectively. A capacity retention of 95% is sustained after 50 cycles at 0.1 C rate charge/discharge and room temperature. Moreover, charging the symmetrical cells with Li4C8H2O6 nanosheets as the initial active materials of both positive and negative electrodes produces all-organic LIBs with an average operation voltage of 1.8 V and an energy density of about 130 Wh kg(-1), enlightening the design and application of organic Li-reservoir compounds with nanostructures for all organic LIBs.
C1 [Wang, Shiwen; Wang, Lijiang; Zhang, Kai; Zhu, Zhiqiang; Tao, Zhanliang; Chen, Jun] Nankai Univ, Key Lab Adv Energy Mat Chem, Minist Educ, Coll Chem,Synerget Innovat Ctr Chem Sci & Engn, Tianjin 300071, Peoples R China.
RP Tao, ZL (reprint author), Nankai Univ, Key Lab Adv Energy Mat Chem, Minist Educ, Coll Chem,Synerget Innovat Ctr Chem Sci & Engn, Tianjin 300071, Peoples R China.
EM taozhl@nankai.edu.cn; chenabc@nankai.edu.cn
RI Chen, Jun/D-4873-2016
FU Programs of National 973 [2011CB935900]; NSFC [21231005, 51231003]; 111
   Project [B12015]
FX This work was supported by the Programs of National 973 (2011CB935900),
   NSFC (21231005 and 51231003), and 111 Project (B12015).
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NR 30
TC 69
Z9 70
U1 34
U2 246
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD SEP
PY 2013
VL 13
IS 9
BP 4404
EP 4409
DI 10.1021/nl402239p
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 296BA
UT WOS:000330158900070
PM 23978244
ER

PT J
AU Wu, H
   Xu, M
   Wang, YC
   Zheng, GF
AF Wu, Hao
   Xu, Ming
   Wang, Yongcheng
   Zheng, Gengfeng
TI Branched Co3O4/Fe2O3 nanowires as high capacity lithium-ion battery
   anodes
SO NANO RESEARCH
LA English
DT Article
DE Co3O4; alpha-Fe2O3; nanowire; branched; lithium-ion battery; Nyquist
   plot
ID ELECTROCHEMICAL ENERGY-STORAGE; CO3O4 NANOPARTICLES; ARRAYS;
   PERFORMANCE; GRAPHENE; ELECTRODES; NANOTUBES; HETEROSTRUCTURES;
   NANOMATERIALS; COMPOSITE
AB We report a facile, two-step hydrothermal synthesis of a novel Co3O4/alpha-Fe2O3 branched nanowire heterostructure, which can serve as a good candidate for lithium-ion battery anodes with high Li+ storage capacity and stability. The single-crystalline, primary Co3O4 nanowire trunk arrays directly grown on Ti substrates allow for efficient electrical and ionic transport. The secondary alpha-Fe2O3 branches provide enhanced surface area and high theoretical Li+ storage capacity, and can also serve as volume spacers between neighboring Co3O4 NW arrays to maintain electrolyte penetration as well as reduce the aggregation during Li+ intercalation, thus leading to improved electrochemical energy storage performance.
C1 [Wu, Hao; Xu, Ming; Wang, Yongcheng; Zheng, Gengfeng] Fudan Univ, Dept Chem, Adv Mat Lab, Shanghai 200433, Peoples R China.
RP Zheng, GF (reprint author), Fudan Univ, Dept Chem, Adv Mat Lab, Shanghai 200433, Peoples R China.
EM gfzheng@fudan.edu.cn
RI Zheng, Gengfeng/G-7023-2011
OI Zheng, Gengfeng/0000-0002-1803-6955
FU National Key Basic Research Program of China [2013CB934104]; National
   Natural Science Foundation of China (NSFC) [21071033]; Program for New
   Century Excellent Talents in University [NCET-10-0357]; Program for
   Professor of Special Appointment (Eastern Scholar) at Shanghai
   Institutions of Higher Learning
FX We thank the following funding agencies for supporting this work: the
   National Key Basic Research Program of China (No. 2013CB934104), the
   National Natural Science Foundation of China (NSFC) (No. 21071033), the
   Program for New Century Excellent Talents in University (No.
   NCET-10-0357), and the Program for Professor of Special Appointment
   (Eastern Scholar) at Shanghai Institutions of Higher Learning.
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NR 33
TC 69
Z9 71
U1 36
U2 317
PU TSINGHUA UNIV PRESS
PI BEIJING
PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA
SN 1998-0124
J9 NANO RES
JI Nano Res.
PD MAR
PY 2013
VL 6
IS 3
BP 167
EP 173
DI 10.1007/s12274-013-0292-z
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 105QR
UT WOS:000316087300002
ER

PT J
AU Chen, TT
   Deng, F
   Zhu, J
   Chen, CF
   Sun, GB
   Ma, SL
   Yang, XJ
AF Chen, Tingting
   Deng, Fang
   Zhu, Jia
   Chen, Caifeng
   Sun, Genban
   Ma, Shulan
   Yang, Xiaojing
TI Hexagonal and cubic Ni nanocrystals grown on graphene: phase-controlled
   synthesis, characterization and their enhanced microwave absorption
   properties
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; MONODISPERSE NICKEL NANOPARTICLES;
   ELECTROMAGNETIC-WAVE ABSORPTION; MAGNETIC-PROPERTIES; FEPT
   NANOPARTICLES; FACILE SYNTHESIS; ANODE MATERIAL; NANOCOMPOSITES;
   COMPOSITES; DECOMPOSITION
AB Hexagonal close-packed Ni (h-Ni) nanocrystals and face-centered cubic Ni (c-Ni) nanoflowers with uniform size and high dispersion have been successfully assembled on graphene nanosheets (GN) via a facile one-step solution-phase strategy under different reaction conditions, where the reduction process of graphite oxide (GO) sheets into GN was accompanied by the generation of Ni nanocrystals. The reduction of GO by this method is effective, which was confirmed by X-ray diffraction (XRD), Fourier transform infrared (FTIR) and Raman spectroscopy and is comparable to conventional methods. The phase and morphology of nickel can be easily tuned by varying the reaction temperature and solvent. It was shown that the as-formed h-Ni nanocrystals with a diameter as small as 3 nm are grown densely and uniformly on the graphene sheets, and as a result the aggregation of the h-Ni nanocrystals was effectively prevented. In addition, c-Ni nanospheres assembled by c-Ni nanocrystals with a size of 15 nm were also uniformly deposited on the graphene sheets. The investigation of the microwave absorbability reveals that the three Ni/GN nanocomposites exhibit excellent microwave absorbability, which is stronger than the corresponding Ni nanostructures.
C1 [Chen, Tingting; Deng, Fang; Zhu, Jia; Chen, Caifeng; Sun, Genban; Ma, Shulan; Yang, Xiaojing] Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China.
RP Sun, GB (reprint author), Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China.
EM gbsun@bnu.edu.cn; yang.xiaojing@bnu.edu.cn
FU Natural Science Foundation of China (NSFC) [20901010, 50872012,
   20871018]
FX This work was supported by the Natural Science Foundation of China
   (NSFC, no. 20901010, 50872012 and 20871018).
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NR 55
TC 69
Z9 69
U1 30
U2 152
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 30
BP 15190
EP 15197
DI 10.1039/c2jm31171b
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 971PI
UT WOS:000306215900055
ER

PT J
AU Evanoff, K
   Benson, J
   Schauer, M
   Kovalenko, I
   Lashmore, D
   Ready, WJ
   Yushin, G
AF Evanoff, Kara
   Benson, Jim
   Schauer, Mark
   Kovalenko, Igor
   Lashmore, David
   Ready, W. Jud
   Yushin, Gleb
TI Ultra Strong Silicon-Coated Carbon Nanotube Nonwoven Fabric as a
   Multifunctional Lithium-Ion Battery Anode
SO ACS NANO
LA English
DT Article
DE batteries; composite materials; multifunctional materials; electrodes;
   silicon
ID ELECTRICAL-CONDUCTIVITY; THERMAL-PROPERTIES; AMORPHOUS-SILICON;
   RAMAN-SCATTERING; GRAPHENE PAPER; ELECTRODES; INSERTION; COMPOSITES;
   NANOWIRES; GRAPHITE
AB Materials that can perform simultaneous functions allow for reductions in the total system mass and volume. Developing technologies to produce flexible batteries with good performance lit combination with high specific strength is strongly desired for weight- and power-sensitive applications such as unmanned or aerospace vehicles, high-performance ground vehicles, robotics, and smart textiles. State of the art battery electrode fabrication techniques are not conducive to the development of multifunctional materials due to their inherently low strength and conductivities. Here, we present a scalable method utilizing carbon nanotube (CNT) nonwoven fabric-based technology to develop flexible, electrochemically stable (similar to 494 mAh.g(-1) for 150 cycles). battery anodes that can be produced on an industrial scale and demonstrate specific strength higher than that Of titanium copper, and even a structural steel. Similar methods can be utilized for the formation of various' cathode and anode composites with tunable strength and energy and power densities.
C1 [Evanoff, Kara; Benson, Jim; Kovalenko, Igor; Ready, W. Jud; Yushin, Gleb] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
   [Evanoff, Kara; Ready, W. Jud] Georgia Tech Res Inst, Electroopt Syst Lab, Atlanta, GA 30332 USA.
   [Schauer, Mark; Lashmore, David] Nanocomp Technol Inc, Concord, NH 03301 USA.
RP Yushin, G (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
EM yushin@gatech.edu
RI Yushin, Gleb/B-4529-2013
OI Yushin, Gleb/0000-0002-3274-9265
FU AFOSR [FA9550-09-1-0151]; Robert Shackelford Fellowship
FX We thank J.T. Lee for TGA analysis, N. Nitta for EDS analysis, and D.
   Lewis for conductivity measurements. The work was partially supported by
   AFOSR (Grant FA9550-09-1-0151). K.E. was supported by the Robert
   Shackelford Fellowship.
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U1 31
U2 272
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2012
VL 6
IS 11
BP 9837
EP 9845
DI 10.1021/nn303393p
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 043CY
UT WOS:000311521700053
PM 23075213
ER

PT J
AU Tao, HC
   Fan, LZ
   Mei, YF
   Qu, XH
AF Tao, Hua-Chao
   Fan, Li-Zhen
   Mei, Yongfeng
   Qu, Xuanhui
TI Self-supporting Si/Reduced Graphene Oxide nanocomposite films as anode
   for lithium ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Silicon; Reduced Graphene Oxide; Lithium ion batteries; Anode
ID SILICON; PERFORMANCE; NANOWIRES; STORAGE
AB Self-supporting Si/Reduced Graphene Oxide (RGO) nanocomposite films have been prepared by thermal reduction of Si/graphene oxide nanocomposite, which is fabricated by dispersing silicon nanoparticles into an aqueous suspension of graphene oxide nanosheets. The Si nanoparticles are well encapsulated in a RGO matrix and the Si/RGO composite has much higher reversible discharge capacity and a better cycle stability than pure nanosized Si particles as well as the RGO. Such enhancement can be attributed to the RGO matrix, which offers an efficient electrically conductive channel and a flexible mechanical support for strain release. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Tao, Hua-Chao; Fan, Li-Zhen; Qu, Xuanhui] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
   [Mei, Yongfeng] Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China.
RP Fan, LZ (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
EM fanlizhen@ustb.edu.cn
FU NSF of China; NCET; Fundamental Research Funds for the Central
   Universities of China; Beijing Municipal Science & Technology New Star
   Plan; Fok Ying-Tong Education Foundation; IRTG
FX The authors acknowledge financial supports from NSF of China, NCET, and
   Fundamental Research Funds for the Central Universities of China,
   Beijing Municipal Science & Technology New Star Plan and Fok Ying-Tong
   Education Foundation. Y.F.M. acknowledges the support from the IRTG
   program. The authors acknowledge helpful discussion with Professor Hong
   Li and he also kindly provided Si nanoparticles.
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NR 18
TC 68
Z9 69
U1 12
U2 156
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD DEC
PY 2011
VL 13
IS 12
BP 1332
EP 1335
DI 10.1016/j.elecom.2011.08.001
PG 4
WC Electrochemistry
SC Electrochemistry
GA 874FM
UT WOS:000298940800012
ER

PT J
AU Xu, K
   Lam, YF
   Zhang, SS
   Jow, TR
   Curtis, TB
AF Xu, Kang
   Lam, Yiufai
   Zhang, Sheng S.
   Jow, T. Richard
   Curtis, Timothy B.
TI Solvation sheath of Li+ in nonaqueous electrolytes and its implication
   of graphite/electrolyte interface chemistry
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID IONIZATION-MASS-SPECTROSCOPY; UNDERSTAND SURFACE-CHEMISTRY; LITHIUM-ION
   BATTERIES; CARBON ANODES; GRAPHITE; ETHYLENE; DICARBONATE; REDUCTION;
   PRODUCT
AB The formation chemistry of graphite/electrolyte interface and its dependence on electrolyte bulk composition were investigated by conducting electrochemical impedance analyses on interfaces systematically formed in various electrolytes and NMR identification of surface species harvested therefrom. The interpretation of these analyses strongly suggests that Li+ solvation sheath structure is central in defining the anode surface chemistry, because solvent molecules preferentially recruited by Li+ into the solvation sheath would be preferentially reduced on graphene surface upon initial charge of the electrode. Due to the preference of Li+ in binding the more polar molecules from the electrolyte solvent mixture, the contributions from cyclic and linear carbonates to the interface chemistry are unsymmetrical, and ethylene carbonate, the universal cosolvent in all electrolyte formulations, consequently becomes the favored chemical source for the interfacial ingredients. Since the chemical composition of the interface dictates Li+ transport kinetics at low temperatures, the understandings about how the electrolyte cosolvents share the responsibility for the graphite/electrolyte interfacial chemistry will benefit the efforts to tailor an interface that is more tolerant toward the operation of Li ion devices at sub-zero temperatures.
C1 USA, Res Lab, Electrochem Branch, Sensor & Electron Devices Directorate, Adelphi, MD 20783 USA.
   Univ Maryland, Dept Chem & Biochem, Adelphi, MD 20783 USA.
RP Xu, K (reprint author), USA, Res Lab, Electrochem Branch, Sensor & Electron Devices Directorate, Adelphi, MD 20783 USA.
EM cxu@arl.army.mil
RI Zhang, Sheng/A-4456-2012; Xu, Kang/C-6054-2013
OI Zhang, Sheng/0000-0002-2624-9248; 
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NR 25
TC 68
Z9 69
U1 12
U2 52
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD MAY 24
PY 2007
VL 111
IS 20
BP 7411
EP 7421
DI 10.1021/jp068691u
PG 11
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 169CH
UT WOS:000246569800026
ER

PT J
AU Zhang, L
   Wu, HB
   Yan, Y
   Wang, X
   Lou, XW
AF Zhang, Lei
   Wu, Hao Bin
   Yan, Ya
   Wang, Xin
   Lou, Xiong Wen (David)
TI Hierarchical MoS2 microboxes constructed by nanosheets with enhanced
   electrochemical properties for lithium storage and water splitting
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID HYDROGEN EVOLUTION REACTION; ION BATTERIES; HOLLOW NANOSTRUCTURES;
   FACILE SYNTHESIS; ANODE MATERIALS; GRAPHENE; PERFORMANCE; NANOWIRES;
   NANOTUBES; GROWTH
AB Hierarchical MoS2 microboxes constructed by ultrathin nanosheets are synthesized by a facile template-assisted strategy. The first step involves the L-cysteine assisted uniform growth of hierarchical MoS2 nanosheets on MnCO3 microcube templates which are at the same time converted to MnS. Hierarchical MoS2 microboxes can be obtained by selectively dissolving MnS through acid washing. When evaluated as an anode material for lithium-ion batteries, the hierarchical MoS2 microboxes manifest high specific capacity and excellent cycling performance. The hierarchical MoS2 microboxes also show enhanced electrocatalytic activity for electrochemical hydrogen evolution from water.
C1 [Zhang, Lei; Wu, Hao Bin; Yan, Ya; Wang, Xin; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
RP Zhang, L (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM wangxin@ntu.edu.sg; nvlou@ntu.edu.sg
RI Wang, Xin/G-6206-2010; Wu, Haobin/D-1572-2014; Lou , Xiong Wen
   (David)/D-2648-2009; Zhang, Lei/A-4182-2013; Yan, Ya/G-1693-2015
OI Wu, Haobin/0000-0002-0725-6442; Zhang, Lei/0000-0002-6385-5773; Yan,
   Ya/0000-0001-9218-4430
CR Zhou M, 2013, NANO TODAY, V8, P598, DOI 10.1016/j.nantod.2013.12.002
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NR 34
TC 67
Z9 68
U1 103
U2 340
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD OCT
PY 2014
VL 7
IS 10
BP 3302
EP 3306
DI 10.1039/c4ee01932f
PG 5
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AQ5YK
UT WOS:000342884300011
ER

PT J
AU Chen, DZ
   Wang, GS
   He, S
   Liu, J
   Guo, L
   Cao, MS
AF Chen, Dezhi
   Wang, Guang-Sheng
   He, Shuai
   Liu, Jia
   Guo, Lin
   Cao, Mao-Sheng
TI Controllable fabrication of mono-dispersed RGO-hematite nanocomposites
   and their enhanced wave absorption properties
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID LITHIUM ION BATTERIES; MICROWAVE-ABSORPTION; ANODE MATERIAL; TIO2
   NANOPARTICLES; CARBON NANOTUBES; GRAPHENE; PERFORMANCE; OXIDE;
   COMPOSITES; HYBRID
AB Novel RGO-hematite nanocomposites have been successfully fabricated using a surfactant-governed approach in the presence of polyvinylpyrrolidone (PVP) under mild wet chemical conditions (105 degrees C). A series of characterization methods including X-ray diffraction (XRD), Raman spectroscopy, scanning electron microscopy (SEM) and transmission electron microscopy (TEM) indicated that the as-prepared single-crystal hematite particles with relatively uniform size are embedded in RGO layers to form unique quasi shell-core nanostructures. The microwave absorption properties of the RGO-hematite composites were studied in detail; as an absorber, the RGO-hematite nanocomposites possess excellent microwave absorbing properties. The enhanced microwave absorbing properties were also explained based on the structures of the nanocomposites.
C1 [Chen, Dezhi; Wang, Guang-Sheng; He, Shuai; Guo, Lin] Beihang Univ, Sch Chem & Environm, Minist Educ, Key Lab Bioinspired Smart Interfacial Sci & Techn, Beijing 100191, Peoples R China.
   [Liu, Jia; Cao, Mao-Sheng] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
   [Chen, Dezhi] Nanchang Hangkong Univ, Sch Environm & Chem Engn, Key Lab Jiangxi Prov Persistent Pollutants Contro, Nanchang 330063, Peoples R China.
RP Chen, DZ (reprint author), Beihang Univ, Sch Chem & Environm, Minist Educ, Key Lab Bioinspired Smart Interfacial Sci & Techn, Beijing 100191, Peoples R China.
EM wanggsh@buaa.edu.cn; guolin@buaa.edu.cn; caomaosheng@bit.edu.cn
RI Wang, Guang-Sheng/G-4098-2015; 
OI Cao, Mao-Sheng/0000-0001-6810-9422
FU National Basic Research Program of China [2010CB934700, 2007CB310500];
   National Natural Science Foundation of China [5110223, 50725208,
   20973019]; State Key Project of Fundamental Research for Nanoscience and
   Nanotechnology [2006CB932301]
FX This work was supported by the National Basic Research Program of China
   (2010CB934700 and 2007CB310500) and the National Natural Science
   Foundation of China (5110223, 50725208 and 20973019), as well as the
   State Key Project of Fundamental Research for Nanoscience and
   Nanotechnology (2006CB932301).
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NR 51
TC 67
Z9 67
U1 36
U2 155
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 19
BP 5996
EP 6003
DI 10.1039/c3ta10664k
PG 8
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 130RF
UT WOS:000317936000027
ER

PT J
AU Wang, B
   Cheng, JL
   Wu, YP
   Wang, D
   He, DN
AF Wang, B.
   Cheng, J. L.
   Wu, Y. P.
   Wang, D.
   He, D. N.
TI Porous NiO fibers prepared by electrospinning as high performance anode
   materials for lithium ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Lithium-ion batteries; Anode materials; Electrospinning; Porous NiO
ID ELECTROCHEMICAL PERFORMANCE; ELECTRODE MATERIALS; HIGH-CAPACITY;
   STORAGE; NANOFIBERS; COMPOSITE; FABRICATION; GRAPHENE; OXIDE
AB We report a facile and scalable electrospinning method for preparing porous NiO fiber material by using a carbonized carbon as the self-sacrificing template. The as-prepared NiO fibers demonstrated a good electrochemical performance as anode materials for Li-ion batteries, including high reversible capacity of approximately 638 mAh g(-1) over 50 cycles, high rate capability with a discharge capacity of 477 mAh g(-1) even at a current density of 1760 mA g(-1), and good cycling performance. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Cheng, J. L.] Fudan Univ, Dept Macromol Sci, Shanghai 200433, Peoples R China.
   [Wang, B.; Wu, Y. P.] Fudan Univ, New Energy & Mat Lab NEML, Dept Chem, Shanghai 200433, Peoples R China.
   [Wang, B.; Wu, Y. P.] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
   [Wang, D.; He, D. N.] Natl Engn Res Ctr Nanotechnol, Shanghai, Peoples R China.
RP Cheng, JL (reprint author), Fudan Univ, Dept Macromol Sci, 220 Handan Rd, Shanghai 200433, Peoples R China.
EM jenny.jlcheng@gmail.com; wuyp@fudan.edu.cn
RI cheng, Jianli/K-1496-2014; Wu, Yuping/H-1593-2011
OI Wu, Yuping/0000-0002-0833-1205
FU International Science & Technology Cooperation Program of China
   [2010DFA61770, 2012DFG11660]
FX The authors would like to acknowledge the support from International
   Science & Technology Cooperation Program of China (2010DFA61770 and
   2012DFG11660). The authors also thank Prof. Yanbao Fu for sharing
   interesting and valuable discussions.
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NR 30
TC 67
Z9 68
U1 15
U2 181
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD SEP
PY 2012
VL 23
BP 5
EP 8
DI 10.1016/j.elecom.2012.07.003
PG 4
WC Electrochemistry
SC Electrochemistry
GA 021PM
UT WOS:000309897800002
ER

PT J
AU Lee, E
   Persson, KA
AF Lee, Eunseok
   Persson, Kristin A.
TI Li Absorption and Intercalation in Single Layer Graphene and Few Layer
   Graphene by First Principles
SO NANO LETTERS
LA English
DT Article
DE Li-ion batteries anode; Graphene; Li absorption; Li intercalation;
   First-principles calculation; Cluster expansion method
ID LITHIUM-ION BATTERIES; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY
   CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; MECHANISMS; INSERTION;
   STORAGE; SHEETS; METALS
AB We present an exhaustive first-principles investigation of Li absorption and intercalation in single layer graphene and few layer graphene, as compared to bulk graphite. For single layer graphene, the cluster expansion method is used to systemically search for the lowest energy ionic configuration as a function of absorbed Li content. It is predicted that there exists no Li arrangement that stabilizes Li absorption on the surface of single layer graphene unless that surface includes defects. From this result follows that defect-poor single layer graphene exhibits significantly inferior capacity compared to bulk graphite. For few layer graphene, we calibrate a semiempirical potential to include the effect of van der Waals interactions, which is essential to account for the contribution of empty (no Li) gallery to the total energy. We identify and analyze the Li intercalation mechanisms in few layer graphene and map out the sequence in stable phases as we move from single layer graphene, through few layer, to bulk graphite.
C1 [Lee, Eunseok; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
RP Lee, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM eunseoklee@lbl.gov
FU Office of Vehicle Technologies of the U.S. Department of Energy
   [DE-AC02-05CH11231]
FX Work at the Lawrence Berkeley National Laboratory was supported by the
   Assistant Secretary for Energy Efficiency and Renewable Energy, Office
   of Vehicle Technologies of the U.S. Department of Energy, under Contract
   No. DE-AC02-05CH11231.
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NR 35
TC 66
Z9 66
U1 17
U2 160
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD SEP
PY 2012
VL 12
IS 9
BP 4624
EP 4628
DI 10.1021/nl3019164
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 002YW
UT WOS:000308576000034
PM 22920219
ER

PT J
AU Liu, SY
   Xie, J
   Zheng, YX
   Cao, GS
   Zhu, TJ
   Zhao, XB
AF Liu, Shuang-Yu
   Xie, Jian
   Zheng, Yun-Xiao
   Cao, Gao-Shao
   Zhu, Tie-Jun
   Zhao, Xin-Bing
TI Nanocrystal manganese oxide (Mn3O4, MnO) anchored on graphite nanosheet
   with improved electrochemical Li-storage properties
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Mn3O4; MnO; Graphene; Graphite nanosheet; Electrochemical properties
ID LITHIUM-ION BATTERIES; NEGATIVE-ELECTRODE MATERIALS; REDUCED GRAPHENE
   OXIDE; ANODE MATERIAL; REVERSIBLE CAPACITY; PERFORMANCE; CELLS;
   INTERCALATION; NANOPARTICLES; REACTIVITY
AB Graphite nanosheet anchored with nanocrystal manganese oxide (Mn3O4, MnO) was synthesized by a facile in situ one-pot solvothennal route. It was found that nanosized Mn3O4 and MnO particles (30-50 nm) were homogeneously anchored on graphite nanosheet. During the hydrothermal reaction, the reduction of graphite oxide to graphite nanosheet and the formation of manganese oxide occur simultaneously, forming a manganese-oxide/graphite nanosheet sandwich structure. In this sandwich structure, the electrochemical properties of Mn3O4 and MnO can be obviously improved because of the buffering, confining and conducting effects of the graphite nanosheet. The good electrochemical performance of manganese-oxide/graphite nanosheet composites makes them potential application as anodes in Li-ion batteries. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Liu, Shuang-Yu; Xie, Jian; Zheng, Yun-Xiao; Cao, Gao-Shao; Zhu, Tie-Jun; Zhao, Xin-Bing] Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
RP Zhao, XB (reprint author), Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
EM zhaoxb@zju.edu.cn
FU Zhejiang University, China; Fundamental Research Funds for the Central
   Universities [2010QNA4003]; Ph.D. Programs Foundation of Ministry of
   Education of China [20100101120024]; Foundation of Education Office of
   Zhejiang Province [Y201016484]; Science Technology Department of
   Zhejiang Province [2011R10021]; National Natural Science Foundation of
   China [51101139]
FX This work was supported by Zijin Program of Zhejiang University, China,
   the Fundamental Research Funds for the Central Universities (No.
   2010QNA4003), the Ph.D. Programs Foundation of Ministry of Education of
   China (No. 20100101120024), the Foundation of Education Office of
   Zhejiang Province (No. Y201016484), the Qianjiang Talents Project of
   Science Technology Department of Zhejiang Province (2011R10021), and the
   National Natural Science Foundation of China (No. 51101139).
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NR 49
TC 66
Z9 69
U1 26
U2 183
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD APR 1
PY 2012
VL 66
BP 271
EP 278
DI 10.1016/j.electacta.2012.01.094
PG 8
WC Electrochemistry
SC Electrochemistry
GA 921BB
UT WOS:000302451900038
ER

PT J
AU Zhao, B
   Zhang, GH
   Song, JS
   Jiang, Y
   Zhuang, H
   Liu, P
   Fang, T
AF Zhao, Bing
   Zhang, Guohua
   Song, Jinsong
   Jiang, Yong
   Zhuang, Hua
   Liu, Peng
   Fang, Tao
TI Bivalent tin ion assisted reduction for preparing graphene/SnO2
   composite with good cyclic performance and lithium storage capacity
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Co-precipitation; GNS/SnO2 composite; Graphene; Lithium storage; Anode
   material
ID ANODE MATERIAL; CARBON; BATTERIES; OXIDE
AB Co-precipitation method of SnCl2 center dot 2H(2)O and graphene oxide (GO) solution was performed to fleetly prepare graphene/SnO2 composite. The structure and composition of the nanocomposite were detected by means of XRD, SEM, TEM and FT-IR. The GO was reduced by bivalent tin ions to graphene nanosheet (GNS) via solution reaction and SnO2 nano-crystals with size of 4-6 nm were homogeneously distributed on the matrix of GNS. It was found that the disorder degree of graphene in GNS/SnO2 composite prepared by the bivalent tin ion assisted reduction method was much lower than that of GNS obtained via pyrolysis reduction. The possible mechanism for this phenomenon was discussed in detail. The N-2 adsorption tests showed an ink-bottle-like pore structure of GNS/SnO2 and the SnO2 nanoparticles were confined in the interlayer of GNS without agglomeration. These structural features were desirable and enabled GNS/SnO2 an excellent anode material in lithium ion battery. The electrochemical tests showed that the composite could deliver a reversible capacity of 775.3 mAh/g and capacity retention of 98% after 50 cycles. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Zhao, Bing; Zhang, Guohua; Song, Jinsong; Jiang, Yong; Zhuang, Hua; Liu, Peng; Fang, Tao] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
RP Jiang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
EM jiangyong@shu.edu.cn
FU Shanghai Municipal Education Commission [10YZ03, 10YZ05]; Natural
   Science Foundation of Shanghai [09ZR1411800, 10ZR1411300]; Shanghai Key
   Laboratory of Green Chemistry and Chemical Processes (ECNU); Laboratory
   of Chemical Engineering (ECUST); Shanghai Leading Academic Discipline
   Project [S30109]
FX This work is supported by the Innovation Program of Shanghai Municipal
   Education Commission (10YZ03 and 10YZ05), Natural Science Foundation of
   Shanghai (09ZR1411800 and 10ZR1411300), Shanghai Key Laboratory of Green
   Chemistry and Chemical Processes (ECNU), Laboratory of Chemical
   Engineering (ECUST), and Shanghai Leading Academic Discipline Project
   (no. S30109).
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NR 31
TC 66
Z9 67
U1 13
U2 80
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD AUG 30
PY 2011
VL 56
IS 21
BP 7340
EP 7346
DI 10.1016/j.electacta.2011.06.037
PG 7
WC Electrochemistry
SC Electrochemistry
GA 821NW
UT WOS:000294982700014
ER

PT J
AU Nitta, N
   Yushin, G
AF Nitta, Naoki
   Yushin, Gleb
TI High-Capacity Anode Materials for Lithium- Ion Batteries: Choice of
   Elements and Structures for Active Particles
SO PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION
LA English
DT Article
DE lithium; Li-ion; high capacity; battery; review
ID TRANSMISSION ELECTRON-MICROSCOPY; LONG CYCLE LIFE; ALLOYED SN-FE(-C)
   POWDERS; SILICON THIN-FILMS; ONE-POT SYNTHESIS; IN-SITU XRD; IMPROVED
   ELECTROCHEMICAL PERFORMANCE; CORE-SHELL NANOPARTICLES; METAL NITRIDE
   ELECTRODES; ALIGNED CARBON NANOTUBE
AB Growing market demand for portable energy storage has triggered significant research on high-capacity lithium-ion (Li-ion) battery anodes. Various elements have been utilized in innovative structures to enable these anodes, which can potentially increase the energy density and decrease the cost of Li-ion batteries. In this review, electrode and material parameters are considered in anode fabrication. The periodic table is then used to explore how the choice of anode material affects rate performance, cycle stability, Li-ion insertion/extraction potentials, voltage hysteresis, volumetric and specific capacities, and other critical parameters. Silicon (Si), germanium (Ge), and tin (Sn) anodes receive more attention in literature and in this review, but other elements, such as antimony (Sb), lead (Pb), magnesium (Mg), aluminum (Al), gallium (Ga), phosphorus (P), arsenic (As), bismuth (Bi), and zinc (Zn) are also discussed. Among conversion anodes focus is placed on oxides, nitrides, phosphides, and hydrides. Nanostructured carbon (C) receives separate consideration. Issues in high- capacity research, such as volume change, insufficient coulombic efficiency, and solid electrolyte interphase (SEI) layer stability are elucidated. Finally, advanced carbon composites utilizing carbon nanotubes (CNT), graphene, and size preserving external shells are discussed, including high mass loading (thick) electrodes and electrodes capable of providing load-bearing properties.
C1 [Nitta, Naoki; Yushin, Gleb] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
RP Nitta, N (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
EM yushin@gatech.edu
RI Yushin, Gleb/B-4529-2013
OI Yushin, Gleb/0000-0002-3274-9265
FU US Air Force Office of Scientific Research (AFOSR) [FA9550-13-1-0054];
   Energy Efficiency & Resources program of the Korea Institute of Energy
   Technology Evaluation and Planning (KETEP); Korea government Ministry of
   Knowledge Economy [20118510010030]; US NSF IGERT NESAC program
FX This work was partially supported by the US Air Force Office of
   Scientific Research (AFOSR) (grant FA9550-13-1-0054) and by the Energy
   Efficiency & Resources program of the Korea Institute of Energy
   Technology Evaluation and Planning (KETEP) funded by the Korea
   government Ministry of Knowledge Economy (grants 20118510010030). Naoki
   Nitta acknowledges a doctoral fellowship supported by the US NSF IGERT
   NESAC program.
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NR 294
TC 65
Z9 65
U1 134
U2 606
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0934-0866
EI 1521-4117
J9 PART PART SYST CHAR
JI Part. Part. Syst. Charact.
PD MAR
PY 2014
VL 31
IS 3
BP 317
EP 336
DI 10.1002/ppsc.201300231
PG 20
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AD0MK
UT WOS:000332928100002
ER

PT J
AU Roberts, AD
   Li, X
   Zhang, HF
AF Roberts, Aled D.
   Li, Xu
   Zhang, Haifei
TI Porous carbon spheres and monoliths: morphology control, pore size
   tuning and their applications as Li-ion battery anode materials
SO CHEMICAL SOCIETY REVIEWS
LA English
DT Review
ID RECHARGEABLE LITHIUM BATTERIES; METAL-ORGANIC FRAMEWORKS;
   ENERGY-STORAGE; RATE CAPABILITY; SURFACE-AREA; PERFORMANCE;
   NANOPARTICLES; ELECTRODE; NANOSPHERES; POLYMER
AB The development of the next generation of advanced lithium-ion batteries (LIBs) requires new & advanced materials and novel fabrication techniques in order to push the boundaries of performance and open up new and exciting markets. Structured carbon materials, with controlled pore features on the micron and nanometer scales, are explored as advanced alternatives to conventional graphite as the active material of the LIB anode. Mesoporous carbon materials, carbon nanotube-based materials, and graphene-based materials have been extensively investigated and reviewed. Morphology control (e.g., colloids, thin films, nanofibrous mats, monoliths) and hierarchical pores (particularly the presence of large pores) exhibit an increasing influence on LIB performance. This tutorial review focuses on the synthetic techniques for preparation of porous carbon spheres and carbon monoliths, including hydrothermal carbonization, emulsion templating, ice templating and new developments in making porous carbons from sustainable biomass and metalorganic framework templating. We begin with a brief introduction to LIBs, defining key parameters and terminology used to assess the performance of anode materials, and then address synthetic techniques for the fabrication of carbon spheres & monoliths and the relevant composites, followed, respectively, by a review of their performance as LIB anode materials. The review is completed with a prospective view on the possible direction of future research in this field.
C1 [Roberts, Aled D.; Zhang, Haifei] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England.
   [Roberts, Aled D.; Li, Xu] ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore.
RP Li, X (reprint author), ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore.
EM x-li@imre.a-star.edu.sg; zhanghf@liv.ac.uk
RI Zhang, Haifei/F-3868-2011
OI Zhang, Haifei/0000-0001-5142-5824
FU University of Liverpool; Singapore A*STAR
FX AR is grateful for the joint PhD studentship between the University of
   Liverpool and Singapore A*STAR.
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NR 50
TC 65
Z9 65
U1 142
U2 561
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0306-0012
EI 1460-4744
J9 CHEM SOC REV
JI Chem. Soc. Rev.
PY 2014
VL 43
IS 13
BP 4341
EP 4356
DI 10.1039/c4cs00071d
PG 16
WC Chemistry, Multidisciplinary
SC Chemistry
GA AI8CA
UT WOS:000337131200005
PM 24705734
ER

PT J
AU Yan, Y
   Yin, YX
   Xin, S
   Guo, YG
   Wan, LJ
AF Yan, Yang
   Yin, Ya-Xia
   Xin, Sen
   Guo, Yu-Guo
   Wan, Li-Jun
TI Ionothermal synthesis of sulfur-doped porous carbons hybridized with
   graphene as superior anode materials for lithium-ion batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID RATE CAPABILITY; LI-ION; STORAGE; CARBONIZATION; PERFORMANCE;
   CONVERSION; CAPACITY; SHEETS
AB Sulfur-doped porous carbons hybridized with graphene (SPC@G) have been synthesized via a simple ionothermal method. The obtained SPC@G nanocomposite exhibits both high capacity and excellent rate performance, making it a promising anode material for lithium-ion batteries.
C1 [Yan, Yang; Yin, Ya-Xia; Xin, Sen; Guo, Yu-Guo; Wan, Li-Jun] Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn; wanlijun@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2012CB932900, 2011CB935700];
   National Natural Science Foundation of China [91127044, 21121063];
   Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2012CB932900 and 2011CB935700), the National Natural Science
   Foundation of China (Grant Nos. 91127044 and 21121063), and the Chinese
   Academy of Sciences.
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NR 32
TC 65
Z9 66
U1 33
U2 241
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PY 2012
VL 48
IS 86
BP 10663
EP 10665
DI 10.1039/c2cc36234a
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 014WF
UT WOS:000309405700023
PM 23011577
ER

PT J
AU Choi, SH
   Kang, YC
AF Choi, Seung Ho
   Kang, Yun Chan
TI Yolk-Shell, Hollow, and Single-Crystalline ZnCo2O4 Powders: Preparation
   Using a Simple One-Pot Process and Application in Lithium-Ion Batteries
SO CHEMSUSCHEM
LA English
DT Article
DE anode materials; energy conversion; lithium ion batteries;
   nanoparticles; spray pyrolysis
ID HIGH-PERFORMANCE ANODE; ELECTROCHEMICAL PERFORMANCE; REVERSIBLE
   CAPACITY; ALLOY ANODES; LI; NANOPARTICLES; NANOMATERIALS; GRAPHENE;
   MICROSPHERES; COBALT
AB The electrochemical properties of yolk-shell-structured, multi-component, transition-metal oxides have not yet been properly compared to those of hollow-structured or nanoscale powders. In this study, yolk-shell, hollow, and single-crystalline ZnCo2O4 powders with uniform compositions are prepared by using simple gas-phase reaction methods. Double-shelled ZnCo2O4 yolk-shell powder is prepared directly from the spray solution by using spray pyrolysis. Single-crystalline ZnCo2O4 nanopowder is prepared by means of flame spray pyrolysis. The yolk-shell ZnCo2O4 powder shows higher charge and discharge capacities than the hollow and single-crystalline powders. The yolk-shell, hollow, and single-crystalline ZnCo2O4 powders deliver discharge capacities of 753, 586, and 206mAhg(-1), respectively, after 200 cycles at a charge/discharge rate of 3Ag(-1), and the corresponding capacity retentions measured after the first cycle are 99, 74, and 27%, respectively. The yolk-shell ZnCo2O4 powders are structurally stable during cycling and have good electrochemical properties even at high current densities.
C1 [Choi, Seung Ho; Kang, Yun Chan] Konkuk Univ, Dept Chem Engn, Seoul 143701, South Korea.
RP Choi, SH (reprint author), Konkuk Univ, Dept Chem Engn, 1 Hwayang Dong, Seoul 143701, South Korea.
EM yckang@konkuk.ac.kr
RI Kang, Yun Chan/H-2457-2015
OI Kang, Yun Chan/0000-0001-5769-5761
FU National Research Foundation of Korea (NRF); Korea government (MEST)
   [2012R1A2A2A02046367]
FX This work was supported by the National Research Foundation of Korea
   (NRF) grant funded by the Korea government (MEST) (No.
   2012R1A2A2A02046367).
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U2 176
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1864-5631
EI 1864-564X
J9 CHEMSUSCHEM
JI ChemSusChem
PD NOV
PY 2013
VL 6
IS 11
BP 2111
EP 2116
DI 10.1002/cssc.201300300
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 250HA
UT WOS:000326840000019
PM 23908071
ER

PT J
AU Tang, YP
   Wu, DQ
   Chen, S
   Zhang, F
   Jia, JP
   Feng, XL
AF Tang, Yanping
   Wu, Dongqing
   Chen, Si
   Zhang, Fan
   Jia, Jinping
   Feng, Xinliang
TI Highly reversible and ultra-fast lithium storage in mesoporous
   graphene-based TiO2/SnO2 hybrid nanosheets
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID ION BATTERY ELECTRODES; AMORPHOUS OXIDE; ANODE MATERIAL; PERFORMANCE;
   SNO2; GROWTH; NANOPARTICLES; FABRICATION; NANOWIRES; GRAPHITE
AB A facile and scalable step-wise approach has been developed to fabricate graphene-based TiO2/SnO2 hybrid nanosheets (TiO2@SnO2@GN). With uniform staggered distribution of rutile SnO2 and TiO2 nanocrystals in a 2D mesoporous manner, TiO2@SnO2@GN with low content of graphene (similar to 5 wt%) manifests superior reversible capacity and excellent rate capability as an anode material in lithium-ion batteries.
C1 [Tang, Yanping; Wu, Dongqing; Chen, Si; Zhang, Fan; Feng, Xinliang] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Jia, Jinping] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China.
   [Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Tang, YP (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Dongchuan Rd 800, Shanghai 200240, Peoples R China.
EM fan-zhang@sjtu.edu.cn; feng@mpip-mainz.mpg.de
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NR 47
TC 64
Z9 64
U1 36
U2 270
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD AUG
PY 2013
VL 6
IS 8
BP 2447
EP 2451
DI 10.1039/c3ee40759d
PG 5
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 185QB
UT WOS:000321983800017
ER

PT J
AU Yu, HL
   Ma, C
   Ge, BH
   Chen, YJ
   Xu, Z
   Zhu, CL
   Li, CY
   Ouyang, QY
   Gao, P
   Li, JQ
   Sun, CW
   Qi, LH
   Wang, YM
   Li, FH
AF Yu, Hailong
   Ma, Chao
   Ge, Binghui
   Chen, Yujin
   Xu, Zheng
   Zhu, Chunling
   Li, Chunyan
   Ouyang, Qiuyun
   Gao, Peng
   Li, Jianqi
   Sun, Chunwen
   Qi, Lihong
   Wang, Yumei
   Li, Fanghua
TI Three-Dimensional Hierarchical Architectures Constructed by
   Graphene/MoS2 Nanoflake Arrays and Their Rapid Charging/Discharging
   Properties as Lithium-Ion Battery Anodes
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE graphene; lithium-ion battery; molybdenum; MoS2 nanoflake arrays;
   nanostructures; three-dimensional architectures
ID ELECTROMAGNETIC ABSORPTION PROPERTIES; ELECTROCHEMICAL PERFORMANCES;
   MOS2 NANOPARTICLES; EXFOLIATED MOS2; RATE CAPABILITY; HIGH-CAPACITY;
   STORAGE; NANOCOMPOSITES; CARBON; CATALYSTS
C1 [Yu, Hailong; Chen, Yujin; Xu, Zheng; Li, Chunyan; Ouyang, Qiuyun; Qi, Lihong] Harbin Engn Univ, Coll Sci, Harbin 150001, Peoples R China.
   [Ma, Chao; Ge, Binghui; Li, Jianqi; Sun, Chunwen; Wang, Yumei; Li, Fanghua] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
   [Zhu, Chunling; Gao, Peng] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China.
RP Chen, YJ (reprint author), Harbin Engn Univ, Coll Sci, Harbin 150001, Peoples R China.
EM chenyujin@hrbeu.edu.cn; gaopeng@hrbeu.edu.cn; csun@iphy.ac.cn
RI Sun, Chunwen/A-9860-2008; Ma, Chao/J-4569-2015
OI Sun, Chunwen/0000-0002-4916-4028; 
FU National Natural Science Foundation of China [51072038, 51272050,
   61205113, 51172275, 21001035]; Program for NCET in University
   [NECT-10-0049]; Outstanding Youth Foundation of Heilongjiang Province
   [JC201008]; Special Funds for Major State Basic Research Projects
   [2010CB934200]
FX We thank the National Natural Science Foundation of China (Grant Nos.
   51072038, 51272050, 61205113, 51172275 and 21001035), Program for NCET
   in University (Grant No. NECT-10-0049), Outstanding Youth Foundation of
   Heilongjiang Province (Grant No JC201008) for the financial support of
   this research and also the Special Funds for Major State Basic Research
   Projects (Grant No. 2010CB934200).
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NR 43
TC 64
Z9 65
U1 45
U2 402
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD MAY
PY 2013
VL 19
IS 19
BP 5818
EP 5823
DI 10.1002/chem.201300072
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 136LX
UT WOS:000318364500004
PM 23505063
ER

PT J
AU Chen, JS
   Lou, XW
AF Chen, Jun Song
   Lou, Xiong Wen (David)
TI SnO2 and TiO2 nanosheets for lithium-ion batteries
SO MATERIALS TODAY
LA English
DT Article
ID ONE-POT SYNTHESIS; GAS-SENSING PROPERTIES; EXPOSED 001 FACETS; ANATASE
   TIO2; STORAGE PROPERTIES; GRAPHENE NANOSHEETS; SINGLE-CRYSTALS; HOLLOW
   SPHERES; CAPACITY; NANOSTRUCTURES
AB Recent developments in nanotechnology and materials science offer potential solutions to the questions of how to improve performance and safety, as well as enhance the reliability of lithium-ion batteries (LIBs): the dominant power source for portable electronic devices. A wide range of nanostructured materials have been shown to exhibit enhanced electrochemical properties as promising electrode materials for high-performance LIBs. In this review article, we will discuss two metal oxides with sheet-like nanostructures: tin dioxide (SnO2) and titanium dioxide (TiO2). For SnO2 nanosheets, we discuss different systems for synthesizing such nanostructures and their application as the anode material for LIBs. In view of many recent review articles summarizing the various strategies for the preparation of TiO2 nanosheets, here we will stress the effect of this unique structure with exposed (001) facets on their lithium storage properties. By looking at these metal oxide nanosheets, we aim to provide some rational understanding of this unique category of nanomaterials and their electrochemical properties associated with their, novel structures.
C1 [Chen, Jun Song; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637457, Singapore.
   [Chen, Jun Song; Lou, Xiong Wen (David)] Nanyang Technol Univ, Energy Res Inst, Singapore 637553, Singapore.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 70 Nanyang Dr, Singapore 637457, Singapore.
EM xwlou@ntu.edu.sg
RI Lou , Xiong Wen (David)/D-2648-2009
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NR 64
TC 64
Z9 64
U1 21
U2 262
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 1369-7021
J9 MATER TODAY
JI Mater. Today
PD JUN
PY 2012
VL 15
IS 6
BP 246
EP 254
PG 9
WC Materials Science, Multidisciplinary
SC Materials Science
GA 970WE
UT WOS:000306162200016
ER

PT J
AU Li, Y
   Zhu, SM
   Liu, QL
   Gu, JJ
   Guo, ZP
   Chen, ZX
   Feng, CL
   Zhang, D
   Moon, WJ
AF Li, Yao
   Zhu, Shenmin
   Liu, Qinglei
   Gu, Jiajun
   Guo, Zaiping
   Chen, Zhixin
   Feng, Chuanliang
   Zhang, Di
   Moon, Won-Jin
TI Carbon-coated SnO2@C with hierarchically porous structures and graphite
   layers inside for a high-performance lithium-ion battery
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ELECTRODE MATERIALS; MESOPOROUS CARBON; STORAGE CAPACITY; SNO2
   NANOTUBES; ANODE MATERIAL; COMPOSITE; TIN; NANOWIRES; SURFACE
AB A high-performance anode material was prepared from a hierarchically structured activated carbon which contains in situ graphene and nano-graphite. The activated carbon was immersed in a solution of SnCl2 center dot 2H(2)O and subjected to ultrasound. As a result, nanoparticles of SnO2 were uniformly deposited on the surface of the activated carbon. The composite material was then coated with a thin layer of carbon by soaking it in a sucrose solution, followed by carbonization of the adsorbed sucrose at 500 degrees C. The resulting composite showed an outstanding high-rate cycling performance that can deliver an initial discharge capacity of 1417 mAh g(-1) and maintain a discharge capacity of more than 400 mAh g(-1) after 100 cycles at a high current density of 1000 mA g(-1). This outstanding electrochemical performance is likely to be related to a unique combination of the excellent electrical conductivity of the activated carbon with graphite layers formed inside, its hierarchical pore structure which enhances lithium-ion transportation, and the carbon coating which alleviates the effects of volume changes, shortens the distance for Li+ diffusion, facilitates the transmission of electrons, and keeps the structure stable.
C1 [Li, Yao; Zhu, Shenmin; Liu, Qinglei; Gu, Jiajun; Feng, Chuanliang; Zhang, Di] Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China.
   [Guo, Zaiping; Chen, Zhixin] Univ Wollongong, Fac Engn, Wollongong, NSW 2522, Australia.
   [Moon, Won-Jin] Korea Basic Sci Inst, Gwang Ju Ctr, Kwangju 500757, South Korea.
RP Zhu, SM (reprint author), Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China.
EM zhangdi@sjtu.edu.cn
RI Zhu, Shenmin/J-2481-2013
OI Zhu, Shenmin/0000-0003-3145-4446
FU Morgan Crucible Company; National Science Foundation of China [50772067,
   51072117, 51171110]; National Basic Research Program of China (973
   Program) [2010CB619600]; Shanghai Science and Technology Committee
   [10JC1407600]; Shanghai Jiao Tong University
FX The authors gratefully acknowledge financial support for this research
   from the Morgan Crucible Company, the National Science Foundation of
   China (Nos. 50772067, 51072117, 51171110), National Basic Research
   Program of China (973 Program) (No. 2010CB619600), Shanghai Science and
   Technology Committee (No. 10JC1407600) and Shanghai Jiao Tong University
   Innovation Fund For Postgraduates. We also thank the Shanghai Jiao Tong
   University (SJTU) Instrument Analysis Center for the measurements.
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NR 28
TC 64
Z9 64
U1 23
U2 126
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 6
BP 2766
EP 2773
DI 10.1039/c1jm14290a
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 877KI
UT WOS:000299178500058
ER

PT J
AU Etacheri, V
   Yourey, JE
   Bartlett, BM
AF Etacheri, Vinodkumar
   Yourey, Joseph E.
   Bartlett, Bart M.
TI Chemically Bonded TiO2-Bronze Nanosheet/Reduced Graphene Oxide Hybrid
   for High-Power Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE lithium ion batteries; nanosheets; reduced graphene oxide; titanium
   dioxide; anode
ID PHOTOCATALYTIC H-2-PRODUCTION ACTIVITY; NANOSTRUCTURED TIO2(B); ANODE
   PERFORMANCES; STORAGE; NANOCOMPOSITES; ANATASE; NANOPARTICLES;
   COMPOSITES; ELECTRODES; NANOWIRES
AB Although Li-ion batteries have attracted significant interest due to their higher energy density, lack of high rate performance electrode materials and intrinsic safety issues challenge their commercial applications. Herein, we demonstrate a simple photocatalytic reduction method that simultaneously reduces graphene oxide (GO) and anchors (010)-faceted mesoporous bronze-phase titania (TiO2-B) nanosheets to reduced graphene oxide (RGO) through Ti3+-C bonds. Formation of Ti3+-C bonds during the photocatalytic reduction process was identified using electron paramagnetic resonance (EPR) and X-ray photoelectron spectroscopy (XPS) techniques. When cycled between 1-3 V (vs Li+/0), these chemically bonded TiO2-B/RGO hybrid nanostructures show significantly higher Li-ion storage capacities and rate capability compared to bare TiO2-B nanosheets and a physically mixed TiO2-B/RGO composite. In addition, 80% of the initial specific (gravimetric) capacity was retained even after 1000 charge-discharge cycles at a high rate of 40C The improved electrochemical performance of TiO2-B/RGO nanoarchitectures is attributed to the presence of exposed (010) facets, mesoporosity, and efficient interfacial charge transfer between RGO monolayers and TiO2-B nanosheets.
C1 [Etacheri, Vinodkumar; Yourey, Joseph E.; Bartlett, Bart M.] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA.
RP Bartlett, BM (reprint author), Univ Michigan, Dept Chem, 930 North Univ Ave, Ann Arbor, MI 48109 USA.
EM bartmb@umich.edu
RI Bartlett, Bart/F-1233-2013
OI Bartlett, Bart/0000-0001-8298-5963
FU University of Michigan Energy Institute; National Science Foundation
   [DMR-1253347]; NSF [DMR-0320710, DMR-0315633]
FX We thank the University of Michigan Energy Institute for a Postdoctoral
   Partnerships for Innovation Fellowship for V.E. This work was supported
   by funding from the National Science Foundation (DMR-1253347).
   Spectroscopic (XPS) and microscopic (SEM, TEM, and AFM) characterization
   techniques at the University of Michigan Electron Microbeam Analysis
   Laboratory were funded by NSF Grant Nos. DMR-0320710 and DMR-0315633,
   respectively.
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NR 62
TC 63
Z9 65
U1 57
U2 317
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD FEB
PY 2014
VL 8
IS 2
BP 1491
EP 1499
DI 10.1021/nn405534r
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AB8SB
UT WOS:000332059200044
PM 24446910
ER

PT J
AU Zhou, XS
   Yin, YX
   Cao, AM
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Yin, Ya-Xia
   Cao, An-Min
   Wan, Li-Jun
   Guo, Yu-Guo
TI Efficient 3D Conducting Networks Built by Graphene Sheets and Carbon
   Nanoparticles for High-Performance Silicon Anode
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium-ion batteries; 3D conducting networks; silicon; graphene; carbon
   nanoparticles; anode materials
ID LITHIUM-ION BATTERIES; SELECTIVE DETECTION; FACILE SYNTHESIS; COATED
   SILICON; HIGH-CAPACITY; STORAGE; OXIDE; NANOSPHERES; FABRICATION;
   PARTICLES
AB The utilization of silicon particles as anode materials for lithium-ion batteries is hindered by their low intrinsic electric conductivity and large volume changes during cycling. Here we report a novel Si nanoparticle-carbon nanoparticle/graphene composite, in which the addition of carbon nanoparticles can effectively alleviate the aggregation of Si nanoparticles by separating them from each other, and help graphene sheets build efficient 3D conducting networks for Si nanoparticles. Such Si-C/G composite shows much improved electrochemical properties in terms of specific capacity and cycling performance (ca. 1521 mA h g(-1) at 0.2 C after 200 cycles), as well as a favorable high-rate capability.
C1 [Zhou, Xiaosi; Yin, Ya-Xia; Cao, An-Min; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2009CB930400,
   2012CB932900]; National Natural Science Foundation of China [91127044,
   21121063]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2011CB935700, 2009CB930400, and 2012CB932900), the National
   Natural Science Foundation of China (Grants 91127044 and 21121063), and
   the Chinese Academy of Sciences.
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NR 37
TC 63
Z9 63
U1 15
U2 156
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY
PY 2012
VL 4
IS 5
BP 2824
EP 2828
DI 10.1021/am3005576
PG 5
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 945OF
UT WOS:000304285200069
PM 22563769
ER

PT J
AU Cao, HQ
   Li, BJ
   Zhang, JX
   Lian, F
   Kong, XH
   Qu, MZ
AF Cao, Huaqiang
   Li, Baojun
   Zhang, Jingxian
   Lian, Fang
   Kong, Xianghua
   Qu, Meizhen
TI Synthesis and superior anode performance of TiO2@reduced graphene oxide
   nanocomposites for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ANATASE TIO2 NANOSHEETS; PHOTOCATALYTIC ACTIVITY; MESOPOROUS ANATASE;
   STRUCTURAL-CHANGES; PARTICLE-SIZE; HIGH-POWER; INTERCALATION; INSERTION;
   STORAGE; TIO2-GRAPHENE
AB Herein, we report the synthesis of TiO2-reduced graphene oxide composite (termed as TGC) nanostructures using tetrabutyl titanate as the titanium source via a solvothermal route. The TGC nanostructures were characterized by transmission electron microscopy, scanning electron microscopy, Fourier transform infrared spectroscopy, Raman spectroscopy, X-ray diffraction, X-ray photoelectron spectroscopy, and adsorption-desorption isotherms for nitrogen measurements. The TGC was used as the anode of lithium ion batteries for investigation. The hybrid nanocomposite exhibited remarkable improvement in lithium ion insertion/extraction behaviour compared with TiO2, which showed an initial irreversible capacity and a reversible capacity of 386.4 and 152.6 mAh g(-1) for TGC after 100 cycles at a high charge rate of 5 C (1000 mA g(-1)), compared to 69.5 and 9.7 mAh g(-1) for TiO2, respectively. The enhanced electrochemical performance of TGC is attributed to the increased conductivity in the presence of reduced graphene oxide in TGC, the small size of the TiO2 particles in TGC, which can shorten the transport paths for both Li+ ions and electrons, and the enlarged electrode-electrolyte contact area, leading to more electroactive sites in TGC.
C1 [Cao, Huaqiang; Li, Baojun] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Zhang, Jingxian; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
   [Lian, Fang; Kong, Xianghua] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
FU National High Technology Research and Development Program ("863"
   Program) of China [2012AA030306, 2009AA03Z226]; National Natural Science
   Foundation of China [20921001]
FX Financial supports from the National High Technology Research and
   Development Program ("863" Program) of China (2012AA030306 and
   2009AA03Z226) and the National Natural Science Foundation of China (No.
   20921001) are acknowledged.
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NR 61
TC 63
Z9 64
U1 14
U2 123
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 19
BP 9759
EP 9766
DI 10.1039/c2jm00007e
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 931HN
UT WOS:000303207100049
ER

PT J
AU Park, SK
   Yu, SH
   Pinna, N
   Woo, S
   Jang, B
   Chung, YH
   Cho, YH
   Sung, YE
   Piao, Y
AF Park, Seung-Keun
   Yu, Seung-Ho
   Pinna, Nicola
   Woo, Seunghee
   Jang, Byungchul
   Chung, Young-Hoon
   Cho, Yong-Hun
   Sung, Yung-Eun
   Piao, Yuanzhe
TI A facile hydrazine-assisted hydrothermal method for the deposition of
   monodisperse SnO2 nanoparticles onto graphene for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID GRAPHITE OXIDE; ANODE MATERIAL; HIGH-CAPACITY; TIN OXIDE; AQUEOUS
   DISPERSIONS; STORAGE PROPERTIES; COMPOSITE; ELECTRODE; PERFORMANCE;
   ENCAPSULATION
AB In this manuscript, we introduce a facile hydrothermal method for the controlled growth of SnO2 nanoparticles onto graphene oxide. Hydrazine plays a fundamental role in controlling the formation and crystallization of SnO2 nanoparticles, and the reduction of graphene oxide to graphene. The SnO2-graphene composite consists of 3-4 nm monodisperse SnO2 nanocrystals homogeneously dispersed at the surface of graphene. It is demonstrated that the composite can accommodate the large volume change of SnO2 which occurs during lithiation-delithiation cycles. When used as an anode material for lithium ion batteries, it exhibits a first discharge capacity of 1662 mA h g(-1), which rapidly stabilizes and still remains at 626 mA h g(-1) even after 50 cycles, when cycled at a current density of 100 mA g(-1). Even at the very high current density of 3200 mA g(-1), the composite displays a stable capacity of 383 mA h g(-1) after 50 cycles.
C1 [Yu, Seung-Ho; Pinna, Nicola; Chung, Young-Hoon; Sung, Yung-Eun] Seoul Natl Univ, WCU, Sch Chem & Biol Engn,Coll Med, Program Chem Convergence Energy & Environm C2E2, Seoul 151744, South Korea.
   [Park, Seung-Keun; Jang, Byungchul; Piao, Yuanzhe] Seoul Natl Univ, Grad Sch Convergence Sci & Technol, Dept Nano Sci & Technol, Suwon 443270, South Korea.
   [Pinna, Nicola] Univ Aveiro, CICECO, Dept Chem, P-3810193 Aveiro, Portugal.
   [Woo, Seunghee] Seoul Natl Univ, Dept Chem, Seoul 151747, South Korea.
   [Cho, Yong-Hun] Kookmin Univ, Sch Adv Mat Engn, Seoul 136702, South Korea.
   [Piao, Yuanzhe] Adv Inst Convergence Technol, Suwon 443270, Gyeonggi Do, South Korea.
RP Sung, YE (reprint author), Seoul Natl Univ, WCU, Sch Chem & Biol Engn,Coll Med, Program Chem Convergence Energy & Environm C2E2, Seoul 151744, South Korea.
EM parkat9@snu.ac.kr; ysung@snu.ac.kr
RI Park, Seung-Keun/E-8420-2011; Pinna, Nicola/G-2307-2010
OI Park, Seung-Keun/0000-0002-0373-163X; Pinna, Nicola/0000-0003-1273-803X
FU National Research Foundation of Korea (NRF); Ministry of Education,
   Science and Technology [2011-0025391]; Korea Research Council of
   Fundamental Science and Technology (KRCF); Korean Government (MEST)
   [NRF-C1AAA001-2010-0029065]; MEST [2009-0093814]; NRF
FX This research was supported by the Basic Science Research Program
   through the National Research Foundation of Korea (NRF) funded by the
   Ministry of Education, Science and Technology (No. 2011-0025391) and
   partial support from the Korea Research Council of Fundamental Science
   and Technology (KRCF) through the project of 'Development of
   Characterization Techniques for Nano-materials Safety'. YES acknowledges
   financial support from the National Research Foundation of Korea Grant
   funded by the Korean Government (MEST) (NRF-C1AAA001-2010-0029065).
   Yong-Hun Cho acknowledges financial support by the Priority Research
   Centers Program through NRF funded by MEST (2009-0093814).
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NR 42
TC 63
Z9 63
U1 18
U2 109
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 6
BP 2520
EP 2525
DI 10.1039/c1jm14199f
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 877KI
UT WOS:000299178500027
ER

PT J
AU Wang, ZY
   Zhang, H
   Li, N
   Shi, ZJ
   Gu, ZN
   Cao, GP
AF Wang, Zhiyong
   Zhang, Hao
   Li, Nan
   Shi, Zujin
   Gu, Zhennan
   Cao, Gaoping
TI Laterally Confined Graphene Nanosheets and Graphene/SnO2 Composites as
   High-Rate Anode Materials for Lithium-Ion Batteries
SO NANO RESEARCH
LA English
DT Article
DE Carbon; graphene; anode; lithium-ion batteries; SnO2; nanomaterials
ID HIGH-RATE CAPABILITY; RATE PERFORMANCE; HIGH-POWER; ELECTRODES;
   GRAPHITE; INTERCALATION; STORAGE; DIFFUSION; INSERTION; CAPACITY
AB High-rate anode materials for lithium-ion batteries are desirable for applications that require high power density. We demonstrate the advantageous rate capability of few-layered graphene nanosheets, with widths of 100-200 nm, over micro-scale graphene nanosheets. Possible reasons for the better performance of the former include their smaller size and better conductivity than the latter. Combination of SnO2 nanoparticles with graphene was used to further improve the gravimetric capacities of the electrode at high charge discharge rates. Furthermore, the volumetric capacity of the composites was substantially enhanced compared to pristine graphene due to the higher density of the composites.
C1 [Wang, Zhiyong; Li, Nan; Shi, Zujin; Gu, Zhennan] Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China.
   [Zhang, Hao; Cao, Gaoping] Res Inst Chem Def, Beijing 100083, Peoples R China.
RP Shi, ZJ (reprint author), Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China.
EM zjshi@pku.edu.cn
RI Wang, Zhiyong/C-3241-2012
FU National Natural Science Foundation of China [90206048, 20371004];
   Ministry of Science and Technology of China [2006CB932701, 2007AA03Z311]
FX The authors gratefully acknowledge the National Natural Science
   Foundation of China (Nos. 90206048 and 20371004) and the Ministry of
   Science and Technology of China (Grant Nos. 2006CB932701 and
   2007AA03Z311) for financial support.
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NR 30
TC 63
Z9 66
U1 7
U2 61
PU TSINGHUA UNIV PRESS
PI BEIJING
PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA
SN 1998-0124
J9 NANO RES
JI Nano Res.
PD OCT
PY 2010
VL 3
IS 10
BP 748
EP 756
DI 10.1007/s12274-010-0041-5
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 677UK
UT WOS:000284017100009
ER

PT J
AU Lee, SH
   Sridhar, V
   Jung, JH
   Karthikeyan, K
   Lee, YS
   Mukherjee, R
   Koratkar, N
   Oh, IK
AF Lee, Si-Hwa
   Sridhar, Vadahanambi
   Jung, Jung-Hwan
   Karthikeyan, Kaliyappan
   Lee, Yun-Sung
   Mukherjee, Rahul
   Koratkar, Nikhil
   Oh, Il-Kwon
TI Graphene-Nanotube-Iron Hierarchical Nanostructure as Lithium Ion Battery
   Anode
SO ACS NANO
LA English
DT Article
DE bio-inspired hierarchy; graphene-nanotube-iron composite;
   three-dimensional nanostructure; anode material; lithium-ion batteries
ID SOLAR-CELLS; PERFORMANCE; COMPOSITE; REDUCTION; STORAGE; FILMS; OXIDE
AB In this study, we report a novel route via microwave irradiation to synthesize a bio-inspired hierarchical graphene-nanotube-iron three-dimensional nanostructure as an anode material in lithium-ion batteries. The nanostructure comprises vertically aligned carbon nanotubes grown directly on graphene sheets along with shorter branches of carbon nanotubes stemming out from both the graphene sheets and the vertically aligned carbon nanotubes. This bio-inspired hierarchical structure provides a three-dimensional conductive network for efficient charge-transfer and prevents the agglomeration and restacking of the graphene sheets enabling Li-ions to have greater access to the electrode material. In addition, functional iron-oxide nanoparticles decorated within the three-dimensional hierarchical structure provides outstanding lithium storage characteristics, resulting in very high specific capacities. The anode material delivers a reversible capacity of similar to 1024 mA.h.g(-1) even after prolonged cycling along with a Coulombic efficiency in excess of 99%, which reflects the ability of the hierarchical network to prevent agglomeration of the iron-oxide nanoparticles.
C1 [Lee, Si-Hwa; Sridhar, Vadahanambi; Jung, Jung-Hwan; Oh, Il-Kwon] Korea Adv Inst Sci & Technol, Div Ocean Syst Engn, Sch Mech Aerosp & Syst Engn, Graphene Res Ctr,KAIST Inst NanoCentury, Taejon 305701, South Korea.
   [Jung, Jung-Hwan] Univ Texas Dallas, AG MacDiarmid NanoTech Inst, Richardson, TX 75080 USA.
   [Karthikeyan, Kaliyappan; Lee, Yun-Sung] Chonnam Natl Univ, Fac Appl Chem Engn, Kwangju 500757, South Korea.
   [Mukherjee, Rahul; Koratkar, Nikhil] Rensselaer Polytech Inst, Jonsson Engn Ctr 4009, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
RP Oh, IK (reprint author), Korea Adv Inst Sci & Technol, Div Ocean Syst Engn, Sch Mech Aerosp & Syst Engn, Graphene Res Ctr,KAIST Inst NanoCentury, 291 Daehak Ro, Taejon 305701, South Korea.
EM ikoh@kaistac.kr
RI Mukherjee, Rahul/H-8174-2013; OH, ILKWON/B-7121-2011; Sridhar,
   V/B-4660-2010; 
OI Mukherjee, Rahul/0000-0002-2358-9247; Sridhar, V/0000-0003-1833-460X;
   Kaliyappan, Karthikeyan/0000-0001-8218-5237
FU International Cooperation of the Korea Institute of Energy Technology
   Evaluation and Planning (KETEP); Korea government Ministry of Knowledge
   Economy [20128510010050]; National Research Foundation of Korea; Korean
   government [2012R1A2A2A01047543]
FX This work was supported by the International Cooperation of the Korea
   Institute of Energy Technology Evaluation and Planning (KETEP) grant
   funded by the Korea government Ministry of Knowledge Economy (No.
   20128510010050). This work was supported by a National Research
   Foundation of Korea grant funded by the Korean government
   (2012R1A2A2A01047543).
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NR 40
TC 62
Z9 62
U1 25
U2 215
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD MAY
PY 2013
VL 7
IS 5
BP 4242
EP 4251
DI 10.1021/nn4007253
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 156XD
UT WOS:000319856300061
PM 23550743
ER

PT J
AU Yang, XL
   Fan, KC
   Zhu, YH
   Shen, JH
   Jiang, X
   Zhao, P
   Luan, SR
   Li, CZ
AF Yang, Xiaoling
   Fan, Kaicai
   Zhu, Yihua
   Shen, Jianhua
   Jiang, Xin
   Zhao, Peng
   Luan, Shaorong
   Li, Chunzhong
TI Electric Papers of Graphene-Coated Co3O4 Fibers for High-Performance
   Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE graphene paper; Co3O4 fiber; anode; lithium-ion batteries
ID ANODE MATERIAL; REVERSIBLE CAPACITY; STORAGE PROPERTIES; CYCLING
   STABILITY; MESOPOROUS CO3O4; ENERGY-STORAGE; OXIDE SHEETS;
   NANOPARTICLES; PARTICLES; NANOCOMPOSITE
AB A facile strategy to synthesize the novel composite paper of graphene nanosheets (GNS) coated Co3O4 fibers is reported as an advanced anode material for high-performance lithium-ion batteries (LIBs). The GNS were able to deposit onto Co3O4 fibers and form the coating via electrostatic interactions. The unique hybrid paper is evaluated as an anode electrode for LIBs, and it exhibits a very large reversible capacity (similar to 840 mA h g(-1) after 40 cycles), excellent cyclic stability and good rate capacity. The substantially excellent electrochemical performance of the graphene/Co3O4 composite paper is the result from its unique features. Notably, the flexible structure of graphenic scaffold and the strong interaction between graphene and Co3O4 fibers are beneficial for providing excellent electronic conductivity, short transportation length for lithium ions, and elastomeric space to accommodate volume varies upon Li+ insertion/extraction.
C1 [Yang, Xiaoling; Fan, Kaicai; Zhu, Yihua; Shen, Jianhua; Jiang, Xin; Zhao, Peng; Li, Chunzhong] E China Univ Sci & Technol, Sch Mat Sci & Engn, Key Lab Ultrafine Mat, Minist Educ, Shanghai, Peoples R China.
   [Luan, Shaorong] E China Univ Sci & Technol, Sch Chem & Mol Engn, Res Ctr Anal & Test, Shanghai, Peoples R China.
RP Yang, XL (reprint author), E China Univ Sci & Technol, Sch Mat Sci & Engn, Key Lab Ultrafine Mat, Minist Educ, 130 Meilong Rd, Shanghai, Peoples R China.
EM xlyang@ecust.edu.cn; yhzhu@ecust.edu.cn
RI Li, Chunzhong/B-1103-2015
OI Li, Chunzhong/0000-0001-7897-5850
FU National Natural Science Foundation of China [21236003, 21206042,
   20925621, 20976054, 21176083]; Fundamental Research Funds for the
   Central Universities; Program for Changjiang Scholars and Innovative
   Research Team in University [IRT0825]; Shanghai Leading Academic
   Discipline Project [B502]
FX We thank the National Natural Science Foundation of China (21236003,
   21206042, 20925621, 20976054, and 21176083), the Fundamental Research
   Funds for the Central Universities, and the Program for Changjiang
   Scholars and Innovative Research Team in University (IRT0825), and the
   Shanghai Leading Academic Discipline Project (project number: B502) for
   financial supports.
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TC 62
Z9 62
U1 25
U2 255
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD FEB 13
PY 2013
VL 5
IS 3
BP 997
EP 1002
DI 10.1021/am302685t
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 091WE
UT WOS:000315079700070
PM 23320959
ER

PT J
AU Hassoun, J
   Bonaccorso, F
   Agostini, M
   Angelucci, M
   Betti, MG
   Cingolani, R
   Gemmi, M
   Mariani, C
   Panero, S
   Pellegrini, V
   Scrosati, B
AF Hassoun, Jusef
   Bonaccorso, Francesco
   Agostini, Marco
   Angelucci, Marco
   Betti, Maria Grazia
   Cingolani, Roberto
   Gemmi, Mauro
   Mariani, Carlo
   Panero, Stefania
   Pellegrini, Vittorio
   Scrosati, Bruno
TI An Advanced Lithium-Ion Battery Based on a Graphene Anode and a Lithium
   Iron Phosphate Cathode
SO NANO LETTERS
LA English
DT Article
DE Graphene; nanoflakes; inks; anode; lithium ion battery
ID FEW-LAYER GRAPHENE; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE;
   HIGH-QUALITY; THIN-FILMS; STORAGE; GRAPHITE; EXFOLIATION; STABILITY;
   INTERCALATION
AB We report an advanced lithium-ion battery based on a graphene ink anode and a lithium iron phosphate cathode. By carefully balancing the cell composition and suppressing the initial irreversible capacity of the anode in the round of few cycles, we demonstrate an optimal battery performance in terms of specific capacity, that is, 165 mAhg(-1), of an estimated energy density of about 190 Wh kg(-1) and a stable operation for over 80 charge-discharge cycles. The components of the battery are low cost and potentially scalable. To the best of our knowledge, complete, graphene-based, lithium ion batteries having performances comparable with those offered by the present technology are rarely reported; hence, we believe that the results disclosed in this work may open up new opportunities for exploiting graphene in the lithium-ion battery science and development.
C1 [Hassoun, Jusef; Agostini, Marco; Panero, Stefania] Univ Roma La Sapienza, Dept Chem, I-00185 Rome, Italy.
   [Bonaccorso, Francesco; Cingolani, Roberto; Pellegrini, Vittorio; Scrosati, Bruno] Ist Italiano Tecnol, Graphene Labs, I-16163 Genoa, Italy.
   [Scrosati, Bruno] Ist Italiano Tecnol, I-16163 Genoa, Italy.
   [Bonaccorso, Francesco] CNR, Ist Proc Chim Fis, I-98158 Messina, Italy.
   [Bonaccorso, Francesco; Pellegrini, Vittorio] CNR, Ist Nanosci, NEST, I-56127 Pisa, Italy.
   [Bonaccorso, Francesco; Pellegrini, Vittorio] Scuola Normale Super Pisa, I-56127 Pisa, Italy.
   [Angelucci, Marco; Betti, Maria Grazia; Mariani, Carlo] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy.
   [Gemmi, Mauro] Ist Italiano Tecnol, Ctr Nanotechnol Innovat NEST, I-56127 Pisa, Italy.
RP Hassoun, J (reprint author), Univ Roma La Sapienza, Dept Chem, I-00185 Rome, Italy.
EM Jusef.hassoun@uniroma1.it; francesco.bonaccorso@iit.it;
   bruno.scrosati@gmail.com
RI Gemmi, Mauro/C-9978-2015; Betti, Maria Grazia/F-5410-2011; Bonaccorso,
   Francesco/N-6752-2015; 
OI Betti, Maria Grazia/0000-0002-6244-0306; Bonaccorso,
   Francesco/0000-0001-7238-9420; Hassoun, Jusef/0000-0002-8218-5680
FU Graphene Flagship [CNECT-ICT-604391]; Lancaster University through the
   Distinguished Visitor Programme in Physical Sciences
FX We acknowledge C. Coletti and F. Carillo for useful discussions and the
   Graphene Flagship (contract no. CNECT-ICT-604391) for financial support.
   V.P. acknowledges support of the Lancaster University through the
   Distinguished Visitor Programme in Physical Sciences.
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NR 51
TC 61
Z9 61
U1 33
U2 146
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2014
VL 14
IS 8
BP 4901
EP 4906
DI 10.1021/nl502429m
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AN2WH
UT WOS:000340446200108
PM 25026051
ER

PT J
AU Zhu, J
   Zhang, GH
   Yu, XZ
   Li, QH
   Lu, BA
   Xu, Z
AF Zhu, Jian
   Zhang, Guanhua
   Yu, Xinzhi
   Li, Qiuhong
   Lu, Bingan
   Xu, Zhi
TI Graphene double protection strategy to improve the SnO2 electrode
   performance anodes for lithium-ion batteries
SO NANO ENERGY
LA English
DT Article
DE Nanocomposite; SnO2@graphene@graphene; Double protection; Lithium-ion
   batteries
ID HOLLOW NANOSTRUCTURES; NANOWALL ARRAYS; STORAGE; CARBON; COMPOSITES;
   SUPERCAPACITORS; NANOSHEETS; NANOTUBES; CAPACITY; GROWTH
AB SnO2 is considered as one of the most promising anode material because of its high lithium storage capability. However, poor cycling performance caused by serious aggregation and considerable volume change upon cycling hampers its industrial application. In this paper, a simple synthesis route is demonstrated for the preparation of SnO2@graphene@graphene (SnO2@G@G) for Lithium ion battery applications. The graphene was initially treated using strong sonicate to form numerous highly dispersed small graphene nanosheets (SGNSs) in the solution. SnO2@graphene (SnO2@G) composite is obtained in the form of a nonwoven mat by electrospinning followed by calcination at 450 degrees C in air. SnO2@G@G composite was prepared by using a simple solution mixing method. The novel SnO2@G@G composite exhibits enhanced electrochemical performance as anode material for LIBs. Furthermore, this simple and efficient synthesis strategy is versatile and can be extended to fabrication of various types of composites between graphene and metal oxides which could be widely used in many fields, like transparent and flexibility electrode. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Zhu, Jian; Zhang, Guanhua; Yu, Xinzhi; Li, Qiuhong; Lu, Bingan; Xu, Zhi] Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
RP Lu, BA (reprint author), Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM luba2012@hnu.edu.cn
FU National Natural Science Foundation of China [11274107, 61204109];
   Fundamental Research Funds for the Central Universities [531107040664,
   531106010012]
FX We gratefully acknowledge financial support from the National Natural
   Science Foundation of China (Grant nos. 11274107 and 61204109), and
   Fundamental Research Funds for the Central Universities (No.
   531107040664 and 531106010012).
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SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD JAN
PY 2014
VL 3
BP 80
EP 87
DI 10.1016/j.nanoen.2013.10.009
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AA2HI
UT WOS:000330915300009
ER

PT J
AU Yu, P
   Ritter, JA
   White, RE
   Popov, BN
AF Yu, P
   Ritter, JA
   White, RE
   Popov, BN
TI Ni-composite microencapsulated graphite as the negative electrode in
   lithium-ion batteries - I. Initial irreversible capacity study
SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY
LA English
DT Article
ID PROPYLENE CARBONATE; CO2 ADDITION; SYSTEM; ANODE; DECOMPOSITION;
   INSERTION; CELLS
AB A novel approach for suppressing the solvated lithium intercalation in graphite was developed by microencapsulating graphite with nanosized Ni-composite particles. The Ni-composite graphite showed great improvement in charge-discharge performance, coulomb efficiency, and cycling behavior when used as the negative electrode in a Li-ion cell with propylene carbonate (PC)-based electrolyte. For example, a 10 wt % Ni-composite coating increased the initial charge-discharge coulomb efficiency of SFG75 graphite (75 mu m, Timcal America) from 59 to 84% and the reversible capacity by 30-40 mAh/g. The Ni-composite coating con consisted of nanosized particles distributed over the surface of the graphite particle, which effectively blocked some of the edge surfaces exposed to the electrolyte. This minimized solvated lithium intercalation at these edge sites, which subsequently minimized the PC reduction within the graphite and the exfoliation of the graphene layers, and also gas evolution. Corresponding improvements in both the charge-discharge performance and safety of the negative electrode in a rechargeable Li-ion cell resulted. (C) 2000 The Electrochemical Society. S0013-4651(99)08-113-6. All rights reserved.
C1 Univ S Carolina, Dept Chem Engn, Ctr Electrochem Engn, Columbia, SC 29208 USA.
RP Yu, P (reprint author), Univ S Carolina, Dept Chem Engn, Ctr Electrochem Engn, Columbia, SC 29208 USA.
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U1 3
U2 18
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PI PENNINGTON
PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA
SN 0013-4651
J9 J ELECTROCHEM SOC
JI J. Electrochem. Soc.
PD APR
PY 2000
VL 147
IS 4
BP 1280
EP 1285
DI 10.1149/1.1393350
PG 6
WC Electrochemistry; Materials Science, Coatings & Films
SC Electrochemistry; Materials Science
GA 302AY
UT WOS:000086343800009
ER

PT J
AU Kim, H
   Cho, MY
   Kim, MH
   Park, KY
   Gwon, H
   Lee, Y
   Roh, KC
   Kang, K
AF Kim, Haegyeom
   Cho, Min-Young
   Kim, Mok-Hwa
   Park, Kyu-Young
   Gwon, Hyeokjo
   Lee, Yunsung
   Roh, Kwang Chul
   Kang, Kisuk
TI A Novel High-Energy Hybrid Supercapacitor with an Anatase TiO2-Reduced
   Graphene Oxide Anode and an Activated Carbon Cathode
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID LITHIUM-ION BATTERIES; HIGH-POWER; RECHARGEABLE BATTERIES;
   ELECTROCHEMICAL CAPACITORS; ELECTRODE MATERIAL; STORAGE DEVICES; SULFUR
   CATHODES; TIO2 ANATASE; PERFORMANCE; EFFICIENT
AB A hybrid supercapacitor with high energy and power densities is reported. It comprises a composite anode of anatase TiO2 and reduced graphene oxide and an activated carbon cathode in a non-aqueous electrolyte. While intercalation compounds can provide high energy typically at the expense of power, the anatase TiO2 nanoparticles are able to sustain both high energy and power in the hybrid supercapacitor. At a voltage range from 1.0 to 3.0 V, 42 W h kg(-1) of energy is achieved at 800 W kg(-1). Even at a 4-s charge/discharge rate, an energy density as high as 8.9 W h kg(-1) can be retained. The high energy and power of this hybrid supercapacitor bridges the gap between conventional batteries with high energy and low power and supercapacitors with high power and low energy.
C1 [Kim, Haegyeom; Park, Kyu-Young; Gwon, Hyeokjo; Kang, Kisuk] Seoul Natl Univ, Dept Mat Sci & Engn, RIAM, Seoul, South Korea.
   [Cho, Min-Young; Kim, Mok-Hwa; Roh, Kwang Chul] KICET, Seoul 153801, South Korea.
   [Lee, Yunsung] Chonnam Natl Univ, Fac Appl Chem Engn, Kwangju 500757, South Korea.
   [Kang, Kisuk] Seoul Natl Univ, Ctr Nanoparticle Res, IBS, Seoul 151742, South Korea.
RP Kang, K (reprint author), Seoul Natl Univ, Dept Mat Sci & Engn, RIAM, 599 Gwanak Ro, Seoul, South Korea.
EM matlgen1@snu.ac.kr
RI Kang, Kisuk/B-5776-2011; Kim, Haegyeom/E-4448-2011; 
OI Kim, Haegyeom/0000-0002-5962-8244
FU Energy Efficiency and Resources R&D program under the Ministry of
   Knowledge Economy, Republic of Korea [20112020100070]; Human Resources
   Development program of the Korea Institute of Energy Technology
   Evaluation and Planning (KETEP) [20124010203320]; Korean government
   through the Ministry of Trade, Industry and Energy; National Research
   Foundation of Korea; Korean Government (MEST) [NRF-2009-0094219];
   Converging Research Center Program through the Ministry of Education,
   Science and Technology [2012K001267]
FX This work was supported by (i) the Energy Efficiency and Resources R&D
   program (20112020100070) under the Ministry of Knowledge Economy,
   Republic of Korea, (ii) the Human Resources Development program
   (20124010203320) of the Korea Institute of Energy Technology Evaluation
   and Planning (KETEP) grant, which was funded by the Korean government
   through the Ministry of Trade, Industry and Energy., (iii) the National
   Research Foundation of Korea Grant Funded by the Korean Government
   (MEST) (NRF-2009-0094219), and (iv) the Converging Research Center
   Program through the Ministry of Education, Science and Technology
   (2012K001267).
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NR 54
TC 60
Z9 61
U1 51
U2 250
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD NOV
PY 2013
VL 3
IS 11
BP 1500
EP 1506
DI 10.1002/aenm.201300467
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AA2XJ
UT WOS:000330957200014
ER

PT J
AU Luo, YS
   Luo, JS
   Zhou, WW
   Qi, XY
   Zhang, H
   Yu, DYW
   Li, CM
   Fan, HJ
   Yu, T
AF Luo, Yongsong
   Luo, Jingshan
   Zhou, Weiwei
   Qi, Xiaoying
   Zhang, Hua
   Yu, Denis Y. W.
   Li, Chang Ming
   Fan, Hong Jin
   Yu, Ting
TI Controlled synthesis of hierarchical graphene-wrapped TiO2@Co3O4 coaxial
   nanobelt arrays for high-performance lithium storage
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ION BATTERY APPLICATIONS; ANODE MATERIAL; HIGH-CAPACITY; CORE/SHELL
   NANOWIRES; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; OXIDE; TIO2; LI;
   ELECTRODE
AB As one of the most important research areas in lithium-ion batteries (LIBs), well-designed nanostructures have been regarded as key for solving problems such as lithium ion diffusion, the collection and transport of electrons, and the large volume changes during cycling processes. Here, hierarchical graphene-wrapped TiO2@Co3O4 coaxial nanobelt arrays (G-TiO2@Co3O4 NBs) have been fabricated and further investigated as the electrode materials for LIBs. The results show that the yielded G-TiO2@Co3O4 NBs possess a high reversible capacity, an outstanding cycling performance, and superior rate capability compared to TiO2 and TiO2@Co3O4 nanobelt array (TiO2@Co3O4 NBs) electrodes. The core-shell TiO2@Co3O4 NBs may contain many cavities and provide more extra spaces for lithium ion storage. The introduction of graphene into nanocomposite electrodes is favorable for increasing their electrical conductivity and flexibility. The integration of hierarchical core-shell nanobelt arrays and conducting graphene may induce a positive synergistic effect and contribute to the enhanced electrochemical performances of the electrode. The fabrication strategy presented here is facile, cost-effective, and can offer a new pathway for large-scale energy storage device applications.
C1 [Luo, Yongsong; Luo, Jingshan; Zhou, Weiwei; Fan, Hong Jin; Yu, Ting] Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore.
   [Luo, Yongsong; Yu, Denis Y. W.; Fan, Hong Jin; Yu, Ting] Nanyang Technol Univ ERIAN, Energy Res Inst, Singapore 639789, Singapore.
   [Qi, Xiaoying; Zhang, Hua] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Li, Chang Ming] Southwest Univ, Inst Clean Energy & Adv Mat, Chongqing 400700, Peoples R China.
   [Li, Chang Ming] Nanyang Technol Univ, Div Bioengn, Sch Chem & Biomed Engn, Singapore 637371, Singapore.
   [Yu, Ting] Natl Univ Singapore, Dept Phys, Fac Sci, Singapore 117542, Singapore.
   [Luo, Yongsong] Xinyang Normal Univ, Sch Phys & Elect Engn, Xinyang 464000, Peoples R China.
RP Luo, YS (reprint author), Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore.
EM yuting@ntu.edu.sg
RI Fan, Hongjin/A-2662-2010; Qi, Xiaoying/C-1359-2014; Zhang,
   Hua/A-1302-2009; Qi, Xiaoying/F-9585-2016; 
OI Fan, Hongjin/0000-0003-1237-4555; Yu, Ting/0000-0002-0113-2895; Luo,
   Jingshan/0000-0002-1770-7681; Yu, Denis/0000-0002-5883-7087
FU Singapore National Research Foundation under NRF RF Award
   [NRF-RF2010-07]; MOE Tier 2 [MOE2009-T2-1-037]; CRP Award
   [NRF-CRP4-2008-03]
FX This work is supported by the Singapore National Research Foundation
   under NRF RF Award no. NRF-RF2010-07, MOE Tier 2 MOE2009-T2-1-037 and
   CRP Award no.: NRF-CRP4-2008-03.
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NR 65
TC 60
Z9 62
U1 41
U2 267
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 2
BP 273
EP 281
DI 10.1039/c2ta00064d
PG 9
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085RJ
UT WOS:000314631700020
ER

PT J
AU Wang, DN
   Li, XF
   Wang, JJ
   Yang, JL
   Geng, DS
   Li, RY
   Cai, M
   Sham, TK
   Sun, XL
AF Wang, Dongniu
   Li, Xifei
   Wang, Jiajun
   Yang, Jinli
   Geng, Dongsheng
   Li, Ruying
   Cai, Mei
   Sham, Tsun-Kong
   Sun, Xueliang
TI Defect-Rich Crystalline SnO2 Immobilized on Graphene Nanosheets with
   Enhanced Cycle Performance for Li Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID REVERSIBLE LITHIUM STORAGE; CARBON; OXIDE; NANOTUBES; ANODES; GROWTH
AB A one-step microwave-assisted hydrothermal method (MAHM) has been developed to synthesize SnO2/graphene composites. It is shown that fine SnO2 nanoparticles with an average size of 3.5 nm can be homogeneously deposited on graphene nanosheets (GNSs) using this technique. The electronic structure as revealed from X-ray absorption near edge structure (XANES) shows that the SnO2 nanoparticles are abundant in surface defects with oxygen vacancies, which facilitate the immobilization of SnO2 onto GNSs by electronic interaction. Carbon K edge XANES provide direct evidence of strong interaction between SnO2 and GNSs. The SnO2/graphene nanocomposites deliver a superior reversible capacity of 635 mAh g(-1) after 100 cycles and display excellent rate performance. All these desirable features strongly indicate that SnO2/graphene composite is a promising anode material in high-performance lithium ion batteries.
C1 [Wang, Dongniu; Sham, Tsun-Kong] Univ Western Ontario, Dept Chem, London, ON N6A 5B7, Canada.
   [Wang, Dongniu; Li, Xifei; Wang, Jiajun; Yang, Jinli; Geng, Dongsheng; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B7, Canada.
   [Cai, Mei] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Sham, TK (reprint author), Univ Western Ontario, Dept Chem, London, ON N6A 5B7, Canada.
EM tsham@uwo.ca; xsun@eng.uwo.ca
RI Li, Xifei/A-1966-2012; Sun, Andy (Xueliang)/I-4535-2013; Geng,
   Dongsheng/G-7124-2011; Sun, Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; 
FU Natural Sciences and Engineering Research Council of Canada (NSERC);
   General Motors of Canada; Canada Research Chair (CRC); Canada Foundation
   for Innovation (CFI); Ontario Innovation Trust (OTT) Program; University
   of Western Ontario
FX This research was supported by Natural Sciences and Engineering Research
   Council of Canada (NSERC), General Motors of Canada, Canada Research
   Chair (CRC), Canada Foundation for Innovation (CFI), Ontario Innovation
   Trust (OTT) Program, and University of Western Ontario. The Canadian
   Light Source is supported by CFI, NSERC, NRC, CHIR, and the University
   of Saskatchewan. The technical assistance of Tom Regier and David
   Chevrier of the Canadian Light Source is gratefully acknowledged.
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NR 34
TC 60
Z9 60
U1 25
U2 142
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD OCT 25
PY 2012
VL 116
IS 42
BP 22149
EP 22156
DI 10.1021/jp306041y
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 024PL
UT WOS:000310121000006
ER

PT J
AU Fu, YS
   Wan, YH
   Xia, H
   Wang, X
AF Fu, Yongsheng
   Wan, Yunhai
   Xia, Hui
   Wang, Xin
TI Nickel ferrite-graphene heteroarchitectures: Toward high-performance
   anode materials for lithium-ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Nickel ferrite; Graphene; Lithium-ion batteries; Heteroarchitecture
ID NEGATIVE-ELECTRODE; STORAGE; ALPHA-FE2O3
AB A NiFe2O4-graphene heteroarchitecture with differing graphene content is prepared by a straightforward hydrothermal strategy. The NiFe2O4-graphene (with 20 wt% graphene) nanocomposite as the anode material for lithium-ion batteries shows a high specific reversible capacity up to 960 mAh g(-1) with good cycling stability and rate capability. The superior electrochemical performance of the NiFe2O4-graphene nanocomposite can be attributed to its unique heteroarchitecture, which enables high utilization of active material, good structural stability and fast charge transport. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Fu, Yongsheng; Xia, Hui; Wang, Xin] Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Jiangsu, Peoples R China.
   [Wan, Yunhai; Xia, Hui] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China.
RP Wang, X (reprint author), Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Jiangsu, Peoples R China.
EM jasonxiahui@gmail.com; wxin@public1.ptt.js.cn
RI XIA, Hui/G-4533-2012; 
OI XIA, Hui/0000-0001-8730-8312; Xia, Hui/0000-0002-2517-2410
FU NNSF of China [21171094, 51102134]; DFSR [A2620110010]; PAPD of Jiangsu;
   NUST [2011PYXM03, 2011ZDJH21]; Department of Education of Jiangsu
   Province [CXZZ11_0245]
FX This investigation was supported by NNSF of China (No. 21171094,
   51102134), DFSR (No. A2620110010), PAPD of Jiangsu, NUST Research
   Funding (2011PYXM03, 2011ZDJH21) and the Department of Education of
   Jiangsu Province (CXZZ11_0245).
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NR 20
TC 60
Z9 60
U1 16
U2 127
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 1
PY 2012
VL 213
BP 338
EP 342
DI 10.1016/j.jpowsour.2012.04.039
PG 5
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 971ZR
UT WOS:000306246800040
ER

PT J
AU Xu, Y
   Yi, R
   Yuan, B
   Wu, XF
   Dunwell, M
   Lin, QL
   Fei, L
   Deng, SG
   Andersen, P
   Wang, DH
   Luo, HM
AF Xu, Yun
   Yi, Ran
   Yuan, Bin
   Wu, Xiaofei
   Dunwell, Marco
   Lin, Qianglu
   Fei, Ling
   Deng, Shuguang
   Andersen, Paul
   Wang, Donghai
   Luo, Hongmei
TI High Capacity MoO2/Graphite Oxide Composite Anode for Lithium-Ion
   Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID STORAGE CAPACITY; GRAPHENE; PERFORMANCE; INSERTION; HYBRID; CARBON;
   NANOPARTICLES; GRAPHITE; CO3O4
AB Nanostructured MoO2/graphite oxide (GO) composites are synthesized by a simple solvothermal method. X-ray diffraction and transmission electron microscopy analyses show that with the addition of GO and the increase in GO content in the precursor solutions, MoO3 rods change to MoO2 nanorods and then further to MoO2 nanoparticles, and the nanorods or nanoparticles are uniformly distributed on the surface of the GO sheets in the composites. The MoO2/GO composite with 10 wt % GO exhibits a reversible capacity of 720 mAh/g at a current density of 100 mA/g and 560 mAh/g at a high current density of 800 mA/g after 30 cycles. The improved reversible capacity, rate capacity, and cycling performance of the composites are attributed to synergistic reaction between MoO2 and GO.
C1 [Yi, Ran; Wang, Donghai] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA.
   [Xu, Yun; Yuan, Bin; Wu, Xiaofei; Dunwell, Marco; Lin, Qianglu; Fei, Ling; Deng, Shuguang; Andersen, Paul; Luo, Hongmei] New Mexico State Univ, Dept Chem Engn, Las Cruces, NM 88003 USA.
RP Wang, DH (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA.
EM dwang@psu.edu; hluo@nmsu.edu
RI Deng, Shuguang/G-5926-2011; Yi, Ran/E-1535-2012; Wang,
   Donghai/L-1150-2013
OI Deng, Shuguang/0000-0003-2892-3504; Wang, Donghai/0000-0001-7261-8510
FU New Mexico State University; New Mexico Consortium; Los Alamos National
   Laboratory; Penn State; Office of Vehicle Technologies of the U.S.
   Department of Energy [DE-AC02-05CH11231, 6951378]
FX H.L. acknowledges the funding support from New Mexico State University,
   New Mexico Consortium, and Los Alamos National Laboratory. D.W.
   acknowledges support from Penn State and the Assistant Secretary for
   Energy Efficiency and Renewable Energy, Office of Vehicle Technologies
   of the U.S. Department of Energy under contract no. DE-AC02-05CH11231,
   subcontract no. 6951378 under the Batteries for Advanced Transportation
   Technologies (BATT) Program.
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PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD FEB 2
PY 2012
VL 3
IS 3
BP 309
EP 314
DI 10.1021/jz201619r
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 886ND
UT WOS:000299860200007
PM 26285844
ER

PT J
AU Yang, XL
   Fan, KC
   Zhu, YH
   Shen, JH
   Jiang, X
   Zhao, P
   Li, CZ
AF Yang, Xiaoling
   Fan, Kaicai
   Zhu, Yihua
   Shen, Jianhua
   Jiang, Xin
   Zhao, Peng
   Li, Chunzhong
TI Tailored graphene-encapsulated mesoporous Co3O4 composite microspheres
   for high-performance lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID SOLID-LIQUID ROUTE; ANODE MATERIAL; HIGH-CAPACITY; HIGH-POWER;
   ELECTROCHEMICAL PERFORMANCE; CYCLIC PERFORMANCE; STORAGE PROPERTIES;
   METAL-OXIDES; LI; NANOPARTICLES
AB Graphene-encapsulated mesoporous Co3O4 microspheres have been successfully fabricated through a facile self-assembly approach. Driven by the mutual electrostatic interactions, the mesoporous Co3O4 microspheres prepared by a nanocasting method are fully wrapped by graphene shells. We performed the evaluation as anode materials for Li-ion batteries: the composites exhibit a first discharge capacity of 1533 mA h g(-1) and rapidly stabilize while remaining at a reversible capacity up to 820 mA h g(-1) during all the discharge-charge cycles at a current of 100 mA g(-1). The substantially improved electrochemical performance of the Co3O4-graphene composites were ascribed to the synergistic effects between the conductive graphene shells and mesoporous Co3O4 microspheres. Notably, the graphene shells not only act as buffers to accommodate the volume variation of Co3O4 but also serve as the reliable conductive channels of the electrode. In addition, the mesostructure of the mesoporous Co3O4 microspheres provides extra space for the storage of Li+ and significantly reduces paths for both Li+ ion and electron diffusion.
C1 [Yang, Xiaoling; Fan, Kaicai; Zhu, Yihua; Shen, Jianhua; Jiang, Xin; Zhao, Peng; Li, Chunzhong] E China Univ Sci & Technol, Sch Mat Sci & Engn, Minist Educ, Key Lab Ultrafine Mat, Shanghai 200237, Peoples R China.
RP Yang, XL (reprint author), E China Univ Sci & Technol, Sch Mat Sci & Engn, Minist Educ, Key Lab Ultrafine Mat, Shanghai 200237, Peoples R China.
EM yhzhu@ecust.edu.cn
RI Li, Chunzhong/B-1103-2015
OI Li, Chunzhong/0000-0001-7897-5850
FU National Natural Science Foundation of China [20925621, 20976054,
   21176083]; Special Projects for Nanotechnology of Shanghai
   [11nm0500800]; Fundamental Research Funds for the Central Universities
   [WD1013015, WD1114005]; Program for Changjiang Scholars and Innovative
   Research Team in University [IRT0825]; Shanghai Leading Academic
   Discipline Project [B502]
FX We thank the National Natural Science Foundation of China (20925621,
   20976054, and 21176083), the Special Projects for Nanotechnology of
   Shanghai (11nm0500800) the Fundamental Research Funds for the Central
   Universities (WD1013015 and WD1114005), and the Program for Changjiang
   Scholars and Innovative Research Team in University (IRT0825), and the
   Shanghai Leading Academic Discipline Project (project number: B502) for
   financial supports.
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NR 64
TC 60
Z9 61
U1 17
U2 116
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 33
BP 17278
EP 17283
DI 10.1039/c2jm32571c
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 981MR
UT WOS:000306972900082
ER

PT J
AU Huang, XD
   Zhou, XF
   Zhou, L
   Qian, K
   Wang, YH
   Liu, ZP
   Yu, CZ
AF Huang, Xiaodan
   Zhou, Xufeng
   Zhou, Liang
   Qian, Kun
   Wang, Yunhua
   Liu, Zhaoping
   Yu, Chengzhong
TI A Facile One-Step Solvothermal Synthesis of SnO2/Graphene Nanocomposite
   and Its Application as an Anode Material for Lithium-Ion Batteries
SO CHEMPHYSCHEM
LA English
DT Editorial Material
DE graphene; lithium; materials science; nanostructures; solvothermal
   synthesis
ID SNO2 NANOPARTICLES; TIN; CAPACITY; STORAGE; CARBON; ELECTRODES;
   NANOTUBES; OXIDE
C1 [Zhou, Xufeng; Liu, Zhaoping] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
   [Huang, Xiaodan; Zhou, Liang; Qian, Kun; Wang, Yunhua] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China.
   [Huang, Xiaodan; Zhou, Liang; Qian, Kun; Wang, Yunhua] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.
   [Yu, Chengzhong] Univ Queensland, AIBN, Brisbane, Qld 4072, Australia.
RP Liu, ZP (reprint author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
EM liuzp@nimte.ac.cn; c.yu@uq.edu.au
RI Zhou, Liang/K-2063-2012; Yu, Chengzhong/I-8663-2012
CR Bockstaller MR, 2005, ADV MATER, V17, P1331, DOI 10.1002/adma.200500167
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NR 28
TC 60
Z9 62
U1 9
U2 96
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1439-4235
J9 CHEMPHYSCHEM
JI ChemPhysChem
PD FEB 7
PY 2011
VL 12
IS 2
BP 278
EP 281
DI 10.1002/cphc.201000376
PG 4
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 727IQ
UT WOS:000287792300008
PM 21275019
ER

PT J
AU Zheng, FC
   Yang, Y
   Chen, QW
AF Zheng, Fangcai
   Yang, Yang
   Chen, Qianwang
TI High lithium anodic performance of highly nitrogen-doped porous carbon
   prepared from a metal-organic framework
SO NATURE COMMUNICATIONS
LA English
DT Article
ID LI-ION BATTERIES; ELECTRODE MATERIALS; RATE CAPABILITY; DIRECT
   CARBONIZATION; STORAGE PERFORMANCE; SUPERHIGH CAPACITY; NANOPOROUS
   CARBONS; GRAPHENE SHEETS; NANOFIBER WEBS; NANOTUBES
AB Theoretical and experimental results have revealed that the lithium-ion storage capacity for nitrogen-doped graphene largely depends on the nitrogen-doping level. However, most nitrogen-doped carbon materials used for lithium-ion batteries are reported to have a nitrogen content of approximately 10 wt% because a higher number of nitrogen atoms in the two-dimensional honeycomb lattice can result in structural instability. Here we report nitrogen-doped graphene particle analogues with a nitrogen content of up to 17.72 wt% that are prepared by the pyrolysis of a nitrogen-containing zeolitic imidazolate framework at 800 degrees C under a nitrogen atmosphere. As an anode material for lithium-ion batteries, these particles retain a capacity of 2,132 mA hg(-1) after 50 cycles at a current density of 100 mA g(-1), and 785 mAh g(-1) after 1,000 cycles at 5 A g(-1). The remarkable performance results from the graphene analogous particles doped with nitrogen within the hexagonal lattice and edges.
C1 [Zheng, Fangcai; Yang, Yang; Chen, Qianwang] Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
   [Zheng, Fangcai; Yang, Yang; Chen, Qianwang] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230026, Peoples R China.
   [Chen, Qianwang] Chinese Acad Sci, Hefei Inst Phys Sci, High Field Magnet Lab, Hefei 230031, Peoples R China.
RP Chen, QW (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
EM cqw@ustc.edu.cn
RI Chen, Qianwang/F-6785-2010
FU National Natural Science Foundation (NSFC) [21271163, U1232211]
FX This work was supported by the National Natural Science Foundation
   (NSFC, 21271163, U1232211). The calculations were completed on the
   supercomputing system in the Supercomputing Center of USTC. We thank H.
   Zhong for his help on the schematic illustration.
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NR 65
TC 59
Z9 59
U1 100
U2 307
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2041-1723
J9 NAT COMMUN
JI Nat. Commun.
PD NOV
PY 2014
VL 5
AR 5261
DI 10.1038/ncomms6261
PG 10
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AU6AX
UT WOS:000345685500001
PM 25374050
ER

PT J
AU Mo, RW
   Lei, ZY
   Sun, KN
   Rooney, D
AF Mo, Runwei
   Lei, Zhengyu
   Sun, Kening
   Rooney, David
TI Facile Synthesis of Anatase TiO2 Quantum- Dot/GrapheneNanosheet
   Composites with Enhanced Electrochemical Performance for Lithium-Ion
   Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE emulsion technique; TiO2 quantum dots; graphene; lithium-ion batteries
ID ANODE MATERIAL; HIGH-CAPACITY; PHOTOCATALYTIC ACTIVITY; ELECTRODE
   MATERIALS; CATHODE MATERIAL; STORAGE; NANOSHEETS; INSERTION; GRAPHITE;
   CARBON
C1 [Mo, Runwei; Lei, Zhengyu; Sun, Kening] Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, Harbin 150001, Peoples R China.
   [Rooney, David] Queens Univ Belfast, Sch Chem & Chem Engn, Belfast BT9 5AG, Antrim, North Ireland.
RP Sun, KN (reprint author), Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, Harbin 150001, Peoples R China.
EM keningsunhit@126.com; d.rooney@qub.ac.uk
RI Rooney, David/B-6035-2015
OI Rooney, David/0000-0001-5036-2497
FU National Natural Science Foundation of China [21076023]
FX This work was financially supported by National Natural Science
   Foundation of China (21076023).
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NR 46
TC 59
Z9 59
U1 66
U2 363
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD APR
PY 2014
VL 26
IS 13
BP 2084
EP 2088
DI 10.1002/adma.201304338
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AD9XA
UT WOS:000333616700016
PM 24347361
ER

PT J
AU Su, QM
   Xie, D
   Zhang, J
   Du, GH
   Xu, BS
AF Su, Qingmei
   Xie, Dong
   Zhang, Jun
   Du, Gaohui
   Xu, Bingshe
TI In Situ Transmission Electron Microscopy Observation of the Conversion
   Mechanism of Fe2O3/Graphene Anode during Lithiation-Delithiation
   Processes
SO ACS NANO
LA English
DT Article
DE metal oxide; transmission electron microscopy; lithium ion battery;
   conversion mechanism
ID LITHIUM-ION BATTERIES; STORAGE PROPERTIES; PERFORMANCE; GRAPHENE; FE2O3;
   OXIDE; NANOPARTICLES; MICROSPHERES; ALPHA-FE2O3; NANOSHEETS
AB Transition metal oxides have attracted tremendous attention as anode materials for lithium ion batteries (LIBs) recently. However, their electrochemical processes and fundamental mechanisms remain unclear. Here we report the direct observation of the dynamic behaviors and the conversion mechanism of Fe2O3/graphene in LIBs by in situ transmission electron microscopy (TEM). Upon lithiation, the Fe2O3 nanoparticles showed obvious volume expansion and morphological changes, and the surfaces of the electrode were covered by a nanocrystalline Li2O layer. Single-crystalline Fe2O3 nanoparticles were found to transform to multicrystalline nanoparticles consisting of many Fe nanograins embedded in Li2O matrix. Surprisingly, the delithiated product was not Fe2O3 but FeO, accounting for the irreversible electrochemical process and the large capacity fading of the anode material In the first cycle. The charge-discharge processes of Fe2O3 in LIBs are different from previously recognized mechanism, and are found to be a fully reversible electrochemical phase conversion between Fe and FeO nanograins accompanying the formation and disappearance of the Li2O layer. The macroscopic electrochemical performance of Fe2O3/graphene was further correlated with the microcosmic in situ TEM results.
C1 [Su, Qingmei; Xie, Dong; Zhang, Jun; Du, Gaohui] Zhejiang Normal Univ, Inst Phys Chem, Jinhua 321004, Peoples R China.
   [Su, Qingmei; Xu, Bingshe] Taiyuan Univ Technol, Coll Mat Sci & Engn, Taiyuan 030024, Shanxi, Peoples R China.
RP Du, GH (reprint author), Zhejiang Normal Univ, Inst Phys Chem, Jinhua 321004, Peoples R China.
EM gaohuidu@zjnu.edu.cn
FU Program for New Century Excellent Talents In University of Ministry of
   Education of China [NCET-11-1081]; National Science Foundation of China
   [21203168]
FX This work was supported by the Program for New Century Excellent Talents
   In University of Ministry of Education of China (NCET-11-1081) and the
   National Science Foundation of China (No. 21203168).
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NR 29
TC 59
Z9 59
U1 32
U2 176
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD OCT
PY 2013
VL 7
IS 10
BP 9115
EP 9121
DI 10.1021/nn403720p
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 242AF
UT WOS:000326209100084
PM 24015669
ER

PT J
AU Xu, CH
   Sun, J
   Gao, L
AF Xu, Chaohe
   Sun, Jing
   Gao, Lian
TI Controllable synthesis of monodisperse ultrathin SnO2 nanorods on
   nitrogen-doped graphene and its ultrahigh lithium storage properties
SO NANOSCALE
LA English
DT Article
ID ION BATTERIES; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; OXIDE PAPER;
   ELECTRODES; COMPOSITES; STABILITY; ANODE
AB Monodisperse ultrathin SnO2 nanorods on nitrogen-doped graphene were firstly synthesized by a facile one-step hydrothermal strategy. The uniformed composites with high nitrogen content and ultrathin SnO2 nanorods of 2.5-4.0 nm in diameter and 10-15 nm in length show a high reversible specific capacity, superior rate capability and outstanding cycling stability (803 mA h g(-1)) as anode materials for lithium ion batteries, owing to the synergistic effect between GS and SnO2 and nitrogen-doping, which can greatly decrease the energy barrier for Li penetrating the pyridinic defects and improve the electronic structures. This work opens the door to prepare metal oxide/GS-N composites with superior lithium storage properties and engineering of graphene composites for advanced energy storage.
C1 [Xu, Chaohe; Sun, Jing; Gao, Lian] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
RP Sun, J (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, 1295 Dingxi Rd, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn; liagao@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU National Natural Science Foundation of China [50972153, 509721157,
   51072215]; Shanghai Municipal Committee of Science and Technology
   [10DZ0505000]
FX This work is supported by the National Natural Science Foundation of
   China (Grant no. 50972153, 509721157 and 51072215) and Shanghai
   Municipal Committee of Science and Technology (Grant no. 10DZ0505000).
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NR 41
TC 59
Z9 59
U1 11
U2 103
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 17
BP 5425
EP 5430
DI 10.1039/c2nr31357j
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 987TF
UT WOS:000307439900024
PM 22832436
ER

PT J
AU Hsieh, CT
   Lin, CY
   Lin, JY
AF Hsieh, Chien-Te
   Lin, Chi-Yuan
   Lin, Jia-Yi
TI High reversibility of Li intercalation and de-intercalation in
   MnO-attached graphene anodes for Li-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene nanosheets; Manganese oxide; Lithium-ion battery; Anode; Rate
   capability
ID LITHIUM STORAGE; OXIDE; NANOPARTICLES; MANGANESE; PERFORMANCE;
   FABRICATION; ELECTRODES; NANOSHEETS; NANOTUBES; COMPOSITE
AB A composite of graphene nanosheets (GNs) supported by MnO nanocrystals has been fabricated through a simple chemical-wet impregnation followed by the thermal reduction route. The hybrid contains MnO nanoparticles with an average size of 20 nm uniformly dispersed on GNs as observed by transmission electron microscopy and X-ray diffraction analysis. The MnO-attached GN anode delivers a reversible capacity of 635 mAh/g at 0.2 C in the voltage range between 0.01 and 3.5 V. The MnO doping in the GN network plays a positive role in improving the Coulombic efficiency (92.7%) at the 1st cycle and rate capability (capacity retention (5 C/0.2 C): >70%). The superior cell performance of the GN anodes is ascribed to its unique framework, which intimately combines the conductive GNs with well-dispersed MnO nanoparticles. This present work sheds some light on the feasibility of the MnO-attached GN anodes for high-performance Li-ion batteries. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Hsieh, Chien-Te; Lin, Chi-Yuan; Lin, Jia-Yi] Yuan Ze Univ, Yuan Ze Fuel Cell Ctr, Dept Chem Engn & Mat Sci, Tao Yuan 320, Taiwan.
RP Hsieh, CT (reprint author), Yuan Ze Univ, Yuan Ze Fuel Cell Ctr, Dept Chem Engn & Mat Sci, Tao Yuan 320, Taiwan.
EM cthsieh@saturn.yzu.edu.tw
FU National Science Council of the Republic of China [NSC
   100-2120-M-155-001, NSC 100-2221-E-155-031, NSC 99-2632-E-155-001-MY3]
FX The authors are very grateful for the financial support from the
   National Science Council of the Republic of China under the contracts
   NSC 100-2120-M-155-001, NSC 100-2221-E-155-031, and NSC
   99-2632-E-155-001-MY3.
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NR 29
TC 59
Z9 63
U1 12
U2 92
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD OCT 1
PY 2011
VL 56
IS 24
BP 8861
EP 8867
DI 10.1016/j.electacta.2011.07.100
PG 7
WC Electrochemistry
SC Electrochemistry
GA 829RI
UT WOS:000295601600106
ER

PT J
AU Ren, H
   Yu, RB
   Wang, JY
   Jin, Q
   Yang, M
   Mao, D
   Kisailus, D
   Zhao, HJ
   Wang, D
AF Ren, Hao
   Yu, Ranbo
   Wang, Jiangyan
   Jin, Quan
   Yang, Mei
   Mao, Dan
   Kisailus, David
   Zhao, Huijun
   Wang, Dan
TI Muftishelled TiO2 Hollow Microspheres as Anodes with Superior Reversible
   Capacity for Lithium Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE TiO2; multishelled; hollow microsphere; lithium ion battery; anode;
   electrode
ID SENSITIZED SOLAR-CELLS; STORAGE PROPERTIES; FACILE SYNTHESIS; SPHERES;
   ANATASE; PERFORMANCE; GRAPHENE; NANOPARTICLES; NANOMATERIALS; CAPABILITY
AB Herein, uniform multishelled TiO2 hollow microspheres were synthesized, especially 3- and 4-shelled TiO2 hollow microspheres were synthesized for the first time by a simple sacrificial method capable of controlling the shell thickness, intershell spacing, and number of internal multishells, which are achieved by controlling the size, charge, and diffusion rate of the titanium coordination ions as well as the calcination process. Used as anodes for lithium ion batteries, the multishelled TiO2 hollow microspheres show excellent rate capacity, good cycling performance, and high specific capacity. A superior capacity, up to 237 mAh/g with minimal irreversible capacity after 100 cycles is achieved at a current rate of 1 C (167.5 mA/g), and a capacity of 119 mAh/g is achieved at a current rate of 10 C even after 1200 cycles.
C1 [Ren, Hao; Yu, Ranbo] Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Dept Phys Chem, Beijing 100083, Peoples R China.
   [Wang, Jiangyan; Jin, Quan; Yang, Mei; Mao, Dan; Kisailus, David; Wang, Dan] Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China.
   [Zhao, Huijun] Griffith Univ, Ctr Clean Environm & Energy, Southport, Qld 4222, Australia.
RP Yu, RB (reprint author), Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Dept Phys Chem, 30 Xueyuan Rd, Beijing 100083, Peoples R China.
EM ranboyu@ustb.edu.cn; danwang@ipe.ac.cn
RI Zhao, Huijun/H-5882-2015
OI Zhao, Huijun/0000-0002-3028-0459
FU National Natural Science Foundation of China [21031005, 21203201,
   51072020, 21271021, 51202248, 51172235, 51272165]; National Science Fund
   for Distinguished Young Scholars [21325105]; Foundation for State Key
   Laboratory of Multiphase Complex Systems [MPCS-2012-A-08, MPCS-2014-A-04
   Y425016124]
FX We are grateful for financial support from the National Natural Science
   Foundation of China (Nos. 21031005, 21203201, 51072020, 21271021,
   51202248, 21203201, 51172235, 51272165), National Science Fund for
   Distinguished Young Scholars (No. 21325105), and the Foundation for
   State Key Laboratory of Multiphase Complex Systems (No. MPCS-2012-A-08,
   No. MPCS-2014-A-04 Y425016124.J. Q.).
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NR 41
TC 58
Z9 59
U1 72
U2 252
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2014
VL 14
IS 11
BP 6679
EP 6684
DI 10.1021/nl503378a
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AU6PE
UT WOS:000345723800103
PM 25317725
ER

PT J
AU Perera, SD
   Liyanage, AD
   Nijem, N
   Ferraris, JP
   Chabal, YJ
   Balkus, KJ
AF Perera, Sanjaya D.
   Liyanage, Anjalee D.
   Nijem, Nour
   Ferraris, John P.
   Chabal, Yves J.
   Balkus, Kenneth J., Jr.
TI Vanadium oxide nanowire - Graphene binder free nanocomposite paper
   electrodes for supercapacitors: A facile green approach
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene; Binder free composite paper electrodes; Flexible electrodes;
   Supercapacitors; Vanadium oxide nanowires
ID LITHIUM ION BATTERIES; ELECTROCHEMICAL PROPERTIES; ENERGY-STORAGE;
   CARBON NANOTUBES; CATHODE MATERIAL; GRAPHITE OXIDE; COMPOSITES;
   NANOPARTICLES; REDUCTION; PERFORMANCE
AB Vanadium oxide has attracted interest for energy storage applications due to its high theoretical capacitance and stable layered structure. The low electronic conductivity, of V2O5 necessitates combining with conducting materials, typically carbon. However combining with conductive carbon materials may require binders, which compromise the active surface. In this study, V2O5 nanowire (VNWs)-graphene composite flexible paper electrodes were prepared without using binders. Graphene introduces conductivity and electric double layer capacitance (EDLC) to the composite. Graphene sheets were prepared using an alkaline deoxygenation process (hGO), which is a green alternative to traditional hydrazine reduction. Coin cell type supercapacitors were assembled using the hGO-VNW paper electrodes as the anode and spectracarb fiber cloth as the cathode in a two-electrode cell configuration. Electrochemical studies for different compositions of VNWs on hGO are reported. The composite electrode hGO-VNW120, showed balanced EDL and pseudocapacitance as well as an energy density of 38.8 Wh kg(-1) at a power density of 455 W kg(-1). The maximum power density of 3.0 kW kg(-1) was delivered at a constant current discharge rate of 5.5 A g. The device prepared using hGO-VNW120 anode showed a specific capacitance of 80 F g(-1). (C) 2012 Elsevier B.V. All rights reserved.
C1 [Perera, Sanjaya D.; Liyanage, Anjalee D.; Ferraris, John P.; Balkus, Kenneth J., Jr.] Univ Texas Dallas, Dept Chem, Richardson, TX 75080 USA.
   [Perera, Sanjaya D.; Liyanage, Anjalee D.; Ferraris, John P.; Balkus, Kenneth J., Jr.] Univ Texas Dallas, Alan G MacDiarmid Nanotech Inst, Richardson, TX 75080 USA.
   [Nijem, Nour; Chabal, Yves J.] Univ Texas Dallas, Dept Mat Sci & Engn, Lab Surface & Nanostruct Modificat, Richardson, TX 75080 USA.
RP Balkus, KJ (reprint author), Univ Texas Dallas, Dept Chem, 800 West Campbell Rd, Richardson, TX 75080 USA.
EM balkus@utdallas.edu
RI Chabal, Yves/A-5998-2011; Perera, Sanjaya/E-4542-2013
OI Chabal, Yves/0000-0002-6435-0347; 
FU Department of Energy [DE-EE004186]
FX We would like to acknowledge the Department of Energy (DE-EE004186) for
   financial support.
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NR 55
TC 58
Z9 58
U1 32
U2 463
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD MAY 15
PY 2013
VL 230
BP 130
EP 137
DI 10.1016/j.jpowsour.2012.11.118
PG 8
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 099FF
UT WOS:000315606000020
ER

PT J
AU Park, S
   Kim, S
AF Park, Sukeun
   Kim, Seok
TI Effect of carbon blacks filler addition on electrochemical behaviors of
   Co3O4/graphene nanosheets as a supercapacitor electrodes
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene nanosheets; Cobalt oxide; Carbon blacks; Supercapacitor
ID FUNCTIONALIZED GRAPHENE SHEETS; PERFORMANCE ANODE MATERIALS; LITHIUM ION
   BATTERIES; AQUEOUS DISPERSIONS; ENERGY DENSITY; STORAGE; OXIDE;
   NANOPARTICLES; COMPOSITES; CO3O4
AB A series of cobalt oxide/graphene nanocomposites have been successfully synthesized by adding carbon blacks filler. We have introduced carbon blacks to act as a structural modifier in fabricating graphene based composites. The composites were prepared by ultrasonication and microwave-assisted methods. Microstructure measurements showed that carbon blacks could be conductive links among layers of graphene and cobalt oxide particles (5-7 nm in size), which was deposited on the edge surfaces of nanosheets. This composite could function as a stable structured blocks for preventing an aggolomeration of graphene layers. The electrochemical properties are investigated by cyclic voltammetry (CV), galvanostatic charge/discharge and electrochemical impedance spectroscopy (EIS). The prepared nanocomposites showed the superior capacitive performance with good rate capability, large specific capacitance, and excellent cyclic performance. Among various samples, Co3O4/GNS-CB (15 wt.%) showed the largest specific capacitance of 341 F g(-1) at a scan rate of 10 mV s(-1) in 6 M KOH electrolyte. Therefore, the prepared composite could be potential electrode materials for supercapacitors. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Park, Sukeun; Kim, Seok] Pusan Natl Univ, Dept Chem & Biochem Engn, Pusan 609735, South Korea.
RP Kim, S (reprint author), Pusan Natl Univ, Dept Chem & Biochem Engn, San 30, Pusan 609735, South Korea.
EM seokkim@pusan.ac.kr
FU Converging Research Center Program through the Ministry of Education,
   Science and Technology [2012K001261]
FX This research was supported by the Converging Research Center Program
   through the Ministry of Education, Science and Technology (grant no.:
   2012K001261).
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NR 36
TC 58
Z9 60
U1 21
U2 218
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 1
PY 2013
VL 89
BP 516
EP 522
DI 10.1016/j.electacta.2012.11.075
PG 7
WC Electrochemistry
SC Electrochemistry
GA 098OI
UT WOS:000315558200067
ER

PT J
AU Kong, JH
   Yee, WA
   Yang, LP
   Wei, YF
   Phua, SL
   Ong, HG
   Ang, JM
   Li, X
   Lu, XH
AF Kong, Junhua
   Yee, Wu Aik
   Yang, Liping
   Wei, Yuefan
   Phua, Si Lei
   Ong, Hock Guan
   Ang, Jia Ming
   Li, Xu
   Lu, Xuehong
TI Highly electrically conductive layered carbon derived from polydopamine
   and its functions in SnO2-based lithium ion battery anodes
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID GRAPHENE; CAPACITY; MELANIN
AB Thin carbonized polydopamine (C-PDA) coatings are found to have similar structures and electrical conductivities to those of multilayered graphene doped with heteroatoms. Greatly enhanced electrochemical properties are achieved with C-PDA-coated SnO2 nanoparticles where the coating functions as a mechanical buffer layer and conducting bridge.
C1 [Kong, Junhua; Yee, Wu Aik; Yang, Liping; Phua, Si Lei; Ong, Hock Guan; Ang, Jia Ming; Lu, Xuehong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Li, Xu] ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore.
   [Wei, Yuefan] Nanyang Technol Univ, Sch Mech & Aerosp Engn, Singapore 639798, Singapore.
RP Lu, XH (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM ASXHLu@ntu.edu.sg
RI Yang, Liping/F-6081-2011; Lu, Xuehong/A-2232-2011
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NR 21
TC 58
Z9 58
U1 21
U2 192
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
J9 CHEM COMMUN
JI Chem. Commun.
PY 2012
VL 48
IS 83
BP 10316
EP 10318
DI 10.1039/c2cc35284b
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 010XU
UT WOS:000309128600014
PM 22983398
ER

PT J
AU Zhou, JS
   Ma, LL
   Song, HH
   Wu, B
   Chen, XH
AF Zhou, Jisheng
   Ma, Lulu
   Song, Huaihe
   Wu, Bin
   Chen, Xiaohong
TI Durable high-rate performance of CuO hollow
   nanoparticles/graphene-nanosheet composite anode material for
   lithium-ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Copper oxide; Hollow nanoparticles; Graphene; Anode; Lithium-ion
   batteries
ID ELECTRODE MATERIALS; NANOTUBES; OXIDATION; METAL
AB Copper oxide hollow nanoparticles/graphene-nanosheet composites are prepared using the Kirkendall-effect approach. The composites exhibit a durable lifetime cycle at high rates. The reversible capacity of the material attains 640 mAhg(-1) at 50 mAg(-1) and the capacity retention is ca. 96% when the current density is increased 10 times. At 1 Ag(-1) (ca. 1.7 C), the reversible capacity reaches 485 mAhg(-1) and remains at 281 mAhr(-1) after 500 cycles, indicating that the capacity fading is less than 0.4 mAhg(-1) per cycle. This excellent electrochemical performance can be attributed to the hollow interior of CuO nanoparticles as well as synergistic effect between CuO and graphene. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Zhou, Jisheng; Ma, Lulu; Song, Huaihe; Wu, Bin; Chen, Xiaohong] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Key Lab Carbon Fiber & Funct Polymers, Minist Educ, Beijing 100029, Peoples R China.
   [Ma, Lulu] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
RP Song, HH (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Key Lab Carbon Fiber & Funct Polymers, Minist Educ, Beijing 100029, Peoples R China.
EM songhh@mail.buct.edu.cn
FU National Natural Science Foundation of China [50572003, 50972004];
   Xinjiang Key Laboratory of Electronic Information Materials and Devices
   [XJYS0901-2010-03]; Foundation of Excellent Doctoral Dissertation of
   Beijing City [YB20081001001]
FX This work was supported by the National Natural Science Foundation of
   China (50572003 and 50972004), the Opening Project of Xinjiang Key
   Laboratory of Electronic Information Materials and Devices
   (XJYS0901-2010-03), and the Foundation of Excellent Doctoral
   Dissertation of Beijing City (YB20081001001).
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NR 24
TC 58
Z9 60
U1 9
U2 114
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD DEC
PY 2011
VL 13
IS 12
BP 1357
EP 1360
DI 10.1016/j.elecom.2011.08.011
PG 4
WC Electrochemistry
SC Electrochemistry
GA 874FM
UT WOS:000298940800018
ER

PT J
AU Guan, Q
   Cheng, JL
   Wang, B
   Ni, W
   Gu, GF
   Li, XD
   Huang, L
   Yang, GC
   Nie, FD
AF Guan, Qun
   Cheng, Jianli
   Wang, Bin
   Ni, Wei
   Gu, Guifang
   Li, Xiaodong
   Huang, Ling
   Yang, Guangcheng
   Nie, Fude
TI Needle-like Co3O4 Anchored on the Graphene with Enhanced Electrochemical
   Performance for Aqueous Supercapacitors
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE needle-like Co3O4; graphene; aqueous supercapacitor; electrochemical
   performance; needle-like CoO; urchin-like spheres
ID LITHIUM-ION BATTERIES; OXYGEN REDUCTION REACTION; GREEN SYNTHESIS;
   GRAPHITE OXIDE; ANODE MATERIAL; ONE-POT; FACILE; NANOCOMPOSITE;
   COMPOSITES; NANOSHEETS
AB We synthesized the needle-like cobalt oxide/graphene composites with different mass ratios, which are composed of cobalt oxide (Co3O4 or CoO) needle homogeneously anchored on graphene nanosheets as the template, by a facile hydrothermal method. Without the graphene as the template, the cobalt precursor tends to group into urchin-like spheres formed by many fine needles. When used as electrode materials of aqueous supercapacitor, the composites of the needle-like Co3O4/graphene (the mass ratio of graphene oxide(GO) and Co(NO3)(2)center dot 6H(2)O is 1:5) exhibit a high specific capacitance of 157.7 F g(-1) at a current density of 0.1 A g(-1) in 2 mol L-1 KOH aqueous solution as well as good rate capability. Meanwhile, the capacitance retention keeps about 70% of the initial value after 4000 cycles at a current density of 0.2 A g(-1). The enhancement of excellent electrochemical performances may be attributed to the synergistic effect of graphene and cobalt oxide components in the unique multiscale structure of the composites.
C1 [Guan, Qun] Southwest Univ Sci & Technol, Mianyang 643000, Peoples R China.
   [Guan, Qun; Cheng, Jianli; Wang, Bin; Ni, Wei; Gu, Guifang; Li, Xiaodong; Huang, Ling; Yang, Guangcheng; Nie, Fude] China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Peoples R China.
   [Guan, Qun; Cheng, Jianli; Wang, Bin; Ni, Wei; Gu, Guifang; Li, Xiaodong; Huang, Ling; Yang, Guangcheng; Nie, Fude] New Mat Ctr Sichuan Prov, Mianyang 621900, Peoples R China.
RP Wang, B (reprint author), China Acad Engn Phys, Inst Chem Mat, Mianyang 621900, Peoples R China.
EM edward.bwang@gmail.com; niefude@caep.ac.cn
RI Ni, Wei/N-7319-2013; cheng, Jianli/K-1496-2014
OI Ni, Wei/0000-0003-0965-2470; 
FU Startup Foundation of China Academy of Engineering Physics, Institute of
   Chemical Materials [KJCX201301, KJCX201306]; National High-tech Research
   and Development Program (863 Program) [2013AA050905]
FX This work was supported by the Startup Foundation of China Academy of
   Engineering Physics, Institute of Chemical Materials (KJCX201301 and
   KJCX201306) and National High-tech Research and Development Program (863
   Program: No. 2013AA050905).
CR Sun YQ, 2011, ENERG ENVIRON SCI, V4, P1113, DOI 10.1039/c0ee00683a
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NR 39
TC 57
Z9 57
U1 47
U2 267
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY 28
PY 2014
VL 6
IS 10
BP 7626
EP 7632
DI 10.1021/am5009369
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA AI1TZ
UT WOS:000336639200078
PM 24716615
ER

PT J
AU Ge, MY
   Rong, JP
   Fang, X
   Zhang, AY
   Lu, YH
   Zhou, CW
AF Ge, Mingyuan
   Rong, Jiepeng
   Fang, Xin
   Zhang, Anyi
   Lu, Yunhao
   Zhou, Chongwu
TI Scalable preparation of porous silicon nanoparticles and their
   application for lithium-ion battery anodes
SO NANO RESEARCH
LA English
DT Article
DE porous silicon nanoparticles; scalable production; lithium-ion battery
ID LONG CYCLE LIFE; NANOWIRES; PERFORMANCE; PARTICLES
AB Nanostructured silicon has generated significant excitement for use as the anode material for lithium-ion batteries; however, more effort is needed to produce nanostructured silicon in a scalable fashion and with good performance. Here, we present a direct preparation of porous silicon nanoparticles as a new kind of nanostructured silicon using a novel two-step approach combining controlled boron doping and facile electroless etching. The porous silicon nanoparticles have been successfully used as high performance lithium-ion battery anodes, with capacities around 1,400 mA center dot h/g achieved at a current rate of 1 A/g, and 1,000 mA center dot h/g achieved at 2 A/g, and stable operation when combined with reduced graphene oxide and tested over up to 200 cycles. We attribute the overall good performance to the combination of porous silicon that can accommodate large volume change during cycling and provide large surface area accessible to electrolyte, and reduced graphene oxide that can serve as an elastic and electrically conductive matrix for the porous silicon nanoparticles.
C1 [Ge, Mingyuan; Rong, Jiepeng; Fang, Xin; Zhang, Anyi; Zhou, Chongwu] Univ So Calif, Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA.
   [Lu, Yunhao] Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
   [Zhou, Chongwu] Univ So Calif, Dept Elect Engn, Los Angeles, CA 90089 USA.
RP Zhou, CW (reprint author), Univ So Calif, Dept Chem Engn & Mat Sci, 3710 McClintock Ave, Los Angeles, CA 90089 USA.
EM chongwuz@usc.edu
RI Zhou, Chongwu/F-7483-2010; Rong, Jiepeng/B-3624-2015; Fang,
   Xin/P-8002-2015
FU University of Southern California; High-Performance Computing and
   Communications at University of Southern California
FX This work was supported by University of Southern California. This work
   was also supported by High-Performance Computing and Communications at
   University of Southern California.
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PI BEIJING
PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA
SN 1998-0124
J9 NANO RES
JI Nano Res.
PD MAR
PY 2013
VL 6
IS 3
BP 174
EP 181
DI 10.1007/s12274-013-0293-y
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 105QR
UT WOS:000316087300003
ER

PT J
AU Hu, CG
   Xiao, Y
   Zhao, Y
   Chen, N
   Zhang, ZP
   Cao, MH
   Qu, LT
AF Hu, Chuangang
   Xiao, Ying
   Zhao, Yang
   Chen, Nan
   Zhang, Zhipan
   Cao, Minhua
   Qu, Liangti
TI Highly nitrogen-doped carbon capsules: scalable preparation and
   high-performance applications in fuel cells and lithium ion batteries
SO NANOSCALE
LA English
DT Article
ID OXYGEN REDUCTION REACTION; ANODE MATERIALS; ELECTROCHEMICAL PROPERTIES;
   GRAPHENE NANORIBBONS; FUNCTIONAL-GROUPS; RATE CAPABILITY; ELECTRODES;
   CATALYSTS; ELECTROCATALYSIS; NANOSPHERES
AB Highly nitrogen-doped carbon capsules (hN-CCs) have been successfully prepared by using inexpensive melamine and glyoxal as precursors via solvothermal reaction and carbonization. With a great promise for large scale production, the hN-CCs, having large surface area and high-level nitrogen content (N/C atomic ration of ca. 13%), possess superior crossover resistance, selective activity and catalytic stability towards oxygen reduction reaction for fuel cells in alkaline medium. As a new anode material in lithium-ion battery, hN-CCs also exhibit excellent cycle performance and high rate capacity with a reversible capacity of as high as 1046 mA h g(-1) at a current density of 50 mA g(-1) after 50 cycles. These features make the hN-CCs developed in this study promising as suitable substitutes for the expensive noble metal catalysts in the next generation alkaline fuel cells, and as advanced electrode materials in lithium-ion batteries.
C1 [Hu, Chuangang; Xiao, Ying; Zhao, Yang; Chen, Nan; Zhang, Zhipan; Cao, Minhua; Qu, Liangti] Beijing Inst Technol, Minist Educ China, Key Lab Cluster Sci, Beijing 100081, Peoples R China.
RP Qu, LT (reprint author), Beijing Inst Technol, Minist Educ China, Key Lab Cluster Sci, Beijing 100081, Peoples R China.
EM lqu@bit.edu.cn
FU National Basic Research Program of China [2011CB013000]; NSFC [21004006,
   21174019, 51161120361]; Fok Ying Tong Education Foundation [131043]; 111
   Project [B07012];  [NCET-10-0047]
FX This project is sponsored by National Basic Research Program of China
   (2011CB013000), NSFC (no. 21004006, 21174019, 51161120361), Fok Ying
   Tong Education Foundation (no. 131043), the 111 Project B07012, and
   NCET-10-0047. We also thank Engineer Yuting Zuo of General Research
   Institute for Nonferrous Metals for the SEM work.
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NR 56
TC 57
Z9 57
U1 20
U2 143
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 7
BP 2726
EP 2733
DI 10.1039/c3nr34002c
PG 8
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 106CV
UT WOS:000316120100024
PM 23426378
ER

PT J
AU Hu, T
   Sun, X
   Sun, HT
   Yu, MP
   Lu, FY
   Liu, CS
   Lian, J
AF Hu, Tao
   Sun, Xiang
   Sun, Hongtao
   Yu, Mingpeng
   Lu, Fengyuan
   Liu, Changsheng
   Lian, Jie
TI Flexible free-standing graphene-TiO2 hybrid paper for use as lithium ion
   battery anode materials
SO CARBON
LA English
DT Article
ID STORAGE; PERFORMANCE; OXIDE; NANOSHEETS; ELECTRODES
AB Flexible and binder-free graphene-TiO2 paper was prepared by a simple route. A unique 3-D nano-structure was achieved with nano-sized TiO2 intercalated between graphene layers as pillars, significantly increasing the Li-ion insertion/extraction rate. At a current rate of 2 Ag-1, the specific capacity can reach 122 mAhg(-1) after 100 charge/discharge cycles. More remarkably, the flexible graphene/TiO2 hybrid paper shows an excellent stability when the rates decrease from 4 Ag-1 back to 200 mAg(-1) with the retained capacity of 175 mAhg(-1). (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Hu, Tao; Sun, Xiang; Sun, Hongtao; Yu, Mingpeng; Lu, Fengyuan; Lian, Jie] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
   [Hu, Tao; Liu, Changsheng] Northeastern Univ, Minist Educ, Key Lab Anisotropy & Texture Mat, Shenyang 110004, Liaoning, Peoples R China.
RP Lian, J (reprint author), Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
EM lianj@rpi.edu
RI Lu, Fengyuan/A-2875-2011; Hu, Tao/J-8779-2013; Sun, Hongtao/N-6597-2013
OI Lu, Fengyuan/0000-0003-1912-2713; Sun, Hongtao/0000-0003-3259-6091
FU NSF [DMR 1151028]; China Scholarship Council; Fundamental Research Funds
   for the Central Universities [N100702001]
FX This work was supported by a NSF career award under the Award number of
   DMR 1151028. T. Hu and C. Liu also acknowledge the State Scholarship
   Fund of the China Scholarship Council and the Fundamental Research Funds
   for the Central Universities (N100702001).
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PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD JAN
PY 2013
VL 51
BP 322
EP 326
DI 10.1016/j.carbon.2012.08.059
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 036CZ
UT WOS:000311005300036
ER

PT J
AU Wang, G
   Liu, T
   Luo, YJ
   Zhao, Y
   Ren, ZY
   Bai, JB
   Wang, H
AF Wang, Gang
   Liu, Ting
   Luo, Yongjun
   Zhao, Yan
   Ren, Zhaoyu
   Bai, Jinbo
   Wang, Hui
TI Preparation of Fe2O3/graphene composite and its electrochemical
   performance as an anode material for lithium ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Iron oxide; Graphene nanosheets; Anode material; Lithium ion batteries
ID CAPACITY; INTERCALATION; ELECTRODE; HYBRID; CARBON; NANOCOMPOSITE;
   STABILITY; INSERTION
AB The micro-sized sphere Fe2O3 particles doped with graphene nanosheets were prepared by a facile hydrothermal method. The obtained Fe2O3/graphene composite as the anode material for lithium ion batteries showed a high discharge capacity of 660 mAh g(-1) during up to 100 cycles at the current density of 160 mA g(-1) and good rate capability. The excellent electrochemical performance of the composite can be attributed to that graphene served as dispersing medium to prevent Fe2O3 microparticles from agglomeration and provide an excellent electronic conduction pathway. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Wang, Gang; Liu, Ting; Luo, Yongjun; Wang, Hui] NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
   [Zhao, Yan; Ren, Zhaoyu] NW Univ Xian, Natl Key Lab Photoelect Technol & Funct Mat, Natl Photoelect Technol & Funct Mat & Applicat In, Inst Photon & Photon Technol,Culture Base, Xian 710069, Peoples R China.
   [Bai, Jinbo] Ecole Cent Paris, Lab MSS MAT, CNRS UMR 8579, F-92295 Chatenay Malabry, France.
RP Wang, H (reprint author), NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
EM huiwang@nwu.edu.cn
RI Bai, Jinbo/F-8552-2010
FU National Natural Science Foundation of China [21061130551, 20873099,
   10974152]; National Basic Research Program of China (973 Program)
   [2009CB626611]; Ph. D. Programs Foundation of Ministry of Education of
   China [20096101110002]; NWU [09YYB04]; National Innovation Experiment
   Program For University Students [091069710]
FX The project was supported by the financial supports of the International
   cooperation research program of National Natural Science Foundation of
   China (No. 21061130551), the National Basic Research Program of China
   (973 Program) (No. 2009CB626611), the Ph. D. Programs Foundation of
   Ministry of Education of China (No. 20096101110002), the National
   Natural Science Foundation of China (Nos. 20873099 and 10974152), NWU
   Doctorate Dissertation of Excellence Funds (No. 09YYB04), and National
   Innovation Experiment Program For University Students (091069710).
CR Wang SQ, 2010, J POWER SOURCES, V195, P5379, DOI 10.1016/j.jpowsour.2010.03.035
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   Stoller MD, 2008, NANO LETT, V8, P3498, DOI 10.1021/nl802558y
   Chen LB, 2009, ELECTROCHIM ACTA, V54, P4198, DOI 10.1016/j.electacta.2009.02.065
   Lafont U, 2010, J PHYS CHEM C, V114, P1372, DOI 10.1021/jp908786t
   Zhan SY, 2010, J ALLOY COMPD, V502, P92, DOI 10.1016/j.jallcom.2010.03.133
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   Cai CA, 2011, J ALLOY COMPD, V509, P909, DOI 10.1016/j.jallcom.2010.09.129
   Hang BT, 2008, J POWER SOURCES, V178, P402, DOI 10.1016/j.jpowsour.2007.12.001
   Kim YJ, 2011, J ALLOY COMPD, V509, P4367, DOI 10.1016/j.jallcom.2011.01.061
   NuLi YN, 2008, ELECTROCHIM ACTA, V53, P4213, DOI DOI 10.1016/J.ELECTACTA.2007.12.067
   Wu FX, 2011, J ALLOY COMPD, V509, P3711, DOI 10.1016/j.jallcom.2010.12.182
   Zhang YH, 2009, NANOTECHNOLOGY, V20, DOI 10.1088/0957-4484/20/18/185504
   Zhou ZB, 2010, J ALLOY COMPD, V507, P309, DOI 10.1016/j.jallcom.2010.07.188
NR 34
TC 57
Z9 57
U1 14
U2 118
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD JUN 16
PY 2011
VL 509
IS 24
BP L216
EP L220
DI 10.1016/j.jallcom.2011.03.151
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 766OF
UT WOS:000290793000002
ER

PT J
AU Liang, RL
   Cao, HQ
   Qian, D
   Zhang, JX
   Qu, MZ
AF Liang, Renlong
   Cao, Huaqiang
   Qian, Dong
   Zhang, Jingxian
   Qu, Meizhen
TI Designed synthesis of SnO2-polyaniline-reduced graphene oxide
   nanocomposites as an anode material for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID RAMAN-SCATTERING; FACILE SYNTHESIS; NANOPARTICLES; NANOWIRES; STORAGE;
   ELECTRODES; NANOSHEETS; COMPOSITE
AB Three dimensional SnO2-based nanocomposites, i.e., SnO2 nanoparticles anchored on polyaniline nanoplates@reduced graphene oxide nanosheets (SPG) via pi-pi stacking, present excellent cyclability and high capacity with a reversible storage capacity of 573.6 mA h g(-1) accompanied by coulombic efficiency of 99.26% over 50 cycles when used as an anode in a lithium ion battery.
C1 [Liang, Renlong; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Liang, Renlong; Qian, Dong] Cent S Univ, Coll Chem & Chem Engn, Changsha 410083, Peoples R China.
   [Zhang, Jingxian; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn; qiandong6@vip.sina.com
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]
FX The authors gratefully acknowledge financial support from the National
   Natural Science Foundation of China (No. 20921001 and 20535020), the
   Innovation Method Fund of China (No. 20081885189), the National High
   Technology Research and Development Program of China (No. 2009AA03Z321).
CR Elias DC, 2009, SCIENCE, V323, P610, DOI 10.1126/science.1167130
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NR 38
TC 57
Z9 57
U1 17
U2 85
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2011
VL 21
IS 44
BP 17654
EP 17657
DI 10.1039/c1jm13934g
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 839SX
UT WOS:000296390600018
ER

PT J
AU Wu, YP
   Jiang, C
   Wan, C
   Holze, R
AF Wu, YP
   Jiang, C
   Wan, C
   Holze, R
TI Modified natural graphite as anode material for lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE lithium ion batteries; natural graphite; nitric acid; anode material
ID INITIAL IRREVERSIBLE CAPACITY; ELECTROCHEMICAL PERFORMANCE; SURFACE
   MODIFICATION; SECONDARY BATTERIES; NEGATIVE ELECTRODE; CARBON;
   OXIDATION; COMPOSITE; COKE
AB A concentrated nitric acid solution was used as an oxidant to modify the electrochemical performance of natural graphite as anode material for lithium ion batteries. Results of X-ray photoelectron spectroscopy, electron paramagnetic resonance, thermogravimmetry, differential thermal analysis, high resolution electron microscopy, and measurement of the reversible capacity suggest that the surface structure of natural graphite was changed, a fresh dense layer of oxides was formed. Some structural imperfections were removed, and the stability of the graphite structure increased. These changes impede decomposition of electrolyte solvent molecules, co-intercalation of solvated lithium ions and movement of graphene planes along the a-axis direction. Concomitantly, more micropores were introduced, and thus, lithium intercalation and deintercalation were favored and more sites were provided for lithium storage. Consequently, the reversible capacity and the cycling behavior of the modified natural graphite were much improved by the oxidation. Obviously, the liquid-solid oxidation is advantageous in controlling the uniformity of the products. (C) 2002 Elsevier Science B.V. All rights reserved.
C1 Tsing Hua Univ, Div Chem Engn, INET, Beijing 102201, Peoples R China.
   Tech Univ Chemnitz, Inst Chem, AG Elektrochem, D-09107 Chemnitz, Germany.
RP Wu, YP (reprint author), Tsing Hua Univ, Div Chem Engn, INET, Beijing 102201, Peoples R China.
RI Wu, Yuping/H-1593-2011
OI Wu, Yuping/0000-0002-0833-1205
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NR 34
TC 57
Z9 61
U1 1
U2 28
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 23
PY 2002
VL 111
IS 2
BP 329
EP 334
AR PII S0378-7753(02)00349-X
DI 10.1016/S0378-7753(02)00349-X
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 600MA
UT WOS:000178393300013
ER

PT J
AU Shiva, K
   Matte, HSSR
   Rajendra, HB
   Bhattacharyya, AJ
   Rao, CNR
AF Shiva, Konda
   Matte, H. S. S. Ramakrishna
   Rajendra, H. B.
   Bhattacharyya, Aninda J.
   Rao, C. N. R.
TI Employing synergistic interactions between few-layer WS2 and reduced
   graphene oxide to improve lithium storage, cyclability and rate
   capability of Li-ion batteries
SO NANO ENERGY
LA English
DT Article
DE Chalcogenides; Reduced graphene oxide; Lithium-ion batteries;
   Cyclability and rate capability; Percolation
ID TUNGSTEN DISULFIDE; ANODE MATERIAL; MOS2; CARBON; NANOTUBES;
   NANOPARTICLES; PERFORMANCE; DESIGN
AB The aim of the contribution is to introduce a high performance anode alternative to graphite for lithium-ion batteries (LiBs). A simple process was employed to synthesize uniform graphene-like few-layer tungsten sulfide (WS2) supported on reduced graphene oxide (RGO) through a hydrothermal synthesis route. The WS2-RGO (80:20 and 70:30) composites exhibited good enhanced electrochemical performance and excellent rate capability performance when used as anode materials for lithium-ion batteries. The specific capacity of the WS2-RGO composite delivered a capacity of 400-450 mAh g(-1) after 50 cycles when cycled at a current density of 100 mA g(-1). At 4000 mA g(-1), the composites showed a stable capacity of approximately 180-240 mAh g(-1), respectively. The noteworthy electrochemical performance of the composite is not additive, rather it is synergistic in the sense that the electrochemical performance is much superior compared to both WS2 and RGO. As the observed lithiation/delithiation for WS2-RGO is at a voltage 1.0 V (approximate to 0.1 V for graphite, Li* /Li), the lithium-ion battery with WS2-RGO is expected to possess high interface stability, safety and management of electrical energy is expected to be more efficient and economic. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Shiva, Konda; Rajendra, H. B.; Bhattacharyya, Aninda J.; Rao, C. N. R.] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India.
   [Matte, H. S. S. Ramakrishna; Rao, C. N. R.] Jawaharlal Nehru Ctr Adv Sci Res, Chem & Phys Mat Unit, Bangalore 560064, Karnataka, India.
RP Bhattacharyya, AJ (reprint author), Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India.
EM aninda_jb@sscu.iisc.ernet.in
RI Matte, Krishna/F-1790-2011; Ahirwal, Ashish /F-2532-2013; Bhattacharyya,
   Aninda/P-3744-2015
OI Matte, Krishna/0000-0001-8279-8447; Ahirwal, Ashish
   /0000-0002-9127-6541; Bhattacharyya, Aninda/0000-0002-0736-0004
FU SSCU; IISc; CSIR; Department of Science and Technology (DST)-Nano
   Mission; Ministry of Communication and Information Technology (MCIT,
   Centre of Excellence in Nanoelectronics, Phase II grant) of Government
   of India
FX The authors thank for JNCASR for TEM and Raman spectroscopy facilities.
   Konda Shiva acknowledges SSCU, IISc, CSIR for SRF. AJB thanks Department
   of Science and Technology (DST)-Nano Mission and Ministry of
   Communication and Information Technology (MCIT, Centre of Excellence in
   Nanoelectronics, Phase II grant) of Government of India for financial
   support.
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NR 27
TC 56
Z9 56
U1 53
U2 275
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD SEP
PY 2013
VL 2
IS 5
BP 787
EP 793
DI 10.1016/j.nanoen.2013.02.001
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 240YS
UT WOS:000326134200025
ER

PT J
AU Su, DW
   Kim, HS
   Kim, WS
   Wang, GX
AF Su, Dawei
   Kim, Hyun-Soo
   Kim, Woo-Seong
   Wang, Guoxiu
TI Mesoporous Nickel Oxide Nanowires: Hydrothermal Synthesis,
   Characterisation and Applications for Lithium-Ion Batteries and
   Supercapacitors with Superior Performance
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE hydrothermal synthesis; lithium-ion batteries; mesoporous materials;
   nanostructures; nickel oxide
ID HIGH-POWER; ELECTROCHEMICAL PROPERTIES; GRAPHENE NANOSHEETS; ELECTRODE
   MATERIALS; STORAGE PROPERTIES; CATHODE MATERIALS; HIGH-CAPACITY; LI
   STORAGE; CO3O4; NANOCOMPOSITE
AB Mesoporous nickel oxide nanowires were synthesized by a hydrothermal reaction and subsequent annealing at 400?degrees C. The porous one-dimensional nanostructures were analysed by field-emission SEM, high-resolution TEM and N2 adsorption/desorption isotherm measurements. When applied as the anode material in lithium-ion batteries, the as-prepared mesoporous nickel oxide nanowires demonstrated outstanding electrochemical performance with high lithium storage capacity, satisfactory cyclability and an excellent rate capacity. They also exhibited a high specific capacitance of 348 F?g-1 as electrodes in supercapacitors.
C1 [Su, Dawei; Wang, Guoxiu] Univ Technol Sydney, Ctr Clean Energy Technol, Sch Chem & Forens Sci, Sydney, NSW 2007, Australia.
   [Kim, Hyun-Soo] Korea Electrotechnol Res Inst, Battery Res Ctr, Chang Won 641120, South Korea.
   [Kim, Woo-Seong] Daejung Energy Mat Co Ltd, Inchon 405820, South Korea.
RP Wang, GX (reprint author), Univ Technol Sydney, Ctr Clean Energy Technol, Sch Chem & Forens Sci, Sydney, NSW 2007, Australia.
EM Guoxiu.Wang@uts.edu.au
FU Australian Research Council (ARC) through the ARC Discovery Project
   [DP0772999]; ARC Linkage project [LP0989134]
FX We acknowledge the Australian Research Council (ARC) for financial
   support through the ARC Discovery Project (DP0772999) and the ARC
   Linkage project (LP0989134).
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NR 47
TC 56
Z9 57
U1 10
U2 101
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD JUN
PY 2012
VL 18
IS 26
BP 8224
EP 8229
DI 10.1002/chem.201200086
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 960LC
UT WOS:000305388300033
PM 22589171
ER

PT J
AU Liu, HD
   Huang, JM
   Li, XL
   Liu, J
   Zhang, YX
   Du, K
AF Liu, Hongdong
   Huang, Jiamu
   Li, Xinlu
   Liu, Jia
   Zhang, Yuxin
   Du, Kun
TI Flower-like SnO2/graphene composite for high-capacity lithium storage
SO APPLIED SURFACE SCIENCE
LA English
DT Article
DE Flower-like SnO2; Graphene; Lithium-ion batteries; Anode
ID ION BATTERIES; ANODE MATERIAL; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE;
   GRAPHENE OXIDE; ELECTRODE; SILICON; SNO2; NANOCOMPOSITE; STABILITY
AB Flower-like SnO2/graphene composite is synthesized by a simple hydrothermal method for high-capacity lithium storage. The as-prepared products are characterized by XRD, FTIR, FESEM, TGA and Nitrogen adsorption/desorption. The electrochemical performance of the flower-like SnO2/graphene composite is measured by cyclic voltammetry and galvanostatic charge/discharge cycling. The results show that the flower-like SnO2 nanorod clusters are 800 nm in size and homogeneously adhere on graphene sheets. The flower-like SnO2/graphene composite displays superior Li-battery performance with large reversible capacity, excellent cyclic performance and good rate capability. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Liu, Hongdong; Huang, Jiamu; Li, Xinlu; Liu, Jia; Zhang, Yuxin; Du, Kun] Chongqing Univ, Coll Mat Sci & Engn, Chongqing 400045, Peoples R China.
RP Huang, JM (reprint author), Chongqing Univ, Coll Mat Sci & Engn, Chongqing 400045, Peoples R China.
EM huangjiamu@cqu.edu.cn; lixinlu@cqu.edu.cn
RI Zhang, Yu Xin/D-1524-2009
OI Zhang, Yu Xin/0000-0003-4698-5645
FU Fundamental Research Funds for the Central Universities [CDJXS10 13 11
   58]
FX This work was supported by Fundamental Research Funds for the Central
   Universities (no. CDJXS10 13 11 58).
CR Liu NA, 2011, ACS NANO, V5, P6487, DOI 10.1021/nn2017167
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NR 37
TC 56
Z9 58
U1 18
U2 136
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0169-4332
J9 APPL SURF SCI
JI Appl. Surf. Sci.
PD MAR 15
PY 2012
VL 258
IS 11
BP 4917
EP 4921
DI 10.1016/j.apsusc.2012.01.119
PG 5
WC Chemistry, Physical; Materials Science, Coatings & Films; Physics,
   Applied; Physics, Condensed Matter
SC Chemistry; Materials Science; Physics
GA 901UG
UT WOS:000300992300016
ER

PT J
AU Latorre-Sanchez, M
   Atienzar, P
   Abellan, G
   Puche, M
   Fornes, V
   Ribera, A
   Garcia, H
AF Latorre-Sanchez, Marcos
   Atienzar, Pedro
   Abellan, Gonzalo
   Puche, Marta
   Fornes, Vicente
   Ribera, Antonio
   Garcia, Hermenegildo
TI The synthesis of a hybrid graphene-nickel/manganese mixed oxide and its
   performance in lithium-ion batteries
SO CARBON
LA English
DT Article
ID LAYERED DOUBLE HYDROXIDE; CAPACITY ANODE MATERIAL; SECONDARY BATTERY;
   CARBON MATERIALS; CONVERSION
AB Mixing of aqueous suspensions of delaminated NiMn layered double hydroxide (LDH) and graphene oxide leads to the instantaneous precipitation of a hybrid material that after calcination under inert atmosphere at 450 degrees C leads to Ni6MnO8 nanoparticles deposited on larger reconstituted graphene sheets. This material exhibits electrical conductivity similar to graphite, superparamagnetism and can be used as an anode for Li-ion batteries. A maximum capacity value of 1030 mAh g(-1) was found during the first discharge, and capacity values higher than 400 mAh g(-1) were still achieved after 10 cycles. The methodology used here should allow the preparation of a large variety of hybrid graphene-metal oxide materials starting from other LDHs in which the properties derived from both constituents coexist. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Latorre-Sanchez, Marcos; Atienzar, Pedro; Puche, Marta; Fornes, Vicente; Garcia, Hermenegildo] Univ Politecn Valencia, Inst Tecnol Quim, CSIC, Valencia 46022, Spain.
   [Abellan, Gonzalo; Ribera, Antonio] Univ Valencia, Inst Ciencia Mol, Valencia 46980, Spain.
RP Garcia, H (reprint author), Univ Politecn Valencia, Inst Tecnol Quim, CSIC, Ave Naranjos S-N, Valencia 46022, Spain.
EM hgarcia@qim.upv.es
RI Garcia, Hermenegildo/E-3296-2010; Ribera, Antonio/D-5583-2013; Atienzar,
   Pedro/A-2998-2009; Abellan, Gonzalo/B-3451-2013
OI Garcia, Hermenegildo/0000-0002-9664-493X; Ribera,
   Antonio/0000-0001-6314-7438; Atienzar, Pedro/0000-0002-0356-021X;
   Abellan, Gonzalo/0000-0003-1564-6210
FU EU; Spanish MCINN with FEDER [CSD2007-00010, CTQ-2008-06720, CTQ
   2009-15896]; Generalitat Valenciana; Spanish ministry of Education; Juan
   de la Cierva
FX This work has been supported by the EU (ERC SPINMOL Advanced Grant), the
   Spanish MCINN with FEDER cofinancing (Project Consolider-Ingenio in
   Molecular Nanoscience CSD2007-00010, CTQ-2008-06720, and CTQ 2009-15896)
   and the Generalitat Valenciana (PROMETEO program). ML and PA thank the
   Spanish ministry of Education for a postgraduate scholarship and a Juan
   de la Cierva research contract, respectively.
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NR 33
TC 56
Z9 57
U1 16
U2 169
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD FEB
PY 2012
VL 50
IS 2
BP 518
EP 525
DI 10.1016/j.carbon.2011.09.007
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 853AD
UT WOS:000297397700020
ER

PT J
AU Hou, JH
   Cao, CB
   Idrees, F
   Ma, XL
AF Hou, Jianhua
   Cao, Chuanbao
   Idrees, Faryal
   Ma, Xilan
TI Hierarchical Porous Nitrogen-Doped Carbon Nanosheets Derived from Silk
   for Ultrahigh-Capacity Battery Anodes and Supercapacitors
SO ACS NANO
LA English
DT Article
DE Li-ion battery; supercapacitors; hierarchical porous; nitrogen-doped;
   carbon nanosheets
ID LITHIUM-ION BATTERIES; HIGH-PERFORMANCE ANODE; ELECTROCHEMICAL
   ENERGY-STORAGE; OXYGEN REDUCTION REACTION; MESOPOROUS CARBON; DENSITY
   SUPERCAPACITORS; GRAPHENE NANOSHEETS; SURFACE-AREA; NANOTUBES;
   ELECTRODES
AB Hierarchical porous nitrogen-doped carbon (HPNC) nanosheets (NS) have been prepared via simultaneous activation and graphitization of biomass-derived natural silk. The as-obtained HPNC-NS show favorable features for electrochemical energy storage such as high specific surface area (S-BET: 2494 m(2)/g), high volume of hierarchical pores (2.28 cm(3)/g), nanosheet structures, rich N-doping (4.7%), and defects. With respect to the multiple synergistic effects of these features, a lithium-ion battery anode and a two-electrode-based supercapacitor have been prepared. A reversible lithium storage capacity of 1865 mA h/g has been reported, which is the highest for N-doped carbon anode materials to the best of our knowledge. The HPNC-NS supercapacitor's electrode in ionic liquid,electrolytes exhibit a capacitane of 242 F/g and energy density of 102 W h/kg (48W h/L), with high cycling life stability (9% loss after 10 000 cycles). Thus, a high-performance Li-ion battery and supercapacitors were successfully assembled for the same electrode material, which was obtained through a one-step and facile large-scale synthesis route. It is promising for next-generation hybrid energy storage and renewable delivery devices.
C1 [Hou, Jianhua; Cao, Chuanbao; Idrees, Faryal; Ma, Xilan] Beijing Inst Technol, Reseach Ctr Mat Sci, Beijing 100081, Peoples R China.
RP Cao, CB (reprint author), Beijing Inst Technol, Reseach Ctr Mat Sci, Beijing 100081, Peoples R China.
EM cbcao@bit.edu.cn
RI Cao, Chuanbao/J-5396-2013
OI Cao, Chuanbao/0000-0003-2830-4383
FU National Natural Science Foundation (NNSF), China [50972017]
FX C-B.C. designed the experiments. J-H.H. prepared the samples and
   performed the experiments. F.I. and X-L.M. participated in interpreting
   and analyzing the data. C-B.C. and J-H.H. wrote the manuscript. This
   work was supported by the National Natural Science Foundation (NNSF),
   China (grant no. 50972017).
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NR 74
TC 55
Z9 55
U1 249
U2 533
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD MAR
PY 2015
VL 9
IS 3
BP 2556
EP 2564
DI 10.1021/nn506394r
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA CE4HN
UT WOS:000351791800032
PM 25703427
ER

PT J
AU Cao, XH
   Zheng, B
   Rui, XH
   Shi, WH
   Yan, QY
   Zhang, H
AF Cao, Xiehong
   Zheng, Bing
   Rui, Xianhong
   Shi, Wenhui
   Yan, Qingyu
   Zhang, Hua
TI Metal Oxide-Coated Three-Dimensional Graphene Prepared by the Use of
   Metal-Organic Frameworks as Precursors
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE composite materials; lithium-ion batteries; metal-organic frameworks;
   photocatalysis; three-dimensional graphene networks
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIAL;
   CHEMICAL-VAPOR-DEPOSITION; ULTRATHIN GRAPHITE; HYDROGEN STORAGE;
   SOLAR-CELLS; COMPOSITES; MOF; NETWORKS; FOAM
AB A simple method for the preparation of metal-oxide-coated three-dimensional (3D) graphene composites was developed. The metal-organic frameworks (MOFs) that served as the precursors of the metal oxides were first synthesized on the 3D graphene networks (3DGNs). The desired metal oxide/3DGN composites were then obtained by a two-step annealing process. As a proof-of-concept application, the obtained ZnO/3DGN and Fe2O3/3DGN materials were used in a photocatalytic reaction and a lithium-ion battery, respectively. We believe this method could be extended to the synthesis of other metal oxide/3DGN composites with 3D structures simply through the appropriate choice of specific MOFs as precursors.
C1 [Cao, Xiehong; Zheng, Bing; Rui, Xianhong; Shi, Wenhui; Yan, Qingyu; Zhang, Hua] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
RP Zhang, H (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM HZhang@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; Rui, Xianhong/D-2604-2015; Cao,
   Xiehong/I-9665-2014; Zhang, Hua/A-1302-2009
OI Rui, Xianhong/0000-0003-1125-0905; Cao, Xiehong/0000-0002-3004-7518; 
FU Singapore MOE under AcRF [ARC 10/10, MOE2010-T2-1-060, ARC 26/13,
   MOE2013-T2-1-034, RG 61/12, RGT18/13]; Singapore National Research
   Foundation; Campus for Research Excellence and Technological Enterprise
   (CREATE) program "Nanomaterials for Energy and Water Management"; 
   [M4080865.070.706022]
FX This project was supported by Singapore MOE under AcRF Tier 2 (ARC
   10/10, No. MOE2010-T2-1-060; ARC 26/13, No. MOE2013-T2-1-034), and AcRF
   Tier 1 (RG 61/12, RGT18/13), and Start-Up Grant M4080865.070.706022.
   This research was also funded by the Singapore National Research
   Foundation, and publication was supported by the Campus for Research
   Excellence and Technological Enterprise (CREATE) program "Nanomaterials
   for Energy and Water Management".
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NR 67
TC 55
Z9 55
U1 168
U2 708
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD JAN 27
PY 2014
VL 53
IS 5
BP 1404
EP 1409
DI 10.1002/anie.201308013
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA AH9ZG
UT WOS:000336504500040
PM 24459058
ER

PT J
AU Mahmood, N
   Zhang, CZ
   Liu, F
   Zhu, JH
   Hou, YL
AF Mahmood, Nasir
   Zhang, Chenzhen
   Liu, Fei
   Zhu, Jinghan
   Hou, Yanglong
TI Hybrid of Co3Sn2@Co Nanoparticles and Nitrogen-Doped Graphene as a
   Lithium Ion Battery Anode
SO ACS NANO
LA English
DT Article
DE architectured anode; hydrothermal process; Co3Sn2@Co; nitrogen-doped
   graphene; lithium ion battery
ID OXYGEN REDUCTION REACTION; ELECTROCHEMICAL PERFORMANCE; REDUCED
   GRAPHENE; FACILE SYNTHESIS; STORAGE; OXIDE; CAPACITY; SHEETS; ELECTRODE;
   COMPOSITE
AB A facile strategy was designed for the fabrication of hybrid of Co3Sn2@Co nanoparticles (NPs) and nitrogen-doped graphene (NG) sheets through a hydrothermal synthesis, followed by annealing process. Core-shell architecture of Co3Sn2@Co pin on NG is designed for the dual encapsulation of Co3Sn2 with adaptable ensembles of Co and NG to address the structural and interfacial stability concerns facing tin-based anodes. In the resulted unique architecture of Co3Sn2@Co-NG hybrid, the sealed cobalt cover prevents the direct exposer of Sn with electrolyte because of encapsulated structure and keeps the structural and interfacial integrity of Co3Sn2. However, the elastically strong, flexible and conductive NG overcoat accommodates the volume changes and therefore brings the structural and electrical stabilization of Co3Sn2@Co NPs. As a result, Co3Sn2@Co-NG hybrid exhibits extraordinary reversible capacity of 1615 mAh/g at 250 mA/g after 100 cycles with excellent capacity retention of 102%. The hybrid bears superior rate capability with reversible capacity of 793.9 mAh/g at 2500 mA/g and Coulombic efficiency nearly 100%.
C1 [Mahmood, Nasir; Zhang, Chenzhen; Liu, Fei; Zhu, Jinghan; Hou, Yanglong] Peking Univ, Dept Mat Sci & Engn, Coll Engn, Beijing 100871, Peoples R China.
RP Hou, YL (reprint author), Peking Univ, Dept Mat Sci & Engn, Coll Engn, Beijing 100871, Peoples R China.
EM hou@pku.edu.cn
RI Hou, Yanglong/B-8688-2012
FU National Basic Research Program of China [2010CB934601]; NSFC [51125001,
   51172005, 90922033]; Natural Science Foundation of Beijing [2122022];
   Doctoral Program [20120001110078]; Aerostatic Science Foundation
   [2010ZF71003]; Fok Ying Tong Foundation [122043]
FX This work was supported by the National Basic Research Program of China
   (2010CB934601), the NSFC (51125001, 51172005, 90922033), the Natural
   Science Foundation of Beijing (2122022), the Doctoral Program
   (20120001110078), Aerostatic Science Foundation (2010ZF71003) and Fok
   Ying Tong Foundation (122043).
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NR 52
TC 55
Z9 55
U1 21
U2 176
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD NOV
PY 2013
VL 7
IS 11
BP 10307
EP 10318
DI 10.1021/nn4047138
PG 12
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 262QH
UT WOS:000327752200079
PM 24127745
ER

PT J
AU Ren, JG
   Wu, QH
   Tang, H
   Hong, G
   Zhang, WJ
   Lee, ST
AF Ren, Jian-Guo
   Wu, Qi-Hui
   Tang, Hao
   Hong, Guo
   Zhang, Wenjun
   Lee, Shuit-Tong
TI Germanium-graphene composite anode for high-energy lithium batteries
   with long cycle life
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ION BATTERIES; HIGH-CAPACITY; NANOWIRES; GE; NANOSTRUCTURES;
   NANOPARTICLES; NANOTUBES; NETWORKS; STORAGE; HYBRID
AB The high-energy lithium ion battery is an ideal power source for electric vehicles and grid-scale energy storage applications. Germanium is a promising anode material for lithium ion batteries due to its high specific capacity, but still suffers from poor cyclability. Here, we report a facile preparation of a germanium-graphene nanocomposite using a low-pressure thermal evaporation approach, by which crystalline germanium particles are uniformly deposited on graphene surfaces or embedded into graphene sheets. The nanocomposite exhibits a high Coulombic efficiency of 80.4% in the first cycle and a capacity retention of 84.9% after 400 full cycles in a half cell, along with high utilization of germanium in the composite and high rate capability. These outstanding properties are attributed to the monodisperse distribution of high-quality germanium particles in a flexible graphene framework. This preparation approach can be extended to other active elements that can be easily evaporated (e.g., sulfur, phosphorus) for the preparation of graphene-based composites for lithium ion battery applications.
C1 [Ren, Jian-Guo; Wu, Qi-Hui; Tang, Hao; Hong, Guo; Lee, Shuit-Tong] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China.
   [Ren, Jian-Guo; Wu, Qi-Hui; Hong, Guo; Zhang, Wenjun] City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
RP Ren, JG (reprint author), Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China.
EM apannale@suda.edu.cn
RI Zhang, WJ/C-6995-2012
FU Research Grants Council of Hong Kong SAR, China - GRF Grant
   [CityU102010]; National Natural Science Foundation of China [51072126,
   51132006]; National Basic Research Program of China (973 program)
   [2009CB623703, 2012CB932402]; Priority Academic Program Development of
   Jiangsu Higher Education Institutions (PAPD)
FX This work was funded by Research Grants Council of Hong Kong SAR, China
   - GRF Grant (no. CityU102010), National Natural Science Foundation of
   China (no. 51072126, 51132006), National Basic Research Program of China
   (973 program) (no. 2009CB623703, 2012CB932402) and a Project Funded by
   the Priority Academic Program Development of Jiangsu Higher Education
   Institutions (PAPD).
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NR 32
TC 55
Z9 56
U1 15
U2 181
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 5
BP 1821
EP 1826
DI 10.1039/c2ta01286c
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085UP
UT WOS:000314640100040
ER

PT J
AU Chen, YM
   Lu, ZG
   Zhou, LM
   Mai, YW
   Huang, HT
AF Chen, Yuming
   Lu, Zhouguang
   Zhou, Limin
   Mai, Yiu-Wing
   Huang, Haitao
TI Triple-coaxial electrospun amorphous carbon nanotubes with hollow
   graphitic carbon nanospheres for high- performance Li ion batteries
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID HIGH-RATE CAPABILITY; LITHIUM STORAGE; ANODE MATERIALS; NANOFIBERS;
   GRAPHENE; CAPACITY; HYBRID; FIBER
AB We prepared amorphous carbon nanotubes decorated with hollow graphitic carbon nanospheres (ACNHGCNs) using a novel triple-coaxial electrospinning method and characterized the electrochemical performance of these ACNHGCNs as anode materials for lithium ion batteries (LIBs). The ACNHGCNs displayed a very high reversible specific capacity of similar to 969 mA h g(-1) at a current density of 50 mA g(-1), which is nearly 2.6 times the theoretical capacity of graphite (372 mA h g(-1)). The ACNHGCNs also showed a high volumetric capacity of similar to 1.42 A h cm(-3) and good cycling stability and outstanding rate capability. The prepared ACNHGCNs can be a promising alternative anode material used for high-energy, low-cost and environmentally friendly lithium ion batteries.
C1 [Chen, Yuming; Lu, Zhouguang; Zhou, Limin; Mai, Yiu-Wing] Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China.
   [Mai, Yiu-Wing] Univ Sydney, Sch Aerosp Mech & Mechatron Engn J07, CAMT, Sydney, NSW 2006, Australia.
   [Huang, Haitao] Hong Kong Polytech Univ, Dept Appl Phys, Hong Kong, Hong Kong, Peoples R China.
   [Huang, Haitao] Hong Kong Polytech Univ, Mat Res Ctr, Hong Kong, Hong Kong, Peoples R China.
RP Chen, YM (reprint author), Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China.
EM mmlmzhou@inet.polyu.edu.hk
RI Huang, Haitao/F-9697-2010; Mai, YW/K-8436-2012; Lu,
   Zhouguang/G-6240-2013; Chen, Yuming/H-7812-2014
OI Lu, Zhouguang/0000-0001-9375-7747; 
FU Research Grant Council of the Hong Kong Special Administration Region
   [PolyU 5349/10E]; Hong Kong Polytechnic University [1-BD08]
FX The authors are grateful for the support received from the Research
   Grant Council of the Hong Kong Special Administration Region (grant:
   PolyU 5349/10E) and The Hong Kong Polytechnic University (grant:
   1-BD08).
CR Kaskhedikar NA, 2009, ADV MATER, V21, P2664, DOI 10.1002/adma.200901079
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NR 37
TC 55
Z9 55
U1 32
U2 172
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD JUL
PY 2012
VL 5
IS 7
BP 7898
EP 7902
DI 10.1039/c2ee22085g
PG 5
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 962GS
UT WOS:000305530900025
ER

PT J
AU Qu, BH
   Chen, YJ
   Zhang, M
   Hu, LL
   Lei, DN
   Lu, BA
   Li, QH
   Wang, YG
   Chen, LB
   Wang, TH
AF Qu, Baihua
   Chen, Yuejiao
   Zhang, Ming
   Hu, Lingling
   Lei, Danni
   Lu, Bingan
   Li, Qiuhong
   Wang, Yanguo
   Chen, Libao
   Wang, Taihong
TI beta-Cobalt sulfide nanoparticles decorated graphene composite
   electrodes for high capacity and power supercapacitors
SO NANOSCALE
LA English
DT Article
ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL SUPERCAPACITORS; ENERGY-STORAGE;
   ANODE MATERIAL; PERFORMANCE; ARRAYS; COS2; NANOSTRUCTURES; SPHERES;
   CARBON
AB Electrochemical supercapacitors have drawn much attention because of their high power and reasonably high energy densities. However, their performances still do not reach the demand of energy storage. In this paper beta-cobalt sulfide nanoparticles were homogeneously distributed on a highly conductive graphene (CS-G) nanocomposite, which was confirmed by transmission electron microscopy analysis, and exhibit excellent electrochemical performances including extremely high values of specific capacitance (similar to 1535 F g(-1)) at a current density of 2 A g(-1), high-power density (11.98 kW kg(-1)) at a discharge current density of 40 A g(-1) and excellent cyclic stability. The excellent electrochemical performances could be attributed to the graphene nanosheets (GNSs) which could maintain the mechanical integrity. Also the CS-G nanocomposite electrodes have high electrical conductivity. These results indicate that high electronic conductivity of graphene nanocomposite materials is crucial to achieving high power and energy density for supercapacitors.
C1 [Qu, Baihua; Chen, Yuejiao; Zhang, Ming; Hu, Lingling; Lei, Danni; Lu, Bingan; Li, Qiuhong; Wang, Yanguo; Chen, Libao; Wang, Taihong] Hunan Univ, Key Lab Micronano Optoelect Devices, State Key Lab Chemobiosensing & Chemometr, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   [Wang, Yanguo] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China.
RP Chen, LB (reprint author), Hunan Univ, Key Lab Micronano Optoelect Devices, State Key Lab Chemobiosensing & Chemometr, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM lbchen@hnu.edu.cn; thwang@hnu.edu.cn
RI Wang, Taihong/K-8968-2012; Qu, Baihua/H-9594-2012; Zhang,
   Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU Scholarship Award for Excellent Doctoral Student; Ministry of Education;
   National Natural Science Foundation of China [21103046, 60796078,
   21003041, 11274107, 61204109]; Hunan Provincial Natural Science
   Foundation of China [11JJ7004, 10JJ1011]; Hunan Provincial Innovation
   Foundation for Postgraduate [CX2012B125]
FX This work was partly supported from Scholarship Award for Excellent
   Doctoral Student granted by Ministry of Education (2012). We thank the
   financial support of the National Natural Science Foundation of China
   (Grant no. 21103046, 60796078, 21003041, 11274107, and 61204109), the
   Hunan Provincial Natural Science Foundation of China (Grant no. 11JJ7004
   and 10JJ1011), and the Hunan Provincial Innovation Foundation for
   Postgraduate (Grant no. CX2012B125). The authors thank Dr Jiabiao Lian
   (The Chinese University of Hong Kong) for TEM measurement and Professor
   Weifeng Wei at Central South University for XRD and Raman spectra
   measurement. Special thanks to Dr Chengchao Li (Hunan University) for
   stimulating discussion.
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NR 42
TC 55
Z9 55
U1 32
U2 163
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 24
BP 7810
EP 7816
DI 10.1039/c2nr31902k
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 044RS
UT WOS:000311641500029
PM 23147355
ER

PT J
AU Shou, QL
   Cheng, JP
   Zhang, L
   Nelson, BJ
   Zhang, XB
AF Shou, Qingliang
   Cheng, Jipeng
   Zhang, Li
   Nelson, Bradley J.
   Zhang, Xiaobin
TI Synthesis and characterization of a nanocomposite of goethite nanorods
   and reduced graphene oxide for electrochemical capacitors
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Nanocomposites; Goethite; Nanorods; Reduced graphene oxide;
   Electrochemical capacitance
ID LITHIUM-ION BATTERIES; ALPHA-FEOOH; CARBON NANOTUBES; ANODE MATERIAL;
   ALPHA-FE2O3 NANORODS; IRON-OXIDE; NANOPARTICLES; FE3O4; SUPERCAPACITOR;
   PERFORMANCE
AB We report a one-step synthesis of a nanocomposite of goethite (alpha-FeOOH) nanorods and reduced graphene oxide (RGO) using a solution method in which ferrous cations serve as a reducing agent of graphite oxide (GO) to graphene and a precursor to grow goethite nanorods. As-prepared goethite nanorods have an average length of 200 nm and a diameter of 30 nm and are densely attached on both sides of the RGO sheets. The electrochemical properties of the nanocomposite were characterized by cyclic voltammetry (CV) and chronopotentiometry (CP) charge-discharge tests. The results showed that goethite/RGO composites have a high electrochemical capacitance of 165.5 F g(-1) with an excellent recycling capability making the material promising for electrochemical capacitors. (C) 2011 Elsevier Inc. All rights reserved.
C1 [Shou, Qingliang; Cheng, Jipeng; Zhang, Xiaobin] Zhejiang Univ, State Key Lab Silicon Mat, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
   [Zhang, Li; Nelson, Bradley J.] ETH, Inst Robot & Intelligent Syst, CH-8092 Zurich, Switzerland.
RP Cheng, JP (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
EM chengjp@zju.edu.cn; lizhang@ethz.ch
RI Zhang, Li/G-7384-2012; Cheng, Jipeng/J-9300-2013; Nelson,
   Bradley/B-7761-2013
OI Nelson, Bradley/0000-0001-9070-6987
FU State Key Laboratory of Zhejiang University, P. R. China [SKL 2009-4];
   Sino-Swiss Science and Technology Cooperation (SSSTC) [EG 08-092009];
   opening foundation of Zhejiang Provincial Top Key Discipline [20110905]
FX We thank the FIRST lab of ETH Zurich for technical support. Funding for
   this research was partially provided by the open funding (Grant nr. SKL
   2009-4) of the State Key Laboratory of Zhejiang University, P. R. China,
   the Sino-Swiss Science and Technology Cooperation (SSSTC, Grant nr. EG
   08-092009) and the opening foundation of Zhejiang Provincial Top Key
   Discipline (No. 20110905).
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NR 40
TC 55
Z9 55
U1 22
U2 154
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD JAN
PY 2012
VL 185
BP 191
EP 197
DI 10.1016/j.jssc.2011.11.020
PG 7
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 874EA
UT WOS:000298937000030
ER

PT J
AU Tang, YF
   Huang, FQ
   Zhao, W
   Liu, ZQ
   Wan, DY
AF Tang, Yufeng
   Huang, Fuqiang
   Zhao, Wei
   Liu, Zhanqiang
   Wan, Dongyun
TI Synthesis of graphene-supported Li4Ti5O12 nanosheets for high rate
   battery application
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; RATE CAPABILITY; ELECTROCHEMICAL PERFORMANCE;
   SPINEL LI4TI5O12; HYBRID MATERIALS; ANODE MATERIAL; HIGH-CAPACITY;
   STORAGE; ELECTRODES
AB The composite structure of Li4Ti5O12 (LTO) nanosheets rooted on two-dimensional graphene (GR) was proposed to achieve an enhanced rate performance for high rate lithium ion batteries. Such a nanostructured material of graphene-supported Li4Ti5O12 nanosheets (GR-LTOs) was fabricated by using TiO2 colloid-containing graphene oxide (GO) sheets as precursor in a hydrothermal reaction. TiO2 colloids serve as the seeds to realize the growth of LTO on GR and ensure the tight bonding between GR and LTO to benefit the charge transfer from the two types of sheets. The GR-LTOs sample possesses excellent electrochemical properties with good cycle stability and a high specific capacity of 140 mA h g(-1) at 20 C. It demonstrates that LTO nanosheets, graphene sheets, and their tightly-bonded interfaces provide short ion diffusion distance and good electron conduction in such a composite structure.
C1 [Tang, Yufeng; Huang, Fuqiang; Zhao, Wei; Liu, Zhanqiang; Wan, Dongyun] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China.
   [Tang, Yufeng; Huang, Fuqiang; Zhao, Wei; Liu, Zhanqiang; Wan, Dongyun] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
   [Huang, Fuqiang] Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China.
RP Huang, FQ (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China.
EM huangfq@mail.sic.ac.cn
RI 赵, 伟/D-7147-2014
FU National 973 & 863 Program of China [2009CB939903, 2011AA050505]; NSF of
   China [50821004, 61106088, 50902143, 21101164, 61076062, 51102263,
   20901083]; Science and Technology Commission of Shanghai [10520706700,
   10JC1415800]
FX This work is financially supported by National 973 & 863 Program of
   China Grant No. 2009CB939903 & 2011AA050505, NSF of China Grant No.
   50821004 & 61106088 & 50902143 & 21101164 & 61076062 & 51102263,
   National Science Foundation of China Grant 20901083 and Science and
   Technology Commission of Shanghai Grant No. 10520706700 & 10JC1415800.
CR Shi Y, 2011, J POWER SOURCES, V196, P8610, DOI 10.1016/j.jpowsour.2011.06.002
   Kang KS, 2006, SCIENCE, V311, P977, DOI 10.1126/science.1122152
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NR 25
TC 55
Z9 56
U1 19
U2 150
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 22
BP 11257
EP 11260
DI 10.1039/c2jm30624g
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 942QO
UT WOS:000304062300046
ER

PT J
AU Cho, YJ
   Kim, HS
   Im, H
   Myung, Y
   Jung, GB
   Lee, CW
   Park, J
   Park, MH
   Cho, J
   Kang, HS
AF Cho, Yong Jae
   Kim, Han Sung
   Im, Hyungsoon
   Myung, Yoon
   Jung, Gyeong Bok
   Lee, Chi Woo
   Park, Jeunghee
   Park, Mi-Hee
   Cho, Jaephil
   Kang, Hong Seok
TI Nitrogen-Doped Graphitic Layers Deposited on Silicon Nanowires for
   Efficient Lithium-Ion Battery Anodes
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID CARBON NITRIDE NANOTUBES; CORE-SHELL NANOWIRES; HIGH-CAPACITY; SECONDARY
   BATTERIES; ARRAYS; ELECTRODES; DIAMETER; SINGLE; ATOMS
AB Nitrogen (N)-doped graphitic layers were deposited as shells on pregrown silicon nanowires by chemical vapor deposition. Graphite-like and pyridine-like structures were selectively chosen for 3 and 10% N doping, respectively. Increasing the thickness of the undoped graphitic layers from 20 to 50 nm led to an increase in the charge capacity of the lithium ion battery from 800 to 1040 mA h/g after 45 cycles. Graphite-like 3% N-doping in the 50 nm-thick shell increases the charge capacity by 21% (i.e., to 1260 mA big), while pyridine-like 10% N-doping in the 20 nm-thick shell increases it by 36% (i.e., to 1090 rnA h/g). This suggests that both pyridine- and graphite-like structures can be effective for lithium intercalation. First principles calculations of the graphene sheets show that the large storage capacity of both N-doping structures comes from the formation of dangling bonds around the pyridine-like local motives upon lithium intercalation.
C1 [Cho, Yong Jae; Kim, Han Sung; Im, Hyungsoon; Myung, Yoon; Jung, Gyeong Bok; Lee, Chi Woo; Park, Jeunghee] Korea Univ, Dept Chem, Jochiwon 339700, South Korea.
   [Park, Mi-Hee; Cho, Jaephil] Ulsan Natl Inst Sci & Technol, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea.
   [Kang, Hong Seok] Jeonju Univ, Dept Nano & Adv Mat, Coll Engn, Chonju 560709, Chonbuk, South Korea.
RP Park, J (reprint author), Korea Univ, Dept Chem, Jochiwon 339700, South Korea.
EM parkjh@korea.ac.kr; jpcho@unist.ac.kr; hsk@jj.ac.kr
RI Cho, Jaephil/E-4265-2010; Park, Mi-Hee/F-9995-2010
FU NRF [20100000181, 2009-82528, 2010-0029164]; IITA
   [2008-C1090-0804-0013]; WCU [R31-10035]; Ministry of Education, Science
   and Technology [2010-0007815]; MOST; POSTECH; Korea Institute of Science
   and Technology Information [KSC-2008-S03-0008]
FX This study was supported by the NRF (20100000181; 2009-82528;
   2010-0029164), IITA (2008-C1090-0804-0013), and WCU program (R31-10035).
   This work was also supported by the Basic Science Research Program
   through the NRF of Korea funded by the Ministry of Education, Science
   and Technology (2010-0007815). The HVEM (Daejeon) measurements were
   performed at the KBSI. The experiments at the PLS were partially
   supported by MOST and POSTECH. Computations were performed using a
   supercomputer of the Korea Institute of Science and Technology
   Information under the Contract No. KSC-2008-S03-0008.
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NR 48
TC 55
Z9 55
U1 8
U2 105
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD MAY 19
PY 2011
VL 115
IS 19
BP 9451
EP 9457
DI 10.1021/jp201485j
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 761UV
UT WOS:000290427400018
ER

PT J
AU Chen, YJ
   Zhu, J
   Qu, BH
   Lu, BA
   Xu, Z
AF Chen, Yuejiao
   Zhu, Jian
   Qu, Baihua
   Lu, Bingan
   Xu, Zhi
TI Graphene improving lithium-ion battery performance by construction of
   NiCo2O4/graphene hybrid nanosheet arrays
SO NANO ENERGY
LA English
DT Article
DE Graphene hybrid arrays; Lithium-ion battery; Pulverization; Cycling
   stability
ID ELECTROCHEMICAL PERFORMANCE; ANODE MATERIAL; REVERSIBLE CAPACITY;
   NANOWIRE ARRAYS; STORAGE; OXIDE; SUPERCAPACITORS; NANOPARTICLES;
   MICROSPHERES; CAPABILITY
AB NiCo2O4 is a potential lithium-ion battery (LIB) anode material that can be applied to the industrial production for commercial applications. However, the capacity and cycling stability of the LIB based on NiCo2O4 should be improved first. Herein, graphene-based NiCo2O4 nanosheet arrays directly grown on nickel foam have been successfully synthesized. This composites array shows significantly improved lithium storage properties with higher reversible capacity and better cycling stability than NiCo2O4 nanosheets. The three-dimensional graphene not only serves as a conductive network to increase the conductivity of the NiCo2O4, but also can offer effective buffering to accommodate the lithiation-induced stress which is beneficial to lithium storage and cycling stability.(C) 2013 Published by Elsevier Ltd.
C1 [Chen, Yuejiao; Zhu, Jian; Qu, Baihua; Lu, Bingan; Xu, Zhi] Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
RP Lu, BA (reprint author), Hunan Univ, State Key Lab Chemo Biosensing & Chemometr, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM luba2012@hnu.edu.cn; patrick_xuyang@163.com
RI Qu, Baihua/H-9594-2012
FU National Natural Science Foundation of China [21303046]; Research Fund
   for the Doctoral Program of Higher Education [20130161120014];
   Scholarship Award for Excellent Doctoral Students; Ministry of Education
FX This work was supported by National Natural Science Foundation of China
   (Grant nos. 21303046), the Research Fund for the Doctoral Program of
   Higher Education (Grant nos. 20130161120014), and a Scholarship Award
   for Excellent Doctoral Students granted by the Ministry of
   Education(2012).
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NR 40
TC 54
Z9 54
U1 46
U2 233
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD JAN
PY 2014
VL 3
BP 88
EP 94
DI 10.1016/j.nanoen.2013.10.008
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AA2HI
UT WOS:000330915300010
ER

PT J
AU Wang, B
   Li, XL
   Qiu, TF
   Luo, B
   Ning, J
   Li, J
   Zhang, XF
   Liang, MH
   Zhi, LJ
AF Wang, Bin
   Li, Xianglong
   Qiu, Tengfei
   Luo, Bin
   Ning, Jing
   Li, Jing
   Zhang, Xianfeng
   Liang, Minghui
   Zhi, Linjie
TI High Volumetric Capacity Silicon-Based Lithium Battery Anodes by
   Nanoscale System Engineering
SO NANO LETTERS
LA English
DT Article
DE Silicon nanowire; graphene; volumetric capacity; nanoscale system
   engineering lithium ion battery
ID LI-ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; LONG CYCLE LIFE;
   NANOSTRUCTURED SILICON; RECHARGEABLE BATTERIES; SUPPORTED SILICON;
   PERFORMANCE; SI; NANOWIRES; NANOCOMPOSITES
AB The nanostructuring of silicon (Si) has recently received great attention, as it holds potential to deal with the dramatic volume change of Si and thus improve lithium storage performance. Unfortunately, such transformative materials design principle has generally been plagued by the relatively low tap density of Si and hence mediocre volumetric capacity (and also volumetric energy density) of the battery. Here, we propose and demonstrate an electrode consisting of a textured silicon@graphitic carbon nanowire array. Such a unique electrode structure is designed based on a nanoscale system engineering strategy. The resultant electrode prototype exhibits unprecedented lithium storage performance, especially in terms of volumetric capacity, without the expense of compromising other components of the battery. The fabrication method is simple and scalable, providing new avenues for the rational engineering of Si-based electrodes simultaneously at the individual materials unit scale and the materials ensemble scale.
C1 [Wang, Bin; Li, Xianglong; Qiu, Tengfei; Luo, Bin; Ning, Jing; Li, Jing; Zhang, Xianfeng; Liang, Minghui; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Li, XL (reprint author), Natl Ctr Nanosci & Technol, 11 Beiyitiao, Beijing 100190, Peoples R China.
EM lixl@nanoctr.cn; zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
FU Ministry of Science and Technology of China [2012CB933403]; National
   Natural Science Foundation of China [21173057, 21273054, 51302045];
   Beijing Municipal Science and Technology Commission [Z121100006812003];
   Chinese Academy of Sciences
FX The authors acknowledge support from the Ministry of Science and
   Technology of China (2012CB933403), the National Natural Science
   Foundation of China (Grants 21173057, 21273054, and 51302045), the
   Beijing Municipal Science and Technology Commission (Z121100006812003),
   and the Chinese Academy of Sciences.
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NR 54
TC 54
Z9 54
U1 21
U2 191
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2013
VL 13
IS 11
BP 5578
EP 5584
DI 10.1021/nl403231v
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 253TH
UT WOS:000327111700092
PM 24164145
ER

PT J
AU Zhou, XS
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Wan, Li-Jun
   Guo, Yu-Guo
TI Electrospun Silicon Nanoparticle/Porous Carbon Hybrid Nanofibers for
   Lithium-Ion Batteries
SO SMALL
LA English
DT Article
DE electrospinning; silicon nanoparticles; porous carbon nanofibers;
   lithium-ion batteries; hybrid materials
ID IMPROVED ANODE MATERIALS; STRUCTURAL EVOLUTION; NEGATIVE ELECTRODES;
   STORAGE DEVICES; SI; LI; GRAPHENE; PERFORMANCE; CATHODE; NANOCOMPOSITES
C1 Beijing Natl Lab Mol Sci BNLMS, Chinese Acad Sci CAS, Inst Chem, CAS Key Lab Mol, Beijing 100190, Peoples R China.
   Beijing Natl Lab Mol Sci BNLMS, Chinese Acad Sci CAS, Inst Chem, CAS Key Lab Mol, Beijing 100190, Peoples R China.
   [Zhou, Xiaosi; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2009CB930400, 2011CB935700,
   2012CB932900]; National Natural Science Foundation of China [51225204,
   91127044, 21073205]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2009CB930400, 2011CB935700 and 2012CB932900), the National
   Natural Science Foundation of China (Grant Nos. 51225204, 91127044 and
   21073205), and the Chinese Academy of Sciences.
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NR 52
TC 54
Z9 54
U1 41
U2 186
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD AUG 26
PY 2013
VL 9
IS 16
BP 2684
EP 2688
DI 10.1002/smll.201202071
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 262MD
UT WOS:000327738600005
PM 23463677
ER

PT J
AU Zhao, HB
   Pan, LY
   Xing, SY
   Luo, J
   Xu, JQ
AF Zhao, Hongbin
   Pan, Lanying
   Xing, Siyi
   Luo, Jun
   Xu, Jiaqiang
TI Vanadium oxides-reduced graphene oxide composite for lithium-ion
   batteries and supercapacitors with improved electrochemical performance
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Vanadium oxides; Cathode; Rechargeable battery; Supercapacitor; Reduced
   graphene oxide
ID CYCLIC PERFORMANCE; ANODE MATERIAL; V2O5; CAPACITY; ELECTRODES; ARRAYS;
   XPS; VO2; INTERCALATION; NANOCOMPOSITE
AB A facile approach to the surface reduced graphene oxide (rGO) modification of micro-nano structured vanadium oxides composites are developed as cathode materials of lithium ions batteries (LIBs) and supercapacitors (SCPs) for the first time. The as-prepared V2O5-rGO and VO2-rGO composites exhibit remarkably enhanced cycling performance when being used as cathode materials in LIBs and SCPs, respectively. The uniform coating of graphene around the surface of vanadium oxides ensures good close electrical contact, therefore higher specific capacity and enhanced cycling performance than pure VO2 and V2O5 electrodes. Meanwhile, the cycling performance enhancement and capacity decay mechanism are presented, which is not only important to design electrode materials in LIBs and SCPs, but also extendable to the design and fabrication of other functional materials for energy storage and transfer systems. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Zhao, Hongbin; Pan, Lanying; Xing, Siyi; Luo, Jun; Xu, Jiaqiang] Shanghai Univ, Coll Sci, Shanghai 200444, Peoples R China.
RP Xu, JQ (reprint author), Shanghai Univ, Coll Sci, 99 Shangda Rd, Shanghai 200444, Peoples R China.
EM hongbinzhao@shu.edu.cn; xujiaqiang@shu.edu.cn
FU National Natural Science Foundation of China [61071040]; Shanghai
   Municipal Education Commission [J50102]; Innovative Foundation of
   Shanghai University
FX We acknowledge the financial support from the National Natural Science
   Foundation of China (Grant No. 61071040), Leading Academic Discipline
   Project of Shanghai Municipal Education Commission (No. J50102) and
   Innovative Foundation of Shanghai University. We thank Instrumental
   Analysis and Research Center of Shanghai University. Thank Yamei Zhu
   (College of Foreign Language, Changchun Institute of Technology,
   Changchun, China) to polish the language.
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NR 53
TC 54
Z9 56
U1 42
U2 397
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JAN 15
PY 2013
VL 222
BP 21
EP 31
DI 10.1016/j.jpowsour.2012.08.036
PG 11
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 037TR
UT WOS:000311129900004
ER

PT J
AU Park, SK
   Yu, SH
   Woo, S
   Quan, B
   Lee, DC
   Kim, MK
   Sung, YE
   Piao, Y
AF Park, Seung-Keun
   Yu, Seung-Ho
   Woo, Seunghee
   Quan, Bo
   Lee, Dong-Chan
   Kim, Min Kun
   Sung, Yung-Eun
   Piao, Yuanzhe
TI A simple L-cysteine-assisted method for the growth of MoS2 nanosheets on
   carbon nanotubes for high-performance lithium ion batteries
SO DALTON TRANSACTIONS
LA English
DT Article
ID ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCES; HYDROTHERMAL SYNTHESIS;
   GRAPHENE; COMPOSITES; NANOWIRES; STORAGE; SUPERCAPACITORS;
   NANOCOMPOSITES; NANOPARTICLES
AB We introduce a simple process to synthesize few-layered MoS2 nanosheets supported on coaxial carbon nanotubes through an L-cysteine-assisted hydrothermal route, in which L-cysteine, a cheap and ordinary amino acid, plays a fundamental role in controlling the morphology of the hybrid material and the binder to help the growth of MoS2 nanosheets on the surface of the carbon nanotubes. It is also demonstrated that the polypeptide formed by L-cysteine can be transformed into amorphous carbon by heat treatment under an inert atmosphere. The materials exhibit high capacity and excellent cycling performance when used as anode materials for lithium ion batteries. The specific capacity of a composite with 1 : 4 molar ratio of MoS2 to carbon nanotubes is 736.5 mAh g(-1) after the first cycle, increased for several initial cycles, and remains at 823.4 mAh g(-1) even after 30 cycles, when cycled at a current density of 100 mA g(-1). At a very high current density of 1600 mA g(-1), the material shows a stable capacity of approximately 530 mAh g(-1) after 30 cycles. The noteworthy improvement in the electrochemical performance of the material can be attributed to their unique structure and the synergistic effects of amorphous carbon and few-layered MoS2.
C1 [Park, Seung-Keun; Quan, Bo; Piao, Yuanzhe] Seoul Natl Univ, Grad Sch Convergence Sci & Technol, Dept Nano Sci & Technol, Suwon 443270, South Korea.
   [Yu, Seung-Ho; Lee, Dong-Chan; Kim, Min Kun; Sung, Yung-Eun] Seoul Natl Univ, Coll Engn, Sch Chem & Biol Engn, WCU Program Chem Convergence Energy & Environm C2, Seoul 151744, South Korea.
   [Woo, Seunghee] Seoul Natl Univ, Dept Chem, Seoul 151747, South Korea.
   [Piao, Yuanzhe] Adv Inst Convergence Technol, Suwon 443270, Gyeonggi Do, South Korea.
RP Sung, YE (reprint author), Seoul Natl Univ, Coll Engn, Sch Chem & Biol Engn, WCU Program Chem Convergence Energy & Environm C2, Seoul 151744, South Korea.
EM parkat9@snu.ac.kr; ysung@snu.ac.kr
RI Park, Seung-Keun/E-8420-2011
OI Park, Seung-Keun/0000-0002-0373-163X
FU Center for Integrated Smart Sensors; Ministry of Education, Science and
   Technology as Global Frontier Project [CISS-2012M3A6A6054186]; Basic
   Science Research Program through the National Research Foundation of
   Korea (NRF); Ministry of Education, Science and Technology
   [2011-0025391]; National Research Foundation of Korea Grant; Korean
   Government (MEST) [NRF-C1AAA001-2010-0029065]; Fundamental R&D Program
   for Technology of World Premier Materials; Ministry of Knowledge
   Economy, Republic of Korea
FX Y. P. acknowledges financial support by the Center for Integrated Smart
   Sensors funded by the Ministry of Education, Science and Technology as
   Global Frontier Project (CISS-2012M3A6A6054186) and by the Basic Science
   Research Program through the National Research Foundation of Korea (NRF)
   funded by the Ministry of Education, Science and Technology (No.
   2011-0025391). Y.-E. S. acknowledges financial support from the National
   Research Foundation of Korea Grant funded by the Korean Government
   (MEST) (NRF-C1AAA001-2010-0029065) and the Fundamental R&D Program for
   Technology of World Premier Materials funded by the Ministry of
   Knowledge Economy, Republic of Korea.
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NR 28
TC 54
Z9 55
U1 23
U2 276
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1477-9226
J9 DALTON T
JI Dalton Trans.
PY 2013
VL 42
IS 7
BP 2399
EP 2405
DI 10.1039/c2dt32137h
PG 7
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 074HT
UT WOS:000313804200011
PM 23208383
ER

PT J
AU Wang, RH
   Xu, CH
   Sun, J
   Liu, YQ
   Gao, L
   Lin, CC
AF Wang, Ronghua
   Xu, Chaohe
   Sun, Jing
   Liu, Yangqiao
   Gao, Lian
   Lin, Chucheng
TI Free-standing and binder-free lithium-ion electrodes based on robust
   layered assembly of graphene and Co3O4 nanosheets
SO NANOSCALE
LA English
DT Article
ID PERFORMANCE ANODE MATERIAL; REDUCED GRAPHENE; BATTERY ANODES;
   ELECTROCHEMICAL PERFORMANCE; RECHARGEABLE BATTERIES; REVERSIBLE
   CAPACITY; CYCLIC PERFORMANCE; STORAGE PROPERTIES; FACILE SYNTHESIS; RATE
   CAPABILITY
AB Free-standing and binder-free Co3O4/graphene films were fabricated through vacuum filtration and thermal treatment processes, in which sheet-like Co3O4 and graphene were assembled into a robust lamellar hierarchical structure via electrostatic interactions. The morphological compatibility coupled with strong interfacial interactions between Co3O4 and graphene significantly promoted the interfacial electron and lithium ion transport. When used as a binder-less and free-standing electrode for lithium-ion batteries, the hybrid film delivered a high specific capacity (similar to 1400 mA h g(-1) at 100 mA g(-1) based on the total electrode weight), enhanced rate capability and excellent cyclic stability (similar to 1200 mA h g(-1) at 200 mA g(-1) after 100 cycles). This effective strategy will provide new insight into the design and synthesis of many other composite electrodes for high-performance lithium-ion batteries.
C1 [Wang, Ronghua; Xu, Chaohe; Sun, Jing; Liu, Yangqiao; Gao, Lian; Lin, Chucheng] Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, Shanghai 200050, Peoples R China.
RP Sun, J (reprint author), Chinese Acad Sci, State Key Lab High Performance Ceram & Superfine, Shanghai Inst Ceram, 1295 Dingxi Rd, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU 973 Project [2012CB932303]; National Natural Science Foundation of China
   [51172261]
FX This work is supported by the 973 Project (2012CB932303), the National
   Natural Science Foundation of China (Grant no. 51172261).
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NR 69
TC 54
Z9 54
U1 22
U2 146
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 15
BP 6960
EP 6967
DI 10.1039/c3nr01392h
PG 8
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 181NY
UT WOS:000321675600042
PM 23793785
ER

PT J
AU Chockla, AM
   Panthani, MG
   Holmberg, VC
   Hessel, CM
   Reid, DK
   Bogart, TD
   Harris, JT
   Mullins, CB
   Korgel, BA
AF Chockla, Aaron M.
   Panthani, Matthew G.
   Holmberg, Vincent C.
   Hessel, Colin M.
   Reid, Dariya K.
   Bogart, Timothy D.
   Harris, Justin T.
   Mullins, C. Buddie
   Korgel, Brian A.
TI Electrochemical Lithiation of Graphene-Supported Silicon and Germanium
   for Rechargeable Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; FLUOROETHYLENE CARBONATE;
   NANOSTRUCTURED SILICON; REVERSIBLE CAPACITY; SI ELECTRODES; LI STORAGE;
   NANOWIRES; PERFORMANCE; OXIDE
AB Binder-free graphene-supported Ge nanowires, Si nanowires, and Si nanocrystals were studied for use as negative electrode materials in rechargeable lithium ion batteries (LIBs). Graphene obtained from reduced graphene oxide (RGO) helped stabilize electrochemical cycling of all of the nanomaterials. However, differential capacity plots revealed competition between RGO and Si/Ge lithiation. At high Si/Ge loading (>50% w/w) and low cycle rates (<C/10), only lithiation of Si and Ge occurs, but at higher cycle rates (>C/10), RGO lithiation begins to dominate. Under those conditions, only Ge nanowires exhibited significant lithiation relative to RGO, most likely due to the inherently faster lithiation of Ge compared to Si.
C1 [Chockla, Aaron M.; Panthani, Matthew G.; Holmberg, Vincent C.; Hessel, Colin M.; Reid, Dariya K.; Bogart, Timothy D.; Harris, Justin T.; Mullins, C. Buddie; Korgel, Brian A.] Univ Texas Austin, Dept Chem Engn, Texas Mat Inst, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA.
RP Korgel, BA (reprint author), Univ Texas Austin, Dept Chem Engn, Texas Mat Inst, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA.
EM korgel@che.utexas.edu
RI Korgel, Brian/I-5771-2013; Panthani, Matthew/C-8829-2014; 
OI Panthani, Matthew/0000-0002-3795-2051; Holmberg,
   Vincent/0000-0002-9591-8951
FU Robert A. Welch Foundation [F-1464, F-1436]; Air Force Research
   Laboratory [FA-8650-07-2-5061]; Fannie and John Hertz Foundation; NSF;
   program "Understanding Charge Separation and Transfer at Interfaces in
   Energy Materials (EFRC:CST)," an Energy Frontier Research Center; U.S.
   Department of Energy Office of Science, Office of Basic Energy Sciences
   [DE-SC0001091]
FX Financial support of this research was provided by the Robert A. Welch
   Foundation (BAK F-1464 and CBM F-1436) and the Air Force Research
   Laboratory (FA-8650-07-2-5061). V.C.H. acknowledges the Fannie and John
   Hertz Foundation and the NSF Graduate Research Fellowship Program for
   financial support. J.T.H. acknowledges financial support as part of the
   program "Understanding Charge Separation and Transfer at Interfaces in
   Energy Materials (EFRC:CST)," an Energy Frontier Research Center funded
   by the U.S. Department of Energy Office of Science, Office of Basic
   Energy Sciences, under Award No. DE-SC0001091.
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TC 54
Z9 54
U1 7
U2 182
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD JUN 7
PY 2012
VL 116
IS 22
BP 11917
EP 11923
DI 10.1021/jp302344b
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 953QY
UT WOS:000304888700010
ER

PT J
AU Tian, LL
   Zhuang, QC
   Li, J
   Wu, C
   Shi, YL
   Sun, SG
AF Tian, Leilei
   Zhuang, Quanchao
   Li, Jia
   Wu, Chao
   Shi, Yueli
   Sun, Shigang
TI The production of self-assembled Fe2O3-graphene hybrid materials by a
   hydrothermal process for improved Li-cycling
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Ferric oxide; Graphene; Hybrid materials; Lithium ion batteries; Cyclic
   performance
ID LITHIUM-ION BATTERIES; SIZED FE2O3-LOADED CARBON; ANODE MATERIAL;
   ELECTROCHEMICAL PROPERTIES; ELECTRODE MATERIALS; ALPHA-FE2O3; STORAGE;
   PERFORMANCE; NANOPARTICLES; OXIDE
AB An easy and effective strategy is developed to produce alpha-Fe2O3 nanoparticles (NPs) anchored on conducting graphene sheets by a hydrothermal reaction, without any reducing agents. Scanning electron microscopy shows that the alpha-Fe2O3 NPs are 70-85 nm in size and homogeneously anchored on the graphene sheets. As high-performance anodes for lithium-ion batteries, the obtained material exhibits an excellent reversible capacity of similar to 1050 mAh g(-1) based on the total mass. Its cycling performance and rate capability are drastically improved, exhibiting a high charge capacity of 1000 +/- 50 mAh g(-1) with no noticeable capacity fading up to 100 cycles in the voltage range 0.1-3.0V at 50 mA g(-1). These results highlight the importance of the anchoring of NPs on graphene sheets for maximum use of electrochemically active Fe2O3 NPs and graphene for energy storage applications. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Tian, Leilei; Zhuang, Quanchao; Li, Jia; Wu, Chao; Shi, Yueli] China Univ Min & Technol, Sch Mat Sci & Engn, Li Ion Batteries Lab, Xuzhou 221116, Peoples R China.
   [Tian, Leilei; Wu, Chao] China Univ Min &Technol, Sch Chem Engn & Technol, Xuzhou 221116, Peoples R China.
   [Sun, Shigang] Xiamen Univ, Coll Chem & Chem Engn, Dept Chem, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Peoples R China.
RP Zhuang, QC (reprint author), China Univ Min & Technol, Sch Mat Sci & Engn, Li Ion Batteries Lab, Xuzhou 221116, Peoples R China.
EM zhuangquanchao@126.com
RI Tian, Lei-Lei/H-9590-2012; SKL, PCOSS/D-4395-2013; Sun, S.G./G-3408-2010
OI Tian, Lei-Lei/0000-0001-5987-2944; 
FU Major State Basic Research Development Program of China [2009CB220102];
   Fundamental Research Funds for the Central Universities [2010LKHX03,
   2010QNB04, 2010QNB05]
FX This work was supported in part by financial supports from Major State
   Basic Research Development Program of China (2009CB220102) and the
   Fundamental Research Funds for the Central Universities (2010LKHX03,
   2010QNB04, 2010QNB05). The authors are grateful for assistance with SEM
   and XRD measurements from Dr. Rui Huang at Department of Chemistry,
   College of Chemistry and Chemical Engineering, Xiamen University.
CR Zou YQ, 2011, J PHYS CHEM C, V115, P20747, DOI 10.1021/jp206876t
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NR 40
TC 54
Z9 57
U1 14
U2 123
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD MAR 30
PY 2012
VL 65
BP 153
EP 158
DI 10.1016/j.electacta.2012.01.034
PG 6
WC Electrochemistry
SC Electrochemistry
GA 912NJ
UT WOS:000301806600022
ER

PT J
AU Lu, LQ
   Wang, Y
AF Lu, Li Qiang
   Wang, Yong
TI Facile synthesis of graphene-supported shuttle- and urchin-like CuO for
   high and fast Li-ion storage
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Anode materials; CuO; Graphene nanosheets; Lithium ion batteries
ID ELECTRODE MATERIALS; ANODE MATERIAL; BATTERIES; PERFORMANCE;
   MICROSPHERES; CAPACITY
AB Graphene nanosheet (GNS) supported shuttle- and urchin-like CuO nanostructures are prepared by a facile low-temperature solution route. CuO nanoshuttles or urchin-like nanostructures are dispersed uniformly on GNS, forming a three dimensional CuO-GNS layer-by-layer network after stacking. When fabricated as anode materials for lithium-ion batteries, CuO-GNS composites exhibit superior Li-ion storage properties in terms of high capacity, long cycle life, and excellent rate performance. At a large current of 700 mA/g, GNS-supported CuO nanoshuttles show a higher-than-theoretical capacity of 826 mAh/g after 100 cycles, which is even larger than the reversible capacity of 771 mAh/g achieved at 70 mA/g after 40 cycles. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Lu, Li Qiang; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
RP Wang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012
CR Wang B, 2010, J MATER CHEM, V20, P10661, DOI 10.1039/c0jm01941k
   Jung HR, 2011, ELECTROCHIM ACTA, V56, P6722, DOI 10.1016/j.electacta.2011.05.068
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NR 27
TC 54
Z9 56
U1 9
U2 138
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD JAN
PY 2012
VL 14
IS 1
BP 82
EP 85
DI 10.1016/j.elecom.2011.11.010
PG 4
WC Electrochemistry
SC Electrochemistry
GA 891EL
UT WOS:000300199900022
ER

PT J
AU Wen, ZH
   Cui, SM
   Kim, HJ
   Mao, S
   Yu, KH
   Lu, GH
   Pu, HH
   Mao, O
   Chen, JH
AF Wen, Zhenhai
   Cui, Shumao
   Kim, Haejune
   Mao, Shun
   Yu, Kehan
   Lu, Ganhua
   Pu, Haihui
   Mao, Ou
   Chen, Junhong
TI Binding Sn-based nanoparticles on graphene as the anode of rechargeable
   lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ELECTROCHEMICAL-BEHAVIOR; ALLOY ANODES; COMPOSITE; OXIDE; PERFORMANCE;
   ELECTRODES; CAPACITY
AB A facile method has been developed to synthesize Sn-based nanoparticle-decorated graphene through simultaneous growth of SnO2 nanoparticles and a carbonaceous polymer film on graphene oxide sheets followed by heat treatment at various temperatures (250, 550, 750, and 900 degrees C). Detailed characterization of the resulting composite material using transmission electron microscopy and field emission scanning electron microscopy suggests that Sn-based nanoparticles were reliably bound to the graphene surface through a carbon film. Cyclic voltammograms and galvanostatic technique were used to investigate electrochemical properties of the Sn-based composite material as the anode of lithium-ion batteries (LIBs). Samples obtained with 550 degrees C heat treatment, which contained mixed Sn-based components (Sn, SnO, SnO2), exhibit the best electrochemical performance among the series of nanocomposites in terms of specific capacity and cycling stability.
C1 [Wen, Zhenhai; Cui, Shumao; Kim, Haejune; Mao, Shun; Yu, Kehan; Lu, Ganhua; Pu, Haihui; Chen, Junhong] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA.
   [Mao, Ou] Johnson Controls Inc, Global Technol & Innovat, Power Solut, Milwaukee, WI 53209 USA.
RP Chen, JH (reprint author), Univ Wisconsin, Dept Mech Engn, 3200 N Cramer St, Milwaukee, WI 53211 USA.
EM jhchen@uwm.edu
RI wen, zhenhai/D-7165-2011; Yu, Kehan/H-3833-2011; Lu, Ganhua/B-4643-2010;
   Cui, Shumao/O-2987-2013; MAO, SHUN/G-9966-2015
OI wen, zhenhai/0000-0002-0397-4156; Lu, Ganhua/0000-0003-3279-8427; 
FU National Science Foundation [CMMI-0900509]; U.S. Department of Energy
   [DE-EE0003208]; Johnson Controls, Inc.; We Energies
FX The authors acknowledge financial support from the National Science
   Foundation (CMMI-0900509), the U.S. Department of Energy (DE-EE0003208),
   Johnson Controls, Inc., and We Energies.
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NR 43
TC 54
Z9 56
U1 16
U2 123
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 8
BP 3300
EP 3306
DI 10.1039/c2jm14999k
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 884HL
UT WOS:000299695400003
ER

PT J
AU Xiang, HF
   Tian, BB
   Lian, PC
   Li, Z
   Wang, HH
AF Xiang, Hongfa
   Tian, Bingbing
   Lian, Peichao
   Li, Zhong
   Wang, Haihui
TI Sol-gel synthesis and electrochemical performance of Li4Ti5O12/graphene
   composite anode for lithium-ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Li4Ti5O12; Graphene; Lithium-ion battery; Sol-gel; Safety
ID CARBON-COATED LI4TI5O12; REVERSIBLE CAPACITY; GRAPHENE NANOSHEETS;
   CYCLIC PERFORMANCE; ELECTRODE MATERIAL; DOPED LI4TI5O12; NANO-TUBES;
   SPINEL; STORAGE; CELLS
AB Li4Ti5O12/graphene composite was prepared by a facile sol-gel method. The lattice structure and morphology of the composite were investigated by X-ray diffraction (XRD) and scanning electronic microscopy (SEM). The electrochemical performances of the electrodes have been investigated compared with the pristine Li4Ti5O12 synthesized by a similar route. The Li4Ti5O12/graphene composite presents a higher capacity and better cycling performance than Li4Ti5O12 at the cutoff of 2.5-1.0 V, especially at high current rate. The excellent electrochemical performance of Li4Ti5O12/graphene electrode could be attributed to the improvement of electronic conductivity from the graphene sheets. When discharged to 0V, the Li4Ti5O12/graphene composite exhibited a quite high capacity over 274mAhg(-1) below 1.0 V, which was quite beneficial for not only the high energy density but also the safety characteristic of lithium-ion batteries. (C) 2011 Elsevier B. V. All rights reserved.
C1 [Xiang, Hongfa; Tian, Bingbing; Lian, Peichao; Li, Zhong; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
EM hhwang@scut.edu.cn
RI Xiang, Hongfa/I-5126-2012
OI Xiang, Hongfa/0000-0002-6182-1932
FU National Science Foundation of China [21006033]; Program for New Century
   Excellent Talents in Chinese Ministry of Education [NECT-07-0307];
   Fundamental Research Funds for the Central Universities, SCUT
   [2009220038]
FX This work was supported by National Science Foundation of China (grant
   no. 21006033), Program for New Century Excellent Talents in Chinese
   Ministry of Education (No. NECT-07-0307) and the Fundamental Research
   Funds for the Central Universities, SCUT (2009220038).
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NR 36
TC 54
Z9 55
U1 13
U2 119
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD JUN 30
PY 2011
VL 509
IS 26
BP 7205
EP 7209
DI 10.1016/j.jallcom.2011.04.065
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 769II
UT WOS:000291005700004
ER

PT J
AU Wu, P
   Wang, H
   Tang, YW
   Zhou, YM
   Lu, TH
AF Wu, Ping
   Wang, Hui
   Tang, Yawen
   Zhou, Yiming
   Lu, Tianhong
TI Three-Dimensional Interconnected Network of Graphene-Wrapped Porous
   Silicon Spheres: In Situ Magnesiothermic-Reduction Synthesis and
   Enhanced Lithium-Storage Capabilities
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium-ion batteries; anodes; silicon; graphene; interconnected
   network; magnesiothermic reduction
ID LI-ION BATTERIES; SI/C COMPOSITE NANOFIBERS; HIGH-PERFORMANCE ANODE;
   NANOSTRUCTURED SILICON; MESOPOROUS SILICON; CONDUCTIVE NETWORK;
   NANOCOMPOSITE; NANOPARTICLES; ARCHITECTURE; NANOCABLES
AB A novel type of 3D porous Si-G micro/nanostructure (i.e., 3D interconnected network of graphene-wrapped porous silicon spheres, Si@G network) was constructed through layer-by-layer assembly and subsequent in situ magnesiothermic-reduction methodology. Compared with bare Si spheres, the as-synthesized Si@G network exhibits markedly enhanced anodic performance in terms of specific capacity, cycling stability, and rate capability, making it an ideal anode candidate for high-energy, long-life, and high-power lithium-ion batteries.
C1 [Wu, Ping; Wang, Hui; Tang, Yawen; Zhou, Yiming; Lu, Tianhong] Nanjing Normal Univ, Sch Chem & Mat Sci, Jiangsu Collaborat Innovat Ctr Biomed Funct Mat, Jiangsu Key Lab New Power Batteries, Nanjing 210023, Peoples R China.
RP Wu, P (reprint author), Nanjing Normal Univ, Sch Chem & Mat Sci, Jiangsu Collaborat Innovat Ctr Biomed Funct Mat, Jiangsu Key Lab New Power Batteries, Nanjing 210023, Peoples R China.
EM zjuwuping@njnu.edu.cn; zhouyiming@njnu.edu.cn
RI Zhou, Yiming/G-6079-2014; Tang, Yawen/B-7431-2013
FU Natural Science Foundation of Jiangsu Province [BK20130900]; Natural
   Science Foundation of Jiangsu Higher Education Institutions of China
   [13KJB150026]; Industry-Academia Cooperation Innovation Fund Project of
   Jiangsu Province [BY2013001-01, BY2012001]; Priming Scientific Research
   Foundation for Advanced Talents in Nanjing Normal University
   [2013103XGQ0008]; Priority Academic Program Development of Jiangsu
   Higher Education Institutions
FX We appreciate the financial support from the Natural Science Foundation
   of Jiangsu Province (BK20130900), the Natural Science Foundation of
   Jiangsu Higher Education Institutions of China (13KJB150026), the
   Industry-Academia Cooperation Innovation Fund Project of Jiangsu
   Province (BY2013001-01 and BY2012001), the Priming Scientific Research
   Foundation for Advanced Talents in Nanjing Normal University
   (2013103XGQ0008), and a project funded by the Priority Academic Program
   Development of Jiangsu Higher Education Institutions.
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NR 37
TC 53
Z9 53
U1 45
U2 259
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAR 12
PY 2014
VL 6
IS 5
BP 3546
EP 3552
DI 10.1021/am405725u
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA AD0KM
UT WOS:000332922900064
PM 24506494
ER

PT J
AU Mai, YJ
   Tu, JP
   Gu, CD
   Wang, XL
AF Mai, Y. J.
   Tu, J. P.
   Gu, C. D.
   Wang, X. L.
TI Graphene anchored with nickel nanoparticles as a high-performance anode
   material for lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene; Nickel nanoparticles; Anode; Lithium ion battery
ID ELECTROCHEMICAL IMPEDANCE; SURFACE MODIFICATION; REVERSIBLE CAPACITY;
   GRAPHITE-ELECTRODES; LI STORAGE; OXIDE; COMPOSITE; INSERTION;
   NANOSHEETS; CARBONS
AB The surface of graphene is modified by nickel nanoparticles which are in-situ reduced from NiO nanopartidies by graphene. The nickel nanoparticles obtained are up to 10 nm in size and are strongly anchored on the surface of graphene sheets. As an anode material for lithium ion batteries, the graphene-Ni hybrid material delivers a reversible capacity of 675 mAh g(-1) after 35 discharge/charge cycles at a current density of 100 mA g(-1), corresponding to 85% retention of the initial charge capacity. In addition, the graphene-Ni hybrid electrode exhibits much better rate capability compared to its pure counterpart operated at various rates between 200 and 800 mA g(-1). Such enhanced lithium storage performance of the graphene-Ni hybrid electrode can be ascribed to the enhanced electronic transport and Li+ migration through the solid electrolyte interphase (SEI) film as a consequence of that the anchored nickel nanoparticles increase the electronic conductivity and modify the structure of SEI film covering the surface of graphene. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Tu, J. P.] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
RP Tu, JP (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
EM tujp@zju.edu.cn
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NR 46
TC 53
Z9 56
U1 10
U2 124
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JUL 1
PY 2012
VL 209
BP 1
EP 6
DI 10.1016/j.jpowsour.2012.02.073
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 937XZ
UT WOS:000303698800001
ER

PT J
AU Chen, Y
   Song, BH
   Tang, XS
   Lu, L
   Xue, JM
AF Chen, Yu
   Song, Bohang
   Tang, Xiaosheng
   Lu, Li
   Xue, Junmin
TI One-step synthesis of hollow porous Fe3O4 beads-reduced graphene oxide
   composites with superior battery performance
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; CAPACITY ANODE MATERIAL; REVERSIBLE CAPACITY;
   CYCLIC PERFORMANCE; HIGH-POWER; STORAGE; NANOPARTICLES; LI; ELECTRODES;
   NANOSHEETS
AB We report the synthesis of a novel hollow porous Fe3O4 bead-rGO composite structure for lithium ion battery anode application via a facile solvothermal route. The formation of hollow porous Fe3O4 beads and reduction of graphene oxide (GO) into rGO were accomplished in one step by using ethylene glycol (EG) as a reducing agent. In this composite structure, the hollow porous Fe3O4 beads were either chemically attached or tightly wrapped with rGO sheets, leading to a strong synergistic effect between them. As a result, the obtained Fe3O4-rGO composite electrodes could deliver a reversible capacity of 1039 mA h g(-1) after 170 cycles between 3 V and 50 mV at a current density of 100 mA g(-1), with an increment of 30% compared to their initial reversible capacity, demonstrating their superior cycling stability.
C1 [Chen, Yu; Tang, Xiaosheng; Xue, Junmin] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
   [Song, Bohang; Lu, Li] Natl Univ Singapore, Dept Mech Engn, Singapore 117576, Singapore.
RP Xue, JM (reprint author), Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
EM msexuejm@nus.edu.sg
RI Song, Bohang/F-8239-2016
OI Song, Bohang/0000-0002-6477-609X
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NR 39
TC 53
Z9 54
U1 18
U2 116
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 34
BP 17656
EP 17662
DI 10.1039/c2jm32057f
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 985YF
UT WOS:000307305700040
ER

PT J
AU Wu, YP
   Jiang, C
   Wan, C
   Holze, R
AF Wu, YP
   Jiang, C
   Wan, C
   Holze, R
TI Anode materials for lithium ion batteries by oxidative treatment of
   common natural graphite
SO SOLID STATE IONICS
LA English
DT Article
DE lithium ion batteries; natural graphite; oxidation; anode materials
ID INITIAL IRREVERSIBLE CAPACITY; ELECTROCHEMICAL PERFORMANCE; SURFACE
   MODIFICATION; SECONDARY BATTERIES; NEGATIVE ELECTRODE; CARBON;
   COMPOSITE; COKE
AB Modification of graphite has recently moved into the focus of the preparation of anode materials for lithium ion batteries. We report on an oxidative treatment by air and concentrated nitric acid solution to improve the electrochemical performance of a common natural graphite. Results from X-ray photoelectron spectroscopy (XPS), electron paramagnetic resonance (EPR), thermogravimmetry (TG) and differential thermal analysis (DTA), high resolution electron microscopy (HREM), and measurements of the reversible electrochemical capacity suggest that the surface structure of natural graphite is changed and a fresh dense layer of oxides is formed. Structural imperfections are removed and the stability of the graphite structure is increased. These changes inhibit electrolyte decomposition, block intercalation of solvated lithium ions and prevent graphene planes from moving along the a-axis direction. In addition, nanochannels and micropores are introduced, and thus, lithium intercalation and deintercalation are favored and more sites are provided for lithium storage. Consequently, reversible capacity and cycling behavior of the modified natural graphite through the oxidation treatments is improved considerably. Since common natural graphite is low in cost, this method is promising for industrial application. (C) 2003 Elsevier Science B.V. All rights reserved.
C1 Tech Univ Chem, Inst Chem, AG Elektrochem, D-09107 Chemnitz, Germany.
   Tsing Hua Univ, INET, Div Chem Engn, Beijing 102201, Peoples R China.
RP Wu, YP (reprint author), Tech Univ Chem, Inst Chem, AG Elektrochem, D-09107 Chemnitz, Germany.
RI Wu, Yuping/H-1593-2011
OI Wu, Yuping/0000-0002-0833-1205
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NR 32
TC 53
Z9 57
U1 4
U2 31
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0167-2738
J9 SOLID STATE IONICS
JI Solid State Ion.
PD JAN
PY 2003
VL 156
IS 3
BP 283
EP 290
AR PII S0167-2738(02)00680-X
DI 10.1016/S0167-2738(02)00680-X
PG 8
WC Chemistry, Physical; Physics, Condensed Matter
SC Chemistry; Physics
GA 642BW
UT WOS:000180785300005
ER

PT J
AU Sun, J
   Zheng, GY
   Lee, HW
   Liu, N
   Wang, HT
   Yao, HB
   Yang, WS
   Cui, Y
AF Sun, Jie
   Zheng, Guangyuan
   Lee, Hyun-Wook
   Liu, Nian
   Wang, Haotian
   Yao, Hongbin
   Yang, Wensheng
   Cui, Yi
TI Formation of Stable Phosphorus-Carbon Bond for Enhanced Performance in
   Black Phosphorus Nanoparticle-Graphite Composite Battery Anodes
SO NANO LETTERS
LA English
DT Article
DE Black phosphorus; carbon; phosphorus-carbon bond; reversible cycle;
   lithium-ion batteries
ID LITHIUM-ION BATTERIES; FIELD-EFFECT TRANSISTORS; HIGH-CAPACITY;
   ELECTROCHEMICAL ACTIVITY; GRAPHENE; STORAGE; RAMAN; FILMS; RED; SN
AB High specific capacity battery electrode materials have attracted great research attention. Phosphorus as a low-cost abundant material has a high theoretical specific capacity of 2596 mAh/g with most of its capacity at the discharge potential range of 0.4-1.2 V, suitable as anodes. Although numerous research progress have shown other high capacity anodes such as Si, Ge, Sn, and SnO2, there are only a few studies on phosphorus anodes despite its high theoretical capacity. Successful applications of phosphorus anodes have been impeded by rapid capacity fading, mainly caused by large volume change (around 300%) upon lithiation and thus loss of electrical contact. Using the conducting allotrope of phosphorus, "black phosphorus" as starting materials, here we fabricated composites of black phosphorus nanopartide-graphite by mechanochemical reaction in a high energy mechanical milling process. This process produces phosphorus-carbon bonds, which are stable during lithium insertion/extraction, maintaining excellent electrical connection between phosphorus and carbon. We demonstrated high initial discharge capacity of 2786 mAh.g(-1) at 0.2 C and an excellent cycle life of 100 cycles with 80% capacity retention. High specific discharge capacities are maintained at fast C rates (2270, 1750, 1500, and 1240 mAh.g(-1) at C/5, 1, 2, and 4.5 C, respectively).
C1 [Sun, Jie; Lee, Hyun-Wook; Yao, Hongbin; Cui, Yi] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA.
   [Zheng, Guangyuan] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA.
   [Liu, Nian] Stanford Univ, Dept Chem, Stanford, CA 94305 USA.
   [Wang, Haotian] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA.
   [Cui, Yi] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
   [Sun, Jie; Yang, Wensheng] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
RP Yang, WS (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
EM yangws@mail.buct.edu.cn; yicui@stanford.edu
RI zheng, guangyuan/K-6931-2014; Yao, Hongbin/B-8347-2011; 
OI zheng, guangyuan/0000-0003-0286-5908; Lee, Hyun-Wook/0000-0001-9074-1619
FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials
   Sciences and Engineering Division [DE-AC02-76-SFO0515]; National Natural
   Science Foundation of China [51272020, 21236003]; National Research
   Foundation of Korea (NRF) - Ministry of Education, Science and
   Technology [NRF-2012R1A6A3A03038593]
FX We acknowledge the support by the U.S. Department of Energy, Office of
   Basic Energy Sciences, Materials Sciences and Engineering Division,
   under Contract DE-AC02-76-SFO0515. W.Y. acknowledges support from the
   National Natural Science Foundation of China under 51272020 and
   21236003. H.W.L.acknowledges support from the Basic Science Research
   Program through the National Research Foundation of Korea (NRF) funded
   by the Ministry of Education, Science and Technology under
   NRF-2012R1A6A3A03038593.
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NR 51
TC 52
Z9 52
U1 115
U2 359
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD AUG
PY 2014
VL 14
IS 8
BP 4573
EP 4580
DI 10.1021/nl501617j
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AN2WH
UT WOS:000340446200057
PM 25019417
ER

PT J
AU Huang, GC
   Chen, T
   Wang, Z
   Chang, K
   Chen, WX
AF Huang, Guochuang
   Chen, Tao
   Wang, Zhen
   Chang, Kun
   Chen, Weixiang
TI Synthesis and electrochemical performances of cobalt sulfides/graphene
   nanocomposite as anode material of Li-ion battery
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Cobalt sulfides/graphene composite; Graphene oxide sheets; Lithium ion
   battery; Solvothermal route
ID CARBON NANOTUBES; LITHIUM; GRAPHENE; SULFIDE; HYBRID; CO9S8;
   NANOPARTICLES; COMPOSITES; ELECTRODE; POLYMER
AB The cobalt sulfides/graphene nanosheets (GNS) composite is prepared by a facile one-pot solvothermal route in the presence of graphene oxide sheets (GOS). XRD, SEM and TEM characterizations show that sphere-like cobalt sulfides particles with an average size of about 150 nm, which are complicated phases of CoS2, CoS and Co9S8, are highly dispersed on or wrapped in the creasy graphene. The selective nucleation and growth of cobalt sulfides particles on GOS make the particles more uniform in morphology and size. The as-fabricated cobalt sulfides/GNS composite exhibits very high electrochemical lithium storage reversible capacity of about 1018 mAh g(-1). Moreover, the cobalt sulfides/GNS composite still remains reversible capacity of above 950 mAh g(-1) after 50 cycles at a current density of 100 mA g(-1) as well as at the different current densities from 100 to 1000 mA g(-1), proving its excellent cycling durability and high-rate capability. The superior electrochemical performances of the composite may be attributed to the robust composite structure and superior conductivity, high charger mobility, large surface area and good flexibility of graphene. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Huang, Guochuang; Wang, Zhen; Chang, Kun; Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
   [Chen, Tao] Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China.
RP Chen, WX (reprint author), Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
EM weixiangchen@zju.edu.cn
FU Natural Science Foundation of China [21173190]; International Science
   and Technology Cooperation Program of China [2012DFG42100]; Doctoral
   Program of Higher Education of China [2011010113003]; Zhejiang
   Provincial Natural Science Foundation of China [Y4100119]; Science and
   Technology Department of Zhejiang Province [2011C21024]
FX This work is financially supported by the Natural Science Foundation of
   China (21173190), the International Science and Technology Cooperation
   Program of China (2012DFG42100), the Doctoral Program of Higher
   Education of China (2011010113003), the Zhejiang Provincial Natural
   Science Foundation of China (Y4100119) and the Science and Technology
   Department of Zhejiang Province (2011C21024).
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NR 41
TC 52
Z9 53
U1 62
U2 592
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD AUG 1
PY 2013
VL 235
BP 122
EP 128
DI 10.1016/j.jpowsour.2013.01.093
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 134HF
UT WOS:000318200300018
ER

PT J
AU Zhou, XS
   Cao, AM
   Wan, LJ
   Guo, YG
AF Zhou, Xiaosi
   Cao, An-Min
   Wan, Li-Jun
   Guo, Yu-Guo
TI Spin-coated silicon nanoparticle/graphene electrode as a binder-free
   anode for high-performance lithium-ion batteries
SO NANO RESEARCH
LA English
DT Article
DE Spin-coating; binder-free anode; silicon nanoparticles; graphene;
   lithium-ion batteries
ID HIGH-CAPACITY; GRAPHENE OXIDE; STORAGE PERFORMANCE; COLLOIDAL CRYSTALS;
   CARBON NANOTUBES; RATE CAPABILITY; LI; SI; NANOCOMPOSITE; ARCHITECTURE
AB Si has been considered as a promising anode material but its practical application has been severely hindered due to poor cyclability caused by the large volume change during charge/discharge. A new and effective protocol has been developed to construct Si nanoparticle/graphene electrodes with a favorable structure to alleviate this problem. Starting from a stable suspension of Si nanoparticles and graphene oxide in ethanol, spin-coating can be used as a facile method to cast a spin-coated Si nanoparticle/graphene (SC-Si/G) film, in which graphene can act as both an efficient electronic conductor and effective binder with no need for other binders such as polyvinylidenefluoride (PVDF) or polytetrafluoroethylene (PTFE). The prepared SC-Si/G electrode can achieve a high-performance as an anode for lithium-ion batteries benefiting from the following advantages: i) the graphene enhances the electronic conductivity of Si nanoparticles and the void spaces between Si nanoparticles facilitate the lithium ion diffusion, ii) the flexible graphene and the void spaces can effectively cushion the volume expansion of Si nanoparticles. As a result, the binder-free electrode shows a high capacity of 1611 mA center dot h center dot g(-1) at 1 A center dot g(-1) after 200 cycles, a superior rate capability of 648 mA center dot h center dot g(-1) at 10 A center dot g(-1), and an excellent cycle life of 200 cycles with 74% capacity retention.
C1 [Zhou, Xiaosi; Cao, An-Min; Wan, Li-Jun; Guo, Yu-Guo] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2012CB932900, 2011CB935700,
   2009CB930400]; National Natural Science Foundation of China [91127044,
   21121063]; Chinese Academy of Sciences
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2012CB932900, 2011CB935700, and 2009CB930400), the National
   Natural Science Foundation of China (Grant Nos. 91127044 and 21121063),
   and the Chinese Academy of Sciences.
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NR 62
TC 52
Z9 52
U1 28
U2 276
PU TSINGHUA UNIV PRESS
PI BEIJING
PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA
SN 1998-0124
J9 NANO RES
JI Nano Res.
PD DEC
PY 2012
VL 5
IS 12
BP 845
EP 853
DI 10.1007/s12274-012-0268-4
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 055HR
UT WOS:000312406700002
ER

PT J
AU Zhao, YC
   Song, XY
   Song, QS
   Yin, ZL
AF Zhao, Youcheng
   Song, Xinyu
   Song, Qisheng
   Yin, Zhilei
TI A facile route to the synthesis copper oxide/reduced graphene oxide
   nanocomposites and electrochemical detection of catechol organic
   pollutant
SO CRYSTENGCOMM
LA English
DT Article
ID LITHIUM-ION BATTERIES; QUICK-PRECIPITATION METHOD; EXFOLIATED GRAPHITE
   OXIDE; IN-SITU FORMATION; ANODE MATERIAL; CHEMICAL-REDUCTION; CUO
   NANOPARTICLES; LARGE-AREA; COMPOSITE; CARBON
AB A simple and efficient approach of preparing copper oxide/reduced graphene oxide (CuO/rGO) nanocomposite has been demonstrated. CuO/rGO nanocomposites were successfully synthesized through a one-step redox reaction between graphene oxide (GO) sheets and cuprous ions in CuCl without extra reducing agent. Notably, the reduction of GO and the deposition of CuO on the rGO sheets occurred simultaneously during the reaction process, resulting in a uniform and tight distribution of CuO nanoparticles on the reduced GO sheets. Furthermore, the as-prepared CuO/rGO composite (CuCl = 0.02 g) had a large BET surface area (235 m(2) g(-1)) and a porous structure with macropores and mesopores. The as-prepared nanocomposite was exploited in the catalytic oxidation of catechol in aqueous media. The results indicated that the as-prepared copper oxide/rGO nanocomposite exhibited a higher electrocatalytic activity towards catechol oxidation than original CuO nanoparticles or reduced graphene oxide samples. This strategy opens a new facile and simple chemical route to synthesize copper oxide/rGO nanocomposites with excellent properties.
C1 [Zhao, Youcheng; Song, Xinyu; Song, Qisheng; Yin, Zhilei] Shandong Univ, Dept Chem, Jinan 250100, Peoples R China.
RP Song, XY (reprint author), Shandong Univ, Dept Chem, Jinan 250100, Peoples R China.
EM songxy@sdu.edu.cn
FU  [NSFC91022034/E0201]
FX This work was supported by the NSFC91022034/E0201.
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NR 68
TC 52
Z9 52
U1 27
U2 122
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1466-8033
J9 CRYSTENGCOMM
JI Crystengcomm
PY 2012
VL 14
IS 20
BP 6710
EP 6719
DI 10.1039/c2ce25509j
PG 10
WC Chemistry, Multidisciplinary; Crystallography
SC Chemistry; Crystallography
GA 006NY
UT WOS:000308827100053
ER

PT J
AU Chen, SQ
   Chen, P
   Wang, Y
AF Chen, Shuangqiang
   Chen, Peng
   Wang, Yong
TI Carbon nanotubes grown in situ on graphene nanosheets as superior anodes
   for Li-ion batteries
SO NANOSCALE
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; LITHIUM STORAGE; SUPERCAPACITORS;
   NANOSTRUCTURES; ELECTRODE; SHEETS; FILMS
AB Graphene and carbon nanotubes are intriguing alternative anode materials for lithium ion batteries. The prevention of graphene restacking and facilitation of lithium diffusion into CNTs with large aspect ratio are highly desirable for the performance enhancements including capacity, cycliability and rate capability. In this work, we demonstrated that a multilayered graphene-CNT hybrid nanostructure was able to hold such merits. GNS were separated and stabilized by CNTs grown in situ on GNS surface. The length of CNTs was found to be a key factor to the electrochemical performances. The GNS-CNT composite with the shortest CNT decoration displayed highly reversible capacities of 573 mAh g(-1) at a small current of 0.2C and 520 mAh g(-1) at a large current of 2C. The growth and lithium storage mechanism for graphene-CNT composite was also proposed.
C1 [Chen, Shuangqiang; Chen, Peng; Wang, Yong] Shanghai Univ, Dept Chem Engn, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
RP Wang, Y (reprint author), Shanghai Univ, Dept Chem Engn, Sch Environm & Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012; Chen, Shuangqiang/F-5289-2013
FU Shanghai Institutions of Higher Learning; Shanghai Municipal Government
   [09JC1406100, S30109]; National Natural Science Foundation of China
   [50971085]
FX The authors gratefully acknowledge the Program for Professor of Special
   Appointment (Eastern Scholar) at Shanghai Institutions of Higher
   Learning, National Natural Science Foundation of China (50971085), and
   Shanghai Municipal Government (09JC1406100, S30109) for the financial
   support.
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NR 39
TC 52
Z9 54
U1 21
U2 111
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2011
VL 3
IS 10
BP 4323
EP 4329
DI 10.1039/c1nr10642b
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 829XB
UT WOS:000295618200050
PM 21879120
ER

PT J
AU Lin, J
   Raji, ARO
   Nan, KW
   Peng, ZW
   Yan, Z
   Samuel, ELG
   Natelson, D
   Tour, JM
AF Lin, Jian
   Raji, Abdul-Rahman O.
   Nan, Kewang
   Peng, Zhiwei
   Yan, Zheng
   Samuel, Errol L. G.
   Natelson, Douglas
   Tour, James M.
TI Iron Oxide Nanoparticle and Graphene Nanoribbon Composite as an Anode
   Material for High- Performance Li-Ion Batteries
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE graphene nanoribbons; iron oxide; anodes; Li-ion batteries
ID LITHIUM STORAGE; CAPACITY; MAGNETITE; ELECTRODE; HEMATITE; FILMS
AB A composite material made of graphene nanoribbons and iron oxide nanoparticles provides a remarkable route to lithium-ion battery anode with high specific capacity and cycle stability. At a rate of 100 mA/g, the material exhibits a high discharge capacity of similar to 910 mAh/g after 134 cycles, which is >90% of the theoretical li-ion storage capacity of iron oxide. Carbon black, carbon nanotubes, and graphene flakes have been employed by researchers to achieve conductivity and stability in lithium-ion electrode materials. Herein, the use of graphene nanoribbons as a conductive platform on which iron oxide nanoparticles are formed combines the advantages of long carbon nanotubes and flat graphene surfaces. The high capacity over prolonged cycling achieved is due to the synergy between an electrically percolating networks of conductive graphene nanoribbons and the high lithium-ion storage capability of iron oxide nanoparticles.
C1 [Raji, Abdul-Rahman O.; Peng, Zhiwei; Yan, Zheng; Samuel, Errol L. G.; Tour, James M.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
   [Natelson, Douglas] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA.
   [Lin, Jian; Nan, Kewang; Tour, James M.] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77005 USA.
   [Lin, Jian; Natelson, Douglas; Tour, James M.] Rice Univ, Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA.
RP Lin, J (reprint author), Rice Univ, Smalley Inst Nanoscale Sci & Technol, 6100 Main St, Houston, TX 77005 USA.
EM natelson@rice.edu; tour@rice.edu
FU Boeing; AFOSR MURI [FA9550-12-1-0035]; AFOSR [FA9550-09-1-0581]; Sandia
   National Laboratory [1100745]; ONR MURI [00006766, N00014-09-1-1066]
FX J. Lin and A.-R. O. Raji contributed equally to this work. Funding for
   this research was provided by Boeing, the AFOSR MURI (FA9550-12-1-0035),
   the AFOSR (FA9550-09-1-0581), Sandia National Laboratory (1100745) and
   the ONR MURI program (#00006766, N00014-09-1-1066).
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NR 30
TC 51
Z9 51
U1 30
U2 185
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD APR
PY 2014
VL 24
IS 14
BP 2044
EP 2048
DI 10.1002/adfm.201303023
PG 5
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AE2NG
UT WOS:000333809300010
ER

PT J
AU Guo, Q
   Zheng, Z
   Gao, HL
   Ma, J
   Qin, X
AF Guo, Qi
   Zheng, Zhe
   Gao, Hailing
   Ma, Jia
   Qin, Xue
TI SnO2/graphene composite as highly reversible anode materials for lithium
   ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Tin oxide; Graphene; Composite; Lithium-ion batteries
ID GRAPHENE NANOSHEETS; STORAGE; SNO2; OXIDE; NANOCOMPOSITE; CAPACITY;
   PERFORMANCE; MORPHOLOGY
AB Tin oxide (SnO2)/graphene composite is synthesized via a simple wet chemical method using graphene oxide and SnCl2 center dot 2H(2)O as raw materials. Graphene of high reduction degree in the composite can provide high conductivity and large-current discharge capacity. SnO2 nanoparticles with dimension around 5 nm are uniformly distributed on the graphene matrix.
   The SnO2/graphene composite exhibits outstanding electrochemical performance such as high reversible capacities, good cycling stability and excellent high-rate discharge performance. The initial discharge and charge capacities are 1995.8 mAh g(-1) and 1923.5 mAh g(-1), respectively. After 40 cycles, the reversible discharge capacity is still maintained at 1545.7 mAh g(-1) at the current density of 1 A g(-1), indicating that the composite is a promising alternative anode material used for high-storage lithium ion batteries. Crown Copyright (C) 2013 Published by Elsevier B.V. All rights reserved.
C1 [Guo, Qi; Zheng, Zhe; Gao, Hailing; Ma, Jia; Qin, Xue] Tianjin Univ, Sch Sci, Tianjin 300072, Peoples R China.
RP Qin, X (reprint author), Tianjin Univ, Sch Sci, 92 Weijin Rd, Tianjin 300072, Peoples R China.
EM qinxue@tju.edu.cn
FU National Natural Science Foundation of China [20603024]; Open Project of
   Key Lab Adv. Energy Mat. Chem. (Nankai Univ.) [KLAEMC-OP201201]
FX The authors gratefully acknowledge the financial support from the
   National Natural Science Foundation of China (20603024) and the Open
   Project of Key Lab Adv. Energy Mat. Chem. (Nankai Univ.)
   (KLAEMC-OP201201).
CR Masao A, 2009, ELECTROCHEM SOLID ST, V12, pB119, DOI 10.1149/1.3152325
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NR 24
TC 51
Z9 51
U1 13
U2 314
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD OCT 15
PY 2013
VL 240
BP 149
EP 154
DI 10.1016/j.jpowsour.2013.03.116
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 183GY
UT WOS:000321803700020
ER

PT J
AU Wen, Y
   Zhu, YJ
   Langrock, A
   Manivannan, A
   Ehrman, SH
   Wang, CS
AF Wen, Yang
   Zhu, Yujie
   Langrock, Alex
   Manivannan, Ayyakkannu
   Ehrman, Sheryl H.
   Wang, Chunsheng
TI Graphene-Bonded and -Encapsulated Si Nanoparticles for Lithium Ion
   Battery Anodes
SO SMALL
LA English
DT Article
DE silicon; graphene; lithium-ion batteries; aerosols; nanocomposites
ID HIGH-CAPACITY; COMPOSITE ELECTRODE; OXIDE
AB Silicon (Si) has been considered a very promising anode material for lithium ion batteries due to its high theoretical capacity. However, high-capacity Si nanoparticles usually suffer from low electronic conductivity, large volume change, and severe aggregation problems during lithiation and delithiation. In this paper, a unique nanostructured anode with Si nanoparticles bonded and wrapped by graphene is synthesized by a one-step aerosol spraying of surface-modified Si nanoparticles and graphene oxide suspension. The functional groups on the surface of Si nanoparticles (50-100 nm) not only react with graphene oxide and bind Si nanoparticles to the graphene oxide shell, but also prevent Si nanoparticles from aggregation, thus contributing to a uniform Si suspension. A homogeneous graphene-encapsulated Si nanoparticle morphology forms during the aerosol spraying process. The open-ended graphene shell with defects allows fast electrochemical lithiation/delithiation, and the void space inside the graphene shell accompanied by its strong mechanical strength can effectively accommodate the volume expansion of Si upon lithiation. The graphene shell provides good electronic conductivity for Si nanoparticles and prevents them from aggregating during charge/discharge cycles. The functionalized Si encapsulated by graphene sample exhibits a capacity of 2250 mAh g(-1) (based on the total mass of graphene and Si) at 0.1C and 1000 mAh g(-1) at 10C, and retains 85% of its initial capacity even after 120 charge/discharge cycles. The exceptional performance of graphene-encapsulated Si anodes combined with the scalable and one-step aerosol synthesis technique makes this material very promising for lithium ion batteries.
C1 [Wen, Yang; Zhu, Yujie; Langrock, Alex; Ehrman, Sheryl H.; Wang, Chunsheng] Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA.
   [Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA.
RP Wang, CS (reprint author), Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA.
EM cswang@umd.edu
RI Wang, Chunsheng/H-5767-2011; Langrock, Alex/E-8567-2015
OI Wang, Chunsheng/0000-0002-8626-6381; 
FU Department of Energy [DESC0001160]; Maryland NanoCenter and its NispLab;
   Exploratory Technology Research
FX The authors acknowledge financial support from the Department of Energy
   (DESC0001160) under the project science of precision multifunctional
   nanostructures for electrical energy storage, the Exploratory Technology
   Research. We also acknowledge the support of the Maryland NanoCenter and
   its NispLab.
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NR 26
TC 51
Z9 51
U1 23
U2 223
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD AUG 26
PY 2013
VL 9
IS 16
BP 2810
EP 2816
DI 10.1002/smll.201202512
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 262MD
UT WOS:000327738600021
PM 23440956
ER

PT J
AU Fei, L
   Lin, QL
   Yuan, B
   Chen, G
   Xie, P
   Li, YL
   Xu, Y
   Deng, SG
   Smirnov, S
   Luo, HM
AF Fei, Ling
   Lin, Qianglu
   Yuan, Bin
   Chen, Gen
   Xie, Pu
   Li, Yuling
   Xu, Yun
   Deng, Shuguang
   Smirnov, Sergei
   Luo, Hongmei
TI Reduced Graphene Oxide Wrapped FeS Nanocomposite for Lithium-Ion Battery
   Anode with Improved Performance
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE FeS; reduced graphene oxide; nanocomposite; lithium-ion battery
ID STORAGE PROPERTIES; HIGH-CAPACITY; ELECTROCHEMICAL PERFORMANCES;
   SECONDARY BATTERIES; SULFUR BATTERIES; CARBON; NANOPARTICLES;
   NANOSTRUCTURES; COMPOSITES; ELECTRODES
AB A new nanocomposite formulation of the FeS-based anode for lithium-ion batteries is proposed, where FeS nanoparticles wrapped in reduced graphene oxide (RGO) are produced via a facile direct-precipitation approach. The resulting nanocomposite FeS@RGO structure has better lithium ion storage properties, exceeding those of FeS prepared without RGO sheets. The enhanced electrochemical performance is attributed to the robust sheet-wrapped structure with smaller FeS nanoparticles and synergetic effects between FeS and RGO sheets, such as increased conductivity, shortened lithium ion diffusion path, and the effective prevention of polysulfide dissolution.
C1 [Fei, Ling; Lin, Qianglu; Yuan, Bin; Chen, Gen; Li, Yuling; Xu, Yun; Deng, Shuguang; Luo, Hongmei] New Mexico State Univ, Dept Chem Engn, Las Cruces, NM 88003 USA.
   [Xie, Pu] New Mexico State Univ, Dept Mech & Aerosp Engn, Las Cruces, NM 88003 USA.
   [Smirnov, Sergei] New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA.
RP Luo, HM (reprint author), New Mexico State Univ, Dept Chem Engn, Las Cruces, NM 88003 USA.
EM hluo@nmsu.edu
RI Deng, Shuguang/G-5926-2011; CHEN, GEN/K-9436-2014
OI Deng, Shuguang/0000-0003-2892-3504; CHEN, GEN/0000-0003-3504-3572
FU NSF [1131290]; Graduate School at NMSU
FX We thank Dr. Peter Cooke for helping with SEM and acknowledge the
   funding support from the NSF under Grant No. 1131290. L.F. acknowledges
   the Preparing Future Faculty Award from the Graduate School at NMSU.
CR Zhang BA, 2011, CARBON, V49, P4524, DOI 10.1016/j.carbon.2011.06.059
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NR 39
TC 51
Z9 51
U1 43
U2 216
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD JUN 12
PY 2013
VL 5
IS 11
BP 5330
EP 5335
DI 10.1021/am401239f
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 165KY
UT WOS:000320484000112
PM 23673403
ER

PT J
AU Wang, J
   Zhou, J
   Hu, YF
   Regier, T
AF Wang, Jian
   Zhou, Jigang
   Hu, Yongfeng
   Regier, Tom
TI Chemical interaction and imaging of single Co3O4/graphene sheets studied
   by scanning transmission X-ray microscopy and X-ray absorption
   spectroscopy
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID LITHIUM ION BATTERIES; PERFORMANCE ANODE MATERIALS; WALLED CARBON
   NANOTUBES; COBALT OXIDE; REVERSIBLE CAPACITY; GRAPHENE; CO3O4;
   NANOPARTICLES; FABRICATION; ELECTRODES
AB Scanning transmission X-ray microscopy (STXM) has been used to investigate the chemical, electronic and structural nature of Co3O4 nanocrystals grown on single nitrogen-doped graphene sheets through spatially resolved X-ray absorption near edge structure (XANES) spectroscopy and chemical imaging. It has been found that Co3O4 nanocrystals grown on N-doped graphene were partially reduced via Co3+(O-h) to Co2+(O-h), and the reduction varies spatially on and among individual Co3O4 nanocrystal-graphene sheets. Nitrogen sites on graphene have been shown to be major and important anchoring sites for Co3O4 nanocrystals in addition to the carbon and possibly oxygen sites. Macroscopic XANES of Co L-edge and K-edge were also measured to confirm the localized STXM result that Co3+ was partly reduced in the hybrid material. These insights should account for the superior performance of the covalently coupled Co3O4/graphene hybrid in energy related applications.
C1 [Wang, Jian; Zhou, Jigang; Hu, Yongfeng; Regier, Tom] Univ Saskatchewan, Canadian Light Source Inc, Saskatoon, SK S7N 2V3, Canada.
RP Wang, J (reprint author), Univ Saskatchewan, Canadian Light Source Inc, Saskatoon, SK S7N 2V3, Canada.
EM Jian.Wang@lightsource.ca; Jigang.Zhou@lightsource.ca
RI Wang, Jian/M-1805-2013; Zhou, Jigang/N-6831-2014
OI Zhou, Jigang/0000-0001-6644-2862
FU Natural Sciences and Engineering Research Council of Canada; National
   Research Council Canada; Canadian Institutes of Health Research;
   Province of Saskatchewan; Western Economic Diversification Canada;
   University of Saskatchewan; ONR
FX We thank Dr Lachlan MacLean for assistance in data acquisition and
   analysis at CLS SXRMB beamline, and Yongye Liang from Prof. Hongjie
   Dai's group in the Department of Chemistry at Stanford University for
   providing all samples. The Canadian Light Source is supported by the
   Natural Sciences and Engineering Research Council of Canada, the
   National Research Council Canada, the Canadian Institutes of Health
   Research, the Province of Saskatchewan, Western Economic Diversification
   Canada, and the University of Saskatchewan. The work at Stanford
   University was supported in part by ONR.
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NR 52
TC 51
Z9 51
U1 20
U2 207
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD MAR
PY 2013
VL 6
IS 3
BP 926
EP 934
DI 10.1039/c2ee23844f
PG 9
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA 093BC
UT WOS:000315165700028
ER

PT J
AU Zhu, YH
   Liu, W
   Zhang, XY
   He, JC
   Chen, JT
   Wang, YP
   Cao, TB
AF Zhu, Yuanhua
   Liu, Wen
   Zhang, Xinyue
   He, Jinchao
   Chen, Jitao
   Wang, Yapei
   Cao, Tingbing
TI Directing Silicon-Graphene Self-Assembly as a Core/Shell Anode for
   High-Performance Lithium-Ion Batteries
SO LANGMUIR
LA English
DT Article
ID FACILE SYNTHESIS; COMPOSITE FILMS; ENERGY-STORAGE; NANOPARTICLES;
   SHEETS; NANOWIRES; OXIDE; NANOCOMPOSITE; NANOSPHERES; INSERTION
AB There is great interest in utilization of silicon-containing nanostructures as anode materials for lithium-ion batteries but usually limited by manufacturing cost, their intrinsic low electric conductivity, and large volume changes during cycling. Here we present a facile process to fabricate graphene-wrapped silicon nanowires (GNS@Si NWs) directed by electrostatic self-assembly. The highly conductive and mechanical flexible graphene could partially accommodate the large volume change associated with the conversion reaction and also contributed to the enhanced electronic conductivity. The as-prepared GNS@Si NWs delivered a reversible capacity of 1648 mAh.g(-1) with an initial Coulombic efficiency as high as 80%. Moreover, capacity remained 1335 mAh.g(-1) after 80 cycles at a current of 200 mA.g(-1), showing significantly improved electrochemical performance in terms of rate capability and cycling performance.
C1 [Zhu, Yuanhua; Zhang, Xinyue; He, Jinchao; Wang, Yapei] Renmin Univ China, Dept Chem, Beijing 100872, Peoples R China.
   [Liu, Wen; He, Jinchao] Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China.
RP Chen, JT (reprint author), Peking Univ, Coll Chem & Mol Engn, Beijing 100871, Peoples R China.
EM chenjitao@pku.edu.cn; yapeiwang@ruc.edu.cn
RI Chen, Jitao/G-2995-2011
OI Chen, Jitao/0000-0002-2620-5587
FU Fundamental Research Funds for the Central Universities; Research Funds
   of Renmin University of China [20334010, 20473045, 20574040]
FX This work was financially supported by the Fundamental Research Funds
   for the Central Universities and the Research Funds of Renmin University
   of China (20334010, 20473045, and 20574040).
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NR 49
TC 51
Z9 54
U1 17
U2 344
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0743-7463
J9 LANGMUIR
JI Langmuir
PD JAN 15
PY 2013
VL 29
IS 2
BP 744
EP 749
DI 10.1021/la304371d
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science,
   Multidisciplinary
SC Chemistry; Materials Science
GA 072JN
UT WOS:000313667300028
PM 23268716
ER

PT J
AU Tao, LQ
   Zai, JT
   Wang, KX
   Wan, YH
   Zhang, HJ
   Yu, C
   Xiao, YL
   Qian, XF
AF Tao, Liqi
   Zai, Jiantao
   Wang, Kaixue
   Wan, Yihang
   Zhang, Haojie
   Yu, Chao
   Xiao, Yinglin
   Qian, Xuefeng
TI 3D-hierarchical NiO-graphene nanosheet composites as anodes for lithium
   ion batteries with improved reversible capacity and cycle stability
SO RSC ADVANCES
LA English
DT Article
ID FACILE SYNTHESIS; GAS SENSORS; PERFORMANCE; CARBON; STORAGE; SHEETS;
   OXIDE; NANOMATERIALS; NANOTUBES; INSERTION
AB 3D-hierarchical NiO-graphene nanosheet (GNS) composites as high performance anode materials for lithium-ion batteries (LIBs) were synthesized through a simple ultrasonic method, and characterized by X-ray diffraction, Raman spectrum, field emission scanning electron microscopy and transmission electron microscopy. The results show that the 3D-hierarchical NiO carnations with nanoplates as building blocks are homogeneously anchored onto GNS and act as spacers to reduce the stacking of GNS. Electrochemical performances reveal that the obtained 3D-hierarchical NiO-GNS composites exhibit remarkably high reversible lithium storage capacity, good rate capability and improved cycling stability, e.g. approximate 1065 mA h g(-1) of reversible capacity is retained even after 50 cycles at a current density of 200 mA g(-1). The remarkable improvement of electrochemical performances of the obtained composites could be attributed to the decrease of the volume expansion and contraction of NiO and the improvement of the electronic conductivity of composites during the cycling process.
C1 [Qian, Xuefeng] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
   Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China.
RP Qian, XF (reprint author), Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
EM xfqian@sjtu.edu.cn
RI Wang, Kai-Xue/A-4852-2009; 宰(Zai), 建陶(Jiantao)/I-8703-2012; Qian,
   Xuefeng/G-5749-2011; Zhang, Haojie/C-6586-2016
OI Wang, Kai-Xue/0000-0002-2076-5487; 宰(Zai),
   建陶(Jiantao)/0000-0001-7562-6233; Qian, Xuefeng/0000-0002-8199-6502; 
FU National Basic Research Program of China [2009CB930400, 2007CB209705];
   National Natural Science Foundation of China [21071097, 20901050];
   Shanghai Pujiang Program [09PJ1405700]; State Key Laboratory of High
   Performance Ceramics and Superfine Microstructure [SKL200901SIC]
FX The work was supported by National Basic Research Program of China
   (2009CB930400 and 2007CB209705), National Natural Science Foundation of
   China (21071097, 20901050), Shanghai Pujiang Program (09PJ1405700) and
   the key project of State Key Laboratory of High Performance Ceramics and
   Superfine Microstructure (SKL200901SIC).
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NR 44
TC 51
Z9 51
U1 9
U2 112
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 8
BP 3410
EP 3415
DI 10.1039/c2ra00963c
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 915KM
UT WOS:000302023500047
ER

PT J
AU Yang, SN
   Li, GR
   Zhu, Q
   Pan, QM
AF Yang, Shengnan
   Li, Guorui
   Zhu, Qing
   Pan, Qinmin
TI Covalent binding of Si nanoparticles to graphene sheets and its
   influence on lithium storage properties of Si negative electrode
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ION BATTERIES; ANODE MATERIAL; SILICON ANODE; LI BATTERIES; PERFORMANCE;
   NANOSHEETS; NANOCOMPOSITE; REDUCTION; NANOWIRES; INSERTION
AB Improving the lithium storage properties of a Si negative electrode is of great significance for lithium ion batteries. A major challenge is to fabricate Si-based active materials with good electronic conduction and structural integrity in the process of discharging and charging. In this study, Si nanoparticles are covalently bound to the surface of graphene sheets via aromatic linkers through diazonium chemistry. The resulting Si-Ph-G nanocomposite delivers a delithiation capacity of 1079 and 828 mAh g(-1) in the initial and 50th cycle at a current density of 300 mA g(-1), respectively, with a capacity fading rate of 4.5 mAh g(-1) per cycle. The composite still exhibits a reversible capacity of 350 mAh g(-1) in the 40th cycle even at a rate of 4.0 A g(-1). TEM images show that Si nanoparticles are homogeneously distributed on the graphene sheets in the process of lithiation and delithiation. The excellent electrochemical performance of the Si-Ph-G composite is ascribed to the covalent linkages between the Si nanoparticles and graphene sheets, which prevent severe stacking of the graphene sheets and aggregation of Si nanoparticles. The finding of this study offers an alternative approach to improve the lithium storage properties of a Si negative electrode by chemically anchoring electroactive materials to a conducting matrix.
C1 [Yang, Shengnan; Li, Guorui; Zhu, Qing; Pan, Qinmin] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China.
RP Pan, QM (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China.
EM panqm@hit.edu.cn
FU National Natural Science Foundation of China [50803013]
FX This study was financially supported by National Natural Science
   Foundation of China (Grant No. 50803013).
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NR 56
TC 51
Z9 53
U1 15
U2 101
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 8
BP 3420
EP 3425
DI 10.1039/c2jm15232k
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 884HL
UT WOS:000299695400023
ER

PT J
AU Yue, WB
   Lin, ZZ
   Jiang, SH
   Yang, XJ
AF Yue, Wenbo
   Lin, Zhenzhen
   Jiang, Shuhua
   Yang, Xiaojing
TI Preparation of graphene-encapsulated mesoporous metal oxides and their
   application as anode materials for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID NEGATIVE ELECTRODES; CO3O4; PERFORMANCE; CAPACITY; ROUTE; NANOPARTICLES;
   NANOSHEETS; GRAPHITE; CRYSTALS; SHEETS
AB Graphene-encapsulated mesoporous metal oxides (e.g. Co3O4, Cr2O3 and NiO) as novel anode materials for lithium-ion batteries were simply synthesized by adjusting the pH of mesoporous metal oxides and graphene oxide suspensions to set values (e.g. 5-6 for metal oxides, 7-8 for graphene oxide) and mixing the two suspensions in the presence of reducing agents. These composites synthesized by this facile method exhibited superior electrochemical performance, including remarkably high capacity, high rate capability and excellent cycle performance. The improved performance may be attributed to the high dispersion of mesoporous particles separated by graphene nanosheets and the high electrical conductivity of graphene.
C1 [Yue, Wenbo; Lin, Zhenzhen; Jiang, Shuhua; Yang, Xiaojing] Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China.
RP Yue, WB (reprint author), Beijing Normal Univ, Coll Chem, Beijing 100875, Peoples R China.
EM wbyue@bnu.edu.cn; yang.xiaojing@bnu.edu.cn
FU National Natural Science Foundation of China [50872012, 21101014];
   Fundamental Research Funds for the Central Universities
FX This work is financially supported by National Natural Science
   Foundation of China 50872012 and 21101014, the Fundamental Research
   Funds for the Central Universities.
CR Zhang JL, 2010, CHEM COMMUN, V46, P1112, DOI 10.1039/b917705a
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NR 33
TC 51
Z9 51
U1 10
U2 109
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 32
BP 16318
EP 16323
DI 10.1039/c2jm30805c
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 978AB
UT WOS:000306708700024
ER

PT J
AU Rui, XH
   Tan, HT
   Sim, DH
   Liu, WL
   Xu, C
   Hng, HH
   Yazami, R
   Lim, TM
   Yan, QY
AF Rui, Xianhong
   Tan, Huiteng
   Sim, Daohao
   Liu, Weiling
   Xu, Chen
   Hng, Huey Hoon
   Yazami, Rachid
   Lim, Tuti Mariana
   Yan, Qingyu
TI Template-free synthesis of urchin-like Co3O4 hollow spheres with good
   lithium storage properties
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Cobalt oxide; Lithium ion battery; Urchin-like architecture; Hollow
   spheres; High rate capability
ID ION BATTERY ELECTRODES; GRAPHENE OXIDE SHEETS; HIGH-CAPACITY;
   BINDER-FREE; HYDROTHERMAL SYNTHESIS; CATHODE MATERIAL; NANOWIRE ARRAYS;
   PERFORMANCE; ANODES; SUPERCAPACITORS
AB Hierarchical urchin-like hollow spheres (5-8 mu m in diameter) assembled by one-dimensional nanowires consisting of many interconnected Co3O4 nanoparticles (10-50 nm) are successfully synthesized. Co(CO3)(0.5)(OH)center dot 0.11H(2)O precursors are firstly prepared by a hydrothermal process. The morphological evolution process of Co(CO3)(0.5)(OH)center dot 0.11H(2)O hollow urchin precursors is investigated and a plausible mechanism is proposed. Then, the Co(CO3)(0.5)(OH)center dot 0.11H(2)O are converted to Co3O4 through heat treatment in air. As an anode material for lithium ion batteries, urchin-like Co3O4 hollow spheres exhibit highly reversible specific capacities, good cycling stabilities and excellent rate capabilities (e.g., 433 mAh g(-1) at 10 C). The superior performances result from the synergetic effect of integral urchin-like microstructure, small diffusion lengths in the nanoparticle building blocks and sufficient void space to buffer the volume expansion. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Rui, Xianhong; Tan, Huiteng; Sim, Daohao; Liu, Weiling; Xu, Chen; Hng, Huey Hoon; Yazami, Rachid; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Rui, Xianhong; Lim, Tuti Mariana] Nanyang Technol Univ, Sch Civil & Environm Engn, Singapore 639798, Singapore.
   [Lim, Tuti Mariana] Ngee Ann Polytech, Sch Life Sci & Chem Technol, Singapore 599489, Singapore.
   [Yan, Qingyu] Nanyang Technol Univ, Energy Res Inst, Singapore 637459, Singapore.
   [Yan, Qingyu] Nanyang Technol Univ, TUM CREATE Ctr Electromobil, Singapore 637459, Singapore.
RP Yan, QY (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, Block N4-1,Nanyang Ave, Singapore 639798, Singapore.
EM XHRUI@ntu.edu.sg; tmlim@ntu.edu.sg; Alexyan@ntu.edu.sg
RI Yan , Qingyu/A-2237-2011; Lim, Tuti/F-8875-2012; Hng, Huey
   Hoon/A-2246-2011; Rui, Xianhong/D-2604-2015
OI Hng, Huey Hoon/0000-0002-8950-025X; Rui, Xianhong/0000-0003-1125-0905
FU MOE (Singapore) [AcRF Tier 1 RG 31/08]; Singapore Ministry of Education
   [MOE2010-T2-1-017]; A*STAR SERC [1021700144]; Singapore MPA
   [23/04.15.03];  [NRF2009EWT-CERP001-026]
FX The authors gratefully acknowledge AcRF Tier 1 RG 31/08 of MOE
   (Singapore), NRF2009EWT-CERP001-026 (Singapore), Singapore Ministry of
   Education (MOE2010-T2-1-017), A*STAR SERC grant 1021700144 and Singapore
   MPA 23/04.15.03 grant.
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NR 52
TC 50
Z9 50
U1 35
U2 361
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JAN 15
PY 2013
VL 222
BP 97
EP 102
DI 10.1016/j.jpowsour.2012.08.094
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 037TR
UT WOS:000311129900015
ER

PT J
AU Xia, FF
   Hu, XL
   Sun, YM
   Luo, W
   Huang, YH
AF Xia, Fangfang
   Hu, Xianluo
   Sun, Yongming
   Luo, Wei
   Huang, Yunhui
TI Layer-by-layer assembled MoO2-graphene thin film as a high-capacity and
   binder-free anode for lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID STORAGE CAPACITY; ENERGY-STORAGE; PERFORMANCE; ELECTRODES; NANOTUBE;
   NANOPARTICLES; OXIDE
AB Thin films of MoO2 nanoparticles and graphene sheets are created by layer-by-layer (LBL) assembly as binder-free anodes for lithium-ion batteries. Both anionic polyoxometalate clusters and graphene oxide nanosheets with oxygen functional groups on both basal planes and edges are assembled into LBL films with the aid of a cationic polyelectrolyte. After a subsequent thermal treatment in an Ar-H-2 atmosphere, hybrid MoO2-graphene films with three-dimensionally interconnected nanopores are formed, which comprise ultrafine MoO2 nanoparticles homogeneously embedded in the porous network of graphene nanosheets. When used as an anode for lithium-ion batteries, the MoO2-graphene thin-film electrode shows superior electrochemical performance with high specific capacity and excellent cyclability. A high specific capacity of 675.9 mA h g(-1) after 100 discharge-charge cycles is achieved, indicating a promising anode candidate for lithium-storage applications.
C1 [Xia, Fangfang; Hu, Xianluo; Sun, Yongming; Luo, Wei; Huang, Yunhui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
RP Hu, XL (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
EM huxl@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Sun, Yongming/G-7799-2012; Luo, Wei/E-1582-2011; Huang,
   Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU National Natural Science Foundation of China [51002057, 50825203]; 863
   program [2009AA03Z225]; Natural Science Foundation of Hubei Province
   [2008CDA026]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the National Natural Science Foundation of
   China (Grant nos. 51002057 and 50825203), the 863 program (Grant no.
   2009AA03Z225), the Natural Science Foundation of Hubei Province (Grant
   no. 2008CDA026), and the PCSIRT (Program for Changjiang Scholars and
   Innovative Research Team in University). The authors thank Analytical
   and Testing Center of HUST for XRD and SEM measurements.
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NR 32
TC 50
Z9 52
U1 22
U2 152
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 15
BP 4707
EP 4711
DI 10.1039/c2nr30742a
PG 5
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 973AS
UT WOS:000306324000052
PM 22744734
ER

PT J
AU Hu, LR
   Ren, YM
   Yang, HX
   Xu, Q
AF Hu, Lianren
   Ren, Yumei
   Yang, Hongxia
   Xu, Qun
TI Fabrication of 3D Hierarchical MoS2/Polyaniline and MoS2/C Architectures
   for Lithium-Ion Battery Applications
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE MoS2; nanoflowers; hierarchical structures; conductive material;
   lithium-ion batteries
ID PERFORMANCE ANODE MATERIAL; MOLYBDENUM-DISULFIDE MOS2; STORAGE
   PROPERTIES; ASSISTED SYNTHESIS; FACILE SYNTHESIS; ELECTROCHEMICAL
   PERFORMANCES; MOS2/GRAPHENE COMPOSITES; CARBON NANOTUBES; BINDER-FREE;
   NANOSHEETS
AB In this work, three-dimensional (3D) hierarchical MoS2/polyaniline (PANI) nanoflowers were successfully fabricated via a simple hydrothermal method. The crystal structure and morphology of the MoS2/PANI nanoflowers were characterized by SEM, TEM, XRD, XPS, and FT-IR spectra, revealing that the nanoflowers were composed of ultrathin nanoplates which consisted of few-layered MoS2 nanosheets with enlarged interlayer distance of the (002) plane and PANI. The excellent electrochemical performance of the 3D hierarchical MoS2/PANI nanoflowers was demonstrated. Further 3D hierarchical MoS2/C nanoflowers can be prepared conveniently by annealing the MoS2/PANI sample in a N-2 atmosphere at 500 degrees C for 4 h. The obtained MoS2/C sample exhibited more excellent electrochemical performance due to its excellent electronic conductivity resulting from the close integration of MoS2 nanosheets with carbon matrix. High reversible capacity of 888.1 mAh g(-1) with the Coulombic efficiency maintained at above 90% from the first cycle were achieved at a current density of 100 mA g(-1). Even at a current density of 1000 mA g(-1), the reversible capacity of the MoS2/C sample could be retained at 511 mAh g(-1). The excellent electrochemical performance of these two samples could be attributed to the combined action of enlarged interlayer distance of the ultrathin MoS2 nanosheets, 3D architectures, hierarchical structures, and conductive material. Thus, these 3D hierarchical nanoflowers are competent as promising anode materials for high-performance lithium-ion batteries.
C1 [Hu, Lianren; Ren, Yumei; Yang, Hongxia; Xu, Qun] Zhengzhou Univ, Coll Mat Sci & Engn, Zhengzhou 450052, Peoples R China.
RP Xu, Q (reprint author), Zhengzhou Univ, Coll Mat Sci & Engn, Zhengzhou 450052, Peoples R China.
EM qunxu@zzu.edu.cn
FU National Natural Science Foundation of China [51173170, 21101141,
   50955010, 20974102]; Innovation Talents Award of Henan Province
   [114200510019]; State Key Laboratory of Chemical Engineering
   [SKL-ChE-13A04]; Key program of science and technology from Zhengzhou
   Bureau of science and technology [121PZDGG213]
FX We are grateful for the National Natural Science Foundation of China
   (No. 51173170, 21101141, 50955010, 20974102), the financial support from
   the Innovation Talents Award of Henan Province (114200510019), State Key
   Laboratory of Chemical Engineering (No. SKL-ChE-13A04), and the Key
   program of science and technology (121PZDGG213) from Zhengzhou Bureau of
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NR 59
TC 49
Z9 50
U1 84
U2 342
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD AUG 27
PY 2014
VL 6
IS 16
BP 14644
EP 14652
DI 10.1021/am503995s
PG 9
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA AO2CB
UT WOS:000341122000159
PM 25100439
ER

PT J
AU Tritsaris, GA
   Kaxiras, E
   Meng, S
   Wang, EG
AF Tritsaris, Georgios A.
   Kaxiras, Efthimios
   Meng, Sheng
   Wang, Enge
TI Adsorption and Diffusion of Lithium on Layered Silicon for Li-Ion
   Storage
SO NANO LETTERS
LA English
DT Article
DE Lithium-ion battery; energy storage; two-dimensional silicon; adatom
   adsorption; surface diffusion; ab initio calculations
ID PLASTIC-DEFORMATION; BATTERY ANODES; INSERTION; NANOWIRES; ELECTRODES;
   GRAPHITE; ENERGY
AB The energy density of Li-ion batteries depends critically on the specific charge capacity of the constituent electrodes. Silicene, the silicon analogue to graphene, being of atomic thickness could serve as high-capacity host of Li in Li-ion secondary batteries. In this work, we employ first-principles calculations to investigate the interaction of Li with Si in model electrodes of free-standing single-layer and double-layer silicene. More specifically, we identify strong binding sites for Li, calculate the energy barriers accompanying Li diffusion, and present our findings in the context of previous theoretical work related to Li-ion storage in other structural forms of silicon: the bulk and nanowires. The binding energy of Li is similar to 2.2 eV per Li atom and shows small variation with respect to Li content and silicene thickness (one or two layers) while the barriers for Li diffusion are relatively low, typically less than 0.6 eV. We use our theoretical findings to assess the suitability of two-dimensional silicon in the form of silicene layers for Li-ion storage.
C1 [Tritsaris, Georgios A.; Kaxiras, Efthimios] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA.
   [Tritsaris, Georgios A.; Wang, Enge] Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China.
   [Kaxiras, Efthimios] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA.
   [Meng, Sheng] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
RP Meng, S (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
RI Meng, Sheng/A-7171-2010
FU National Science Foundation [OCI-1053575]; NSFC [11222431]; CAS
FX Computations were performed on the Odyssey cluster, supported by the FAS
   Science Division Research Computing Group at Harvard University, the
   Extreme Science and Engineering Discovery Environment (XSEDE), which is
   supported by National Science Foundation Grant OCI-1053575, and the SEAS
   HPC cluster, supported by the Academic Computing Group. S.M.
   acknowledges financial supports from NSFC (Grant 11222431) and CAS.
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NR 44
TC 49
Z9 50
U1 19
U2 282
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD MAY
PY 2013
VL 13
IS 5
BP 2258
EP 2263
DI 10.1021/nl400830u
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 143TZ
UT WOS:000318892400062
PM 23611247
ER

PT J
AU Kim, IT
   Magasinski, A
   Jacob, K
   Yushin, G
   Tannenbaum, R
AF Kim, Il Tae
   Magasinski, Alexandre
   Jacob, Karl
   Yushin, Gleb
   Tannenbaum, Rina
TI Synthesis and electrochemical performance of reduced graphene
   oxide/maghemite composite anode for lithium ion batteries
SO CARBON
LA English
DT Article
ID ONE-POT SYNTHESIS; GRAPHITE OXIDE; STORAGE CAPACITY; LI STORAGE;
   NANOSHEETS; HYBRID; NANOSTRUCTURES; NANOCOMPOSITES; REDUCTION
AB Reduced graphene oxide (rGO) tethered with maghemite (gamma-Fe2O3) was synthesized using a novel modified sol-gel process, where sodium dodecylbenzenesulfonate was introduced into the suspension to prevent the undesirable formation of an iron oxide 3D network. Thus, nearly monodispersed and homogeneously distributed gamma-Fe2O3 magnetic nanoparticles could be obtained on surface of graphene sheets. The utilized thermal treatment process did not require a reducing agent for reduction of graphene oxide. The morphology and structure of the composites were investigated using various characterization techniques. As-prepared rGO/Fe2O3 composites were utilized as anodes for half lithium ion cells. The 40 wt.%-rGO/Fe2O3 composite exhibited high reversible capacity of 690 mA h g(-1) at current density of 500 mA g(-1) and good stability for over 100 cycles, in contrast with that of the pure-Fe2O3 nanoparticles which demonstrated rapid degradation to 224 mA h g(-1) after 50 cycles. Furthermore, the composite showed good rate capability of 280 mA h g(-1) at 10C (similar to 10,000 mA g(-1)). These characteristics could be mainly attributed to both the use of an effective binder, poly(acrylic acid) (PAA), and the specific hybrid structures that prevent agglomeration of nanoparticles and provide buffering spaces needed for volume changes of nanoparticles during insertion/extraction of Li ions. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Kim, Il Tae; Magasinski, Alexandre; Jacob, Karl; Yushin, Gleb] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
   [Tannenbaum, Rina] Univ Alabama Birmingham, Dept Biomed Engn, Sch Med, Birmingham, AL 35294 USA.
   [Tannenbaum, Rina] Univ Alabama Birmingham, UAB Comprehens Canc Ctr, Birmingham, AL 35294 USA.
RP Yushin, G (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
EM yushin@gatech.edu; rina.tannenbaum@gmail.com
RI Yushin, Gleb/B-4529-2013
OI Yushin, Gleb/0000-0002-3274-9265
FU Institute of Paper Science and Technology (IPST) at the Georgia
   Institute of Technology; Energy Efficiency & Resources program of the
   Korea Institute of Energy Technology Evaluation and Planning (KETEP)
   [20118510010030]
FX Il Tae Kim was supported by Paper Science and Engineering (PSE) Graduate
   Fellowships from the Institute of Paper Science and Technology (IPST) at
   the Georgia Institute of Technology. G. Yushin and A. Magasinski were
   supported by the Energy Efficiency & Resources program of the Korea
   Institute of Energy Technology Evaluation and Planning (KETEP) Grant
   20118510010030.
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Z9 49
U1 19
U2 268
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
EI 1873-3891
J9 CARBON
JI Carbon
PD FEB
PY 2013
VL 52
BP 56
EP 64
DI 10.1016/j.carbon.2012.09.004
PG 9
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 079SO
UT WOS:000314192700007
ER

PT J
AU Liu, YT
   Zhu, XD
   Duan, ZQ
   Xie, XM
AF Liu, Yi-Tao
   Zhu, Xiao-Dong
   Duan, Zhi-Qiang
   Xie, Xu-Ming
TI Flexible and robust MoS2-graphene hybrid paper cross-linked by a polymer
   ligand: a high-performance anode material for thin film lithium-ion
   batteries
SO CHEMICAL COMMUNICATIONS
LA English
DT Article
ID STORAGE PROPERTIES; MOS2 NANOSHEETS; ELECTROCHEMICAL PERFORMANCES;
   ASSISTED SYNTHESIS; CARBON NANOTUBES; ORGANIC-SOLVENTS; GRAPHENE OXIDE;
   COMPOSITES; NANOPARTICLES; STRATEGY
AB A flexible and robust MoS2-graphene hybrid paper with an excellent lithium storage capacity is fabricated through cross-linking by a polymer ligand, PEO, and shows potential for the development of high-performance film anodes.
C1 [Liu, Yi-Tao; Duan, Zhi-Qiang; Xie, Xu-Ming] Tsinghua Univ, Dept Chem Engn, Key Lab Adv Mat MOE, Beijing 100084, Peoples R China.
   [Zhu, Xiao-Dong] Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, Harbin 150080, Peoples R China.
RP Xie, XM (reprint author), Tsinghua Univ, Dept Chem Engn, Key Lab Adv Mat MOE, Beijing 100084, Peoples R China.
EM xxm-dce@mail.tsinghua.edu.cn
FU NSFC [21304053, 21274079, 51073088, 21246011]; SRFDP [20110002110032,
   20120002130012]
FX We thank the financial support from NSFC (21304053, 21274079, 51073088
   and 21246011) and SRFDP (20110002110032 and 20120002130012). Y.-T. L.
   acknowledges the China Post-doctoral Science Foundation (2013M530616).
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NR 30
TC 49
Z9 53
U1 24
U2 242
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1359-7345
EI 1364-548X
J9 CHEM COMMUN
JI Chem. Commun.
PY 2013
VL 49
IS 87
BP 10305
EP 10307
DI 10.1039/c3cc45936e
PG 3
WC Chemistry, Multidisciplinary
SC Chemistry
GA 234KU
UT WOS:000325643500031
PM 24064696
ER

PT J
AU Zhuo, LH
   Wu, YQ
   Wang, LY
   Yu, YC
   Zhang, XB
   Zhao, FY
AF Zhuo, Linhai
   Wu, Yingqiang
   Wang, Lingyan
   Yu, Yancun
   Zhang, Xinbo
   Zhao, Fengyu
TI One-step hydrothermal synthesis of SnS2/graphene composites as anode
   material for highly efficient rechargeable lithium ion batteries
SO RSC ADVANCES
LA English
DT Article
ID ELECTROCHEMICAL PERFORMANCES; ASSISTED SYNTHESIS; AMORPHOUS-CARBON;
   FLOWERLIKE SNS2; NICKEL SULFIDE; L-CYSTEINE; NANOCOMPOSITE; CAPABILITY;
   PROPERTY; CAPACITY
AB SnS2/graphene nanosheets (SnS2/GNS) composites were synthesized by a one-step hydrothermalmethod. The composites exhibit remarkably improved Li-storage ability with a good cycling life and high capability superior to that of the pure SnS2 counterpart due to a synergic effect between the graphene and SnS2 nanosheets.
C1 [Zhuo, Linhai; Wu, Yingqiang; Wang, Lingyan; Yu, Yancun; Zhao, Fengyu] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China.
   [Zhang, Xinbo] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Zhuo, Linhai; Wu, Yingqiang; Wang, Lingyan; Yu, Yancun; Zhao, Fengyu] Chinese Acad Sci, Changchun Inst Appl Chem, Lab Green Chem & Proc, Changchun 130022, Peoples R China.
   [Wu, Yingqiang; Wang, Lingyan] Chinese Acad Sci, Beijing 100049, Peoples R China.
RP Zhuo, LH (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China.
EM xbzhang@ciac.jl.cn; zhaofy@ciac.jl.cn
FU  [NSFC20873139];  [KJCX2];  [YWH16];  [20086063]
FX This work was financially supported by NSFC20873139, KJCX2, YWH16, and
   20086063.
CR Choi J, 2011, CHEM COMMUN, V47, P5241, DOI 10.1039/c1cc10317b
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NR 24
TC 49
Z9 49
U1 10
U2 88
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 12
BP 5084
EP 5087
DI 10.1039/c2ra00002d
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA 948ES
UT WOS:000304487000016
ER

PT J
AU Wang, J
   Liu, JL
   Chao, DL
   Yan, JX
   Lin, JY
   Shen, ZX
AF Wang, Jin
   Liu, Jilei
   Chao, Dongliang
   Yan, Jiaxu
   Lin, Jianyi
   Shen, Ze Xiang
TI Self-Assembly of Honeycomb-like MoS2 Nanoarchitectures Anchored into
   Graphene Foam for Enhanced Lithium-Ion Storage
SO ADVANCED MATERIALS
LA English
DT Article
DE molybdenum sulfide; graphene; honeycomb; self-assembly; lithium-ion
   batteries
ID EXCELLENT ELECTROCHEMICAL PERFORMANCE; SUPERIOR CATHODE MATERIALS;
   ATOMIC LAYER DEPOSITION; ANODE MATERIALS; ELECTRODE MATERIALS; ASSISTED
   SYNTHESIS; FACILE SYNTHESIS; RATE CAPABILITY; CARBON SPHERES;
   ENERGY-STORAGE
C1 [Wang, Jin; Shen, Ze Xiang] Nanyang Technol Univ, Interdisciplinary Grad Sch, Energy Res Inst ERI N, Singapore 637553, Singapore.
   [Wang, Jin; Liu, Jilei; Chao, Dongliang; Yan, Jiaxu; Shen, Ze Xiang] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
   [Lin, Jianyi] Nanyang Technol Univ, Energy Res Inst ERI N, Singapore 637553, Singapore.
RP Lin, JY (reprint author), Nanyang Technol Univ, Energy Res Inst ERI N, 50 Nanyang Dr, Singapore 637553, Singapore.
EM Lijy@ntu.edu.sg; Zexiang@ntu.edu.sg
RI Shen, Zexiang/B-6988-2011; Wang, Jin/D-1309-2013; yan, jiaxu/J-5984-2015
OI Wang, Jin/0000-0001-6511-869X; 
CR Fang XP, 2012, MICROPOR MESOPOR MAT, V151, P418, DOI 10.1016/j.micromeso.2011.09.032
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NR 62
TC 48
Z9 50
U1 91
U2 390
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA POSTFACH 101161, 69451 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD NOV 12
PY 2014
VL 26
IS 42
BP 7162
EP 7169
DI 10.1002/adma.201402728
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AT2RS
UT WOS:000344783300002
PM 25250514
ER

PT J
AU Zhang, HW
   Zhou, L
   Noonan, O
   Martin, DJ
   Whittaker, AK
   Yu, CZ
AF Zhang, Hongwei
   Zhou, Liang
   Noonan, Owen
   Martin, Darren J.
   Whittaker, Andrew K.
   Yu, Chengzhong
TI Tailoring the Void Size of Iron Oxide@Carbon Yolk-Shell Structure for
   Optimized Lithium Storage
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
ID ION BATTERY ANODE; HOLLOW CARBON; SPHERES; NANOPARTICLES; GRAPHENE;
   MICROSPHERES; NANOCRYSTALS; NANOSPHERES; UNIFORM; COMPOSITES
AB High-capacity lithium-ion battery anode materials, such as transition metal oxides, Sn and Si, suffer from large volume expansion during lithiation, which causes capacity decay. Introducing sufficient void space to accommodate the volume change is essential to achieve prolonged cycling stability. However, excessive void space may significantly compromise the volumetric energy density. Herein, a method to control the void size in iron oxide@carbon (FeOx@C) yolk-shell structures is developed and the relationship between the void space and electrochemical performance is demonstrated. With an optimized void size, the FeOx@C yolk-shell structure exhibits the best cycling performance. A high reversible capacity of approximate to 810 mA h g(-1) is obtained at 0.2 C, maintaining 790 mA h g(-1) after 100 cycles. This contrasts with FeOx@C materials having either smaller or larger void sizes, in which significant capacity fading is observed during cycling. This contribution provides an effective approach to alleviate the volume expansion problem, which can be generally applied to other anode materials to improve their performance in LIBs.
C1 [Zhang, Hongwei; Zhou, Liang; Noonan, Owen; Martin, Darren J.; Whittaker, Andrew K.; Yu, Chengzhong] Univ Queensland, Australian Inst Bioengn & Nanotechnol, Brisbane, Qld 4072, Australia.
RP Zhou, L (reprint author), Univ Queensland, Australian Inst Bioengn & Nanotechnol, Brisbane, Qld 4072, Australia.
EM l.zhou1@uq.edu.au; c.yu@uq.edu.au
RI Yu, Chengzhong/I-8663-2012; Zhou, Liang/K-2063-2012; McKenzie,
   Warren/J-2137-2014; Whittaker, Andrew/E-6172-2011
OI Whittaker, Andrew/0000-0002-1948-8355
FU Australian Research Council
FX The authors acknowledge the Australian Research Council for financial
   support. The authors also acknowledge the facilities, the scientific and
   technical assistance from Centre for Microscopy and Microanalysis at the
   University of Queensland.
CR He CN, 2013, ACS NANO, V7, P4459, DOI 10.1021/nn401059h
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NR 37
TC 48
Z9 48
U1 46
U2 225
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD JUL 16
PY 2014
VL 24
IS 27
BP 4337
EP 4342
DI 10.1002/adfm.201400178
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AM2XC
UT WOS:000339713500015
ER

PT J
AU Wang, RH
   Xu, CH
   Sun, J
   Gao, L
   Yao, HL
AF Wang, Ronghua
   Xu, Chaohe
   Sun, Jing
   Gao, Lian
   Yao, Heliang
TI Solvothermal-Induced 3D Macroscopic SnO2/Nitrogen-Doped Graphene
   Aerogels for High Capacity and Long-Life Lithium Storage
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE tin oxide; solvothermal; nitrogen doping; graphene; aerogels; lithium
   ion batteries
ID NITROGEN-DOPED GRAPHENE; HIGH-RATE CAPABILITY; ION BATTERY ANODES; SNO2
   NANOPARTICLES; REDUCED GRAPHENE; BINDER-FREE; COMPOSITE; PERFORMANCE;
   NANOSHEETS; OXIDE
AB 3D macroscopic tin oxide/nitrogen-doped graphene frame-works (SnO2/GN) were constructed by a novel solvothermal-induced self-assembly process, using SnO2 colloid as precursor (crystal size of 3-7 nm). Solvothermal treatment played a key role as N,N-dimethylmethanamide (DMF) acted both as reducing reagent and nitrogen source, requiring no additional nitrogen-containing precursors or post-treatment. The SnO2/GN exhibited a 3D hierarchical porous architecture with a large surface area (336 m(2)g(-1)), which not only effectively prevented the agglomeration of SnO2 but also facilitated fast ion and electron transport through 3D pathways. As a result, the optimized electrode with GN content of 44.23% exhibited superior rate capability (1126, 855, and 614 mAh g(-1) at 1000, 3000, and 6000 mA g(-1) respectively) and extraordinary prolonged cycling stability at high current densities (905 mAh g(-1) after 1000 cycles at 2000 mA g(-1)). Electrochemical impedance spectroscopy (EIS) and morphological study demonstrated the structural stability of the electrode. enhanced electrochemical reactivity and good structural stability of the electrode.
C1 [Wang, Ronghua; Xu, Chaohe; Sun, Jing; Gao, Lian; Yao, Heliang] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
RP Sun, J (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, 1295 Ding Xi Rd, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU 973 Project [2012CB932303]; National Natural Science Foundation of China
   [50972153, 51072215, 51172261]
FX This work is supported by the 973 Project (2012CB932303), the National
   Natural Science Foundation of China (Grant No. 50972153, 51072215, and
   51172261).
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NR 65
TC 48
Z9 48
U1 35
U2 203
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAR 12
PY 2014
VL 6
IS 5
BP 3427
EP 3436
DI 10.1021/am405557c
PG 10
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA AD0KM
UT WOS:000332922900049
PM 24555873
ER

PT J
AU Jing, Y
   Zhou, Z
   Cabrera, CR
   Chen, ZF
AF Jing, Yu
   Zhou, Zhen
   Cabrera, Carlos R.
   Chen, Zhongfang
TI Graphene, inorganic graphene analogs and their composites for lithium
   ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-PERFORMANCE ANODE; EXCELLENT ELECTROCHEMICAL PERFORMANCE; METAL
   DICHALCOGENIDE NANOSHEETS; PROMISING CATHODE MATERIAL;
   MOLYBDENUM-DISULFIDE MOS2; CHEMICAL-VAPOR-DEPOSITION; SENSITIZED
   SOLAR-CELLS; HIGH-RATE CAPABILITY; FEW-LAYER GRAPHENE; LI-ION
AB In recent years, two-dimensional (2D) materials, including graphene and inorganic graphene analogs (IGAs), have been the subject of intensive studies due to their novel chemical and physical properties. With apparent high surface-to-volume ratio, 2D materials are promising electrode candidates for lithium ion batteries (LIBs). Compared with three-dimensional bulk crystals, 2D materials have superior structural characteristics, and thus can exhibit higher specific capacity and better high-rate stability. In particular, composites consisting of graphene and IGAs could have enhanced electrochemical performances due to the specific synergic effects, which open up new frontiers in fundamental science and technology. Although the explorations of using IGAs for lithium storage have begun very recently, a timely overview in this field is necessary for developing improved electrode candidates. In this feature article, we summarize the ongoing efforts and studies from both experimental and theoretical communities on developing graphene and IGAs as LIB electrodes. Compared with graphene, we put more emphasis on IGAs, such as transition metal oxides, dichalcogenides, and MXenes, and illustrate the significant advantages of IGAs as electrodes. We also show that due to the effective synergic interactions between graphene and IGAs, their composites step further to achieve reversible high-capacity LIBs. Finally, we discuss the problems and limitations for the practical application of 2D materials to LIBs.
C1 [Jing, Yu; Cabrera, Carlos R.; Chen, Zhongfang] Univ Puerto Rico, Dept Chem, Inst Funct Nanomat, Rio Piedras, PR 00931 USA.
   [Jing, Yu; Zhou, Zhen] Nankai Univ, Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin Key Lab Met & Mol Based Mat Chem,Minist E, Key Lab Adv Energy Mat,Inst New Energy Mat Chem, Tianjin 300071, Peoples R China.
RP Chen, ZF (reprint author), Univ Puerto Rico, Dept Chem, Inst Funct Nanomat, Rio Piedras Campus, Rio Piedras, PR 00931 USA.
EM zhouzhen@nankai.edu.cn; zhongfangchen@gmail.com
RI Zhou, Zhen/C-4517-2008; Chen, Zhongfang/A-3397-2008; Jing,
   Yu/C-9280-2015
OI Zhou, Zhen/0000-0003-3232-9903; 
FU USA by the Department of Defense [W911NF-12-1-0083]; China by the NSFC
   [21273118]; 111 Project [B12015]; MOE Innovation Team [IRT13022]
FX Support in the USA by the Department of Defense (Grant W911NF-12-1-0083)
   and in China by the NSFC (21273118), 111 Project (B12015) and MOE
   Innovation Team (IRT13022) is gratefully acknowledged.
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NR 211
TC 48
Z9 49
U1 42
U2 144
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 31
BP 12104
EP 12122
DI 10.1039/c4ta01033g
PG 19
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AM1RJ
UT WOS:000339625500002
ER

PT J
AU Yan, CL
   Xi, W
   Si, WP
   Deng, JW
   Schmidt, OG
AF Yan, Chenglin
   Xi, Wang
   Si, Wenping
   Deng, Junwen
   Schmidt, Oliver G.
TI Highly Conductive and Strain-Released Hybrid Multilayer Ge/Ti
   Nanomembranes with Enhanced Lithium-Ion-Storage Capability
SO ADVANCED MATERIALS
LA English
DT Article
DE nanomembranes; hybrid structures; multilayer structures; lithium-ion
   batteries
ID HIGH-CAPACITY; ELECTRODE MATERIALS; BATTERY ELECTRODES; ANODE MATERIALS;
   GERMANIUM; PERFORMANCE; GRAPHENE; FILM; CHALLENGES; NANOWIRES
AB Highly conductive and hybridized microtubes relying on strain-released ultrathin Ti/Ge bilayer nanomembranes are reported. These hybrid multilayer microtubes show a remarkably enhanced reversible capacity up to 1495 mA h g(-1) with a high first-cycle Coulombic efficiency of 85%, and demonstrate an excellent capacity of approximate to 930 mA h g(-1) after 100 cycles.
C1 [Yan, Chenglin; Xi, Wang; Si, Wenping; Deng, Junwen; Schmidt, Oliver G.] IFW Dresden, Inst Integrat Nanosci, D-01069 Dresden, Germany.
   [Si, Wenping; Deng, Junwen; Schmidt, Oliver G.] Tech Univ Chemnitz, D-09107 Chemnitz, Germany.
RP Yan, CL (reprint author), IFW Dresden, Inst Integrat Nanosci, Helmholtzstr 20, D-01069 Dresden, Germany.
EM c.yan@ifw-dresden.de; w.xi@ifw-dresden.de
RI Yan, Chenglin/F-6549-2010; Si, Wenping/P-3454-2014
OI Si, Wenping/0000-0002-3064-1533
FU International Research Training Group (IRTG) project; pakt project
   "Electrochemical energy storage in autonomous systems" [49004401];
   Volkswagen Foundation [86 362]
FX This work was financed by the International Research Training Group
   (IRTG) project, the pakt project "Electrochemical energy storage in
   autonomous systems, Nr. 49004401", and the Volkswagen Foundation (86
   362). We express our thanks to Kaikai Song at IFW Dresden for his strong
   support.
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NR 36
TC 48
Z9 48
U1 13
U2 147
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD JAN 25
PY 2013
VL 25
IS 4
BP 539
EP 544
DI 10.1002/adma.201203458
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 074OZ
UT WOS:000313823400009
PM 23109218
ER

PT J
AU Wang, CD
   Li, Y
   Chui, YS
   Wu, QH
   Chen, XF
   Zhang, WJ
AF Wang, Chundong
   Li, Yi
   Chui, Ying-San
   Wu, Qi-Hui
   Chen, Xianfeng
   Zhang, Wenjun
TI Three-dimensional Sn-graphene anode for high-performance lithium-ion
   batteries
SO NANOSCALE
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; AT-CNT NANOSTRUCTURES; C COMPOSITE; ELECTRODE
   MATERIALS; CYCLE PERFORMANCE; TIN; STORAGE; LI; CAPACITY; INTERMETALLICS
AB Tin (Sn) has been considered as one of the most promising anode materials for high- capacity lithium- ion batteries (LIBs) due to its high energy density, abundance, and environmentally benign nature. However, the problems of fast capacity fading at prolonged cycling and poor rate capacity hinder its practical use. Herein, we report the development of a novel architecture of Sn nanoparticle- decorated threedimensional (3D) foothill- like graphene as an anode in LIBs. Electrochemical measurements demonstrated that the 3D Sn- graphene anode delivered a reversible capacity of 466 mA h g(-1) at a current density of 879 mA g(-1) (1 C) after over 4000 cycles and 794 mA h g(-1) at 293 mA g(-1) (1/3 C) after 400 cycles. The capacity at 1/3 C is over 200% that of conventional graphite anodes, suggesting that the 3D Sn- graphene structure enables a significant improvement in the overall performance of a LIB in aspects of capacity, cycle life, and rate capacity.
C1 [Wu, Qi-Hui] City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
   City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China.
RP Wu, QH (reprint author), City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
EM qihuiwu@cityu.edu.hk; apwjzh@cityu.edu.hk
RI Zhang, WJ/C-6995-2012; Wang, C.D. /D-5912-2012; Chen,
   Xianfeng/D-1709-2010
OI Chen, Xianfeng/0000-0002-3189-2756
FU National Natural Science Foundation of China (NCFC) [61176007]; Research
   Grants Council of the Hong Kong Special Administrative Region, China
   [CityU 102010]
FX This work was supported by National Natural Science Foundation of China
   (NCFC Grant 61176007) and Research Grants Council of the Hong Kong
   Special Administrative Region, China (Project no. CityU 102010).
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NR 52
TC 48
Z9 49
U1 25
U2 142
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 21
BP 10599
EP 10604
DI 10.1039/c3nr02872k
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 235ZH
UT WOS:000325762000066
PM 24057017
ER

PT J
AU Sun, YM
   Hu, XL
   Luo, W
   Huang, YH
AF Sun, Yongming
   Hu, Xianluo
   Luo, Wei
   Huang, Yunhui
TI Ultrathin CoO/Graphene Hybrid Nanosheets: A Highly Stable Anode Material
   for Lithium-Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID IMPROVED REVERSIBLE CAPACITY; ELECTRODE MATERIALS; STORAGE CAPACITY;
   CYCLIC PERFORMANCE; NANOWIRE ARRAYS; GRAPHITE OXIDE; HOLLOW SPHERES;
   BINDER-FREE; COO; LI
AB Transition metal oxides are promising high-capacity anode materials for next-generation lithium-ion batteries. However, their cycle life remains insufficient for commercial applications. Developing transition-metal oxide anode materials with a long lifespan through a facile route has become an important issue. This work reports the fabrication of ultrathin CoO/graphene hybrid nanosheets consisting of ultrafine CoO nanoparticles (similar to 5 nm) densely anchored on the graphene nanosheets. They exhibit a high reversible capacity of similar to 1018.0 mAh g(-1) over 520 discharge/charge cycles, and the Coulombic efficiency remains similar to 100% upon cycling, indicating excellent cyclability. The as-obtained CoO/graphene nanocomposite avoids the widespread problem of cracking or pulverization of transition-metal oxide anode materials upon cycling and retains its original morphology and structure even after 520 discharge/charge cycles, benefiting from the synergetic effects of ultrafine CoO nanoparticles and the conductive graphene nanosheets.
C1 [Sun, Yongming; Hu, Xianluo; Luo, Wei; Huang, Yunhui] Huazhong Univ Sci & Technol, Coll Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China.
RP Hu, XL (reprint author), Huazhong Univ Sci & Technol, Coll Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China.
EM huxl@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Luo, Wei/E-1582-2011; Sun, Yongming/G-7799-2012; Huang,
   Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU Natural Science Foundation of China [51002057, 21271078, 50825203]; 863
   program [2009AA03Z225]; Natural Science Foundation of Hubei Province
   [2008CDA026]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 51002057, 21271078 and 50825203), the 863 program (Grant No.
   2009AA03Z225), the Natural Science Foundation of Hubei Province (Grant
   No. 2008CDA026), and the PCSIRT (Program for Changjiang Scholars and
   Innovative Research Team in University). The authors thank Analytical
   and Testing Center of HUST for the XRD and TG/DTA measurements.
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NR 65
TC 48
Z9 51
U1 20
U2 172
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD OCT 4
PY 2012
VL 116
IS 39
BP 20794
EP 20799
DI 10.1021/jp3070147
PG 6
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 014KX
UT WOS:000309375700018
ER

PT J
AU Lian, PC
   Liang, SZ
   Zhu, XF
   Yang, WS
   Wang, HH
AF Lian, Peichao
   Liang, Shuzhao
   Zhu, Xuefeng
   Yang, Weishen
   Wang, Haihui
TI A novel Fe3O4-SnO2-graphene ternary nanocomposite as an anode material
   for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene sheets; Fe3O4; SnO2; Nanocomposite; Lithium-ion batteries
ID REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; AMORPHOUS OXIDE; STORAGE;
   COMPOSITE; TIN; FABRICATION; ELECTRODES; NANOWIRES; STABILITY
AB Fe3O4-SnO2-graphene ternary nanocomposite was firstly synthesized by using a gas-liquid interfacial synthesis approach. The as-prepared nanocomposite was characterized by X-ray diffraction, field emission scanning electron microscopy, and transmission electron microscopy. The scanning electron microscopy and transmission electron microscopy characterization results indicate that Fe3O4-SnO2 nanoparticles were successfully deposited onto the surfaces of graphene sheets during the gas-liquid interfacial reaction process. The electrochemical performances were evaluated by using coin-type cells vs. metallic lithium. The Fe3O4-SnO2-graphene nanocomposite exhibits a high reversible specific capacity of 1198 mAh g(-1) in the 115th cycle at a specific current of 100 mA g(-1) and good rate capability, even at a high specific current of 2000 mA g(-1), the reversible capacity is still as high as 521 mAh g(-1). The good electrochemical performance of the Fe3O4-SnO2-graphene nanocomposite can be attributed to the synergistic effect existing not only between the graphene and metal oxides but also between the Fe3O4 and SnO2. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Lian, Peichao; Liang, Shuzhao; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620
FU National Natural Science Foundation of China [20936001]; SCUT
   [2009220038]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 20936001) and the Fundamental Research Funds
   for the Central Universities, SCUT (2009220038).
CR Li C, 2010, J POWER SOURCES, V195, P2939, DOI 10.1016/j.jpowsour.2009.11.005
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NR 40
TC 48
Z9 51
U1 18
U2 154
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD DEC 30
PY 2011
VL 58
BP 81
EP 88
DI 10.1016/j.electacta.2011.08.088
PG 8
WC Electrochemistry
SC Electrochemistry
GA 871VH
UT WOS:000298765300012
ER

PT J
AU Xiao, XC
   Liu, P
   Wang, JS
   Verbrugge, MW
   Balogh, MP
AF Xiao, Xingcheng
   Liu, Ping
   Wang, John S.
   Verbrugge, M. W.
   Balogh, Michael P.
TI Vertically aligned graphene electrode for lithium ion battery with high
   rate capability
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Graphene; Lithium ion battery; High rate capability; Nanostructure
ID CARBON NANOWALLS; STORAGE; GRAPHITE; BEHAVIOR; ANODE
AB In this paper, we demonstrated that the high rate capability of electrode can be achieved by engineering the existing electrode materials. A simple approach has been developed to align the graphene nanosheet vertically on current collector, which not only facilitates both lithium ion and electron transport, but also simplifies the electrode fabrication without involving binder and conductive additives. The charging rate for the optimized electrode structure can be significantly increased while the graphitic feature of the electrode still retains. We envision the use of this highly stable structure as an integral addition to high capacity anode materials for lithium ion batteries of high power and energy density. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Xiao, Xingcheng; Verbrugge, M. W.; Balogh, Michael P.] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
   [Liu, Ping; Wang, John S.] HRL Labs, Malibu, CA 90265 USA.
RP Xiao, XC (reprint author), Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
EM Xingcheng.Xiao@gm.com; pliu@hrl.com; mark.w.verbrugge@gm.com
RI Liu, Ping/I-5615-2012
CR Kaskhedikar NA, 2009, ADV MATER, V21, P2664, DOI 10.1002/adma.200901079
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NR 16
TC 48
Z9 48
U1 2
U2 53
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD FEB
PY 2011
VL 13
IS 2
BP 209
EP 212
DI 10.1016/j.elecom.2010.12.016
PG 4
WC Electrochemistry
SC Electrochemistry
GA 725AN
UT WOS:000287617700028
ER

PT J
AU Habazaki, H
   Kiriu, M
   Konno, H
AF Habazaki, H.
   Kiriu, M.
   Konno, H.
TI High rate capability of carbon nanofilaments with platelet structure as
   anode materials for lithium ion batteries
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE carbon nanofilaments; platelet structure; lithium ion battery; rate
   capability; intercalation reaction
ID TEMPLATE SYNTHESIS; HIGH-CAPACITY; ELECTRODES; INSERTION; PERFORMANCE;
   NANOFIBERS; ENERGY
AB Carbon nanofilaments (CNFs) with platelet structure have been prepared by liquid phase carbonization using porous anodic alumina template, and their lithium ion insertion/extraction properties have been examined as a function of heat treatment temperature and filament diameter. The CNFs heat-treated at 1000 degrees C reveal higher capacitance and higher rate capability compared with those heat-treated at higher temperatures. Further, it is found that higher reversible capacity is obtained for the CNFs with reduced diameter. The reversible capacity of highly graphitized CNFs formed at 2800 degrees C is less than 200 mA h g(-1) at a current density of 50 mA g(-1), being far lower than the theoretical capacity (372 mA h g(-1)) of graphite. A probable reason is the presence of loop at the edge of graphene layers. (c) 2006 Elsevier B.V. All rights reserved.
C1 Hokkaido Univ, Grad Sch Engn, Sapporo, Hokkaido 0608628, Japan.
RP Habazaki, H (reprint author), Hokkaido Univ, Grad Sch Engn, N13-W8, Sapporo, Hokkaido 0608628, Japan.
EM habazaki@eng.hokudai.ac.jp
RI Habazaki, Hiroki/C-5388-2012
OI Habazaki, Hiroki/0000-0002-7172-8811
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NR 16
TC 48
Z9 48
U1 4
U2 25
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD AUG
PY 2006
VL 8
IS 8
BP 1275
EP 1279
DI 10.1016/j.elecom.2006.06.012
PG 5
WC Electrochemistry
SC Electrochemistry
GA 075FY
UT WOS:000239870800015
ER

PT J
AU Yang, GZ
   Cui, H
   Yang, GW
   Wang, CX
AF Yang, Gongzheng
   Cui, Hao
   Yang, Guowei
   Wang, Chengxin
TI Self-Assembly of Co3V2O8 Multi layered Nanosheets: Controllable
   Synthesis, Excellent Li-Storage Properties, and Investigation of
   Electrochemical Mechanism
SO ACS NANO
LA English
DT Article
DE Co3V2O8; self-assembly; nanosheets; lithium ion battery anodes;
   excellent Li-storage property; electrochemical mechanism
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; NANOSTRUCTURED MATERIALS;
   ENERGY-CONVERSION; SANDWICH-LIKE; PERFORMANCE; GRAPHENE; NANOWIRES;
   OXIDE; NANOPARTICLES
AB Developing electrode materials with both high energy and power densities holds the key for satisfying the urgent demand of energy storage worldwide. Herein, we demonstrate the successful preparation of Co3V2O8 nanostructures that are constructed from self-assembly of ultrathin nanosheets via a simple hydrothermal method followed by annealing in air at 350 degrees C for 2 h. A "slipping-exfoliating-self reassembly" model based on the time-dependent experiments was proposed to elucidate the formation of the hierarchical nanosheets. When tested as lithium ion anodes, the as-synthesized multilayered nanoarchitectures exhibit outstanding reversible capacity (1114 mA h g(-1) retained after 100 cycles) and excellent rate performance (361 mA h g(-1) at a high current density of 10 A g(-1)) for lithium storage. Detailed investigations of the morphological and structural changes of Co3V2O8 upon cycling reveal an interesting kinetics toward lithium ion intercalations, where reversible conversion reactions between Co and CoO are found proceeding on the amorphous lithiated vanadium oxides matrixes. We believe that this observation is a valuable discovery for metal vandates-based lithium ion anodes. The superior electrochemical performances of the multilayered Co3V2O8 nanosheets can be attributed to the unique morphologies and particularly the surface-to-surface constructions that are generated during the lithium ion insertion processes.
C1 [Yang, Gongzheng; Cui, Hao; Yang, Guowei; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
   [Cui, Hao; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China.
RP Wang, CX (reprint author), Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
EM wchengx@mail.sysu.edu.cn
FU National Natural Science Foundation of China [51125008, 11274392]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 51125008 and No. 11274392).
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NR 47
TC 47
Z9 47
U1 80
U2 225
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD MAY
PY 2014
VL 8
IS 5
BP 4474
EP 4487
DI 10.1021/nn406449u
PG 14
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AI1UM
UT WOS:000336640600037
PM 24684444
ER

PT J
AU Zhang, LP
   Niu, JB
   Li, MT
   Xia, ZH
AF Zhang, Lipeng
   Niu, Jianbing
   Li, Mingtao
   Xia, Zhenhai
TI Catalytic Mechanisms of Sulfur-Doped Graphene as Efficient Oxygen
   Reduction Reaction Catalysts for Fuel Cells
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID METAL-FREE ELECTROCATALYSTS; LITHIUM ION BATTERIES; MONOLAYER GRAPHENE;
   CARBON NANOTUBES; SHEETS; PERFORMANCE; GRAPHITE; CATHODE; ARRAYS; ANODE
AB Density functional theory (DFT) was applied to study sulfur-doped graphene clusters as oxygen reduction reaction (ORR) cathode catalysts for fuel cells. Several sulfur-doped graphene clusters with/without Stone-Wales defects were investigated and their electronic structures, reaction free energy, transition states, and energy barriers were calculated to predict their catalytic properties. The results show that sulfur atoms could be adsorbed on the graphene surface, substitute carbon atoms at the graphene edges in the form of sulfur/sulfur oxide, or connect two graphene sheets by forming a sulfur cluster ring. These sulfur-doped graphene clusters with sulfur or sulfur oxide locating at graphene edges show electrocatalytic activity for ORR. Catalytic active sites distribute at the zigzag edge or the neighboring carbon atoms of doped sulfur oxide atoms, which possess large spin or charge density. For those being the active catalytic sites, sulfur atoms with the highest charge density take a two-electron transfer pathway while the carbon atoms with high spin or charge density follow a four-electron transfer pathway. It was predicted from the reaction energy barriers that the sulfur-doped graphene could show ORR catalytic properties comparable to platinum. The prediction is consistent with the experimental results on S-doped graphene.
C1 [Zhang, Lipeng; Niu, Jianbing; Li, Mingtao; Xia, Zhenhai] Univ N Texas, Dept Chem, Dept Mat Sci & Engn, Denton, TX 76203 USA.
RP Xia, ZH (reprint author), Univ N Texas, Dept Chem, Dept Mat Sci & Engn, Denton, TX 76203 USA.
EM zhenhai.xia@unt.edu
RI Li, Mingtao/N-3468-2014
FU AFOSR MURI [FA9550-12-1-0037]; National Science Foundation [IIP-1343270,
   CMMI-1212259]
FX The authors acknowledge the support from AFOSR MURI (FA9550-12-1-0037)
   and the National Science Foundation (IIP-1343270 and CMMI-1212259).
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TC 47
Z9 48
U1 51
U2 276
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD FEB 20
PY 2014
VL 118
IS 7
BP 3545
EP 3553
DI 10.1021/jp410501u
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AB5XJ
UT WOS:000331861700020
ER

PT J
AU Huang, X
   Yu, H
   Chen, J
   Lu, ZY
   Yazami, R
   Hng, HH
AF Huang, Xin
   Yu, Hong
   Chen, Jing
   Lu, Ziyang
   Yazami, Rachid
   Hng, Huey Hoon
TI Ultrahigh Rate Capabilities of Lithium-Ion Batteries from 3D Ordered
   Hierarchically Porous Electrodes with Entrapped Active Nanoparticles
   Configuration
SO ADVANCED MATERIALS
LA English
DT Article
DE lithium-ion batteries; ultrahigh rate capabilities; hierarchically
   porous electrodes; transition metal oxides; entrapped-active
   nanoparticles
ID ADVANCED ENERGY-CONVERSION; ANODE MATERIALS; GRAPHENE SHEETS;
   HIGH-CAPACITY; STORAGE; COMPOSITE; SUPERCAPACITORS; POLYMERIZATION;
   NANOMATERIALS; CHALLENGES
C1 [Huang, Xin; Yu, Hong; Chen, Jing; Lu, Ziyang; Hng, Huey Hoon] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Yu, Hong; Chen, Jing; Yazami, Rachid] Nanyang Technol Univ, Energy Res Inst, Singapore 639798, Singapore.
RP Huang, X (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM xhuang@ntu.edu.sg; ashhhng@ntu.edu.sg
RI Lu, Ziyang /L-7857-2014; Hng, Huey Hoon/A-2246-2011
OI Hng, Huey Hoon/0000-0002-8950-025X
FU Singapore Ministry of Education [MOE2010-T2-1-017]; AstarSTAR SERC
   (Singapore) [1021700144, NRF2009EWT-CERP001-026]; Singapore National
   Research Foundation under CREATE program: EMobility in Megacities;
   Singapore MPA [23/04.15.03 RDP 020/10/113]
FX This work was supported by Singapore Ministry of Education
   (MOE2010-T2-1-017), A<SUP>star</SUP>STAR SERC grant 1021700144,
   NRF2009EWT-CERP001-026 (Singapore), Singapore National Research
   Foundation under CREATE program: EMobility in Megacities, and Singapore
   MPA 23/04.15.03 RDP 020/10/113 grant.
CR Shi Y, 2011, J POWER SOURCES, V196, P8610, DOI 10.1016/j.jpowsour.2011.06.002
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NR 38
TC 47
Z9 47
U1 19
U2 182
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD FEB
PY 2014
VL 26
IS 8
BP 1296
EP 1303
DI 10.1002/adma.201304467
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AB6OS
UT WOS:000331909900018
PM 24449491
ER

PT J
AU Jiang, X
   Yang, XL
   Zhu, YH
   Shen, JH
   Fan, KC
   Li, CZ
AF Jiang, Xin
   Yang, Xiaoling
   Zhu, Yihua
   Shen, Jianhua
   Fan, Kaicai
   Li, Chunzhong
TI In situ assembly of graphene sheets-supported SnS2 nanoplates into 3D
   macroporous aerogels for high-performance lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene; Tin disulfide; Anode; Lithium ion batteries; Aerogels
ID GAS-SENSING PROPERTY; PHOTOCATALYTIC ACTIVITY; CYCLIC PERFORMANCE;
   STORAGE; CAPACITY; OXIDE; LAYER; NANOSTRUCTURES; NANOSHEETS; ANODE
AB Three-dimensional (3D) SnS2/graphene aerogels (SnS2/G-As) have been successfully fabricated via an in situ macroscopy self-assembly of graphene sheets which embedded SnS2 nanoplates in a hydrothermal process, and then freeze-drying to maintain the 3D monolithic architectures. The graphene sheets in high concentration will be easily restacked into 3D architectures driven by combined hydrophobic and pi-pi stacking interactions during hydrothermal reduction process, meanwhile SnS2 facilitate stabilizing such novel graphene networks. The obtained SnS2/G-As show interconnected graphene networks, large surface area and large numbers of macropores. The novel 3D architectures in SnS2/G-As, which can provide rich sites for absorbing lithium ions and facilitate electrolyte contact as well as ionic diffusion, combined with the synergistic effect between the layered SnS2 and the graphene make SnS2/G-As achieve high reversible capacity (656 mA h g(-1) with a coulombic efficiency of over 95% after 30 cycles) and excellent rate capability (240 mA h g(-1) at the rate of 1000 mA g(-1)) when used as an anode in rechargeable LIBs. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Jiang, Xin; Yang, Xiaoling; Zhu, Yihua; Shen, Jianhua; Fan, Kaicai; Li, Chunzhong] E China Univ Sci & Technol, Sch Mat Sci & Engn, Minist Educ, Key Lab Ultrafine Mat, Shanghai 200237, Peoples R China.
RP Zhu, YH (reprint author), E China Univ Sci & Technol, Sch Mat Sci & Engn, Minist Educ, Key Lab Ultrafine Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China.
EM yhzhu@ecust.edu.cn
RI Li, Chunzhong/B-1103-2015
OI Li, Chunzhong/0000-0001-7897-5850
FU National Natural Science Foundation of China [21236003, 21206042,
   20925621, 20976054, 21176083]; Special Projects for Nanotechnology of
   Shanghai [11nm0500800]; Fundamental Research Funds for the Central
   Universities [WD1013015, WD1114005]; Program for Changjiang Scholars and
   Innovative Research Team in University [IRT0825]; Shanghai Leading
   Academic Discipline Project [B502]
FX We thank the National Natural Science Foundation of China (21236003,
   21206042, 20925621, 20976054, and 21176083), the Special Projects for
   Nanotechnology of Shanghai (11nm0500800) the Fundamental Research Funds
   for the Central Universities (WD1013015 and WD1114005), and the Program
   for Changjiang Scholars and Innovative Research Team in University
   (IRT0825), and the Shanghai Leading Academic Discipline Project (project
   number: B502) for financial supports.
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NR 59
TC 47
Z9 47
U1 41
U2 264
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 1
PY 2013
VL 237
BP 178
EP 186
DI 10.1016/j.jpowsour.2013.03.048
PG 9
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 173NH
UT WOS:000321085700026
ER

PT J
AU Rai, AK
   Gim, J
   Anh, LT
   Kim, J
AF Rai, Alok Kumar
   Gim, Jihyeon
   Ly Tuan Anh
   Kim, Jaekook
TI Partially reduced Co3O4/graphene nanocomposite as an anode material for
   secondary lithium ion battery
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Cobalt oxide; Graphene nanosheets; Anode; Lithium ion batteries
ID NEGATIVE ELECTRODE MATERIAL; COBALT OXIDE COMPOSITES; ELECTROCHEMICAL
   PERFORMANCE; HYDROTHERMAL SYNTHESIS; REVERSIBLE CAPACITY; CO3O4
   NANOPARTICLES; CYCLIC PERFORMANCE; STORAGE PROPERTIES; RATE CAPABILITY;
   CARBON
AB A simple urea-assisted, auto-combustion synthesis was used to fabricate pure Co3O4 nanoparticles and their nanocomposite with 10 wt% reduced graphene nanosheets. Samples were annealed at 500 degrees C for 5 h under nitrogen atmosphere and their structures and morphologies were characterized by X-ray diffraction, field-emission scanning electron microscopy, field-emission transmission electron microscopy, Raman spectroscopy and BET surface area analysis. The process led to a nanocomposite containing small (25-50 nm) Co3O4 nanoparticles deposited on the graphene nanosheets. CHN analysis determined the carbon content in pure Co3O4 nanoparticles and Co3O4/CoO/graphene nanocomposite and found to be very low such as 0.091% and 2.41% respectively. In addition, to know the precise amount of CoO in the designed nanocomposite sample, phase fraction Le Bail's technique was used and found to be 20 +/- 0.5%. Using the Co3O4/CoO/graphene nanocomposite as an anode in lithium ion battery led to a higher lithium storage capacity than using pure Co3O4 nanoparticles electrode. The Co3O4/CoO/graphene nanocomposite electrode delivered an initial charge capacity of 890.44 mAh g(-1) and Exhibit 90% of good capacity retention (801.31 mAhg(-1)) after 30 cycles. While pure Co3O4 nanoparticles electrode (877.98 mAh g(-1)) fades quickly, retains only 60% (523.94 mAh g(-1)) after 30 cycles. The improved electrochemical performance of nanocomposite was attributed to higher electron and Li+ ion conductivity and the larger surface area and mechanical flexibility afforded by the graphene nanosheets. At high current densities, both electrodes showed comparable reversible capacities, demonstrating the suitability of the present synthetic technique. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Rai, Alok Kumar; Gim, Jihyeon; Ly Tuan Anh; Kim, Jaekook] Chonnam Natl Univ, Dept Mat Sci & Engn, Kwangju 500757, South Korea.
RP Kim, J (reprint author), Chonnam Natl Univ, Dept Mat Sci & Engn, 300 Yongbong Dong, Kwangju 500757, South Korea.
EM jaekook@chonnam.ac.kr
RI Rai,  Alok Kumar/N-3007-2014
FU World Class University (WCU) program through the Korea Science and
   Engineering Foundation; Ministry of Education, Science and Technology
   [R32-20074, 2009-0094055]; Priority Research Centers Program through the
   National Research Foundation of Korea (NRF)
FX This research was supported by World Class University (WCU) program
   through the Korea Science and Engineering Foundation funded by the
   Ministry of Education, Science and Technology (R32-20074). This work was
   also supported by Priority Research Centers Program through the National
   Research Foundation of Korea (NRF) funded by the Ministry of Education,
   Science and Technology (2009-0094055).
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NR 59
TC 47
Z9 47
U1 15
U2 195
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JUN 30
PY 2013
VL 100
BP 63
EP 71
DI 10.1016/j.electacta.2013.03.140
PG 9
WC Electrochemistry
SC Electrochemistry
GA 165OE
UT WOS:000320492400009
ER

PT J
AU Vinayan, BP
   Ramaprabhu, S
AF Vinayan, B. P.
   Ramaprabhu, S.
TI Facile synthesis of SnO2 nanoparticles dispersed nitrogen doped graphene
   anode material for ultrahigh capacity lithium ion battery applications
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID CARBON; PERFORMANCE; ELECTRODES; OXIDE
AB We report a facile strategy to synthesize SnO2 nanoparticles dispersed nitrogen doped graphene (SnO2/NG). Nitrogen doping of graphene was carried out by the pyrolysis of polypyrrole coated poly(sodium 4-styrenesulfonate) functionalized graphene. The SnO2 nanoparticles are dispersed over nitrogen doped graphene by a modified polyol reduction method. The dispersed SnO2 nanoparticles are 2-3 nm in size with homogeneous dispersion and good crystallinity. The SnO2/NG as an anode material in Li ion batteries displays superior reversible capacity, very good rate capability and excellent cyclic performance (1220 mA h g(-1) after 100th cycle). The impedance measurements show that nitrogen doping can significantly reduce the charge transfer resistance of graphene based electrodes. The factors contributing to the excellent electrochemical performance of the SnO2/NG anode material is discussed. The present work opens a new pathway for the development of metal or metal oxide nanoparticle-nitrogen doped carbon nano-structure based nanocomposites for high performance electrochemical energy devices.
C1 [Vinayan, B. P.; Ramaprabhu, S.] Indian Inst Technol, NFMTC, AENL, Dept Phys, Madras 600036, Tamil Nadu, India.
RP Vinayan, BP (reprint author), Indian Inst Technol, NFMTC, AENL, Dept Phys, Madras 600036, Tamil Nadu, India.
EM ramp@iitm.ac.in
RI S, Ramaprabhu/A-1071-2014
FU IITM, Chennai; DRDO, Government of India
FX The authors are grateful to IITM, Chennai and DRDO, Government of India
   for their support.
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NR 33
TC 47
Z9 48
U1 16
U2 147
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 12
BP 3865
EP 3871
DI 10.1039/c3ta01515g
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 095TB
UT WOS:000315356500006
ER

PT J
AU Wang, B
   Luo, B
   Li, XL
   Zhi, LJ
AF Wang, Bin
   Luo, Bin
   Li, Xianglong
   Zhi, Linjie
TI The dimensionality of Sn anodes in Li-ion batteries
SO MATERIALS TODAY
LA English
DT Article
ID RECHARGEABLE LITHIUM BATTERIES; AT-CNT NANOSTRUCTURES; HOLLOW CARBON;
   TIN OXIDE; ELECTROCHEMICAL LITHIATION; STORAGE CAPABILITY; AMORPHOUS
   OXIDE; GRAPHENE; COMPOSITE; PERFORMANCE
AB As a potential anode material, tin (Sn) has attracted great attention due to its low cost and its high theoretical specific capacity. However, its electrochemical performance is strongly related to its structure, including the crystalline nature, particle size, dimensionality, interface, and so on. In this review article, we will outline Sn-based nanomaterials with different dimensionalities from 0D to 3D, covering the synthesis procedures and their structure-related electrochemical performances when applied as anode materials in lithium ion batteries (LIBs). By discussing their structural dimensionalities, we aim to provide some scientific insights into the development of advanced Sn-based anode nanomaterials for next-generation LIBs.
C1 [Wang, Bin; Luo, Bin; Li, Xianglong; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Zhi, LJ (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
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NR 71
TC 47
Z9 47
U1 22
U2 159
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 1369-7021
J9 MATER TODAY
JI Mater. Today
PD DEC
PY 2012
VL 15
IS 12
BP 544
EP 552
PG 9
WC Materials Science, Multidisciplinary
SC Materials Science
GA 077YX
UT WOS:000314066400012
ER

PT J
AU Jiang, KC
   Wu, XL
   Yin, YX
   Lee, JS
   Kim, J
   Guo, YG
AF Jiang, Ke-Cheng
   Wu, Xing-Long
   Yin, Ya-Xia
   Lee, Jong-Sook
   Kim, Jaekook
   Guo, Yu-Guo
TI Superior Hybrid Cathode Material Containing Lithium-Excess Layered
   Material and Graphene for Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium-ion batteries; hybrid materials; cathode; lithium-excess layered
   materials; graphene
ID IRREVERSIBLE CAPACITY LOSS; CARBON NANOPARTICLES; SURFACE MODIFICATION;
   ANODE MATERIAL; LI-ION; COMPOSITE; PERFORMANCE; NANOFIBERS; ELECTRODES;
   EFFICIENT
AB Graphene-wrapped lithium-excess layered hybrid materials (Li2MnO3 center dot LiMO2, M = Mn, Ni, Co, hereafter abbreviated as LMNCO) have been synthesized and investigated as cathode materials for lithium-ion batteries. Cyclic voltammetry measurement shows a significant reduction of the reaction overpotential in benefit of the graphene conducting framework. The electrochemical impedance spectroscopy results reveal that the graphene can greatly reduce the cell resistance, especially the charge transfer resistance. Our investigation demonstrates that the graphene conducting framework can efficiently alleviate the polarization of pristine LMNCO material leading to an outstanding enhancement in cell performance and cycling stability. The superior electrochemical properties support the fine hybrid structure design by enwrapping active materials in graphene nanosheets for high-capacity and high-rate cathode materials.
C1 [Jiang, Ke-Cheng; Wu, Xing-Long; Yin, Ya-Xia; Guo, Yu-Guo] Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
   [Jiang, Ke-Cheng; Wu, Xing-Long; Yin, Ya-Xia; Guo, Yu-Guo] Chinese Acad Sci, Beijing Natl Lab Mol Sci BNLMS, Beijing 100190, Peoples R China.
   [Lee, Jong-Sook; Kim, Jaekook; Guo, Yu-Guo] Chonnam Natl Univ WCU, Sch Mat Sci & Engn, Kwangju 500757, South Korea.
RP Guo, YG (reprint author), Chinese Acad Sci, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn
RI Wu, Xing-Long/J-8388-2012; Lee, Jong-Sook/D-1035-2013; Guo,
   Yu-Guo/A-1223-2009
OI Wu, Xing-Long/0000-0003-1069-9145; Lee, Jong-Sook/0000-0002-2227-0808;
   Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2012CB932900, 2011CB935700];
   National Natural Science Foundation of China [91127044, 21121063]; WCU
   program through NRF; MEST [R32-2009-000-20074-0]; Chinese Academy of
   Sciences
FX This work was supported by the National Basic Research Program of China
   (Grants 2012CB932900 and 2011CB935700), the National Natural Science
   Foundation of China (Grants 91127044 and 21121063), the WCU program
   through NRF funded by MEST (R32-2009-000-20074-0), and the Chinese
   Academy of Sciences. The authors thank Prof. A. M. Cao for helpful
   discussions.
CR Zhang LS, 2010, J MATER CHEM, V20, P5462, DOI 10.1039/c0jm00672f
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NR 30
TC 47
Z9 50
U1 12
U2 127
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD SEP
PY 2012
VL 4
IS 9
BP 4858
EP 4863
DI 10.1021/am301202a
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 010MZ
UT WOS:000309099800060
PM 22931115
ER

PT J
AU Wang, DW
   Li, YQ
   Wang, QH
   Wang, TM
AF Wang, Dewei
   Li, Yuqi
   Wang, Qihua
   Wang, Tingmei
TI Facile Synthesis of Porous Mn3O4 Nanocrystal-Graphene Nanocomposites for
   Electrochemical Supercapacitors
SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
LA English
DT Article
DE Manganese; Nanoparticles; Graphene; Energy conversion; Electrochemistry;
   Supercapacitors
ID LITHIUM ION BATTERIES; CAPACITY ANODE MATERIAL; LOW-TEMPERATURE;
   HYDROTHERMAL SYNTHESIS; STORAGE; OXIDE; PERFORMANCE; ULTRACAPACITORS;
   NANOPARTICLES; CONVERSION
AB In this work, we describe our efforts to produce Mn3O4-graphene nanocomposites based on a convenient and feasible solution based synthetic route under mild conditions. According to transmission electron microscopy (TEM) and high angle annular dark field scanning transmission electron microscopy (HAADF-STEM) results porous Mn3O4 nanocrystals (NCs), 20-40 nm in size, are uniformly deposited on both sides of the graphene nanosheet (GNS) matrix. Significantly, the as-prepared Mn3O4-graphene nanocomposites exhibit remarkable pseudocapacitive activity including high specific capacitance (236.7 Fg(-1) at 1 Ag-1), good rate capability (133 Fg(-1) at 8 Ag-1), and excellent cyclability (the specific capacitance only decreases by 6.32% of the initial capacitance after 1000 cycles). The excellent pseudocapacitive performance of the Mn3O4-graphene nanocomposites electrode is probably due to the positive synergistic effects between the Mn3O4 and GNS. Namely, the intimate combination of the conductive graphene network with uniformly dispersed porous Mn3O4 NCs not only greatly improves the electrochemical utilization of Mn3O4, but also increases the double-layer capacitance of the graphene sheets. These characteristics make this nanocomposite a very promising electrode material for high performance supercapacitors.
C1 [Wang, Dewei; Li, Yuqi; Wang, Qihua; Wang, Tingmei] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China.
   [Wang, Dewei; Li, Yuqi] Chinese Acad Sci, Grad Sch, Beijing 10039, Peoples R China.
RP Wang, QH (reprint author), Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China.
EM Wangqh@lzb.ac.cn
RI Wang, Dewei/E-5026-2010; li, yuqi/J-5090-2012
FU National Science Foundation for Distinguished Young Scholars of China
   [51025517]; National 973 project of China [2007CB607606]; National
   Defense Basic Scientific Research Project [A1320110011]
FX The authors would like to acknowledge the financial support of the
   National Science Foundation for Distinguished Young Scholars of China
   (grant number 51025517), the financial support of the National 973
   project of China (2007CB607606) and National Defense Basic Scientific
   Research Project (A1320110011). The authors would gratefully thank Dr.
   Liming Tao at the State Key Laboratory of Solid Lubrication for his kind
   assistances.
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NR 57
TC 47
Z9 47
U1 18
U2 178
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 1434-1948
J9 EUR J INORG CHEM
JI Eur. J. Inorg. Chem.
PD FEB
PY 2012
IS 4
BP 628
EP 635
DI 10.1002/ejic.201100983
PG 8
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 908LC
UT WOS:000301490900004
ER

PT J
AU Chen, DZ
   Wei, W
   Wang, RN
   Zhu, JC
   Guo, L
AF Chen, Dezhi
   Wei, Wei
   Wang, Ruining
   Zhu, Jingchao
   Guo, Lin
TI alpha-Fe2O3 nanoparticles anchored on graphene with 3D quasi-laminated
   architecture: in situ wet chemistry synthesis and enhanced
   electrochemical performance for lithium ion batteries
SO NEW JOURNAL OF CHEMISTRY
LA English
DT Article
ID ANODE MATERIAL; REVERSIBLE CAPACITY; ELECTRODE MATERIALS;
   NEGATIVE-ELECTRODE; STORAGE PROPERTIES; GRAPHITE OXIDE; COMPOSITE;
   NANOCOMPOSITE; CONVERSION; NANOSTRUCTURES
AB A novel alpha-Fe2O3/graphene composite is prepared by a simple in situ wet chemistry approach. The alpha-Fe2O3 particles with diameter around 130 nm are homogeneously anchored on graphene nanosheets to form a 3D quasi-laminated architecture. Such a well-organized flexible structure can offer sufficient void space to facilitate the electrolyte penetration, alleviate the effect of the volume change of alpha-Fe2O3 particles and avoid particle-particle aggregation during lithium insertion/desertion. In addition, graphene not only improves the electric conductivity of the composite electrode but also maintains the structural integrity of the composite electrode during long-term cycling. As anode material for Li-ion batteries, the alpha-Fe2O3/graphene composite electrode exhibits a stable capacity of 742 mAh g(-1) up to 50 cycles. The synthesis technique is suitable for practical large-scale production of graphene-based metal oxide composites as advanced electrode materials for rechargeable Li-ion batteries.
C1 [Chen, Dezhi; Wei, Wei; Wang, Ruining; Zhu, Jingchao; Guo, Lin] Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China.
   [Chen, Dezhi] Nanchang Hangkong Univ, Sch Environm & Chem Engn, Nanchang 330063, Peoples R China.
RP Guo, L (reprint author), Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China.
EM guolin@buaa.edu.cn
RI Wang, Ruining/H-5079-2012
OI Wang, Ruining/0000-0003-4638-1454
FU National Basic Research Program of China [2010CB934700]; NSFC [11079002,
   20973019]; Fundamental Research Funds for the Central Universities
FX The authors are thankful for financial support from National Basic
   Research Program of China (No. 2010CB934700), NSFC (11079002 & 20973019)
   and the Fundamental Research Funds for the Central Universities.
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NR 64
TC 47
Z9 47
U1 14
U2 113
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1144-0546
EI 1369-9261
J9 NEW J CHEM
JI New J. Chem.
PY 2012
VL 36
IS 8
BP 1589
EP 1595
DI 10.1039/c2nj40151g
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA 974FK
UT WOS:000306415700011
ER

PT J
AU Wang, X
   Song, L
   Yang, HY
   Xing, WY
   Lu, HD
   Hu, Y
AF Wang, Xin
   Song, Lei
   Yang, Hongyu
   Xing, Weiyi
   Lu, Hongdian
   Hu, Yuan
TI Cobalt oxide/graphene composite for highly efficient CO oxidation and
   its application in reducing the fire hazards of aliphatic polyesters
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; GRAPHITE; GRAPHENE; DEGRADATION; CARBON; ROUTE;
   FILMS; ANODE
AB Tricobalt tetraoxide-functionalized graphene composites (Co3O4/graphene) were prepared to reduce the fire hazards of aliphatic polyesters. Characterization of the Co3O4/graphene by X-ray diffraction (XRD), Raman spectroscopy, transmission electron microscope (TEM) and atomic force microscopy (AFM) confirmed the chemical structure. The incorporation of Co3O4/graphene into both poly (butylene succinate) (PBS) and polylactide (PLA) improved the initial degradation temperature, and slowed down the thermal decomposition process. The heat release rate of PBS-Co3O4/graphene and PLA-Co3O4/graphene composites were reduced by 31% and 40%, respectively, compared with that of the pure PBS and PLA. Moreover, the addition of Co3O4/graphene significantly decreased the gaseous products, including hydrocarbons, carbonyl compounds and carbon monoxide, which is attributed to the combined properties of the barrier effect and high catalytic activity for CO oxidation of Co3O4/graphene.
C1 [Wang, Xin; Song, Lei; Yang, Hongyu; Xing, Weiyi; Lu, Hongdian; Hu, Yuan] Univ Sci & Technol China, State Key Lab Fire Sci, Hefei 230026, Anhui, Peoples R China.
   [Wang, Xin; Hu, Yuan] Univ Sci & Technol China, Suzhou Key Lab Urban Publ Safety, Suzhou Inst Adv Study, Suzhou 215123, Jiangsu, Peoples R China.
   [Lu, Hongdian] Hefei Univ, Dept Chem & Mat Engn, Key Lab Powder & Energy Mat, Hefei 230022, Anhui, Peoples R China.
RP Hu, Y (reprint author), Univ Sci & Technol China, State Key Lab Fire Sci, Hefei 230026, Anhui, Peoples R China.
EM yuanhu@ustc.edu.cn
FU National Natural Science Foundation of China [51036007]; National
   Natrual Science Foundation of China (NSFC); Civil Aviation
   Administration of China (CAAC) [61079015]; Guangdong Province [U1074001]
FX The work was financially supported by the National Natural Science
   Foundation of China (No. 51036007), the joint fund of National Natrual
   Science Foundation of China (NSFC) and Civil Aviation Administration of
   China (CAAC) (No. 61079015), the joint fund of NSFC and Guangdong
   Province (No. U1074001).
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NR 23
TC 47
Z9 50
U1 8
U2 83
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 8
BP 3426
EP 3431
DI 10.1039/c2jm15637g
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 884HL
UT WOS:000299695400024
ER

PT J
AU Zhang, L
   Lou, XW
AF Zhang, Lei
   Lou, Xiong Wen (David)
TI Hierarchical MoS2 Shells Supported on Carbon Spheres for Highly
   Reversible Lithium Storage
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE carbon spheres; core-shell structures; lithium-ion batteries; MoS2;
   nanostructures
ID METAL DICHALCOGENIDE NANOSHEETS; MOLYBDENUM-DISULFIDE MOS2; ION BATTERY
   APPLICATIONS; ELECTROCHEMICAL PERFORMANCE; ANODE MATERIALS; GRAPHENE;
   NANOSTRUCTURES; NANOCOMPOSITES; EXFOLIATION; COMPOSITES
AB Hierarchical MoS2 shells supported on carbon spheres (denoted as C@MoS2) have been synthesized through a one-step hydrothermal method. The obtained hierarchical C@MoS2 microspheres simultaneously integrate the structural and compositional design rationales for high-energy electrode materials based on two-dimensional (2D) nanosheets. When evaluated as an anode material for lithium-ion batteries (LIBs), the hierarchical C@MoS2 microspheres manifest high specific capacity, enhanced cycling stability and good rate capability.
C1 [Zhang, Lei; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM xwlou@ntu.edu.sg
RI Zhang, Lei/A-4182-2013; Lou , Xiong Wen (David)/D-2648-2009
OI Zhang, Lei/0000-0002-6385-5773; 
CR Bindumadhavan K, 2013, CHEM COMMUN, V49, P1823, DOI 10.1039/c3cc38598a
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NR 36
TC 46
Z9 46
U1 67
U2 290
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
EI 1521-3765
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD APR 25
PY 2014
VL 20
IS 18
BP 5219
EP 5223
DI 10.1002/chem.201400128
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA AF7FO
UT WOS:000334879500005
PM 24687902
ER

PT J
AU Choi, SH
   Kang, YC
AF Choi, Seung Ho
   Kang, Yun Chan
TI Crumpled Graphene-Molybdenum Oxide Composite Powders: Preparation and
   Application in Lithium-Ion Batteries
SO CHEMSUSCHEM
LA English
DT Article
DE anode materials; electrochemistry; graphene; lithium-ion batteries;
   molybdenum oxide
ID ELECTROCHEMICAL ENERGY-STORAGE; ENCAPSULATED SI NANOPARTICLES;
   PERFORMANCE ANODE MATERIALS; METAL-OXIDES; ELECTRODE; FABRICATION;
   NANOSHEETS; NANOSTRUCTURES; REDUCTION; ROUTE
AB Crumpled graphene-MoO2 composite powders are directly prepared by means of spray pyrolysis and from a stable graphene oxide colloidal solution in the presence of Mo ions. The crumpled graphene-MoO2 composite powders are transformed into MoO3-based composite powders after post-treatment at 300 degrees C. The transmission electron microscopy and dot-mapping images of the post-treatment composite powders show uniform distribution of MoO3 nanocrystals in the crumpled graphene powders. The two typical D and G bands of graphene are observed at 1350 and 1590 cm(-1), respectively, in the Raman spectrum of the graphene-MoO3 composite. In addition, the crumpled graphene-MoO3 powders exhibit superior electrochemical behavior compared to that of pure MoO3 as an anode material for lithium-ion batteries. The initial discharge capacities of the graphene-MoO3 composite and bare MoO3 powders at a current density of 2 Ag-1 are 1490 and 1225 mAhg(-1), respectively. The capacity retention of the graphene-MoO3 composite is 87% after the first cycle, whereas that of bare MoO3 is 47%, as measured after 100 cycles. The reversible discharge capacity of the graphene-MoO3 composite decreases slightly from 1228 to 845 mAhg(-1) as the current density increases from 0.5 to 3 Ag-1.
C1 [Choi, Seung Ho; Kang, Yun Chan] Konkuk Univ, Dept Chem Engn, Seoul 143701, South Korea.
RP Kang, YC (reprint author), Konkuk Univ, Dept Chem Engn, 1 Hwayang Dong, Seoul 143701, South Korea.
EM yckang@konkuk.ac.kr
RI Kang, Yun Chan/H-2457-2015
OI Kang, Yun Chan/0000-0001-5769-5761
FU National Research Foundation of Korea (NRF) - Korea government (MEST)
   [2012R1A2A2A02046367]; Basic Science Research Program through the
   National Research Foundation of Korea (NRF) - Ministry of Education,
   Science and Technology [2012R1A1B3002382]
FX This work was supported by the National Research Foundation of Korea
   (NRF) grant funded by the Korea government (MEST) (No.
   2012R1A2A2A02046367). This research was supported by Basic Science
   Research Program through the National Research Foundation of Korea (NRF)
   funded by the Ministry of Education, Science and Technology
   (2012R1A1B3002382).
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NR 43
TC 46
Z9 46
U1 26
U2 143
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1864-5631
EI 1864-564X
J9 CHEMSUSCHEM
JI ChemSusChem
PD FEB
PY 2014
VL 7
IS 2
BP 523
EP 528
DI 10.1002/cssc.201300838
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA AI3ZG
UT WOS:000336804000023
PM 24243867
ER

PT J
AU Cheng, JL
   Xin, HL
   Zheng, HM
   Wang, B
AF Cheng, Jianli
   Xin, Huolin
   Zheng, Haimei
   Wang, Bin
TI One-pot synthesis of carbon coated-SnO2/graphene-sheet nanocomposite
   with highly reversible lithium storage capability
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Lithium-ion battery; Tin dioxide; Graphene; One-pot synthesis
ID LI-ION BATTERY; SNO2 NEGATIVE ELECTRODE; ANODE MATERIALS;
   CHEMICAL-CHANGES; MESOPOROUS SNO2; GRAPHENE PAPER; COMPOSITE;
   PERFORMANCE; NANOTUBE; CAPACITY
AB We report a one-pot hydrothermal approach to synthesize carbon coated-SnO2/graphene-sheet (SnO2-C/GNS) nanocomposite. Strong oxidation-reduction reactions to produce GNS by the traditional Hummers' method are avoided. The experiments show that the glucose and tin tetrachloride can intercalate into the thin graphite flake to exfoliate graphite and form SnO2-C/GNS nanocomposite simultaneously during the hydrothermal process. The approach is quite simple and green. Meanwhile, the prepared SnO2-C/GNS nanocomposite as an anode material of lithium-ion batteries exhibits higher lithium storage capacity and better cycling performance compared to SnO2 nanoparticle and SnO2-C microsphere. It still delivers the reversible capacity of 703 mA h g(-1) after 80 cycles at a current density of 100 mA g(-1) and maintains 443 mA h g(-1) after 100 cycles at a current density of 1000 mA g(-1). The improvement in the performance of SnO2-C/GNS nanocomposite can be attributed to the fully confinement of SnO2 nanoparticles between the GNS and the carbon layer, which can effectively prevent the detachment and agglomeration of SnO2 and preserve the integrity of the nanostructure during charge/discharge cycling. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Cheng, Jianli; Wang, Bin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
   [Xin, Huolin; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Wang, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
EM binwang@lbl.gov
RI cheng, Jianli/K-1496-2014; Cheng, Jianli/K-4478-2014; Xin,
   Huolin/E-2747-2010
OI Xin, Huolin/0000-0002-6521-868X
FU National Center for Electron Microscopy, Lawrence Berkeley Lab; U.S.
   Department of Energy [DE-AC02-05CH11231]
FX The authors acknowledge support of the National Center for Electron
   Microscopy, Lawrence Berkeley Lab, which is supported by the U.S.
   Department of Energy under Contract # DE-AC02-05CH11231.
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NR 31
TC 46
Z9 47
U1 28
U2 267
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 15
PY 2013
VL 232
BP 152
EP 158
DI 10.1016/j.jpowsour.2013.01.025
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 141UU
UT WOS:000318752800020
ER

PT J
AU Chen, WM
   Qie, L
   Shen, Y
   Sun, YM
   Yuan, LX
   Hu, XL
   Zhang, WX
   Huang, YH
AF Chen, Wei-Min
   Qie, Long
   Shen, Yue
   Sun, Yong-Ming
   Yuan, Li-Xia
   Hu, Xian-Luo
   Zhang, Wu-Xing
   Huang, Yun-Hui
TI Superior lithium storage performance in nanoscaled MnO promoted by
   N-doped carbon webs
SO NANO ENERGY
LA English
DT Article
DE Lithium-ion battery; Anode; Manganese monoxide; Polypyrrole template;
   Electrochemical performance
ID LI-ION BATTERIES; ANODE MATERIALS; ENERGY-STORAGE; CAPACITY; GRAPHENE;
   COMPOSITES; ELECTRODES
AB Carbon-encapsulated nano-MnO composite with novel multiple structure loaded on N-doped carbon webs (CMNCWs) has been designed and fabricated by using polypyrrole webs as both template and precursor. As an anode material for lithium-ion batteries, CMNCWs exhibit a superhigh reversible capacity and excellent rate capability, delivering a capacity as high as 1268 mA h g(-1) after 700 cycles at a current density of 1.0 A g(-1). Such superior electrochemical performance can be attributed to the unique multiple structure, which cannot only effectively shorten the transport path of Li+ ions and enhance the conductivity, but also relieve the volume change and prevent agglomeration of Mn grains during the phase transformation in the conversion reaction. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Huang, Yun-Hui] Huazhong Univ Sci & Technol, Key Lab Large Format Battery Mat & Syst, Minist Educ, Wuhan 430074, Hubei, Peoples R China.
   Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, Wuhan 430074, Hubei, Peoples R China.
RP Huang, YH (reprint author), Huazhong Univ Sci & Technol, Key Lab Large Format Battery Mat & Syst, Minist Educ, Wuhan 430074, Hubei, Peoples R China.
EM huangyh@mail.hust.edu.cn
RI Huang, Yunhui/C-3752-2014; Hu, Xianluo/E-6442-2010; Qie,
   Long/F-1488-2011
OI Hu, Xianluo/0000-0002-5769-167X; Qie, Long/0000-0003-1693-5911
FU Natural Science Foundation of China [50825203, 21175050]; 863 program
   from the MOST [2011AA11290, 2011DFB70020]; PCSIRT (Program for
   Changjiang Scholars and Innovative Research Team in University)
   [IRT1014]
FX This work was supported by the Natural Science Foundation of China
   (Grant Nos. 50825203 and 21175050), the 863 program from the MOST (Grant
   Nos. 2011AA11290 and 2011DFB70020), and the PCSIRT (Program for
   Changjiang Scholars and Innovative Research Team in University, No.
   IRT1014). In addition, the authors thank Analytical and Testing Center
   of Huazhong University of Science and Technology for XRD, SEM
   measurement.
CR Liu R, 2010, ACS NANO, V4, P4299, DOI 10.1021/nn1010182
   Sun B, 2011, J POWER SOURCES, V196, P3346, DOI 10.1016/j.jpowsour.2010.11.090
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NR 31
TC 46
Z9 48
U1 21
U2 174
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAY
PY 2013
VL 2
IS 3
BP 412
EP 418
DI 10.1016/j.nanoen.2012.11.010
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 156TA
UT WOS:000319845600015
ER

PT J
AU Shi, WH
   Zhu, JX
   Rui, XH
   Cao, XH
   Chen, C
   Zhang, H
   Hng, HH
   Yan, QY
AF Shi, Wenhui
   Zhu, Jixin
   Rui, Xianhong
   Cao, Xiehong
   Chen, Charlottle
   Zhang, Hua
   Hng, Huey Hoon
   Yan, Qingyu
TI Controlled Synthesis of Carbon-Coated Cobalt Sulfide Nanostructures in
   Oil Phase with Enhanced Li Storage Performances
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE cobalt sulfides; solvothermal; carbon coating; dandelion; nanoparticles;
   LIB
ID LITHIUM-ION BATTERIES; HYDROTHERMAL SYNTHESIS; SULFUR BATTERIES;
   GRAPHENE OXIDE; HOLLOW SPHERES; CHALLENGES; CATHODE; CELLS;
   NANOMATERIALS; CAPABILITY
AB A novel solvothermal process was developed for the synthesis of carbon-coated Co9S8 nanodandelions using 1-dodecanethiol as the sulfur source and the soft template. Replacing 1-dodecanethiol with sulfur powder as the sulfur source leads to the formation of 20 nm Co9S8 nanoparticles without carbon coating. When tested as LIB anode, the C@ Co9S8 dandelion delivers a specific capacity of 520 mA h g(-1) at a current density of 1 A g(-1) (1.8 C) during the 50th cycle, which is much higher than that of Co9S8 nanoparticles (e.g. 338 mA h g(-1)). Furthermore, the C@Co9S8 dandelion also exhibits excellent high C-rate performance, e.g., depicts a 10th-cycle capacity of 373 mA h g(-1) at a current density of 6 A g(-1) (10.9 C), which is better than that of many reported anode materials. Such synthesis approach is attractive for the preparation of sulfide anode materials with high Li storage properties.
C1 [Shi, Wenhui; Zhu, Jixin; Rui, Xianhong; Cao, Xiehong; Chen, Charlottle; Zhang, Hua; Hng, Huey Hoon; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Yan, Qingyu] TUM CREATE Ctr Electromobil, Singapore 637459, Singapore.
RP Yan, QY (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
EM alexyan@ntu.edu.sg
RI zhu, Jixin/F-8763-2011; Yan , Qingyu/A-2237-2011; Hng, Huey
   Hoon/A-2246-2011; Rui, Xianhong/D-2604-2015; Cao, Xiehong/I-9665-2014;
   Zhang, Hua/A-1302-2009
OI Hng, Huey Hoon/0000-0002-8950-025X; Rui, Xianhong/0000-0003-1125-0905;
   Cao, Xiehong/0000-0002-3004-7518; 
FU MOE (Singapore) [RG 31/08]; Singapore Ministry of Education
   [MOE2010-T2-1-017]; A*STAR SERC [1021700144]; Singapore MPA
   [23/04.15.03]; Singapore RDP [009/10/102, 020/10/113]; 
   [NRF2009EWT-CERP001-026]
FX The authors gratefully acknowledge AcRF Tier 1 RG 31/08 of MOE
   (Singapore), NRF2009EWT-CERP001-026 (Singapore), Singapore Ministry of
   Education (MOE2010-T2-1-017), A*STAR SERC Grant 1021700144, and
   Singapore MPA 23/04.15.03 RDP 009/10/102 and MPA 23/04.15.03 RDP
   020/10/113 Grant.
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NR 51
TC 46
Z9 47
U1 27
U2 193
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD JUN
PY 2012
VL 4
IS 6
BP 2999
EP 3006
DI 10.1021/am3003654
PG 8
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 964SL
UT WOS:000305716900027
PM 22612396
ER

PT J
AU Komaba, S
   Ozeki, T
   Okushi, K
AF Komaba, S.
   Ozeki, T.
   Okushi, K.
TI Functional interface of polymer modified graphite anode
SO JOURNAL OF POWER SOURCES
LA English
DT Article; Proceedings Paper
CT 14th International Meeting on Lithium Batteries
CY JUN 22-28, 2008
CL Tianjin, PEOPLES R CHINA
SP Tianjin Inst Power Sources, China Ind Assoc Power Sources, Tianjin Local Govt
DE Lithium intercalation; Graphite; Lithium ion battery; Propylene
   carbonate
ID LITHIUM-ION CELLS; ELECTROLYTE-SOLUTIONS; PROPYLENE CARBONATE; NATURAL
   GRAPHITE; LI-ION; BATTERIES; SOLVATION; BEHAVIOR; ALKALI
AB Graphite electrodes were modified by polyacrylic acid (PAA), polymethacrylic acid (PMA), and polyvinyl alcohol (PVA). Their electrochemical properties were examined in 1 mol dm(-3) LiClO(4) ethylene carbonate:dimethyl carbonate (EC:DMC) and propylene carbonate (PC) solutions as an anode of lithium ion batteries. Generally, lithium ions hardly intercalate into graphite in the PC electrolyte due to a decomposition of the PC electrolyte at ca. 0.8V vs. Li/Li(+), and it results in the exfoliation of the graphene layers. However, the modified graphite electrodes with PAA, PMA, and PVA demonstrated the stable charge-discharge performance due to the reversible lithium intercalation not only in the EC:DMC but also in the PC electrolytes since the electrolyte decomposition and co-intercalation of solvent were successfully suppressed by the polymer modification. It is thought that these improvements were attributed to the interfacial function of the polymer layer on the graphite which interacted with the solvated lithium ions at the electrode interface. (C) 2008 Elsevier B.V. All rights reserved.
C1 [Komaba, S.; Ozeki, T.; Okushi, K.] Tokyo Univ Sci, Dept Appl Chem, Shinjuku Ku, Tokyo 1628601, Japan.
RP Komaba, S (reprint author), Tokyo Univ Sci, Dept Appl Chem, Shinjuku Ku, 1-3 Kagurazaka, Tokyo 1628601, Japan.
EM komaba@rs.kagu.tus.ac.jp
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NR 21
TC 46
Z9 46
U1 5
U2 37
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD APR 1
PY 2009
VL 189
IS 1
BP 197
EP 203
DI 10.1016/j.jpowsour.2008.09.092
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 435BG
UT WOS:000265317600032
ER

PT J
AU Xu, K
   Lee, U
   Zhang, SS
   Jow, TR
AF Xu, K
   Lee, U
   Zhang, SS
   Jow, TR
TI Graphite/electrolyte interface formed in LiBOB-based electrolytes - II.
   Potential dependence of surface chemistry on graphitic anodes
SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY
LA English
DT Article
ID PROPYLENE CARBONATE SOLUTIONS; LITHIUM-ION BATTERIES; ELECTROCHEMICAL
   INTERCALATION; ELECTRODES; DECOMPOSITION; BEHAVIOR; SYSTEMS; MODEL;
   CELLS
AB In an attempt to depict a dynamic picture of solid electrolyte interface (SEI) formation on a graphitic anode surface during the initial forming cycle, we employed X-ray photoelectron spectroscopy in combination with a "pre-formation'' technique to establish the dependence of the surface chemistry on the forming potential of the anode. A progressive transition in the 1s electron binding energies of the major elements was observed as the lithiation proceeded. However, the surface chemical species as well as their abundances seemed to stabilize around 0.55 V and remained constant during the subsequent delithiation process, indicating that a stable SEI exists thereafter. Integrating the information revealed by different analyses, we believe that the reductive decomposition of the BOB- anion starts at ca. 1.00 V, while the effective protection of the graphene surface by SEI is available after the anode is lithiated below the potential of 0.55 V vs. Li. (C) 2004 The Electrochemical Society.
C1 USA, Res Lab, Adelphi, MD 20783 USA.
RP Xu, K (reprint author), USA, Res Lab, Adelphi, MD 20783 USA.
EM cxu@arl.army.mil
RI Zhang, Sheng/A-4456-2012; Xu, Kang/C-6054-2013
OI Zhang, Sheng/0000-0002-2624-9248; 
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NR 25
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U1 1
U2 16
PU ELECTROCHEMICAL SOC INC
PI PENNINGTON
PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA
SN 0013-4651
J9 J ELECTROCHEM SOC
JI J. Electrochem. Soc.
PY 2004
VL 151
IS 12
BP A2106
EP A2112
DI 10.1149/1.1812732
PG 7
WC Electrochemistry; Materials Science, Coatings & Films
SC Electrochemistry; Materials Science
GA 870OY
UT WOS:000225068500016
ER

PT J
AU Wang, DN
   Li, XF
   Yang, JL
   Wang, JJ
   Geng, DS
   Li, RY
   Cai, M
   Sham, TK
   Sun, XL
AF Wang, Dongniu
   Li, Xifei
   Yang, Jinli
   Wang, Jiajun
   Geng, Dongsheng
   Li, Ruying
   Cai, Mei
   Sham, Tsun-Kong
   Sun, Xueliang
TI Hierarchical nanostructured core-shell Sn@C nanoparticles embedded in
   graphene nanosheets: spectroscopic view and their application in lithium
   ion batteries
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID X-RAY-ABSORPTION; ANODE MATERIAL; SECONDARY BATTERIES; REVERSIBLE
   CAPACITY; CYCLIC PERFORMANCE; STORAGE PROPERTIES; CARBON NANOTUBE;
   COMPOSITE; STABILITY; ELECTRODES
AB Hierarchical carbon encapsulated tin (Sn@C) embedded graphene nanosheet (GN) composites (Sn@C-GNs) have been successfully fabricated via a simple and scalable one-step chemical vapor deposition (CVD) procedure. The GN supported Sn@C core-shell structures consist of a crystalline tin core, which is thoroughly covered by a carbon shell and more interestingly, extra voids are present between the carbon shell and the tin core. Synchrotron spectroscopy confirms that the metallic tin core is free of oxidation and the existence of charge redistribution transfer from tin to the carbonaceous materials of the shell, facilitating their intimate contact by chemical bonding and resultant lattice variation. The hybrid electrodes of this material exhibit a highly stable and reversible capacity together with an excellent rate capability, which benefits from the improved electrochemical properties of tin provided by the protective carbon matrix, voids and the flexible GN matrices.
C1 [Wang, Dongniu; Li, Xifei; Yang, Jinli; Wang, Jiajun; Geng, Dongsheng; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B7, Canada.
   [Wang, Dongniu; Sham, Tsun-Kong] Univ Western Ontario, Dept Chem, London, ON N6A 5B7, Canada.
   [Cai, Mei] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Sham, TK (reprint author), Univ Western Ontario, Dept Chem, London, ON N6A 5B7, Canada.
EM tsham@uwo.ca; xsun@eng.uwo.ca
RI Sun, Andy (Xueliang)/I-4535-2013; Li, Xifei/A-1966-2012; Geng,
   Dongsheng/G-7124-2011; Sun, Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; 
FU Natural Sciences and Engineering Research Council of Canada (NSERC);
   General Motors of Canada; Canada Research Chair (CRC); Canada Foundation
   for Innovation (CFI); Ontario Innovation Trust (OIT) Program; X-ray
   Science Division (XSD)/Pacific Northwest Consortium (PNC) at Sector 20
   of Advanced Photon Source; University of Western Ontario; CFI; NSERC;
   NRC; CHIR; University of Saskatchewan
FX This research was supported by Natural Sciences and Engineering Research
   Council of Canada (NSERC), General Motors of Canada, Canada Research
   Chair (CRC), Canada Foundation for Innovation (CFI), Ontario Innovation
   Trust (OIT) Program, X-ray Science Division (XSD)/Pacific Northwest
   Consortium (PNC) at Sector 20 of Advanced Photon Source and University
   of Western Ontario. The Canadian Light Source is supported by CFI,
   NSERC, NRC, CHIR, and the University of Saskatchewan.
CR Berger C, 2006, SCIENCE, V312, P1191, DOI 10.1126/science.1125925
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NR 37
TC 45
Z9 46
U1 17
U2 160
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2013
VL 15
IS 10
BP 3535
EP 3542
DI 10.1039/c3cp44172e
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 088PC
UT WOS:000314846600019
PM 23376983
ER

PT J
AU Zhu, J
   Lei, DN
   Zhang, GH
   Li, QH
   Lu, BG
   Wang, TH
AF Zhu, Jian
   Lei, Danni
   Zhang, Guanhua
   Li, Qiuhong
   Lu, Bingan
   Wang, Taihong
TI Carbon and graphene double protection strategy to improve the SnOx
   electrode performance anodes for lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID STORAGE CAPACITY; NANOTUBES; OXIDE; NANOSTRUCTURES; COMPOSITES;
   NANOFIBERS; NANOSHEETS; LAYERS; GROWTH; PAPER
AB SnOx is a promising high-capacity anode material for lithium-ion batteries (LIBs), but it usually exhibits poor cycling stability because of its huge volume variation during the lithium uptake and release process. In this paper, SnOx carbon nanofibers (SnOx@CNFs) are firstly obtained in the form of a nonwoven mat by electrospinning followed by calcination in a 0.02 Mpa environment at 500 degrees C. Then we use a simple mixing method for the synthesis of SnOx@CNF@graphene (SnOx@C@G) nanocomposite. By this technique, the SnOx@CNFs can be homogeneously deposited in graphene nanosheets (GNSs). The highly scattered SnOx@C@G composite exhibits enhanced electrochemical performance as anode material for LIBs. The double protection strategy to improve the electrode performance through producing SnOx@C@G composites is versatile. In addition, the double protection strategy can be extended to the fabrication of various types of composites between metal oxides and graphene nanomaterials, possessing promising applications in catalysis, sensing, supercapacitors and fuel cells.
C1 [Zhu, Jian; Lei, Danni; Zhang, Guanhua; Li, Qiuhong; Lu, Bingan; Wang, Taihong] Hunan Univ, Minist Educ, Key Lab Micronano Optoelect Devices, State Key Lab Chemo Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
RP Lu, BG (reprint author), Hunan Univ, Minist Educ, Key Lab Micronano Optoelect Devices, State Key Lab Chemo Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
EM luba2012@hnu.edu.cn; wangth@hnu.edu.cn
RI Wang, Taihong/K-8968-2012
FU National Natural Science Foundation of China [21003041, 21103046]; Hunan
   Provincial Natural Science Foundation of China [10JJ1011, 11JJ7004]
FX This work was partly supported by the National Natural Science
   Foundation of China (Grant no. 21003041 and 21103046) and the Hunan
   Provincial Natural Science Foundation of China (Grant no. 10JJ1011 and
   11JJ7004).
CR Lim AH, 2012, NANOSCALE, V4, P4694, DOI 10.1039/c2nr31056b
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   Chen JS, 2013, SMALL, V9, P1877, DOI 10.1002/smll.201202601
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NR 49
TC 45
Z9 45
U1 14
U2 104
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 12
BP 5499
EP 5505
DI 10.1039/c3nr00467h
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 155NX
UT WOS:000319756200046
PM 23670638
ER

PT J
AU Wang, G
   Liu, T
   Xie, XL
   Ren, ZY
   Bai, JB
   Wang, H
AF Wang, Gang
   Liu, Ting
   Xie, Xiaoling
   Ren, Zhaoyu
   Bai, Jinbo
   Wang, Hui
TI Structure and electrochemical performance of Fe3O4/graphene
   nanocomposite as anode material for lithium-ion batteries
SO MATERIALS CHEMISTRY AND PHYSICS
LA English
DT Article
DE Composite materials; Chemical synthesis; Electrochemical techniques;
   Electrochemical properties
ID GRAPHENE NANOSHEETS; LI STORAGE; CAPACITY
AB Using hydrothermal method, Fe3O4/graphene nanocomposite is prepared by synthesizing Fe3O4 particles in graphene. The synthesized Fe3O4 is nano-sized sphere particles (100-200 nm) and uniformly distributed on the planes of graphene. Fe3O4/graphene nanocomposite as anode material for lithium ion batteries shows high reversible specific capacity of 771 mAh g(-1) at 50th cycle and good rate capability. The excellent electrochemical performance of the nanocomposite can be attributed to the high surface area and good electronic conductivity of graphene. Due to the high surface area, graphene can prevent Fe3O4 nanoparticles from aggregating and provide enough space to buffer the volume change during the Li insertion/extraction processes in Fe3O4 nanoparticles. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Wang, Gang; Liu, Ting; Xie, Xiaoling; Wang, Hui] NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
   [Ren, Zhaoyu] NW Univ Xian, Natl Key Lab Photoelect Technol & Funct Mat, Culture Base, Natl Photoelect Technol & Funct Mat & Applicat In, Xian 710069, Peoples R China.
   [Bai, Jinbo] Ecole Cent Paris, Lab MSS MAT, CNRS UMR 8579, F-92295 Chatenay Malabry, France.
RP Wang, H (reprint author), NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
EM huiwang@nwu.edu.cn
RI Bai, Jinbo/F-8552-2010
FU National Natural Science Foundation of China [21061130551, 20873099,
   10974152]; National Basic Research Program of China (973 Program)
   [2009CB626611]; Ph.D. Programs Foundation of Ministry of Education of
   China [20096101110002]; NWU [09YYB04]
FX The project was supported by the financial supports of the International
   cooperation research program of National Natural Science Foundation of
   China (no. 21061130551), the National Basic Research Program of China
   (973 Program) (no. 2009CB626611), the Ph.D. Programs Foundation of
   Ministry of Education of China (no. 20096101110002), the National
   Natural Science Foundation of China (nos. 20873099 and 10974152), NWU
   Doctorate Dissertation of Excellence Funds (no. 09YYB04).
CR Wang SQ, 2010, J POWER SOURCES, V195, P5379, DOI 10.1016/j.jpowsour.2010.03.035
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   Yoo E, 2008, NANO LETT, V8, P2277, DOI 10.1021/nl800957b
   Yuan L, 2006, J POWER SOURCES, V159, P345, DOI 10.1016/j.jpowsour.2006.04.048
   Pan DY, 2009, CHEM MATER, V21, P3136, DOI 10.1021/cm900395k
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NR 21
TC 45
Z9 46
U1 11
U2 95
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0254-0584
J9 MATER CHEM PHYS
JI Mater. Chem. Phys.
PD AUG 15
PY 2011
VL 128
IS 3
BP 336
EP 340
DI 10.1016/j.matchemphys.2011.03.049
PG 5
WC Materials Science, Multidisciplinary
SC Materials Science
GA 785LP
UT WOS:000292230800005
ER

PT J
AU Xue, XY
   Ma, CH
   Cui, CX
   Xing, LL
AF Xue, Xin-Yu
   Ma, Chun-Hua
   Cui, Chun-Xiao
   Xing, Li-Li
TI High lithium storage performance of alpha-Fe2O3/graphene nanocomposites
   as lithium-ion battery anodes
SO SOLID STATE SCIENCES
LA English
DT Article
DE Nanocomposites; Graphene; Iron oxide; Lithium-ion battery
ID ELECTROCHEMICAL PROPERTIES; SOLVOTHERMAL SYNTHESIS; CYCLIC PERFORMANCE;
   GRAPHENE; CARBON; GROWTH; NANOPARTICLES; NANOTUBES; COMPOSITE;
   MICROSPHERES
AB Uniformly loaded alpha-Fe2O3/graphene nanocomposites are synthesized via hydrothermal routs. Enhanced lithium storage performance of lithium-ion battery anodes is realized from alpha-Fe2O3/graphene nanocomposites. Compared with pure alpha-Fe2O3 nanostructures, alpha-Fe2O3/graphene nanocomposites exhibit higher reversible capacity and better cycling performance. Their reversible capacity is up to 771 mA h g(-1) at C/10 rate, and maintains 73% after 30 cycles. Such behaviors can be attributed to high electron and Li-ion conductivity, large surface area, good mechanical flexibility of graphene nanosheets and the synergetic effect of graphene and alpha-Fe2O3 nanostructures. Our results indicate that alpha-Fe2O3/graphene nanocomposites are good candidates for high performance lithium-ion battery anodes. (C) 2011 Elsevier Masson SAS. All rights reserved.
C1 [Xue, Xin-Yu; Ma, Chun-Hua; Cui, Chun-Xiao; Xing, Li-Li] Northeastern Univ, Coll Sci, Shenyang 110004, Peoples R China.
RP Xue, XY (reprint author), Northeastern Univ, Coll Sci, Shenyang 110004, Peoples R China.
EM xuexinyu@mail.neu.edu.cn
RI Xue, Xinyu/N-7444-2014
FU Fundamental Research Funds for the Central Universities [N090405017,
   N100405109]; Liaoning Natural Science Foundation [20091027]; Specialized
   Research Fund for the Doctoral Program of Higher Education of China
   [20090042120025]
FX This work was partly supported from the Fundamental Research Funds for
   the Central Universities (N090405017, N100405109), Liaoning Natural
   Science Foundation (20091027), Specialized Research Fund for the
   Doctoral Program of Higher Education of China (20090042120025).
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NR 50
TC 45
Z9 48
U1 14
U2 108
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1293-2558
J9 SOLID STATE SCI
JI Solid State Sci.
PD AUG
PY 2011
VL 13
IS 8
BP 1526
EP 1530
DI 10.1016/j.solidstatesciences.2011.05.015
PG 5
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical; Physics, Condensed
   Matter
SC Chemistry; Physics
GA 815IT
UT WOS:000294520000013
ER

PT J
AU Yu, XY
   Hu, H
   Wang, YW
   Chen, HY
   Lou, XW
AF Yu, Xin-Yao
   Hu, Han
   Wang, Yawen
   Chen, Hongyu
   Lou, Xiong Wen (David)
TI Ultrathin MoS2 Nanosheets Supported on N-doped Carbon Nanoboxes with
   Enhanced Lithium Storage and Electrocatalytic Properties
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE lithium-ion batteries; molybdenum disulfide; MoS2; water splitting
ID EXCELLENT ELECTROCHEMICAL PERFORMANCE; TRANSITION-METAL DICHALCOGENIDES;
   HYDROGEN EVOLUTION REACTION; ION BATTERIES; HOLLOW MICROSPHERES;
   PSEUDOCAPACITIVE PROPERTIES; GENERAL FORMATION; GRAPHENE;
   NANOSTRUCTURES; FABRICATION
AB Molybdenum disulfide (MoS2) has received considerable interest for electrochemical energy storage and conversion. In this work, we have designed and synthesized a unique hybrid hollow structure by growing ultrathin MoS2 nanosheets on N-doped carbon shells (denoted as C@MoS2 nanoboxes). The N-doped carbon shells can greatly improve the conductivity of the hybrid structure and effectively prevent the aggregation of MoS2 nanosheets. The ultrathin MoS2 nanosheets could provide more active sites for electrochemical reactions. When evaluated as an anode material for lithium-ion batteries, these C@MoS2 nanoboxes show high specific capacity of around 1000 mAhg(-1), excellent cycling stability up to 200 cycles, and superior rate performance. Moreover, they also show enhanced electrocatalytic activity for the electrochemical hydrogen evolution.
C1 [Yu, Xin-Yao; Hu, Han; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
   [Yu, Xin-Yao] Chinese Acad Sci, Hefei Inst Phys Sci, Nanomat & Environm Detect Lab, Hefei 230031, Peoples R China.
   [Wang, Yawen; Chen, Hongyu] Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 637371, Singapore.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM xwlou@ntu.edu.sg
RI Yu, Xin-Yao/B-2318-2015; Hu, Han/C-5456-2016; Chen, Hongyu/C-4594-2008
OI Yu, Xin-Yao/0000-0003-3576-5815; Hu, Han/0000-0002-3755-7342; 
CR Wang J, 2014, ADV MATER, V26, P7162, DOI 10.1002/adma.201402728
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NR 40
TC 44
Z9 44
U1 269
U2 432
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD JUN 15
PY 2015
VL 54
IS 25
BP 7395
EP 7398
DI 10.1002/anie.201502117
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA CK7DE
UT WOS:000356390300033
PM 25939884
ER

PT J
AU Hu, CG
   Zhai, XQ
   Liu, LL
   Zhao, Y
   Jiang, L
   Qu, LT
AF Hu, Chuangang
   Zhai, Xiangquan
   Liu, Lili
   Zhao, Yang
   Jiang, Lan
   Qu, Liangti
TI Spontaneous Reduction and Assembly of Graphene oxide into
   Three-Dimensional Graphene Network on Arbitrary Conductive Substrates
SO SCIENTIFIC REPORTS
LA English
DT Article
ID LITHIUM-ION BATTERIES; EXFOLIATED GRAPHITE OXIDE; HIGH-RATE CAPABILITY;
   ANODE MATERIALS; ENERGY-STORAGE; METAL NANOPARTICLES; CARBON NANOTUBES;
   PERFORMANCE; SHEETS; FABRICATION
AB Chemical reduction of graphene oxide (GO) is the main route to produce the mass graphene-based materials with tailored surface chemistry and functions. However, the toxic reducing circumstances, multiple steps, and even incomplete removal of the oxygen-containing groups were involved, and the produced graphenes existed usually as the assembly-absent precipitates. Herein, a substrate-assisted reduction and assembly of GO (SARA-GO) method was developed for spontaneous formation of 3D graphene network on arbitrary conductive substrates including active and inert metals, semiconducting Si, nonmetallic carbon, and even indium-tin oxide glass without any additional reducing agents. The SARA-GO process offers a facile, efficient approach for constructing unique graphene assemblies such as microtubes, multi-channel networks, micropatterns, and allows the fabrication of high-performance binder-free rechargeable lithium-ion batteries. The versatile SARD-GO method significantly improves the processablity of graphenes, which could thus benefit many important applications in sensors and energy-related devices.
C1 [Hu, Chuangang; Zhai, Xiangquan; Liu, Lili; Zhao, Yang; Qu, Liangti] Beijing Inst Technol, Sch Chem, Minist Educ, Key Lab Cluster Sci, Beijing 100081, Peoples R China.
   [Jiang, Lan] Beijing Inst Technol, Sch Mech Engn, Laser Micro Nano Fabricat Lab, Beijing 100081, Peoples R China.
RP Qu, LT (reprint author), Beijing Inst Technol, Sch Chem, Minist Educ, Key Lab Cluster Sci, Beijing 100081, Peoples R China.
EM lqu@bit.edu.cn
RI Liu, Lili/O-4292-2014
FU National Basic Research Program of China [2011CB013000]; NSFC [21004006,
   21174019, 51161120361]; Fok Ying Tong Education Foundation [131043]; 111
   Project [B07012]; research foundation for the doctoral program of higher
   education of China [20101101120036]
FX This work is sponsored by National Basic Research Program of China
   (2011CB013000), NSFC (No. 21004006, 21174019, 51161120361), Fok Ying
   Tong Education Foundation (No. 131043), the 111 Project B07012, and
   research foundation for the doctoral program of higher education of
   China (20101101120036).
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NR 55
TC 44
Z9 45
U1 47
U2 341
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2045-2322
J9 SCI REP-UK
JI Sci Rep
PD JUN 25
PY 2013
VL 3
AR 2065
DI 10.1038/srep02065
PG 10
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA 170JW
UT WOS:000320847200001
PM 23799368
ER

PT J
AU Qu, J
   Yin, YX
   Wang, YQ
   Yan, Y
   Guo, YG
   Song, WG
AF Qu, Jin
   Yin, Ya-Xia
   Wang, Yong-Qing
   Yan, Yang
   Guo, Yu-Guo
   Song, Wei-Guo
TI Layer Structured alpha-Fe2O3 Nanodisk/Reduced Graphene Oxide Composites
   as High-Performance Anode Materials for Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE alpha-Fe2O3; layered nanodisk; reduced graphene oxide; oxygen bridges;
   Li-ion battery
ID STORAGE CAPABILITY; HOLLOW SPHERES; METAL-OXIDES; NANOSHEETS;
   NANOSTRUCTURES; OXIDATION; CATALYSTS; NETWORKS; SOOT; NANOPARTICLES
AB A composited anode material with combined layered alpha-Fe2O3 nanodisks and reduced graphene oxide was produced by an in situ hydrothermal method for lithium-ion batteries. As thin as about 5-nm-thickness alpha-Fe2O3 nanosheets, open channels, and face-to-face tight contact with reduced graphene oxide via oxygen bridges made the composite have a good cyclability and rate performance, especially at high charge/discharge rates.
C1 [Qu, Jin; Yin, Ya-Xia; Wang, Yong-Qing; Yan, Yang; Guo, Yu-Guo; Song, Wei-Guo] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China.
   [Qu, Jin; Yin, Ya-Xia; Wang, Yong-Qing; Yan, Yang; Guo, Yu-Guo; Song, Wei-Guo] Chinese Acad Sci, Inst Chem, Key Lab Mol Nanostruct & Nanotechnol, Beijing 100190, Peoples R China.
   [Qu, Jin; Wang, Yong-Qing; Yan, Yang] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
RP Guo, YG (reprint author), Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China.
EM ygguo@iccas.ac.cn; wsong@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009; Song, Weiguo/D-6041-2016
OI Guo, Yu-Guo/0000-0003-0322-8476; Song, Weiguo/0000-0001-5390-6787
FU National Basic Research Program of China [2009CB930400, 2012CB932900];
   National Natural Science Foundation of China [NSFC 21121063, 51225204];
   Chinese Academy of Sciences [KJCX2-YW-N41]
FX We gratefully thank the National Basic Research Program of China (Grants
   2009CB930400 and 2012CB932900), National Natural Science Foundation of
   China (Grants NSFC 21121063 and 51225204), and Chinese Academy of
   Sciences (Grant KJCX2-YW-N41) for financial support.
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NR 35
TC 44
Z9 44
U1 19
U2 202
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY 8
PY 2013
VL 5
IS 9
BP 3932
EP 3936
DI 10.1021/am400670d
PG 5
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 143AQ
UT WOS:000318839100061
PM 23594186
ER

PT J
AU Fang, X
   Ge, MY
   Rong, JP
   Zhou, CW
AF Fang, Xin
   Ge, Mingyuan
   Rong, Jiepeng
   Zhou, Chongwu
TI Graphene-oxide-coated LiNi0.5Mn1.5O4 as high voltage cathode for lithium
   ion batteries with high energy density and long cycle life
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ELECTROCHEMICAL PROPERTIES; SPINEL LINI0.5MN1.5O4; HIGH-CAPACITY; GEL
   METHOD; PERFORMANCE; CELLS; ANODE; IMPROVEMENT; ELECTRODES; STABILITY
AB Lithium ion batteries are receiving enormous attention as power sources and energy storage devices in the renewable energy field. With the ever increasing demand for higher energy and power density, high voltage cathodes have emerged as an important option for new generation batteries. Here, we report graphene-oxide-coated LiNi0.5Mn1.5O4 as a high voltage cathode and demonstrate that the batteries showed superior cycling performance for up to 1000 cycles. Mildly oxidized graphene oxide coating was found to improve the battery performance by enhancing the conductivity and protecting the cathode surface from undesired reactions with the electrolyte. As a result, the graphene-oxide-coated high voltage cathode LiNi0.5Mn1.5O4 showed 61% capacity retention after 1000 cycles in the cycling test, which converts to only 0.039% capacity decay per cycle. At large current rates of 5 C, 7 C and 10 C, the batteries were able to deliver 77%, 66% and 56% of the 1 C capacity, respectively (1 C 140 mA g(-1)). In contrast, the LiNi0.5Mn1.5O4 cathode without graphene oxide coating showed 88.7% capacity retention after only 100 cycles. The promising results demonstrated the potential of developing high energy density batteries with the high voltage cathode LiNi0.5Mn1.5O4 and improving the battery performance by surface modification with mildly oxidized graphene oxide.
C1 [Fang, Xin; Ge, Mingyuan; Rong, Jiepeng] Univ So Calif, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA.
   [Zhou, Chongwu] Univ So Calif, Ming Hsieh Dept Elect Engn, Los Angeles, CA 90089 USA.
RP Fang, X (reprint author), Univ So Calif, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA.
EM chongwuz@usc.edu
RI Zhou, Chongwu/F-7483-2010; Rong, Jiepeng/B-3624-2015; Fang,
   Xin/P-8002-2015
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NR 58
TC 44
Z9 44
U1 22
U2 155
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 12
BP 4083
EP 4088
DI 10.1039/c3ta01534c
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 095TB
UT WOS:000315356500034
ER

PT J
AU Chen, SQ
   Wang, Y
   Ahn, H
   Wang, GX
AF Chen, Shuangqiang
   Wang, Yong
   Ahn, Hyojun
   Wang, Guoxiu
TI Microwave hydrothermal synthesis of high performance tin-graphene
   nanocomposites for lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene nanosheets; Tin nanoparticles; Microwave hydrothermal
   synthesis; Hydrogen reduction; Lithium ion batteries
ID SN-C COMPOSITE; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE;
   HIGH-CAPACITY; SNO2/GRAPHENE COMPOSITE; STORAGE; OXIDE; MICROSPHERES;
   ELECTRODES; STABILITY
AB Tin-graphene nanocomposites are prepared by a combination of microwave hydrothermal synthesis and a one-step hydrogen gas reduction. Altering the weight ratio between tin and graphene nanosheets has critical influences on their morphologies and electrochemical performances. Field emission scanning electron microscope (FESEM) and transmission electron microscope (TEM) analysis confirm the homogeneous distribution of tin nanoparticles on the surface of graphene nanosheets. When applied as an anode material in lithium ion batteries, tin-graphene nanocomposite exhibits a high lithium storage capacity of 1407 mAh g(-1). The as-prepared tin-graphene nanocomposite also demonstrates an excellent high rate capacity and a stable cycle performance. The superior electrochemical performance could be attributed to the synergistic effect of the three-dimensional nanoarchitecture, in which tin nanoparticles are sandwiched between highly conductive and flexible graphene nanosheets. (c) 2012 Elsevier B.V. All rights reserved.
C1 [Chen, Shuangqiang; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
   [Chen, Shuangqiang; Wang, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
   [Ahn, Hyojun] Gyeongsang Natl Univ, Sch Mat Sci & Engn, Jinju 660701, Gyeongnam, South Korea.
RP Wang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yongwang@shu.edu.cn; Guoxiu.wang@uts.edu.au
RI WANG, Yong/B-1125-2012; Chen, Shuangqiang/F-5289-2013
FU Australian Research Council (ARC) through the ARC Discovery project
   [DP1093855]; National Natural Science Foundation of China [50971085,
   50701029]; Professor of Special Appointment (Eastern Scholar); Chinese
   Scholarship Council; National Research Foundation of Korea through the
   WCU (World Class University) Program [R32-2008-000-20093-0]
FX The authors gratefully acknowledge the financial support from Australian
   Research Council (ARC) through the ARC Discovery project (DP1093855),
   the National Natural Science Foundation of China (50971085, 50701029),
   the Professor of Special Appointment (Eastern Scholar), the Chinese
   Scholarship Council, and the National Research Foundation of Korea
   through the WCU (World Class University) Program (R32-2008-000-20093-0).
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NR 49
TC 44
Z9 46
U1 18
U2 168
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD OCT 15
PY 2012
VL 216
BP 22
EP 27
DI 10.1016/j.jpowsour.2012.05.051
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 999SO
UT WOS:000308335500005
ER

PT J
AU Tang, QW
   Shan, ZQ
   Wang, L
   Qin, X
AF Tang, Qiwei
   Shan, Zhongqiang
   Wang, Li
   Qin, Xue
TI MoO2-graphene nanocomposite as anode material for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE MoO2 nanoparticles; Graphene; Anode material; Nanocomposite; Lithium ion
   batteries
ID HIGH-CAPACITY; NEGATIVE-ELECTRODE; GRAPHENE OXIDE; STORAGE; REDUCTION;
   PERFORMANCE; NANOSHEET; PHASE
AB MoO2-graphene composite was synthesized via a two-step of hydrothermal-calcination method. The morphology and structure of the products were characterized by scanning electron microscopy (SEM), high-resolution transmission electron microscopy (HR-TEM), X-ray power diffraction (XRD), and Raman spectroscopy. The content of the graphene in MoO2-graphene composite was examined by thermogravimetric (TG)-differential scanning calorimetry (DSC) analysis. The electrochemical performances of the products were examined by Galvanostatical charge-discharge method, cyclic voltammetry, and electrochemical impedance spectroscopy (EIS). When used as anode material for lithium ion batteries, the MoO2-graphene composite shows an enhanced cyclic performance and lithium storage property. The first discharge capacity of the composite can reach 674.4 mAh g(-1) with a reversible capacity of 429.9 mAh g(-1). Significantly, the composite can also deliver a reversible capacity of as high as 1009.9 mAh g(-1) after 60 charge/discharge cycles. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Wang, Li; Qin, Xue] Tianjin Univ, Sch Sci, Tianjin 300072, Peoples R China.
   [Tang, Qiwei; Shan, Zhongqiang] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
RP Qin, X (reprint author), Tianjin Univ, Sch Sci, 92 Weijin Rd, Tianjin 300072, Peoples R China.
EM xueqin73@yahoo.com.cn
FU National Natural Science Foundation of China [20603024]
FX We are grateful for the financial support of this research work by the
   National Natural Science Foundation of China (20603024).
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NR 40
TC 44
Z9 48
U1 19
U2 136
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD SEP 30
PY 2012
VL 79
BP 148
EP 153
DI 10.1016/j.electacta.2012.06.093
PG 6
WC Electrochemistry
SC Electrochemistry
GA 994HA
UT WOS:000307920300019
ER

PT J
AU Su, FY
   He, YB
   Li, BH
   Chen, XC
   You, CH
   Wei, W
   Lv, W
   Yang, QH
   Kang, FY
AF Su, Fang-Yuan
   He, Yan-Bing
   Li, Baohua
   Chen, Xue-Cheng
   You, Cong-Hui
   Wei, Wei
   Lv, Wei
   Yang, Quan-Hong
   Kang, Feiyu
TI Could graphene construct an effective conducting network in a high-power
   lithium ion battery?
SO NANO ENERGY
LA English
DT Article
DE Graphene; High-power lithium-ion battery; Ion transport; Conducting
   network; Conductive additive
ID CARBON-BLACK DISTRIBUTION; ELECTROCHEMICAL PROPERTIES; LIFEPO4-C
   COMPOSITE; CATHODE MATERIAL; COATED LIFEPO4; ANODE MATERIAL;
   PERFORMANCE; ELECTRODES; CAPACITY; HYBRID
AB This study is trying to demonstrate whether graphene is able to construct an effective conducting network for both electron and ion transports in cathode system of a high-power lithium ion battery (LIB), not based on a coin cell, but by employing a commercial soft-packaged 10 Ah battery pack as a model system. Compared with the cells using commercial conductive additive (7 wt% carbon black and 3 wt% conductive graphite), a 10 Ah cell using only 1 wt% graphene and 1 wt% carbon black shows lower internal resistance and higher energy density due to the excellent conductivity of graphene. However, owing to the fact that the planar structure of the graphene sheets blocks fast Li+ ion transport, the steric effect resulted heavy polarization occurs at a relatively high charge/discharge rate (>3 C). That is, although flexible and planar graphene helps construct an effective electron transfer network, it retards Li+ ion transport. Thus, for an energy-storing LIB with a low working charge/discharge rate, graphene additive shows apparent superiority over commercial ones even with much less addition fraction and may find its real commercial applications; while, for a high-power LIB which works at higher charge/discharge rate, fast ion transport path is required to be effectively constructed before a real application. Simulation results indicate that further work should be focused on the adjustment of electrode pore structure and modification of graphene steric structure accordingly to construct an unimpeded ion conducting network and provide high speed path for Li+ ion transport. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Su, Fang-Yuan; Chen, Xue-Cheng; You, Cong-Hui; Wei, Wei; Lv, Wei; Yang, Quan-Hong] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
   [He, Yan-Bing; Li, Baohua; Yang, Quan-Hong; Kang, Feiyu] Key Lab Thermal Management Engn & Mat, Shenzhen, Peoples R China.
   [He, Yan-Bing; Li, Baohua; Yang, Quan-Hong; Kang, Feiyu] Tsinghua Univ, Grad Sch Shenzhen, Adv Mat Inst, Shenzhen 518055, Peoples R China.
RP Yang, QH (reprint author), Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
EM qhyangcn@tju.edu.cn; fykang@sz.tsinghua.edu.cn
RI Li, Baohua/A-9347-2012; Li, Baohua/F-6991-2011; Lv, Wei/M-1964-2013
OI Li, Baohua/0000-0002-8469-0162; Lv, Wei/0000-0003-0874-3477
FU National Natural Science Foundation of China [50972101, 51072131];
   Guangdong-Hong Kong Public Bidding Program Special program for Dongguan
   [2009205119]; Program of Guangdong-Ministry of Education cooperation
   [2009B090300011, 2011B090400342]; Program of Introducing Talents of
   Discipline to Universities, China [B06006]; Guangdong Province
   Innovation R&D Team Plan for Energy and Environmental Materials
FX We appreciate the support from National Natural Science Foundation of
   China (Nos. 50972101 and 51072131), Guangdong Province Innovation R&D
   Team Plan for Energy and Environmental Materials, Guangdong-Hong Kong
   Public Bidding Program Special program for Dongguan (2009205119),
   Program of Guangdong-Ministry of Education cooperation (2009B090300011
   and 2011B090400342) and Program of Introducing Talents of Discipline to
   Universities (No. B06006), China.
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NR 37
TC 44
Z9 48
U1 19
U2 151
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAY
PY 2012
VL 1
IS 3
BP 429
EP 439
DI 10.1016/j.nanoen.2012.02.004
PG 11
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 132EH
UT WOS:000318050200014
ER

PT J
AU Cheng, JS
   Du, J
AF Cheng, Jinsheng
   Du, Jin
TI Facile synthesis of germanium-graphene nanocomposites and their
   application as anode materials for lithium ion batteries
SO CRYSTENGCOMM
LA English
DT Article
ID SUGAR-CANE BAGASSE; HIGH-CAPACITY; CARBON; NANOWIRES; COMPOSITE;
   STORAGE; GROWTH
AB A simple and low-cost method to synthesize Ge nanoparticles/graphene (Ge NPs/GR) nanocomposites under mild conditions was developed. The reduction of sugarcane bagasse (SB) derived graphene oxide nanosheets was accompanied by generation of Ge NPs in one step. The resulting nanocomposites exhibit high specific capacity and superior capacity retention of 90% after 15 cycles.
C1 [Cheng, Jinsheng; Du, Jin] Guilin Med Univ, Sch Pharm, Guilin 541004, Peoples R China.
   [Cheng, Jinsheng] Tsinghua Univ, Dept Chem, Key Lab Bioorgan Phosphorus Chem & Chem Biol, Beijing 100084, Peoples R China.
RP Cheng, JS (reprint author), Guilin Med Univ, Sch Pharm, Guilin 541004, Peoples R China.
EM chengjs@mail.ustc.edu.cn
FU Guangxi Zhuang Autonomous Region Science Foundation of China [200908193]
FX This work was financially supported by the Guangxi Zhuang Autonomous
   Region Science Foundation of China (no. 200908193).
CR Wen ZH, 2007, ADV FUNCT MATER, V17, P2772, DOI 10.1002/adfm.200600739
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NR 29
TC 44
Z9 46
U1 4
U2 72
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1466-8033
J9 CRYSTENGCOMM
JI Crystengcomm
PY 2012
VL 14
IS 2
BP 397
EP 400
DI 10.1039/c1ce06251d
PG 4
WC Chemistry, Multidisciplinary; Crystallography
SC Chemistry; Crystallography
GA 872VZ
UT WOS:000298839400013
ER

PT J
AU Li, X
   Lai, C
   Xiao, CW
   Gao, XP
AF Li, X.
   Lai, C.
   Xiao, C. W.
   Gao, X. P.
TI Enhanced high rate capability of dual-phase Li4Ti5O12-TiO2 induced by
   pseudocapacitive effect
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Lithium-ion battery; Titanate; Titania; Dual-phase; Pseudocapacitive
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; TITANATE; STORAGE; CARBON; TIO2;
   PERFORMANCE; NANOTUBES; ELECTRODE; GRAPHENE
AB The dual-phase Li4Ti5O12-TiO2 nanocomposite is successfully synthesized by a hydrothermal route with adding thiourea. The electrochemical performance of the dual-phase nanocomposite as anode for lithium-ion batteries is investigated by the galvanostatic method, cyclic voltammetry and electrochemical impedance spectra. It is demonstrated that the dual-phase Li4Ti5O12-TiO2 nanocomposite presents the improved electrochemical performance over individual single phase Li4Ti5O12 and anatase TiO2 samples. After 300 cycles at 1 C, the dual-phase Li4Ti5O12-TiO2 nanocomposite can still maintain the large discharge capacity of 116 mAh g(-1). It indicates that the as-prepared nanocomposite can endure great changes of various discharge current densities to retain a good stability. The large discharge capacity of 132 mAh g(-1) is also obtained at the large current density of 1600 mA g(-1) upon cycling. In particular, as verified by the cyclic voltammetry, the pseudocapacitive effect is induced due to the presence of abundant phase interfaces in the dual-phase Li4Ti5O12-TiO2 nanocomposite, which is beneficial to the enhanced high rate capability and good cycle stability. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Li, X.; Lai, C.; Xiao, C. W.; Gao, X. P.] Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Tianjin 300071, Peoples R China.
RP Gao, XP (reprint author), Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Tianjin 300071, Peoples R China.
EM xpgao@nankai.edu.cn
RI Lai, Chao/A-8303-2014
FU 973 Program [2009CB220100]; MOE Innovation Team [IRT0927]; Fundamental
   Research Funds for the Central Universities of China
FX Financial Supports from the 973 Program (2009CB220100), MOE Innovation
   Team (IRT0927), and Fundamental Research Funds for the Central
   Universities of China is greatly appreciated.
CR Lai C, 2010, ELECTROCHIM ACTA, V55, P4567, DOI 10.1016/j.electacta.2010.03.010
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NR 33
TC 44
Z9 44
U1 6
U2 73
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD OCT 30
PY 2011
VL 56
IS 25
BP 9152
EP 9158
DI 10.1016/j.electacta.2011.07.101
PG 7
WC Electrochemistry
SC Electrochemistry
GA 834XE
UT WOS:000295997000019
ER

PT J
AU Xia, H
   Hong, CY
   Li, B
   Zhao, B
   Lin, ZX
   Zheng, MB
   Savilov, SV
   Aldoshin, SM
AF Xia, Hui
   Hong, Caiyun
   Li, Bo
   Zhao, Bin
   Lin, Zixia
   Zheng, Mingbo
   Savilov, Serguei V.
   Aldoshin, Serguei M.
TI Facile Synthesis of Hematite Quantum-Dot/Functionalized Graphene-Sheet
   Composites as Advanced Anode Materials for Asymmetric Supercapacitors
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE anodes; asymmetric supercapacitors; functionalized graphene nanosheets;
   hematite; quantum dots
ID ELECTROCHEMICAL ENERGY-STORAGE; LITHIUM-ION BATTERIES; HIGH-PERFORMANCE;
   AQUEOUS-ELECTROLYTE; ACTIVATED CARBON; HIGH-POWER; OXIDE; CAPACITORS;
   DENSITY; FABRICATION
AB For building high-energy density asymmetric supercapacitors, developing anode materials with large specific capacitance remains a great challenge. Although Fe2O3 has been considered as a promising anode material for asymmetric supercapacitors, the specific capacitance of the Fe2O3-based anodes is still low and cannot match that of cathodes in the full cells. In this work, a composite material with well dispersed Fe2O3 quantum dots (QDs, approximate to 2 nm) decorated on functionalized graphene-sheets (FGS) is prepared by a facile and scalable method. The Fe2O3 QDs/FGS composites exhibit a large specific capacitance up to 347 F g(-1) in 1 m Na2SO4 between -1 and 0 V versus Ag/AgCl. An asymmetric supercapacitor operating at 2 V is fabricated using Fe2O3/FGS as anode and MnO2/FGS as cathode in 1 m Na2SO4 aqueous electrolyte. The Fe2O3/FGS//MnO2/FGS asymmetric supercapacitor shows a high energy density of 50.7 Wh kg(-1) at a power density of 100 W kg(-1) as well as excellent cycling stability and power capability. The facile synthesis method and superior supercapacitive performance of the Fe2O3 QDs/FGS composites make them promising as anode materials for high-performance asymmetric supercapacitors.
C1 [Xia, Hui; Hong, Caiyun; Li, Bo] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China.
   [Xia, Hui; Hong, Caiyun; Li, Bo] Nanjing Univ Sci & Technol, Herbert Gleiter Inst Nanosci, Nanjing 210094, Jiangsu, Peoples R China.
   [Zhao, Bin; Lin, Zixia; Zheng, Mingbo] Nanjing Univ, Sch Elect Sci & Engn, Nanjing Natl Lab Microstruct, Nanjing 210093, Jiangsu, Peoples R China.
   [Savilov, Serguei V.] Moscow MV Lomonosov State Univ, Dept Chem, Moscow 119991, Russia.
   [Aldoshin, Serguei M.] Moscow MV Lomonosov State Univ, Dept Phys Chem Engn, Moscow 119991, Russia.
RP Xia, H (reprint author), Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Xiaolingwei 200, Nanjing 210094, Jiangsu, Peoples R China.
EM xiahui@njust.edu.cn
RI Mohd Jasni, Mohamad Redwani/E-7555-2015
OI Mohd Jasni, Mohamad Redwani/0000-0003-4036-4856
FU National Natural Science Foundation of China [51102134, 51202106];
   Natural Science Foundation of Jiangsu Province [BK20131349]; QingLan
   Project of Jiangsu Province; China Postdoctoral Science Foundation
   [2013M530258]; Jiangsu Planned Projects for Postdoctoral Research Funds
   [1202001B]; Russian Scientific Fund [14-43-00072]
FX This work was supported by the National Natural Science Foundation of
   China (No. 51102134, 51202106), the Natural Science Foundation of
   Jiangsu Province (No. BK20131349), the QingLan Project of Jiangsu
   Province, the China Postdoctoral Science Foundation (No. 2013M530258),
   the Jiangsu Planned Projects for Postdoctoral Research Funds (No.
   1202001B), and the Russian Scientific Fund (project No. 14-43-00072).
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NR 46
TC 43
Z9 43
U1 181
U2 424
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD JAN 28
PY 2015
VL 25
IS 4
BP 627
EP 635
DI 10.1002/adfm.201403554
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA CA4EH
UT WOS:000348856500014
ER

PT J
AU Cai, DD
   Li, DD
   Wang, SQ
   Zhu, XF
   Yang, WS
   Zhang, SQ
   Wang, HH
AF Cai, Dandan
   Li, Dongdong
   Wang, Suqing
   Zhu, Xuefeng
   Yang, Weishen
   Zhang, Shanqing
   Wang, Haihui
TI High rate capability of TiO2/nitrogen-doped graphene nanocomposite as an
   anode material for lithium-ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE TiO2; Nitrogen-doped graphene; Anode material; Lithium-ion batteries
ID NITROGEN-DOPED GRAPHENE; ELECTROCHEMICAL PERFORMANCE; PHOTOCATALYTIC
   ACTIVITY; CYCLING PERFORMANCE; TIO2; NANOSHEETS; CAPACITY;
   NANOSTRUCTURES; SHEETS; NANOCRYSTALS
AB TiO2/nitrogen-doped graphene nanocomposite was synthesized by a facile gas/liquid interface reaction. The structure and morphology of the sample were analyzed by X-ray diffraction analysis, X-ray photoelectron spectroscopy, scanning electron microscopy and transmission electron microscopy. The results indicate that nitrogen atoms were successfully doped into graphene sheets. The TiO2 nanoparticles (8-13 nm in size) were homogenously anchored on the nitrogen-doped graphene sheets through gas/liquid interface reaction. The as-prepared TiO2/nitrogen-doped graphene nanocomposite shows a better electrochemical performance than the TiO2/graphene nanocomposite and the bare TiO2 nanoparticles. TiO2/nitrogen-doped graphene nanocomposite exhibits excellent cycling stability and shows high capacity of 136 mAh g(-1) (at a current density of 1000 mA g(-1)) after 80 cycles. More importantly, a high reversible capacity of 109 mAh g(-1) can still be obtained even at a super high current density of 5000 mA g(-1). The superior electrochemical performance is attributed to the good electronic conductivity introduced by the nitrogen-doped graphene sheets and the positive synergistic effect between nitrogen-doped graphene sheets and TiO2 nanoparticles. (C) 2013 Elsevier B. V. All rights reserved.
C1 [Cai, Dandan; Li, Dongdong; Wang, Suqing; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou, Guangdong, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian, Peoples R China.
   [Zhang, Shanqing] Griffith Univ, Ctr Clean Environm & Energy, Environm Futures Ctr, Griffith, Qld 4222, Australia.
   [Zhang, Shanqing] Griffith Univ, Griffith Sch Environm, Griffith, Qld 4222, Australia.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou, Guangdong, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013; Zhang,
   Shanqing/C-2590-2008; Wang, Suqing/G-4930-2016
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620; 
FU Program for Pearl River Scholar; Educational Commission of Guangdong
   Province for Talent Introduction; Fundamental Research Funds for the
   Central Universities, SCUT [2009220038]
FX This work was supported by Program for Pearl River Scholar, by
   Educational Commission of Guangdong Province for Talent Introduction,
   and by the Fundamental Research Funds for the Central Universities, SCUT
   (2009220038).
CR Bavykin DV, 2006, ADV MATER, V18, P2807, DOI 10.1002/adma.200502696
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NR 41
TC 43
Z9 44
U1 18
U2 367
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD JUN 5
PY 2013
VL 561
BP 54
EP 58
DI 10.1016/j.jallcom.2013.01.068
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 113QV
UT WOS:000316683700010
ER

PT J
AU Jiang, Y
   Chen, DD
   Song, JS
   Jiao, Z
   Ma, QL
   Zhang, HJ
   Cheng, LL
   Zhao, B
   Chu, YL
AF Jiang, Yong
   Chen, Dandan
   Song, Jinsong
   Jiao, Zheng
   Ma, Qiliang
   Zhang, Haijiao
   Cheng, Lingli
   Zhao, Bing
   Chu, Yuliang
TI A facile hydrothermal synthesis of graphene porous NiO nanocomposite and
   its application in electrochemical capacitors
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; Nickel oxide; Hydrothermal method; Porous materials;
   Electrochemical capacitor
ID LITHIUM-ION BATTERIES; REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; ANODE
   MATERIAL; COMPOSITE; ELECTRODES; SUPERCAPACITORS; NANOPLATELETS;
   NANOCRYSTALS; NANOTUBES
AB A new porous graphene/NiO has been prepared successfully by hydrothermal method with graphene oxide solution, Ni(NO3)(2)center dot 6H(2)O and urea as raw materials. The as-prepared composite is characterized by X-ray diffraction, Raman, FT-IR, SEM, TEM and nitrogen adsorption/desorption. It is shown that graphene sheets are well decorated by the NiO nanoparticles to form a hierarchical nanostructures with rich porosity (ca. 2-5 nm) and large specific surface area (174.1 m(2) g(-1)). Electrochemical characterization demonstrates that the mesoporous graphene/NiO are capable of delivering a specific capacitance of 429.7 F g(-1) at the current density of 200 mAg(-1) and offer good capacitance retention of 86.1% at 1 A g(-1) after 2000 continuous charge-discharge cycles. These rich and evenly distributed porosity could reduce the transportation distance and offer a robust sustentation of OH- ions due to its "ion-buffering reservoirs", ensuring that sufficient Faradaic reactions can take place at the surfaces of electroactive NiO nanoparticles. It suggests that the hierarchical nanostructure is helpful in improving the electrochemical performance of the oxide. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Jiang, Yong; Chen, Dandan; Song, Jinsong; Jiao, Zheng; Ma, Qiliang; Zhang, Haijiao; Cheng, Lingli; Zhao, Bing] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
   [Chu, Yuliang] Shanghai Univ, Instrumental Anal & Res Ctr, Shanghai 200444, Peoples R China.
   [Zhang, Haijiao] Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200433, Peoples R China.
RP Zhao, B (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
EM bzhao@shu.edu.cn
FU Natural Science Foundation of China [11275121, 21241002]; Innovation
   Program of Shanghai Municipal Education Commission [10YZ03, 10YZ05,
   12YZ013]; Natural Science Foundation of Shanghai [10DZ0500100,
   10ZR1411300]; Shanghai Key Laboratory of Green Chemistry and Chemical
   Processes (ECNU); Laboratory of Chemical Engineering (ECUST); Chinese
   Academy of Sciences [12CS02]
FX This work is supported by the Natural Science Foundation of China
   (11275121, 21241002), Innovation Program of Shanghai Municipal Education
   Commission (10YZ03, 10YZ05 and 12YZ013), Natural Science Foundation of
   Shanghai (10DZ0500100 and 10ZR1411300), Shanghai Key Laboratory of Green
   Chemistry and Chemical Processes (ECNU), Laboratory of Chemical
   Engineering (ECUST), and Chinese Academy of Sciences (12CS02).
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NR 36
TC 43
Z9 45
U1 25
U2 242
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 28
PY 2013
VL 91
BP 173
EP 178
DI 10.1016/j.electacta.2012.12.032
PG 6
WC Electrochemistry
SC Electrochemistry
GA 113ZB
UT WOS:000316707400025
ER

PT J
AU Tong, X
   Wang, H
   Wang, G
   Wan, LJ
   Ren, ZY
   Bai, JT
   Bai, JB
AF Tong, Xin
   Wang, Hui
   Wang, Gang
   Wan, Lijuan
   Ren, Zhaoyu
   Bai, Jintao
   Bai, Jinbo
TI Controllable synthesis of graphene sheets with different numbers of
   layers and effect of the number of graphene layers on the specific
   capacity of anode material in lithium-ion batteries
SO JOURNAL OF SOLID STATE CHEMISTRY
LA English
DT Article
DE Graphene sheets; Lithium-ion battery; Number of layers
ID HIGH-QUALITY GRAPHENE; HIGH-RATE CAPABILITY; GRAPHITE OXIDE;
   CHEMICAL-REDUCTION; CARBON NANOTUBES; LI STORAGE; COMPOSITE; NANOSHEETS;
   NANOPLATELETS; TRANSPARENT
AB High quality graphene sheets are synthesized through efficient oxidation process followed by rapid thermal expansion and reduction by H(2). The number of graphene layers is controlled by tuning the oxidation degree of GOs. The higher the oxidation degree of GOs is getting, the fewer the numbers of graphene layers can be obtained. The material is characterized by elemental analysis, thermogravimetric analysis, scanning electron microscopy, atomic force microscopy, transmission electron microscopy and Fourier transform infrared spectroscopies. The obtained graphene sheets with single, triple and quintuplicate layers as anode materials exhibit a high reversible capacity of 1175, 1007, and 842 mA h g(-1), respectively, which show that the graphene sheets with fewer layers have higher reversible capacity. (C) 2011 Elsevier Inc. All rights reserved.
C1 [Tong, Xin; Wang, Hui; Wang, Gang] NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
   [Wang, Hui; Wan, Lijuan; Ren, Zhaoyu; Bai, Jintao] NW Univ Xian, Natl Key Lab Photoelect Technol & Funct Mat Cultu, Inst Photon & Photon Technol, Natl Photoelect Technol & Funct Mat & Applicat In, Xian 710069, Peoples R China.
   [Bai, Jinbo] Ecole Cent Paris, Lab MSS MAT, CNRS, UMR 8579, F-92295 Chatenay Malabry, France.
RP Wang, H (reprint author), NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
EM huiwang@nwu.edu.cn
RI Bai, Jinbo/F-8552-2010
FU National Basic Research Program of China (973 Program) [2009CB626611];
   National Natural Science Foundation of China [21061130551, 20873099,
   10974152]; Ph.D. Programs Foundation of Ministry of Education of China
   [20096101110002]; NWU [09YYB04, 07YJC03, 09YJC28]
FX The project was supported by the financial supports of the National
   Basic Research Program of China (973 Program) (no. 2009CB626611), the
   International cooperation research program of National Natural Science
   Foundation of China (no. 21061130551), the Ph.D. Programs Foundation of
   Ministry of Education of China (no. 20096101110002), the National
   Natural Science Foundation of China (nos. 20873099 and 10974152), NWU
   Doctorate Dissertation of Excellence Funds (09YYB04), and NWU Graduate
   Cross-discipline Funds (07YJC03 and 09YJC28). The authors are also
   grateful to the State Key Laboratory of Continental Dynamics for the SEM
   measurements.
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U2 32
PU ACADEMIC PRESS INC ELSEVIER SCIENCE
PI SAN DIEGO
PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA
SN 0022-4596
J9 J SOLID STATE CHEM
JI J. Solid State Chem.
PD MAY
PY 2011
VL 184
IS 5
BP 982
EP 989
DI 10.1016/j.jssc.2011.03.004
PG 8
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical
SC Chemistry
GA 763IL
UT WOS:000290549900004
ER

PT J
AU Du, GD
   Seng, KH
   Guo, ZP
   Liu, J
   Li, WX
   Jia, DZ
   Cook, C
   Liu, ZW
   Liu, HK
AF Du, Guodong
   Seng, Kuok Hau
   Guo, Zaiping
   Liu, Jun
   Li, Wenxian
   Jia, Dianzeng
   Cook, Chris
   Liu, Zongwen
   Liu, Huakun
TI Graphene-V2O5 center dot nH(2)O xerogel composite cathodes for lithium
   ion batteries
SO RSC ADVANCES
LA English
DT Article
ID INTERCALATION PROPERTIES; HIGH-PERFORMANCE; ANODE MATERIALS; V2O5;
   ELECTRODES; STORAGE; NANOPARTICLES; CAPACITY
AB A layer structured V2O5 center dot nH(2)O xerogel was synthesized via a simple green hydrothermal technique by dissolving commercial V2O5 powder in de-ionized water and hydrogen peroxide. Graphene-V2O5 center dot nH(2)O xerogel composites were then prepared by mixing and filtration of as-prepared V2O5 center dot nH(2)O xerogel and graphene in the desired ratio. The method is a cost effective and energy saving way to prepare nanostructured composites. Structure and morphology were investigated by X-ray diffraction, thermogravimetric analysis, field emission scanning electron microscopy, and transmission electron microscopy. Heat treatment at different temperatures could yield V2O5 center dot nH(2)O xerogels with different amounts of crystal water, and the presence of graphene in the composites enhanced the thermal stability of V2O5 center dot nH(2)O, in which the phase transformation moved towards higher temperature compared with the sample without graphene. The pristine V2O5 center dot nH(2)O xerogel consisted of thin layers of ribbons with widths around 100 nm. In the composites, the V2O5 center dot nH(2)O ribbons were located on the surface of the graphene sheets. Increasing the graphene content in the composites resulted in better cycling stability when the composites were tested as cathodes in different voltage ranges for lithium ion batteries. The initial and the 50th discharge capacities of the composite cathode with 17.8% graphene are 299 and 174 mAh g(-1), respectively, when cycled between 1.5 and 4.0 V. The capacities decreased to 227 and 156 mAh g(-1), respectively, when cycled between 2.0 and 4.0 V. The initial and the 50th discharge capacities of the composite with 39.6% graphene are 212 and 190 mAh g(-1) in the voltage range of 1.5-4.0 V, and the capacities are 143 and 163 mAh g(-1) when cycled between 2.0 and 4.0 V, respectively. The outstanding electrochemical performance could be attributed to the graphene induced unique structure and morphology.
C1 [Du, Guodong; Seng, Kuok Hau; Guo, Zaiping; Li, Wenxian; Liu, Huakun] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
   [Guo, Zaiping; Cook, Chris] Univ Wollongong, Fac Engn, Wollongong, NSW 2522, Australia.
   [Liu, Jun] Cent S Univ, Dept Mat Sci & Engn, Changsha 410083, Hunan, Peoples R China.
   [Jia, Dianzeng] Xinjiang Univ, Inst Appl Chem, Urumqi 830046, Peoples R China.
   [Liu, Zongwen] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia.
RP Du, GD (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2522, Australia.
EM zguo@uow.edu.au; liujun4982004@yahoo.com.cn; jdz@xju.edu.cn
RI Li, Wenxian/E-7742-2011; Liu, Hua/G-1349-2012
OI Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [LP0991012]
FX Financial support provided by the Australian Research Council (ARC)
   through a Linkage Project (LP0991012) is gratefully acknowledged. The
   authors would also like to thank Dr Tania Silver at the University of
   Wollongong for the critical reading of the manuscript.
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NR 39
TC 43
Z9 44
U1 14
U2 77
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2011
VL 1
IS 4
BP 690
EP 697
DI 10.1039/c1ra00258a
PG 8
WC Chemistry, Multidisciplinary
SC Chemistry
GA 833GB
UT WOS:000295869400021
ER

PT J
AU Liu, J
   Song, KP
   Zhu, CB
   Chen, CC
   van Aken, PA
   Maier, J
   Yu, Y
AF Liu, Jun
   Song, Kepeng
   Zhu, Changbao
   Chen, Chia-Chin
   van Aken, Peter A.
   Maier, Joachim
   Yu, Yan
TI Ge/C Nanowires as High-Capacity and Long-Life Anode Materials for Li-Ion
   Batteries
SO ACS NANO
LA English
DT Article
DE Li-Ion batteries; anodes; Ge; nanowires; carbon encapsulating
ID RECHARGEABLE LITHIUM BATTERIES; CARBON NANOFIBERS; STORAGE; PERFORMANCE;
   HOLLOW; NANOPARTICLES; GRAPHENE; LAYER; OXIDE; SN
AB Germanium-based materials (Ge and GeOx) have recently demonstrated excellent lithium-ion storage ability and are being considered as the most promising candidates to substitute commercial carbon-based anodes of lithium-ion batteries. Nevertheless, practical implementation of Ge-based materials to lithiumion batteries is greatly hampered by the poor cyclability that resulted from the huge volume variation during lithiation/delithiation processes. Herein, uniform carbon-encapsulated Ge and GeOx nanowires were synthesized by a one-step controlled pyrolysis of organic-inorganic hybrid GeOx/ethylenediamine (GeOx/EDA) nanowires in H-2/Ar and Ar atmospheres, respectively. The as-obtained Ge/C and GeOx/C nanowires possess well-defined 0D-in-1D morphology and homogeneous carbon encapsulation, which exhibit excellent Li storage properties including high specific capacities (approximate 1200 and 1000 mA h g(-1) at 0.2C for Ge/C and GeOx/C, respectively). The Ge/C nanowires, in particular, demonstrate superior rate capability with excellent capacity retention and stability (producing high stable discharge capacities of about 770 mA h g(-1) after 500 cycles at 10C), making them promising candidates for future electrodes for high-power U-ion batteries. The improved electrochemical performance arises from synergistic effects of 0D-in-1D morphology and uniform carbon coating, which could effectively accommodate the huge volume change of Ge/GeOx during cycling and maintain perfect electrical conductivity throughout the electrode.
C1 [Yu, Yan] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China.
   [Liu, Jun; Zhu, Changbao; Chen, Chia-Chin; Maier, Joachim; Yu, Yan] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany.
   [Song, Kepeng; van Aken, Peter A.] Max Planck Inst Intelligent Syst, D-70569 Stuttgart, Germany.
RP Yu, Y (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China.
EM yanyumse@ustc.edu.cn
RI Liu, Jun /K-4045-2015; Zhu, Changbao/B-7605-2016; Yu, Yan/C-7031-2012
OI Liu, Jun /0000-0002-7078-8046; 
FU Alexander von Humboldt Foundation; National Natural Science Foundation
   of China [21171015 and 21373195]; Recruitment Program of Global Experts,
   program for New Century Excellent Talents in University (NCET);
   Fundamental Research Funds for the Central Universities [WK2060140014,
   WK2060140016]; Max Planck Society; Chinese Academy Science; European
   Union Seventh Framework Programme [312483]
FX This work was financially supported by the Sofja Kovalevskaja award of
   the Alexander von Humboldt Foundation, the National Natural Science
   Foundation of China (Nos. 21171015 and 21373195), the Recruitment
   Program of Global Experts, program for New Century Excellent Talents in
   University (NCET), the Fundamental Research Funds for the Central
   Universities (WK2060140014, WK2060140016), and Max Planck Society. K.S.
   acknowledges financial support from the Doctor Training Program between
   the Max Planck Society and the Chinese Academy Science. The research
   leading to these results has received funding from the European Union
   Seventh Framework Programme (FP7/2007-2013) under Grant Agreement No.
   312483 (ESTEEM2).
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TC 42
Z9 42
U1 48
U2 226
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD JUL
PY 2014
VL 8
IS 7
BP 7051
EP 7059
DI 10.1021/nn501945f
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AL9LR
UT WOS:000339463100060
PM 24940842
ER

PT J
AU Lee, WJ
   Hwang, TH
   Hwang, JO
   Kim, HW
   Lim, J
   Jeong, HY
   Shim, J
   Han, TH
   Kim, JY
   Choi, JW
   Kim, SO
AF Lee, Won Jun
   Hwang, Tae Hoon
   Hwang, Jin Ok
   Kim, Hyun Wook
   Lim, Joonwon
   Jeong, Hu Young
   Shim, Jongwon
   Han, Tae Hee
   Kim, Je Young
   Choi, Jang Wook
   Kim, Sang Ouk
TI N-doped graphitic self-encapsulation for high performance silicon anodes
   in lithium-ion batteries
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID CARBON NANOTUBE ARRAYS; HIGH-CAPACITY; CORE/SHELL NANOWIRES; SECONDARY
   BATTERIES; GRAPHENE OXIDE; STORAGE; CHARGE; NANOPARTICLES; ADSORPTION;
   CHALLENGES
AB N-doped sites at CNT and graphene trigger spontaneous encapsulation of Si particles by simple pH control at room temperature. Significantly, N-doped CNT encapsulated Si composite electrode materials show remarkable cycle life and rate performance in battery operations. Superior capacity retention of 79.4% is obtained after 200 cycles and excellent rate capability of 914 mA h g(-1) is observed at a 10 C rate.
C1 [Lee, Won Jun; Hwang, Jin Ok; Lim, Joonwon; Shim, Jongwon; Kim, Sang Ouk] Inst for Basic Sci, Ctr Nanomat & Chem React, Taejon 305701, South Korea.
   [Lee, Won Jun; Hwang, Jin Ok; Lim, Joonwon; Shim, Jongwon; Kim, Sang Ouk] Korea Adv Inst Sci & Technol, Taejon 305701, South Korea.
   [Hwang, Tae Hoon; Choi, Jang Wook] Korea Adv Inst Sci & Technol, Grad Sch EEWS WCU, KAIST Inst NanoCentury, Taejon 305701, South Korea.
   [Kim, Hyun Wook; Kim, Je Young] LG Chem Ltd, Battery R&D, Taejon 305380, South Korea.
   [Jeong, Hu Young] UNIST, UNIST Cent Res Facil, Ulsan 689798, South Korea.
   [Jeong, Hu Young] UNIST, Sch Mech & Adv Mat Engn, Ulsan 689798, South Korea.
   [Han, Tae Hee] Hanyang Univ, Dept Organ & Nano Engn, Seoul 133791, South Korea.
RP Lee, WJ (reprint author), Inst for Basic Sci, Ctr Nanomat & Chem React, Taejon 305701, South Korea.
EM jangwookchoi@kaist.ac.kr; sangouk.kim@kaist.ac.kr
RI Choi, Jang Wook/C-1821-2011; Kim, Sang Ouk/C-1632-2011; Han, Tae
   Hee/E-8590-2015; Lee, Won Jun/O-9537-2015
OI Choi, Jang Wook/0000-0001-8783-0901; Kim, Sang Ouk/0000-0003-1513-6042;
   Han, Tae Hee/0000-0001-5950-7103; Lee, Won Jun/0000-0002-7121-057X
FU Institute for Basic Science (IBS) [CA1301-2]; Converging Research
   Program through the Korea government (MEST) [2012K001260]; National
   Research Foundation of Korea (NRF) [NRF-2012-R1A2A1A01011970]
FX This work was principally supported by the Institute for Basic Science
   (IBS) (CA1301-2) and Converging Research Program through the Korea
   government (MEST) (2012K001260). J. W. C. acknowledges a grant from the
   National Research Foundation of Korea (NRF) (NRF-2012-R1A2A1A01011970).
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NR 44
TC 42
Z9 42
U1 41
U2 185
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD FEB
PY 2014
VL 7
IS 2
BP 621
EP 626
DI 10.1039/c3ee43322f
PG 6
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AA9KZ
UT WOS:000331413700010
ER

PT J
AU Chen, Y
   Song, BH
   Li, M
   Lu, L
   Xue, JM
AF Chen, Yu
   Song, Bohang
   Li, Meng
   Lu, Li
   Xue, Junmin
TI Fe-3 O-4 Nanoparticles Embedded in Uniform Mesoporous Carbon Spheres for
   Superior High- Rate Battery Applications
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
DE porous materials; nanostructures; batteries; carbon; mesoporous carbon
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; CYCLIC STABILITY; RATE
   PERFORMANCE; ENERGY-STORAGE; AT-CARBON; NANOCOMPOSITES; GRAPHENE;
   CAPACITY; NANOSTRUCTURES
AB Robust composite structures consisting of Fe3O4 nanoparticles (approximate to 5 nm) embedded in mesoporous carbon spheres with an average size of about 70 nm (IONP@mC) are synthesized by a facile two-step method: uniform Fe3O4 nanoparticles are first synthesized followed by a post-synthetic low-temperature hydrothermal step to encapsulate them in mesoporous carbon spheres. Instead of graphene which has been extensively reported for use in high-rate battery applications as a carbonaceous material combined with metal oxides mesoporous carbon is chosen to enhance the overall performances. The interconnecting pores facilitate the penetration of electrolyte leading to direct contact between electrochemically active Fe3O4 and lithium ion-carrying electrolyte greatly facilitating lithium ion transportation. The interconnecting carbon framework provides continuous 3D electron transportation routes. The anodes fabricated from IONP@mC are cycled under high current densities ranging from 500 to 10 000 mA g(-1). A high reversible capacity of 271 mAh g(-1) is reached at 10 000 mAh g(-1) demonstrating its superior high rate performance.
C1 [Chen, Yu; Li, Meng; Xue, Junmin] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
   [Song, Bohang; Lu, Li] Natl Univ Singapore, Dept Mech Engn, Singapore 117576, Singapore.
RP Chen, Y (reprint author), Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
EM msexuejm@nus.edu.sg
RI Song, Bohang/F-8239-2016
OI Song, Bohang/0000-0002-6477-609X
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NR 43
TC 42
Z9 42
U1 49
U2 211
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1616-301X
EI 1616-3028
J9 ADV FUNCT MATER
JI Adv. Funct. Mater.
PD JAN
PY 2014
VL 24
IS 3
BP 319
EP 326
DI 10.1002/adfm.201300872
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AC9CU
UT WOS:000332832500005
ER

PT J
AU Chen, YJ
   Zhuo, M
   Deng, JW
   Xu, Z
   Li, QH
   Wang, TH
AF Chen, Yuejiao
   Zhuo, Ming
   Deng, Jiwei
   Xu, Zhi
   Li, Qiuhong
   Wang, Taihong
TI Reduced graphene oxide networks as an effective buffer matrix to improve
   the electrode performance of porous NiCo2O4 nanoplates for lithium-ion
   batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ELECTROCHEMICAL PERFORMANCE; ANODE MATERIAL; HIGH-CAPACITY; STORAGE
   PROPERTIES; NANOWIRE ARRAYS; SCALE SYNTHESIS; BINDER-FREE; NANOSHEETS;
   SPINEL; FABRICATION
AB Transition metal oxides are promising high-capacity anode materials for next-generation lithium-ion batteries. However, their cycle life remains a limiting factor with respect to their commercial applications. The development of transition-metal oxide anode materials with long lifespans through a facile route has become an important issue. A straightforward strategy is designed for the fabrication of a NiCo2O4 nanoplates-reduced graphene oxide sheets (NiCo2O4-RGO) composite. It displays a high reversible capacity of 816 mA h g(-1) over 70 cycles with 80.1% capacity retention of the 2nd cycle and excellent rate capability. Its rate capability and cycling stability are enhanced in comparison with those of pure NiCo2O4 nanoplates. The as-obtained nanocomposite avoids the problems of dispersion and aggregation induced by cracking or pulverization of the transition-metal oxide upon cycling. The graphene or reduced graphene oxide not only works as a substrate to provide room for loading scattered grains, but also serves as a conductive network to facilitate the collection and transportation of electrons during the cycling, indirectly increasing the conductivity of NiCo2O4.
C1 [Xu, Zhi; Li, Qiuhong; Wang, Taihong] Hunan Univ, Key Lab Micronano Optoelect Devices, State Key Lab Chemo Biosensing & Chemometr, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   [Chen, Yuejiao; Zhuo, Ming; Deng, Jiwei] Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China.
RP Wang, TH (reprint author), Hunan Univ, Key Lab Micronano Optoelect Devices, State Key Lab Chemo Biosensing & Chemometr, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM liqiuhong2004@hotmail.com; thwang@iphy.ac.cn
RI Wang, Taihong/K-8968-2012
FU National Natural Science Foundation of China [21003041, 21103046]; Hunan
   Provincial Natural Science Foundation of China [10JJ1011, 11JJ7004];
   Specialized Research Fund for the Doctoral Program of Higher Education
   of China [20120161110016]; Scholarship Award for Excellent Doctoral
   Student; Ministry of Education; Hunan Provincial Innovation Foundation
   for Postgraduates [CX2013B166]
FX This study was supported by the National Natural Science Foundation of
   China (Grant no. 21003041, 21103046), Hunan Provincial Natural Science
   Foundation of China (Grant no. 10JJ1011, 11JJ7004), Specialized Research
   Fund for the Doctoral Program of Higher Education of China
   (20120161110016), Scholarship Award for Excellent Doctoral Student
   granted by Ministry of Education and the Hunan Provincial Innovation
   Foundation for Postgraduates (Grant no. CX2013B166).
CR Sun YQ, 2011, ENERG ENVIRON SCI, V4, P1113, DOI 10.1039/c0ee00683a
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NR 38
TC 42
Z9 42
U1 23
U2 129
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 12
BP 4449
EP 4456
DI 10.1039/c3ta14624c
PG 8
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AC3BB
UT WOS:000332388900048
ER

PT J
AU Xu, X
   Fan, ZY
   Ding, SJ
   Yu, DM
   Du, YP
AF Xu, Xin
   Fan, Zhaoyang
   Ding, Shujiang
   Yu, Demei
   Du, Yaping
TI Fabrication of MoS2 nanosheet@TiO2 nanotube hybrid nanostructures for
   lithium storage
SO NANOSCALE
LA English
DT Article
ID ION BATTERY APPLICATIONS; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE;
   ASSISTED SYNTHESIS; HIERARCHICAL MOS2; TIO2; SNO2; GRAPHENE; SHELL;
   NANOCOMPOSITE
AB MoS2 nanosheet@TiO2 nanotube hybrid nanostructures were successfully prepared by a facile two-step method: prefabrication of porous TiO2 nanotubes based on a sol-gel method template against polymeric nanotubes, and then assembly of MoS2 nanoclusters that consist of ultrathin nanosheets through a solvothermal process. These hybrid nanostructures were characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), energy dispersive X-ray (EDX) spectroscopy, X-ray diffraction (XRD) and Brunauer-Emmett-Teller (BET) analysis. When evaluated as an electrode material for lithium ion batteries, the results of the electrochemical test show that the unique MoS2 nanosheet@TiO2 nanotube hybrid nanostructures exhibit outstanding lithium storage performances with high specific capacity and excellent rate capability. The smart architecture of the MoS2 nanosheet@TiO2 nanotube hybrid nanostructures makes a prominent contribution to the excellent electrochemical performance.
C1 [Xu, Xin; Fan, Zhaoyang; Ding, Shujiang; Yu, Demei] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Sch Sci, Dept Appl Chem, Xian 710049, Peoples R China.
   [Xu, Xin; Fan, Zhaoyang; Ding, Shujiang; Yu, Demei] Xi An Jiao Tong Univ, MOE Key Lab Nonequilibrium Synth & Modulat Conden, Sch Sci, Dept Appl Chem, Xian 710049, Peoples R China.
   [Du, Yaping] Xi An Jiao Tong Univ, Frontier Inst Chem, Frontier Inst Sci & Technol, Coll Sci, Xian 710054, Peoples R China.
RP Yu, DM (reprint author), Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Sch Sci, Dept Appl Chem, Xian 710049, Peoples R China.
EM dingsj@mail.xjtu.edu.cn
RI Du, Yaping/B-4440-2012; Ding, Shujiang/G-5025-2011; Xu, Xin/P-5009-2014
OI Ding, Shujiang/0000-0002-5683-0973; 
FU National Natural Science Foundation of China [51273158, 21303131];
   Natural Science Basis Research Plan in Shaanxi Province of China
   [2012JQ6003, 2013KJXX-49]; Ph.D. Programs Foundation of Ministry of
   Education of China [20120201120048]; Program for New Century Excellent
   Talents in University [NCET-13-0449]; Fundamental Research Funds for the
   Central Universities
FX This research was supported partially by the National Natural Science
   Foundation of China (no. 51273158 and 21303131); Natural Science Basis
   Research Plan in Shaanxi Province of China (no. 2012JQ6003 and
   2013KJXX-49); Ph.D. Programs Foundation of Ministry of Education of
   China (no. 20120201120048); Program for New Century Excellent Talents in
   University (NCET-13-0449). The authors are grateful to the Fundamental
   Research Funds for the Central Universities for financial support.
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NR 46
TC 42
Z9 42
U1 80
U2 363
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 10
BP 5245
EP 5250
DI 10.1039/c3nr06736j
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AG1BB
UT WOS:000335148800031
PM 24687092
ER

PT J
AU Jing, Y
   Zhou, Z
   Cabrera, CR
   Chen, ZF
AF Jing, Yu
   Zhou, Zhen
   Cabrera, Carlos R.
   Chen, Zhongfang
TI Metallic VS2 Monolayer: A Promising 2D Anode Material for Lithium Ion
   Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID MAGNETIC-PROPERTIES; DICHALCOGENIDE NANOSHEETS; CARBON NANOTUBES;
   GRAPHITE ANODE; SADDLE-POINTS; GRAPHENE; MOS2; NANORIBBONS; STORAGE;
   TRANSITION
AB By means of density functional theory computations, we systematically investigated the adsorption and diffusion of lithium on the recently synthesized VS2 monolayer, in comparison with MoS2 monolayer and graphite. Intrinsically metallic, VS2 monolayer has a higher theoretical capacity (466 mAh/g), a lower or similar Li diffusion barrier as compared to MoS2 and graphite, and has a low average open-circuit voltage of 0.93 V (vs Li/Li+). Our results suggest that VS2 monolayer can be utilized as a promising anode material for Li ion batteries with high power density and fast charge/discharge rates.
C1 [Jing, Yu; Cabrera, Carlos R.; Chen, Zhongfang] Univ Puerto Rico, Dept Chem, Inst Funct Nanomat, San Juan, PR 00931 USA.
   [Jing, Yu; Zhou, Zhen] Nankai Univ, Tianjin Key Lab Met & Mol Based Mat Chem, Computat Ctr Mol Sci,Inst New Energy Mat Chem, Key Lab Adv Energy Mat Chem,Minist Educ,Synerget, Tianjin 300071, Peoples R China.
RP Zhou, Z (reprint author), Nankai Univ, Tianjin Key Lab Met & Mol Based Mat Chem, Computat Ctr Mol Sci,Inst New Energy Mat Chem, Key Lab Adv Energy Mat Chem,Minist Educ,Synerget, Tianjin 300071, Peoples R China.
EM zhouzhen@nankai.edu.cn; zhongfangchen@gmail.com
RI Zhou, Zhen/C-4517-2008; Chen, Zhongfang/A-3397-2008; Jing,
   Yu/C-9280-2015
OI Zhou, Zhen/0000-0003-3232-9903; 
FU Department of Defense [W911NF-12-1-0083]; NSFC [21073096]; 111 Project
   [B12015]
FX Support in the U.S. by the Department of Defense (Grant
   W911NF-12-1-0083) and in China by NSFC (21073096) and 111 Project
   (B12015) is gratefully acknowledged.
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NR 55
TC 42
Z9 42
U1 63
U2 303
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD DEC 5
PY 2013
VL 117
IS 48
BP 25409
EP 25413
DI 10.1021/jp410969u
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 267ME
UT WOS:000328101200024
ER

PT J
AU Chen, L
   Wei, B
   Zhang, XT
   Li, C
AF Chen, Liang
   Wei, Bin
   Zhang, Xuetong
   Li, Chun
TI Bifunctional Graphene/gamma-Fe2O3 Hybrid Aerogels with Double
   Nanocrystalline Networks for Enzyme Immobilization
SO SMALL
LA English
DT Article
DE graphene; iron oxide; aerogels; double networks; enzyme immobilization
ID LITHIUM ION BATTERIES; GRAPHITE OXIDE; GRAPHENE OXIDE; GLYCYRRHIZIC
   ACID; REDUCED GRAPHENE; GREEN SYNTHESIS; ANODE MATERIAL; STORAGE;
   REDUCTION; NANOARCHITECTURES
AB Highly porous hosting materials with conducting (favorable to electron transfer) and magnetic (favorable to product separation) bicontinuous networks should possess great potentials for immobilization of various enzymes in the field of biocatalytic engineering, but the synthesis of such materials is still a great challenge. Herein, bifunctional graphene/-Fe2O3 hybrid aerogels with quite low density (30-65 mg cm(-3)), large specific surface area (270-414 m(2) g(-1)), high electrical conductivity (0.5-5 x 10(-2) S m(-1)), and superior saturation magnetization (23-54 emu g(-1)) are fabricated. Single networks of either graphene aerogels or -Fe2O3 aerogels are obtained by etching of the hybrid aerogels with acid solution or calcining of the hybrid aerogels in air, indicative of the double networks of the as-synthesized graphene/-Fe2O3 hybrid aerogels for the first time. The resulting bifunctional aerogels are used to immobilize -glucuronidase for biocatalytic transformation of glycyrrhizin into glycyrrhetinic acid monoglucuronide or glycyrrhetinic acid, with high biocatalytic activity and definite repeatability.
C1 [Chen, Liang; Zhang, Xuetong] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
   [Wei, Bin; Li, Chun] Beijing Inst Technol, Sch Life Sci & Technol, Beijing 100081, Peoples R China.
   [Wei, Bin] Shihezi Univ, Sch Chem & Chem Engn, Shihezi 832003, Xinjiang, Peoples R China.
RP Zhang, XT (reprint author), Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.
EM zhangxtchina@yahoo.com; lichun@bit.edu.cn
RI Li, Chun/B-3292-2013
FU National Natural Science Foundation of China [20903009, 21176028,
   20976014]; Innovation Program of the Beijing Institute of Technology
FX The first two authors contributed equally to this work. This work was
   financially supported by the National Natural Science Foundation of
   China (20903009,21176028 and 20976014) and the Innovation Program of the
   Beijing Institute of Technology.
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NR 62
TC 42
Z9 42
U1 36
U2 234
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD JUL 8
PY 2013
VL 9
IS 13
BP 2331
EP 2340
DI 10.1002/smll.201202923
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 193NO
UT WOS:000322566700019
PM 23423944
ER

PT J
AU Ren, JG
   Wu, QH
   Hong, G
   Zhang, WJ
   Wu, HM
   Amine, K
   Yang, JB
   Lee, ST
AF Ren, Jian-Guo
   Wu, Qi-Hui
   Hong, Guo
   Zhang, Wen-Jun
   Wu, Huiming
   Amine, Khalil
   Yang, Junbing
   Lee, Shuit-Tong
TI Silicon-Graphene Composite Anodes for High-Energy Lithium Batteries
SO ENERGY TECHNOLOGY
LA English
DT Article
DE anodes; batteries; graphene; lithium; silicon
ID LI-ION BATTERIES; SOLID-ELECTROLYTE-INTERPHASE; ATOMIC LAYER DEPOSITION;
   LONG CYCLE LIFE; HIGH-CAPACITY; SI; STORAGE; NANOPARTICLES; CONVERSION;
   NANOWIRES
AB A chemical vapor deposition process is introduced to prepare silicon (Si)-graphene composite anode materials for lithium-ion batteries. Highly ordered crystalline Si particles are deposited onto graphene sheets by using a liquid chlorosilane as Si source. The Si-graphene composite exhibits high utilization of Si in charge-discharge processes. The capacity retention of 90% after 500 full cycles and an average Coulombic efficiency in excess of 99.5% are achieved in half cells. Moreover, atomic layer deposition (ALD) Al2O3 coating is directly applied on the Si-graphene electrode, which greatly suppresses the side reactions between the electrode and electrolyte, resulting in the enhancement in initial Coulombic efficiency and reversible capacity. Finally, a 3.6 V full cell device is demonstrated, which works very well by combining a Si-graphene anode with a Li-excess layer-structured composite Li1.2Ni0.2Mn0.6O2 cathode. This approach is very promising for realizing a high-energy lithium-ion battery.
C1 [Ren, Jian-Guo; Wu, Qi-Hui; Hong, Guo; Lee, Shuit-Tong] Soochow Univ, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China.
   [Ren, Jian-Guo; Wu, Qi-Hui; Hong, Guo; Lee, Shuit-Tong] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China.
   [Ren, Jian-Guo; Wu, Qi-Hui; Hong, Guo; Zhang, Wen-Jun] City Univ Hong Kong, Dept Phys & Mat Sci, Ctr Super Diamond & Adv Films COSDAF, Kowloon, Hong Kong, Peoples R China.
   [Wu, Huiming; Amine, Khalil; Yang, Junbing] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.
   [Lee, Shuit-Tong] COSDAF, Melville, NY USA.
RP Yang, JB (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.
EM apannale@suda.edu.cn
RI Zhang, WJ/C-6995-2012
FU Research Grants Council of Hong Kong SAR, China-GRF Grant [CityU102010];
   National Natural Science Foundation of China [51072126, 51132006];
   National Basic Research Program of China (973 program) [2009CB623703,
   2012CB932402, 2012CB932600]; Priority Academic Program Development of
   Jiangsu Higher Education Institutions (PAPD)
FX This work was funded by Research Grants Council of Hong Kong SAR,
   China-GRF Grant (No. CityU102010), National Natural Science Foundation
   of China (No. 51072126, 51132006), National Basic Research Program of
   China (973 program) (No. 2009CB623703, 2012CB932402, 2012CB932600) and a
   Project Funded by the Priority Academic Program Development of Jiangsu
   Higher Education Institutions (PAPD).
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NR 56
TC 42
Z9 42
U1 31
U2 98
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 2194-4288
EI 2194-4296
J9 ENERGY TECHNOL-GER
JI Energy Technol.
PD JAN
PY 2013
VL 1
IS 1
BP 77
EP 84
DI 10.1002/ente.201200038
PG 8
WC Energy & Fuels
SC Energy & Fuels
GA AK3RX
UT WOS:000338343500019
ER

PT J
AU Li, N
   Cao, MH
   Hu, CW
AF Li, Na
   Cao, Minhua
   Hu, Changwen
TI Review on the latest design of graphene-based inorganic materials
SO NANOSCALE
LA English
DT Review
ID LITHIUM-ION BATTERIES; SINGLE-LAYER GRAPHENE; MIYAURA COUPLING REACTION;
   POLYMER MEMORY DEVICES; IN-SITU SYNTHESIS; AMMONIUM-PERCHLORATE; OXIDE
   SHEETS; METAL NANOPARTICLES; ANODE MATERIAL; PHOTOCATALYTIC REDUCTION
AB The breathtakingly fast evolution of research on graphene and its modification methods in the recent 8 years has made possible the various preparations and applications of its derivatives. These hybrid structures exhibit excellent material characteristics including high carrier mobility and radiate recombination rate as well as long-term stability since graphene sheets possess super electrical conductivity, mechanical flexibility and good optical transparency. Besides, the versatile and fascinating properties of the nanostructures grown on graphene layers make it possible to fabricate high-performance electronic, optoelectronic and catalytic devices. This review presents an overview of the latest design of structure, synthetic methods and applications of graphene-based inorganic nanocomposites. The challenges and perspectives of these emerging hybrid heterostructures are also discussed.
C1 [Li, Na; Cao, Minhua; Hu, Changwen] Beijing Inst Technol, Key Lab Cluster Sci, Minist Educ China, Dept Chem, Beijing 100081, Peoples R China.
RP Cao, MH (reprint author), Beijing Inst Technol, Key Lab Cluster Sci, Minist Educ China, Dept Chem, Beijing 100081, Peoples R China.
EM caomh@bit.edu.cn
FU Natural Science Foundation of China [21173021, 21231002, 21276026,
   21271023, 91022006, 20973023]; 111 Project [B07012]; Program of
   Cooperation of the Beijing Education Commission [20091739006];
   specialized research fund for the doctoral program of higher education
   (SRFDP) [20101101110031]
FX This work was financially supported by the Natural Science Foundation of
   China 21173021, 21231002, 21276026, 21271023, 91022006, and 20973023,
   the 111 Project (B07012), the Program of Cooperation of the Beijing
   Education Commission (20091739006), and specialized research fund for
   the doctoral program of higher education (SRFDP. No. 20101101110031).
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NR 234
TC 42
Z9 42
U1 44
U2 327
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 20
BP 6205
EP 6218
DI 10.1039/c2nr31750h
PG 14
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 035UW
UT WOS:000310976800008
PM 22961110
ER

PT J
AU Chen, Y
   Song, BH
   Tang, XS
   Lu, L
   Xue, JM
AF Chen, Yu
   Song, Bohang
   Tang, Xiaosheng
   Lu, Li
   Xue, Junmin
TI Ultrasmall Fe3O4 Nanoparticle/MoS2 Nanosheet Composites with Superior
   Performances for Lithium Ion Batteries
SO SMALL
LA English
DT Article
DE molybdenum disulfide; 2D materials; nanostructures; batteries
ID ANODE MATERIAL; GRAPHENE NANOSHEETS; REVERSIBLE CAPACITY; CYCLIC
   PERFORMANCE; REDUCED GRAPHENE; RATE CAPABILITY; MOS2; LI; STORAGE;
   ELECTRODE
AB A novel composite consisting of graphene-like MoS2 nanosheets and ultrasmall Fe3O4 nanoparticles (approximate to 3.5 nm) is synthesized as an anode for lithium ion battery application. In such composite anode, MoS2 nanosheets provide flexible substrates for the nanoparticle decoration, accommodating the volume changes of Fe3O4 during cycling process; while Fe3O4 nanoparticles primarily act as spacers to stabilize the composite structure, making the active surfaces of MoS2 nanosheets accessible for electrolyte penetration during charge/discharge processes. Owing to the high reversible capacity provided by the MoS2 nanosheets and the superior high rate performance offered by ultrasmall Fe3O4 nanoparticles, superior cyclic and rate performances are achieved by Fe3O4/MoS2 anode during the subsequent electrochemical tests, delivering 1033 and 224 mAh g(-1) at current densities of 2000 and 10 000 mA g(-1), respectively.
C1 [Chen, Yu; Tang, Xiaosheng; Xue, Junmin] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
   [Song, Bohang; Lu, Li] Natl Univ Singapore, Dept Mech Engn, Singapore 117576, Singapore.
RP Xue, JM (reprint author), Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
EM msexuejm@nus.edu.sg
RI Song, Bohang/F-8239-2016
OI Song, Bohang/0000-0002-6477-609X
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EI 1613-6829
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JI Small
PD APR
PY 2014
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BP 1536
EP 1543
DI 10.1002/smll.201302879
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
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SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AE8VH
UT WOS:000334280500014
PM 24376114
ER

PT J
AU Hu, YH
   Sun, XL
AF Hu, Yuhai
   Sun, Xueliang
TI Flexible rechargeable lithium ion batteries: advances and challenges in
   materials and process technologies
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID POLYMER ELECTROLYTE BATTERIES; GRAPHENE PAPER ELECTRODES; ENERGY-STORAGE
   DEVICES; CARBON NANOTUBE PAPER; BINDER-FREE ANODE; CURRENT COLLECTOR;
   COMPOSITE ELECTROLYTES; ALKALINE BATTERIES; ELECTROCHEMICAL PERFORMANCE;
   NUMERICAL-SIMULATION
AB Flexible batteries possess several unique features including high flexibility, lightweight and easy portability, high specific power and energy density, and remarkable rate capability, etc. So far, many different kinds of flexible batteries have been invented. The batteries, according to the electrochemical processes in a cell, can be categorized as flexible alkaline batteries, plastic batteries (or all-polymer batteries), polymer lithium-metal batteries (with lithium foil as an anode), and flexible rechargeable lithium ion batteries (LIBs), etc. Among these, flexible LIBs attract more rapidly increasing attention. As compared to the conventional rechargeable LIBs, fabrication of flexible LIBs is more challenging. An optimal match among the core components, i.e., nanostructured electrode materials, shape-conformable solid electrolytes, and soft current collectors should be achieved, so that the batteries maintain stable electrochemical performances even though they are deformed to fit the powered devices. Thus, fabrication of such batteries is not cost-effective and hence, is also inefficient. In the search for the potential core components for flexible LIBs, much progress has been made in screening solid state electrolytes, soft current collectors and electrode materials, and in electrode design and full LIB cell assembly (particularly in managing to get the three core components to work harmonically). There are also studies focusing on fundamental understanding and simulation of fully flexible LIBs. They reliably anticipate and describe the battery performances that are not easily explored experimentally using the present state-of-the-art technologies. In this review, we systematically summarize the advances in flexible LIBs research, with focus on the development of flexible electrodes. The review proceeds in terms of the processes for making electrodes and full LIB cells so as to emphasize the materials and process technologies. The development of solid state electrolytes and the fundamental understanding and simulation of flexible LIBs are also addressed. The review concludes with a perspective according to the author's experience in the related field, and the potential application of printing processes in flexible LIB fabrication is especially emphasized.
C1 [Hu, Yuhai; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, Fac Engn, London, ON N6A 5B7, Canada.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, Fac Engn, London, ON N6A 5B7, Canada.
EM xsun9@uwo.ca
RI Sun, Xueliang/C-7257-2012
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NR 160
TC 41
Z9 41
U1 54
U2 192
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 28
BP 10712
EP 10738
DI 10.1039/c4ta00716f
PG 27
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AK5AE
UT WOS:000338435200002
ER

PT J
AU Wang, L
   Wang, D
   Dong, ZH
   Zhang, FX
   Jin, J
AF Wang, Lei
   Wang, Dong
   Dong, Zhihui
   Zhang, Fengxing
   Jin, Jian
TI Interface Chemistry Engineering for Stable Cycling of Reduced GO/SnO2
   Nanocomposites for Lithium Ion Battery
SO NANO LETTERS
LA English
DT Article
DE Interface chemistry engineering; RGO/SnO2 nanosheets; polydopamine;
   lithium-ion battery
ID SNO2 HOLLOW NANOSPHERES; NEGATIVE ELECTRODES; ANODE MATERIAL; STORAGE;
   PERFORMANCE; COMPOSITE; CAPACITY; CHALLENGES; NANOWIRES; GRAPHENE
AB From the whole anode electrode of view, we report in this work a system-level strategy of fabrication of reduced graphene oxide (RGO)/SnO2 composite-based anode for lithium ion battery (LIB) to enhance the capacity and cyclic performance of SnO2-based electrode materials. RGO/SnO2 composite was first coated by a nanothick polydopamine (PD) layer and the PD-coated RGO/SnO2 composite was then cross-linked with poly(acrylic acid) (PAA) that was used as a binder to accomplish a whole anode electrode. The cross-link reaction between PAA and PD produced a robust network in the anode system to stabilize the whole anode during cycling. As a result, the designed anode exhibits an outstanding energy capacity up to 718 mAh/g at current density of 100 mA/g after 200 cycles and a good rate performance of 811, 700, 641, and 512 mAh/g at current density of 100, 250, 500, and 1000 mA/g, respectively. Fourier transform IR spectra confirm the formation of cross-link reaction and the stability of the robust network after long-term cycling. Our results indicate the importance of designing interfaces in anode system on achieving improved performance of electrode of LIBs.
C1 [Wang, Lei; Wang, Dong; Dong, Zhihui; Jin, Jian] Chinese Acad Sci, i LAB, Suzhou Inst Nanotech & Nanobion, Suzhou 215123, Jiangsu, Peoples R China.
   [Wang, Lei; Wang, Dong; Dong, Zhihui; Jin, Jian] Chinese Acad Sci, Nanobion Div, Suzhou Inst Nanotech & Nanobion, Suzhou 215123, Jiangsu, Peoples R China.
   [Wang, Lei; Zhang, Fengxing] NW Univ Xian, Key Lab Synth & Nat Funct Mol Chem, Minist Educ, Coll Chem & Mat Sci, Xian 710069, Shaanxi, Peoples R China.
RP Jin, J (reprint author), Chinese Acad Sci, i LAB, Suzhou Inst Nanotech & Nanobion, Suzhou 215123, Jiangsu, Peoples R China.
EM jjin2009@sinano.ac.cn
FU National Basic Research Program of China [2013CB933000, 2010CB934700];
   National Natural Science Foundation of China [21004076]; Key Development
   Project of Chinese Academy of Sciences [KJZD-EW-M01-3]
FX We thank Professor Liwei Chen and Ms. Welling Dong at Suzhou Institute
   of Nanotech and Nanobionics (SINANO) for providing instrument for
   battery assembling. This work was supported by the National Basic
   Research Program of China (Grants 2013CB933000 and 2010CB934700), the
   National Natural Science Foundation of China (Grant 21004076), and the
   Key Development Project of Chinese Academy of Sciences (Grant
   KJZD-EW-M01-3).
CR McDowell MT, 2011, NANO LETT, V11, P4018, DOI 10.1021/nl202630n
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NR 39
TC 41
Z9 42
U1 37
U2 353
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
J9 NANO LETT
JI Nano Lett.
PD APR
PY 2013
VL 13
IS 4
BP 1711
EP 1716
DI 10.1021/nl400269d
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 125OO
UT WOS:000317549300056
PM 23477450
ER

PT J
AU Xia, H
   Qian, YY
   Fu, YS
   Wang, X
AF Xia, Hui
   Qian, Yanyan
   Fu, Yongsheng
   Wang, Xin
TI Graphene anchored with ZnFe2O4 nanoparticles as a high-capacity anode
   material for lithium-ion batteries
SO SOLID STATE SCIENCES
LA English
DT Article
DE Zinc ferrite; Graphene; Anode material; Lithium-ion batteries;
   Nanocomposite
ID HIGH-PERFORMANCE; REVERSIBLE CAPACITY; STORAGE; OXIDE; NANOCOMPOSITES;
   COMPOSITE; FERRITE; HYBRID
AB Heterostructured ZnFe2O4-graphene nanocomposites are synthesized by a facile hydrothermal method. The as-prepared ZnFe2O4-graphene nanocomposites are characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), Brunauer-Emmett-Teller (BET) analysis and galvanostatic charge and discharge measurements. Compared with the pure ZnFe2O4 nanoparticles, the ZnFe2O4-graphene nanocomposites exhibit much larger reversible capacity up to 980 mAh g(-1), greatly improved cycling stability, and excellent rate capability. The superior electrochemical performance of the ZnFe2O4-graphene nanocomposites could be attributed to the synergetic effect between the conducting graphene nanosheets and the ZnFe2O4 nanoparticles. (C) 2012 Elsevier Masson SAS. All rights reserved.
C1 [Xia, Hui; Qian, Yanyan] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China.
   [Xia, Hui; Fu, Yongsheng; Wang, Xin] Nanjing Univ Sci & Technol, Key Lab Soft Chem & Funct Mat, Minist Educ, Nanjing 210094, Jiangsu, Peoples R China.
RP Xia, H (reprint author), Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, 200 Xiaoling wei, Nanjing 210094, Jiangsu, Peoples R China.
EM xiahui@njust.edu.cn; wxin@public1.ptt.js.cn
OI Xia, Hui/0000-0002-2517-2410
FU National Natural Science Foundation of China [21171094, 51102134];
   Priority Academic Program Development of Jiangsu Higher Education
   Institutions; NUST [2011PYXM03, 2011ZDJH21]; Department of Education of
   Jiangsu Province [CXZZ11_0245]
FX This investigation was supported by the National Natural Science
   Foundation of China (No. 21171094, 51102134), A Project Funded by the
   Priority Academic Program Development of Jiangsu Higher Education
   Institutions, NUST Research Funding (2011PYXM03, 2011ZDJH21) and the
   Department of Education of Jiangsu Province (CXZZ11_0245).
CR Zhou L, 2012, ADV MATER, V24, P745, DOI 10.1002/adma.201104407
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NR 33
TC 41
Z9 42
U1 11
U2 150
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1293-2558
J9 SOLID STATE SCI
JI Solid State Sci.
PD MAR
PY 2013
VL 17
BP 67
EP 71
DI 10.1016/j.solidstatesciences.2012.12.001
PG 5
WC Chemistry, Inorganic & Nuclear; Chemistry, Physical; Physics, Condensed
   Matter
SC Chemistry; Physics
GA 110IZ
UT WOS:000316437100011
ER

PT J
AU Liu, Y
   Qiao, Y
   Zhang, WX
   Li, Z
   Hu, XL
   Yuan, LX
   Huang, YH
AF Liu, Yang
   Qiao, Yun
   Zhang, Wu-Xing
   Li, Zhen
   Hu, Xian-Luo
   Yuan, Li-Xia
   Huang, Yun-Hui
TI Coral-like alpha-MnS composites with N-doped carbon as anode materials
   for high-performance lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID HYDROTHERMAL SYNTHESIS; STORAGE PROPERTIES; ELECTRICAL-PROPERTIES;
   MANGANESE SULFIDE; RATE CAPABILITY; HOLLOW SPHERES; NANOSHEETS;
   CAPACITY; GRAPHENE; NANOPARTICLES
AB Coral-like alpha-MnS composites with nitrogen-doped carbon (NC) were designed as anode materials for lithium-ion batteries. A facile two-step method was developed to synthesize the composites. Hydrothermally obtained polyvinyl pyrrolidone (PVP) capped (NH4)(2)Mn-2(SO4)(3) was used as a precursor. The alpha-MnS-NC composites were attained by heating the precursor at different temperatures for an appropriate time in a N-2 atmosphere. The microstructure and morphology were carefully investigated by means of field emission scanning electron microscopy (FE-SEM), transmission electron microscopy (TEM), and powder X-ray diffraction (XRD). As anode materials, the alpha-MnS-NC composites exhibit large reversible capacity, excellent cyclic stability and high rate capability. At a current density of 500 mA g(-1), the discharge capacity reaches as high as 878 mA h g(-1) at the first cycle and remains at 699 mA h g(-1) even after 400 cycles.
C1 [Liu, Yang; Qiao, Yun; Zhang, Wu-Xing; Li, Zhen; Hu, Xian-Luo; Yuan, Li-Xia; Huang, Yun-Hui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
RP Zhang, WX (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
EM zhangwx@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Liu, Yang/H-6110-2013; Huang, Yunhui/C-3752-2014; Qiao, Yun/D-8491-2014;
   Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU Natural Science Foundation of China [50825203, 51002057]; 863 program
   [2011AA11290]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University); Fundamental Research Funds for the Central
   Universities [HUST: 2010QN007]
FX This work was supported by the Natural Science Foundation of China
   (Grant nos. 50825203 and 51002057), the 863 program (Grant no.
   2011AA11290), the PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University), and the Fundamental Research Funds for the
   Central Universities (HUST: 2010QN007). In addition, the authors thank
   Analytical and Testing Center of HUST for XRD, Raman measurements, and
   the State Key Laboratory of Materials Processing and Die & Mould
   Technology of HUST for FE-SEM and EDS measurements.
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NR 43
TC 41
Z9 41
U1 35
U2 219
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PD DEC 7
PY 2012
VL 22
IS 45
BP 24026
EP 24033
DI 10.1039/c2jm35227c
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 043DG
UT WOS:000311522500041
ER

PT J
AU Hwang, SG
   Kim, GO
   Yun, SR
   Ryu, KS
AF Hwang, Seung-Gi
   Kim, Gyeong-Ok
   Yun, Su-Ryeon
   Ryu, Kwang-Sun
TI NiO nanoparticles with plate structure grown on graphene as fast
   charge-discharge anode material for lithium ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; NiO; Anode; Lithium ion batteries
ID CARBONACEOUS MATERIALS; CYCLIC PERFORMANCE; STORAGE; LI; INSERTION;
   OXIDE; ELECTRODES; CAPACITY; NANOSTRUCTURES; NANOCOMPOSITE
AB A graphene/NiO composite was prepared by simple chemical precipitation followed by thermal annealing. The results of XRD, FT-IR, FE-SEM, FE-TEM, and EDS analyses confirmed the presence of NiO nanoparticles with plate structure on the graphene surface. The discharge capacities of graphene, graphene/NiO (37 wt.%), and graphene/NiO (59 wt.%) are about 302, 604, and 856 mAh g(-1) at 5000 mA g(-1) (5 C), respectively. The cells containing 59 wt.% NiO show the best performance, and the graphene nanocomposite materials have high rate properties that are comparable to some of the best results reported in the literature using NiO. This graphene/NiO (37 and 59 wt.%) nanocomposite displays superior LIB performance with large reversible capacity, high Coulombic efficiency, good cyclic performance, and excellent rate capability, highlighting the importance of the anchoring of nanoplate structure NiO on graphene sheets for maximum utilization of electrochemically active graphene/NiO for energy storage applications in high-performance LIB. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Hwang, Seung-Gi; Kim, Gyeong-Ok; Yun, Su-Ryeon; Ryu, Kwang-Sun] Univ Ulsan, Dept Chem, Ulsan 680749, South Korea.
RP Ryu, KS (reprint author), Univ Ulsan, Dept Chem, Daehak Ro 93, Ulsan 680749, South Korea.
EM ryuks@ulsan.ac.kr
FU University of Ulsan, Ulsan, Korea
FX This work was supported by the 2011 Research Fund of the University of
   Ulsan, Ulsan, Korea.
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NR 36
TC 41
Z9 42
U1 12
U2 136
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD SEP 1
PY 2012
VL 78
BP 406
EP 411
DI 10.1016/j.electacta.2012.06.031
PG 6
WC Electrochemistry
SC Electrochemistry
GA 998SA
UT WOS:000308259500054
ER

PT J
AU Kim, GP
   Nam, I
   Kim, ND
   Park, J
   Park, S
   Yi, J
AF Kim, Gil-Pyo
   Nam, Inho
   Kim, Nam Dong
   Park, Junsu
   Park, Soomin
   Yi, Jongheop
TI A synthesis of graphene/Co3O4 thin films for lithium ion battery anodes
   by coelectrodeposition
SO ELECTROCHEMISTRY COMMUNICATIONS
LA English
DT Article
DE Graphene; Poly(ethyleneimine); Cobalt oxide; Coelectrodeposition;
   Lithium ion battery
ID OXIDE; CO3O4
AB We report on a facile strategy for the direct and uniform deposition of a graphene/Co3O4 thin film onto stainless steel substrate (SS) through cathodic deposition. Graphene oxides (GOs) were treated with poly(ethyleneimine) (PEI) which acted as a stabilizer and binder between GOs and cationic metal precursor. For the formation of PEI-modified GOs (PEI-GOs) and Co2+ complexes, the PEI-GOs dispersion was mixed with aqueous phase of Co(NO3)(2), then, the solution was used as the plating bath for coelectrodeposition. Results showed that the PEI-GOs and cobalt oxides were uniformly distributed on the surface of SS evidenced by field emission scanning electron microscopy. The prepared graphene/Co3O4 film was employed as an anode material for lithium ion batteries, and it exhibited not only an enhanced cycleability but also high electronic conductivity. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Kim, Gil-Pyo; Nam, Inho; Kim, Nam Dong; Park, Junsu; Park, Soomin; Yi, Jongheop] SNU, Coll Engn, WCU,Sch Chem & Biol Engn, Program Chem Convergence Energy & Environm C2E2, Seoul, South Korea.
RP Yi, J (reprint author), SNU, Coll Engn, WCU,Sch Chem & Biol Engn, Program Chem Convergence Energy & Environm C2E2, Seoul, South Korea.
EM jyi@snu.ac.kr
FU WCU (World Class University) through the National Research Foundation of
   Korea; Ministry of Education, Science and Technology [R31-10013]
FX This research was supported by WCU (World Class University) program
   through the National Research Foundation of Korea funded by the Ministry
   of Education, Science and Technology (R31-10013).
CR Novoselov KS, 2005, NATURE, V438, P197, DOI 10.1038/nature04233
   Yu DS, 2010, J PHYS CHEM LETT, V1, P467, DOI 10.1021/jz9003137
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NR 14
TC 41
Z9 42
U1 7
U2 102
PU ELSEVIER SCIENCE INC
PI NEW YORK
PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
SN 1388-2481
J9 ELECTROCHEM COMMUN
JI Electrochem. Commun.
PD AUG
PY 2012
VL 22
BP 93
EP 96
DI 10.1016/j.elecom.2012.05.032
PG 4
WC Electrochemistry
SC Electrochemistry
GA 005SP
UT WOS:000308770500024
ER

PT J
AU Hsieh, CT
   Lin, JY
   Mo, CY
AF Hsieh, Chien-Te
   Lin, Jia-Yi
   Mo, Chung-Yu
TI Improved storage capacity and rate capability of Fe3O4-graphene anodes
   for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Iron oxide; Anode; Graphene sheets; Lithium ion battery; Rate capability
ID ELECTROCHEMICAL PROPERTIES; RECHARGEABLE BATTERIES; OXIDE;
   NANOPARTICLES; ELECTRODES; PERFORMANCE; STABILITY; COMPOSITE
AB By employing an ultrasonic deposition followed by heat treatment, magnetite (Fe3O4)-graphene nanosheet (GN) hybrid anode was synthesized to examine its electrochemical performance in Li-ion battery. The Fe3O4 nanocrystals with an average size of 10 nm can be homogeneously incorporated into the GNs to form Fe3O4-GN composites. In comparison with fresh GN anode, the composite anode exhibits high reversible capacity of 753 mAh/g at 0.1 C. high rate capability (533 mAh/g at 5 C), and enhanced cyclic performance with high coulombic efficiency. This improvement can be attributed to the fact that since Fe3O4 acts not only as a redox site but also as a spacer, the Fe3O4-GN hybrid creates a three-dimensional architecture that effectively facilitates ionic diffusion, Li-storage, and electronic transport. This result opens an efficient route for synthesis and application of GN hybrid as anode material for Li-ion batteries with superior performance. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Hsieh, Chien-Te; Lin, Jia-Yi; Mo, Chung-Yu] Yuan Ze Univ, Yuan Ze Fuel Cell Ctr, Dept Chem Engn & Mat Sci, Tao Yuan 320, Taiwan.
RP Hsieh, CT (reprint author), Yuan Ze Univ, Yuan Ze Fuel Cell Ctr, Dept Chem Engn & Mat Sci, Tao Yuan 320, Taiwan.
EM cthsieh@saturn.yzu.edu.tw
FU National Science Council of the Republic of China [NSC
   100-2120-M-155-031, NSC 100-2221-E-155-078, NSC 99-2632-E-155-001-MY3]
FX The authors are very grateful for the financial support from the
   National Science Council of the Republic of China under the contracts
   NSC 100-2120-M-155-031, NSC 100-2221-E-155-078, and NSC
   99-2632-E-155-001-MY3.
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NR 24
TC 41
Z9 41
U1 7
U2 95
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD DEC 30
PY 2011
VL 58
BP 119
EP 124
DI 10.1016/j.electacta.2011.09.008
PG 6
WC Electrochemistry
SC Electrochemistry
GA 871VH
UT WOS:000298765300018
ER

PT J
AU Zhao, Y
   Li, XF
   Yan, B
   Li, DJ
   Lawes, S
   Sun, XL
AF Zhao, Yang
   Li, Xifei
   Yan, Bo
   Li, Dejun
   Lawes, Stephen
   Sun, Xueliang
TI Significant impact of 2D graphene nanosheets on large volume change
   tin-based anodes in lithium-ion batteries: A review
SO JOURNAL OF POWER SOURCES
LA English
DT Review
DE 2D graphene; Tin-based anodes; Tin oxide; Stannate; Lithium-ion
   batteries
ID NITROGEN-DOPED GRAPHENE; HIGH-PERFORMANCE ANODE; HOLLOW ZN2SNO4 BOXES;
   ENHANCED ELECTROCHEMICAL PERFORMANCE; NEGATIVE-ELECTRODE MATERIALS;
   MULTIWALL CARBON NANOTUBES; CHEMICAL-VAPOR-DEPOSITION; LI-STORAGE
   PROPERTIES; LARGE-SCALE SYNTHESIS; ONE-STEP SYNTHESIS
AB Sn-based materials have attracted much attention as anodes in lithium ion batteries (LIBs) due to their low cost, high theoretical capacities, and high energy density. However, their practical applications are limited by the poor cyclability originating from the huge volume changes. Graphene nanosheets (GNSs), a novel two-dimensional carbon sheet with one atom thickness and one of the thinnest materials, significantly address the challenges of Sn-based anodes as excellent buffering materials, showing great research interests in LIBs. In this review, various nanocomposites of GNSs/Sn-based anodes are summarized in detail, including binary and ternary composites. The significant impact of 2D GNSs on the volume change of Sn-based anodes during cycling is discussed, along with with their preparation methods, properties and enhanced LIB performance. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Zhao, Yang; Li, Xifei; Yan, Bo; Li, Dejun; Sun, Xueliang] Tianjin Normal Univ, Coll Phys & Mat Sci, Energy & Mat Engn Ctr, Tianjin 300387, Peoples R China.
   [Lawes, Stephen; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, Nanomat & Energy Lab, London, ON N6A 5B9, Canada.
RP Li, XF (reprint author), Tianjin Normal Univ, Coll Phys & Mat Sci, Energy & Mat Engn Ctr, Tianjin 300387, Peoples R China.
EM xfli2011@hotmail.com; dejunli@mail.tjnu.edu.cn
RI Sun, Xueliang/C-7257-2012; Li, Xifei/A-1966-2012; Zhao, Yang/I-5700-2015
OI Li, Xifei/0000-0002-4828-4183; Zhao, Yang/0000-0002-4148-2603
FU Key Project of Tianjin Municipal Natural Science Foundation of China
   [14JCZDJC32200, 13JCZDJC33900]; National Natural Science Foundation of
   China [51472180, 51272176]; LPMT, CAEP [KF14006, ZZ13007]; CAEP
   [2013A030214]; Science & Technology Depal Intent of Sichuan Province
   [2013GZX0145-3]; Thousand Youth Talents in Tianjin of China
FX This research was supported by Key Project of Tianjin Municipal Natural
   Science Foundation of China (14JCZDJC32200 and 13JCZDJC33900), National
   Natural Science Foundation of China (51472180 and 51272176), LPMT, CAEP
   (KF14006 and ZZ13007), Project 2013A030214 supported by CAEP, Science &
   Technology Depal Intent of Sichuan Province (2013GZX0145-3), and the
   program of Thousand Youth Talents in Tianjin of China.
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NR 267
TC 40
Z9 40
U1 147
U2 435
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD JAN 15
PY 2015
VL 274
BP 869
EP 884
DI 10.1016/j.jpowsour.2014.10.008
PG 16
WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology -
   Other Topics; Materials Science
GA AY0DT
UT WOS:000347268700106
ER

PT J
AU Zhou, F
   Xin, S
   Liang, HW
   Song, LT
   Yu, SH
AF Zhou, Fei
   Xin, Sen
   Liang, Hai-Wei
   Song, Lu-Ting
   Yu, Shu-Hong
TI Carbon Nanofibers Decorated with Molybdenum Disulfide Nanosheets:
   Synergistic Lithium Storage and Enhanced Electrochemical Performance
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE carbon nanofibers; electrochemistry; lithium-ion battery; molybdenum;
   nanostructures
ID ION BATTERIES; SULFUR BATTERIES; ANODE MATERIALS; MOS2; NANOCOMPOSITES;
   CAPACITY; GRAPHENE; INSERTION; NETWORKS
AB Traditional lithium-ion batteries that are based on layered Li intercalation electrode materials are limited by the intrinsically low theoretical capacities of both electrodes and cannot meet the increasing demand for energy. A facile route for the synthesis of a new type of composite nanofibers, namely carbon nanofibers decorated with molybdenum disulfide sheets (CNFs@MoS2), is now reported. A synergistic effect was observed for the two-component anode, triggering new electrochemical processes for lithium storage, with a persistent oxidation from Mo (or MoS2) to MoS3 in the repeated charge processes, leading to an ascending capacity upon cycling. The composite exhibits unprecedented electrochemical behavior with high specific capacity, good cycling stability, and superior high-rate capability, suggesting its potential application in high-energy lithium-ion batteries.
C1 [Zhou, Fei; Xin, Sen; Liang, Hai-Wei; Song, Lu-Ting; Yu, Shu-Hong] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Dept Chem,Div Nanomat & Chem, Hefei 230026, Peoples R China.
   [Xin, Sen] Hefei Univ Technol, Sch Chem Engn, Anhui Key Lab Controllable Chem React & Mat Chem, Hefei 230009, Anhui, Peoples R China.
RP Yu, SH (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Dept Chem,Div Nanomat & Chem, Hefei 230026, Peoples R China.
EM shyu@ustc.edu.cn
RI Liang, Hai-Wei/B-7292-2011; Yu, Shu-Hong/A-1903-2010
OI Yu, Shu-Hong/0000-0003-3732-1011
FU National Basic Research Program of China [2010CB934700, 2013CB933900,
   2014CB931800]; National Natural Science Foundation of China [21431006,
   91022032, 91227103]; Chinese Academy of Sciences [KJZD-EW-M01-1]; China
   Postdoctoral Science Foundation [2012M510160]
FX This work is supported by the National Basic Research Program of China
   (2010CB934700, 2013CB933900, 2014CB931800), the National Natural Science
   Foundation of China (21431006, 91022032, 91227103), the Chinese Academy
   of Sciences (KJZD-EW-M01-1), and the China Postdoctoral Science
   Foundation (2012M510160).
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NR 37
TC 40
Z9 40
U1 59
U2 273
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD OCT 20
PY 2014
VL 53
IS 43
BP 11552
EP 11556
DI 10.1002/anie.201407103
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA AR9CY
UT WOS:000343870400026
PM 25213751
ER

PT J
AU Gao, GX
   Wu, HB
   Lou, XW
AF Gao, Guoxin
   Wu, Hao Bin
   Lou, Xiong Wen (David)
TI Citrate-Assisted Growth of NiCo2O4 Nanosheets on Reduced Graphene Oxide
   for Highly Reversible Lithium Storage
SO ADVANCED ENERGY MATERIALS
LA English
DT Article
ID LI-ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; ANODE MATERIAL;
   ELECTRODE MATERIALS; FACILE SYNTHESIS; CATHODE MATERIAL; PERFORMANCE;
   SUPERCAPACITORS; CAPACITY; ARRAYS
AB Hybrid nanostructures based on graphene and transition metal oxides hold great promise as high-performance electrode materials for next-generation lithium-ion batteries. In this work, the rational design and fabrication of NiCo2O4 nanosheets supported on reduced graphene oxide (denoted as rGO/NiCo2O4) is presented as a novel anode material for highly efficient and reversible lithium storage. A solution method is applied to grow Ni-Co precursor nanosheets on rGO, in which the addition of trisodium citrate is found crucial to guide the formation of uniform Ni-Co precursor nanosheets. Subsequent thermal treatment results in formation of crystalline NiCo2O4 nanosheets on rGO without damaging the morphology. The interconnected NiCo2O4 nanosheets form hierarchically porous films on both sides of rGO. Such a hybrid nanostructure would effectively promote the charge transport and withstand volume variation upon prolonged charge/discharge cycling. As a result, the rGO/NiCo2O4 nanocomposite demonstrates high reversible capacities of 954.3 and 656.5 mAh g(-1) over 50 cycles at current densities of 200 and 500 mA g(-1) respectively, and remarkable capacity retention at increased current densities.
C1 [Gao, Guoxin; Wu, Hao Bin; Lou, Xiong Wen (David)] Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637459, Singapore.
   [Gao, Guoxin] Xi An Jiao Tong Univ, Dept Appl Chem, Sch Sci, Xian 710049, Peoples R China.
RP Lou, XW (reprint author), Nanyang Technol Univ, Sch Chem & Biomed Engn, 62 Nanyang Dr, Singapore 637459, Singapore.
EM xwlou@ntu.edu.sg
RI Wu, Haobin/D-1572-2014; Lou , Xiong Wen (David)/D-2648-2009
OI Wu, Haobin/0000-0002-0725-6442; 
CR Wang HW, 2011, J MATER CHEM, V21, P10504, DOI 10.1039/c1jm10758e
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NR 43
TC 40
Z9 40
U1 75
U2 254
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1614-6832
EI 1614-6840
J9 ADV ENERGY MATER
JI Adv. Energy Mater.
PD OCT 7
PY 2014
VL 4
IS 14
AR 1400422
DI 10.1002/aenm.201400422
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary; Physics, Applied; Physics, Condensed Matter
SC Chemistry; Energy & Fuels; Materials Science; Physics
GA AS6GX
UT WOS:000344363400011
ER

PT J
AU Zhao, CY
   Kong, JH
   Yao, XY
   Tang, XS
   Dong, YL
   Phua, SL
   Lu, XH
AF Zhao, Chenyang
   Kong, Junhua
   Yao, Xiayin
   Tang, Xiaosheng
   Dong, Yuliang
   Phua, Si Lei
   Lu, Xuehong
TI Thin MoS2 Nanoflakes Encapsulated in Carbon Nanofibers as
   High-Performance Anodes for Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE molybdenum disulfide (MoS2); hydrothermal; electrospinning; carbon
   nanofibers; lithium-ion battery; flexible anode
ID MOLYBDENUM-DISULFIDE MOS2; ENERGY-CONVERSION; ELECTROCHEMICAL
   PERFORMANCES; SECONDARY BATTERIES; HYDROGEN EVOLUTION; ASSISTED
   SYNTHESIS; STORAGE PROPERTIES; GRAPHENE; NANOSHEETS; SUPERCAPACITORS
AB In this work, highly flexible MoS2-based lithium-ion battery anodes composed of disordered thin MoS2 nanoflakes encapsulated in amorphous carbon nanofibrous mats were fabricated for the first time through hydrothermal synthesis of graphene-like MoS2, followed by electrospinning and carbonization. X-ray diffraction as well as scanning and transmission electron microscopic studies show that the as-synthesized MoS2 nanoflakes have a thickness of about 5 nm with an expanded interlayer spacing, and their structure and morphology are well-retained after the electrospinning and carbonization. At relatively low MoS2 contents, the nanoflakes are dispersed and well-embedded in the carbon nanofibers. Consequently, excellent electrochemical performance, including good cyclability and high rate capacity, was achieved with the hybrid nanofibrous mat at the MoS2 content of 47%, which may be attributed to the fine thickness and multilayered structure of the MoS2 sheets with an expanded interlayer spacing, the good charge conduction provided by the high-aspect-ratio carbon nanofibers, and the robustness of the nanofibrous mat.
C1 [Zhao, Chenyang; Yao, Xiayin; Dong, Yuliang; Phua, Si Lei; Lu, Xuehong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Kong, Junhua; Tang, Xiaosheng; Lu, Xuehong] Nanyang Technol Univ, Temasek Labs NTU, Singapore 637553, Singapore.
RP Lu, XH (reprint author), Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
EM ASXHLu@ntu.edu.sg
RI Lu, Xuehong/A-2232-2011; Yao, Xiayin/P-3690-2014
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NR 53
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Z9 40
U1 60
U2 274
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD MAY 14
PY 2014
VL 6
IS 9
BP 6392
EP 6398
DI 10.1021/am4058088
PG 7
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA AH4CV
UT WOS:000336075300049
PM 24701987
ER

PT J
AU Yang, Y
   Fan, XJ
   Casillas, G
   Peng, ZW
   Ruan, GD
   Wang, G
   Yacaman, MJ
   Tour, JM
AF Yang, Yang
   Fan, Xiujun
   Casillas, Gilberto
   Peng, Zhiwei
   Ruan, Gedeng
   Wang, Gunuk
   Yacaman, Miguel Jose
   Tour, James M.
TI Three-Dimensional Nanoporous Fe2O3/Fe3C-Graphene Heterogeneous Thin
   Films for Lithium-Ion Batteries
SO ACS NANO
LA English
DT Article
DE heterogeneous structure; nanoporous; lithium-ion battery; thin film;
   anode
ID ANODE MATERIAL; STORAGE PROPERTIES; SILICON NANOWIRES; HIGH-CAPACITY;
   SOLAR-CELLS; HIGH-POWER; TOP-DOWN; GRAPHENE; PERFORMANCE; ELECTRODES
AB Three-dimensional self-organized nanoporous thin films integrated into a heterogeneous Fe2O3/Fe3C-graphene structure were fabricated using chemical vapor deposition. Few-layer graphene coated on the nanoporous thin film was used as a conductive passivation layer, and Fe3C was introduced to improve capacity retention and stability of the nanoporous layer. A possible interfacial lithium storage effect was anticipated to provide additional charge storage in the electrode. These nanoporous layers, when used as an anode in lithium-ion batteries, deliver greatly enhanced cyclability and rate capacity compared with pristine Fe2O3: a specific capacity of 356 mu Ah cm(-2) mu m(-1) (3560 mAh cm(-3) or similar to 1118 mAh g(-1)) obtained at a discharge current density of 50 mu A cm(-2) (similar to 0.17 C) with 88% retention after 100 cycles and 165 mu Ah cm(-2) mu m(-1) (1650 mAh cm(-3) or similar to 518 mAh g(-1)) obtained at a discharge current density of 1000 mu A cm(-2) (similar to 6.6 C) for 1000 cycles were achieved. Meanwhile an energy density of 294 mu Wh cm(-2) mu m(-1) (2.94 Wh cm(-3) or similar to 924 Wh kg(-1)) and power density of 584 mu W cm(-2) mu m(-1) (5.84 W cm(-3) or similar to 1834 W kg(-1)) were also obtained, which may make these thin film anodes promising as a power supply for micro- or even nanosized portable electronic devices.
C1 [Yang, Yang; Fan, Xiujun; Peng, Zhiwei; Ruan, Gedeng; Wang, Gunuk; Tour, James M.] Rice Univ, Dept Chem, Houston, TX 77005 USA.
   [Yang, Yang; Fan, Xiujun; Wang, Gunuk; Tour, James M.] Rice Univ, Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA.
   [Tour, James M.] Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA.
   [Casillas, Gilberto; Yacaman, Miguel Jose] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA.
   [Fan, Xiujun] Beijing Univ Technol, Coll Elect Informat & Control Engn, Beijing 100124, Peoples R China.
RP Tour, JM (reprint author), Rice Univ, Dept Chem, 6100 Main St, Houston, TX 77005 USA.
EM tour@rice.edu
RI Ruan, Gedeng/G-8225-2014; jose yacaman, miguel/B-5622-2009
OI Ruan, Gedeng/0000-0002-7530-8013; 
FU Smalley Institute for Nanoscale Science and Technology; ONR MURI Program
   [00006766, N00014-09-1-1066]; AFOSR MURI Program [FA9550-12-1-0035];
   AFOSR [FA9550-09-1-0581]; National Center for Research Resources [5
   G12RR013646-12]; NSF-PREM [DMR 0934218]; National Institute on Minority
   Health and Health Disparities from the National Institutes of Health
   [G12MD007591]; Chinese Scholarship Council
FX We thank the Peter M. and Ruth L Nicholas Post-Doctoral Fellowship of
   the Smalley Institute for Nanoscale Science and Technology for financial
   support (Y.Y.). Additional funding was provided by the ONR MURI Program
   (00006766, N00014-09-1-1066), the AFOSR MURI Program (FA9550-12-1-0035),
   AFOSR (FA9550-09-1-0581), the National Center for Research Resources (5
   G12RR013646-12), NSF-PREM (DMR 0934218), and the National Institute on
   Minority Health and Health Disparities (G12MD007591) from the National
   Institutes of Health. Support of the Chinese Scholarship Council (X.F.)
   and helpful discussions with Prof. Xio Guo, Beijing University of
   Technology.
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NR 44
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Z9 40
U1 54
U2 262
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD APR
PY 2014
VL 8
IS 4
BP 3939
EP 3946
DI 10.1021/nn500865d
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AF8UH
UT WOS:000334990600092
PM 24669862
ER

PT J
AU Lian, PC
   Wang, JY
   Cai, DD
   Ding, LX
   Jia, QM
   Wang, HH
AF Lian, Peichao
   Wang, Jingyi
   Cai, Dandan
   Ding, Liangxin
   Jia, Qingming
   Wang, Haihui
TI Porous SnO2@C/graphene nanocomposite with 3D carbon conductive network
   as a superior anode material for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene sheets; SnO2; Carbon shell; Nanocomposite; Lithium-ion
   batteries
ID ONE-POT SYNTHESIS; HIGH-PERFORMANCE; REVERSIBLE CAPACITY; STORAGE
   DEVICES; NANOSTRUCTURED MATERIALS; CO3O4 NANOPARTICLES; CYCLIC
   PERFORMANCE; ENERGY-CONVERSION; GRAPHENE; COMPOSITE
AB Porous nano-sized SnO2@C/graphene electrode material with three-dimensional carbon conductive network was designed and prepared. The carbon shell was introduced to suppress the aggregation of nanoparticles and undesired reactions. The excellent electronic conductivity can be guaranteed by a 3D carbon conductive network consisted of graphene sheets and carbon shell. The porous structure can facilitate liquid electrolyte diffusion into the bulk materials. As a result, the as-prepared SnO2@C/graphene nanocomposite as an anode material for lithium-ion batteries exhibits high reversible specific capacity, outstanding cyclability and good rate capability. The first reversible specific capacity is as high as 1115 mAh g(-1) at a specific current of 100 mA g(-1). After 100 cycles at different specific currents from 100 to 1000 mA g(-1), the reversible specific capacity was still maintained at 1015 mAh g(-1) at the specific current of 100 mA g(-1). Even at the high specific current of 1000 mA g(-1), the reversible specific capacity is still as high as 499 mAh g(-1), higher than the theoretical specific capacity of the commonly used graphite anode material (372 mAh g(-1)). The results give the clear evidence that the electrochemical performance of graphene-based electrode materials can be improved by designing proper structure. The preparation approach of porous SnO2@C/graphene nanocomposite reported in this paper may also be applied to fabricate other porous metal oxide@C/graphene electrode materials for high performance lithium-ion batteries. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Lian, Peichao; Wang, Jingyi; Jia, Qingming] Kunming Univ Sci & Technol, Fac Chem Engn, Kunming 650500, Peoples R China.
   [Cai, Dandan; Ding, Liangxin; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
RP Lian, PC (reprint author), Kunming Univ Sci & Technol, Fac Chem Engn, Kunming 650500, Peoples R China.
EM lianpeichao@126.com; hhwang@scut.edu.cn
FU National Science Fund for Distinguished Young Scholars of China
   [21225625]; Scientific Research Start-up Fund of Kunming University of
   Science and Technology for Introducing Talents [KKSY201205133]; Pearl
   River Scholar Program of Guangdong Province, and Education Department
   Science Foundation of Yunnan Province [2012Y539]
FX This work was financially supported by the National Science Fund for
   Distinguished Young Scholars of China (No. 21225625), Scientific
   Research Start-up Fund of Kunming University of Science and Technology
   for Introducing Talents (KKSY201205133), Pearl River Scholar Program of
   Guangdong Province, and Education Department Science Foundation of
   Yunnan Province (Grant No. 2012Y539).
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NR 44
TC 40
Z9 41
U1 29
U2 191
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JAN 10
PY 2014
VL 116
BP 103
EP 110
DI 10.1016/j.electacta.2013.11.007
PG 8
WC Electrochemistry
SC Electrochemistry
GA AB0PK
UT WOS:000331494400014
ER

PT J
AU Chen, P
   Su, Y
   Liu, H
   Wang, Y
AF Chen, Peng
   Su, Yun
   Liu, Hong
   Wang, Yong
TI Interconnected Tin Disulfide Nanosheets Grown on Graphene for LiIon
   Storage and Photocatalytic Applications
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE reduced graphene oxide; SnS2 nanosheet; sheet-on-sheet; lithium ion
   batteries; photocatalyst
ID LITHIUM-ION BATTERIES; HIGH-PERFORMANCE ANODE; VISIBLE-LIGHT;
   HYDROTHERMAL SYNTHESIS; AQUEOUS CR(VI); NANOCOMPOSITE PHOTOCATALYST;
   SOLVOTHERMAL SYNTHESIS; FACILE SYNTHESIS; ENERGY-STORAGE; HIGH-CAPACITY
AB Reduced graphene oxide (RGO) nanosheet-supported SnS2 nanosheets are prepared by a one-step microwave-assisted technique. These SnS2 nanosheets are linked with each other and dispersed uniformly on RGO surface. The SnS2-RGO sheet-on-sheet nanostructure exhibits good electrochemical performances as an anode material for lithium ion batteries. It shows larger-than-theoretical reversible capacities at 0.1 C and excellent high-rate capability at 1 C and 5 C. The composite is also for the first time identified as an excellent visible light-driven catalyst of rhodamine B and phenol with high degradation efficiencies. The removal rates of rhodamine B and phenol are 100 and 83.2%, respectively, for the SnS2-RGO composite, whereas these values are only 64.8 and 51.5% for pristine SnS2 after the same irradiation times. The outstanding electrochemical or photocatalytic performances of the composite have been attributed to the complementary
C1 [Chen, Peng; Su, Yun; Liu, Hong; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shanghai 200444, Peoples R China.
RP Liu, H (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM liuhong@shu.edu.cn; yongwang@shu.edu.cn
RI WANG, Yong/B-1125-2012
FU National Natural Science Foundation of China [51271105]; Shanghai
   Municipal Government [1lYZ15, 11JC1403900, 11SG38, 12ZR1410300, S30109]
FX The authors gratefully acknowledge the financial support from the
   follow-up Program for Professor of Special Appointment (Eastern
   Scholar), National Natural Science Foundation of China (51271105), and
   Shanghai Municipal Government (1lYZ15, 11JC1403900, 11SG38, 12ZR1410300,
   S30109).
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NR 69
TC 40
Z9 40
U1 34
U2 152
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD NOV 27
PY 2013
VL 5
IS 22
BP 12073
EP 12082
DI 10.1021/am403905x
PG 10
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 263MI
UT WOS:000327812300080
PM 24156609
ER

PT J
AU Hu, YH
   Li, XF
   Wang, JJ
   Li, RY
   Sun, XL
AF Hu, Yuhai
   Li, Xifei
   Wang, Jiajun
   Li, Ruying
   Sun, Xueliang
TI Free-standing graphene-carbon nanotube hybrid papers used as current
   collector and binder free anodes for lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene; Graphene paper; Free standing; Anode; Lithium ion battery;
   Electrochemical energy storage
ID REVERSIBLE CAPACITY; ENERGY-STORAGE; IN-SITU; ELECTRODES; NANOSHEETS;
   STABILITY; SHEETS; OXIDE; FILM
AB Free-standing hybrid papers were fabricated by the vacuum-assisted filtration of graphene nanosheets (GNS) and carbon nanotubes (CNTs) both suspended in water, an approach that is environmentally benign. The CNTs are randomly dispersed between the GNS and hence, the hybrid papers exhibit high mechanical strength and flexibility even after being annealed at 800 degrees C. Electrochemical properties of the hybrid papers are strongly dependent on the CNT/GN ratios. Highest lithium ion storage capacities were obtained in the paper with a CNT/GN ratio of 2:1. The initial reversible specific capacities are similar to 375 mAh g(-1) at 100 mA g(-1). The capacities remain above 330 mAh g(-1) after 100 cycles, which are about 100 mAh g(-1) higher than those of the graphene paper with nearly the same mass. The improved capacities were attributed to the contribution of the CNTs, which prevent restacking of the GNS, increase cross-plane electric conductivity of the paper and simultaneously, store Li ions. These results suggest that graphene-CNT hybrid paper has a high potential to be used as collector and binder free anodes for lithium ion batteries. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Hu, Yuhai; Li, Xifei; Wang, Jiajun; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
EM xsun9@uwo.ca
RI Sun, Andy (Xueliang)/I-4535-2013; Li, Xifei/A-1966-2012; Sun,
   Xueliang/C-7257-2012; wang, jiajun/H-3315-2012
OI Li, Xifei/0000-0002-4828-4183; 
FU Natural Science and Engineering Research Council of Canada (NSERC);
   Canada Research Chair (CRC) Program; Canadian Foundation for Innovation
   (CFI); Ontario Research Fund (ORF); University of Western Ontario
FX This research was supported by the Natural Science and Engineering
   Research Council of Canada (NSERC), Canada Research Chair (CRC) Program,
   Canadian Foundation for Innovation (CFI), Ontario Research Fund (ORF),
   Early Researcher Award (ERA) and the University of Western Ontario.
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NR 35
TC 40
Z9 41
U1 37
U2 255
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 1
PY 2013
VL 237
BP 41
EP 46
DI 10.1016/j.jpowsour.2013.02.065
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 173NH
UT WOS:000321085700007
ER

PT J
AU Chen, DY
   Ji, G
   Ding, B
   Ma, Y
   Qu, BH
   Chen, WX
   Lee, JY
AF Chen, Dongyun
   Ji, Ge
   Ding, Bo
   Ma, Yue
   Qu, Baihua
   Chen, Weixiang
   Lee, Jim Yang
TI In situ nitrogenated graphene-few-layer WS2 composites for fast and
   reversible Li+ storage
SO NANOSCALE
LA English
DT Article
ID LITHIUM ION BATTERIES; METAL DICHALCOGENIDE NANOSHEETS; ORDERED
   MESOPOROUS MOS2; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE; TUNGSTEN
   DISULFIDE; CYCLIC PERFORMANCE; CAPACITY; OXIDE; NANOPARTICLES
AB Two-dimensional nanosheets can leverage on their open architecture to support facile insertion and removal of Li+ as lithium-ion battery electrode materials. In this study, two two-dimensional nanosheets with complementary functions, namely nitrogen-doped graphene and few-layer WS2, were integrated via a facile surfactant-assisted synthesis under hydrothermal conditions. The layer structure and morphology of the composites were confirmed by X-ray diffraction, scanning electron microscopy and high-resolution transmission microscopy. The effects of surfactant amount on the WS2 layer number were investigated and the performance of the layered composites as high energy density lithium-ion battery anodes was evaluated. The composite formed with a surfactant : tungsten precursor ratio of 1 : 1 delivered the best cyclability (average of only 0.08% capacity fade per cycle for 100 cycles) and good rate performance (80% capacity retention with a 50-fold increase in current density from 100 mA g(-1) to 5000 mA g(-1)), and may find uses in power-oriented applications.
C1 [Chen, Dongyun; Ji, Ge; Ding, Bo; Ma, Yue; Qu, Baihua; Lee, Jim Yang] Natl Univ Singapore, Dept Chem & Biomol Engn, Singapore 119260, Singapore.
   [Chen, Weixiang] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China.
RP Lee, JY (reprint author), Natl Univ Singapore, Dept Chem & Biomol Engn, 10 Kent Ridge Crescent, Singapore 119260, Singapore.
EM cheleejy@nus.edu.sg
RI Qu, Baihua/H-9594-2012; Ma, Yue/B-9975-2014; LEE, Jim Yang/E-5904-2010
FU A*STAR [1220203049 (R279-000-370-305)]; International Science and
   Technology Cooperation Program of China [2012DFG42100]; Natural Science
   Foundation of China [21173190]; Doctoral Program of Higher Education of
   China [2011010113003]; International Science and Technology Cooperation
   Program of Zhejiang Province [2013C34G2010042]
FX This work was financially supported by A*STAR Project 1220203049
   (R279-000-370-305), the International Science and Technology Cooperation
   Program of China (2012DFG42100), the Natural Science Foundation of China
   (21173190), the Doctoral Program of Higher Education of China
   (2011010113003) and the International Science and Technology Cooperation
   Program of Zhejiang Province (2013C34G2010042).
CR Sun YQ, 2011, ENERG ENVIRON SCI, V4, P1113, DOI 10.1039/c0ee00683a
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NR 38
TC 40
Z9 40
U1 24
U2 212
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 17
BP 7890
EP 7896
DI 10.1039/c3nr02920d
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 198YA
UT WOS:000322958800030
PM 23851576
ER

PT J
AU Wang, CD
   Chui, YS
   Ma, RG
   Wong, TL
   Ren, JG
   Wu, QH
   Chen, XF
   Zhang, WJ
AF Wang, Chundong
   Chui, Ying-San
   Ma, Ruguang
   Wong, Tailun
   Ren, Jian-Guo
   Wu, Qi-Hui
   Chen, Xianfeng
   Zhang, Wenjun
TI A three-dimensional graphene scaffold supported thin film silicon anode
   for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-CAPACITY; ELECTROCHEMICAL PERFORMANCE; NANOSTRUCTURED MATERIALS;
   ENERGY-CONVERSION; SI NANOPARTICLES; STORAGE DEVICES; ALLOY ANODES; LI;
   NANOWIRES; COMPOSITE
AB Three-dimensional (3D) silicon (Si) thin films supported on a graphene scaffold were prepared as an anode electrode for lithium-ion batteries. The as-prepared Si anode exhibited a gravimetric capacity as high as 1560 mA h g(-1) at a current density of 797 mA g(-1) and a capacity retention of 84% after 500 cycles relative to the capacity value in the 50th cycle. Meanwhile, specific capacities of 1083 and 803 mA h g(-1) were demonstrated after 1200 cycles at 2390 mA g(-1) and 7170 mA g(-1), respectively. The high specific capacity and excellent cyclability and rate performance could be ascribed to the highly porous 3D architecture of the graphene scaffold, which possesses good electrical conductivity and the feature of mechanical flexibility. The results presented here pave a new way for synthesis of Si-graphene hybrid materials using microwave plasma-enhanced chemical vapor deposition as robust and scalable Si-based anodes for lithium ion batteries.
C1 [Wang, Chundong; Chui, Ying-San; Wong, Tailun; Ren, Jian-Guo; Wu, Qi-Hui; Chen, Xianfeng; Zhang, Wenjun] City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
   [Wang, Chundong; Chui, Ying-San; Ma, Ruguang; Wong, Tailun; Ren, Jian-Guo; Wu, Qi-Hui; Chen, Xianfeng; Zhang, Wenjun] City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China.
RP Ren, JG (reprint author), City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
EM renjg123@gmail.com; apwjzh@cityu.edu.hk
RI Wang, C.D. /D-5912-2012; Zhang, WJ/C-6995-2012; Chen,
   Xianfeng/D-1709-2010
OI Chen, Xianfeng/0000-0002-3189-2756
FU National Natural Science Foundation of China (NCFC) [61176007]; Research
   Grants Council of the Hong Kong Special Administrative Region, China
   [CityU 102010]
FX This work was supported by the National Natural Science Foundation of
   China (NCFC Grant 61176007) and the Research Grants Council of the Hong
   Kong Special Administrative Region, China (Project no. CityU 102010).
CR Zhou XS, 2012, ADV ENERGY MATER, V2, P1086, DOI 10.1002/aenm.201200158
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NR 57
TC 40
Z9 40
U1 18
U2 133
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 35
BP 10092
EP 10098
DI 10.1039/c3ta11740e
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 201IA
UT WOS:000323132700003
ER

PT J
AU Xie, J
   Liu, SY
   Cao, GS
   Zhu, TJ
   Zhao, XB
AF Xie, Jian
   Liu, Shuangyu
   Cao, Gaoshao
   Zhu, Tiejun
   Zhao, Xinbing
TI Self-assembly of CoS2/graphene nanoarchitecture by a facile one-pot
   route and its improved electrochemical Li-storage properties
SO NANO ENERGY
LA English
DT Article
DE Cobalt sulfide; Graphene; Nanoarchitecture; Electrochemical property; Li
   battery
ID LITHIUM-ION BATTERIES; REDUCED GRAPHENE OXIDE; REVERSIBLE CAPACITY;
   ELECTRODE MATERIALS; COBALT SULFIDE; GRAPHITE OXIDE; PERFORMANCE; ANODE;
   NANOSHEETS; REDUCTION
AB A CoS2/graphene nanoarchitecture was synthesized by a facile one-step hydrothermal route using graphite oxide, thioacetamide, and CoCl2 center dot 6H(2)O as the starting materials. The growth of CoS2 and the reduction of the graphite oxide occur simultaneously. CoS2 nanocrystals with a size of 100-150 nm are uniformly anchored on the both sides of the graphene nanosheets, forming a unique CoS2/graphene hybrid nanostructure. The electrochemical tests showed that the nanocomposite exhibits obviously enhanced Li-storage properties compared with bare CoS2. The improvement in electrochemical properties could be attributed to the formation of two-dimensional conductive networks, homogeneous dispersion and immobilization of CoS2 nanoparticles, and the enhanced wetting of active material with the electrolyte by in situ introduced graphene nanosheets. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Zhao, Xinbing] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
   Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
RP Zhao, XB (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
EM zhaoxb@zju.edu.cn
FU National Natural Science Foundation of China [51101139]; Ph.D. Programs
   Foundation of Ministry of Education of China [20100101120024];
   Foundation of Education Office of Zhejiang Province [Y201016484];
   Qianjiang Talents Project of Science Technology Department of Zhejiang
   Province [2011R10021]; Key Science and Technology Innovation Team of
   Zhejiang Province [2010R50013]
FX We appreciate the support from the National Natural Science Foundation
   of China (No. 51101139), the Ph.D. Programs Foundation of Ministry of
   Education of China (No. 20100101120024), the Foundation of Education
   Office of Zhejiang Province (No. Y201016484), the Qianjiang Talents
   Project of Science Technology Department of Zhejiang Province (No.
   2011R10021), Key Science and Technology Innovation Team of Zhejiang
   Province under Grant number 2010R50013.
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   Thackeray M.M., 1982, MAT RES B, V1, P405
NR 45
TC 40
Z9 40
U1 45
U2 251
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD JAN
PY 2013
VL 2
IS 1
BP 49
EP 56
DI 10.1016/j.nanoen.2012.07.010
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 132EK
UT WOS:000318050500009
ER

PT J
AU Zhang, M
   Lei, DN
   Yu, XZ
   Chen, LB
   Li, QH
   Wang, YG
   Wang, TH
   Cao, GZ
AF Zhang, Ming
   Lei, Danni
   Yu, Xinzhi
   Chen, Libao
   Li, Qiuhong
   Wang, Yanguo
   Wang, Taihong
   Cao, Guozhong
TI Graphene oxide oxidizes stannous ions to synthesize tin sulfide-graphene
   nanocomposites with small crystal size for high performance lithium ion
   batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID ELECTROCHEMICAL PERFORMANCE; ANODE MATERIAL; SNS2; STORAGE; HYBRID;
   SULFUR; CARBON; NANOSTRUCTURES; DEPOSITION; EFFICIENCY
AB This study reports a novel strategy of preparing graphene composites by employing graphene oxide as precursor and oxidizer. It is demonstrated that graphene oxide can oxidize stannous ions to form SnS2 and is simultaneously reduced to graphene, directly resulting in the formation of SnSx-graphene (1 < x < 2) nanocomposites. The particle size of SnSx in the nanocomposites is tailored to be about 5 nm, which is much smaller than that obtained in a previous study. As anodic materials for lithium ion batteries, SnSx-graphene nanocomposites retain a discharge capacity of 860 mA h g(-1) after 150 cycles at a charge-discharge rate of 0.2 C, higher than the theoretical capacities of SnS2 (645 mA h g(-1)) and SnS (782 mA h g(-1)) based on the traditional mechanism. A possible new mechanism, that Li2S arising from tin sulfide in the first discharge cycle could be reversibly decomposed at a low potential to storage lithium, is proposed based on experimental results to explain the excellent properties of SnSx-graphene nanocomposites.
C1 [Zhang, Ming; Lei, Danni; Yu, Xinzhi; Chen, Libao; Li, Qiuhong; Wang, Yanguo; Wang, Taihong] Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
   [Zhang, Ming; Lei, Danni; Yu, Xinzhi; Chen, Libao; Li, Qiuhong; Wang, Yanguo; Wang, Taihong] Hunan Univ, State Key Lab Chemol Biosensing & Chemometr, Changsha 410082, Hunan, Peoples R China.
   [Zhang, Ming; Cao, Guozhong] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.
RP Wang, TH (reprint author), Hunan Univ, Key Lab Micronano Optoelect Devices, Minist Educ, Changsha 410082, Hunan, Peoples R China.
EM thwang@iphy.ac.cn; gzcao@u.washington.edu
RI Cao, Guozhong/E-4799-2011; Wang, Taihong/K-8968-2012; Zhang,
   Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU '973' National Key Basic Research Program of China [2007CB310500];
   National Natural Science Foundation of China [21003041, 21103046]; Hunan
   Provincial Natural Science Foundation of China [10JJ1011, 11JJ7004];
   China Scholarship Council; National Science Foundation [CMMI-1030048]
FX This work was partly supported by the '973' National Key Basic Research
   Program of China (2007CB310500), the National Natural Science Foundation
   of China (21003041, 21103046), the Hunan Provincial Natural Science
   Foundation of China (10JJ1011 and 11JJ7004) and the China Scholarship
   Council. This research has been also financially supported in part by
   the National Science Foundation (CMMI-1030048).
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NR 55
TC 40
Z9 41
U1 32
U2 181
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PD NOV 21
PY 2012
VL 22
IS 43
BP 23091
EP 23097
DI 10.1039/c2jm34864k
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 032LX
UT WOS:000310721400037
ER

PT J
AU Chen, SQ
   Yeoh, WK
   Liu, Q
   Wang, GX
AF Chen, Shuangqiang
   Yeoh, Waikong
   Liu, Qi
   Wang, Guoxiu
TI Chemical-free synthesis of graphene-carbon nanotube hybrid materials for
   reversible lithium storage in lithium-ion batteries
SO CARBON
LA English
DT Article
ID ORGANIC-SOLVENT DISPERSIONS; RAMAN-SPECTROSCOPY; WATER; FILMS; OXIDE;
   ORIENTATION; SILYLATION; MEMBRANES; RELEASE; ROUTE
AB Graphene-carbon nanotube hybrid materials were successfully prepared through the pi-pi interaction without using any chemical reagent. We found that the ratio between carbon nanotube and graphene had critical influences on the state in aqueous solution and morphology of hybrid materials. Field emission scanning electron microscope and transmission electron microscope analysis confirmed that graphene nanosheets wrap around individual carbon nanotubes and form a homogeneous three-dimensional hybrid nano-structure. When applied as an anode material in lithium ion batteries, graphene-carbon nanotube hybrid materials demonstrated a high reversible lithium storage capacity, a high Coulombic efficiency and an excellent cyclability. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Chen, Shuangqiang; Wang, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
   [Yeoh, Waikong] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia.
   [Liu, Qi] Changzhou Univ, Sch Petrochem Engn, Changzhou 213164, Jiangsu, Peoples R China.
RP Wang, GX (reprint author), Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
EM Guoxiu.Wang@uts.edu.au
RI Chen, Shuangqiang/F-5289-2013
FU Australian Research Council (ARC) [DP1093855]; International Science and
   Technology Cooperation Project of Changzhou City [CZ20110023]; Chinese
   Scholarship Council (CSC)
FX This project is financially supported by the Australian Research Council
   (ARC) through the ARC Discovery Project (DP1093855) and the
   International Science and Technology Cooperation Project of Changzhou
   City (CZ20110023). The author S. Q. Chen gratefully acknowledges the
   support from the Chinese Scholarship Council (CSC).
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NR 50
TC 40
Z9 41
U1 7
U2 101
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD OCT
PY 2012
VL 50
IS 12
BP 4557
EP 4565
DI 10.1016/j.carbon.2012.05.040
PG 9
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 984QQ
UT WOS:000307206600028
ER

PT J
AU Fu, YS
   Chen, Q
   He, MY
   Wan, YH
   Sun, XQ
   Xia, H
   Wang, X
AF Fu, Yongsheng
   Chen, Qun
   He, Mingyang
   Wan, Yunhai
   Sun, Xiaoqiang
   Xia, Hui
   Wang, Xin
TI Copper Ferrite-Graphene Hybrid: A Multifunctional Heteroarchitecture for
   Photocatalysis and Energy Storage
SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
LA English
DT Article
ID LITHIUM-ION BATTERIES; VISIBLE-LIGHT IRRADIATION; EXFOLIATED GRAPHITE
   OXIDE; HIGH-PERFORMANCE; ANODE MATERIAL; REVERSIBLE CAPACITY; CO3O4
   NANOPARTICLES; COMPOSITE; DEGRADATION; REDUCTION
AB A straightforward strategy is designed for the fabrication of CuFe2O4-graphene heteroarchitecture via a one-step hydrothermal route to allow multifunctional properties, i.e., magnetic cycling, high photocatalytic activity under visible light irradiation, and excellent electrochemical behaviors for use as the anode in lithium-ion batteries (LIBs). Transmission electron microscopy (TEM) observations indicate that graphene sheets are exfoliated and decorated with hexagonal CuFe2O4 nanoflakes. The photocatalytic activity measurements demonstrate that the combination of CuFe2O4 and graphene results in a dramatic conversion of the inert CuFe2O4 into a highly active catalyst for the degradation of methylene blue (MB) under visible light irradiation. CuFe2O4 nanoparticles themselves have excellent magnetic properties, which makes the CuFe2O4-graphene heteroarchitecture magnetically recyclable in a suspension system. It should be pointed out that the CuFe2O4-graphene (with 25 wt % graphene) heteroarchitecture as anode material for LIBs shows a high specific reversible capacity up to 1165 mAh g(-1) with good cycling stability and rate capability. The superior photocatalytic activity and electrochemical performance of the CuFe2O4-graphene nanocomposite can be attributed to its unique heteroarchitechture, which provides the remarkable synergistic effect between the CuFe2O4 nanoflakes and the graphene sheets.
C1 [Fu, Yongsheng; Chen, Qun; He, Mingyang; Sun, Xiaoqiang] Changzhou Univ, Key Lab Fine Petrochem Engn, Changzhou 213164, Peoples R China.
   [Fu, Yongsheng; Wang, Xin] Nanjing Univ Sci & Technol, Minist Educ, Key Lab Soft Chem & Funct Mat, Nanjing 210094, Jiangsu, Peoples R China.
   [Wan, Yunhai; Xia, Hui] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China.
RP Sun, XQ (reprint author), Changzhou Univ, Key Lab Fine Petrochem Engn, Changzhou 213164, Peoples R China.
EM xqsun@cczu.edu.cn; jasonxiahui@gmail.com; wxin@public1.ptt.js.cn
OI Xia, Hui/0000-0002-2517-2410
FU NNSF of China [21171094, 51102134]; DFSR [A2620110010]; PAPD of Jiangsu;
   NUST Research Funding [2011PYXM03, 2011ZDJH21]; Department of Education
   of Jiangsu Province [CXZZ11_0245]
FX This investigation was supported by NNSF of China (Nos. 21171094,
   51102134), DFSR (No. A2620110010), PAPD of Jiangsu, NUST Research
   Funding (2011PYXM03, 2011ZDJH21), and the Department of Education of
   Jiangsu Province (CXZZ11_0245).
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NR 59
TC 40
Z9 41
U1 13
U2 185
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0888-5885
J9 IND ENG CHEM RES
JI Ind. Eng. Chem. Res.
PD SEP 12
PY 2012
VL 51
IS 36
BP 11700
EP 11709
DI 10.1021/ie301347j
PG 10
WC Engineering, Chemical
SC Engineering
GA 002YP
UT WOS:000308575300016
ER

PT J
AU Prakash, A
   Chandra, S
   Bahadur, D
AF Prakash, Anand
   Chandra, Sudeshna
   Bahadur, D.
TI Structural, magnetic, and textural properties of iron oxide-reduced
   graphene oxide hybrids and their use for the electrochemical detection
   of chromium
SO CARBON
LA English
DT Article
ID LITHIUM-ION BATTERIES; CORE-SHELL NANOPARTICLES; GRAPHITE OXIDE; ANODE
   MATERIAL; THERAPEUTIC APPLICATIONS; SHEETS; TRANSPARENT; REDUCTION;
   CAPACITY; STORAGE
AB Superparamagnetic Fe3O4 nanoparticles were anchored on reduced graphene oxide (RGO) nanosheets by co-precipitation of iron salts in the presence of different amounts of graphene oxide (GO). A pH dependent zeta potential and good aqueous dispersions were observed for the three hybrids of Fe3O4 and RGO. The structure, morphology and microstructure of the hybrids were examined by X-ray diffraction, transmission electron microscopy (TEM), Fourier transform infrared spectroscopy, Raman and X-ray photoelectron spectroscopy. TEM images reveal lattice fringes (d(311) = 0.26 nm) of Fe3O4 nanoparticles with clear stacked layers of RGO nanosheets. The textural properties including the pore size distribution and loading of Fe3O4 nanoparticles to form Fe3O4-RGO hybrids have been controlled by changing the concentration of GO. An observed maximum (similar to 10 nm) in pore size distribution for the sample with 0.25 mg ml(-1) of GO is different from that prepared using 1.0 mg ml(-1) GO. The superparamagnetic behavior is also lost in the latter and it exhibits a ferrimagnetic nature. The electrochemical behavior of the hybrids towards chromium ion was assessed and a novel electrode system using cyclic voltammetry for the preparation of an electrochemical sensor platform is proposed. The textural properties seem to influence the electrochemical and magnetic behavior of the hybrids. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Prakash, Anand; Chandra, Sudeshna; Bahadur, D.] Indian Inst Technol, Dept Met Engn & Mat Sci, Bombay 400076, Maharashtra, India.
RP Bahadur, D (reprint author), Indian Inst Technol, Dept Met Engn & Mat Sci, Bombay 400076, Maharashtra, India.
EM dhirenb@iitb.ac.in
FU Department of Science and Technology (DST); Department of Information
   Technology (DIT), Government of India
FX Financial supports from Department of Science and Technology (DST) and
   Department of Information Technology (DIT), Government of India are
   gratefully acknowledged. The authors are thankful to the Centre for
   Research in Nanotechnology & Science (CRNTS) for TEM and Raman
   facilities.
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NR 39
TC 40
Z9 41
U1 9
U2 138
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD SEP
PY 2012
VL 50
IS 11
BP 4209
EP 4219
DI 10.1016/j.carbon.2012.05.002
PG 11
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 979MM
UT WOS:000306824100028
ER

PT J
AU Xing, LL
   Cui, CX
   Ma, CH
   Xue, XY
AF Xing, Lili
   Cui, Chunxiao
   Ma, Chunhua
   Xue, Xinyu
TI Facile synthesis of alpha-MnO2/graphene nanocomposites and their high
   performance as lithium-ion battery anode
SO MATERIALS LETTERS
LA English
DT Article
DE Carbon materials; Nanocomposites; Energy storage and conversion
ID REVERSIBLE CAPACITY; CYCLIC PERFORMANCE; GRAPHENE; STORAGE; ELECTRODES;
   MNO2; NANOSHEETS
AB alpha-MnO2/graphene nanocomposites are synthesized via a facile wet-chemical route, and alpha-MnO2 nanosheets are uniformly distributed on the surface of graphene. Their high performance as lithium ion battery anodes is obtained. Their reversible capacity at C/10 rate is up to 726.5 mA h/g, and maintains up to 635.5 mA h/g after 30 cycles. Such a performance can be partly attributed to high electron conductivity, excellent flexibility and high specific surface area of graphene. Also, alpha-MnO2 nanostructures can play a role in preventing the pile of graphene nanosheets with the loss of their active surface area. The present results indicate that alpha-MnO2/graphene nanocomposites have potential applications in lithium-ion battery anodes. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Xing, Lili; Cui, Chunxiao; Ma, Chunhua; Xue, Xinyu] Northeastern Univ, Coll Sci, Shenyang 110004, Peoples R China.
RP Xue, XY (reprint author), Northeastern Univ, Coll Sci, Shenyang 110004, Peoples R China.
EM xuexinyu@mail.neu.edu.cn
RI Xue, Xinyu/N-7444-2014
FU Fundamental Research Funds for the Central Universities [N090405017,
   N100405109]; Liaoning Natural Science Foundation [20091027]; Specialized
   Research Fund for the Doctoral Program of Higher Education of China
   [20090042120025]
FX This work was partly supported from the Fundamental Research Funds for
   the Central Universities (N090405017, N100405109), Liaoning Natural
   Science Foundation (20091027), and Specialized Research Fund for the
   Doctoral Program of Higher Education of China (20090042120025).
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NR 22
TC 40
Z9 44
U1 10
U2 95
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0167-577X
J9 MATER LETT
JI Mater. Lett.
PD JUL 31
PY 2011
VL 65
IS 14
BP 2104
EP 2106
DI 10.1016/j.matlet.2011.04.093
PG 3
WC Materials Science, Multidisciplinary; Physics, Applied
SC Materials Science; Physics
GA 788KQ
UT WOS:000292444200005
ER

PT J
AU Yin, PT
   Shah, S
   Chhowalla, M
   Lee, KB
AF Yin, Perry T.
   Shah, Shreyas
   Chhowalla, Manish
   Lee, Ki-Bum
TI Design, Synthesis, and Characterization of Graphene-Nanoparticle Hybrid
   Materials for Bioapplications
SO CHEMICAL REVIEWS
LA English
DT Review
ID ENHANCED RAMAN-SCATTERING; STEM-CELL DIFFERENTIATION;
   FIELD-EFFECT-TRANSISTOR; LITHIUM ION BATTERIES; UP-CONVERSION
   NANOPARTICLES; RESONANCE ENERGY-TRANSFER; IN-SITU SYNTHESIS; PERFORMANCE
   ANODE MATERIALS; SURFACE-PLASMON RESONANCE; OXYGEN REDUCTION REACTION
C1 [Yin, Perry T.; Lee, Ki-Bum] Rutgers State Univ, Dept Biomed Engn, Piscataway, NJ 08854 USA.
   [Shah, Shreyas; Lee, Ki-Bum] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA.
   [Chhowalla, Manish] Rutgers State Univ, Dept Mat Sci & Engn, Piscataway, NJ 08854 USA.
   [Lee, Ki-Bum] Rutgers State Univ, Inst Adv Mat Devices & Nanotechnol IAMDN, Piscataway, NJ 08854 USA.
RP Lee, KB (reprint author), Rutgers State Univ, Dept Biomed Engn, Piscataway, NJ 08854 USA.
EM kblee@rutgers.edu
RI Lee, Ki-Bum/G-7503-2015
FU NIH Director's Innovator Award [1DP20D006462-01]; National Institute of
   Neurological Disorders and Stroke (NINNDS) [1R21N5085S69-01]; NSF
   [9CHE-1429062, CBET-12365080]; N.J. Commission on Spinal Cord grant
   [CSCR13ERG005]; Busch Biomedical Grant Program; Collaborative Research
   Travel Grant (CRTG) from the Burroughs Wellcome Fund; American Cryostem
   Corp.; Rutgers Faculty Research Grant Program; NIH Biotechnology
   Training Grant
FX K.-B.L. acknowledges financial support from the NIH Director's Innovator
   Award [1DP20D006462-01], National Institute of Neurological Disorders
   and Stroke (NINNDS) [1R21N5085S69-01], the NSF 9CHE-1429062 and
   CBET-12365080, the N.J. Commission on Spinal Cord grant [CSCR13ERG005],
   the Busch Biomedical Grant Program, the Collaborative Research Travel
   Grant (CRTG) from the Burroughs Wellcome Fund, American Cryostem Corp.,
   and the Rutgers Faculty Research Grant Program. P.T.Y. would also like
   to acknowledge the NIH Biotechnology Training Grant. Finally, S.S.
   acknowledges NSF DGE 0801620, Integrative Graduate Education and
   Research Traineeship (IGERT) on the Integrated Science and Engineering
   of Stem Cells.
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NR 342
TC 39
Z9 39
U1 163
U2 329
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0009-2665
EI 1520-6890
J9 CHEM REV
JI Chem. Rev.
PD APR 8
PY 2015
VL 115
IS 7
BP 2483
EP 2531
DI 10.1021/cr500537t
PG 49
WC Chemistry, Multidisciplinary
SC Chemistry
GA CF7QE
UT WOS:000352750600001
PM 25692385
ER

PT J
AU Liu, Y
   Wang, W
   Gu, L
   Wang, YW
   Ying, YL
   Mao, YY
   Sun, LW
   Peng, XS
AF Liu, Yu
   Wang, Wei
   Gu, Lin
   Wang, Yewu
   Ying, Yulong
   Mao, Yiyin
   Sun, Luwei
   Peng, Xinsheng
TI Flexible CuO Nanosheets/Reduced-Graphene Oxide Composite Paper:
   Binder-Free Anode for High-Performance Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE flexible; CuO nanosheets/reduced-graphene oxide; binder-free anode;
   Li-ion battery
ID SUPERCAPACITOR ELECTRODES; ENHANCED CAPACITANCE; HYBRID; STORAGE;
   NANORODS; FILMS; NANOCOMPOSITE; STABILITY; NETWORKS; SHEETS
AB Flexible free-standing CuO nanosheets (NSs)/reduced graphene oxide (r-GO) hybrid lamellar paper was fabricated through vacuum filtration and hydrothermal reduction processes. A unique three-dimensional nanoporous network was achieved with CuO NSs homogeneously embedded within the r-GO layers. This hybrid lamellar composite paper was examined as a binder-free anode for lithium ion batteries, and demonstrated excellent cyclic retention with the specific capacity of 736.8 mA h g(-1) after 50 cycles. This is much higher than 219.1 mA h g(-1) of the pristine CuO NSs and 60.2 mA h g(-1) of r-GO film at the same current density of 67 mA g(-1). The high capacitance and excellent cycling performance were generated from the integrated nanoporous structure compose of CuO NSs spaced r-GO layers, which offered an efficient electrically conducting channels, favored electrolyte penetration, and buffered to the volume variations during the lithiation and delithiation process. These outstanding electrochemical capabilities of CuO NSs/r-GO paper holds great promise for flexible binder-free anode for lithium ion batteries.
C1 [Liu, Yu; Ying, Yulong; Mao, Yiyin; Sun, Luwei; Peng, Xinsheng] Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   [Wang, Wei; Gu, Lin; Wang, Yewu] Zhejiang Univ, Dept Phys, Hangzhou 310027, Peoples R China.
   [Wang, Wei; Gu, Lin; Wang, Yewu] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   [Peng, Xinsheng] Zhejiang Univ, Cyrus Tang Ctr Sensor Mat & Applicat, Hangzhou 310027, Peoples R China.
RP Peng, XS (reprint author), Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
EM pengxinsheng@zju.edu.cn
RI Peng, Xinsheng/A-1295-2009
FU National Natural Science Foundations of China [NSFC 21003105, 21271154,
   51272232]; Ministry of Education of China [20110101110028]; SRF for
   ROCS, SEM
FX This work was supported by the National Natural Science Foundations of
   China (NSFC 21003105, 21271154, 51272232), Doctoral Fund of Ministry of
   Education of China (20110101110028), and the project-sponsored by SRF
   for ROCS, SEM.
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NR 41
TC 39
Z9 39
U1 26
U2 244
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD OCT 9
PY 2013
VL 5
IS 19
BP 9850
EP 9855
DI 10.1021/am403136e
PG 6
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 243ZJ
UT WOS:000326356600083
PM 24010720
ER

PT J
AU Chen, Y
   Song, BH
   Lu, L
   Xue, JM
AF Chen, Yu
   Song, Bohang
   Lu, Li
   Xue, Junmin
TI Ultra-small Fe3O4 nanoparticle decorated graphene nanosheets with
   superior cyclic performance and rate capability
SO NANOSCALE
LA English
DT Article
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; REDUCED GRAPHENE; ENERGY-STORAGE;
   REVERSIBLE CAPACITY; ELECTRODE MATERIALS; CARBON; OXIDE; NANOCOMPOSITES;
   ARCHITECTURE
AB Advanced anode materials for next generation lithium ion batteries have attracted great interest due to the ever increasing demand for powerful, light-weight, and compact electrical devices. In this work, graphene nanosheets decorated with ultra-small Fe3O4 nanoparticles (USIO/G) were synthesized via a facile hydrothermal method. Compared with other reported Fe3O4-based anode composites, USIO/G demonstrated superior cyclic ability and excellent rate capability owing to its ultra-small size of active lithium storage sites, Fe3O4, with an average diameter less than 5 nm. Furthermore, graphene nanosheets played an important role in the overall electrochemical performance of the composite by enhancing the electrical conductivity, forming a flexible network, and providing extra lithium storage sites. The obtained composites were tested for electrochemical performance for a total number of 2120 cycles: a rate capability test with current densities ranged from 90 to 7200 mA g(-1) for 920 cycles, followed by a cycling test at 1800 mA g(-1) for 1200 cycles. For the rate capability test, steady reversible capacities were delivered under each current density with final reversible capacities of 1177, 1096, 833, 488, 242, and 146 mA h g(-1) at 90, 180, 900, 1800, 3600, and 7200 mA g(-1), respectively. The subsequent cyclic test demonstrated the superior cyclic stability of USIO/G and a reversible capacity of 437 mA h g(-1) at the 2120th cycle was delivered.
C1 [Chen, Yu; Xue, Junmin] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
   [Song, Bohang; Lu, Li] Natl Univ Singapore, Dept Mech Engn, Singapore 117576, Singapore.
RP Xue, JM (reprint author), Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
EM msexuejm@nus.edu.sg
RI Song, Bohang/F-8239-2016
OI Song, Bohang/0000-0002-6477-609X
CR Yu Y, 2013, ADV ENERGY MATER, V3, P281, DOI 10.1002/aenm.201200496
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NR 34
TC 39
Z9 39
U1 12
U2 127
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 15
BP 6797
EP 6803
DI 10.1039/c3nr01826a
PG 7
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 181NY
UT WOS:000321675600021
PM 23765405
ER

PT J
AU Kim, H
   Son, Y
   Park, C
   Cho, J
   Choi, HC
AF Kim, Hyungki
   Son, Yoonkook
   Park, Chibeom
   Cho, Jaephil
   Choi, Hee Cheul
TI Catalyst-free Direct Growth of a Single to a Few Layers of Graphene on a
   Germanium Nanowire for the Anode Material of a Lithium Battery
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE graphene; lithium ion battery; nanowires; surface chemistry
ID EPITAXIAL GRAPHENE; ION BATTERIES; GE NANOWIRES; CAPACITY; PERFORMANCE;
   GRAPHITE; CARBON; NANOSTRUCTURES; SPECTROSCOPY; TEMPERATURE
C1 [Kim, Hyungki; Park, Chibeom; Choi, Hee Cheul] Pohang Univ Sci & Technol, Dept Chem, Pohang 790784, South Korea.
   [Kim, Hyungki; Park, Chibeom; Choi, Hee Cheul] Pohang Univ Sci & Technol, Div Adv Mat Sci, Pohang 790784, South Korea.
   [Son, Yoonkook; Cho, Jaephil] UNIST, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea.
RP Cho, J (reprint author), UNIST, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea.
EM jpcho@unist.ac.kr; choihc@postech.edu
RI Cho, Jaephil/E-4265-2010; Choi, Hee Cheul/C-8208-2012
FU National Research Foundation of Korea (NRF); MEST [2012-003040,
   2012-053500, 2012-0009599, 2010-00285]; KOSEF through EPB center
   [2012-00000526]; ITRC by the MKE Korea [1415123286]
FX This work was supported by the National Research Foundation of Korea
   (NRF) grant funded by MEST (grant numbers 2012-003040, 2012-053500,
   2012-0009599, and 2010-00285), KOSEF through EPB center (grant number
   2012-00000526), and ITRC by the MKE Korea (grant number 1415123286). The
   authors thank Hyun Jin Park in NCNT for his technical assistance in TEM
   analysis.
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NR 33
TC 39
Z9 39
U1 15
U2 174
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PY 2013
VL 52
IS 23
BP 5997
EP 6001
DI 10.1002/anie.201300896
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA 155IY
UT WOS:000319742400016
PM 23616396
ER

PT J
AU Wang, L
   Li, YH
   Han, ZD
   Chen, L
   Qian, B
   Jiang, XF
   Pinto, J
   Yang, G
AF Wang, Lu
   Li, Yuhong
   Han, Zhida
   Chen, Lin
   Qian, Bin
   Jiang, Xuefan
   Pinto, Joao
   Yang, Gang
TI Composite structure and properties of Mn3O4/graphene oxide and
   Mn3O4/graphene
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID LITHIUM ION BATTERIES; EXFOLIATED GRAPHITE OXIDE; LOW-TEMPERATURE
   SYNTHESIS; CAPACITY ANODE MATERIAL; ELECTROCHEMICAL CAPACITORS;
   SUPERCAPACITOR ELECTRODES; AQUEOUS DISPERSIONS; CO3O4 NANOPARTICLES;
   MN3O4 NANOCRYSTALS; ASSISTED SYNTHESIS
AB Colloidal Mn3O4 nanocrystals supported by graphene oxide (GO) and reduced graphene oxide (RGO) (Mn3O4/GO and Mn3O4/RGO nanocomposites) have been fabricated through a facile synthetic route with ultrasonic-assisted in ethanol amine (ETA)-water system. It is proposed that in the formation mechanism of these intriguing nanocomposites, investigated by transmission electron microscopy (TEM), high resolution transmission electron microscopy (HRTEM), ultraviolet-visible absorption spectroscopy (UV-vis), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and Raman spectroscopy, the manganese ions are anchored on GO nanosheets (GOs) or enwrapped in curved RGO nanosheets (RGOs), followed by the nucleation and growth of Mn3O4 nanoparticles in ethanol ETA-water system via hydrolysis and oxidation, which in turn results in the exfoliation of GOs or RGOs. Based on the surface properties of GO and RGO, this work firstly explains how the synergetic compositing structure of Mn3O4/GO and Mn3O4/RGO nanocomposites plays a very important role in their properties for electrochemical capacitors (ECs) or lithium ion batteries (LIBs). The opinions we put forward may be readily extended to a strong basis for other classes of hybrids based on GOs or RGOs to make a wise choice between the ECs and LIBs applications.
C1 [Wang, Lu; Li, Yuhong; Han, Zhida; Qian, Bin; Jiang, Xuefan; Yang, Gang] Changshu Inst Technol, Dept Chem, Jiangsu Lab Adv Funct Mat, Changshu 215500, Peoples R China.
   [Wang, Lu; Chen, Lin] Jiangsu Univ Sci & Technol, Sch Mat Sci & Engn, Zhenjiang 212003, Peoples R China.
   [Pinto, Joao; Yang, Gang] Univ Aveiro, Dept Phys, P-3810193 Aveiro, Portugal.
   [Pinto, Joao; Yang, Gang] Univ Aveiro, I3N, P-3810193 Aveiro, Portugal.
RP Yang, G (reprint author), Changshu Inst Technol, Dept Chem, Jiangsu Lab Adv Funct Mat, Changshu 215500, Peoples R China.
EM gyang@cslg.edu.cn
RI Universidade Aveiro, Departamento Fisica/E-4128-2013; 
OI Pinto, Joao/0000-0002-6002-1060
FU NSF of Jiangsu Province of China [BK2010262]; NSF of Jiangsu Educational
   Department of China [10KJA480001]; NSF of China [51172032, 11174043]
FX The work was sponsored by the Qing Lan Project, NSF of Jiangsu Province
   of China (Grant no. BK2010262), NSF of Jiangsu Educational Department of
   China (Grant no. 10KJA480001), and NSF of China (Grant no. 51172032,
   11174043).
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NR 59
TC 39
Z9 40
U1 31
U2 183
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 29
BP 8385
EP 8397
DI 10.1039/c3ta10237h
PG 13
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 176NA
UT WOS:000321310200012
ER

PT J
AU Zhao, B
   Liu, P
   Zhuang, H
   Jiao, Z
   Fang, T
   Xu, WW
   Lu, B
   Jiang, Y
AF Zhao, Bing
   Liu, Peng
   Zhuang, Hua
   Jiao, Zheng
   Fang, Tao
   Xu, Weiwen
   Lu, Bo
   Jiang, Yong
TI Hierarchical self-assembly of microscale leaf-like CuO on graphene
   sheets for high-performance electrochemical capacitors
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID LITHIUM-ION BATTERIES; ELECTRODE MATERIALS; CYCLIC PERFORMANCE; STORAGE
   CAPACITY; ANODE MATERIAL; NANOSTRUCTURES; COMPOSITE; CU2O; NANOSHEETS;
   NANOWIRES
AB In this paper, a leaf-like porous CuO-graphene nanostructure is synthesized by a hydrothermal method. The as-prepared composite is characterized using XRD, Raman, SEM, TEM and nitrogen adsorption-desorption. The growth mechanism is discussed by monitoring the early growth stages. It is shown that the CuO nanoleaves are formed through oriented attachment of tiny Cu(OH)(2) nanowires. Electrochemical characterization demonstrates that the leaf-like CuO-graphene are capable of delivering specific capacitances of 331.9 and 305 F g(-1) at current densities of 0.6 and 2 A g(-1), respectively. A capacity retention of 95.1% can be maintained after 1000 continuous charge-discharge cycles, which may be attributed to the improvement of electrical contact by graphene and mechanical stability by the layer-by-layer structure. The method provides a facile and straightforward approach to synthesize CuO nanosheets on graphene and may be readily extended to the preparation of other classes of hybrids based on graphene sheets for technological applications.
C1 [Zhao, Bing; Liu, Peng; Zhuang, Hua; Jiao, Zheng; Fang, Tao; Xu, Weiwen; Jiang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
   [Lu, Bo] Shanghai Univ, Instrumental Anal & Res Ctr, Shanghai 200444, Peoples R China.
RP Zhao, B (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China.
EM jiangyong@shu.edu.cn
FU Innovation Program of Shanghai Municipal Education Commission [10YZ03,
   10YZ05, 12YZ013]; Science and Technology Committee [10DZ0500100,
   11DZ110020]; Natural Science Foundation of Shanghai [10ZR1411300];
   Shanghai Key Laboratory of Green Chemistry and Chemical Processes
   (ECNU); Laboratory of Chemical Engineering (ECUST); Shanghai Leading
   Academic Discipline Project [S30109]
FX This work is supported by the Innovation Program of Shanghai Municipal
   Education Commission (10YZ03, 10YZ05 and 12YZ013), Science and
   Technology Committee (10DZ0500100 and 11DZ110020), Natural Science
   Foundation of Shanghai (10ZR1411300), Shanghai Key Laboratory of Green
   Chemistry and Chemical Processes (ECNU), Laboratory of Chemical
   Engineering (ECUST), and Shanghai Leading Academic Discipline Project
   (S30109).
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NR 47
TC 39
Z9 39
U1 11
U2 185
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 2
BP 367
EP 373
DI 10.1039/c2ta00084a
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085RJ
UT WOS:000314631700034
ER

PT J
AU Zhu, XJ
   Hu, J
   Dai, HL
   Ding, L
   Jiang, L
AF Zhu, Xian-Jun
   Hu, Jing
   Dai, Huai-Li
   Ding, Lei
   Jiang, Li
TI Reduced graphene oxide and nanosheet-based nickel oxide microsphere
   composite as an anode material for lithium ion battery
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Reduced graphene oxide; Nickel oxide; Lithium ion batteries; Anode;
   Homogeneous coprecipitation
ID NIO; PERFORMANCE; ELECTRODES; REACTIVITY; CAPACITY; LI; NANOSTRUCTURES;
   NANOTUBES; HYBRID; CO3O4
AB Reduced graphene oxide and nickel oxide composite was prepared by homogeneous coprecipitation and subsequent annealing. Characterizations show that NiO particles have a nanosheet-based microsphere structure and anchor uniformly on the surface of reduced graphene oxide platelets. As an anode for Li ion batteries, the composite has 1641 mAh g(-1) and 1097 mAh g(-1) specific capacities for the first discharge and charge, respectively, higher than the theoretical capacity of NiO. It shows an excellent cycling performance with a discharge capacity of 1041 mAh g(-1) after 50 cycles at a current of 100 mA g(-1), and has a good rate capacity with 727 mAh g(-1) at a current of 1600 mA g(-1). The results show a synergistic effect of nanosheet-based NiO microspheres and reduced graphene oxide platelets in the composite for improved electrochemical performance. (C) 2011 Elsevier Ltd. All rights reserved.
C1 [Zhu, Xian-Jun; Hu, Jing; Dai, Huai-Li; Ding, Lei; Jiang, Li] Cent China Normal Univ, Coll Chem, Wuhan 430079, Hubei, Peoples R China.
RP Zhu, XJ (reprint author), Cent China Normal Univ, Coll Chem, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.
EM xianjunzhu@yahoo.com.cn
FU Natural Science Foundation of Hubei Province [2011CDB161]; Scientific
   Research Foundation for the Returned Overseas Chinese Scholars, State
   Education Ministry (SRF for ROCS, SEM)
FX This work was supported by the Natural Science Foundation of Hubei
   Province (No. 2011CDB161) and the Scientific Research Foundation for the
   Returned Overseas Chinese Scholars, State Education Ministry (SRF for
   ROCS, SEM).
CR Wang B, 2010, J MATER CHEM, V20, P10661, DOI 10.1039/c0jm01941k
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NR 33
TC 39
Z9 39
U1 4
U2 104
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD MAR 1
PY 2012
VL 64
BP 23
EP 28
DI 10.1016/j.electacta.2011.12.040
PG 6
WC Electrochemistry
SC Electrochemistry
GA 910DL
UT WOS:000301617300004
ER

PT J
AU Huang, XL
   Chai, J
   Jiang, T
   Wei, YJ
   Chen, G
   Liu, WQ
   Han, DX
   Niu, L
   Wang, LM
   Zhang, XB
AF Huang, Xiao-lei
   Chai, Jia
   Jiang, Tao
   Wei, Ying-Jin
   Chen, Gang
   Liu, Wan-qiang
   Han, Dongxue
   Niu, Li
   Wang, Limin
   Zhang, Xin-bo
TI Self-assembled large-area Co(OH)(2) nanosheets/ionic liquid modified
   graphene heterostructures toward enhanced energy storage
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIAL; COBALT HYDROXIDE;
   LI-ION; ELECTRODE MATERIALS; OXIDE SHEETS; FILMS; COMPOSITE;
   INTERCALATION; TRANSPARENT
AB Large-area Co(OH)(2) nanosheets have been successfully coated with ionic liquid modified graphene via a general strategy. The advantageous combination of graphene and the 2D structure of the Co(OH)(2) nanosheets endows the obtained heterostructures with a remarkable lithium-storage performance, including high reversible capacity and superior cyclic and rate performance.
C1 [Chai, Jia; Han, Dongxue; Niu, Li] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China.
   [Huang, Xiao-lei; Liu, Wan-qiang; Wang, Limin; Zhang, Xin-bo] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Jiang, Tao] FAW Grp Corp R&D Ctr, Changchun 130011, Peoples R China.
   [Wei, Ying-Jin; Chen, Gang] Jilin Univ, Coll Phys, Changchun 130012, Peoples R China.
   [Wei, Ying-Jin; Chen, Gang] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China.
   [Huang, Xiao-lei; Chai, Jia] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China.
RP Han, DX (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China.
EM dxhan@ciac.jl.cn; xbzhang@ciac.jl.cn
RI ZHANG, Xinbo/G-8698-2011; XiaoLei, Huang/I-3210-2014; 
OI ZHANG, Xinbo/0000-0002-5806-159X; XiaoLei, Huang/0000-0002-2211-4813;
   Wang, Limin/0000-0001-9618-9239
FU Chinese Academy of Sciences; National Natural Science Foundation of
   China [21101147]; Jilin Province Science and Technology Development
   Program [20100102, 20116008]
FX This work was financially supported by 100 Talents Programme of The
   Chinese Academy of Sciences, National Natural Science Foundation of
   China (Grant No. 21101147), and the Jilin Province Science and
   Technology Development Program (Grant No. 20100102 and 20116008).
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NR 50
TC 39
Z9 40
U1 8
U2 75
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 8
BP 3404
EP 3410
DI 10.1039/c2jm15377g
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 884HL
UT WOS:000299695400021
ER

PT J
AU Li, XF
   Yang, JL
   Hu, YH
   Wang, JJ
   Li, YL
   Cai, M
   Li, RY
   Sun, XL
AF Li, Xifei
   Yang, Jinli
   Hu, Yuhai
   Wang, Jiajun
   Li, Yongliang
   Cai, Mei
   Li, Ruying
   Sun, Xueliang
TI Novel approach toward a binder-free and current collector-free anode
   configuration: highly flexible nanoporous carbon nanotube electrodes
   with strong mechanical strength harvesting improved lithium storage
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LI-ION BATTERIES; HIGH-CAPACITY; RECHARGEABLE BATTERIES; CONTROLLED
   MORPHOLOGY; CYCLING PERFORMANCE; GRAPHENE NANOSHEETS; SILICON;
   DEPOSITION; CATHODE; FILMS
AB In this work, we developed a novel flexible nanoporous carbon nanotube film to use as a binder-free and current collector-free anode electrode for lithium ion batteries, providing a new approach to flexible energy devices. The proposed novel anode configuration shows better cycling performance and rate capability than the conventional electrode architecture. Moreover, this unique configuration exhibits good flexibility and robust mechanical strength, which has the potential to be applied to flexible lithium ion batteries. Our findings may provide a new anode configuration for lithium ion batteries with improved cycling stability and rate capability.
C1 [Li, Xifei; Yang, Jinli; Hu, Yuhai; Wang, Jiajun; Li, Yongliang; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
   [Cai, Mei] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Li, Xifei/A-1966-2012; Li, Yongliang/H-3179-2011; Sun, Andy
   (Xueliang)/I-4535-2013; Sun, Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; Li, Yongliang/0000-0002-5008-0868; 
FU Natural Science and Engineering Research Council of Canada (NSERC);
   General Motors of Canada; Canada Research Chair (CRC) Program; Canadian
   Foundation for Innovation (CFI); Ontario Research Fund (ORF); Early
   Researcher Award (ERA); University of Western Ontario
FX This research was supported by the Natural Science and Engineering
   Research Council of Canada (NSERC), General Motors of Canada, Canada
   Research Chair (CRC) Program, Canadian Foundation for Innovation (CFI),
   Ontario Research Fund (ORF), Early Researcher Award (ERA) and the
   University of Western Ontario. The authors are in debt to Dr. Yong Zhang
   for his kind help on drawing. X. Li is grateful to Springpower
   International, Inc. and the MITACS Elevate Strategic Fellowship Program.
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NR 59
TC 39
Z9 39
U1 12
U2 90
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 36
BP 18847
EP 18853
DI 10.1039/c2jm33297c
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 992PE
UT WOS:000307790300024
ER

PT J
AU Deng, D
   Lee, JY
AF Deng, Da
   Lee, Jim Yang
TI One-step synthesis of polycrystalline carbon nanofibers with periodic
   dome-shaped interiors and their reversible lithium-ion storage
   properties
SO CHEMISTRY OF MATERIALS
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; NONDESTRUCTIVE PURIFICATION; NANOTUBES;
   GROWTH; CVD; NANOPARTICLES; PYROLYSIS; BATTERIES; SYSTEM
AB Carbon nanofibers and carbon nanotubes continue to draw unwavering interest from industrial and academic communities because of their fascinating properties and their projected application values. This paper reports a one-step synthesis of high-purity carbon nanofibers with dome-shaped interiors by the noncatalytic thermal decomposition of acetylene over a copper surface at atmospheric pressure. These uniquely shaped carbon nanofibers were impurity free, and their dome-shaped interiors could be repeated with high periodicity throughout the length. In addition, Y-junction and forklike carbon nanofibers with the same internal structure were also formed as byproducts. The growth of these unique carbon nanomaterials could be rationalized by a mechanism based on the autocatalytic chemical vapor deposition of 3D graphene flakes. Preliminary electrochemical measurements indicated that the carbon nanofibers could be used as the active anode material for lithium-ion batteries, delivering good cyclability and a reversible capacity of similar to 260 mAh/g at the high specific current of 100 mA/g.
C1 Natl Univ Singapore, Fac Engn, Dept Chem & Biomol Engn, Singapore 119260, Singapore.
   Natl Univ Singapore, Singapore MIT Alliance, Singapore 117576, Singapore.
RP Lee, JY (reprint author), Natl Univ Singapore, Fac Engn, Dept Chem & Biomol Engn, Singapore 119260, Singapore.
EM cheleejy@nus.edu.sg
RI Deng, Da/B-1769-2012; LEE, Jim Yang/E-5904-2010
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NR 35
TC 39
Z9 40
U1 3
U2 23
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0897-4756
J9 CHEM MATER
JI Chem. Mat.
PD AUG 21
PY 2007
VL 19
IS 17
BP 4198
EP 4204
DI 10.1021/cm0707206
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 199JQ
UT WOS:000248692500016
ER

PT J
AU Zhou, GM
   Li, L
   Wang, DW
   Shan, XY
   Pei, SF
   Li, F
   Cheng, HM
AF Zhou, Guangmin
   Li, Lu
   Wang, Da-Wei
   Shan, Xu-yi
   Pei, Songfeng
   Li, Feng
   Cheng, Hui-Ming
TI A Flexible Sulfur-Graphene-Polypropylene Separator Integrated Electrode
   for Advanced Li-S Batteries
SO ADVANCED MATERIALS
LA English
DT Article
DE flexible; graphene; integrated electrode; lithium-sulfur batteries
ID LITHIUM-ION BATTERIES; ENERGY-STORAGE; CARBON; PERFORMANCE; CATHODES;
   PROGRESS; PROSPECTS; ANODES; PAPER
C1 [Zhou, Guangmin; Li, Lu; Shan, Xu-yi; Pei, Songfeng; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
   [Wang, Da-Wei] Univ New S Wales, UNSW Australia, Sch Chem Engn, Sydney, NSW 2052, Australia.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn; cheng@imr.ac.cn
RI Pei, Songfeng/E-5598-2010
FU MOST [2014CB932402]; National Science Foundation of China [51221264,
   51172239, 51102243, 51372253]
FX The authors acknowledge financial support from MOST (2014CB932402) and
   the National Science Foundation of China (Nos. 51221264, 51172239,
   51102243, and 51372253). The authors thank Ms. H. Wang for mechanical
   property measurements, Dr. Q. Z. Guo for interfacial adhesive force
   tests, Dr. S. G. Wang for XRM characterization, and Mr. R. S. Song and
   Mr. K. Huang for the synthesis of the G@PP separator.
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NR 45
TC 38
Z9 38
U1 139
U2 397
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
EI 1521-4095
J9 ADV MATER
JI Adv. Mater.
PD JAN 27
PY 2015
VL 27
IS 4
BP 641
EP 647
DI 10.1002/adma.201404210
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA CA2XQ
UT WOS:000348769700004
PM 25377991
ER

PT J
AU An, QY
   Lv, F
   Liu, QQ
   Han, CH
   Zhao, KN
   Sheng, JZ
   Wei, QL
   Yan, MY
   Mai, LQ
AF An, Qinyou
   Lv, Fan
   Liu, Qiuqi
   Han, Chunhua
   Zhao, Kangning
   Sheng, Jinzhi
   Wei, Qiulong
   Yan, Mengyu
   Mai, Liqiang
TI Amorphous Vanadium Oxide Matrixes Supporting Hierarchical Porous
   Fe3O4/Graphene Nanowires as a High-Rate Lithium Storage Anode
SO NANO LETTERS
LA English
DT Article
DE Iron oxides; vanadium oxides; graphene; hierarchical porous nanowires;
   lithium ion battery
ID ION BATTERY ANODE; SILICON NANOWIRES; PERFORMANCE; CARBON; IRON;
   SUPERCAPACITORS; NANOPARTICLES; MICROSPHERES; GRAPHENE; CATHODE
AB Developing electrode materials with both high energy and power densities holds the key for satisfying the urgent demand of energy storage worldwide. In order to realize the fast and efficient transport of ions/electrons and the stable structure during the charge/discharge process, hierarchical porous Fe3O4/graphene nanowires supported by amorphous vanadium oxide matrixes have been rationally synthesized through a facile phase separation process. The porous structure is directly in situ constructed from the FeVO4 center dot 1.1H(2)O@graphene nanowires along with the crystallization of Fe3O4 and the amorphization of vanadium oxide without using any hard templates. The hierarchical porous Fe3O4/VOx/graphene nanowires exhibit a high Coulombic efficiency and outstanding reversible specific capacity (1146 mAh g(-1)). Even at the high current density of 5 A g(-1), the porous nanowires maintain a reversible capacity of similar to 500 mAh g(-1). Moreover, the amorphization and conversion reactions between Fe and Fe3O4 of the hierarchical porous Fe3O4/VOx/graphene nanowires were also investigated by in situ X-ray diffraction and X-ray photoelectron spectroscopy. Our work demonstrates that the amorphous vanadium oxides matrixes supporting hierarchical porous Fe3O4/graphene nanowires are one of the most attractive anodes in energy storage applications.
C1 [An, Qinyou; Lv, Fan; Liu, Qiuqi; Han, Chunhua; Zhao, Kangning; Sheng, Jinzhi; Wei, Qiulong; Yan, Mengyu; Mai, Liqiang] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, WUT Harvard Joint Nano Key Lab, Wuhan 430070, Peoples R China.
RP Mai, LQ (reprint author), Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, WUT Harvard Joint Nano Key Lab, Wuhan 430070, Peoples R China.
EM hch5927@whut.edu.cn; mlq518@whut.edu.cn
RI Yan, Mengyu/F-8252-2015; Wei, Qiulong/M-1319-2015; Yan,
   Mengyu/M-1298-2015
OI Wei, Qiulong/0000-0002-9551-8309; Yan, Mengyu/0000-0003-1028-0627
FU National Basic Research Program of China [2013CB934103, 2012CB933003];
   National Science Fund for Distinguished Young Scholarsthe National
   Natural Science Foundation of China [51272197, 51302203]; International
   Science and Technology Cooperation Program of China [2013DFA50840];
   Hubei Science Fund for Distinguished Young Scholars [2014CFA035];
   Fundamental Research Funds for the Central Universities [2014-YB-001,
   2014-YB-002, 2014-ZY-016, 2013-ZD-7, 2014-VII-007]; Students Innovation
   and Entrepreneurship Training Program [20131049701008]
FX This work was supporting by the National Basic Research Program of China
   (2013CB934103, 2012CB933003), The National Science Fund for
   Distinguished Young Scholarsthe National Natural Science Foundation of
   China (51272197, 51302203), the International Science and Technology
   Cooperation Program of China (2013DFA50840), the Hubei Science Fund for
   Distinguished Young Scholars (2014CFA035), the Fundamental Research
   Funds for the Central Universities (2014-YB-001, 2014-YB-002,
   2014-ZY-016, 2013-ZD-7, 2014-VII-007), and the Students Innovation and
   Entrepreneurship Training Program (20131049701008). Thanks to Professor
   C. M. Lieber of Harvard University and Professor D. Y. Zhao of Fudan
   University for strong support and stimulating discussion.
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NR 55
TC 38
Z9 39
U1 41
U2 216
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD NOV
PY 2014
VL 14
IS 11
BP 6250
EP 6256
DI 10.1021/nl5025694
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AU6PE
UT WOS:000345723800035
PM 25314630
ER

PT J
AU Ko, M
   Chae, S
   Jeong, S
   Oh, P
   Cho, J
AF Ko, Minseong
   Chae, Sujong
   Jeong, Sookyung
   Oh, Pilgun
   Cho, Jaephil
TI Elastic a-Silicon Nanoparticle Backboned Graphene Hybrid as a
   Self-Compacting Anode for High-Rate Lithium Ion Batteries
SO ACS NANO
LA English
DT Article
DE silicon anode; volume expansion; rate capability; hybrid composite; Li
   ion battery
ID AMORPHOUS-SILICON; RECHARGEABLE BATTERIES; NEGATIVE ELECTRODES;
   ELECTROCHEMICAL PERFORMANCE; ENERGY-STORAGE; ALLOY ANODES; LITHIATION;
   PARTICLES; OXIDE; COMPOSITES
AB Although various Si-based graphene nanocomposites provide enhanced electrochemical performance, these candidates still yield low initial coloumbic efficiency, electrical disconnection, and fracture due to huge volume changes after extended cycles lead to severe capacity fading and increase in internal impedance. Therefore, an innovative structure to solve these problems is needed. In this study, an amorphous (a) silicon nanoparticle backboned graphene nanocomposite (a-SBG) for high power lithium ion battery anodes was prepared. The a-SBG provides ideal electrode structures a uniform distribution of amorphous silicon nanoparticle islands (particle size <10 nm) on both sides of graphene sheets which address the improved kinetics and cycling stability issues of the silicon anodes a-Si in the composite shows elastic behavior during lithium alloying and dealloying: the pristine particle size is restored after cycling, and the electrode thickness decreases during the cycles as a result of self-compacting. This noble architecture facilitates superior electrochemical performance in Li ion cells, with a specific energy of 468 W h kg(-1) and 288 W h kg(-1) under a specific power of 7 kW kg(-1) and 11 kW kg(-1), respectively.
C1 [Ko, Minseong; Chae, Sujong; Jeong, Sookyung; Oh, Pilgun; Cho, Jaephil] UNIST, Sch Energy & Chem Engn, Dept Energy Engn, Ulsan 689798, South Korea.
RP Cho, J (reprint author), UNIST, Sch Energy & Chem Engn, Dept Energy Engn, Ulsan 689798, South Korea.
EM jpcho@unist.ac.kr
RI Cho, Jaephil/E-4265-2010
FU C-ITRC (Convergence Information Technology Research Center) support
   program [NIPA-2013-H0301-13-1009]
FX This research was supported by C-ITRC (Convergence Information
   Technology Research Center) support program (NIPA-2013-H0301-13-1009)
   supervised by the NIPA (National IT Industry Promotion Agency) through
   the Ministry of Science, ICT and Future Planning, Korea.
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NR 55
TC 38
Z9 38
U1 32
U2 190
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD AUG
PY 2014
VL 8
IS 8
BP 8591
EP 8599
DI 10.1021/nn503294z
PG 9
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AO0IM
UT WOS:000340992300110
PM 25078072
ER

PT J
AU Rai, AK
   Anh, LT
   Gim, J
   Mathew, V
   Kang, J
   Paul, BJ
   Singh, NK
   Song, J
   Kim, J
AF Rai, Alok Kumar
   Anh, Ly Tuan
   Gim, Jihyeon
   Mathew, Vinod
   Kang, Jungwon
   Paul, Baboo Joseph
   Singh, Nitish Kumar
   Song, Jinju
   Kim, Jaekook
TI Facile approach to synthesize CuO/reduced graphene oxide nanocomposite
   as anode materials for lithium-ion battery
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Copper oxide; Graphene; Spex mill; Anode; Lithium ion battery
ID ELECTRODE MATERIALS; REVERSIBLE CAPACITY; PERFORMANCE; CUO; CU2O;
   MICROSPHERES; NANOSPHERES; STORAGE
AB An efficient synthesis is used for the first time to prepare CuO/reduced graphene oxide nanocomposite anode materials for lithium ion batteries. Initially, copper oxide (CuO) nanoparticles are synthesized via a simple, facile and inexpensive microwave-assisted method within short reaction times (<20 min) and subsequent heat treatment at 500 degrees C for 5 h. The obtained pure CuO nanoparticles are mixed with 10 wt% of graphene nanosheets by the use of spex mill for 1 min. By short-time spex-milling, a unique CuO/reduced graphene oxide nanocomposite is obtained with a microstructure of multi-scale CuO nanoparticles homogeneously dispersed in a graphene matrix. The synthesized samples are characterized using X-ray diffraction and field-emission transmission electron microscopy studies. The spex-milled nanocomposite anode exhibits better electrochemical performance with higher reversible capacity and excellent cyclability in comparison with pure CuO nanoparticles. The initial discharge capacity of the pure CuO nanoparticles and their nanocomposite are 785.2 mAh g(-1), and 1043.3 mAh g(-1) with reversible capacity retention of 392.1 mAh g(-1) and 516.4 mAh g(-1) after 45 cycles respectively. The excellent electrochemical performance of CuO/reduced graphene oxide nanocomposite can be attributed to their unique structures, which intimately combine the conductive graphene nanosheets network with uniformly dispersed CuO nanoparticles. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Rai, Alok Kumar; Anh, Ly Tuan; Gim, Jihyeon; Mathew, Vinod; Kang, Jungwon; Paul, Baboo Joseph; Singh, Nitish Kumar; Song, Jinju; Kim, Jaekook] Chonnam Natl Univ, Dept Mat Sci & Engn, Kwangju 500757, South Korea.
RP Kim, J (reprint author), Chonnam Natl Univ, Dept Mat Sci & Engn, 300 Yongbong Dong, Kwangju 500757, South Korea.
EM jaekook@chonnam.ac.kr
RI Rai,  Alok Kumar/N-3007-2014
FU Priority Research Centers Program through the National Research
   Foundation of Korea (NRF); Ministry of Education, Science and Technology
   [2009-0094055]; MKE (The Ministry of Knowledge Economy), Korea, under
   the ITRC (Information Technology Research Center)
   [NIPA-2012-H0301-12-1009]
FX This work was supported by Priority Research Centers Program through the
   National Research Foundation of Korea (NRF) funded by the Ministry of
   Education, Science and Technology (2009-0094055). This research was also
   supported by the MKE (The Ministry of Knowledge Economy), Korea, under
   the ITRC (Information Technology Research Center) support program
   supervised by the NIPA (National IT Industry Promotion Agency)
   (NIPA-2012-H0301-12-1009).
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NR 46
TC 38
Z9 39
U1 15
U2 297
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD DEC 15
PY 2013
VL 244
SI SI
BP 435
EP 441
DI 10.1016/j.jpowsour.2012.11.112
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 219MR
UT WOS:000324511600062
ER

PT J
AU Zhou, XS
   Bao, JC
   Dai, ZH
   Guo, YG
AF Zhou, Xiaosi
   Bao, Jianchun
   Dai, Zhihui
   Guo, Yu-Guo
TI Tin Nanoparticles Impregnated in Nitrogen-Doped Graphene for Lithium-Ion
   Battery Anodes
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID ENERGY-STORAGE DEVICES; HOLLOW CARBON; ELECTROCHEMICAL PERFORMANCE;
   SILICON NANOPARTICLES; MESOPOROUS CARBON; COMPOSITE ANODES; ELECTRODES;
   GRAPHITE; NANOCOMPOSITE; NANOCRYSTALS
AB Tin possesses a high theoretical specific capacity as anode materials for Li-ion batteries, and considerable efforts have been contributed to mitigating the capacity fading along with its huge volume expansion during lithium insertion and extraction processes, mainly through nanostructured material design. Herein, we present Sn nanoparticles encapsulated in nitrogen-doped graphene sheets through heat-treatment of the SnO2 nanocrystals/nitrogen-doped graphene hybrid. The specific architecture of the as-prepared Sn@N-RGO involves three advantages, including a continuous graphene conducting network, coating Sn surface through Sn-N and Sn-O bonding generated between Sn nanoparticles and graphene, and porous and flexible structure for accommodating the large volume changes of Sn nanoparticles. As an anode material for lithium-ion batteries, the hybrid exhibits a reversible capacity of 481 mA h g(-1) after 100 cycles under 0.1 A g(-1) and a charge capacity as high as 307 mA h g(-1) under 2 A g(-1).
C1 [Zhou, Xiaosi; Bao, Jianchun; Dai, Zhihui] Nanjing Normal Univ, Sch Chem & Mat Sci, Jiangsu Key Lab Biofunct Mat, Nanjing 210023, Jiangsu, Peoples R China.
   [Zhou, Xiaosi; Guo, Yu-Guo] Chinese Acad Sci, CAS Key Lab Mol Nanostruct & Nanotechnol, BNLMS, Inst Chem, Beijing 100190, Peoples R China.
RP Zhou, XS (reprint author), Nanjing Normal Univ, Sch Chem & Mat Sci, Jiangsu Key Lab Biofunct Mat, Nanjing 210023, Jiangsu, Peoples R China.
EM zhouxiaosi@njnu.edu.cn; daizhihuii@njnu.edu.cn; ygguo@iccas.ac.cn
RI Guo, Yu-Guo/A-1223-2009
OI Guo, Yu-Guo/0000-0003-0322-8476
FU National Basic Research Program of China [2011CB935700, 2012CB932900];
   National Natural Science Foundation of China [51225204, 91127044,
   21121063]; Chinese Academy of Sciences; Priority Academic Program
   Development of Jiangsu Higher Education Institutions; Program for
   Jiangsu Collaborative Innovation Center of Biomedical Functional
   Materials
FX This work was supported by the National Basic Research Program of China
   (Grant Nos. 2011CB935700 and 2012CB932900), the National Natural Science
   Foundation of China (Grant Nos. 51225204, 91127044 and 21121063), and
   the Chinese Academy of Sciences. We also appreciate the financial
   support from the Priority Academic Program Development of Jiangsu Higher
   Education Institutions and the Program for Jiangsu Collaborative
   Innovation Center of Biomedical Functional Materials.
CR Zhou XS, 2012, ADV ENERGY MATER, V2, P1086, DOI 10.1002/aenm.201200158
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NR 61
TC 38
Z9 38
U1 21
U2 198
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD DEC 5
PY 2013
VL 117
IS 48
BP 25367
EP 25373
DI 10.1021/jp409668m
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 267ME
UT WOS:000328101200018
ER

PT J
AU Fan, ZJ
   Yan, J
   Ning, GQ
   Wei, T
   Zhi, LJ
   Wei, F
AF Fan, Zhuangjun
   Yan, Jun
   Ning, Guoqing
   Wei, Tong
   Zhi, Linjie
   Wei, Fei
TI Porous graphene networks as high performance anode materials for lithium
   ion batteries
SO CARBON
LA English
DT Article
ID STORAGE; CARBON; NANOSHEETS; CAPACITY; OXIDE
AB Porous graphene obtained by chemical vapor deposition (CVD) using porous MgO sheets as template is demonstrated to exhibit a high reversible capacity (1723 mAh g(-1)), excellent high-rate capability and cycling stability for Li-ion batteries. The simple CVD approach offers a new way for large-scale production of porous graphene materials for energy storage. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Fan, Zhuangjun; Yan, Jun; Wei, Tong] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Key Lab Superlight Mat & Surface Technol, Minist Educ, Harbin 150001, Peoples R China.
   [Ning, Guoqing] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China.
   [Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
   [Wei, Fei] Tsinghua Univ, Beijing Key Lab Green Chem React Engn & Technol, Dept Chem Engn, Beijing 100084, Peoples R China.
RP Fan, ZJ (reprint author), Harbin Engn Univ, Coll Mat Sci & Chem Engn, Key Lab Superlight Mat & Surface Technol, Minist Educ, Harbin 150001, Peoples R China.
EM fanzhj666@163.com
RI Yan, Jun/D-4360-2011; Wei, Fei/H-4809-2012
OI Yan, Jun/0000-0002-9967-3912; 
FU National Science Foundation of China [51077014, 21003028, 51202043];
   Fundamental Research Funds for the Central Universities; Program for New
   Century Excellent Talents in University [NCET-10-0050]; Postdoctoral
   Science-Research Developmental Foundation of Heilongjiang Province
   [LBH-Q12113]; Excellent Youth Foundation of Heilongjiang Province of
   China [JC201210]
FX The authors acknowledge financial support from the National Science
   Foundation of China (51077014, 21003028 and 51202043), Fundamental
   Research Funds for the Central Universities, Program for New Century
   Excellent Talents in University (NCET-10-0050), Postdoctoral
   Science-Research Developmental Foundation of Heilongjiang Province
   (LBH-Q12113) and Excellent Youth Foundation of Heilongjiang Province of
   China (JC201210).
CR Zhou Y, 2009, CHEM MATER, V21, P2950, DOI 10.1021/cm9006603
   Pan DY, 2009, CHEM MATER, V21, P3136, DOI 10.1021/cm900395k
   Uthaisar C, 2010, NANO LETT, V10, P2838, DOI 10.1021/nl100865a
   Su YZ, 2012, ACS NANO, V6, P8349, DOI 10.1021/nn303091t
   Wang XL, 2009, APPL PHYS LETT, V95, DOI 10.1063/1.3259650
   Wang GX, 2009, CARBON, V47, P2049, DOI 10.1016/j.carbon.2009.03.053
   Wang HL, 2011, NANO LETT, V11, P2644, DOI 10.1021/nl200658a
   Bai JW, 2010, NAT NANOTECHNOL, V5, P190, DOI [10.1038/nnano.2010.8, 10.1038/NNANO.2010.8]
   Su DS, 2010, CHEMSUSCHEM, V3, P136, DOI 10.1002/cssc.200900182
   Zhou HS, 2003, ADV MATER, V15, P2107, DOI 10.1002/adma.200306125
   Ning GQ, 2011, CHEM COMMUN, V47, P5976, DOI 10.1039/c1cc11159k
   Mukherjee R, 2012, ACS NANO, V6, P7867, DOI 10.1021/nn303145j
   Yoo E, NANO LETT
NR 13
TC 38
Z9 40
U1 22
U2 210
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD AUG
PY 2013
VL 60
BP 558
EP 561
DI 10.1016/j.carbon.2013.04.053
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 180MB
UT WOS:000321598200065
ER

PT J
AU Li, C
   Wang, XS
   Chen, F
   Zhang, CL
   Zhi, X
   Wang, K
   Cui, DX
AF Li, Chao
   Wang, Xiansong
   Chen, Feng
   Zhang, Chunlei
   Zhi, Xiao
   Wang, Kan
   Cui, Daxiang
TI The antifungal activity of graphene oxide-silver nanocomposites
SO BIOMATERIALS
LA English
DT Article
DE Graphene oxide; Carbon nanoscrolls; Silver nanopartides; Antifungal
   activity; Controlled drug release
ID LITHIUM-ION BATTERIES; ANODE MATERIAL; NANOPARTICLES; SHEETS;
   NANOSHEETS; REDUCTION; RELEASE; CARBON; CELLS; NANOMATERIALS
AB Graphene oxide (GO)-based nanocomposites' antibacteria activity exhibits great potential in clinical application. Herein we reported for the first time the preparation and enhanced antifungal activity of carbon nanoscrolls (CNSs) filled with silver nanoparticles (AgNPs). The nanoscrolls filled with silver nanoparticles were prepared by sonication, TEM picture showed AgNPs filled and wrapped inside prepared nanocomposites, the antifungal test showed that CNSs-AgNPs exhibited ideal lengthened activities against Candida albicans and Candida tropical compared with the GO-AgNPs nanocomposites based on silver nanoparticles directly deposited on the surface of grapheme oxides, which is caused by CNS-AgNPs' controlled durative slow-releasing of silver ion. It is also observed that graphene oxides exhibited no antifungal activity. In conclusion, the carbon nanoscrolls composed of graphene oxides and silver nanoparticles own enhanced and lengthened antifungal activity, and have great potential in applications such as clinical nosocomial infections and local antifungal therapy. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Li, Chao; Wang, Xiansong; Chen, Feng; Zhang, Chunlei; Zhi, Xiao; Wang, Kan; Cui, Daxiang] Shanghai Jiao Tong Univ, Res Inst Micro Nano Sci & Technol, Minist Educ, Dept Bionano Sci & Engn,Key Lab Thin Film & Micro, Shanghai 200240, Peoples R China.
RP Cui, DX (reprint author), Shanghai Jiao Tong Univ, Res Inst Micro Nano Sci & Technol, Minist Educ, Dept Bionano Sci & Engn,Key Lab Thin Film & Micro, Shanghai 200240, Peoples R China.
EM dxcui@sjtu.edu.cn
RI Chen, Feng/D-6406-2012; 1203, Feng/E-4310-2016
OI Chen, Feng/0000-0002-1162-1684; 1203, Feng/0000-0002-1162-1684
FU Chinese 973 Project [2010CB933901]; National Natural Science Foundation
   of China [81225010, 81101169, 31100717]; New Century Excellent Talent of
   Ministry of Education of China [NCET-08-0350]; Special Infection
   Diseases Key Project of China [2009ZX10004-311]; Doctorial Position
   Budget [20070248050]
FX This work was supported by Chinese 973 Project (2010CB933901), the
   National Natural Science Foundation of China (No. 81225010, 81101169 and
   31100717), New Century Excellent Talent of Ministry of Education of
   China (NCET-08-0350), Special Infection Diseases Key Project of China
   (2009ZX10004-311) and Doctorial Position Budget (20070248050).
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NR 60
TC 38
Z9 39
U1 19
U2 167
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 0142-9612
J9 BIOMATERIALS
JI Biomaterials
PD MAY
PY 2013
VL 34
IS 15
BP 3882
EP 3890
DI 10.1016/j.biomaterials.2013.02.001
PG 9
WC Engineering, Biomedical; Materials Science, Biomaterials
SC Engineering; Materials Science
GA 120KH
UT WOS:000317168700015
PM 23465487
ER

PT J
AU Zhang, M
   Jia, MQ
AF Zhang, Mei
   Jia, Mengqiu
TI High rate capability and long cycle stability Fe3O4-graphene
   nanocomposite as anode material for lithium ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Graphene; Fe3O4 nanoparticles; Nanocomposite; Anode; Lithium ion
   batteries
ID HIGH-PERFORMANCE ANODE; ONE-POT SYNTHESIS; ELECTROCHEMICAL PERFORMANCE;
   REVERSIBLE CAPACITY; FE3O4 NANOPARTICLES; STORAGE CAPACITY; FACILE
   SYNTHESIS; OXIDE COMPOSITE; GRAPHENE; LI
AB We developed one-spot in situ synthesis method to form nanocomposite of reduced graphene oxide (RGO) sheets with Fe3O4 nanoparticles for lithium ion battery applications. A transmission electron microscopy image has shown that the as-formed Fe3O4 nanoparticles are about 10 nm in average size, and uniformly anchor on RGO sheets as spacers to keep the neighboring sheets separated. The Fe3O4-RGO nanocomposite exhibits improved rate capability of 436 mA h g(-1) at 2400 mA g(-1). It delivers a high capacity of 1188 mA h g(-1) at 100 mA g(-1) after 1000 cycles of charge and discharge at various rates from 100 to 6000 mA g(-1), indicating outstanding cycle stability. The improved electrochemical performance can be attributed to the important interfacial interaction between small-sized Fe3O4 nanoparticles and ultrathin RGO nanosheets, and suggests that Fe3O4-RGO nanocomposite with superior performance will be a promising anode material for lithium ion batteries. (C) 2012 Elsevier B. V. All rights reserved.
C1 [Zhang, Mei; Jia, Mengqiu] Beijing Univ Chem Technol, Coll Mat Sci & Engn, Beijing 100029, Peoples R China.
RP Jia, MQ (reprint author), Beijing Univ Chem Technol, Coll Mat Sci & Engn, Beijing 100029, Peoples R China.
EM jiamq@mail.buct.edu.cn
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   Huang XH, 2010, ELECTROCHIM ACTA, V55, P8981, DOI 10.1016/j.electacta.2010.08.039
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   Tian LL, 2012, ELECTROCHIM ACTA, V65, P153, DOI 10.1016/j.electacta.2012.01.034
   Zhu T, 2011, J PHYS CHEM C, V115, P9814, DOI 10.1021/jp2013754
   Chen S, 2010, J PHYS CHEM C, V114, P11829, DOI 10.1021/jp1048474
   Zhou JS, 2011, ELECTROCHEM COMMUN, V13, P1357, DOI 10.1016/j.elecom.2011.08.011
   Lian PC, 2011, ELECTROCHIM ACTA, V58, P81, DOI 10.1016/j.electacta.2011.08.088
   Ni SB, 2011, J ALLOY COMPD, V509, pL305, DOI 10.1016/j.jallcom.2011.06.007
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NR 42
TC 38
Z9 41
U1 11
U2 244
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
EI 1873-4669
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD FEB 25
PY 2013
VL 551
BP 53
EP 60
DI 10.1016/j.jallcom.2012.09.115
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 072EI
UT WOS:000313651600011
ER

PT J
AU Cai, DD
   Wang, SQ
   Lian, PC
   Zhu, XF
   Li, DD
   Yang, WS
   Wang, HH
AF Cai, Dandan
   Wang, Suqing
   Lian, Peichao
   Zhu, Xuefeng
   Li, Dongdong
   Yang, Weishen
   Wang, Haihui
TI Superhigh capacity and rate capability of high-level nitrogen-doped
   graphene sheets as anode materials for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Nitrogen-doped; Graphene sheets; Anode material; Lithium-ion batteries
ID OXYGEN-REDUCTION REACTION; CARBON NANOTUBES; GRAPHITE OXIDE; LI STORAGE;
   NANOSHEETS; 1ST-PRINCIPLES; PERFORMANCE; CATALYST; UREA
AB A new facile approach is proposed to synthesize nitrogen-doped graphene sheets with the nitrogen-doping level as high as 7.04 at.% by thermal annealing pristine graphene sheets and low-cost industrial material melamine. The high-level nitrogen-doped graphene sheets exhibit a superhigh initial reversible capacity of 1123 mAh g(-1) at a current density of 50 mA g(-1). More significantly, even at an extremely high current density of 20 A g(-1), highly stable capacity of about 241 mAh g(-1) could still be obtained. Such an electrochemical performance is superior to those previously reported nitrogen-doped graphene sheets. The excellent electrochemical performance can be attributed to the two-dimensional structure, disordered surface morphology, high nitrogen-doping level, and the existence of pyridinic nitrogen atoms. The results indicate that the high-level nitrogen-doped graphene sheets could be a promising anode material for high-performance lithium-ion batteries. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Cai, Dandan; Wang, Suqing; Li, Dongdong; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou, Peoples R China.
   [Lian, Peichao] Kunming Univ Sci & Technol, Fac Chem Engn, Kunming, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013; Wang,
   Suqing/G-4930-2016
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620; 
FU National Natural Science Foundation of China [20936001]; Fundamental
   Research Funds for the Central Universities, SCUT [2009220038];
   Cooperation Project in Industry, Education and Research of Guangdong
   Province; Ministry of Education of China [2010B090400518]
FX This work was financially supported by the National Natural Science
   Foundation of China (no. 20936001), the Cooperation Project in Industry,
   Education and Research of Guangdong Province and Ministry of Education
   of China (no. 2010B090400518) and the Fundamental Research Funds for the
   Central Universities, SCUT (2009220038).
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NR 42
TC 38
Z9 39
U1 15
U2 200
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 15
PY 2013
VL 90
BP 492
EP 497
DI 10.1016/j.electacta.2012.11.105
PG 6
WC Electrochemistry
SC Electrochemistry
GA 105AI
UT WOS:000316037600063
ER

PT J
AU Lavoie, N
   Malenfant, PRL
   Courtel, FM
   Abu-Lebdeh, Y
   Davidson, IJ
AF Lavoie, Nathalie
   Malenfant, Patrick R. L.
   Courtel, Fabrice M.
   Abu-Lebdeh, Yaser
   Davidson, Isobel J.
TI High gravimetric capacity and long cycle life in Mn3O4/graphene
   platelet/LiCMC composite lithium-ion battery anodes
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Graphene; Manganese oxide; Li-ion batteries; Anode materials; Lithium
   carboxymethyl cellulose (LiCMC)
ID REVERSIBLE CAPACITY; NEGATIVE-ELECTRODE; BINDER CHEMISTRY; GRAPHENE
   OXIDE; GRAPHITE OXIDE; PERFORMANCE; NANOPARTICLES; MN3O4; ALPHA-FE2O3;
   FABRICATION
AB We report the synthesis, characterization and battery performance of a novel Mn3O4/graphene composite based on graphene platelets and also an Mn3O4/reduced-graphene-oxide composite for comparison. The electrodes were cast from aqueous dispersions in which lithium carboxymethyl cellulose was used as a binder thus enabling an aqueous based process for anode fabrication. The Mn3O4/graphene-platelet and the Mn3O4/reduced-graphene-oxide composites anode system possess high gravimetric capacities (similar to 700 mAh g(-1)) and excellent cycling stability (>100 cycles). Crown Copyright (C) 2012 Published by Elsevier B.V. All rights reserved.
C1 [Lavoie, Nathalie; Malenfant, Patrick R. L.; Courtel, Fabrice M.; Abu-Lebdeh, Yaser; Davidson, Isobel J.] Natl Res Council Canada, Ottawa, ON K1A 0R6, Canada.
RP Abu-Lebdeh, Y (reprint author), Natl Res Council Canada, 1200 Montreal Rd, Ottawa, ON K1A 0R6, Canada.
EM Patrick.Malenfant@nrc-cnrc.gc.ca; Yaser.Abu-Lebdeh@nrc-cnrc.gc.ca
RI Courtel, Fabrice/J-9332-2012
OI Courtel, Fabrice/0000-0002-6214-1883
FU Natural Resources Canada's Office of Energy Research and Development
   (Electric Mobility Program of Energy Research and Development: PERD
   project) [C51.003]
FX This work was supported by Natural Resources Canada's Office of Energy
   Research and Development (Electric Mobility Program of Energy Research
   and Development: PERD project number C51.003).
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NR 32
TC 38
Z9 39
U1 14
U2 116
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 1
PY 2012
VL 213
BP 249
EP 254
DI 10.1016/j.jpowsour.2012.03.055
PG 6
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 971ZR
UT WOS:000306246800031
ER

PT J
AU Bai, S
   Chen, SQ
   Shen, XP
   Zhu, GX
   Wang, GX
AF Bai, Song
   Chen, Shuangqiang
   Shen, Xiaoping
   Zhu, Guoxing
   Wang, Guoxiu
TI Nanocomposites of hematite (alpha-Fe2O3) nanospindles with crumpled
   reduced graphene oxide nanosheets as high-performance anode material for
   lithium-ion batteries
SO RSC ADVANCES
LA English
DT Article
ID IMPROVED REVERSIBLE CAPACITY; MAGNETIC-PROPERTIES; LI-STORAGE;
   COMPOSITES; ELECTRODES; STABILITY
AB Nanocomposites of Fe2O3 nanospindles with crumpled reduced graphene oxide (RGO) nanosheets were prepared using a facile solvothermal synthesis method. The RGO-Fe2O3 nanocomposite with about 24.4 wt% RGO demonstrated an excellent electrochemical performance as a promising anode material for lithium-ion batteries (LIBs), which achieved a high reversible capacity of 969 mA h g(-1) after 100 cycles at a current density of 100 mA g(-1) (0.1 C). Furthermore, it also exhibited a large capacity of 336 mA h g(-1) after 100 cycles at the high rate of 5 C. The cycling performance and reversible capacities of the RGO-Fe2O3 composites were much better than those of bare Fe2O3 nanospindles and pure RGO nanosheets, as well as previously reported RGO-Fe2O3 nanocomposites. The enhanced performance towards lithium storage can be ascribed to the crumpled RGO nanosheets, which may act as efficient volume buffer and electron conductor in the composites. The strategy proposed here could be extended to produce other nanocomposites based on crumpled graphene nanosheets for various applications.
C1 [Bai, Song; Shen, Xiaoping; Zhu, Guoxing] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.
   [Chen, Shuangqiang; Wang, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Sydney, NSW 2007, Australia.
RP Bai, S (reprint author), Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.
EM xiaopingshen@163.com
RI Chen, Shuangqiang/F-5289-2013
FU National Natural Science Foundation of China [51272094, 51072071,
   51102117]
FX The authors are grateful for financial support from the National Natural
   Science Foundation of China (No. 51272094, 51072071 and 51102117).
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NR 38
TC 38
Z9 38
U1 9
U2 103
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 29
BP 10977
EP 10984
DI 10.1039/c2ra21411c
PG 8
WC Chemistry, Multidisciplinary
SC Chemistry
GA 051QS
UT WOS:000312142700029
ER

PT J
AU Kohs, W
   Santner, HJ
   Hofer, F
   Schrottner, H
   Doninger, J
   Barsukov, I
   Buqa, H
   Albering, JH
   Moller, KC
   Besenhard, JO
   Winter, M
AF Kohs, W
   Santner, HJ
   Hofer, F
   Schrottner, H
   Doninger, J
   Barsukov, I
   Buqa, H
   Albering, JH
   Moller, KC
   Besenhard, JO
   Winter, M
TI A study on electrolyte interactions with graphite anodes exhibiting
   structures with various amounts of rhombohedral phase
SO JOURNAL OF POWER SOURCES
LA English
DT Article; Proceedings Paper
CT 11th International Meeting on Lithium Batteries
CY JUN 24-28, 2002
CL MONTEREY, CALIFORNIA
DE graphite anode; lithium-ion battery; solid electrolyte interphase (SEI);
   electrolyte additive; rhombohedral phase
ID LITHIUM-ION BATTERIES; INTERCALATION; CARBONS; CHOICE; CELLS
AB The lithium-ion battery anode performance of graphites with and without high amounts of rhombohedral phase in the structure has been investigated. A main outcome was that in addition to possible graphite bulk structure effects, there are also strong influences of the graphite surface and the graphite "sub-surface" (part of the graphite bulk at the border of the particle near the surface) on the solid electrolyte interphase (SEI) formation process and on the tendency to solvent co-intercalation into graphite. Using transmission electron microscopy with atomic resolution, we indeed could determine unique and also different surface and "sub-surface" morphologies for the two graphites. In case of the graphite without rhombohedral phase, unique convoluted graphene layers could be determined at the prismatic surfaces; in case of the graphite with a high rhombohedral phase content a strongly disordered, approximately 1 nm thick "sub-surface" layer could be determined. The anode performance depends primarily on these surface and "sub-surface" graphite properties and the used electrolytes. The differences in the "sub-surface" layer structure have a most significant influence on the performance in an ethylene carbonate/dimethyl carbonate electrolyte. The differences in surface structure and morphology are considered to have the highest impact in a propylene carbonate/ethylene sulfite-based electrolyte. For ethylene carbonate/diethyl carbonate electrolyte, the performance differences are small so that no strong dependence on surface or "sub-surface" structures could be observed. (C) 2003 Elsevier Science B.V. All rights reserved.
C1 Graz Univ Technol, Inst Chem Technol Inorgan Mat, A-8010 Graz, Austria.
   Super Graphite Co, Chicago, IL 60606 USA.
   Graz Univ Technol, Res Inst Electron Microscopy, Graz, Austria.
RP Winter, M (reprint author), Graz Univ Technol, Inst Chem Technol Inorgan Mat, A-8010 Graz, Austria.
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NR 15
TC 38
Z9 39
U1 1
U2 18
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 1
PY 2003
VL 119
SI SI
BP 528
EP 537
DI 10.1016/S0378-7753(03)00278-7
PG 10
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 694XC
UT WOS:000183799600099
ER

PT J
AU Yuan, FW
   Tuan, HY
AF Yuan, Fang-Wei
   Tuan, Hsing-Yu
TI Scalable Solution-Grown High-Germanium-Nanoparticle-Loading Graphene
   Nanocomposites as High-Performance Lithium-Ion Battery Electrodes: An
   Example of a Graphene-Based Platform toward Practical Full-Cell
   Applications
SO CHEMISTRY OF MATERIALS
LA English
DT Article
ID LONG CYCLE LIFE; ANODE MATERIALS; HIGH-CAPACITY; HYBRID NANOSHEETS;
   FACILE SYNTHESIS; COMPOSITE ANODE; GE NANOWIRES; NANOCRYSTALS; STORAGE;
   SILICON
AB Graphene in the form of graphene/nanocrystal nanocomposites can improve the electrochemical performance of nanocrystals for lithium-ion (Li-ion) battery anodes, which is especially important for high-capacity Li-alloy materials such as Si and Ge. For practical full-cell applications, graphene composite electrodes consisting of a large portion of active materials (i.e., a surface of graphene sheets evenly distributed with dense nanoparticles) are required. We have developed a facile solution-based method to synthesize subgram quantities of nanocomposites composed of reduced graphene oxide (RGO) sheets covered with a high concentration (similar to 80 wt %) of single-crystal 4.90(+/- 0.80) nm diameter Ge nanoparticles. Subsequently, carbon-coated Ge nanoparticles/RGO (Ge/RGO/C) sandwich structures were formed via a carbonization process. The high-nanoparticle-loading nanocomposites exhibited superior Li-ion battery anode performance when examined with a series of comprehensive tests, such as receiving a practical capacity of Ge (1332 mAh/g) close (96.2%) to its theoretical value (1384 mAh/g) when cycled at a 0.2 C rate and having a high-rate capability over hundreds of cycles. Furthermore, the performance of the full cells assembled using a Ge/RGO/C anode and an LiCoO2 cathode were evaluated. The cells were able to power a wide range of electronic devices, including an light-emitting-diode (LED) array consisting of over 150 bulbs, blue LED arrays, a scrolling LED marquee, and an electric fan. Thus, this study demonstrates a proof of concept of the use of graphene-based nanocomposites toward practical Li-ion battery applications.
C1 [Yuan, Fang-Wei; Tuan, Hsing-Yu] Natl Tsing Hua Univ, Dept Chem Engn, Hsinchu 30013, Taiwan.
RP Tuan, HY (reprint author), Natl Tsing Hua Univ, Dept Chem Engn, 101,Sect 2,Kuang Fu Rd, Hsinchu 30013, Taiwan.
EM hytuan@che.nthu.edu.tw
FU National Science Council of Taiwan [NSC 102-2221-E-007-023-MY3, NSC
   102-2221-E-007-090-MY2, NSC 101-2623-E-007-013-IT,
   NSC102-2633-M-007-002]; Ministry of Economic Affairs, Taiwan
   [101-EC-17-A-09-S1-198]; National Tsing Hua University [102N2051E1,
   102N2061E1]
FX We acknowledge the financial support from the National Science Council
   of Taiwan (NSC 102-2221-E-007-023-MY3, NSC 102-2221-E-007-090-MY2, NSC
   101-2623-E-007-013-IT, and NSC102-2633-M-007-002), the Ministry of
   Economic Affairs, Taiwan (101-EC-17-A-09-S1-198), National Tsing Hua
   University (102N2051E1 and 102N2061E1), and the assistance from Center
   for Energy and Environmental Research, National Tsing-Hua University.
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NR 62
TC 37
Z9 37
U1 26
U2 165
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0897-4756
EI 1520-5002
J9 CHEM MATER
JI Chem. Mat.
PD MAR 25
PY 2014
VL 26
IS 6
BP 2172
EP 2179
DI 10.1021/cm5002016
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA AD8TT
UT WOS:000333539300024
ER

PT J
AU Sun, HT
   Sun, X
   Hu, T
   Yu, MP
   Lu, FY
   Lian, J
AF Sun, Hongtao
   Sun, Xiang
   Hu, Tao
   Yu, Mingpeng
   Lu, Fengyuan
   Lian, Jie
TI Graphene-Wrapped Mesoporous Cobalt Oxide Hollow Spheres Anode for
   High-Rate and Long-Life Lithium Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID NEGATIVE ELECTRODE MATERIAL; ELECTROCHEMICAL PROPERTIES; REVERSIBLE
   CAPACITY; NANOWIRE ARRAYS; CO3O4 NANOTUBES; CARBON SPHERES; PERFORMANCE;
   STORAGE; NANOPARTICLES; COO
AB Transition metal oxides, used as LIB anodes, typically experience significant capacity fading at high rates and long cycles due to chemical and mechanical degradations upon cycling. In this work, an effective strategy is implemented to mitigate capacity fading of Co3O4 at high rates by use of hollow and mesoporous Co3O4 spheres and graphene sheets in a core-shell geometry. The core-shell structure exhibits a high reversible capacity of 1076 inAh g(-1) at a current density of 0.1 A g(-1), and excellent rate performance from 0.1 to 5.0 A g(-1). The graphene/Co3O4 nanosphere composite electrode also displays an exceptional cyclic stability with an extraordinarily high reversible capacity over 600 mAh g(-1) after 500 cycles at a high current density of 1.0 A g(-1) without signs of further degradation. The highly conductive graphene nanosheets wrapping up on surfaces and interfaces of metal oxide nanospheres provide conductive pathways for effective charge transfer. The mesoporous features of graphene and hollow metal oxide nanosphere also enable fast diffusion of lithium ions for the charge/discharge process. The highly flexible and mechanically robust graphene nanosheets prevent particle agglomeration and buffer volume expansion of Co3O4 upon cycling. The unique nanostructure of Co3O4 wrapped up with highly flexible and conductive graphene nanosheets represents an effective strategy that may be applied for various metal oxide electrodes to mitigate the mechanical degradation and capacity fading, critical for developing advanced electrochemical energy storage systems with long cycle life and high rate performance.
C1 [Sun, Hongtao; Sun, Xiang; Hu, Tao; Yu, Mingpeng; Lu, Fengyuan; Lian, Jie] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
RP Lian, J (reprint author), Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
EM LIANJ@rpi.edu
RI Sun, Hongtao/N-6597-2013; Lu, Fengyuan/A-2875-2011
OI Sun, Hongtao/0000-0003-3259-6091; Lu, Fengyuan/0000-0003-1912-2713
FU NSF DMR Ceramic program under a NSF career award [DMR 1151028]
FX This work was financially supported by the NSF DMR Ceramic program under
   a NSF career award of DMR 1151028.
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U1 44
U2 291
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD FEB 6
PY 2014
VL 118
IS 5
BP 2263
EP 2272
DI 10.1021/jp408021m
PG 10
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AA5QC
UT WOS:000331153700004
ER

PT J
AU Sun, WW
   Wang, Y
AF Sun, Weiwei
   Wang, Yong
TI Graphene-based nanocomposite anodes for lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID HIGH-PERFORMANCE ANODE; IN-SITU SYNTHESIS; NITROGEN-DOPED GRAPHENE;
   LI-STORAGE PROPERTIES; ONE-POT SYNTHESIS; ONE-STEP SYNTHESIS;
   BINDER-FREE ANODE; IMPROVED REVERSIBLE CAPACITY; ENHANCED CYCLIC
   PERFORMANCE; CHEMICAL-VAPOR-DEPOSITION
AB Graphene-based nanocomposites have been demonstrated to be promising high-capacity anodes for lithium ion batteries to satisfy the ever-growing demands for higher capacity, longer cycle life and better high-rate performance. Synergetic effects between graphene and the introduced second-phase component are generally observed. In this feature review article, we will focus on the recent work on four different categories of graphene-based nanocomposite anodes by us and others: graphene-transitional metal oxide, graphene-Sn/Si/Ge, graphene-metal sulfide, and graphene-carbon nanotubes. For the supported materials on graphene, we will emphasize the non-zero dimensional (non-particle) morphologies such as two dimensional nanosheet/nanoplate and one dimensional nanorod/nanofibre/nanotube morphologies. The synthesis strategies and lithium-ion storage properties of these highlighted electrode morphologies are distinct from those of the commonly obtained zero dimensional nanoparticles. We aim to stress the importance of structure matching in the composites and their morphology-dependent lithium-storage properties and mechanisms.
C1 [Sun, Weiwei; Wang, Yong] Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shanghai 200444, Peoples R China.
RP Wang, Y (reprint author), Shanghai Univ, Sch Environm & Chem Engn, Dept Chem Engn, Shangda Rd 99, Shanghai 200444, Peoples R China.
EM yangwang@shu.edu.cn
RI WANG, Yong/B-1125-2012
FU National Natural Science Foundation of China [51271105, 51201095];
   Shanghai Municipal Government [13YZ012, 11JC1403900, 11SG38]; Innovative
   Research Team [IRT13078]
FX The authors gratefully acknowledge the follow-up Program for Professor
   of Special Appointment in Shanghai (Eastern Scholar), the National
   Natural Science Foundation of China (51271105 and 51201095), the
   Shanghai Municipal Government (13YZ012, 11JC1403900, 11SG38) and the
   Innovative Research Team (IRT13078) for financial support. The authors
   also thank the Lab for Microstructure, Shanghai University, for
   materials characterization.
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NR 341
TC 37
Z9 37
U1 80
U2 284
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 20
BP 11528
EP 11552
DI 10.1039/c4nr02999b
PG 25
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AQ7MB
UT WOS:000343000800002
PM 25177843
ER

PT J
AU Nam, I
   Kim, ND
   Kim, GP
   Park, J
   Yi, J
AF Nam, Inho
   Kim, Nam Dong
   Kim, Gil-Pyo
   Park, Junsu
   Yi, Jongheop
TI One step preparation of Mn3O4/graphene composites for use as an anode in
   Li ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Energy storage; Graphenes; Composite materials; Lithium-ion batteries;
   Manganese oxides
ID LITHIUM STORAGE; MN OXIDE; GRAPHENE; PERFORMANCE; CAPACITY; ELECTRODES;
   NANOSHEETS; REDUCTION; HYBRID
AB A one step method for the fabrication of Mn3O4 nanoparticles/graphene composite materials is described. An in-situ transformation technique using an aqueous phase at ambient conditions is employed. During the process of forming Mn3O4 nanoparticles, graphene oxide is simultaneously reduced to a graphene nanosheet which simplifies the overall process and eliminates the need for an additional reduction step, which is generally energy consuming and produces toxic by-products. The resulting materials were characterized using XPS, XRD, TEM, STEM-EDS and electrochemical analysis. The Mn3O4 nanoparticles with uniform size (about 14 nm) and shape are highly dispersed on the surface of graphene. The material exhibits a reversible capacity of over 500 mAh g(-1), at a current density of 60 mA g(-1) with less significant fades after 40 cycles. Furthermore, its rate capability and cycling stability are enhanced in comparison with that of the pure Mn3O4 nanoparticles. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Nam, Inho; Kim, Nam Dong; Kim, Gil-Pyo; Park, Junsu; Yi, Jongheop] Seoul Natl Univ, World Class Univ Program Chem Convergence Energy, Sch Chem & Biol Engn, Inst Chem Proc, Seoul 151742, South Korea.
RP Yi, J (reprint author), Seoul Natl Univ, World Class Univ Program Chem Convergence Energy, Sch Chem & Biol Engn, Inst Chem Proc, Seoul 151742, South Korea.
EM jyi@snu.ac.kr
FU WCU (World Class University) program, through the National Research
   Foundation of Korea; Ministry of Education, Science and Technology
   [R31-10013]
FX This research was supported by WCU (World Class University) program,
   through the National Research Foundation of Korea, funded by the
   Ministry of Education, Science and Technology (R31-10013).
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Z9 37
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PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD DEC 15
PY 2013
VL 244
SI SI
BP 56
EP 62
DI 10.1016/j.jpowsour.2013.04.055
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 219MR
UT WOS:000324511600010
ER

PT J
AU Wang, SX
   Yang, LP
   Stubbs, LP
   Li, X
   He, CB
AF Wang, Su-Xi
   Yang, Liping
   Stubbs, Ludger Paul
   Li, Xu
   He, Chaobin
TI Lignin-Derived Fused Electrospun Carbon Fibrous Mats as High Performance
   Anode Materials for Lithium Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lignin; carbon fiber; electrospinning; free-standing; nitrogen doping;
   lithium ion batteries
ID DOPED GRAPHENE; NANOFIBER WEBS; CAPACITY; POLYMER; FIBERS; NETWORKS;
   PRECURSORS; MECHANISM
AB A novel biomass-based nitrogen-doped freestanding fused carbon fibrous mat was fabricated from lignin-polyethylene oxide (PEO) (90:10) blend via electrospinning followed by carbonization and thermal annealing in the presence of urea. The morphology and structure of the carbon fibers were characterized by field-emission scanning electron microscopy, Raman spectroscopy, X-ray photoelectron spectroscopy, and elemental analysis, and their electrochemical properties were investigated for the first time as anode in lithium ion batteries (LIBs). The fused carbon fibers without nitrogen doping exhibited high specific capacity up to 445 mA h g(-1) at a current density of 30 mA g(-1) (comparable to polyacrylonitrile (PAN) derived carbon nanofibers) and good cyclic stability at different current rates. After thermal annealing to as high as 576 mA h g(-1) and still maintained a good capacity of about 200 mAh g(-1) even at a high current rate of 2000 mA g(-1). This research demonstrates the great promise of lignin-derived nanocarbon materials for applications in energy storage systems. in the presence of urea, the charge capacity was further improved
C1 [Wang, Su-Xi; Li, Xu; He, Chaobin] ASTAR, Inst Mat Res & Engn, Singapore 117602, Singapore.
   [Yang, Liping; Stubbs, Ludger Paul] ASTAR, Inst Chem & Engn Sci, Singapore 627833, Singapore.
   [Li, Xu] Natl Univ Singapore, Dept Chem, Singapore 117543, Singapore.
   [He, Chaobin] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore.
RP Li, X (reprint author), ASTAR, Inst Mat Res & Engn, 3 Res Link, Singapore 117602, Singapore.
EM x-li@imre.a-star.edu.sg; cb-he@imre.a-star.edu.sg
RI Yang, Liping/F-6081-2011; He, Chaobin/G-5755-2011
FU Agency for Science, Technology and Research (A*STAR, Singapore)
   [1124004040]
FX The authors acknowledge the financial support from the Agency for
   Science, Technology and Research (A*STAR, Singapore), Project
   1124004040.
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NR 45
TC 37
Z9 39
U1 42
U2 202
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD DEC 11
PY 2013
VL 5
IS 23
BP 12275
EP 12282
DI 10.1021/am4043867
PG 8
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 272DD
UT WOS:000328439600008
PM 24256294
ER

PT J
AU Fang, XP
   Hua, CX
   Wu, CR
   Wang, XF
   Shen, LY
   Kong, QY
   Wang, JZ
   Hu, YS
   Wang, ZX
   Chen, LQ
AF Fang, Xiangpeng
   Hua, Chunxiu
   Wu, Chengren
   Wang, Xuefeng
   Shen, Lanyao
   Kong, Qingyu
   Wang, Jiazhao
   Hu, Yongsheng
   Wang, Zhaoxiang
   Chen, Liquan
TI Synthesis and Electrochemical Performance of Graphene-like WS2
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE absorption; electrochemistry; lithium storage; sulfur; tungsten
ID LITHIUM-ION BATTERIES; LINI0.5MN0.5O2 CATHODE MATERIAL; OXYGEN
   COORDINATION COMPLEX; X-RAY-ABSORPTION; GRAPHITE ANODE; STORAGE; MOS2;
   NANOSHEETS; CARBON; TIS2
AB Graphene-like and platelike WS2 were obtained by solid-state reactions. High-resolution (HR) TEM, BET, and Raman scattering studies show that the graphene-like WS2 is a few-layer-structured material. It exhibits better electrochemical performances than the platelike WS2. Structural characterization indicates that metallic W and Li2S are the end products of discharge (0.01V versus Li+/Li), whereas metallic W and S are the recharge (3.00V) products. In addition, X-ray absorption near-edge structure (XANES) characterization shows that the d electrons of W deviate towards the Li (or S) atom during the discharge/charge process, thus forming a weak bond between W and Li2S (or S).
C1 [Fang, Xiangpeng; Hua, Chunxiu; Wu, Chengren; Wang, Xuefeng; Shen, Lanyao; Hu, Yongsheng; Wang, Zhaoxiang; Chen, Liquan] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
   [Kong, Qingyu] Soc Civile Synchrotron SOLEIL, LOrme Merisiers, F-91192 Gif Sur Yvette, France.
   [Fang, Xiangpeng; Wu, Chengren] Dongguan Amperex Technol Ltd, Dongguan 523808, Peoples R China.
   [Wang, Jiazhao] Univ Wollongong, Inst Superconducting & Elect Mat, Fairy Meadow, NSW 2519, Australia.
RP Kong, QY (reprint author), Soc Civile Synchrotron SOLEIL, LOrme Merisiers, St Aubin BP 48, F-91192 Gif Sur Yvette, France.
EM kong@synchrotron-soleil.fr; zxwang@iphy.ac.cn
RI Wang, Jiazhao/G-4972-2011; Hu, Yong-Sheng/H-1177-2011
OI Hu, Yong-Sheng/0000-0002-8430-6474
FU National 973 Program of China [2009CB220100]; National 863 Program
   [2009AA033101]; Open Foundation of Beijing Key Laboratory of Environment
   Science and Engineering; China-Australia Sci-Tech Collaboration
   Foundation (NSFC) [51011120044]
FX This work was financially supported by the National 973 Program of China
   (2009CB220100), the National 863 Program (2009AA033101), the Open
   Foundation of Beijing Key Laboratory of Environment Science and
   Engineering, and the China-Australia Sci-Tech Collaboration Foundation
   (NSFC no. 51011120044).
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NR 38
TC 37
Z9 38
U1 38
U2 422
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD APR
PY 2013
VL 19
IS 18
BP 5694
EP 5700
DI 10.1002/chem.201204254
PG 7
WC Chemistry, Multidisciplinary
SC Chemistry
GA 135IQ
UT WOS:000318282200026
PM 23463589
ER

PT J
AU Zhou, GW
   Wang, JL
   Gao, PF
   Yang, XW
   He, YS
   Liao, XZ
   Yang, J
   Ma, ZF
AF Zhou, Guan-Wei
   Wang, Jiulin
   Gao, Pengfei
   Yang, Xiaowei
   He, Yu-Shi
   Liao, Xiao-Zhen
   Yang, Jun
   Ma, Zi-Feng
TI Facile Spray Drying Route for the Three-Dimensional
   Graphene-Encapsulated Fe2O3 Nanoparticles for Lithium Ion Battery Anodes
SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
LA English
DT Article
ID REDUCED GRAPHENE; ELECTROCHEMICAL PERFORMANCE; COMPOSITE-MATERIALS;
   NEXT-GENERATION; LI-STORAGE; NANOCOMPOSITES; NANOSHEETS; FILMS; OXIDE;
   SUPERCAPACITORS
AB Crumbled graphene sheet-wrapped nano-Fe2O3 (Fe2O3@GS) composites with a three-dimension (3D) hierarchical structure have been made by a facile and efficient spray drying route with a following mild heat reduction in air. In the as-obtained composites, the crumpled GS around Fe2O3 particles could not only provide a 3D conductive matrix but also buffer the volume change of Fe2O3. Fe2O3 particles which evenly distribute in the crumpled GS could also act as spacers to avoid the close restacking of GS. Compared to the bare Fe2O3, the Fe2O3@GS composites as Li ion battery anodes show dramatically improved electrochemical performance including cyclic stability and rate capability owing to the special encapsulated structure and the excellent synergistic effect between the two components.
C1 [Zhou, Guan-Wei; Wang, Jiulin; Gao, Pengfei; He, Yu-Shi; Liao, Xiao-Zhen; Yang, Jun; Ma, Zi-Feng] Shanghai Jiao Tong Univ, Dept Chem Engn, Inst Electrochem & Energy Technol, Shanghai 200240, Peoples R China.
   [Ma, Zi-Feng] Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Shanghai 200240, Peoples R China.
   [Yang, Xiaowei; He, Yu-Shi] Monash Univ, Dept Mat Engn, Clayton, Vic 3800, Australia.
RP He, YS (reprint author), Shanghai Jiao Tong Univ, Dept Chem Engn, Inst Electrochem & Energy Technol, Shanghai 200240, Peoples R China.
EM ys-he@sjtu.edu.cn
RI Yang, Xiaowei/H-1188-2012; Wang, Jiulin/G-2694-2010; 
OI Yang, Xiaowei/0000-0002-4862-7422; He, Yushi/0000-0001-9971-8474
FU National Basic Research Program of China [2007CB209705]; Natural Science
   Foundation of China [21006063, 21073120, 51272156]; Science and
   Technology Commission of Shanghai Municipality [10DZ1202702]; China
   Scholarship Council Fellowship
FX We are grateful for the financial support of this work by the National
   Basic Research Program of China (2007CB209705), the Natural Science
   Foundation of China (21006063, 21073120, 51272156), the Science and
   Technology Commission of Shanghai Municipality (10DZ1202702), and the
   China Scholarship Council Fellowship.
CR Zou YQ, 2011, J PHYS CHEM C, V115, P20747, DOI 10.1021/jp206876t
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NR 52
TC 37
Z9 38
U1 23
U2 253
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0888-5885
J9 IND ENG CHEM RES
JI Ind. Eng. Chem. Res.
PD JAN 23
PY 2013
VL 52
IS 3
BP 1197
EP 1204
DI 10.1021/ie302469b
PG 8
WC Engineering, Chemical
SC Engineering
GA 079AC
UT WOS:000314141500022
ER

PT J
AU Huang, H
   Fang, JW
   Xia, Y
   Tao, XY
   Gan, YP
   Du, J
   Zhu, WJ
   Zhang, WK
AF Huang, Hui
   Fang, Junwu
   Xia, Yang
   Tao, Xinyong
   Gan, Yongping
   Du, Jun
   Zhu, Wenjun
   Zhang, Wenkui
TI Construction of sheet-belt hybrid nanostructures from one-dimensional
   mesoporous TiO2(B) nanobelts and graphene sheets for advanced
   lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID NEGATIVE ELECTRODE MATERIAL; RATE PERFORMANCE; ELECTROCHEMICAL
   PERFORMANCE; STORAGE PROPERTIES; TIO2-B NANOWIRES; ANODE MATERIAL; LI
   STORAGE; OXIDE; NANOSHEETS; INTERCALATION
AB TiO2(B) is considered as a new kind of anode material, and an alternative to graphite, for high-power lithium ion batteries (LIBs) due to its characteristic pseudocapacitive energy storage mechanism. Herein, we firstly report the synthesis of one-dimensional (1D) mesoporous TiO2(B) nanobelts by hydrothermal treatment of commercial TiO2 (P25) powders in NaOH medium. The as-prepared TiO2(B) nanobelts, with typical sizes of 50-100 nm in width and several micrometers in length, have mesopore channels in the range of 10-30 nm. Moreover, we demonstrate the use of graphene as an excellent mini-current collector to in situ construct unique hybrid sheet-belt nanostructures (G-TiO2(B)) to optimize the performance. Such a 1D mesoporous TiO2(B) structure can provide numerous open channels for the electrolyte to access and facilitate the ultrafast diffusion of lithium ions. In addition, the introduced graphene layers will both be favorable for the fast electron transport in the electrode and make a great contribution to the specific capacity. As a consequence, this G-TiO2(B) hybrid can deliver an ultrahigh reversible capacity (over 430 mA h g(-1) at a low current density of 0.15 A g(-1)), and present a superior rate capability (210 mA h g(-1) at 3 A g(-1)).
C1 [Huang, Hui; Fang, Junwu; Xia, Yang; Tao, Xinyong; Gan, Yongping; Du, Jun; Zhu, Wenjun; Zhang, Wenkui] Zhejiang Univ Technol, Coll Chem Engn & Mat Sci, Hangzhou 310014, Zhejiang, Peoples R China.
RP Huang, H (reprint author), Zhejiang Univ Technol, Coll Chem Engn & Mat Sci, Hangzhou 310014, Zhejiang, Peoples R China.
EM msechem@zjut.edu.cn
RI Tao, Xinyong/G-9005-2011
OI Tao, Xinyong/0000-0003-4084-7743
FU National Natural Science Foundation of China [20673100, 51172205,
   51002138]; Natural Science Foundation of Zhejiang Province [Y4110523];
   Qianjiang Project of Zhejiang Province [2010R10029]; New Century
   Excellent Talents in University [NCET 111079]; Program of Potential
   Talents in Zhejiang Province [2011R403058]
FX This work was supported by the National Natural Science Foundation of
   China (20673100 51172205 and 51002138), the Natural Science Foundation
   of Zhejiang Province (Y4110523), Qianjiang Project of Zhejiang Province
   (2010R10029), New Century Excellent Talents in University (NCET 111079)
   and the Program of Potential Talents in Zhejiang Province (2011R403058).
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TC 37
Z9 37
U1 20
U2 176
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 7
BP 2495
EP 2500
DI 10.1039/c2ta00593j
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085VT
UT WOS:000314643100019
ER

PT J
AU Zheng, MB
   Qiu, DF
   Zhao, B
   Ma, LY
   Wang, XR
   Lin, ZX
   Pan, LJ
   Zheng, YD
   Shi, Y
AF Zheng, Mingbo
   Qiu, Danfeng
   Zhao, Bin
   Ma, Luyao
   Wang, Xinran
   Lin, Zixia
   Pan, Lijia
   Zheng, Youdou
   Shi, Yi
TI Mesoporous iron oxide directly anchored on a graphene matrix for
   lithium-ion battery anodes with enhanced strain accommodation
SO RSC ADVANCES
LA English
DT Article
ID REVERSIBLE CAPACITY; CO3O4 NANOPARTICLES; ELECTRODE MATERIALS; STORAGE
   CAPABILITY; REDUCED GRAPHENE; RATE-PERFORMANCE; COMPOSITES; NANOSHEETS;
   NANOTUBES; NANOSTRUCTURES
AB A continuous mesoporous iron oxide nanofilm was directly formed on graphene nanosheets through the in situ thermal decomposition of Fe(NO3)(3)center dot 9H(2)O and was anchored tightly on the graphene surface. The lithiation-induced strain was naturally accommodated, owing to the constraint effect of graphene and the mesoporous structure. Hence, the pulverization of the iron oxide nanofilm was effectively prevented.
C1 [Zheng, Mingbo; Qiu, Danfeng; Zhao, Bin; Ma, Luyao; Wang, Xinran; Lin, Zixia; Pan, Lijia; Zheng, Youdou; Shi, Yi] Nanjing Univ, Sch Elect Sci & Engn, Nanjing Natl Lab Microstruct, Nanjing 210093, Jiangsu, Peoples R China.
RP Zheng, MB (reprint author), Nanjing Univ, Sch Elect Sci & Engn, Nanjing Natl Lab Microstruct, Nanjing 210093, Jiangsu, Peoples R China.
EM yshi@nju.edu.cn
RI Wang, Xinran/E-8392-2010; Ma, Luyao/L-8087-2013; 
OI Pan, Lijia/0000-0002-8917-7843
FU National Natural Science Foundation of China [51202106, 61076017,
   60928009]; Fundamental Research Funds for the Central Universities
   [1127021010]; 973 Project [2013CB932900]
FX We thank Dr Ping He from the National Institute of Advanced Industrial
   Science and Technology of Japan for the electro-chemistry analysis,
   Prof. Runsheng Huang and Dr Wei Liu from Nangjing University for the
   Mossbauer measurement and analysis and Dr Huan Pang from Nangjing
   University for the SEM and TEM measurements. This work was supported by
   the National Natural Science Foundation of China (No. 51202106, 61076017
   and 60928009), the Fundamental Research Funds for the Central
   Universities (No. 1127021010) and 973 Project under grant No.
   2013CB932900.
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NR 50
TC 37
Z9 37
U1 7
U2 109
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2013
VL 3
IS 3
BP 699
EP 703
DI 10.1039/c2ra22702a
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA 052KR
UT WOS:000312197000004
ER

PT J
AU Huang, XD
   Zhou, XF
   Qian, K
   Zhao, DY
   Liu, ZP
   Yu, CZ
AF Huang, Xiaodan
   Zhou, Xufeng
   Qian, Kun
   Zhao, Dongyuan
   Liu, Zhaoping
   Yu, Chengzhong
TI A magnetite nanocrystal/graphene composite as high performance anode for
   lithium-ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Fe3O4; Graphene; Lithium-ion batteries; Solvothermal
ID GRAPHENE; CARBON; ELECTRODES; STORAGE; CAPABILITIES; NANOSHEETS;
   STABILITY; CAPACITY
AB A facile single step solvothermal route has been developed to prepare a composite of Fe3O4 nanoparticles and graphene nanosheets. The synthetic protocol takes advantage of the ethylene glycol assisted partial reduction of Fe3+ species to form Fe3O4, the reduction of graphene oxide into graphene, and the preferential attachment of fine Fe3O4 nanoparticles onto graphene sheets in one step. No additional reductive agent or calcination step is needed, which favors an effective, operationally simple and low-cost preparation process. The cycling properties of Fe3O4/graphene nanocomposite have been evaluated by galvanostatic charge-discharge measurements. The effect of graphene additive ratios on electrochemical performance has been investigated. The results show that the nanocomposite with a moderate graphene content of 18.5 wt% integrates high reversible capacity and good cyclic stability, delivering a capacity of 750 mAh/g after 40 cycles at 50 mA/g. Crown Copyright (C) 2011 Published by Elsevier B. V. All rights reserved.
C1 [Zhou, Xufeng; Liu, Zhaoping] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
   [Huang, Xiaodan; Zhao, Dongyuan; Yu, Chengzhong] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China.
   [Huang, Xiaodan; Qian, Kun; Yu, Chengzhong] Univ Queensland, Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia.
   [Huang, Xiaodan; Qian, Kun; Yu, Chengzhong] Univ Queensland, Australian Inst Bioengn & Nanotechnol, Brisbane, Qld 4072, Australia.
RP Liu, ZP (reprint author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China.
EM iuzp@nimte.ac.cn; c.yu@uq.edu.au
RI Yu, Chengzhong/I-8663-2012; Zhao, Dongyuan/E-5796-2010
FU State Key Research Program of China [2010CB226901]; Australia Research
   Council
FX We thank the State Key Research Program of China (2010CB226901) and the
   Australia Research Council for their financial supports.
CR Wang SQ, 2010, J POWER SOURCES, V195, P5379, DOI 10.1016/j.jpowsour.2010.03.035
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NR 36
TC 37
Z9 38
U1 13
U2 103
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
EI 1873-4669
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD FEB 15
PY 2012
VL 514
BP 76
EP 80
DI 10.1016/j.jallcom.2011.10.087
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 866UR
UT WOS:000298411300013
ER

PT J
AU Chen, TQ
   Pan, LK
   Liu, XJ
   Yu, K
   Sun, Z
AF Chen, Taiqiang
   Pan, Likun
   Liu, Xinjiuan
   Yu, Kai
   Sun, Zhuo
TI One-step synthesis of SnO2-reduced graphene oxide-carbon nanotube
   composites via microwave assistance for lithium ion batteries
SO RSC ADVANCES
LA English
DT Article
ID SENSITIZED SOLAR-CELLS; ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE;
   GRAPHITE OXIDE; HYBRID FILMS; LI-STORAGE; IN-SITU; SUPERCAPACITORS;
   NANOCOMPOSITE; SNO2
AB A facile one-step microwave-assisted method was developed to fabricate SnO2-reduced graphene oxide (RGO)-carbon nanotube (CNT) composites. The as-prepared composites were applied as anode materials for lithium ion batteries and it is found that RGO and CNTs play an important role in the enhancement of the electrochemical performance due to a synergistic effect of SnO2, RGO and CNTs, in which RGO sheets support SnO2 nanoparticles and CNTs act as wires conductively connecting the large RGO sheets together. A SnO2-RGO-CNT composite with 60 wt.% SnO2 achieves a maximum capacity of 502 mA h g(-1) after 50 cycles at 100 mA g(-1) and even at a high current density of 1000 mA g(-1), a capacity of 344 mA h g(-1) is maintained.
C1 [Chen, Taiqiang; Pan, Likun; Liu, Xinjiuan; Yu, Kai; Sun, Zhuo] China Normal Univ, Dept Phys, Minist Educ, Engn Res Ctr Nanophoton & Adv Instrument, Shanghai 200062, Peoples R China.
RP Chen, TQ (reprint author), China Normal Univ, Dept Phys, Minist Educ, Engn Res Ctr Nanophoton & Adv Instrument, Shanghai 200062, Peoples R China.
EM lkpan@phy.ecnu.edu.cn
RI Chen, Taiqiang/I-6611-2013; Pan, Likun/F-7232-2012; Liu,
   Xinjuan/F-2218-2015
OI Pan, Likun/0000-0001-9294-1972; Liu, Xinjuan/0000-0002-3041-6635
FU Special Project for Nanotechnology of Shanghai [11 nm0501200]
FX This work was supported by Special Project for Nanotechnology of
   Shanghai (No. 11 nm0501200).
CR Zhang BA, 2011, CARBON, V49, P4524, DOI 10.1016/j.carbon.2011.06.059
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   Yang ZX, 2011, RSC ADV, V1, P1834, DOI 10.1039/c1ra00500f
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   Ji LW, 2012, RSC ADV, V2, P192, DOI 10.1039/c1ra00676b
   Hong TK, 2010, ACS NANO, V4, P3861, DOI 10.1021/nn100897g
   Zhang M, 2010, J MATER CHEM, V20, P5538, DOI 10.1039/c0jm00638f
   Yan J, 2010, ELECTROCHIM ACTA, V55, P6973, DOI 10.1016/j.electacta.2010.06.081
   Lu XJ, 2011, ELECTROCHIM ACTA, V56, P5115, DOI 10.1016/j.electacta.2011.03.066
   Wu ZS, 2011, ACS NANO, V5, P5463, DOI 10.1021/nn2006249
   Lu T, 2010, ELECTROCHIM ACTA, V55, P4170, DOI 10.1016/j.electacta.2010.02.095
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   Zhao DD, 2011, NANO-MICRO LETT, V3, P62, DOI 10.1007/BF03353653
NR 54
TC 37
Z9 37
U1 22
U2 99
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 31
BP 11719
EP 11724
DI 10.1039/c2ra21740f
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 051SJ
UT WOS:000312147400018
ER

PT J
AU Kang, YR
   Li, YL
   Hou, F
   Wen, YY
   Su, D
AF Kang, Yan-Ru
   Li, Ya-Li
   Hou, Feng
   Wen, Yang-Yang
   Su, Dong
TI Fabrication of electric papers of graphene nanosheet shelled cellulose
   fibres by dispersion and infiltration as flexible electrodes for energy
   storage
SO NANOSCALE
LA English
DT Article
ID LITHIUM-ION BATTERIES; NANOCOMPOSITE PAPER; RAMAN-SPECTROSCOPY; CARBON
   NANOTUBES; CONDUCTIVE PAPER; DEVICES; FILMS; SUPERCAPACITORS; OXIDE
AB An electrically conductive and electrochemically active composite paper of graphene nanosheet (GNS) coated cellulose fibres was fabricated via a simple paper-making process of dispersing chemically synthesized GNS into a cellulose pulp, followed by infiltration. The GNS nanosheet was deposited onto the cellulose fibers, forming a coating, during infiltration. It forms a continuous network through a bridge of interconnected cellulose fibres at small GNS loadings (3.2 wt%). The GNS/cellulose paper is as flexible and mechanically tough as the pure cellulose paper. The electrical measurements show the composite paper has a sheet resistance of 1063 Omega square(-1) and a conductivity of 11.6 S m(-1). The application of the composite paper as a flexible double layer supercapacitor in an organic electrolyte (LiPF6) displays a high capacity of 252 F g(-1) at a current density of 1 A g(-1) with respect to GNS. Moreover, the paper can be used as the anode in a lithium battery, showing distinct charge and discharge performances. The simple process for synthesising the GNS functionalized cellulose papers is attractive for the development of high performance papers for electrical, electrochemical and multifunctional applications.
C1 [Kang, Yan-Ru; Li, Ya-Li; Hou, Feng; Wen, Yang-Yang; Su, Dong] Tianjin Univ, Key Lab Adv Ceram & Machining Technol, Sch Mat Sci & Engn, Minist Educ, Tianjin 300072, Peoples R China.
RP Li, YL (reprint author), Tianjin Univ, Key Lab Adv Ceram & Machining Technol, Sch Mat Sci & Engn, Minist Educ, Weijin Rd 92, Tianjin 300072, Peoples R China.
EM liyali@tju.edu.cn
FU National Basic Research Program of China [2010CB934700]; Chinese
   Ministry of Education [309010]; Key Laboratory of Advanced Ceramics and
   Machining Technology (Tianjin University) Ministry of Education
   [ACMT-2008-03]
FX This work is supported by the National Basic Research Program of China
   (Grant. No. 2010CB934700), and Key Grant Project of Chinese Ministry of
   Education (309010), Fund of Key Laboratory of Advanced Ceramics and
   Machining Technology (Tianjin University) Ministry of Education
   (ACMT-2008-03).
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NR 29
TC 37
Z9 38
U1 22
U2 157
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 10
BP 3248
EP 3253
DI 10.1039/c2nr30318c
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 936QB
UT WOS:000303604000038
PM 22535335
ER

PT J
AU Li, BJ
   Cao, HQ
   Zhang, JX
   Qu, MZ
   Lian, F
   Kong, XH
AF Li, Baojun
   Cao, Huaqiang
   Zhang, Jingxian
   Qu, Meizhen
   Lian, Fang
   Kong, Xianghua
TI SnO2-carbon-RGO heterogeneous electrode materials with enhanced anode
   performances in lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID HOLLOW NANOSPHERES; TIN-NANOPARTICLES; STORAGE CAPACITY; SNO2;
   COMPOSITE; GRAPHENE
AB Anchoring SnO2 NPs encapsulated in carbon shells onto RGO exhibits superior anode performances in lithium ion batteries with specific capacities of 622 mA h g(-1) after 100 cycles.
C1 [Li, Baojun; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Zhang, Jingxian; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
   [Lian, Fang; Kong, Xianghua] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
FU National Natural Science Foundation of China [20921001, 20535020];
   Innovation Method Fund of China [20081885189]; National High Technology
   Research and Development Program of China [2009AA03Z321]; China
   Postdoctoral Science Foundation [20100470302]
FX Financial supports from the National Natural Science Foundation of China
   (no. 20921001 and 20535020), the Innovation Method Fund of China (no.
   20081885189), the National High Technology Research and Development
   Program of China (no. 2009AA03Z321), and the China Postdoctoral Science
   Foundation (no. 20100470302) are acknowledged.
CR Zhang LS, 2010, J MATER CHEM, V20, P5462, DOI 10.1039/c0jm00672f
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NR 37
TC 37
Z9 37
U1 2
U2 41
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 7
BP 2851
EP 2854
DI 10.1039/c2jm13706b
PG 4
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 881RI
UT WOS:000299504200007
ER

PT J
AU Wang, G
   Bai, JT
   Wang, YH
   Ren, ZY
   Bai, JB
AF Wang, Gang
   Bai, Jintao
   Wang, Yuhang
   Ren, Zhaoyu
   Bai, Jinbo
TI Prepartion and electrochemical performance of a cerium oxide-graphene
   nanocomposite as the anode material of a lithium ion battery
SO SCRIPTA MATERIALIA
LA English
DT Article
DE Cerium oxide; Graphene; Nanocomposite; Lithium ion battery;
   Electrochemistry
ID CARBON NANOTUBES; LI STORAGE; SPHEROIDS; PROPERTY
AB A nanocomposite of CeO(2) graphene was prepared by a simple hydrothermal method and its electrochemical properties were investigated as a possible anode material for lithium ion batteries. Morphological characterization revealed that quasi-spherical CeO(2) particles with a size of similar to 100 nm were dispersed randomly on the graphene matrix. The nanocomposite shows a greater capacity for reversal and a better performance rate than a bare CeO(2) electrode. The better electrochemical performance could be attributed to the unique structure of the nanocomposite, which combines the conductive graphene network with dispersed CeO(2) particles. (C) 2011 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
C1 [Bai, Jintao; Ren, Zhaoyu] NW Univ Xian, Inst Photon & Photon Technol, Culture Base,Natl Photoelect Technol & Funct Mat, Natl Key Lab Photoelect Technol & Funct Mat, Xian 710069, Peoples R China.
   [Wang, Gang; Wang, Yuhang] NW Univ Xian, Coll Chem & Mat Sci, Minist Educ, Key Lab Synthet & Nat Funct Mol Chem, Xian 710069, Peoples R China.
   [Bai, Jinbo] Ecole Cent Paris, CNRS UMR 8579, Lab MSS MAT, F-92295 Chatenay Malabry, France.
RP Bai, JT (reprint author), NW Univ Xian, Inst Photon & Photon Technol, Culture Base,Natl Photoelect Technol & Funct Mat, Natl Key Lab Photoelect Technol & Funct Mat, Xian 710069, Peoples R China.
EM jintaobai@sina.cn
RI Bai, Jinbo/F-8552-2010
FU National Natural Science Foundation of China [21061130551, 10974152];
   National Basic Research Program of China (973 Program) [2009CB626611];
   PhD Programs Foundation of Ministry of Education of China
   [20096101110002]; NWU [09YYB04]
FX This project was supported financially by the International Cooperation
   Research Program of the National Natural Science Foundation of China
   (No. 21061130551), the National Basic Research Program of China (973
   Program) (No. 2009CB626611), the PhD Programs Foundation of Ministry of
   Education of China (No. 20096101110002), the National Natural Science
   Foundation of China (No. 10974152) and the NWU Doctorate Dissertation of
   Excellence Funds (No. 09YYB04).
CR Wang SQ, 2010, J POWER SOURCES, V195, P5379, DOI 10.1016/j.jpowsour.2010.03.035
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NR 20
TC 37
Z9 40
U1 7
U2 62
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 1359-6462
J9 SCRIPTA MATER
JI Scr. Mater.
PD AUG
PY 2011
VL 65
IS 4
BP 339
EP 342
DI 10.1016/j.scriptamat.2011.05.001
PG 4
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary;
   Metallurgy & Metallurgical Engineering
SC Science & Technology - Other Topics; Materials Science; Metallurgy &
   Metallurgical Engineering
GA 788LE
UT WOS:000292445600017
ER

PT J
AU XUE, JS
   MYRTLE, K
   DAHN, JR
AF XUE, JS
   MYRTLE, K
   DAHN, JR
TI AN EPOXY-SILANE APPROACH TO PREPARE ANODE MATERIALS FOR RECHARGEABLE
   LITHIUM ION BATTERIES
SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY
LA English
DT Article
ID SILICON; CHEMISTRY
AB A series of carbonaceous materials containing silicon and oxygen have been synthesized via pyrolysis of epoxy-silane composites prepared from hardened mixtures of epoxy novolac resin and epoxy-functional silane. Chemical composition of the pyrolyzed materials has been determined to be C1-y-zSizOy by a combination thermogravimetric analysis, Auger electron spectroscopy, carbon, hydrogen, and nitrogen analyses, and wet chemical analyses. Pyrolysis of the epoxy novolac resin gives pure carbon made up predominantly of single graphene sheets having lateral dimension of about 20 Angstrom which are stacked like a ''house of cards.'' Pyrolysis of the pure epoxy-functional silane gives C0.50Si0.19O0.31 with a glassy structure. X-ray diffraction and electrochemical tests show that pyrolyzed materials prepared from mixtures initially containing less than 50% (by weight) silane are mixtures of the carbon Single-layer phase and the glassy phase, while those initially with greater than 50% silane show predominantly the glassy phase. The reversible specific capacity of these materials increases from about 500 mAh/g for the pure disordered carbon up to about 770 mAh/g in the material which contains the most silicon and oxygen. However, the voltage profile develops hysteresis of about 1 V and the irreversible capacity associated with the first reaction with lithium increases as the silicon and oxygen contents are increased. Further work is needed to eliminate these drawbacks.
RP XUE, JS (reprint author), SIMON FRASER UNIV,DEPT PHYS,BURNABY,BC V5A 1S6,CANADA.
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NR 25
TC 37
Z9 46
U1 3
U2 28
PU ELECTROCHEMICAL SOC INC
PI PENNINGTON
PA 10 SOUTH MAIN STREET, PENNINGTON, NJ 08534
SN 0013-4651
J9 J ELECTROCHEM SOC
JI J. Electrochem. Soc.
PD SEP
PY 1995
VL 142
IS 9
BP 2927
EP 2935
DI 10.1149/1.2048667
PG 9
WC Electrochemistry; Materials Science, Coatings & Films
SC Electrochemistry; Materials Science
GA RV179
UT WOS:A1995RV17900024
ER

PT J
AU Rao, CNR
   Gopalakrishnan, K
   Govindaraj, A
AF Rao, C. N. R.
   Gopalakrishnan, K.
   Govindaraj, A.
TI Synthesis, properties and applications of graphene doped with boron,
   nitrogen and other elements
SO NANO TODAY
LA English
DT Review
DE Graphene; Doped graphene; Borocarbonitride; Supercapacitors; Lithium
   battery; Oxygen reduction reaction
ID CHEMICAL-VAPOR-DEPOSITION; OXYGEN REDUCTION REACTION; LITHIUM-ION
   BATTERIES; HIGH-PERFORMANCE SUPERCAPACITOR; SINGLE-LAYER GRAPHENE; ANODE
   MATERIALS; ELECTROCATALYTIC ACTIVITY; ELECTRONIC-PROPERTIES; CARBON
   NANOMATERIALS; QUANTUM CAPACITANCE
AB Chemical doping of graphene becomes necessary to create a band gap which is useful for various applications. Furthermore, chemical doping of elements like boron and nitrogen in graphene gives rise to useful properties. Since chemically doped graphene is both of academic and technical importance, we have prepared this article on the present status of various aspects of this important class of materials. In doing so, we have covered the recent literature on this subject citing all the major references. Some of the aspects that we have covered are the synthesis of chemically doped graphene followed by properties and applications. The applications discussed relate to gas adsorption, lithium batteries, supercapacitors, oxygen reduction reaction, field emission and photochemical water splitting. Characterization of chemically doped graphene also included. We believe that the article will be useful to all those interested in graphene and related materials and provides the present status of the subject. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Rao, C. N. R.; Gopalakrishnan, K.; Govindaraj, A.] Jawaharlal Nehru Ctr Adv Sci Res, Chem & Phys Mat Unit, Int Ctr Mat Sci, CSIR Ctr Excellence Chem, Bangalore 560064, Karnataka, India.
   [Rao, C. N. R.; Gopalakrishnan, K.; Govindaraj, A.] Jawaharlal Nehru Ctr Adv Sci Res, Sheik Saqr Lab, Bangalore 560064, Karnataka, India.
   [Rao, C. N. R.; Govindaraj, A.] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 566012, Karnataka, India.
RP Rao, CNR (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, Chem & Phys Mat Unit, Int Ctr Mat Sci, CSIR Ctr Excellence Chem, Bangalore 560064, Karnataka, India.
EM cnrrao@jncasr.ac.in
RI Ahirwal, Ashish /F-2532-2013
OI Ahirwal, Ashish /0000-0002-9127-6541
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NR 125
TC 36
Z9 36
U1 69
U2 347
PU ELSEVIER SCI LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
SN 1748-0132
EI 1878-044X
J9 NANO TODAY
JI Nano Today
PD JUN
PY 2014
VL 9
IS 3
BP 324
EP 343
DI 10.1016/j.nantod.2014.04.010
PG 20
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA AO6SE
UT WOS:000341481000008
ER

PT J
AU Yue, WB
   Yang, S
   Ren, Y
   Yang, XJ
AF Yue, Wenbo
   Yang, Sheng
   Ren, Yu
   Yang, Xiaojing
TI In situ growth of Sn, SnO on graphene nanosheets and their application
   as anode materials for lithium-ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; Tin; Tin monoxide; Lithium-ion battery
ID NANOPARTICLES; OXIDE; CAPACITY; PERFORMANCE; STORAGE; CO3O4; MORPHOLOGY;
   ARRAYS; GAS
AB Graphene-based metals or metal oxides commonly show outstanding electrochemical performance due to superior properties of graphene. However, it still remains a challenge to directly grow low-valence oxides (e.g. tin monoxide) on graphene surface in term of the oxidizability of graphene oxide, which is normally adopted as a precursor for graphene. Herein, we report a novel strategy for preparation of tin and tin monoxide on graphene nanosheets by selectively using the reducing agent and the precipitant. Moreover, in contrast to free particles formed in solution, nanoscale tin or tin monoxide particles well-dispersed on graphene exhibited enhanced electro-chemical properties, including higher reversible capacities, better cycle performances, and higher rate capabilities. This facile one-step method may provide an attractive alternative approach for preparation of high-performance electrodes consisting of graphene and low-valence compounds.(C) 2013 Elsevier Ltd. All rights reserved.
C1 [Yue, Wenbo; Yang, Sheng; Yang, Xiaojing] Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China.
   [Ren, Yu] Natl Inst Clean & Low Carbon Energy, Beijing 102209, Peoples R China.
RP Yue, WB (reprint author), Beijing Normal Univ, Coll Chem, 19 Xinjiekou Wai St, Beijing 100875, Peoples R China.
EM wbyue@bnu.edu.cn; yang.xiaojing@bnu.edu.cn
RI Ren, Yu/F-7262-2010
OI Ren, Yu/0000-0001-8572-5489
FU National Natural Science Foundation of China [21101014, 21273022,
   51272030]; Beijing Municipal Natural Science Foundation [2112022]
FX This work is financially supported by National Natural Science
   Foundation of China (21101014, 21273022 and 51272030), Beijing Municipal
   Natural Science Foundation (2112022).
CR Yang S, 2012, RSC ADV, V2, P8827, DOI 10.1039/c2ra20746j
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NR 35
TC 36
Z9 36
U1 19
U2 161
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD MAR 1
PY 2013
VL 92
BP 412
EP 420
DI 10.1016/j.electacta.2013.01.058
PG 9
WC Electrochemistry
SC Electrochemistry
GA 111KL
UT WOS:000316520100053
ER

PT J
AU Li, XF
   Zhong, Y
   Cai, M
   Balogh, MP
   Wang, DN
   Zhang, Y
   Li, RY
   Sun, XL
AF Li, Xifei
   Zhong, Yu
   Cai, Mei
   Balogh, Michael P.
   Wang, Dongniu
   Zhang, Yong
   Li, Ruying
   Sun, Xueliang
TI Tin-alloy heterostructures encapsulated in amorphous carbon nanotubes as
   hybrid anodes in rechargeable lithium ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Sn anode; Volume change; Buffer zone; Cyclic performance; Rate
   capability
ID GRAPHENE NANOSHEETS; RAMAN-SPECTROSCOPY; BINDER-FREE; SECONDARY
   BATTERIES; NEGATIVE ELECTRODE; STORAGE PROPERTIES; COMPOSITE ANODES;
   HOLLOW CARBON; SN; PERFORMANCE
AB Sn anode in rechargeable lithium ion batteries (LIBs) is currently being intensely investigated due to high reversible capacity and energy density as compared to the commercialized graphite anode. However, large volume change upon cycling causes poor cyclic performance, which prevents the practical application of Sn anode in LIBs. In this study, the nanosized MxSn (M = Ni, Fe, and Cr) alloys were encapsulated in amorphous carbon nanotubes (ACNTs) creating hybrid anode heterostructures. The structure of the hybrid anodes was confirmed by X-ray diffraction (XRD), field emission scanning electron microscope (FE-SEM) and high angle dark field scanning transmission electron microscope (HAADF-STEM), and demonstrated that Ni3Sn4, FeSn2, and Cr2Sn3 alloys exist in the hybrid anodes as both nanowires and nanoparticles. The galvanostatic cycling originating from over 330 charge-discharge cycles indicated that encapsulation of Ni3Sn4, FeSn2, and Cr2Sn3 into ACNTs results in surprisingly excellent cycling performance, high rate capability, and increased initial coulombic efficiency (81.4%). Ex situ HAADF-STEM images of anodes after cycles showed that one-dimensional ACNTs as well as electrochemically inactive phase M (Ni, Fe, and Cr) in MxSn function as good matrices, offering "buffer zone" to effectively accommodate the mechanical stress induced by Sn anode expansion and shrinkage. Importantly, ACNTs enable electrical contact of Sn nanoparticles with the current collectors. Therefore, our design can significantly overcome electrochemical degradation of anodes with large volume change, resulting in increased LIB performance. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Li, Xifei; Zhong, Yu; Wang, Dongniu; Zhang, Yong; Li, Ruying; Sun, Xueliang] Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
   [Cai, Mei; Balogh, Michael P.] Gen Motors R&D Ctr, Warren, MI 48090 USA.
RP Sun, XL (reprint author), Univ Western Ontario, Dept Mech & Mat Engn, London, ON N6A 5B9, Canada.
EM xsun@eng.uwo.ca
RI Sun, Andy (Xueliang)/I-4535-2013; Li, Xifei/A-1966-2012; Sun,
   Xueliang/C-7257-2012
OI Li, Xifei/0000-0002-4828-4183; 
FU Natural Science and Engineering Research Council of Canada (NSERC);
   General Motors of Canada; Canada Research Chair (CRC) Program; Canadian
   Foundation for Innovation (CFI); Ontario Research Fund (ORF); Early
   Researcher Award (ERA); University of Western Ontario; Springpower
   International, Inc.; MITACS Elevate Strategic Fellowship Program
FX This research was supported by the Natural Science and Engineering
   Research Council of Canada (NSERC), General Motors of Canada, the Canada
   Research Chair (CRC) Program, Canadian Foundation for Innovation (CFI),
   Ontario Research Fund (ORF), Early Researcher Award (ERA) and the
   University of Western Ontario. X. Li is grateful to Springpower
   International, Inc. and the MITACS Elevate Strategic Fellowship Program.
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   Zhong Y., UNPUB
NR 66
TC 36
Z9 37
U1 16
U2 164
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 1
PY 2013
VL 89
BP 387
EP 393
DI 10.1016/j.electacta.2012.11.097
PG 7
WC Electrochemistry
SC Electrochemistry
GA 098OI
UT WOS:000315558200050
ER

PT J
AU Wang, B
   Li, XL
   Luo, B
   Jia, YY
   Zhi, LJ
AF Wang, Bin
   Li, Xianglong
   Luo, Bin
   Jia, Yuying
   Zhi, Linjie
TI One-dimensional/two-dimensional hybridization for self-supported
   binder-free silicon-based lithium ion battery anodes
SO NANOSCALE
LA English
DT Article
ID NANOSTRUCTURED SILICON; GRAPHENE; NANOWIRES; ELECTRODE; NANOPARTICLES;
   NANOSHEETS; INSERTION; OXIDE; SIZE
AB A unique silicon-based anode for lithium ion batteries is developed via the facile hybridization of one-dimensional silicon nanowires and two-dimensional graphene sheets. The resulting paper-like film holds advantages highly desirable for not only accommodating the volume change of silicon, but also facilitating the fast transport of electron and lithium ions.
C1 [Wang, Bin; Li, Xianglong; Luo, Bin; Jia, Yuying; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Li, XL (reprint author), Natl Ctr Nanosci & Technol, 11 Beiyitiao Zhongguancun, Beijing 100190, Peoples R China.
EM lixl@nanoctr.cn; zhilj@nanoctr.cn
RI Li, Xianglong/A-9010-2010; Luo, Bin/P-7836-2015
OI Li, Xianglong/0000-0002-6200-1178; Luo, Bin/0000-0003-2088-6403
FU National Natural Science Foundation of China [20973044, 21173057,
   21273054]; Ministry of Science and Technology of China [2009DPA41220,
   2012CB933403]; Chinese Academy of Sciences [KJCX2-YW-H21]; Guangdong-CAS
   strategic cooperation Program [2009B091300007]
FX Financial support from the National Natural Science Foundation of China
   (Grant no. 20973044, 21173057, 21273054), the Ministry of Science and
   Technology of China (no. 2009DPA41220 and no. 2012CB933403), the Chinese
   Academy of Sciences (no. KJCX2-YW-H21), and the Guangdong-CAS strategic
   cooperation Program (2009B091300007) is acknowledged. The authors also
   acknowledge kind help of Dr S. T. Picraux at Los Alamos National
   Laboratory.
CR Zhou XS, 2012, ADV ENERGY MATER, V2, P1086, DOI 10.1002/aenm.201200158
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NR 32
TC 36
Z9 36
U1 10
U2 124
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2013
VL 5
IS 4
BP 1470
EP 1474
DI 10.1039/c3nr33288h
PG 5
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 083PM
UT WOS:000314477300026
PM 23334474
ER

PT J
AU Lu, Y
   Wang, XL
   Mai, YJ
   Xiang, JY
   Zhang, H
   Li, L
   Gu, CD
   Tu, JP
   Mao, SX
AF Lu, Yi
   Wang, Xiuli
   Mai, Yongjin
   Xiang, Jiayuan
   Zhang, Heng
   Li, Lu
   Gu, Changdong
   Tu, Jiangping
   Mao, Scott X.
TI Ni2P/Graphene Sheets as Anode Materials with Enhanced Electrochemical
   Properties versus Lithium
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID LI-ION BATTERIES; NEGATIVE-ELECTRODE; HIGH-CAPACITY; REVERSIBLE
   CAPACITY; NI2P NANOPARTICLES; NICKEL PHOSPHIDE; METAL PHOSPHIDE;
   PERFORMANCE; STORAGE; CARBON
AB Hybridizing Ni2P/graphene sheet composite is successfully accomplished via a one-pot solvothermal method. As anode materials for lithium-ion batteries, the Ni2P spheres with sizes of 10-30 nm can effectively prevent the agglomeration of graphene sheets. In turn, the graphene sheets with good electrical conductivity serve as a conducting network for fast electron transfer between the active materials and charge collector, as well as buffered spaces to accommodate the volume expansion/contraction during cycling. The cyclic stability and rate capability of Ni2P are significantly improved after the incorporation of graphene sheets. After 50 cycles, the Ni2P/graphene sheet hybrid delivers a capacity of 450 mA h g(-1) and 360 mA h g(-1) at a current density of 54.2 and 542 mA g(-1), respectively. The voltage hysteresis of Ni2P with and without graphene sheets is also discussed. The incorporation of graphene sheets can partly decrease the voltage polarization, and modify the thickness of solid electrolyte interface (SEI) film.
C1 [Lu, Yi; Wang, Xiuli; Mai, Yongjin; Zhang, Heng; Li, Lu; Gu, Changdong; Tu, Jiangping] Zhejiang Univ, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
   [Lu, Yi; Wang, Xiuli; Mai, Yongjin; Zhang, Heng; Li, Lu; Gu, Changdong; Tu, Jiangping] Zhejiang Univ, Dept Mat Sci & Engn, Hangzhou 310027, Peoples R China.
   [Xiang, Jiayuan] Narada Power Source Co Ltd, Hangzhou 311105, Zhejiang, Peoples R China.
   [Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA.
RP Wang, XL (reprint author), Zhejiang Univ, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, State Key Lab Silicon Mat, Hangzhou 310027, Peoples R China.
EM wangxl@zju.edu.cn; tujp@zju.edu.cn
FU National Natural Science Foundation of China [51271169]; Fundamental
   Research Funds for the Central Universities [2011QNA4006]; Key Science
   and Technology Innovation Team of Zhejiang Province [2010R50013]
FX This work was supported by the National Natural Science Foundation of
   China (51271169), Fundamental Research Funds for the Central
   Universities (2011QNA4006), and Key Science and Technology Innovation
   Team of Zhejiang Province (2010R50013). The authors also thank Dr. Li'na
   Wang, Mr. Wei Huang, and Xinting Cong for help in operating the TEM.
CR Zafiropoulou I, 2010, J PHYS CHEM C, V114, P7582, DOI 10.1021/jp910160g
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NR 51
TC 36
Z9 36
U1 22
U2 131
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD OCT 25
PY 2012
VL 116
IS 42
BP 22217
EP 22225
DI 10.1021/jp3073987
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 024PL
UT WOS:000310121000013
ER

PT J
AU Wan, DY
   Yang, CY
   Lin, TQ
   Tang, YF
   Zhou, M
   Zhong, YJ
   Huang, FQ
   Lin, JH
AF Wan, Dongyun
   Yang, Chongyin
   Lin, Tianquan
   Tang, Yufeng
   Zhou, Mi
   Zhong, Yajuan
   Huang, Fuqiang
   Lin, Jianhua
TI Low-Temperature Aluminum Reduction of Graphene Oxide, Electrical
   Properties, Surface Wettability, and Energy Storage Applications
SO ACS NANO
LA English
DT Article
DE graphene oxide; Al reduction; surface wettability; thermal energy
   storage; lithium ion battery
ID GRAPHITE OXIDE; TRANSPARENT CONDUCTORS; RAMAN-SPECTRA; SHEETS; CARBON;
   FILMS; FUNCTIONALIZATION; LAYERS
AB Low-temperature aluminum (Al) reduction is first introduced to reduce graphene oxide (GO) at 100-200 degrees C in a two-zone furnace. The melted Al metal exhibits an excellent deoxygen ability to produce well-crystallized reduced graphene oxide (RGO) papers with a low O/C ratio of 0.058 (Al-RGO), compared with 0.201 in the thermally reduced one (T-RGO). The Al-RGO papers possess outstanding mechanical flexibility and extremely high electrical conductivities sheet resistance R-s similar to 1.75 Omega/sq), compared with 20.12 Omega/sq of T-RGO. More interestingly, very nice hydrophobic nature (90.5 degrees) was observed, significantly superior to the reported chemically or thermally reduced papers. These enhanced properties are attributed to the low oxygen content in the RGO papers. During the aluminum reduction, highly active H atoms from H2O reacted with melted Al promise an efficient oxygen removal. This method was also applicable to reduce graphene oxide foams, which were used in the G0/SA (stearic acid) composite as a highly thermally conductive reservoir to hold the phase change material for thermal energy storage. The Al-reduced RGO/SnS2 composites were further used in an anode material of lithium ion batteries possessing a higher specific capacity. Overall, low-temperature Al reduction is an effective method to prepare highly conductive RGO papers and related composites for flexible energy conversion and storage device applications.
C1 [Wan, Dongyun; Yang, Chongyin; Lin, Tianquan; Tang, Yufeng; Zhou, Mi; Zhong, Yajuan; Huang, Fuqiang] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China.
   [Huang, Fuqiang; Lin, Jianhua] Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China.
RP Huang, FQ (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China.
EM huangfq@mail.sic.ac.cn; jhlin@pku.edu.cn
RI Lin, Tianquan/I-3030-2012
FU National 973 and 863 Program of China [2009CB939903, 2011AA050505]; NSF
   of China [11274328, 51125006, 91122034, 51121064, 51102263, 21101164,
   61076062]; NSF of Shanghai [11ZR1441900]; STC of Shanghai [10JC1415800]
FX Financial support from National 973 and 863 Program of China Grant Nos.
   2009CB939903 and 2011AA050505, NSF of China Grant Nos. 11274328,
   51125006, 91122034, 51121064, 51102263, 21101164, and 61076062, NSF of
   Shanghai Grant No. 11ZR1441900, and STC of Shanghai Grant No.
   10JC1415800 is acknowledged.
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NR 43
TC 36
Z9 36
U1 20
U2 215
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
J9 ACS NANO
JI ACS Nano
PD OCT
PY 2012
VL 6
IS 10
BP 9068
EP 9078
DI 10.1021/nn303228r
PG 11
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 024FW
UT WOS:000310096100067
PM 22984901
ER

PT J
AU Yue, YH
   Han, PX
   He, X
   Zhang, KJ
   Liu, ZH
   Zhang, CJ
   Dong, SM
   Gu, L
   Cui, GL
AF Yue, Yanhua
   Han, Pengxian
   He, Xiang
   Zhang, Kejun
   Liu, Zhihong
   Zhang, Chuanjian
   Dong, Shanmu
   Gu, Lin
   Cui, Guanglei
TI In situ synthesis of a graphene/titanium nitride hybrid material with
   highly improved performance for lithium storage
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID LI-ION BATTERIES; TITANIUM NITRIDE; CARBON NANOTUBES; ANODE MATERIALS;
   FILMS; TIN; NANOPARTICLES; NANOSHEETS; CAPACITY
AB A graphene/titanium nitride (G/TiN) hybrid as an anode material of lithium ion batteries is prepared by a simple in situ hydrolysis method combined with ammonia annealing. TiN nanoparticles as obtained are similar to 5 nm in size and homogeneously anchored on G. The G/TiN hybrid anode delivers a reversible capacity as high as 646 mA h g(-1) at 20 mA g(-1) and exhibits an enhanced initial coulombic efficiency of 75%, much higher than that of pure graphene (G: 52%) in the first cycle. The capacity retention is as much as 86% after 200 cycles. At a current density of 2000 mA g(-1), the hybrid anode still retains 325 mA h g(-1) while that of G is only 98 mA h g(-1). It is demonstrated that the G/TiN hybrids display a superior electrochemical performance owing to the highly efficient mixed (electron and Li+) conducting network. The internal defects between G layers induced by nitrogen-doping in G/TiN may improve reversible Li storage, whereas the catalytic sites on the surface of G related to the decomposition of the electrolyte may be occupied by TiN, leading to a decreased irreversible capacity. Moreover, the formation of Li3N in the interface is beneficial to interface transport, which is confirmed by aberration-corrected scanning transmission electron microscopy. The anchoring of TiN nanoparticles on G is promising prospect for energy storage applications in high performance lithium-ion batteries.
C1 [He, Xiang; Gu, Lin] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
   [Yue, Yanhua; Han, Pengxian; Zhang, Kejun; Liu, Zhihong; Zhang, Chuanjian; Dong, Shanmu; Cui, Guanglei] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
RP Gu, L (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
EM l.gu@iphy.ac.cn; cuigl@qibebt.ac.cn
RI Cui, Guanglei/D-4816-2011; Han, Pengxian/D-6159-2011; Gu,
   Lin/D-9631-2011
OI Gu, Lin/0000-0002-7504-031X
FU Chinese Academy of Sciences; National Key Basic Research Program of
   China [2011CB935700]; Shandong Province Funds for Distinguished Young
   Scientist [JQ200906]; National Natural Science Foundation of China
   [20971077]
FX We appreciate the support of the "100 Talents" program of the Chinese
   Academy of Sciences, National Key Basic Research Program of China (Grant
   No. 2011CB935700), Shandong Province Funds for Distinguished Young
   Scientist (Grant No. JQ200906) and National Natural Science Foundation
   of China (Grant No. 20971077).
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Z9 37
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U2 111
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
EI 1364-5501
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 11
BP 4938
EP 4943
DI 10.1039/c2jm16128a
PG 6
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 896MP
UT WOS:000300571400057
ER

PT J
AU Kong, DB
   He, HY
   Song, Q
   Wang, B
   Lv, W
   Yang, QH
   Zhi, LJ
AF Kong, Debin
   He, Haiyong
   Song, Qi
   Wang, Bin
   Lv, Wei
   Yang, Quan-Hong
   Zhi, Linjie
TI Rational design of MoS2@graphene nanocables: towards high performance
   electrode materials for Lithium ion batteries
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Article
ID MOLYBDENUM-DISULFIDE MOS2; STORAGE PROPERTIES; ENERGY-CONVERSION; FACILE
   SYNTHESIS; ANODE MATERIALS; HIGH-CAPACITY; BINDER-FREE; THIN-FILM;
   NANOCOMPOSITES; NANOSHEETS
AB Here, we have successfully developed a novel contact mode between MoS2 and graphene, where graphene rolls up into a hollow nanotube and thin MoS2 nanosheets are uniformly standing on the inner surface of graphitic nanotubes, thus forming mechanically robust, freestanding, interwoven MoS2@graphene nanocable webs (MoS2@G). Such a hybrid structure can maximize the MoS2 loading in the electrode in which over 90% of MoS2 nanosheets with stacked layer number of less than 5 can be installed. Remarkably, when calculated on the basis of the whole electrode, this binder free electrode not only shows high specific capacity (ca. 1150 mA h g(-1)) and excellent cycling performance (almost 100% capacity retention even after 160 cycles at a current density of 0.5 A g(-1)) but exhibits a surprisingly high-rate capability of 700 mA h g(-1) at the rate of 10 A g(-1) despite such a high MoS2 loading content, which is one of the best results of MoS2-based electrode materials ever reported thus far.
C1 [Kong, Debin; Yang, Quan-Hong; Zhi, Linjie] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
   [Kong, Debin; He, Haiyong; Song, Qi; Wang, Bin; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
   [Kong, Debin; Lv, Wei; Yang, Quan-Hong; Zhi, Linjie] Synergist Innovat Ctr Chem & Chem Engn Tianjin, Tianjin 300072, Peoples R China.
RP Kong, DB (reprint author), Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China.
EM qhyangcn@tju.edu.cn; zhilj@nanoctr.cn
RI Lv, Wei/M-1964-2013
OI Lv, Wei/0000-0003-0874-3477
FU Ministry of Science and Technology of China [2012CB933403,
   2014CB932403]; National Natural Science Foundation of China [20973044,
   21173057, 51372167]; Chinese Academy of Sciences
FX The authors would like to thank Bin Luo and Lin Shi for their help and
   discussions and the financial support from the Ministry of Science and
   Technology of China (nos 2012CB933403 and 2014CB932403), the National
   Natural Science Foundation of China (Grant nos 20973044, 21173057 and
   51372167), and the Chinese Academy of Sciences.
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NR 49
TC 35
Z9 35
U1 35
U2 170
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PD OCT
PY 2014
VL 7
IS 10
BP 3320
EP 3325
DI 10.1039/c4ee02211d
PG 6
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA AQ5YK
UT WOS:000342884300014
ER

PT J
AU Liu, YC
   Zhao, YP
   Jiao, LF
   Chen, J
AF Liu, Yongchang
   Zhao, Yanping
   Jiao, Lifang
   Chen, Jun
TI A graphene-like MoS2/graphene nanocomposite as a highperformance anode
   for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID METAL DICHALCOGENIDE NANOSHEETS; MOLYBDENUM-DISULFIDE MOS2; STORAGE
   PROPERTIES; MOS2-GRAPHENE COMPOSITES; ASSISTED SYNTHESIS; PERFORMANCE;
   NANOPARTICLES; MICROSPHERES; SULFUR; FILMS
AB In this article, we report on the preparation of a graphene-like MoS2/graphene nanocomposite by hydrolysis of lithiated MoS2 (LiMoS2) and its application as the anode material for lithium ion batteries. When the mass ratio of graphene/LiMoS2 is 15/100, the obtained composite (MoS2/GNS-15) displays a flower-like architecture composed of exfoliated nanosheets. The structure analyses further demonstrate that graphene-like MoS2 is supported on the surface of graphene nanosheets (GNS) and some of the interlayer spacings of MoS2 are enlarged with the intercalation of graphene. The reversible capacity of the MoS2/GNS-15 nanocomposite is similar to 1400mA h g(-1) in the initial cycle and remains 1351 mA h g(-1) after 200 cycles at 100 mA g(-1). Furthermore, the capacity can reach 591 mA h g(-1) even at a high current density of 1000 mA g(-1). The excellent electrochemical performance of MoS2/GNS-15 is due to the synergetic effect between highly conductive GNS and graphene-like MoS2. On one hand, the GNS matrix can offer two-dimensional conductive networks and effectively suppress the aggregation of layered MoS2 during the lithiation/delithiation process. On the other hand, graphene-like MoS2 with an enlarged gallery can ensure the flooding of the electrolyte, provide more active sites and tower the diffusion energy barrier of Li+ ions.
C1 [Liu, Yongchang; Zhao, Yanping; Jiao, Lifang; Chen, Jun] Nankai Univ, Collaborat Innovat Ctr Chem Sci & Engn, Coll Chem, Key Lab Adv Energy Mat Chem MOE, Tianjin 300071, Peoples R China.
RP Jiao, LF (reprint author), Nankai Univ, Collaborat Innovat Ctr Chem Sci & Engn, Coll Chem, Key Lab Adv Energy Mat Chem MOE, Tianjin 300071, Peoples R China.
EM jiaolf@nankai.edu.cn
RI Chen, Jun/D-4873-2016; Jiao(焦), Lifang(丽芳)/G-4953-2015
FU programs of National 973 [2011CB935900]; NSFC [51231003]; MOE [B12015,
   113016A, IRT-13R30]
FX This work was financially supported by the programs of National 973
   (2011CB935900), NSFC (51231003) and MOE (B12015, 113016A and IRT-13R30).
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NR 51
TC 35
Z9 35
U1 45
U2 260
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PD AUG 28
PY 2014
VL 2
IS 32
BP 13109
EP 13115
DI 10.1039/c4ta01644k
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AN1MJ
UT WOS:000340347700060
ER

PT J
AU Wang, HL
   Xu, ZW
   Li, Z
   Cui, K
   Ding, J
   Kohandehghan, A
   Tan, XH
   Zahiri, B
   Olsen, BC
   Holt, CMB
   Mitlin, D
AF Wang, Huanlei
   Xu, Zhanwei
   Li, Zhi
   Cui, Kai
   Ding, Jia
   Kohandehghan, Alireza
   Tan, Xuehai
   Zahiri, Benjamin
   Olsen, Brian C.
   Holt, Chris M. B.
   Mitlin, David
TI Hybrid Device Employing Three-Dimensional Arrays of MnO in Carbon
   Nanosheets Bridges Battery-Supercapacitor Divide
SO NANO LETTERS
LA English
DT Article
DE Energy storage; anode; Li-ion capacitor; 3D arrays; MnO; hybrid device
ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; ANODE MATERIALS;
   ELECTRODE MATERIALS; FACILE SYNTHESIS; PERFORMANCE; GRAPHENE; LI;
   CAPACITORS; NANOTUBES
AB It is a challenge to meld the energy of secondary batteries with the power of supercapacitors. Herein, we created electrodes finely tuned for this purpose, consisting of a monolayer of MnO nanocrystallites mechanically anchored by pore-surface terminations of 3D arrays of graphene-like carbon nanosheets ("3D-MnO/CNS"). The biomass-derived carbon nanosheets should offer a synthesis cost advantage over comparably performing designer nanocarbons, such as graphene or carbon nanotubes. High Li storage capacity is achieved by bulk conversion and intercalation reactions, while high rates are maintained through-stable similar to 20 nm scale diffusion distances. For example, 1332 mAh g(-1) is reached at 0.1 A g(-1), 567 mAh CI at 5 A g(-1), and 285 mAh g(-1) at 20 A g(-1) with negligible degradation at 500 cycles. We employed 3D-MnO/CNS (anode) and carbon nanosheets (cathode) to create a hybrid capacitor displaying among the most promising performances reported: based on the active materials, it delivers 184 Wh kg(-1) at 83 W kg(-1)and 90 Wh kg(-1) at 15 000 W kg(-1) with 76% capacity retention after 5000 cycles.
C1 [Wang, Huanlei; Xu, Zhanwei; Li, Zhi; Ding, Jia; Kohandehghan, Alireza; Tan, Xuehai; Zahiri, Benjamin; Olsen, Brian C.; Holt, Chris M. B.; Mitlin, David] Univ Alberta, Edmonton, AB T6G 2V4, Canada.
   [Wang, Huanlei; Xu, Zhanwei; Li, Zhi; Cui, Kai; Ding, Jia; Kohandehghan, Alireza; Tan, Xuehai; Zahiri, Benjamin; Olsen, Brian C.; Holt, Chris M. B.; Mitlin, David] Natl Res Council Canada, Natl Inst Nanotechnol NINT, Edmonton, AB T6G 2M9, Canada.
   [Wang, Huanlei] Ocean Univ China, Inst Mat Sci & Engn, Qingdao 266100, Peoples R China.
RP Li, Z (reprint author), Univ Alberta, Edmonton, AB T6G 2V4, Canada.
EM lizhicn@gmail.com; dmitlin@ualberta.ca
RI Wang, Huanlei/F-2061-2013; Li, Zhi/H-3377-2011; 
OI Li, Zhi/0000-0003-1668-4948; Olsen, Brian/0000-0001-9758-3641
FU AITF; NINT NRC
FX This work was supported by AITF and NINT NRC.
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NR 63
TC 35
Z9 35
U1 63
U2 374
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD APR
PY 2014
VL 14
IS 4
BP 1987
EP 1994
DI 10.1021/nl500011d
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AF2WE
UT WOS:000334572400047
PM 24617337
ER

PT J
AU Park, SK
   Jin, A
   Yu, SH
   Ha, J
   Jang, B
   Bong, S
   Woo, S
   Sung, YE
   Piao, Y
AF Park, Seung-Keun
   Jin, Aihua
   Yu, Seung-Ho
   Ha, Jeonghyun
   Jang, Byungchul
   Bong, Sungyool
   Woo, Seunghee
   Sung, Yung-Eun
   Piao, Yuanzhe
TI In Situ Hydrothermal Synthesis of Mn3O4 Nanoparticles on Nitrogen-doped
   Graphene as High-Performance Anode materials for Lithium Ion Batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE lithium ion battery; anode; manganese oxide; graphene; doping
ID IMPROVED REVERSIBLE CAPACITY; ELECTROCHEMICAL PERFORMANCE; SYNERGISTIC
   CATALYST; CO3O4 NANOCRYSTALS; STORAGE PROPERTIES; CYCLIC STABILITY;
   FACILE; COMPOSITES; NANOSHEETS; HYBRID
AB Developing new electrode materials with high specific capacity for excellent lithium ion storage properties is very desirable. In this paper, we introduce a simple hydrothermal method for the growth of Mn3O4 nanoparticles onto nitrogen-doped graphene (N-doped graphene) for high-performance lithium ion battery (LIB) anodes. Hydrazine plays a fundamental role in the formation of such nanostructures as it can act both as a reducing agent and as a nitrogen source. In the synthesized composite, highly crystalline Mn3O4 nanoparticles with average sizes of 20-50 nm are homogeneously dispersed on both sides of the N-doped graphene. The nitrogen content in the doped graphene is confirmed by elemental analyzer, and 2 wt% of the sample is found to be composed of nitrogen element. The as-prepared Mn3O4/N-doped graphene composites exhibit remarkable electrochemical performance, including high reversible specific capacity, outstanding cycling stability, and excellent rate capability (approximately 400 mA h g(-1) at 2.0 A g(-1)) when used as the anode material for LIBs. The improvement in the electrochemical properties of the material can be attributed to graphene, which acts as both an electron conductor and a volume buffer layer, and nitrogen doping allows for fast electron and ion transfer by decreasing the energy barrier. This type of metal oxide/N-doped graphene composites can be promising candidates for high-performance anode materials for LIBs. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Park, Seung-Keun; Ha, Jeonghyun; Jang, Byungchul; Bong, Sungyool; Piao, Yuanzhe] Seoul Natl Univ, Grad Sch Convergence Sci & Technol, Program Nano Sci & Technol, Suwon 443270, South Korea.
   [Jin, Aihua; Yu, Seung-Ho; Sung, Yung-Eun] Seoul Natl Univ, Ctr Nanoparticle Res, Inst Basic Sci, Seoul 151744, South Korea.
   [Jin, Aihua; Yu, Seung-Ho; Sung, Yung-Eun] Seoul Natl Univ, Sch Chem & Biol Engn, Seoul 151744, South Korea.
   [Yu, Seung-Ho] Seoul Natl Univ, RIAM, Seoul 151742, South Korea.
   [Bong, Sungyool; Piao, Yuanzhe] Adv Inst Convergence Technol, Suwon 443270, Gyeonggi Do, South Korea.
   [Woo, Seunghee] Seoul Natl Univ, Dept Chem, Seoul 151747, South Korea.
RP Sung, YE (reprint author), Seoul Natl Univ, Ctr Nanoparticle Res, Inst Basic Sci, Seoul 151744, South Korea.
EM ysung@snu.ac.kr; parkat9@snu.ac.kr
FU Center for Integrated Smart Sensors; Ministry of Science, ICT & Future
   Planning as Global Frontier Project [CISS-2012M3A6A6054193]; Basic
   Science Research Program through the National Research Foundation of
   Korea (NRF); Ministry of Science, ICT & Future Planning [2013-053595];
   Korean Ministry of Education, Science, and Technology through Institute
   of Basic Science (IBS) program
FX Y. P. acknowledges This work was supported by the Center for Integrated
   Smart Sensors funded by the Ministry of Science, ICT & Future Planning
   as Global Frontier Project (CISS-2012M3A6A6054193) and partial support
   from the Basic Science Research Program through the National Research
   Foundation of Korea (NRF) funded by the Ministry of Science, ICT &
   Future Planning (no. 2013-053595). Y. -E. S. acknowledges financial
   support by the Korean Ministry of Education, Science, and Technology
   through Institute of Basic Science (IBS) program.
CR Bai ZC, 2013, NANOSCALE, V5, P2442, DOI 10.1039/c3nr33211j
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NR 48
TC 35
Z9 35
U1 29
U2 161
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 20
PY 2014
VL 120
BP 452
EP 459
DI 10.1016/j.electacta.2013.12.018
PG 8
WC Electrochemistry
SC Electrochemistry
GA AE2BL
UT WOS:000333778200057
ER

PT J
AU Zhu, YQ
   Guo, HZ
   Wu, Y
   Cao, CB
   Tao, S
   Wu, ZY
AF Zhu, Youqi
   Guo, Huizi
   Wu, Yu
   Cao, Chuanbao
   Tao, Shi
   Wu, Ziyu
TI Surface-enabled superior lithium storage of high-quality ultrathin NiO
   nanosheets
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ION BATTERIES; HIGH-CAPACITY; PERFORMANCE; ELECTRODES; ANODE;
   SUPERCAPACITORS; MICROSPHERES; GRAPHENE; DYNAMICS; HYBRID
AB Two-dimensional nanomaterials hold great potential for next-generation energy storage and conversion devices. Here, we report a large-scale synthesis of high-quality ultrathin NiO nanosheets. The well-defined nanosheets show a graphene-like morphology with large planar area, ultrathin thickness (<2 nm), and high percentage of surface atoms. In comparison with the bulk material, the NiO nanosheets exhibit unique surface and electronic structure with considerable under-coordinated surface nickel atoms and crystal lattice volume expansion. The detected local coordination geometry and the electronic states endow the ultrathin NiO nanosheets with great potential in surface-dependent electrochemical reactions and catalytic processes. When used as anode materials for lithium-ion batteries, the ultrathin NiO nanosheets exhibit a high reversible lithium storage capacity of 715.2 mA h g(-1) at 200 mA g(-1) current density in 130 cycles with an excellent cycling stability and rate capability. In particular, the large-area ultrathin 2D nanostructure can shorten lithium ion diffusion paths and provide a large exposed surface for more lithium-insertion channels. The large-scale and cost-efficient synthesis and the excellent electrochemical performance highlight the high-quality ultrathin 2D NiO nanosheets as a competitive anode material for lithium-ion batteries.
C1 [Zhu, Youqi; Guo, Huizi; Wu, Yu; Cao, Chuanbao] Beijing Inst Technol, Res Ctr Mat Sci, Beijing 100081, Peoples R China.
   [Tao, Shi; Wu, Ziyu] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China.
RP Cao, CB (reprint author), Beijing Inst Technol, Res Ctr Mat Sci, Beijing 100081, Peoples R China.
EM cbcao@bit.edu.cn
RI Cao, Chuanbao/J-5396-2013
OI Cao, Chuanbao/0000-0003-2830-4383
FU National Natural Science Foundation of China [50972017, 21371023];
   Research Fund for the Doctoral Program of Higher Education of China
   [20101101110026]
FX This work was financially supported by the National Natural Science
   Foundation of China (Grant no. 50972017 and 21371023) and Research Fund
   for the Doctoral Program of Higher Education of China (Grant no.
   20101101110026).
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NR 51
TC 35
Z9 35
U1 21
U2 81
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 21
BP 7904
EP 7911
DI 10.1039/c4ta00257a
PG 8
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AH2AW
UT WOS:000335924100038
ER

PT J
AU Chen, SQ
   Bao, P
   Wan, GX
AF Chen, Shuangqiang
   Bao, Peite
   Wan, Guoxiu
TI Synthesis of Fe2O3-CNT-graphene hybrid materials with an open
   three-dimensional nanostructure for high capacity lithium storage
SO NANO ENERGY
LA English
DT Article
DE Bamboo-like carbon nanotubes; Fe2O3 nanorings; Graphene nanosheets;
   Chemical vapor deposition; Lithium ion battery
ID LI-ION BATTERIES; ANODE MATERIAL; ALPHA-FE2O3 NANOTUBES; GRAPHENE
   NANOSHEETS; GAS SENSORS; CARBON; COMPOSITE; PERFORMANCE; OXIDE;
   CHALLENGES
AB Fe2O3-CNT-graphene nanosheet (Fe2O3-CNT-GNS) hybrid materials were synthesized using a chemical vapor deposition method. The as-prepared materials consist of Fe2O3 nanorings, bamboo-like carbon nanotubes and graphene nanosheets, which form an open three-dimensional architecture. For the first time, we observed the growth of bamboo-like carbon nanotubes with open tips, which were catalyzed by iron nanorings. When applied as anode materials in lithium ion batteries, the Fe2O3-CNT-GNS hybrid materials exhibited a high specific capacity of 984 mAh g(-1) with a superior cycling stability and high rate capability. This could be ascribed to short Li+ diffusion path of bamboo-like CNTs, more active reaction sites provided by graphene layers inside CNTs, flexible and highly conductive graphene nanosheets, and an open three-dimensional structure. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Chen, Shuangqiang; Wan, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
   [Bao, Peite] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
RP Wan, GX (reprint author), Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
EM Guoxiu.Wang@uts.edu.au
RI Chen, Shuangqiang/F-5289-2013
FU Australian Research Council (ARC) [DP1093855]; Chinese Scholarship
   Council (CSC)
FX This project is financially supported by the Australian Research Council
   (ARC) through the ARC Discovery project (DP1093855). The author
   Shuangqiang Chen gratefully acknowledges the support from the Chinese
   Scholarship Council (CSC).
CR Zou YQ, 2011, J PHYS CHEM C, V115, P20747, DOI 10.1021/jp206876t
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NR 48
TC 35
Z9 35
U1 34
U2 273
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAY
PY 2013
VL 2
IS 3
BP 425
EP 434
DI 10.1016/j.nanoen.2012.11.012
PG 10
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 156TA
UT WOS:000319845600017
ER

PT J
AU Qi, Y
   Zhang, H
   Du, N
   Yang, DR
AF Qi, Yue
   Zhang, Hui
   Du, Ning
   Yang, Deren
TI Highly loaded CoO/graphene nanocomposites as lithium-ion anodes with
   superior reversible capacity
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-RATE CAPABILITIES; GRAPHENE NANOSHEETS; HIGH-PERFORMANCE; CO3O4
   NANOPARTICLES; LI STORAGE; BATTERIES; COMPOSITES; COBALT; ARRAYS; PHASE
AB This paper reports a facile approach for the synthesis of highly loaded CoO/graphene nanocomposites in an oil-phase solution with Co(acac)(3) as the cobalt precursor. Based on a thermal decomposition process, octahedral CoO nanocrystals (NCs) with a high density were homogeneously anchored onto the graphene nanosheets. These as-prepared graphene based nanocomposites with a high loading of CoO NCs exhibited superior electrochemical properties as anode materials for lithium-ion batteries, including a large reversible capacity, excellent cyclic performance, and high rate capability. Their robust composite structures, large quantity of accessible active sites, and synergistic effects between CoO NCs and graphene may be responsible for the substantially enhanced performance.
C1 [Qi, Yue; Zhang, Hui; Du, Ning; Yang, Deren] Zhejiang Univ, Dept Mat Sci & Engn, Cyrus Tang Ctr Sensor Mat & Applicat, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
RP Qi, Y (reprint author), Zhejiang Univ, Dept Mat Sci & Engn, Cyrus Tang Ctr Sensor Mat & Applicat, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
EM meszhanghui@zju.edu.cn
RI yang, deren/J-3311-2012; Zhang, Hui/E-8915-2012
OI yang, deren/0000-0002-1745-2105; 
FU 863 Project [2011AA050517]; NSFC [51002133]; Innovation Team Project of
   Zhejiang Province [2009R50005]
FX The authors appreciate the financial support from the 863 Project (no.
   2011AA050517), NSFC (no. 51002133) and Innovation Team Project of
   Zhejiang Province (2009R50005).
CR Sun YM, 2012, J PHYS CHEM C, V116, P20794, DOI 10.1021/jp3070147
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NR 31
TC 35
Z9 35
U1 11
U2 114
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 6
BP 2337
EP 2342
DI 10.1039/c2ta00929c
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 085VP
UT WOS:000314642700049
ER

PT J
AU Song, HW
   Li, N
   Cui, H
   Wang, CX
AF Song, Huawei
   Li, Na
   Cui, Hao
   Wang, Chengxin
TI Enhanced capability and cyclability of SnO2-graphene oxide hybrid anode
   by firmly anchored SnO2 quantum dots
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL LITHIATION; CARBON NANOTUBES;
   STORAGE CAPACITY; TIN; PERFORMANCE; ELECTRODE; HETEROSTRUCTURES;
   DEPOSITION; NANOSHEETS
AB A SnO2-graphene oxide (GO) hybrid composite was prepared by binding SnO2 nanocrystals smaller than 5 nm in GO using a facile hydrothermal method. Aided by hydrophilic radicals, such as hydroxyl and carboxyl, in in situ forming SnO2 quantum dots, the active material and the flexible support are highly coupled. When used as an anode material for lithium ion batteries (LIBs), the hybrid composite electrode delivers a high reversible capacity of nearly 800 mA h g(-1) (based on the total weight of the composite, discharging at 100 mA g(-1)) with more than 90% retention for 200 cycles. Besides the excellent cycling performance at various rates, the composite also exhibits a superior rate performance at 10 A g(-1) with recoverable initial reversible capacity and a long lifespan of 1000 cycles with 80% capacity retention, outperforming most previous SnO2-graphene hybrid electrodes.
C1 [Song, Huawei; Li, Na; Cui, Hao; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
   [Cui, Hao; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China.
RP Wang, CX (reprint author), Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
EM wchengx@mail.sysu.edu.cn
RI Song, Huawei/K-7097-2014
FU National Nature Science Foundation of China [51125008, 11274392]
FX This work was financially supported by the National Nature Science
   Foundation of China (no. 51125008 and no. 11274392).
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NR 34
TC 35
Z9 35
U1 11
U2 108
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 26
BP 7558
EP 7562
DI 10.1039/c3ta11442b
PG 5
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 162DR
UT WOS:000320245400002
ER

PT J
AU Wang, Z
   Zhang, X
   Li, Y
   Liu, ZT
   Hao, ZP
AF Wang, Zhuo
   Zhang, Xin
   Li, Yang
   Liu, Zhaotie
   Hao, Zhengping
TI Synthesis of graphene-NiFe2O4 nanocomposites and their electrochemical
   capacitive behavior
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID LITHIUM-ION BATTERIES; SUPERCAPACITOR DEVICES; CARBON MATERIALS; ANODE
   MATERIALS; COMPOSITES; ELECTRODE; STORAGE; NANOPARTICLES; COFE2O4;
   SPINEL
AB Reduced graphite oxide-NiFe2O4 (RGO-NiFe2O4) composites were synthesized by adding different amounts of NH3 center dot H2O into a mixed aqueous solution of graphite oxide, Ni(NO3)(2) and Fe(NO3)(3) at room temperature. NH3 center dot H2O was used to adjust the synthesis system's pH value. The morphology and the microstructure of the as-prepared composites were characterized by X-ray diffraction (XRD), Brunauer-Emmett-Teller (BET) and transmission electron microscope (TEM) techniques. The structure characterizations indicate that NiFe2O4 successfully deposited on the surface of the RGO and the morphologies of RGO-NiFe2O4 show a transparent structure with NiFe2O4 homogeneously distributed on the RGO surfaces. Capacitive properties of the synthesized electrodes were studied using cyclic voltammetry and electrochemical impedance spectroscopy in a three-electrode experimental setup using 1 M Na2SO4 aqueous solution as electrolyte. It is found that the pH value plays an important role in controlling the electrochemical properties of these electrodes. Among the synthesized electrodes, RGO-NiFe10 (pH = 10) shows the best capacitive properties because of its suitable particle size and good dispersion property. It could be anticipated that the synthesized electrodes will gain promising applications as novel electrode materials in supercapacitors and other devices by virtue of their outstanding characteristics of controllable capacitance and facile synthesis.
C1 [Wang, Zhuo; Zhang, Xin; Li, Yang; Hao, Zhengping] Chinese Acad Sci, Dept Environm Nanomat, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China.
   [Liu, Zhaotie] Shaanxi Normal Univ, Key Lab Appl Surface & Colloid Chem, Sch Chem & Chem Engn, Xian 710062, Peoples R China.
RP Wang, Z (reprint author), Chinese Acad Sci, Dept Environm Nanomat, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China.
EM zpinghao@rcees.ac.cn
FU National Basic Research Program of China [2010CB732300]
FX This work was financially supported by National Basic Research Program
   of China (2010CB732300).
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NR 46
TC 35
Z9 36
U1 37
U2 206
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 21
BP 6393
EP 6399
DI 10.1039/c3ta10433h
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 139EX
UT WOS:000318565700013
ER

PT J
AU Yang, AK
   Xue, Y
   Zhang, Y
   Zhang, XF
   Zhao, H
   Li, XJ
   He, YJ
   Yuan, ZB
AF Yang, Ankang
   Xue, Ying
   Zhang, Yang
   Zhang, Xiaofang
   Zhao, Hong
   Li, Xiangjun
   He, Yujian
   Yuan, Zhuobin
TI A simple one-pot synthesis of graphene nanosheet/SnO2 nanoparticle
   hybrid nanocomposites and their application for selective and sensitive
   electrochemical detection of dopamine
SO JOURNAL OF MATERIALS CHEMISTRY B
LA English
DT Article
ID LITHIUM-ION BATTERIES; GRAPHITE OXIDE; RAMAN-SPECTROSCOPY; CARBON
   ELECTRODES; HYDROGEN STORAGE; ANODE MATERIAL; PERFORMANCE; REDUCTION;
   SHEETS; SINGLE
AB A novel one-pot synthesis of graphene nanosheet/SnO2 nanoparticle hybrid nanocomposites (GN/SnO2) was realized by using graphene oxide nanosheets (GONs) functionalized with sodium dodecyl sulfonate and SnCl2 as the starting materials. The morphology and structure of the synthesized SDS-GN/SnO2 nanocomposites were characterized by Raman spectroscopy, transmission electron microscopy (TEM) and X-ray diffraction analysis. It was found that SnO2 nanoparticles were homogeneously distributed on the graphene nanosheets. The electrochemical behavior of dopamine (DA) at the SDS-GN/SnO2 nanoparticle modified electrode was studied by cyclic voltammetry (CV) and differential pulse voltammetry (DPV). The results showed that the modified electrode exhibited excellent electrocatalytic activity towards the electrochemical oxidation of DA. The separation of the oxidation peak potentials for ascorbic acid (AA)-DA, uric acid (UA)-DA and UA-AA obtained by DPV is about 132 mV, 128 mV and 260 mV, respectively, which allows selective and sensitive detection of DA in the presence of AA and UA. The anodic peak currents were linear with the concentration of DA in the range from 1.0 x 10(-7) to 1.0 x 10(-5) M with a coefficient of 0.9980. The detection limit was 80 nM (S/N = 3). The proposed method could be applied for the determination of DA in real human urine samples.
C1 [Yang, Ankang; Xue, Ying; Zhang, Yang; Zhang, Xiaofang; Zhao, Hong; Li, Xiangjun; He, Yujian; Yuan, Zhuobin] Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China.
RP Yang, AK (reprint author), Univ Chinese Acad Sci, Sch Chem & Chem Engn, 19A YuQuan Rd, Beijing 100049, Peoples R China.
EM hongzhao@ucas.ac.cn
FU Major National Scientific Research Plan of China (973 Program)
   [2011CB933202]; National Natural Science Foundation of China [21205132];
   State Key Laboratory of Environmental Chemistry and Ecotoxicology
   [KF2010-23]
FX This work was supported by a grant from the Major National Scientific
   Research Plan of China (973 Program) (Grant no. 2011CB933202), the
   National Natural Science Foundation of China (Grant no. 21205132) and
   the State Key Laboratory of Environmental Chemistry and Ecotoxicology
   (Grant no. KF2010-23).
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NR 65
TC 35
Z9 35
U1 20
U2 160
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-750X
EI 2050-7518
J9 J MATER CHEM B
JI J. Mat. Chem. B
PY 2013
VL 1
IS 13
BP 1804
EP 1811
DI 10.1039/c3tb00513e
PG 8
WC Materials Science, Biomaterials
SC Materials Science
GA 100SL
UT WOS:000315722500005
ER

PT J
AU Chen, YM
   Lu, ZG
   Zhou, LM
   Mai, YW
   Huang, HT
AF Chen, Yuming
   Lu, Zhouguang
   Zhou, Limin
   Mai, Yiu-Wing
   Huang, Haitao
TI In situ formation of hollow graphitic carbon nanospheres in electrospun
   amorphous carbon nanofibers for high-performance Li-based batteries
SO NANOSCALE
LA English
DT Article
ID LITHIUM-ION BATTERIES; HIGH-RATE CAPABILITY; ANODE MATERIALS; SECONDARY
   BATTERIES; HIGH-CAPACITY; STORAGE; NANOTUBES; NANOSTRUCTURES;
   INTERCALATION; ELECTROLYTE
AB We report on in situ formation of hollow graphitic carbon nanospheres (HGCNs) in amorphous carbon nanofibers (ACNFs) by a combination of electrospinning, calcination and acid treatment. The prepared carbon nanofibers contain many HGCNs on which defects such as discontinuous graphene sheets with a large d-spacing in their wall exist and provide extra sites for Li+ storage and serve as buffers for withstanding large volume expansion and shrinkage during the Li insertion and extraction procedure. Furthermore, some exposed HGCNs on the surface of the ACNFs as well as hollow structures are favorable for lithium ion diffusion from different orientations and sufficient contact between active material and electrolyte. In addition, the high conductivity architectures facilitate collection and transport of electrons during the cycling process. As a result, the ACNFs/HGCNs display a high reversible specific gravimetric capacity of similar to 750 mA h g(-1) and volumetric capacity of similar to 1.1 A h cm(-3) with outstanding rate capability and good cycling stability, which is superior to those of carbon nanofibers (CNFs), carbon nanotubes (CNTs), porous ACNFs, graphene nanosheets (GNSs), GNSs/CNFs, hollow carbon nanospheres and graphite. The synthesis process is simple, low-cost and environmentally friendly, providing new avenues for the rational engineering of high-energy carbon-based anode materials.
C1 [Chen, Yuming; Lu, Zhouguang; Zhou, Limin; Mai, Yiu-Wing] Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China.
   [Mai, Yiu-Wing] Univ Sydney, Sch Aerosp Mech & Mechatron Engn J07, Ctr Adv Mat Technol CAMT, Sydney, NSW 2006, Australia.
   [Huang, Haitao] Hong Kong Polytech Univ, Dept Appl Phys, Hong Kong, Hong Kong, Peoples R China.
   [Huang, Haitao] Hong Kong Polytech Univ, Mat Res Ctr, Hong Kong, Hong Kong, Peoples R China.
   [Lu, Zhouguang] S Univ Sci & Technol China, Div Micro & Nano Mat & Devices, Shenzhen, Guangdong, Peoples R China.
RP Zhou, LM (reprint author), Hong Kong Polytech Univ, Dept Mech Engn, Hong Kong, Hong Kong, Peoples R China.
EM mmlmzhou@inet.polyu.edu.hk
RI Huang, Haitao/F-9697-2010; Mai, YW/K-8436-2012; Lu,
   Zhouguang/G-6240-2013; Chen, Yuming/H-7812-2014
OI Lu, Zhouguang/0000-0001-9375-7747; 
FU Research Grant Council of the Hong Kong Special Administration Region
   [PolyU 5349/10E]; Hong Kong Polytechnic University [1-BD08, G-YX2G]
FX The authors are grateful for the support received from the Research
   Grant Council of the Hong Kong Special Administration Region (grant:
   PolyU 5349/10E) and The Hong Kong Polytechnic University (grants: 1-BD08
   and G-YX2G).
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NR 49
TC 35
Z9 35
U1 21
U2 109
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PD NOV 7
PY 2012
VL 4
IS 21
BP 6800
EP 6805
DI 10.1039/c2nr31557b
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 035IR
UT WOS:000310940500020
PM 23000946
ER

PT J
AU Zhang, Y
   Wang, X
   Zeng, L
   Song, SY
   Liu, DP
AF Zhang, Yu
   Wang, Xiao
   Zeng, Liang
   Song, Shuyan
   Liu, Dapeng
TI Green and controlled synthesis of Cu2O-graphene hierarchical nanohybrids
   as high-performance anode materials for lithium-ion batteries via an
   ultrasound assisted approach
SO DALTON TRANSACTIONS
LA English
DT Article
ID SHAPE-CONTROLLED SYNTHESIS; STORAGE CAPACITY; NANOPARTICLES; OXIDE;
   NANOCRYSTALS; MONODISPERSE; CELLS; CU2O
AB A low-cost, fast, facile, green method, namely an ultrasound assisted approach, has been developed for the controlled synthesis of Cu2O-graphene hybrid nanomaterials. By the protection of graphene nanosheets, the as-obtained anode material exhibited enhanced lithium ion battery performance.
C1 [Wang, Xiao; Song, Shuyan; Liu, Dapeng] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Jilin, Peoples R China.
   [Zhang, Yu] Hiroshima Univ, Inst Adv Mat Res, Higashihiroshima 7398530, Japan.
   [Zeng, Liang] Hiroshima Univ, ADSM, Dept Quantum Matter, Higashihiroshima 7398530, Japan.
RP Liu, DP (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, 5625 Renmin St, Changchun 130022, Jilin, Peoples R China.
EM liudp@ciac.jl.cn
RI Zeng, Liang/E-4849-2010; Zhang, Yu/A-5935-2010; Liu, Dapeng/G-6691-2012
OI Liu, Dapeng/0000-0002-4847-1552
FU National Natural Science Foundation of China [20901075, 21001101]
FX This work was supported by the National Natural Science Foundation of
   China (Grant Nos. 20901075 and 21001101).
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PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1477-9226
EI 1477-9234
J9 DALTON T
JI Dalton Trans.
PY 2012
VL 41
IS 15
BP 4316
EP 4319
DI 10.1039/c2dt12461k
PG 4
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 914NA
UT WOS:000301955900007
PM 22434347
ER

PT J
AU Zhou, JW
   Qin, J
   Zhang, X
   Shi, CS
   Liu, EZ
   Li, JJ
   Zhao, NQ
   He, CN
AF Zhou, Jingwen
   Qin, Jian
   Zhang, Xiang
   Shi, Chunsheng
   Liu, Enzuo
   Li, Jiajun
   Zhao, Naiqin
   He, Chunnian
TI 2D Space-Confined Synthesis of Few-Layer MoS2 Anchored on Carbon
   Nanosheet for Lithium-Ion Battery Anode
SO ACS NANO
LA English
DT Article
DE 2D space-confined synthesis; MOS2; carbon nanosheet; intimate
   interfacial contact; 3D network; lithium-ion battery anode
ID ASSISTED HYDROTHERMAL SYNTHESIS; ORDERED MESOPOROUS MOS2;
   HIGH-PERFORMANCE ANODES; STORAGE PROPERTIES; MOLYBDENUM-DISULFIDE;
   FACILE SYNTHESIS; ELECTROCHEMICAL PERFORMANCE; MOS2-GRAPHENE COMPOSITES;
   GRAPHENE; HYBRID
AB A facile and scalable 2D spatial confinement strategy is developed for in situ synthesizing highly crystalline MoS2 nanosheets with few layers (<= 5 layers) anchored on 3D-porous carbon nanosheet networks (3D FL-MoS2@PCNNs) as lithium-ion battery anode. During the synthesis, 3D self-assembly of cubic NaCl particles is adopted to not only serve as a template to direct the growth of 3D porous carbon nanosheet networks, but also create a 2D-confined space to achieve the construction of few-layer MOS2 nanosheets robustly lain on the surface of carbon nanosheet walls. In the resulting 3D architecture, the intimate contact between the surfaces of MoS2 and carbon nanosheets can effectively avoid the aggregation and restacking of MoS2 as well as remarkably enhance the structural integrity of the electrode, while the conductive matrix of 3D porous carbon nanosheet networks can ensure fast transport of both electrons and ions in the whole electrode. As a result, this unique 3D architecture manifests an outstanding long-life cycling capability at high rates, namely, a specific capacity as large as 709 mAh g(-1) is delivered at 2 A g(-1) and maintains similar to 95.2% even after 520 deep charge/discharge cycles. Apart from promising lithium-ion battery anode, this 3D FL-MoS2@PCNN composite also has immense potential for applications in other areas such as supercapacitor, catalysis, and sensors.
C1 [Zhou, Jingwen; Qin, Jian; Zhang, Xiang; Shi, Chunsheng; Liu, Enzuo; Li, Jiajun; Zhao, Naiqin; He, Chunnian] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
   [Zhou, Jingwen; Qin, Jian; Zhang, Xiang; Shi, Chunsheng; Liu, Enzuo; Li, Jiajun; Zhao, Naiqin; He, Chunnian] Tianjin Univ, Tianjin Key Lab Composites & Funct Mat, Tianjin 300072, Peoples R China.
   [Liu, Enzuo; Zhao, Naiqin; He, Chunnian] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300072, Peoples R China.
RP Zhao, NQ (reprint author), Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
EM nqzhao@tju.edu.cn; cnhe08@tju.edu.cn
FU National Natural Science Foundation of China [51422104, 51472177];
   Foundation for the Author of National Excellent Doctoral Dissertation of
   China [201145]; Program for New Century Excellent Talents in University
   [NCET-12-0408]; National Basic Research Program of China [2010CB934700]
FX The authors acknowledge the financial support by the National Natural
   Science Foundation of China (No. 51422104, and No. 51472177) and
   Foundation for the Author of National Excellent Doctoral Dissertation of
   China (No. 201145), Program for New Century Excellent Talents in
   University (NCET-12-0408), and National Basic Research Program of China
   (2010CB934700).
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NR 64
TC 34
Z9 34
U1 222
U2 430
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD APR
PY 2015
VL 9
IS 4
BP 3837
EP 3848
DI 10.1021/nn506850e
PG 12
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA CH2PL
UT WOS:000353867000045
PM 25791011
ER

PT J
AU Chen, MH
   Liu, JL
   Chao, DL
   Wang, J
   Yin, JH
   Lin, JY
   Fan, HJ
   Shen, ZX
AF Chen, Minghua
   Liu, Jilei
   Chao, Dongliang
   Wang, Jin
   Yin, Jinghua
   Lin, Jianyi
   Fan, Hong Jin
   Shen, Ze Xiang
TI Porous alpha-Fe2O3 nanorods supported on carbon nanotubes-graphene foam
   as superior anode for lithium ion batteries
SO NANO ENERGY
LA English
DT Article
DE Iron oxide; Graphene foam; Carbon nanotubes; Electrochemical energy
   storage; Lithium ion battery
ID IMPROVED ELECTROCHEMICAL PERFORMANCE; FE2O3 NANOPARTICLES;
   SUPERCAPACITIVE PERFORMANCE; STORAGE CAPABILITY; ELECTRODES; ARRAYS;
   NANOSTRUCTURES; SANDWICH
AB A novel flexible and lightweight Fe2O3-based lithium-ion battery anode has been developed by growing porous alpha-Fe2O3 nanorods onto carbon nanotubes-graphene foam (CNT-GF). The CNT-GF 3D network provides a highly conductive, high surface areas and lightweight scaffold for the active Fe2O3 nanorods. Such unique electrodes for lithium-ion battery exhibit an 80% initial columbic efficiency, high-rate capabilities, and >1000 mA h/g capacities at 200 mA/g up to 300 cycles without obvious fading. These properties can be attributed to the fast electrochemical reaction kinetics and electron transport rendered by the conductive 3D network. Our structural design protocol can be extended to many other nanostructured metal oxides or sulfides, and thus provides a new strategy for construction of high-performance electrodes for energy storage. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Chen, Minghua; Yin, Jinghua] Harbin Univ Sci & Technol, Sch Appl Sci, Harbin 150080, Peoples R China.
   [Chen, Minghua; Liu, Jilei; Chao, Dongliang; Wang, Jin; Fan, Hong Jin; Shen, Ze Xiang] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
   [Liu, Jilei; Lin, Jianyi; Fan, Hong Jin; Shen, Ze Xiang] Nanyang Technol Univ, Energy Res Inst NTU, Singapore 639798, Singapore.
RP Fan, HJ (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
EM fanhj@ntu.edu.sg; zexiang@ntu.edu.sg
RI Shen, Zexiang/B-6988-2011; Fan, Hongjin/A-2662-2010; Wang,
   Jin/D-1309-2013
OI Fan, Hongjin/0000-0003-1237-4555; Wang, Jin/0000-0001-6511-869X
CR Hu YY, 2013, NAT MATER, V12, P1130, DOI [10.1038/nmat3784, 10.1038/NMAT3784]
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NR 39
TC 34
Z9 35
U1 63
U2 205
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
EI 2211-3282
J9 NANO ENERGY
JI Nano Energy
PD OCT
PY 2014
VL 9
BP 364
EP 372
DI 10.1016/j.nanoen.2014.08.011
PG 9
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AT0NN
UT WOS:000344632800041
ER

PT J
AU Chen, RJ
   Zhao, T
   Wu, WP
   Wu, F
   Li, L
   Qian, J
   Xu, R
   Wu, HM
   Albishri, HM
   Al-Bogami, AS
   Abd El-Hady, D
   Lu, J
   Amine, K
AF Chen, Renjie
   Zhao, Teng
   Wu, Weiping
   Wu, Feng
   Li, Li
   Qian, Ji
   Xu, Rui
   Wu, Huiming
   Albishri, Hassan M.
   Al-Bogami, A. S.
   Abd El-Hady, Deia
   Lu, Jun
   Amine, Khalil
TI Free-Standing Hierarchically Sandwich-Type Tungsten Disulfide
   Nanotubes/Graphene Anode for Lithium-Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Lithium-ion batteries; anode material; graphene; tungsten disulfide
   nanotube; sandwich type structure; electrochemical performance
ID WS2 NANOTUBES; GRAPHENE; PERFORMANCE; STORAGE; NANOPARTICLES; CAPACITY;
   HYBRID
AB Transition metal dichalcogenides (TMD), analogue of graphene, could form various dimensionalities. Similar to carbon, one-dimensional (1D) nanotube of TMD materials has wide application in hydrogen storage, Li-ion batteries, and supercapacitors due to their unique structure and properties. Here we demonstrate the feasibility of tungsten disulfide nanotubes (WS2-NTs)/graphene (GS) sandwich-type architecture as anode for lithium-ion batteries for the first time. The graphene-based hierarchical architecture plays vital roles in achieving fast electron/ion transfer, thus leading to good electrochemical performance. When evaluated as anode, WS2NTs/GS hybrid could maintain a capacity of 318.6 mA/g over 500 cycles at a current density of 1A/g. Besides, the hybrid anode does not require any additional polymetric binder, conductive additives, or a separate metal current-collector. The relatively high density of this hybrid is beneficial for high capacity per unit volume. Those characteristics make it a potential anode material for light and high-performance lithium-ion batteries.
C1 [Chen, Renjie; Zhao, Teng; Wu, Feng; Li, Li; Qian, Ji] Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China.
   [Wu, Weiping] Cambridge Ink Technol Ltd, Cambridge CB1 2BB, England.
   [Xu, Rui; Wu, Huiming; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60440 USA.
   [Albishri, Hassan M.; Al-Bogami, A. S.; Abd El-Hady, Deia; Amine, Khalil] King Abdulaziz Univ, Fac Sci, Jeddah 80203, Saudi Arabia.
RP Chen, RJ (reprint author), Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China.
EM chenrj@bit.edu.cn; wufeng863@vip.sina.com; junlu@anl.gov; amine@anl.gov
RI Al-Bogami, Abdullah/H-7774-2012; Wu, Weiping/F-9016-2011
OI Wu, Weiping/0000-0003-1462-6402
FU National Science Foundation of China (NSFC) [21373028]; National 863
   Program [2011AA11A256]; New Century Educational Talents Plan of Chinese
   Education Ministry [NCET-12-0050]; Beijing Nova Program
   [Z121103002512029]; U.S. Department of Energy from the Vehicle
   Technologies Office, Department of Energy, Office of Energy Efficiency
   and Renewable Energy (EERE) [DE-AC0206CH11357]; Division of Materials
   Science, Basic Energy Sciences, Department of Energy, Office of Science.
   Argonne National Laboratory, a U.S. Department of Energy Office of
   Science laboratory [DE-AC02-06CH11357]; Deanship of Scientific research
   (DSR), King Abdulaziz University, Jeddah under the HiCi Project
   [11-130-1434HiCi]; DSR
FX This work was supported by the National Science Foundation of China
   (NSFC, 21373028), the National 863 Program (2011AA11A256), New Century
   Educational Talents Plan of Chinese Education Ministry (NCET-12-0050),
   and Beijing Nova Program (Z121103002512029). This work was also
   supported by the U.S. Department of Energy under Contract
   DE-AC0206CH11357 from the Vehicle Technologies Office, Department of
   Energy, Office of Energy Efficiency and Renewable Energy (EERE) and
   Division of Materials Science, Basic Energy Sciences, Department of
   Energy, Office of Science. Argonne National Laboratory, a U.S.
   Department of Energy Office of Science laboratory, is operated under
   Contract No. DE-AC02-06CH11357. This project was also funded by the
   Deanship of Scientific research (DSR), King Abdulaziz University, Jeddah
   under the HiCi Project (Grant 11-130-1434HiCi). The authors (H.M.A.,
   D.A.E., A.S.A, and K.A.) thank the DSR for their technical and financial
   support. The authors also acknowledge the U.S.-China Electric Vehicle
   and Battery Technology Collaboration between Argonne National Laboratory
   and Beijing Institute of Technology.
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NR 31
TC 34
Z9 35
U1 61
U2 253
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD OCT
PY 2014
VL 14
IS 10
BP 5899
EP 5904
DI 10.1021/nl502848z
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AQ7RH
UT WOS:000343016400065
PM 25163033
ER

PT J
AU Favors, Z
   Wang, W
   Bay, HH
   George, A
   Ozkan, M
   Ozkan, CS
AF Favors, Zachary
   Wang, Wei
   Bay, Hamed Hosseini
   George, Aaron
   Ozkan, Mihrimah
   Ozkan, Cengiz S.
TI Stable Cycling of SiO2 Nanotubes as High-Performance Anodes for
   Lithium-Ion Batteries
SO SCIENTIFIC REPORTS
LA English
DT Article
ID GRAPHENE SHEETS; ELECTROCHEMICAL CHARACTERIZATION; FOAM ARCHITECTURES;
   SILICON NANOWIRES; ENERGY-STORAGE; CARBON; NANOPARTICLES; ELECTRODES;
   SUPERCAPACITORS; DEGRADATION
AB Herein, SiO2 nanotubes have been fabricated via a facile two step hard-template growth method and evaluated as an anode for Li-ion batteries. SiO2 nanotubes exhibit a highly stable reversible capacity of 1266 mAhg(-1) after 100 cycles with negligible capacity fading. SiO2 NT anodes experience a capacity increase throughout the first 80 cycles through Si phase growth via SiO2 reduction. The hollow morphology of the SiO2 nanotubes accommodates the large volume expansion experienced by Si-based anodes during lithiation and promotes preservation of the solid electrolyte interphase layer. The thin walls of the SiO2 nanotubes allow for effective reduction in Li-ion diffusion path distance and, thus, afford a favorable rate cyclability. The high aspect ratio character of these nanotubes allow for a relatively scalable fabrication method of nanoscale SiO2-based anodes.
C1 [Favors, Zachary; Wang, Wei; Bay, Hamed Hosseini; George, Aaron; Ozkan, Cengiz S.] Univ Calif Riverside, Dept Mech Engn, Mat Sci & Engn Program, Riverside, CA 92521 USA.
   [Wang, Wei; Ozkan, Mihrimah] Univ Calif Riverside, Dept Chem, Dept Elect Engn, Riverside, CA 92521 USA.
RP Ozkan, CS (reprint author), Univ Calif Riverside, Dept Mech Engn, Mat Sci & Engn Program, Riverside, CA 92521 USA.
EM mihri@ee.ucr.edu; cozkan@engr.ucr.edu
RI Wang, Wei/C-1492-2012
OI Wang, Wei/0000-0001-6587-8859
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NR 54
TC 34
Z9 34
U1 36
U2 104
PU NATURE PUBLISHING GROUP
PI LONDON
PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND
SN 2045-2322
J9 SCI REP-UK
JI Sci Rep
PD APR 15
PY 2014
VL 4
DI 10.1038/srep04605
PG 7
WC Multidisciplinary Sciences
SC Science & Technology - Other Topics
GA AE8WW
UT WOS:000334284700001
PM 24732245
ER

PT J
AU Li, L
   Zhou, GM
   Weng, Z
   Shan, XY
   Li, F
   Cheng, HM
AF Li, Lu
   Zhou, Guangmin
   Weng, Zhe
   Shan, Xu-Yi
   Li, Feng
   Cheng, Hui-Ming
TI Monolithic Fe2O3/graphene hybrid for highly efficient lithium storage
   and arsenic removal
SO CARBON
LA English
DT Article
ID METAL ION REMOVAL; REDUCED GRAPHENE; ANODE MATERIAL; BATTERIES; OXIDE;
   PERFORMANCE; CARBON; ADSORPTION; SUPERCAPACITORS; COMPOSITES
AB We fabricated a monolithic Fe2O3/graphene hybrid directly by hydrothermal reaction of ferrous oxalate dihydrate and graphene oxide Without using a reducing agent. The reduced graphene oxide formed an interconnected network structure that can be used as a support for homogeneous distribution of active Fe2O3 nanoparticles. The graphene network and the pore channels in the hybrid facilitate fast electron transfer and ion transport. This hybrid can be directly used as a free-standing anode for lithium ion batteries, which simplifies the fabrication procedure of electrodes, and also exhibited a high capacity of 1062 mA h g(-1) at 100 mA g(-1), high rate capability and excellent cyclic stability over 100 cycles. Furthermore, as a self-supported adsorbent, it provides a new idea on loading active materials to the suitable substrate, which can be used as a promising material for water purification due to its easy collection and excellent capability in removing As(V) from water. The results demonstrate the promising applications of bulk reduced assembly of graphene with functional metal oxides, which will be helpful for future development of graphene-based multifunctional materials. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Li, Lu; Zhou, Guangmin; Weng, Zhe; Shan, Xu-Yi; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Li, Feng/C-9991-2010
FU National Science Foundation of China [51221264, 51372253, 51172239]
FX This work was supported by National Science Foundation of China (Nos.
   51221264,51372253 and 51172239). We thank Dr. Ronghui Li for the
   experiments and discussion of arsenic removal and Mr. Wei Shen for the
   helpful discussion in this work.
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NR 52
TC 34
Z9 34
U1 26
U2 186
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
EI 1873-3891
J9 CARBON
JI Carbon
PD FEB
PY 2014
VL 67
BP 500
EP 507
DI 10.1016/j.carbon.2013.10.022
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 285FO
UT WOS:000329379300054
ER

PT J
AU Wang, Y
   Han, ZJ
   Yu, SF
   Song, RR
   Song, HH
   Ostrikov, K
   Yang, HY
AF Wang, Ye
   Han, Zhao Jun
   Yu, Siu Fung
   Song, Ran Ran
   Song, Huai He
   Ostrikov, Kostya (Ken)
   Yang, Hui Ying
TI Core-leaf onion-like carbon/MnO2 hybrid nano-urchins for rechargeable
   lithium-ion batteries
SO CARBON
LA English
DT Article
ID ANODE MATERIAL; ELECTROCHEMICAL PERFORMANCE; MNO2 NANOSTRUCTURES;
   ELECTRODE MATERIALS; ENERGY-STORAGE; CYCLE LIFE; COMPOSITE;
   NANOCOMPOSITES; CHALLENGES; GRAPHENE
AB A hybrid nano-urchin structure consisting of spherical onion-like carbon and MnO2 nano-sheets is synthesized by a facile and environmentally-friendly hydrothermal method. Lithium-ion batteries incorporating the hybrid nano-urchin anode exhibit reversible lithium storage with superior specific capacity, enhanced rate capability, stable cycling performance, and nearly 100% Coulombic efficiency. These results demonstrate the effectiveness of designing hybrid nano-architectures with uniform and isotropic structure, high loading of electrochemically-active materials, and good conductivity for the dramatic improvement of lithium storage. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Wang, Ye; Yang, Hui Ying] Singapore Univ Technol & Design, Singapore 138682, Singapore.
   [Han, Zhao Jun; Ostrikov, Kostya (Ken)] CSIRO Mat Sci & Engn, Lindfield, NSW 2070, Australia.
   [Yu, Siu Fung] Hong Kong Polytech Univ, Dept Appl Phys, Kowloon, Hong Kong, Peoples R China.
   [Song, Ran Ran; Song, Huai He] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Key Lab Carbon Fibre & Funct Polymers, Minist Educt, Beijing 100029, Peoples R China.
   [Ostrikov, Kostya (Ken)] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
   [Ostrikov, Kostya (Ken)] Univ Wollongong, Australian Inst Innovat Mat, Wollongong, NSW 2522, Australia.
RP Yang, HY (reprint author), Singapore Univ Technol & Design, 20 Dover Dr, Singapore 138682, Singapore.
EM yanghuiying@sutd.edu.sg
RI Yu, Siu/C-7670-2012; 
OI Yu, Siu/0000-0003-0354-3767; Ostrikov, Kostya (Ken)/0000-0001-8672-9297
FU SUTD-ZJU [ZJURP1100104]; CSIRO's OCE Science Leader Program; Sensors and
   Sensor Network Transformational Capability Platform (TCP); DECRA from
   the Australian Research Council (ARC); Australian Research Council (ARC)
FX This work is supported by the SUTD-ZJU research grant ZJURP1100104,
   CSIRO's OCE Science Leader Program, and Sensors and Sensor Network
   Transformational Capability Platform (TCP). Z.J.H. and K.O. acknowledge
   the DECRA and Future Fellowships from the Australian Research Council
   (ARC).
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NR 45
TC 34
Z9 34
U1 13
U2 140
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
J9 CARBON
JI Carbon
PD NOV
PY 2013
VL 64
BP 230
EP 236
DI 10.1016/j.carbon.2013.07.057
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 224OT
UT WOS:000324898600027
ER

PT J
AU Wang, ZH
   Xiong, XQ
   Qie, L
   Huang, YH
AF Wang, Zhaohui
   Xiong, Xiaoqin
   Qie, Long
   Huang, Yunhui
TI High-performance lithium storage in nitrogen-enriched carbon nanofiber
   webs derived from polypyrrole
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Lithium-ion batteries; Anode; Nitrogen-doped carbon; Polypyrrole
   template; Electrochemical performance
ID HIGH-RATE CAPABILITY; ION BATTERIES; DOPED GRAPHENE; SECONDARY BATTERY;
   ANODE MATERIAL; NANOTUBES; TEMPLATE; CAPACITY; 1ST-PRINCIPLES;
   POLYANILINE
AB Nitrogen-doped carbon nanofiber webs (N-CNFWs) are prepared by direct pyrolyzation of polypyrrole (PPy) nanofiber webs at 600 degrees C. The structure and morphology of N-CNFWs are characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), Fourier-transform infrared spectroscopy (FTIR), Raman spectra and elemental analysis. Both the doped N content and the N existing type in carbon, change with the pyrolysis time. As anode material for lithium-ion battery, the N-CNFWs show high capacity and good rate capability. The reversible capacity is up to 668 mAh g(-1) at a current density of 0.1 A g(-1) and 238 mAh g(-1) at 5 A g(-1), which can be ascribed to the nanofiber structure and high nitrogen content. (c) 2013 Elsevier Ltd. All rights reserved.
C1 [Wang, Zhaohui; Xiong, Xiaoqin; Qie, Long; Huang, Yunhui] Huazhong Univ Sci & Technol, State Key Lab Mat Proc & Die & Mould Technol, Sch Mat Sci & Engn, Wuhan 430074, Hubei, Peoples R China.
RP Huang, YH (reprint author), Huazhong Univ Sci & Technol, State Key Lab Mat Proc & Die & Mould Technol, Sch Mat Sci & Engn, Wuhan 430074, Hubei, Peoples R China.
EM huangyh@hust.edu.cn
RI Huang, Yunhui/C-3752-2014; Wang, Zhaohui/D-5825-2013; Qie,
   Long/F-1488-2011
OI Qie, Long/0000-0003-1693-5911
FU Natural Science Foundation of China [21175050]; MOST [2011AA11290,
   2011DFB70020]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the Natural Science Foundation of China
   (Grant No. 21175050), the MOST (Grant Nos. 2011AA11290 and
   2011DFB70020), and the PCSIRT (Program for Changjiang Scholars and
   Innovative Research Team in University). In addition, the authors thank
   Analytical and Testing Center of Huazhong University of Science and
   Technology for XRD, FTIR, Raman and TEM measurements.
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NR 42
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Z9 34
U1 20
U2 133
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD SEP 1
PY 2013
VL 106
BP 320
EP 326
DI 10.1016/j.electacta.2013.05.088
PG 7
WC Electrochemistry
SC Electrochemistry
GA 202CZ
UT WOS:000323192400042
ER

PT J
AU Xiao, W
   Wang, ZX
   Guo, HJ
   Zhang, YH
   Zhang, Q
   Gan, L
AF Xiao, Wei
   Wang, Zhixing
   Guo, Huajun
   Zhang, Yunhe
   Zhang, Qian
   Gan, Lei
TI A facile PVP-assisted hydrothermal fabrication of Fe2O3/Graphene
   composite as high performance anode material for lithium ion batteries
SO JOURNAL OF ALLOYS AND COMPOUNDS
LA English
DT Article
DE Lithium ion batteries; Anode; Hematite; Graphene; Hydrothermal method
ID NEGATIVE-ELECTRODE MATERIALS; ELECTROCHEMICAL PERFORMANCE; ALPHA-FE2O3
   NANOPARTICLES; GRAPHENE SHEETS; CYCLE STABILITY; RATE CAPABILITY;
   ONE-STEP; LI; STORAGE; OXIDE
AB A simple PVP(polyvinylpyrrolidone)-assisted hydrothermal method is designed to prepare Fe2O3/Graphene composite. While the major crystalline phase of hematite is revealed by X-ray diffraction (XRD), the coexistence of Fe2O3 and graphene are demonstrated by Fourier transform infrared spectra (FI-IR) and Raman spectra studies. Meanwhile, the content of graphene in composite is determined by thermogravimetric analysis (TG). The scanning electron microscopy (SEM) and transmission electron microscope (TEM) images both illustrate the effective combination of Fe2O3 particles and graphene. Furthermore, owing to the synergic effects between Fe2O3 and graphene, Fe2O3/Graphene composite exhibits remarkable cycle performance with highly reversible charge capacity of 1092 mA h g (1) after 50 cycles at the current density of 50 mA g (1), and superior rate performance with highly reversible charge capacity of 501 mA h g (1) at the current density of 1000 mA g (1). For comparison, as absence of the good attachment between graphene and Fe2O3, the bare Fe2O3 and Fe2O3/Graphene composite prepared without assistance of PVP show worse cycle performance. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Xiao, Wei; Wang, Zhixing; Guo, Huajun; Zhang, Yunhe; Zhang, Qian; Gan, Lei] Cent S Univ, Sch Met Sci & Engn, Changsha 410083, Hunan, Peoples R China.
RP Wang, ZX (reprint author), Cent S Univ, Sch Met Sci & Engn, Changsha 410083, Hunan, Peoples R China.
EM wangjiexikeen@csu.edu.cn
FU National Basic Research Program of China Major Special Plan of Science
   and Technology of Hunan Province, China [2011FJ1005]
FX The project was sponsored by the National Basic Research Program of
   China Major Special Plan of Science and Technology of Hunan Province,
   China (Grant No. 2011FJ1005).
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NR 68
TC 34
Z9 34
U1 18
U2 295
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-8388
EI 1873-4669
J9 J ALLOY COMPD
JI J. Alloy. Compd.
PD MAY 25
PY 2013
VL 560
BP 208
EP 214
DI 10.1016/j.jallcom.2012.12.166
PG 7
WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy &
   Metallurgical Engineering
SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering
GA 113QC
UT WOS:000316681600034
ER

PT J
AU Kohandehghan, A
   Kalisvaart, P
   Cui, K
   Kupsta, M
   Memarzadeh, E
   Mitlin, D
AF Kohandehghan, Alireza
   Kalisvaart, Peter
   Cui, Kai
   Kupsta, Martin
   Memarzadeh, Elmira
   Mitlin, David
TI Silicon nanowire lithium-ion battery anodes with ALD deposited TiN
   coatings demonstrate a major improvement in cycling performance
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID SOLID-ELECTROLYTE INTERPHASE; ATOMIC LAYER DEPOSITION; LI-ION; TITANIUM
   NITRIDE; ENERGY-STORAGE; SI-NANOWIRES; ELECTROCHEMICAL PERFORMANCE;
   GRAPHENE; LITHIATION; COMPOSITE
AB We demonstrate that nanometer-scale TiN coatings deposited by atomic layer deposition (ALD), and to a lesser extent by magnetron sputtering, will significantly improve the electrochemical cycling performance of silicon nanowire lithium-ion battery (LIB) anodes. A 5 nm thick ALD coating resulted in optimum cycling capacity retention (55% vs. 30% for the bare nanowire baseline, after 100 cycles) and coulombic efficiency (98% vs. 95%, at 50 cycles), also more than doubling the high rate capacity retention (e. g. 740 mA h g(-1) vs. 330 mA h g(-1), at 5 C). We employed a variety of advanced analytical techniques such as electron energy loss spectroscopy (EELS), focused ion beam analysis (FIB) and X-ray photoelectron spectroscopy (XPS) to elucidate the origin of these effects. The conformal 5 nm TiN remains sufficiently intact to limit the growth of the solid electrolyte interphase (SEI), which in turn both improves the overall coulombic efficiency and reduces the life-ending delamination of the nanowire assemblies from the underlying current collector. Our findings should provide a broadly applicable coating design methodology that will improve the performance of any nanostructured LIB anodes where SEI growth is detrimental.
C1 [Kohandehghan, Alireza; Kalisvaart, Peter; Memarzadeh, Elmira; Mitlin, David] Univ Alberta, Dept Chem & Mat Engn, Edmonton, AB T6G 2V4, Canada.
   [Cui, Kai; Kupsta, Martin; Mitlin, David] NRC, Natl Inst Nanotechnol NINT, Edmonton, AB T6G 2M9, Canada.
RP Kalisvaart, P (reprint author), Univ Alberta, Dept Chem & Mat Engn, 9107 116th St, Edmonton, AB T6G 2V4, Canada.
EM pkalisvaart@gmail.com; dmitlin@ualberta.ca
FU NINT-NRC; NSERC
FX This work was financially supported by NINT-NRC and NSERC Discovery.
   Professor Hao Zhang is acknowledged for valuable discussions.
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NR 76
TC 34
Z9 34
U1 15
U2 114
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 41
BP 12850
EP 12861
DI 10.1039/c3ta12964k
PG 12
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 231JP
UT WOS:000325413000022
ER

PT J
AU Zhang, F
   Cao, HQ
   Yue, DM
   Zhang, JX
   Qu, MZ
AF Zhang, Fan
   Cao, Huaqiang
   Yue, Dongmei
   Zhang, Jingxian
   Qu, Meizhen
TI Enhanced Anode Performances of Polyaniline-TiO2-Reduced Graphene Oxide
   Nanocomposites for Lithium Ion Batteries
SO INORGANIC CHEMISTRY
LA English
DT Article
ID NANOSTRUCTURED MATERIALS; MESOPOROUS ANATASE; TIO2; STORAGE;
   NANOPARTICLES; NANOSPINDLES; ELECTRODES; TRANSPORT; CAPACITY; SPHERES
AB Here, we report a three-layer-structured hybrid nanostructure consisting of transition metal oxide TiO2 nanoparticles sandwiched between carbonaceous polymer polyaniline (PANI) and graphene nanosheets (termed as PTG), which, by simultaneously hindering the agglomeration of TiO2 nanoparticles and enhancing the conductivity of PTG electrode, enables fast discharge and charge. It was demonstrated that the PTG exhibited improved electrochemical performance compared to pure TiO2. As a result, PTG nanocomposite is a promising anode material for highly efficient lithium ion batteries (LIBs) with fast charge/discharge rate and high enhanced cycling performance [discharge capacity of 149.8 mAh/g accompanying Coulombic efficiency of 99.19% at a current density of 5C (1000 mA/g) after 100 cycles] compared to pure TiO2. We can conclude that the concept of applying three-layer-structured graphene-based nanocomposite to electrode in LIBs may open a new area of research for the development of practical transition-metal oxide graphene-based electrodes which will be important to the progress of the LIBs science and technology.
C1 [Zhang, Fan; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Zhang, Fan; Yue, Dongmei] Beijing Univ Chem Technol, Coll Mat Sci & Engn, Beijing 100029, Peoples R China.
   [Zhang, Jingxian; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn; yuedm@mail.buct.edu.cn
FU National Natural Science Foundation of China [20921001]
FX The authors acknowledge financial supports from the National Natural
   Science Foundation of China (20921001).
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NR 54
TC 34
Z9 35
U1 13
U2 176
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0020-1669
J9 INORG CHEM
JI Inorg. Chem.
PD SEP 3
PY 2012
VL 51
IS 17
BP 9544
EP 9551
DI 10.1021/ic301378j
PG 8
WC Chemistry, Inorganic & Nuclear
SC Chemistry
GA 998RS
UT WOS:000308258700050
PM 22906577
ER

PT J
AU Hsieh, CT
   Lin, JS
   Chen, YF
   Teng, HS
AF Hsieh, Chien-Te
   Lin, Jiun-Sheng
   Chen, Yu-Fu
   Teng, Hsisheng
TI Pulse Microwave Deposition of Cobalt Oxide Nanoparticles on Graphene
   Nanosheets as Anode Materials for Lithium Ion Batteries
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID SNO2/GRAPHENE COMPOSITE; IMPEDANCE SPECTROSCOPY; RECHARGEABLE BATTERIES;
   REVERSIBLE CAPACITY; RATE CAPABILITY; CO3O4; PERFORMANCE; ELECTRODES;
   INTERCALATION; MORPHOLOGY
AB We report the high capacity, superior rate capability, and excellent cyclic stability of graphene nanosheets (GNs) decorated with Co3O4 nanoparticles as anodes in Li-ion batteries. A pulse microwave-assisted (MA) polyol method (total period: 30 min) is adopted to deposit cobalt oxides onto the GNs in water and ethylene glycol (EC), forming two types of Co3O4@GN hybrids. The selection of solvent in the MA process plays a central role in affecting the crystallinity, dispersion, and particle size of cobalt oxide particles. The The resulting Co3O4@GN hybrid, prepared by the MA method in EG, shows a homogeneous dispersion of Co3O4 nanocrystals with an average size of 10 nm. The Co(3)O(4)DGN hybrid displays advantages of high reversible capacity, excellent cycleability, and high rate capability. This improved cyclic performance can be attributed to the formation of a three-dimensional GN framework decorated with Co3O4 nanocrystals, leading to fast diffusion of Li ions (diffusion coefficient: 5.82 X 10(-12) cm(2) s(-1)) and low internal resistance (equivalent series resistance: 92.2 Omega) determined by electrochemical impedance spectroscopy. With its ease of MA fabrication and good performance, the Co3O4@GN hybrid will hold promise in practical Li-ion batteries.
C1 [Hsieh, Chien-Te; Lin, Jiun-Sheng; Chen, Yu-Fu] Yuan Ze Univ, Dept Chem Engn & Mat Sci, Tao Yuan 32003, Taiwan.
   [Teng, Hsisheng] Natl Cheng Kung Univ, Dept Chem Engn, Tainan 70101, Taiwan.
RP Hsieh, CT (reprint author), Yuan Ze Univ, Dept Chem Engn & Mat Sci, Tao Yuan 32003, Taiwan.
EM cthsieh@saturn.yzu.edu.tw
RI Teng, Hsisheng/K-5845-2012
FU National Science Council of Taiwan [NSC 101-2628-E-155-001-MY3, NSC
   99-2632-E-155-001-MY3, NSC 101-3113-E-006-011]; Industrial Technology
   Research Institute South [B327HK3310]; Bureau of Energy, Ministry of
   Economic Affairs, Taiwan [101-D0204-2]
FX Prof. Hsieh is grateful for the financial support from the National
   Science Council of Taiwan under contracts NSC 101-2628-E-155-001-MY3 and
   NSC 99-2632-E-155-001-MY3. Prof. H. Teng acknowledges the support from
   the National Science Council of Taiwan (NSC 101-3113-E-006-011) and the
   Industrial Technology Research Institute South (B327HK3310), and the
   Bureau of Energy, Ministry of Economic Affairs, Taiwan (101-D0204-2).
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NR 28
TC 34
Z9 34
U1 2
U2 83
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
EI 1932-7455
J9 J PHYS CHEM C
JI J. Phys. Chem. C
PD JUL 26
PY 2012
VL 116
IS 29
BP 15251
EP 15258
DI 10.1021/jp3041499
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA 978FE
UT WOS:000306725200008
ER

PT J
AU Cai, DD
   Lian, PC
   Zhu, XF
   Liang, SZ
   Yang, WS
   Wang, HH
AF Cai, Dandan
   Lian, Peichao
   Zhu, Xuefeng
   Liang, Shuzhao
   Yang, Weishen
   Wang, Haihui
TI High specific capacity of TiO2-graphene nanocomposite as an anode
   material for lithium-ion batteries in an enlarged potential window
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; TiO2; Nanocomposite; Anode material; Lithium-ion batteries
ID SUPERIOR ELECTRODE PERFORMANCE; ELECTROCHEMICAL PERFORMANCE; CYCLING
   PERFORMANCE; GRAPHENE NANOSHEETS; TIO2 NANOCRYSTALS; PARTICLE-SIZE; LI
   STORAGE; ANATASE; NANOSTRUCTURES; COMPOSITES
AB TiO2-graphene nanocomposite was first synthesized by a facile gas/liquid interface reaction. The structure and morphology were characterized by X-ray diffraction, scanning electron microscopy, transmission electron microscopy, and Brunauer-Emmett-Teller measurements. The results indicate that TiO2 nanoparticles (ca. 10 nm in mean grain size) were successfully deposited onto the graphene sheets during the gas/liquid interfacial reaction process. The electrochemical performance was evaluated by using coin-type cells versus metallic lithium in an enlarged potential window of 0.01-3.0 V. A high specific charge capacity of 499 mAh g(-1) was obtained at a current density of 100 mA g(-1). More strikingly, the TiO2-graphene nanocomposite exhibits excellent rate capability, even at a high current density of 3000 mA g(-1), the specific charge capacity was still as high as 150 mAh g(-1). The high specific charge capacities can be attributed to the facts that graphene possesses high electronic conductivity, and the lithium storage performance of graphene is delivered during discharge/charge processes of TiO2-graphene nanocomposite between 0.01 and 3.0 V. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Cai, Dandan; Lian, Peichao; Liang, Shuzhao; Wang, Haihui] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
   [Zhu, Xuefeng; Yang, Weishen] Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Peoples R China.
RP Wang, HH (reprint author), S China Univ Technol, Sch Chem & Chem Engn, Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China.
EM hhwang@scut.edu.cn
RI Yang, Weishen/P-1623-2014; Zhu, Xuefeng/G-8809-2013
OI Yang, Weishen/0000-0001-9615-7421; Zhu, Xuefeng/0000-0001-5932-7620
FU National Natural Science Foundation of China [20936001]; Cooperation
   Project in Industry, Education and Research of Guangdong Province;
   Ministry of Education of China [20108090400518]; Fundamental Research
   Funds for the Central Universities, SCUT [2009220038]
FX This work was financially supported by the National Natural Science
   Foundation of China (No. 20936001), the Cooperation Project in Industry,
   Education and Research of Guangdong Province and Ministry of Education
   of China (No. 20108090400518) and the Fundamental Research Funds for the
   Central Universities, SCUT (2009220038).
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NR 47
TC 34
Z9 36
U1 11
U2 106
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JUL 15
PY 2012
VL 74
BP 65
EP 72
DI 10.1016/j.electacta.2012.03.170
PG 8
WC Electrochemistry
SC Electrochemistry
GA 960FI
UT WOS:000305373000010
ER

PT J
AU Ji, LW
   Xin, HLL
   Kuykendall, TR
   Wu, SL
   Zheng, HM
   Rao, MM
   Cairns, EJ
   Battaglia, V
   Zhang, YG
AF Ji, Liwen
   Xin, Huolin L.
   Kuykendall, Tevye R.
   Wu, Shao-Ling
   Zheng, Haimei
   Rao, Mumin
   Cairns, Elton J.
   Battaglia, Vincent
   Zhang, Yuegang
TI SnS2 nanoparticle loaded graphene nanocomposites for superior energy
   storage
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID LITHIUM-ION BATTERIES; ANODE MATERIALS; PERFORMANCE; CAPACITY;
   NANOSTRUCTURES; CONVERSION; FUTURE; LAYERS; CELLS; OXIDE
AB SnS2 nanoparticle-loaded graphene nanocomposites were synthesized via one-step hydrothermal reaction. Their electrochemical performance was evaluated as the anode for rechargeable lithium-ion batteries after thermal treatment in an Ar environment. The electrochemical testing results show a high reversible capacity of more than 800 mA h g(-1) at 0.1 C rate and 200 mA h g(-1) for up to 5 C rate. The cells also exhibit excellent capacity retention for up to 90 cycles even at a high rate of 2 C. This electrochemical behavior can be attributed to the well-defined morphology and nanostructures of these as-synthesized nanocomposites, which is characterized by high-resolution transmission electron microscopy and electron energy-loss spectroscopy.
C1 [Ji, Liwen; Kuykendall, Tevye R.; Zhang, Yuegang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
   [Xin, Huolin L.; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
   [Wu, Shao-Ling; Rao, Mumin; Cairns, Elton J.; Battaglia, Vincent] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.
   [Rao, Mumin; Cairns, Elton J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.
RP Zhang, YG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.
EM yzhang5@lbl.gov
RI Zhang, Y/E-6600-2011; Cairns, Elton/E-8873-2012; Xin, Huolin/E-2747-2010
OI Zhang, Y/0000-0003-0344-8399; Cairns, Elton/0000-0002-1179-7591; Xin,
   Huolin/0000-0002-6521-868X
FU Office of Science, Office of Basic Energy Sciences, of the U. S.
   Department of Energy [E-AC02-05CH11231]
FX This work was supported by the Office of Science, Office of Basic Energy
   Sciences, of the U. S. Department of Energy under contract No.
   DE-AC02-05CH11231. HLX thanks Qingyun Mao of Cornell University for the
   FEFF simulations of the sulfur L2,3 edges.
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TC 34
Z9 34
U1 13
U2 96
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
EI 1463-9084
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2012
VL 14
IS 19
BP 6981
EP 6986
DI 10.1039/c2cp40790f
PG 6
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 931WX
UT WOS:000303251100034
PM 22495542
ER

PT J
AU Luo, B
   Zhi, LJ
AF Luo, Bin
   Zhi, Linjie
TI Design and construction of three dimensional graphene- based composites
   for lithium ion battery applications
SO ENERGY & ENVIRONMENTAL SCIENCE
LA English
DT Review
ID HIGH-PERFORMANCE ANODE; NITROGEN-DOPED GRAPHENE; IN-SITU SYNTHESIS;
   VERTICALLY ALIGNED GRAPHENE; ONE-STEP SYNTHESIS; ENHANCED
   ELECTROCHEMICAL PERFORMANCE; METAL DICHALCOGENIDE NANOSHEETS; IMPROVED
   REVERSIBLE CAPACITY; CORE-SHELL NANOSTRUCTURES;
   CHEMICAL-VAPOR-DEPOSITION
AB Three dimensional graphene- based composites (3DGCs) have attracted significant attention for lithium ion battery applications due to their unique structures and attractive properties. A large number of 3DGCs with novel structures and functions have been developed in the past few years. This review summarizes the current progress of 3DGCs, including their preparation and application in lithium ion batteries, especially from the viewpoint of structural and interfacial engineering, which have attracted more and more attention for the development of high performance electrode systems.
C1 [Luo, Bin; Zhi, Linjie] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China.
RP Luo, B (reprint author), Natl Ctr Nanosci & Technol, Beiyitiao 11, Beijing 100190, Peoples R China.
EM zhilj@nanoctr.cn
RI Luo, Bin/P-7836-2015
OI Luo, Bin/0000-0003-2088-6403
FU Ministry of Science and Technology of China [2012CB933403]; National
   Natural Science Foundation of China [21173057, 21273054]; Beijing
   Municipal Science and Technology Commission [Z121100006812003]; Chinese
   Academy of Sciences.
FX The authors acknowledge the support from the Ministry of Science and
   Technology of China (no. 2012CB933403), the National Natural Science
   Foundation of China (Grant no. 21173057, 21273054), the Beijing
   Municipal Science and Technology Commission (Z121100006812003), and the
   Chinese Academy of Sciences.
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NR 368
TC 33
Z9 34
U1 170
U2 322
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1754-5692
EI 1754-5706
J9 ENERG ENVIRON SCI
JI Energy Environ. Sci.
PY 2015
VL 8
IS 2
BP 456
EP 477
DI 10.1039/c4ee02578d
PG 22
WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical;
   Environmental Sciences
SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology
GA CB4RZ
UT WOS:000349616900005
ER

PT J
AU Guo, JX
   Jiang, B
   Zhang, X
   Liu, HT
AF Guo, Jinxue
   Jiang, Bin
   Zhang, Xiao
   Liu, Hongtian
TI Monodisperse SnO2 anchored reduced graphene oxide nanocomposites as
   negative electrode with high rate capability and long cyclability for
   lithium-ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Tin oxide; Reduced graphene oxides; Lithium-ion batteries; Anode;
   Composites
ID NITROGEN-DOPED GRAPHENE; OXYGEN-REDUCTION REACTION; CAPACITY ANODE
   MATERIAL; ONE-POT SYNTHESIS; STORAGE CAPACITY; HOLLOW NANOSPHERES;
   CARBON NANOTUBES; FACILE SYNTHESIS; POROUS SNO2; PERFORMANCE
AB In this manuscript, we present a facile and friendly wet chemical method to prepare monodisperse SnO2 nanocrystals assembled on reduced graphene oxide (RGO). Aided with sodium dodecyl sulfonate, small SnO2 nanoparticles (similar to 5 nm) are deposited onto the flexible support evenly and tightly. A cheap compound, urea, is used for the controlled precipitation of SnO2 and the reduction of graphene oxide. When tested as the anode material, the hybrid composite electrode delivers excellent cyclability at high current density, such as high reversible capacity over 1000 mAh g(-1) after 400 cycles at 0.5 A g(-1) and similar to 560 mAh g(-1) after 400 cycles at 1 A g(-1). The composites also exhibit superior rate capability varying from 0.1 to 4 A g(-1), and possess capacity of 423 mAh g(-1) at 4 A g(-1). This synthesis strategy seems to be suitable for industrial production and can also be extended to produce a variety of metal oxide/RGO composites. (C) 2014 Elsevier B.V. All rights reserved.
C1 [Guo, Jinxue; Jiang, Bin; Zhang, Xiao; Liu, Hongtian] Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266042, Peoples R China.
RP Zhang, X (reprint author), Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Qingdao 266042, Peoples R China.
EM zhx1213@126.com
RI Guo, Jinxue/C-9071-2014
OI Guo, Jinxue/0000-0003-3263-7260
FU National Natural Science Foundation of China [21003079]; Natural Science
   Foundation [ZR2011BM018]; Research Award Fund for Outstanding
   Middle-Aged and Young Scientist of Shandong Province [BS2011CL020];
   Qingdao Project of Science and Technology [12-1-4-3-(20)-jch]
FX This work was financially supported by National Natural Science
   Foundation of China (21003079), Natural Science Foundation
   (ZR2011BM018), Research Award Fund for Outstanding Middle-Aged and Young
   Scientist (BS2011CL020) of Shandong Province and Qingdao Project of
   Science and Technology (12-1-4-3-(20)-jch).
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   Ji LW, 2011, ENERG ENVIRON SCI, V4, P2682, DOI 10.1039/c0ee00699h
   Ren JG, 2011, J POWER SOURCES, V196, P8701, DOI 10.1016/j.jpowsour.2011.06.036
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   Tarascon JM, 2001, NATURE, V414, P359, DOI 10.1038/35104644
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NR 52
TC 33
Z9 33
U1 31
U2 277
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD SEP 15
PY 2014
VL 262
BP 15
EP 22
DI 10.1016/j.jpowsour.2014.03.085
PG 8
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA AI8TL
UT WOS:000337199800003
ER

PT J
AU Wang, RH
   Xu, CH
   Du, M
   Sun, J
   Gao, L
   Zhang, P
   Yao, HL
   Lin, CC
AF Wang, Ronghua
   Xu, Chaohe
   Du, Meng
   Sun, Jing
   Gao, Lian
   Zhang, Peng
   Yao, Heliang
   Lin, Chucheng
TI Solvothermal-Induced Self-Assembly of Fe2O3/GS Aerogels for High
   Li-Storage and Excellent Stability
SO SMALL
LA English
DT Article
ID LITHIUM-ION BATTERIES; PERFORMANCE ANODE MATERIAL; REDUCED GRAPHENE
   OXIDE; ELECTROCHEMICAL PERFORMANCE; HYBRID MATERIALS; NANOPARTICLES;
   ARCHITECTURES; NANOSHEETS; COMPOSITE; CARBON
AB A novel solvothermal-induced self-assembly approach, using colloid sol as precursor, is developed to construct monolithic 3D metal oxide/GS (graphene sheets) aerogels. During the solvothermal process, graphene oxide (GO) is highly reduced to GS and self-assembles into 3D macroscopic hydrogels, accompanying with in situ transformation of colloid sol to metal oxides. As a proof of concept, Fe2O3/GS aerogels are synthesized based on Fe(OH)(3) sol, in which GS self-assemble into an interconnected macroporous framework and Fe2O3 nanocrystals (20-50 nm) uniformly deposit on GS. Benefitting from the integration of macroporous structures, large surface area, high electrical conductivity, and good electrode homogeneity, the hybrid electrode manifests a superior rate capability (930, 660 and 520 mAh g(-1) at 500, 2000 and 4000 mA g(-1), respectively) and excellent prolonged cycling stability at high rates (733 mAh g(-1) during 1000 charge/discharge cycles at 2000 mA g(-1)), demonstrating its great potential for application in high performance lithium ion batteries. The work described here provides a versatile pathway to construct various graphene-based hybrid aerogels.
C1 [Wang, Ronghua; Xu, Chaohe; Du, Meng; Sun, Jing; Gao, Lian; Yao, Heliang; Lin, Chucheng] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
   [Gao, Lian; Zhang, Peng] Shanghai Jiao Tong Univ, Sch Mat Sci & Engn, State Key Lab Metall Matrix Composite Mat, Shanghai 200240, Peoples R China.
RP Sun, J (reprint author), Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China.
EM jingsun@mail.sic.ac.cn; liangao@mail.sic.ac.cn
RI chaohe, xu/B-6493-2011
OI chaohe, xu/0000-0002-1345-1420
FU 973 Project [2012CB932303]; National Natural Science Foundation of China
   [51172261]
FX This work is supported by the 973 Project (2012CB932303), the National
   Natural Science Foundation of China (Grant No. 51172261).
CR Wei W, 2013, ADV MATER, V25, P2909, DOI 10.1002/adma.201300445
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NR 48
TC 33
Z9 33
U1 42
U2 141
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1613-6810
EI 1613-6829
J9 SMALL
JI Small
PD JUN 12
PY 2014
VL 10
IS 11
SI SI
BP 2260
EP 2269
DI 10.1002/smll.201303371
PG 10
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AJ6JO
UT WOS:000337799300014
PM 24678007
ER

PT J
AU Oh, YJ
   Yoo, JJ
   Kim, YI
   Yoon, JK
   Yoon, HN
   Kim, JH
   Park, SB
AF Oh, Young Joon
   Yoo, Jung Joon
   Kim, Yong Il
   Yoon, Jae Kook
   Yoon, Ha Na
   Kim, Jong-Huy
   Park, Seung Bin
TI Oxygen functional groups and electrochemical capacitive behavior of
   incompletely reduced graphene oxides as a thin-film electrode of
   supercapacitor
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Oxygen functional groups; Reduced graphene oxide; Thin-film electrode;
   Pseudocapacitance; Supercapacitor
ID LITHIUM-ION BATTERIES; CHEMICAL-REDUCTION; ENERGY-STORAGE; GRAPHITE
   OXIDE; TRANSPARENT; SENSOR; TEMPERATURE; PERFORMANCE; ANODE
AB For incompletely reduced graphene oxides (RGOs), an effect of oxygen functional groups such as carboxyl, phenol, carbonyl, and quinone on electrochemical capacitive behavior was studied. To prepare RGO thin-film electrodes, a simple fabrication process by (i) dropping and evaporating the graphene oxide (GO) solution, (ii) irradiating pulsed light, and (iii) heat-treating at 200 similar to 360 degrees C was applied. It was notable that the pulsed light irradiation was effective to prevent the disfiguring of deposited GO thinfilm during the thermal reduction. From XRD analyses, interlayer distances of the RGOs were gradually decreased from 0.379 to 0.354 nm. As increasing the thermal reduction temperature from 200 to 360 degrees C, XPS O Is spectra analyses showed that the atomic percentages of carboxyl and phenol of the RGOs were sustained as 5.40 +/- 0.36 and 4.77 +/- 0.41 at% respectively. Meanwhile, those of carbonyl and quinone of the RGOs were gradually declined from 3.10 to 1.81 and from 1.32 to 0.65 at% with different thermal reduction temperature respectively. For all RGO thin-film electrodes, the specific capacitance from the CV measurement in 6 M KOH was sustained as ca. 220 F g(-1) at the scan of 5 mV s(-1). However, in 1 M H2SO4, the specific capacitance was gradually decreased from 171 to 136 F g(-1). After 100,000 cycles in 6M KOH, 1 M H2SO4, and 0.5 M Na2SO4, the RGO (200 degrees C) electrodes showed ca. 92, 54, and 104% of the initial capacitances respectively. The atomic percentages of the oxygen functional groups involved in the pseudocapacitive Faradaic reaction were decreased after the cycle test. Especially in 1 M H2SO4, quinone group was decreased to ca. 48% of initial atomic percentage, which seems to be a main reason for the drastic reduction of capacitance. The specific pseudocapacitance per unit atomic percentage for either carboxyl or phenol group in 6 M KOH was obtained as 12.59 F g(-1) at%(-1). For carbonyl group in 1 M H2SO4, it was a slightly deviated value as 13.55 F g(-1) at%(-1). For quinone group in 1 M H2SO4, it was 27.09 F (C) 2013 Jong-Huy Kim. Published by Elsevier Ltd. All rights reserved.
C1 [Oh, Young Joon; Yoo, Jung Joon; Kim, Yong Il; Yoon, Jae Kook; Yoon, Ha Na; Kim, Jong-Huy] Korea Inst Energy Res, Energy Storage Dept, Taejon 305343, South Korea.
   [Oh, Young Joon; Park, Seung Bin] Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Taejon 305701, South Korea.
RP Kim, JH (reprint author), Korea Inst Energy Res, Energy Storage Dept, 152 Gajeong Ro, Taejon 305343, South Korea.
EM kjhy@kier.re.kr; SeungBinPark@kaist.ac.kr
RI Park, Seung/B-8360-2011
FU KIER; Korea Research Council of Industrial Science and Technology (ISTK)
   based on Cooperative Research Program for National Labs
FX Authors would like to express lots of gratitude for the research grant
   from the KIER and the Korea Research Council of Industrial Science and
   Technology (ISTK) based on Cooperative Research Program for National
   Labs.
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NR 45
TC 33
Z9 33
U1 25
U2 124
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
EI 1873-3859
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JAN 10
PY 2014
VL 116
BP 118
EP 128
DI 10.1016/j.electacta.2013.11.040
PG 11
WC Electrochemistry
SC Electrochemistry
GA AB0PK
UT WOS:000331494400016
ER

PT J
AU Hassan, FM
   Chabot, V
   Elsayed, AR
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   Chen, ZW
AF Hassan, Fathy M.
   Chabot, Victor
   Elsayed, Abdel Rahman
   Xiao, Xingcheng
   Chen, Zhongwei
TI Engineered Si Electrode Nanoarchitecture: A Scalable Postfabrication
   Treatment for the Production of Next-Generation Li-Ion Batteries
SO NANO LETTERS
LA English
DT Article
DE Nanostructures; silicon; lithium-ion battery; flash heat treatment; rate
   capability; electrochemical performance
ID SILICON NANOWIRES; COMPOSITE ELECTRODES; STORAGE PERFORMANCE; NEGATIVE
   ELECTRODE; LITHIUM STORAGE; GRAPHENE FILMS; ANODE MATERIAL; CARBON;
   GRAPHITE; PHOTOLUMINESCENCE
AB A novel, economical flash heat treatment of the fabricated silicon based electrodes is introduced to boost the performance and cycle capability of Li-ion batteries. The treatment reveals a high mass fraction of Si, improved interfacial contact, synergistic SiO2/C coating, and a conductive cellular network for improved conductivity, as well as flexibility for stress compensation. The enhanced electrodes achieve a first cycle efficiency of similar to 84% and a maximum charge capacity of 3525 mA h g(-1), almost 84% of silicon's theoretical maximum. Further, a stable reversible charge capacity of 1150 mA h g(-1) at 1.2 A g(-1) can be achieved over 500 cycles. Thus, the flash heat treatment method introduces a promising avenue for the production of industrially viable, next-generation Li-ion batteries.
C1 [Hassan, Fathy M.; Chabot, Victor; Elsayed, Abdel Rahman; Chen, Zhongwei] Univ Waterloo, Dept Chem Engn, Waterloo, ON N2L 3G1, Canada.
   [Xiao, Xingcheng] Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
RP Xiao, XC (reprint author), Gen Motors Global Res & Dev Ctr, Warren, MI 48090 USA.
EM xingcheng.xiao@gm.com; zhwchen@uwaterloo.ca
RI Hassan, Fathy/D-4204-2009; chen, zhongwei/A-5605-2015
OI Hassan, Fathy/0000-0002-4884-7820; 
FU Natural Sciences and Engineering Research Council of Canada (NSERC);
   University of Waterloo; Waterloo Institute for Nanotechnology; Office of
   Vehicle Technologies of the U.S. Department of Energy
   [DE-AC02-05CH11231, 7056410]
FX The authors would like to acknowledge financial support from the Natural
   Sciences and Engineering Research Council of Canada (NSERC), the
   University of Waterloo, and the Waterloo Institute for Nanotechnology.
   TEM, EELS, and HAADF-STEM were obtained at the Canadian Center for
   Electron Microscopy (CCEM) located at McMaster University. X.C.X. also
   acknowledges the support by the Assistant Secretary for Energy
   Efficiency and Renewable Energy, Office of Vehicle Technologies of the
   U.S. Department of Energy under contract no. DE-AC02-05CH11231,
   subcontract no. 7056410 under the Batteries for Advanced Transportation
   Technologies (BATT) Program.
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NR 69
TC 33
Z9 33
U1 24
U2 176
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD JAN
PY 2014
VL 14
IS 1
BP 277
EP 283
DI 10.1021/nl403943g
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 288BJ
UT WOS:000329586700044
PM 24329030
ER

PT J
AU Kang, WP
   Tang, YB
   Li, WY
   Li, ZP
   Yang, X
   Xu, J
   Lee, CS
AF Kang, Wenpei
   Tang, Yongbing
   Li, Wenyue
   Li, Zhangpeng
   Yang, Xia
   Xu, Jun
   Lee, Chun-Sing
TI Porous CuCo2O4 nanocubes wrapped by reduced graphene oxide as
   high-performance lithium-ion battery anodes
SO NANOSCALE
LA English
DT Article
ID ELECTROCHEMICAL ENERGY-STORAGE; ELECTRODE MATERIALS; HIGH-CAPACITY;
   REVERSIBLE CAPACITY; CO3O4 NANOPARTICLES; NEGATIVE-ELECTRODE; HOLLOW
   SPHERES; METAL OXIDE; SPINEL; MICROSPHERES
AB A composite of porous CuCo2O4 nanocubes well wrapped by reduced graphene oxide (rGO) sheets has been synthesized by a facile microwave-assisted solvothermal reaction and applied as anode in lithium ion batteries (LIBs). The porous structure of the CuCo2O4 nanocubes not only provides a high surface area for contact with the electrolyte, but also assists by accommodating volume change upon charging-discharging. Impedance measurements and transmission electron microscopy show that incorporation of rGO further decreases the charge transfer resistance and improves the structural stability of the composite. As an anode material for a LIB, the composite exhibits a high stable capacity of similar to 570 mA h g (1) at a current density of 1000 mA g (1) after 350 cycles. With a high specific surface area and a low charge transfer resistance, the composite anode shows impressive performance especially at high current density. The LIB shows a high capacity of similar to 450 mA h g(-1) even at a high current density of 5000 mA g(-1), demonstrating the composite's potential for applications in LIBs with long cycling life and high power density.
C1 [Kang, Wenpei; Tang, Yongbing; Li, Wenyue; Li, Zhangpeng; Yang, Xia; Xu, Jun; Lee, Chun-Sing] City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China.
   [Kang, Wenpei; Tang, Yongbing; Li, Wenyue; Li, Zhangpeng; Yang, Xia; Xu, Jun; Lee, Chun-Sing] City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Hong Kong, Hong Kong, Peoples R China.
   [Tang, Yongbing; Li, Wenyue] Chinese Acad Sci, Funct Thin Films Res Ctr, Shenzhen Inst Adv Technol, Beijing 100864, Peoples R China.
RP Tang, YB (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, Hong Kong, Hong Kong, Peoples R China.
EM tangyb@siat.ac.cn; apcslee@cityu.edu.hk
RI LEE, Chun-Sing/B-6254-2013; Xu, Jun/G-4786-2011; 
OI LEE, Chun-Sing/0000-0001-6557-453X; LI, Zhangpeng/0000-0001-8509-4875
FU National Natural Science Foundation of China [51272217, 51302238];
   Collaboration Project of City University of Hong Kong; Shenzhen Huawei
   [YB2012090343]
FX This project has been financially supported by National Natural Science
   Foundation of China (nos 51272217, 51302238), Collaboration Project of
   City University of Hong Kong and Shenzhen Huawei (YB2012090343).
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NR 54
TC 33
Z9 33
U1 50
U2 215
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 12
BP 6551
EP 6556
DI 10.1039/c4nr00446a
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AI8FI
UT WOS:000337143900039
PM 24736868
ER

PT J
AU Zhou, Q
   Zhao, ZB
   Wang, ZY
   Dong, YF
   Wang, XZ
   Gogotsi, Y
   Qiu, JS
AF Zhou, Quan
   Zhao, Zongbin
   Wang, Zhiyu
   Dong, Yanfeng
   Wang, Xuzhen
   Gogotsi, Yury
   Qiu, Jieshan
TI Low temperature plasma synthesis of mesoporous Fe3O4 nanorods grafted on
   reduced graphene oxide for high performance lithium storage
SO NANOSCALE
LA English
DT Article
ID ONE-POT SYNTHESIS; ION BATTERY ANODE; CAPABILITY; CAPACITY; SPHERES;
   NANOPARTICLES; NANOSPHERES; FABRICATION; COMPOSITES; FE2O3
AB Transition metal oxide coupling with carbon is an effective method for improving electrical conductivity of battery electrodes and avoiding the degradation of their lithium storage capability due to large volume expansion/contraction and severe particle aggregation during the lithium insertion and desertion process. In our present work, we develop an effective approach to fabricate the nanocomposites of porous rod-shaped Fe3O4 anchored on reduced graphene oxide (Fe3O4/rGO) by controlling the in situ nucleation and growth of beta-FeOOH onto the graphene oxide (beta-FeOOH/GO) and followed by dielectric barrier discharge (DBD) hydrogen plasma treatment. Such well-designed hierarchical nanostructures are beneficial for maximum utilization of electrochemically active matter in lithium ion batteries and display superior Li uptake with high reversible capacity, good rate capability, and excellent stability, maintaining 890 mA h g(-1) capacity over 100 cycles at a current density of 500 mA g(-1).
C1 [Zhou, Quan; Zhao, Zongbin; Dong, Yanfeng; Wang, Xuzhen; Gogotsi, Yury; Qiu, Jieshan] Dalian Univ Technol, Sch Chem Engn, State Key Lab Fine Chem, Carbon Res Lab,Liaoning Key Lab Energy Mat & Chem, Dalian 116023, Peoples R China.
   [Wang, Zhiyu] Tech Univ Dresden, D-01062 Dresden, Germany.
   [Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, AJ Drexel Nanotechnol Inst, Philadelphia, PA 19104 USA.
RP Zhao, ZB (reprint author), Dalian Univ Technol, Sch Chem Engn, State Key Lab Fine Chem, Carbon Res Lab,Liaoning Key Lab Energy Mat & Chem, Dalian 116023, Peoples R China.
EM zbzhao@dlut.edu.cn; jqiu@dlut.edu.cn
RI Wang, Zhiyu/G-3762-2014
OI Wang, Zhiyu/0000-0002-2739-9889
FU NSFC [51072028, 21176043]; Cheung Kong Scholarship
FX This work was supported by the NSFC (no. 51072028, 21176043).
   Collaboration between Drexel University and Dalian University of
   Technology was supported by the Cheung Kong Scholarship. The authors are
   thankful to Yulia Buranova for assistance with HRTEM analysis and to
   Michael Naguib for helpful comments (both at Drexel University).
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NR 43
TC 33
Z9 33
U1 39
U2 208
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 4
BP 2286
EP 2291
DI 10.1039/c3nr05423c
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AA0PE
UT WOS:000330796700041
PM 24413631
ER

PT J
AU Chen, L
   Wang, ZY
   He, CN
   Zhao, NQ
   Shi, CS
   Liu, EZ
   Li, JJ
AF Chen, Long
   Wang, Zhiyuan
   He, Chunnian
   Zhao, Naiqin
   Shi, Chunsheng
   Liu, Enzuo
   Li, Jiajun
TI Porous Graphitic Carbon Nanosheets as a High-Rate Anode Material for
   Lithium-Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE two dimensional; carbon nanosheets; high-rate anode; lithium-ion battery
ID HIGH-RATE CAPABILITY; ENERGY-STORAGE; GRAPHENE NANOSHEETS; HIGH-POWER;
   PERFORMANCE; OXIDE; NANOSPHERES; ELECTRODE; SHEETS; NANOPARTICLES
AB Two-dimensional (2D) porous graphitic carbon nanosheets (PGC nanosheets) as a high-rate anode material for lithium storage were synthesized by an easy, low-cost, green, and scalable strategy that involves the preparation of the PGC nanosheets with Fe and Fe3O4 nanoparticles embedded (indicated with (Fe&Fe3O4)@PGC nanosheets) using glucose as the carbon precursor, iron nitrate as the metal precursor, and a surface of sodium chloride as the template followed by the subsequent elimination of the Fe and Fe3O4 nanoparticles from the (Fe&Fe3O4)@PGC nanosheets by acid dissolution. The unique 2D integrative features and porous graphitic characteristic of the carbon nanosheets with high porosity, high electronic conductivity, and outstanding mechanical flexibility and stability are very favorable for the fast and steady transfer of electrons and ions. As a consequence, a very high reversible capacity of up to 722 mAh/g at a current density of 100 mA/g after 100 cycles, a high rate capability (535, 380, 200, and 115 mAh/g at 1, 10, 20, and 30 C, respectively, 1 C = 372 mA/g), and a superior cycling performance at an ultrahigh rate (112 mAh/g at 30 C after 570 charge-discharge cycles) are achieved by using these nanosheets as a lithium-ion-battery anode material.
C1 [Chen, Long; Wang, Zhiyuan; He, Chunnian; Zhao, Naiqin; Shi, Chunsheng; Liu, Enzuo; Li, Jiajun] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
   [Chen, Long; Wang, Zhiyuan; He, Chunnian; Zhao, Naiqin; Shi, Chunsheng; Liu, Enzuo; Li, Jiajun] Tianjin Univ, Tianjin Key Lab Composites & Funct Mat, Tianjin 300072, Peoples R China.
   [He, Chunnian; Zhao, Naiqin] Collaborat Innovat Ctr Chem Sci & Engn, Tianjin 300072, Peoples R China.
RP He, CN (reprint author), Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China.
EM cnhe08@tju.edu.cn
FU National Natural Science Foundation of China [51002188, 51272173];
   Foundation for the Author of National Excellent Doctoral Dissertation of
   China [201145]; Natural Science Foundation of Tianjin City
   [12JCYBJC11700]; Program for New Century Excellent Talents in University
   [NCET-12-0408]; Elite Scholar Program of Tianjin University; Innovation
   Foundation of Tianjin University; National Basic Research Program of
   China [2010CB934700]; Key Projects for the Science & Technology Pillar
   Program of Tianjin City [12ZCZDGX00800]
FX The authors acknowledge financial support by the National Natural
   Science Foundation of China (nos. 51002188 and 51272173), the Foundation
   for the Author of National Excellent Doctoral Dissertation of China (no.
   201145), the Natural Science Foundation of Tianjin City (no.
   12JCYBJC11700), the Program for New Century Excellent Talents in
   University (no. NCET-12-0408), the Elite Scholar Program of Tianjin
   University, Innovation Foundation of Tianjin University, National Basic
   Research Program of China (no. 2010CB934700), and the Key Projects for
   the Science & Technology Pillar Program of Tianjin City (no.
   12ZCZDGX00800).
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NR 48
TC 33
Z9 33
U1 20
U2 152
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
EI 1944-8252
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD OCT 9
PY 2013
VL 5
IS 19
BP 9537
EP 9545
DI 10.1021/am402368p
PG 9
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 243ZJ
UT WOS:000326356600040
PM 24016841
ER

PT J
AU Zhuang, XD
   Zhang, F
   Wu, DQ
   Forler, N
   Liang, HW
   Wagner, M
   Gehrig, D
   Hansen, MR
   Laquai, F
   Feng, XL
AF Zhuang, Xiaodong
   Zhang, Fan
   Wu, Dongqing
   Forler, Nina
   Liang, Haiwei
   Wagner, Manfred
   Gehrig, Dominik
   Hansen, Michael Ryan
   Laquai, Frederic
   Feng, Xinliang
TI Two-Dimensional Sandwich-Type, Graphene-Based Conjugated Microporous
   Polymers
SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
LA English
DT Article
DE conjugated microporous polymers; donor-acceptor systems; graphene;
   oxygen reduction reaction; porous carbon
ID HIGH-SURFACE-AREA; METAL-FREE ELECTROCATALYSTS; OXYGEN REDUCTION
   REACTIONS; LITHIUM ION BATTERIES; ORGANIC POLYMERS; ENERGY-STORAGE;
   ANODE MATERIAL; NITROGEN; PERFORMANCE; SUPERCAPACITORS
C1 [Zhuang, Xiaodong; Zhang, Fan; Wu, Dongqing; Feng, Xinliang] Shanghai Jiao Tong Univ, Coll Chem & Chem Engn, Shanghai 200240, Peoples R China.
   [Forler, Nina; Liang, Haiwei; Wagner, Manfred; Gehrig, Dominik; Hansen, Michael Ryan; Laquai, Frederic; Feng, Xinliang] Max Planck Inst Polymer Res, D-55128 Mainz, Germany.
RP Zhang, F (reprint author), Shanghai Jiao Tong Univ, Coll Chem & Chem Engn, 800 Dongchuan Rd, Shanghai 200240, Peoples R China.
EM fan-zhang@sjtu.edu.cn; feng@mpip-mainz.mpg.de
RI Hansen, Michael Ryan/A-4519-2011; Liang, Hai-Wei/B-7292-2011; Zhuang,
   Xiao-Dong/A-1519-2012; 
OI Hansen, Michael Ryan/0000-0001-7114-8051; Zhuang,
   Xiao-Dong/0000-0002-4090-0420; Laquai, Frederic/0000-0002-5887-6158
FU National Basic Research Program of China (973 Program) [2012CB933404];
   Natural Science Foundation of China [21174083, 21102091]; BASF; Shanghai
   Pujiang Program [11J1405400]; PhD Programs Foundation of the Ministry of
   Education of the People's Republic China for Young Scholars
   [20110073120039]; ERC
FX This work was financially supported by the National Basic Research
   Program of China (973 Program: 2012CB933404), the Natural Science
   Foundation of China (21174083 and 21102091), BASF, the Shanghai Pujiang
   Program (11J1405400), the PhD Programs Foundation of the Ministry of
   Education of the People's Republic China for Young Scholars
   (20110073120039), and an ERC grant on 2DMATER.
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NR 60
TC 33
Z9 33
U1 27
U2 219
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 1433-7851
EI 1521-3773
J9 ANGEW CHEM INT EDIT
JI Angew. Chem.-Int. Edit.
PD SEP 9
PY 2013
VL 52
IS 37
BP 9668
EP 9672
DI 10.1002/anie.201304496
PG 5
WC Chemistry, Multidisciplinary
SC Chemistry
GA 210JW
UT WOS:000323829600014
PM 23893563
ER

PT J
AU Sun, J
   Liu, HM
   Chen, X
   Evans, DG
   Yang, WS
   Duan, X
AF Sun, Jie
   Liu, Haimei
   Chen, Xu
   Evans, David G.
   Yang, Wensheng
   Duan, Xue
TI Carbon Nanorings and Their Enhanced Lithium Storage Properties
SO ADVANCED MATERIALS
LA English
DT Article
DE carbon nanorings; confined interlayer galleries; layered double
   hydroxides; lithium-ion batteries; anode materials
ID LAYERED DOUBLE HYDROXIDES; GRAPHENE NANORIBBONS; EMERGENT NANOLIGHTS;
   GRAPHITIC CARBON; NANOTUBES; ADSORPTION; DIAMETER; DEVICES
C1 [Sun, Jie; Liu, Haimei; Chen, Xu; Evans, David G.; Yang, Wensheng; Duan, Xue] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
RP Yang, WS (reprint author), Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China.
EM yangws@mail.buct.edu.cn
FU National Basic Research Program of China [2011CBA00508]; National
   Natural Science Foundation of China [51272020, 21236003]; Excellent
   Ph.D. Thesis Fund of Beijing [YB20101001001]
FX This work was funded by the National Basic Research Program of China
   (Grant No. 2011CBA00508), the National Natural Science Foundation of
   China (51272020, 21236003) and the Excellent Ph.D. Thesis Fund of
   Beijing (YB20101001001).
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NR 32
TC 33
Z9 35
U1 16
U2 196
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0935-9648
J9 ADV MATER
JI Adv. Mater.
PD FEB 25
PY 2013
VL 25
IS 8
BP 1125
EP 1130
DI 10.1002/adma.201203108
PG 6
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 092ES
UT WOS:000315102600005
PM 23161553
ER

PT J
AU Yu, YX
AF Yu, Yang-Xin
TI Can all nitrogen-doped defects improve the performance of graphene anode
   materials for lithium-ion batteries?
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID OXYGEN REDUCTION REACTIONS; DENSITY-FUNCTIONAL THEORY; LAYER GRAPHENE;
   SINGLE-LAYER; 1ST-PRINCIPLES; MOLECULES; STORAGE; ABSORPTION;
   ADSORPTION; STABILITY
AB The electronic and adsorption properties of graphene can be changed significantly through substitutional doping with nitrogen and nitrogen decoration of vacancies. Here ab initio density functional theory with a dispersion correction was used to investigate the stability, magnetic and adsorption properties of nine defects in graphene, including both nitrogen substitutional doping and nitrogen decoration of vacancies. The results indicate that only pyridinic N2V2 defect in graphene shows a ferromagnetic spin structure with high magnetic moment and magnetic stabilization energy. Not all nitrogen-doped defects can improve the capacity of the lithium-ion batteries. The adsorption energies of a lithium atom on nitrogen-substituted graphenes are more positive, indicating that they are meta-stable and no better than the pristine graphene as anode materials of lithium-ion batteries. Nitrogen-decorated single and double vacancy defects, especially for the pyridinic N2V2 defect in graphene, can greatly improve the reversible capacity of the battery in comparison with the pristine graphene. The theoretical prediction of the reversible capacity of the battery is 1039 mA h g(-1) for the nitrogen-doped graphene material synthesized by Wu et al., which is in good agreement with the experimental data (1043 mA h g(-1)). The theoretical computations suggest that nitrogen-decorated single and double vacancy defects in graphene are the promising candidate for anode materials of lithium-ion batteries. Each nitrogen atom in the decoration can improve the reversible capacity of the battery by 63.3-124.5 mA h g(-1) in a 4 x 4 supercell of graphene. The present work provides crucial information for the development of N-doped graphene-based anode materials of lithium-ion batteries.
C1 Tsinghua Univ, Dept Chem Engn, Lab Chem Engn Thermodynam, Beijing 100084, Peoples R China.
RP Yu, YX (reprint author), Tsinghua Univ, Dept Chem Engn, Lab Chem Engn Thermodynam, Beijing 100084, Peoples R China.
EM yangxyu@mail.tsinghua.edu.cn
RI Yang, Weida/F-4844-2012
FU National Natural Science Foundation of China [21176132]; Specialized
   Research Fund for the Doctorial Program of High Education of China
   [20100002110024]
FX I gratefully acknowledge Ms Yong-Jun Du for her help in preparing the
   manuscript. This research was supported by the National Natural Science
   Foundation of China (Grant No. 21176132) and Specialized Research Fund
   for the Doctorial Program of High Education of China (Grant No.
   20100002110024).
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NR 48
TC 33
Z9 33
U1 16
U2 105
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2013
VL 15
IS 39
BP 16819
EP 16827
DI 10.1039/c3cp51689j
PG 9
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 222RX
UT WOS:000324749900054
PM 24002442
ER

PT J
AU Yin, JF
   Cao, HQ
   Zhou, ZF
   Zhang, JX
   Qu, MZ
AF Yin, Jiefu
   Cao, Huaqiang
   Zhou, Zhongfu
   Zhang, Jingxian
   Qu, Meizhen
TI SnS2@reduced graphene oxide nanocomposites as anode materials with high
   capacity for rechargeable lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID MICROWAVE-ASSISTED SYNTHESIS; ELECTROCHEMICAL PERFORMANCE;
   STRUCTURAL-CHARACTERIZATION; RAMAN-SCATTERING; FACILE SYNTHESIS; X-RAY;
   SNS2; STORAGE; SNO2; COMPOSITES
AB Nanostructured electrode materials have been studied extensively with the aim of enhancing lithium ion and electron transport, lowering the stress caused by their volume changes during the charge/discharge processes of electrodes, and decreasing overpotential of the electrode reactions in lithium ion batteries. In this work, we develop a new synthetic route to high capacity "double-sandwich-like" SnS2-based nanocomposites (i.e., SnS2-reduced graphene oxide, termed as SSG) which can be used as an anode material in LIBs with improved electrochemical properties, such as large initial discharge capacity (1032 mA h g(-1)), high reversible discharge capacity (738 mA h g(-1), or 1421 mA h cm(-3) at 2nd cycle), and excellent cyclability (564 mA h g(-1), or 1087 mA h cm(-3) after 60 cycles, corresponding to similar to 76.5% of the initial reversible capacity), with an excellent coulombic efficiency of similar to 96.9%. The electrochemical reaction mechanism of SnS2 with lithium has been suggested to be the alloy-type storage lithium mechanism.
C1 [Yin, Jiefu; Cao, Huaqiang] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Zhou, Zhongfu] Shanghai Univ, Key Lab Mat Microstruct, Shanghai 200444, Peoples R China.
   [Zhang, Jingxian; Qu, Meizhen] Chinese Acad Sci, Chengdu Inst Organ Chem, Chengdu 610041, Peoples R China.
RP Cao, HQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM hqcao@mail.tsinghua.edu.cn
FU National Natural Science Foundation of China [21271112, 21231005,
   20921001]
FX Financial support from the National Natural Science Foundation of China
   (nos. 21271112, 21231005 & 20921001) is acknowledged.
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NR 50
TC 33
Z9 33
U1 38
U2 205
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PD DEC 7
PY 2012
VL 22
IS 45
BP 23963
EP 23970
DI 10.1039/c2jm35137d
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 043DG
UT WOS:000311522500033
ER

PT J
AU Jiang, YZ
   Yuan, TZ
   Sun, WP
   Yan, M
AF Jiang, Yinzhu
   Yuan, Tianzhi
   Sun, Wenping
   Yan, Mi
TI Electrostatic Spray Deposition of Porous SnO2/Graphene Anode Films and
   Their Enhanced Lithium-Storage Properties
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE electrochemical spray deposition; tin oxide; graphene; thin films;
   lithium ion battery
ID LI-ION BATTERIES; NEGATIVE-ELECTRODE; CYCLIC PERFORMANCE; GRAPHENE
   OXIDE; COMPOSITE; CAPACITY; MECHANISMS; NANOTUBES
AB Porous SnO2/graphene composite thin films are prepared as anodes for lithium ion batteries by the electrostatic spray deposition technique. Reticular-structured SnO2 is formed on both the nickel foam substrate and the surface of graphene sheets according to the scanning electron microscopy (SEM) results. Such an assembly mode of graphene and SnO2 is highly beneficial to the electrochemical performance improvement by increasing the electrical conductivity and releasing the volume change of the anode. The novel engineered anode possesses 2134.3 mA h g(-1) of initial discharge capacity and good capacity retention of 551.0 mA h g(-1) up to the 100th cycle at a current density of 200 mA g(-1). This anode also exhibits excellent rate capability, with a reversible capacity of 507.7 mA h g(-1) after 100 cycles at a current density of 800 mA g(-1). The results demonstrate that such a film-type hybrid anode shows great potential for application in high-energy lithium-ion batteries.
C1 [Jiang, Yinzhu; Yuan, Tianzhi; Yan, Mi] Zhejiang Univ, State Key Lab Silicon Mat, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
   [Sun, Wenping] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China.
RP Jiang, YZ (reprint author), Zhejiang Univ, State Key Lab Silicon Mat, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China.
EM yzjiang@zju.edu.cn; mse_yanmi@zju.edu.cn
RI Sun, Wenping/F-6789-2010; Jiang, Yinzhu/D-2479-2010
OI Sun, Wenping/0000-0002-4120-5147; Jiang, Yinzhu/0000-0003-0639-2562
FU National Natural Science Foundation of China [51102213]
FX This work is supported by National Natural Science Foundation of China
   (Grant 51102213).
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Z9 33
U1 12
U2 157
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD NOV
PY 2012
VL 4
IS 11
BP 6216
EP 6220
DI 10.1021/am301788m
PG 5
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 043DA
UT WOS:000311521900065
PM 23106602
ER

PT J
AU Tao, HC
   Fan, LZ
   Yan, XQ
   Qu, XH
AF Tao, Hua-Chao
   Fan, Li-Zhen
   Yan, Xiaoqin
   Qu, Xuanhui
TI In situ synthesis of TiO2-graphene nanosheets composites as anode
   materials for high-power lithium ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Graphene; Titanium dioxide; Anode; Lithium ion batteries; Nanocomposites
ID TIO2-B NANOWIRES; GRAPHENE; ANATASE; INTERCALATION; PERFORMANCE;
   INSERTION; HYBRID; NANOCOMPOSITE; NANOTUBES; TITANIA
AB TiO2-graphene nanosheets (GNS) composites are prepared via an in situ chemical synthesis method, which enables a homogenous dispersion of TiO2 nanoparticles on the graphene nanosheets. The obtained TiO2-GNS composites are anatase-GNS, while TiO2 is nanosized rutile without the incorporation of GNS. The resulting TiO2-GNS composites are employed as anode materials for lithium-ion batteries, showing a high initial reversible capacity of 306 mAh g(-1) as well as a good cycling stability. The TiO2-GNS composites can deliver 60 mAh g(-1) at a current rate as high as 5 A g(-1) and demonstrate negligible fade even after 400 cycles. The superior electrochemical performances of the TiO2-GNS composites can be attributed to their unique structures, which intimately combine the conductive graphene nanosheets network with uniformly dispersed TiO2 nanoparticles. The TiO2-GNS composites could be promising candidate materials for high-power, low-cost, and environmentally friendly anodes for lithium ion batteries. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Tao, Hua-Chao; Fan, Li-Zhen; Yan, Xiaoqin; Qu, Xuanhui] Beijing Univ Sci & Technol, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
RP Fan, LZ (reprint author), Beijing Univ Sci & Technol, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
EM fanlizhen@ustb.edu.cn
FU NSF of China; Fundamental Research Funds for the Central Universities of
   China; State Key Laboratory of New Ceramic and Fine Processing (Tsinghua
   University)
FX This work was supported by NSF of China, Fundamental Research Funds for
   the Central Universities of China and State Key Laboratory of New
   Ceramic and Fine Processing (Tsinghua University).
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NR 37
TC 33
Z9 35
U1 12
U2 116
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD MAY 1
PY 2012
VL 69
BP 328
EP 333
DI 10.1016/j.electacta.2012.03.022
PG 6
WC Electrochemistry
SC Electrochemistry
GA 942EE
UT WOS:000304024400045
ER

PT J
AU Shiva, K
   Rajendra, HB
   Subrahmanyam, KS
   Bhattacharyya, AJ
   Rao, CNR
AF Shiva, Konda
   Rajendra, H. B.
   Subrahmanyam, K. S.
   Bhattacharyya, Aninda J.
   Rao, C. N. R.
TI Improved Lithium Cyclability and Storage in Mesoporous SnO2
   Electronically Wired with Very Low Concentrations (=1?%) of Reduced
   Graphene Oxide
SO CHEMISTRY-A EUROPEAN JOURNAL
LA English
DT Article
DE electron transfer; graphene; lithium-ion batteries; nanotechnology; tin
   dioxide
ID LI-ION BATTERIES; ANODE MATERIALS; ELECTRODES; CAPACITY; SHEETS;
   NANOSTRUCTURES; INSERTION; PHASE
C1 [Shiva, Konda; Rajendra, H. B.; Bhattacharyya, Aninda J.; Rao, C. N. R.] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India.
   [Subrahmanyam, K. S.; Rao, C. N. R.] Jawaharlal Nehru Ctr Adv Sci Res, Chem & Phys Mat Unit, Bangalore 560064, Karnataka, India.
RP Bhattacharyya, AJ (reprint author), Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India.
EM aninda_jb@sscu.iisc.ernet.in
RI Ahirwal, Ashish /F-2532-2013; Bhattacharyya, Aninda/P-3744-2015
OI Ahirwal, Ashish /0000-0002-9127-6541; Bhattacharyya,
   Aninda/0000-0002-0736-0004
FU CSIR (Council for Scientific and Industrial Reseaarch); DST Nano
   Mission, Govt. India
FX The authors thank JNCASR for the use of TEM facilities and CEN (Centre
   for Excellence in Nanoelectronics) for Raman spectroscopy. K. S.
   acknowledges the CSIR (Council for Scientific and Industrial Reseaarch)
   for a Senior Research Fellowship. A.J.B. thanks DST Nano Mission, Govt.
   India for financial support.
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NR 32
TC 33
Z9 33
U1 4
U2 64
PU WILEY-V C H VERLAG GMBH
PI WEINHEIM
PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY
SN 0947-6539
J9 CHEM-EUR J
JI Chem.-Eur. J.
PD APR
PY 2012
VL 18
IS 15
BP 4489
EP 4494
DI 10.1002/chem.201200352
PG 6
WC Chemistry, Multidisciplinary
SC Chemistry
GA 917HC
UT WOS:000302162500005
PM 22415964
ER

PT J
AU Jian, ZL
   Zhao, L
   Wang, R
   Hu, YS
   Li, H
   Chen, W
   Chen, LQ
AF Jian, Zelang
   Zhao, Liang
   Wang, Rui
   Hu, Yong-Sheng
   Li, Hong
   Chen, Wen
   Chen, Liquan
TI The low-temperature (400 degrees C) coating of few-layer graphene on
   porous Li4Ti5O12 via C28H16Br2 pyrolysis for lithium-ion batteries
SO RSC ADVANCES
LA English
DT Article
ID CARBON; SPINEL; ELECTRODE; INTERCALATION; LI4+XTI5O12; PERFORMANCE;
   ABSORPTION; INSERTION; ANODE
AB Porous Li4Ti5O12 coated with few-layer graphene was prepared via the low-temperature pyrolysis of C28H16Br2 at 400 degrees C. The coating layer was very thin and uniform. The coated sample shows superior Li storage performance compared with the as-prepared sample. Capacities of 131 and 104 mA h g(-1) can be reached at current rates of 5 and 10 C, respectively. Moreover, cyclic performance is significantly improved after coating. The capacity decreases from 144.6 to 124.4 mA h g(-1) after 2400 cycles at a current rate of 2 C in a half cell versus Li/Li+, with high capacity retention of 86%.
C1 [Jian, Zelang; Chen, Wen] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Sch Mat Sci & Engn, Wuhan 430070, Peoples R China.
   [Jian, Zelang; Zhao, Liang; Wang, Rui; Hu, Yong-Sheng; Li, Hong; Chen, Liquan] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
RP Jian, ZL (reprint author), Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Sch Mat Sci & Engn, Wuhan 430070, Peoples R China.
EM yshu@aphy.iphy.ac.cn; chenw@whut.edu.cn
RI ZHAO, LIANG/G-6059-2011; Li, Hong/C-4643-2008; Wang, Rui/B-8840-2012;
   Hu, Yong-Sheng/H-1177-2011
OI Li, Hong/0000-0002-8659-086X; Hu, Yong-Sheng/0000-0002-8430-6474
FU "863'' Project [2009AA033101]; "973'' Projects [2010CB833102]; NSFC
   [50972164]; Science and Technology Planning Project of Guangdong
   Province [2010A090602001]; CAS [KJCX2-YW-W26]; Ministry of Education
   [109111]
FX We thank the invaluable discussions with Prof. Michel Armand. This work
   was supported by funding from "863'' Project (2009AA033101), "973''
   Projects (2010CB833102), NSFC (50972164), Science and Technology
   Planning Project of Guangdong Province (2010A090602001), CAS project
   (KJCX2-YW-W26), the 100 Talent Project of the Chinese Academy of
   Sciences and Scientific Research Key Project Fund of Ministry of
   Education (109111).
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NR 38
TC 33
Z9 33
U1 5
U2 42
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2046-2069
J9 RSC ADV
JI RSC Adv.
PY 2012
VL 2
IS 5
BP 1751
EP 1754
DI 10.1039/c2ra01263d
PG 4
WC Chemistry, Multidisciplinary
SC Chemistry
GA 892XA
UT WOS:000300317700006
ER

PT J
AU Jeong, SK
   Inaba, M
   Iriyarna, Y
   Abe, T
   Ogumi, Z
AF Jeong, Soon-Ki
   Inaba, Minoru
   Iriyarna, Yasutoshi
   Abe, Takeshi
   Ogumi, Zernpachi
TI Interfacial reactions between graphite electrodes and propylene
   carbonate-based solutions: Electrolyte-concentration dependence of
   electrochemical lithium intercalation reaction
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE graphite negative electrode; propylene carbonate; lithium intercalation;
   atomic force microscopy; surface film
ID SURFACE-FILM FORMATION; ATOMIC-FORCE MICROSCOPY; NEGATIVE ELECTRODE; ION
   BATTERIES; CATHODIC DECOMPOSITION; ANODES; CELLS; FRICTION; SOLVENT; AFM
AB This study examines the electrochemical reactions occurring at graphite negative electrodes of lithium-ion batteries in a propylene carbonate (PC) electrolyte that contains different concentrations of lithium salts such as, LiClO4, LiPF6 or LiN(SO2C2F5)(2). The electrode reactions are significantly affected by the electrolyte concentration. In concentrated solutions, lithium ions are reversibly intercalated within the graphite to form stage I lithium-graphite intercalation compounds (Li-GICs), regardless of the lithium salt used. On the other hand, electrolyte decomposition and exfoliation of the graphene layers occur continuously in the low-concentration range. In situ analysis with atomic force microscopy reveals that a thin film (thickness of similar to 8 nm) forms on the graphite surface in a concentrated solution, e.g., 3.27 mol kg(-1) LiN(SO2C2F5)(2)/PC, after the first potential cycle between 2.9 and 0 V versus Li+/Li. There is no evidence of the co-intercalation of solvent molecules in the concentrated solution. (C) 2007 Published by Elsevier B.V.
C1 [Jeong, Soon-Ki] Soonchunhyang Univ, Dept Chem Engn, Chungnam 336745, South Korea.
   [Inaba, Minoru] Doshisha Univ, Fac Engn, Dept Mol Sci & Technol, Kyoto 6100321, Japan.
   [Iriyarna, Yasutoshi; Abe, Takeshi; Ogumi, Zernpachi] Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan.
RP Jeong, SK (reprint author), Soonchunhyang Univ, Dept Chem Engn, Chungnam 336745, South Korea.
EM hamin611@sch.ac.kr
RI Abe, Takeshi/F-2544-2010
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NR 35
TC 33
Z9 33
U1 8
U2 41
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD JAN 3
PY 2008
VL 175
IS 1
BP 540
EP 546
DI 10.1016/j.jpowsour.2007.08.065
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 253IY
UT WOS:000252513100069
ER

PT J
AU Xiang, HQ
   Fang, SB
   Jiang, YY
AF Xiang, HQ
   Fang, SB
   Jiang, YY
TI Carbonaceous anodes for lithium-ion batteries prepared from phenolic
   resins with different cross-linking densities
SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY
LA English
DT Article
ID CARBONS
AB The effect of cross-link density of phenolic resin precursor on the capacity of as-prepared carbon was investigated. The results show that a higher cross-link density of phenolic resin is beneficial to the charge capacity of the carbon, and the charge capacity of carbon prepared from phenolic resin with the highest cross-link density is greater than the theoretical capacity of carbonaceous materials. Moreover, the charge curves exhibit a potential plateau at approximately 1 V vs. Li/Li+, and the increase of charge capacity results mainly from the lengthening of this plateau. To explain this phenomenon, we proposed a mechanism that, except for the lithium intercalated between graphene layers, lithium is doped mainly at the edges of graphene layers rather than the surfaces of graphene layers, and it is the interaction between lithium and atoms at the edges that leads to the plateau at about 1 V.
RP Xiang, HQ (reprint author), CHINESE ACAD SCI,INST CHEM,BEIJING 100080,PEOPLES R CHINA.
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NR 17
TC 33
Z9 37
U1 5
U2 8
PU ELECTROCHEMICAL SOC INC
PI PENNINGTON
PA 10 SOUTH MAIN STREET, PENNINGTON, NJ 08534
SN 0013-4651
J9 J ELECTROCHEM SOC
JI J. Electrochem. Soc.
PD JUL
PY 1997
VL 144
IS 7
BP L187
EP L190
DI 10.1149/1.1837794
PG 4
WC Electrochemistry; Materials Science, Coatings & Films
SC Electrochemistry; Materials Science
GA XM567
UT WOS:A1997XM56700004
ER

PT J
AU Liu, JL
   Chen, MH
   Zhang, LL
   Jiang, J
   Yan, JX
   Huang, YZ
   Lin, JY
   Fan, HJ
   Shen, ZX
AF Liu, Jilei
   Chen, Minghua
   Zhang, Lili
   Jiang, Jian
   Yan, Jiaxu
   Huang, Yizhong
   Lin, Jianyi
   Fan, Hong Jin
   Shen, Ze Xiang
TI A Flexible Alkaline Rechargeable Ni/Fe Battery Based on Graphene
   Foam/Carbon Nanotubes Hybrid Film
SO NANO LETTERS
LA English
DT Article
DE Ni/Fe cell-flexible battery; graphene foam; carbon nanotubes; hybrid
   electrodes
ID LITHIUM-ION BATTERIES; NICKEL-HYDROXIDE ELECTRODE; ELECTROCHEMICAL
   PERFORMANCE; ENERGY-STORAGE; AQUEOUS-ELECTROLYTE; IRON BATTERY;
   THIN-FILMS; ANODE; SUPERCAPACITORS; BEHAVIOR
AB The development of portable and wearable electronics has promoted increasing demand for high-performance power sources with high energy/power density, low cost, lightweight, as well as ultrathin and flexible features. Here, a new type of flexible Ni/Fe cell is designed and fabricated by employing Ni(OH)(2) nanosheets and porous Fe2O3 nanorods grown on lightweight graphene foam (GF)/carbon nanotubes (CNTs) hybrid films as electrodes. The assembled f-Ni/Fe cells are able to deliver high energy/power densities (100.7 Wh/kg at 287 W/kg and 70.9 Wh/kg at 1.4 kW/kg, based on the total mass of active materials) and outstanding cycling stabilities (retention 89.1% after 1000 charge/discharge cycles). Benefiting from the use of ultralight and thin GF/CNTs hybrid films as current collectors, our f-Ni/Fe cell can exhibit a volumetric energy density of 16.6 Wh/l (based on the total volume of full cell), which is comparable to that of thin film battery and better than that of typical commercial supercapacitors. Moreover, the f-Ni/Fe cells can retain the electrochemical performance with repeated bendings. These features endow our f-Ni/Fe cells a highly promising candidate for next generation flexible energy storage systems.
C1 [Liu, Jilei; Chen, Minghua; Jiang, Jian; Yan, Jiaxu; Fan, Hong Jin; Shen, Ze Xiang] Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore.
   [Zhang, Lili] ASTAR, Heterogeneous Catalysis, Inst Chem Engn & Sci, Singapore 627833, Singapore.
   [Huang, Yizhong] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Liu, Jilei; Yan, Jiaxu] Nanyang Technol Univ, ERI N, Singapore 639798, Singapore.
RP Fan, HJ (reprint author), Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore.
EM fanhj@ntu.edu.sg; zexiang@ntu.edu.sg
RI yan, jiaxu/J-5984-2015; jiang, jian/F-9144-2011; Huang Yizhong,
   .Yizhong/A-2252-2011; Fan, Hongjin/A-2662-2010; Shen,
   Zexiang/B-6988-2011; Zhang, lili/J-4905-2015
OI jiang, jian/0000-0002-9175-4582; Fan, Hongjin/0000-0003-1237-4555; 
FU Energy Research Institute @NTU (ERI@N); SERC Public Sector Research
   Funding, Agency for Science, Technology, and Research (A*STAR)
   [1121202012]
FX The authors acknowledge support from the Energy Research Institute @NTU
   (ERI@N). H.J.F. thanks the support by SERC Public Sector Research
   Funding (Grant 1121202012), Agency for Science, Technology, and Research
   (A*STAR).
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NR 38
TC 32
Z9 32
U1 61
U2 218
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
EI 1530-6992
J9 NANO LETT
JI Nano Lett.
PD DEC
PY 2014
VL 14
IS 12
BP 7180
EP 7187
DI 10.1021/nl503852m
PG 8
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
   Physics, Condensed Matter
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AW5NY
UT WOS:000346322800065
PM 25402965
ER

PT J
AU Yue, J
   Gu, X
   Chen, L
   Wang, NN
   Jiang, XL
   Xu, HY
   Yang, J
   Qian, YT
AF Yue, Jie
   Gu, Xin
   Chen, Liang
   Wang, Nana
   Jiang, Xiaolei
   Xu, Huayun
   Yang, Jian
   Qian, Yitai
TI General synthesis of hollow MnO2, Mn3O4 and MnO nanospheres as superior
   anode materials for lithium ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-CAPACITY; FACILE SYNTHESIS; EXCELLENT PERFORMANCE; STORAGE
   PROPERTIES; CARBON; LI; NANOTUBES; GRAPHENE; SPHERES; SHELL
AB The use of manganese oxides as promising candidates for anode materials in lithium ion batteries has attracted a significant amount of attention recently. Here, we develop a general approach to synthesize hollow nanospheres of MnO2, Mn3O4 and MnO, using carbon nanospheres as a template and a reagent. Depending on the calcination temperature, time and atmosphere, hollow nanospheres of MnO2 assembled by randomly dispersed nanosheets, or hollow nanospheres of Mn3O4 and MnO composed of aggregated nanoparticles, are produced. The electrochemical properties of the three hollow nanoparticles are investigated in terms of cycling stability and rate capability. They deliver the specific capacities of 840, 1165 or 1515 mA h g(-1) after 60 cycles at 100 mA g(-1) for MnO2, Mn3O4 and MnO. Even at 500 mA g(-1), the reversible capacities could be still kept at 637, 820, and 1050 mA h g(-1) after 150 cycles. The outstanding performances might be related with their hollow structure, porous surface and nanoscale size.
C1 [Yue, Jie; Gu, Xin; Chen, Liang; Wang, Nana; Jiang, Xiaolei; Xu, Huayun; Yang, Jian; Qian, Yitai] Shandong Univ, Sch Chem & Chem Engn, Minist Educ, Key Lab Colloid & Interface Chem, Jinan 250100, Peoples R China.
   [Qian, Yitai] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Dept Chem, Hefei 230026, Peoples R China.
RP Yang, J (reprint author), Shandong Univ, Sch Chem & Chem Engn, Minist Educ, Key Lab Colloid & Interface Chem, Jinan 250100, Peoples R China.
EM yangjian@sdu.edu.cn; ytqian@ustc.edu.cn
RI gu, xin/E-2213-2014; Chen, Liang/D-2779-2014; Yang,  Jian/F-1147-2014;
   Qian, Yitai/F-9692-2010
FU 973 Project of China [2011 CB935901]; National Nature Science
   Foundations of China [91022033, 51172076, 21203111]; Shandong Provincial
   Natural Science Foundation for Distinguished Young Scholar [JQ201205];
   Independent Innovation Foundation of Shandong University [2012ZD007];
   Shandong University
FX This work was supported by the 973 Project of China (no. 2011 CB935901),
   National Nature Science Foundations of China (no. 91022033, 51172076,
   21203111), Shandong Provincial Natural Science Foundation for
   Distinguished Young Scholar (JQ201205), Independent Innovation
   Foundation of Shandong University (2012ZD007), and new-faculty start-up
   funding in Shandong University.
CR Li Q, 2013, ACS APPL MATER INTER, V5, P10975, DOI 10.1021/am403215j
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NR 40
TC 32
Z9 32
U1 67
U2 288
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PD NOV 7
PY 2014
VL 2
IS 41
BP 17421
EP 17426
DI 10.1039/c4ta03924f
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AQ4JW
UT WOS:000342763300028
ER

PT J
AU Kim, TW
   Woo, MA
   Regis, M
   Choi, KS
AF Kim, Tae Woo
   Woo, Myong A.
   Regis, Morrisa
   Choi, Kyoung-Shin
TI Electrochemical Synthesis of Spinel Type ZnCo2O4 Electrodes for Use as
   Oxygen Evolution Reaction Catalysts
SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS
LA English
DT Article
ID LITHIUM-ION BATTERIES; WATER OXIDATION; NEGATIVE-ELECTRODE; COBALT
   OXIDE; CO3O4; REDUCTION; GRAPHENE; ELECTROCATALYSTS; HYBRID; ANODE
AB A new electrochemical synthesis route was developed to prepare spinel-type ZnCo2O4 and Co3O4 as high quality thin film-type electrodes for use as electrocatalysts for oxygen evolution reaction (OER). Whereas Co3O4 contains Co2+ in the tetrahedral sites and Co3+ in the octahedral sites in the spinel structure, ZnCo2O4 contains only Co3+ in the octahedral sites; Co in the tetrahedral sites is replaced by Zn2+. Therefore, by comparing the catalytic properties of ZnCo2O4 and Co3O4 electrodes prepared with comparable surface morphologies and thicknesses, it was possible to examine whether Co2+ in Co3O4 is catalytically active for OER. The electrocatalytic properties of ZnCo2O4 and Co3O4 for OER in both 1 M KOH (pH 13.8) and 0.1 M phosphate buffer (pH 7) solutions were investigated and compared. The results suggest that the Co2+ in Co3O4 is not catalytically critical for OER and ZnCo2O4 can be a more economical and environmentally benign replacement for Co3O4 as an OER catalyst.
C1 [Kim, Tae Woo; Woo, Myong A.; Choi, Kyoung-Shin] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA.
   [Regis, Morrisa] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA.
RP Choi, KS (reprint author), Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA.
EM kschoi@chem.wisc.edu
FU Center for Chemical Innovation of the National Science Foundation
   (POWERING THE PLANET) [CHE-1305124]
FX This work was supported by the Center for Chemical Innovation of the
   National Science Foundation (POWERING THE PLANET, grant no.
   CHE-1305124).
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NR 26
TC 32
Z9 32
U1 17
U2 150
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1948-7185
J9 J PHYS CHEM LETT
JI J. Phys. Chem. Lett.
PD JUL 3
PY 2014
VL 5
IS 13
BP 2370
EP 2374
DI 10.1021/jz501077u
PG 5
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Atomic, Molecular & Chemical
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AK8QN
UT WOS:000338693200033
PM 26279561
ER

PT J
AU Hu, T
   Sun, X
   Sun, HT
   Xin, GQ
   Shao, DL
   Liu, CS
   Lian, J
AF Hu, Tao
   Sun, Xiang
   Sun, Hongtao
   Xin, Guoqing
   Shao, Dali
   Liu, Changsheng
   Lian, Jie
TI Rapid synthesis of nitrogen-doped graphene for a lithium ion battery
   anode with excellent rate performance and super-long cyclic stability
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID CARBON NANOTUBES; REDUCED GRAPHENE; PAPER ELECTRODES; ENERGY-STORAGE;
   NANOSHEETS; OXIDE; CAPACITY; DEPOSITION; SHEETS; CELLS
AB Chemical doping of nitrogen into graphene can significantly enhance the reversible capacity and cyclic stability of the graphene-based lithium ion battery (LIB) anodes, and first principles calculations based on density functional theory suggested that pyridinic-N shows stronger binding with Li with reduced energy barrier for Li diffusion and thus is more effective for Li storage than pyrrolic and graphitic-N. Here, we report a novel and rapid (B30 seconds) process to fabricate nitrogen-doped graphene (NGr) by simultaneous thermal reduction of graphene oxide with ammonium hydroxide. The porous NGr with dominant pyridinic N atoms displays greatly enhanced reversible capacities, rate performance and exceptional cyclic stability as compared with pristine graphene. The reversible discharge capacity of the NGr electrode cycled between 0.01-3 V can reach 453 mA h g(-1) after 550 cycles at a charge rate of 2 A g(-1) (B5.4 C), and 180 mA h g(-1) after 2000 cycles at a high charge rate of 10 A g(-1) (B27 C) without any capacity fading. When charged within 0.01-1.5 V, the NGr anode still exhibits high reversible capacities of 224 mA h g(-1) and 169 mA h g(-1) after 700 cycles and 800 cycles at a charge rate of 1 A g(-1) and 5 A g(-1), respectively. Ex situ X-ray photoelectron spectroscopy (XPS) analysis of the NGr electrode upon lithiation and delithiation indicated that the pyridinic-N dominates the capacity enhancement at 3 V, while the pyrrolic-N contributes primarily to Li ion storage below 1.5 V.
C1 [Hu, Tao; Liu, Changsheng] Northeastern Univ, Minist Educ, Key Lab Anisotropy & Texture Mat, Shenyang 110004, Liaoning, Peoples R China.
   [Hu, Tao; Sun, Xiang; Sun, Hongtao; Xin, Guoqing; Lian, Jie] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
   [Shao, Dali] Rensselaer Polytech Inst, Dept Elect Comp & Syst Engn, Troy, NY 12180 USA.
RP Lian, J (reprint author), Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA.
EM lianj@rpi.edu
RI Sun, Hongtao/N-6597-2013; Shao, Dali/J-5870-2014
OI Sun, Hongtao/0000-0003-3259-6091; 
FU NSF [DMR 1151028]; State Scholarship Fund of the China Scholarship
   Council [2011608043]; Fundamental Research Funds for the Central
   Universities [N100702001]
FX This work was supported by a NSF career award under the Award number of
   DMR 1151028. T. Hu and C. S. Liu also acknowledge the State Scholarship
   Fund of the China Scholarship Council (File No. 2011608043) and the
   Fundamental Research Funds for the Central Universities (N100702001).
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NR 48
TC 32
Z9 32
U1 16
U2 138
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
EI 1463-9084
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2014
VL 16
IS 3
BP 1060
EP 1066
DI 10.1039/c3cp54494j
PG 7
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 274ZE
UT WOS:000328643900028
PM 24287587
ER

PT J
AU Huang, G
   Zhang, FF
   Zhang, LL
   Du, XC
   Wang, JW
   Wang, LM
AF Huang, Gang
   Zhang, Feifei
   Zhang, Leilei
   Du, Xinchuan
   Wang, Jianwei
   Wang, Limin
TI Hierarchical NiFe2O4/Fe2O3 nanotubes derived from metal organic
   frameworks for superior lithium ion battery anodes
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID STORAGE CAPABILITY; FACILE PREPARATION; REDUCED GRAPHENE; PERFORMANCE;
   COMPOSITE; OXIDE; NANOPARTICLES; NANOCOMPOSITES; NANOWIRES; MATRIX
AB A simple method for the synthesis of NiFe2O4/Fe2O3 nanotubes by annealing core-shell Fe2Ni MIL-88/Fe MIL-88 metal organic frameworks (MOFs) has been developed. The crystalline phase, morphology and specific surface area (BET) of the resulting sample have been systematically characterized. The results indicate that the NiFe2O4/Fe2O3 nanotubes, which have diameters of 78 nm and lengths of around 1 mu m, are composed of nano-sized primary particles. The electrochemical performance of the NiFe2O4/Fe2O3 nanotubes when used as an anode material for lithium ion batteries has also been tested. A reversible specific capacity of 936.9 mA h g(-1) was achieved at a current density of 100 mA g(-1) up to 100 cycles. Even at 2000 mA g(-1), the discharge capacity of the composite anode could still reach 423.6 mA h g(-1). The enhanced electrochemical performance of the NiFe2O4/Fe2O3 nanotube anode can be ascribed to the rational design of the hierarchical porous hollow structures and the synergetic effect of different functional components.
C1 [Huang, Gang; Zhang, Feifei; Zhang, Leilei; Du, Xinchuan; Wang, Jianwei; Wang, Limin] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
   [Wang, Limin] Changzhou Inst Energy Storage Mat & Devices, Changzhou 213000, Peoples R China.
   [Huang, Gang; Zhang, Feifei; Zhang, Leilei; Du, Xinchuan; Wang, Jianwei] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
RP Wang, LM (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, Changchun 130022, Peoples R China.
EM lmwang@ciac.ac.cn
RI Huang, Gang/E-9539-2016; 
OI Huang, Gang/0000-0003-2518-8145; Wang, Limin/0000-0001-9618-9239
FU National Nature Science Foundation of China [20111061]
FX This work is supported by the National Nature Science Foundation of
   China (Grant no. 20111061).
CR Li CC, 2010, CHEM-EUR J, V16, P5215, DOI 10.1002/chem.200901632
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NR 32
TC 32
Z9 32
U1 55
U2 180
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 21
BP 8048
EP 8053
DI 10.1039/c4ta00200h
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AH2AW
UT WOS:000335924100057
ER

PT J
AU Zhang, M
   Yan, FL
   Tang, X
   Li, QH
   Wang, TH
   Cao, GZ
AF Zhang, Ming
   Yan, Feilong
   Tang, Xuan
   Li, Qiuhong
   Wang, Taihong
   Cao, Guozhong
TI Flexible CoO-graphene-carbon nanofiber mats as binder-free anodes for
   lithium-ion batteries with superior rate capacity and cyclic stability
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ELECTROCHEMICAL PROPERTIES; SECONDARY BATTERY; HIGH-POWER; PERFORMANCE;
   OXIDE; STORAGE; CO3O4; NANOPARTICLES; COMPOSITE; ELECTRODES
AB Flexible mats composed of CoO-graphene-carbon nanofibers have been prepared by electrospinning and a subsequent thermal treatment. The flexible mats of CoO-graphene-carbon annealed at 650 degrees C exhibited discharge capacities of 760 and 690 mA h g(-1) at the 252nd and 352nd cycle, respectively, at a current density of 500 mA g(-1), which are much higher than those of pure carbon, graphene-carbon, and CoO-carbon nanofibers at the respective cycles. The CoO-graphene-carbon nanofibers can deliver a discharge capacity of 400 mA h g(-1) at a current density of 2 A g(-1), which is also higher than the values obtain for CoO-carbon and graphene-carbon nanofibers. The improved electrochemical properties of the flexible CoO-graphene-carbon nanofiber mats could be ascribed to the framework, which allows for fast diffusion of Li+, the presence of graphene, which enhances the conductivity and the mechanical properties of the mats, and the defective sites that arise from the introduced CoO and graphene which can store Li+. It is believed that the electrospinning method used to combine the material with graphene could be a useful approach to prepare flexible mats for lithium-ion batteries, supercapacitors, and fuel cells.
C1 [Zhang, Ming; Yan, Feilong; Tang, Xuan; Li, Qiuhong; Wang, Taihong] Hunan Univ, State Key Lab Chemobiosensing & Chemometr, Minist Educ, Key Lab Micronano Optoelect Devices, Changsha 410082, Hunan, Peoples R China.
   [Zhang, Ming; Cao, Guozhong] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.
RP Zhang, M (reprint author), Hunan Univ, State Key Lab Chemobiosensing & Chemometr, Minist Educ, Key Lab Micronano Optoelect Devices, Changsha 410082, Hunan, Peoples R China.
EM zhangming@hnu.edu.cn; thwang@hnu.edu.cn; gzcao@uw.edu
RI Cao, Guozhong/E-4799-2011; Wang, Taihong/K-8968-2012; Zhang,
   Ming/F-1456-2014
OI Zhang, Ming/0000-0003-4307-2058
FU National Science Foundation (NSF) [CMMI-1030048]; NESAC/BIO [EB-002027];
   University of Washington TGIF grant; National Natural Science Foundation
   of China [61376073, 21103046]; Hunan Provincial Natural Science
   Foundation of China [10JJ1011, 11JJ7004]; China Scholarship Council;
   Fundamental Research Funds for the Central Universities
FX This research work has been financially supported in part by the
   National Science Foundation (NSF, CMMI-1030048), NESAC/BIO (EB-002027),
   and the University of Washington TGIF grant. Part of this work was
   conducted at the University of Washington NanoTech User Facility, a
   member of the NSF National Nanotechnology Infrastructure Network (NNIN).
   Ming Zhang would like to acknowledge the National Natural Science
   Foundation of China (61376073 and 21103046), the Hunan Provincial
   Natural Science Foundation of China (10JJ1011 and 11JJ7004), the China
   Scholarship Council and Fundamental Research Funds for the Central
   Universities.
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NR 63
TC 32
Z9 32
U1 35
U2 137
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 16
BP 5890
EP 5897
DI 10.1039/c4ta00311j
PG 8
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AD8OF
UT WOS:000333524800043
ER

PT J
AU Xia, GF
   Li, N
   Li, DY
   Liu, RQ
   Wang, C
   Li, Q
   Lu, XJ
   Spendelow, JS
   Zhang, JL
   Wu, G
AF Xia, Guofeng
   Li, Ning
   Li, Deyu
   Liu, Ruiqing
   Wang, Chen
   Li, Qing
   Lu, Xujie
   Spendelow, Jacob S.
   Zhang, Junliang
   Wu, Gang
TI Graphene/Fe2O3/SnO2 Ternary Nanocomposites as a High-Performance Anode
   for Lithium Ion Batteries
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE lithium ion batteries; anode materials; Fe2O3; SnO2; reduced graphene
   oxide; graphene nanocomposites
ID NITROGEN-DOPED GRAPHENE; REVERSIBLE CAPACITY; OXYGEN REDUCTION;
   OXIDE-FILMS; STORAGE; COMPOSITE; HOLLOW; NANOPARTICLES; FABRICATION;
   TEMPLATE
AB We report an rGO/Fe2O3/SnO2 ternary nanocomposite synthesized via homogeneous precipitation of Fe2O3 nanoparticles onto graphene oxide (GO) followed by reduction of GO with SnCl2. The reduction mechanism of GO with SnCl2 and the effects of reduction temperature and time were examined. Accompanying the reduction of GO, particles of SnO2 were deposited on the GO surface. In the graphene nanocomposite, Fe2O3 nanoparticles with a size of similar to 20 nm were uniformly dispersed surrounded by SnO2 nanoparticles, as demonstrated by transmission electron microscopy analysis. Due to the different lithium insertion/extraction potentials, the major role of SnO2 nanoparticles is to prevent aggregation of Fe2O3 during the cycling. Graphene can serve as a matrix for Li+ and electron transport and is capable of relieving the stress that would otherwise accumulate in the Fe2O3 nanoparticles during Li uptake/release. In turn, the dispersion of nanoparticles on graphene can mitigate the restacking of graphene sheets. As a result, the electrochemical performance of rGO/Fe2O3/SnO2 ternary nanocomposite as an anode in Li ion batteries is significantly improved, showing high initial discharge and charge capacities of 1179 and 746 mAhg(-1), respectively. Importantly, nearly 100% discharge charge efficiency is maintained during the subsequent 100 cycles with a specific capacity above 700 mAhg(-1).
C1 [Xia, Guofeng; Li, Ning; Li, Deyu; Liu, Ruiqing; Wang, Chen] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China.
   [Li, Qing; Lu, Xujie; Spendelow, Jacob S.; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.
   [Xia, Guofeng; Zhang, Junliang] Shanghai Jiao Tong Univ, Sch Mech Engn, Shanghai 200240, Peoples R China.
RP Li, N (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China.
EM lininghit@263.net; wugang@lanl.gov
RI Wu, Gang/E-8536-2010; LU, Xujie/L-9672-2014; Li, Qing/G-4502-2011
OI Wu, Gang/0000-0003-4956-5208; 
FU Los Alamos National Laboratory Early Career Laboratory-Directed Research
   and Development (LDRD) Program [20110483ER]
FX Financial support from the Los Alamos National Laboratory Early Career
   Laboratory-Directed Research and Development (LDRD) Program (20110483ER)
   for this work is gratefully acknowledged.
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NR 51
TC 32
Z9 32
U1 22
U2 138
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
J9 ACS APPL MATER INTER
JI ACS Appl. Mater. Interfaces
PD SEP 11
PY 2013
VL 5
IS 17
BP 8607
EP 8614
DI 10.1021/am402124r
PG 8
WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
SC Science & Technology - Other Topics; Materials Science
GA 294BJ
UT WOS:000330017100047
PM 23947768
ER

PT J
AU Zhu, JS
   Wang, DL
   Wang, L
   Lang, XS
   You, WL
AF Zhu, Junsheng
   Wang, Dianlong
   Wang, Lin
   Lang, Xiaoshi
   You, Wanlong
TI Facile synthesis of sulfur coated SnO2-graphene nanocomposites for
   enhanced lithium ion storage
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE SnO2; Sulfur; Graphene; Nanocomposites; Lithium-ion batteries
ID IMPROVED REVERSIBLE CAPACITY; ANODE MATERIAL; CYCLIC PERFORMANCE; TIN
   OXIDE; BATTERIES; STABILITY; COMPOSITE; NANOSHEETS; GRAPHENE; ELECTRODES
AB A simple and low temperature hydrothermal synthesis approach has been developed to prepare sulfur coated SnO2-graphene nanocomposites as an anode material for lithium-ion batteries. The electrochemical performance of the composites was characterized by galvanostatic charge-discharge tests, cyclic voltammetry and electrochemical impedance spectroscopy measurements. Results show that the composite material exhibits a reversible capacity of 819 mAh g(-1) after 200 cycles at 500 mA g(-1) and an excellent rate capability of 580 mAh g(-1) at a high current density of 4000 mA g(-1). The extraordinary performance could be ascribed to the positive synergistic effect of the combination of the nanosized particles of SnO2, the excellent conductivity of graphene and the effects of the coating layer of sulfur. (C) 2013 Elsevier Ltd. All rights reserved.
C1 [Zhu, Junsheng; Wang, Dianlong; Wang, Lin; Lang, Xiaoshi; You, Wanlong] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China.
RP Wang, DL (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, POB 411, Harbin 150001, Peoples R China.
EM dlwang@hit.edu.cn
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NR 32
TC 32
Z9 33
U1 12
U2 146
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD FEB 28
PY 2013
VL 91
BP 323
EP 329
DI 10.1016/j.electacta.2012.12.116
PG 7
WC Electrochemistry
SC Electrochemistry
GA 113ZB
UT WOS:000316707400045
ER

PT J
AU Yue, WB
   Jiang, SH
   Huang, WJ
   Gao, ZQ
   Li, J
   Ren, Y
   Zhao, XH
   Yang, XJ
AF Yue, Wenbo
   Jiang, Shuhua
   Huang, Wenjing
   Gao, Ziqi
   Li, Jie
   Ren, Yu
   Zhao, Xinhua
   Yang, Xiaojing
TI Sandwich-structural graphene-based metal oxides as anode materials for
   lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID NICKEL-OXIDE; PERFORMANCE; NANOPARTICLES; NANOSHEETS; CAPACITY; STORAGE;
   SUPERCAPACITORS; FABRICATION; ELECTRODES; COMPOSITE
AB Graphene-based metal oxides commonly show outstanding electrochemical performance due to the superior properties of graphene. However, the as-formed metal oxides decorated on graphene prefer to disintegrate or aggregate together, and the graphene-metal oxide hybrids also randomly aggregate themselves, resulting in capacity fading and poor cycling stability. Herein, the graphene-based metal oxides are further protected by graphene nanosheets through a stepwise heterocoagulation method, producing a layered sandwich structure. Compared to the normal graphene-based metal oxides, the sandwich-like graphene-based composites exhibit higher reversible capacities, better cycle performances, and higher rate capabilities. Such sandwich structure can avoid the aggregation of the composites and also act as an ideal strain buffer to alleviate the volume change of metal oxides during cycles. Moreover, the electronic conductivity of the electrode can be further enhanced by the introduction of additional graphene nanosheets. This double layer protection strategy is very effective and may be extended to prepare other high-capacity electrode materials for lithium-ion batteries.
C1 [Yue, Wenbo; Jiang, Shuhua; Huang, Wenjing; Gao, Ziqi; Li, Jie; Zhao, Xinhua; Yang, Xiaojing] Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China.
   [Ren, Yu] Natl Inst Clean And Low Carbon Energy, Beijing 102209, Peoples R China.
RP Yue, WB (reprint author), Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China.
EM wbyue@bnu.edu.cn
RI Ren, Yu/F-7262-2010
OI Ren, Yu/0000-0001-8572-5489
FU National Natural Science Foundation of China [21101014, 21273022,
   51272030]; Beijing Municipal Natural Science Foundation [2112022]
FX This work was financially supported by National Natural Science
   Foundation of China (21101014, 21273022 and 51272030) and Beijing
   Municipal Natural Science Foundation (2112022).
CR Yang S, 2012, RSC ADV, V2, P8827, DOI 10.1039/c2ra20746j
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NR 32
TC 32
Z9 32
U1 11
U2 59
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 23
BP 6928
EP 6933
DI 10.1039/c3ta11012e
PG 6
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 148UJ
UT WOS:000319272800030
ER

PT J
AU Bhaskar, A
   Deepa, M
   Rao, TN
   Varadaraju, UV
AF Bhaskar, Akkisetty
   Deepa, Melepurath
   Rao, T. N.
   Varadaraju, U. V.
TI Enhanced nanoscale conduction capability of a MoO2/Graphene composite
   for high performance anodes in lithium ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Molybdenum dioxide; Graphene; Lithium ion batteries; Conducting atomic
   force microscopy; Anode
ID GRAPHENE; CHALLENGES; GRAPHITE; OXIDE; CONVERSION; NANOSHEETS;
   REDUCTION; CAPACITY; VAPOR
AB A MoO2/Graphene composite as a high performance anode for Li ion batteries is synthesized by a one pot in-situ low temperature solution phase reduction method. Electron microscopy and Raman spectroscopy results confirm that 20 graphene layers entrap MoO2 nanoparticles homogeneously in the composite. X-ray photoelectron spectroscopy shows the presence of oxygen functionalities on graphene, which allows intimate contact between MoO2 nanoparticles and the graphene. Conductive atomic force microscopy reveals an extraordinarily high nanoscale electronic conductivity for MoO2/Graphene, greater by 8 orders of magnitude in comparison to bulk MoO2. The layered nanostructure and the conductive matrix provide uninhibited conducting pathways for fast charge transfer and transport between the oxide nanoparticles and graphene which are responsible for the high rate capability, a large lithium ion capacity of 770 mAh g(-1). and an excellent cycling stability (550 mAh g(-1) reversible capacity retained even after 1000 cycles!) at a current density of 540 mA g(-1), thereby rendering it to be superior to previously reported values for neat MoO2 or MoO2/Graphene composite. Impedance analyses demonstrate a lowered interfacial resistance for the composite in comparison to neat MoO2. Our results demonstrate the enormous promise that MoO2/Graphene holds for practical Li-ion batteries. (C) 2012 Elsevier B.V. All rights reserved.
C1 [Bhaskar, Akkisetty; Deepa, Melepurath] Indian Inst Technol Hyderabad, Yeddumailaram 502205, Andhra Pradesh, India.
   [Rao, T. N.] ARCI, Ctr Nanomat, Hyderabad 500005, Andhra Pradesh, India.
   [Varadaraju, U. V.] Indian Inst Technol, Dept Chem, Madras 600036, Tamil Nadu, India.
RP Deepa, M (reprint author), Indian Inst Technol Hyderabad, Ordnance Factory Estate, Yeddumailaram 502205, Andhra Pradesh, India.
EM mdeepa@iith.ac.in
FU International Advanced Research Centre for Powder Metallurgy and New
   Materials (ARCI); Indo-French Centre for the Promotion of Advanced
   Research (CEFIPRA)
FX We thank International Advanced Research Centre for Powder Metallurgy
   and New Materials (ARCI) and Indo-French Centre for the Promotion of
   Advanced Research (CEFIPRA) for financial support and Dr. Dinesh
   Rangappa for TEM characterization.
CR Zhang LS, 2010, J MATER CHEM, V20, P5462, DOI 10.1039/c0jm00672f
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NR 34
TC 32
Z9 34
U1 18
U2 174
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
J9 J POWER SOURCES
JI J. Power Sources
PD OCT 15
PY 2012
VL 216
BP 169
EP 178
DI 10.1016/j.jpowsour.2012.05.050
PG 10
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 999SO
UT WOS:000308335500024
ER

PT J
AU Wang, DL
   Yu, YC
   He, H
   Wang, J
   Zhou, WD
   Abruna, HD
AF Wang, Deli
   Yu, Yingchao
   He, Huan
   Wang, Jie
   Zhou, Weidong
   Abruna, Hector D.
TI Template-Free Synthesis of Hollow-Structured Co3O4 Nanoparticles as
   High-Performance Anodes for Lithium-Ion Batteries
SO ACS NANO
LA English
DT Article
DE cobalt oxides; hollowed structure; anode materials; lithium battery;
   electrochemistry
ID OXYGEN REDUCTION REACTION; STORAGE PROPERTIES; NANOSTRUCTURES;
   NANOCRYSTALS; GRAPHENE; SPHERES; NANOPOROSITY; MICROSPHERES;
   FABRICATION; STABILITY
AB We have developed a template-free procedure to synthesize Co3O4 hollow-structured nanoparticles on a Vulcan XC-72 carbon support. The material was synthesized via an impregnationreduction method followed by air oxidation. In contrast to spherical particles, the hollow-structured Co3O4 nanoparticles exhibited excellent lithium storage capacity, rate capability, and cycling stability when used as the anode material in lithium-ion batteries. Electrochemical testing showed that the hollow-structured Co3O4 particles delivered a stable reversible capacity of about 880 mAh/g (near the theoretical capacity of 890 mAh/g) at a current density of 50 mA/g after 50 cycles. The superior electrochemical performance is attributed to its unique hollow structure, which combines nano- and microscale properties that facilitate electron transfer and enhance structural robustness.
C1 [Wang, Deli; He, Huan; Wang, Jie] Huazhong Univ Sci & Technol, Key Lab Large Format Battery Mat & Syst, Sch Chem & Chem Engn, Minist Educ, Wuhan 430074, Peoples R China.
   [Yu, Yingchao; Zhou, Weidong; Abruna, Hector D.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA.
RP Wang, DL (reprint author), Huazhong Univ Sci & Technol, Key Lab Large Format Battery Mat & Syst, Sch Chem & Chem Engn, Minist Educ, Wuhan 430074, Peoples R China.
EM wangdl81125@hust.edu.cn; hda1@cornell.edu
RI Wang, Deli/K-5029-2012; Wang, Jie/H-3638-2015
FU Department of Energy [DE-FG02-87ER45298]; Energy Materials Center at
   Cornell (EMC2), an Energy Frontier Research Center - US. Department of
   Energy, Office of Basic Energy Sciences [DE-SC0001086]; Natural Science
   Foundation of China [21306060]; Program for New Century Excellent
   Talents in Universities of China [NCET-13-0237]; Doctoral Fund of
   Ministry of Education of China [20130142120039]; Fundamental Research
   Funds for the Central University [2013TS136, 2014YQ009]
FX This work was supported by the Department of Energy though grant
   DE-FG02-87ER45298 and by the Energy Materials Center at Cornell (EMC2),
   an Energy Frontier Research Center funded by the US. Department of
   Energy, Office of Basic Energy Sciences, under Award Number
   DE-SC0001086. The authors acknowledge helpful discussions with Yajuan Li
   and Richard Robinson. D.W. acknowledges the financial support from
   Natural Science Foundation of China (21306060), the Program for New
   Century Excellent Talents in Universities of China (NCET-13-0237), the
   Doctoral Fund of Ministry of Education of China (20130142120039), and
   the Fundamental Research Funds for the Central University (2013TS136,
   2014YQ009).
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NR 49
TC 31
Z9 31
U1 87
U2 261
PU AMER CHEMICAL SOC
PI WASHINGTON
PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
EI 1936-086X
J9 ACS NANO
JI ACS Nano
PD FEB
PY 2015
VL 9
IS 2
BP 1775
EP 1781
DI 10.1021/nn506624g
PG 7
WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
   Nanotechnology; Materials Science, Multidisciplinary
SC Chemistry; Science & Technology - Other Topics; Materials Science
GA CB9GR
UT WOS:000349940500073
PM 25602513
ER

PT J
AU Song, HW
   Li, N
   Cui, H
   Wang, CX
AF Song, Huawei
   Li, Na
   Cui, Hao
   Wang, Chengxin
TI Enhanced storage capability and kinetic processes by pores- and
   hetero-atoms- riched carbon nanobubbles for lithium-ion and sodium-ion
   batteries anodes
SO NANO ENERGY
LA English
DT Article
DE Ionic liquid; Carbon nanobubbles; Nitrogen-doped; Lithium ion battery;
   Sodium ion battery
ID EXCELLENT CYCLING STABILITY; ELECTROCHEMICAL PROPERTIES; GRAPHENE
   SHEETS; POROUS CARBON; HIGH-CAPACITY; PERFORMANCE; PRECURSORS;
   NANOTUBES; CARBONIZATION; LIQUIDS
AB Efficient electrodes with impressive storage capability and fast kinetic processes are urgently needed in meeting the demand for high energy and large rate powering devices. Through a simple silica templated ionic liquids (ILs) impregnating method and an annealing process, nitrogen and oxygen co-doped carbon nanobubbles are synthesized. The fabricated carbon nanobubbles feature multiscale nanopores and abundant few-layer graphitic zones in the thin shells of several nanometers. When used as anodes for lithium-ion batteries (LIBs) and sodiumion batteries (SIBs), the nanobubbles not only exhibit excellent storage capability and rate performance, but also achieve enhancing cyclibility in the long-term cycles. Further analysis on the charging curves and the electrochemical impedance spectroscopy (EIS) reveal the enhancing cyclibility and storage capability might depend on the interfacial capacitance derived from quasi-connection between Li+ or Na+ and the hetero-atom evolving dissociative groups, while the superior rate performance might be attributed to the low interfacial charge-transfer resistance in the carbon nanobubbles electrode. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Song, Huawei; Li, Na; Cui, Hao; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
   [Cui, Hao; Wang, Chengxin] Sun Yat Sen Zhongshan Univ, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China.
RP Wang, CX (reprint author), Sun Yat Sen Zhongshan Univ, Sch Phys Sci & Engn, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Guangdong, Peoples R China.
EM wchengx@mail.sysu.edu.cn
RI Song, Huawei/K-7097-2014
FU National Natural Science Foundation of China [51125008, 11274392]
FX This work was financially supported by the National Natural Science
   Foundation of China (Nos. 51125008 and 11274392).
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NR 45
TC 31
Z9 31
U1 34
U2 177
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
J9 NANO ENERGY
JI Nano Energy
PD MAR
PY 2014
VL 4
BP 81
EP 87
DI 10.1016/j.nanoen.2013.12.017
PG 7
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AF0GR
UT WOS:000334392800011
ER

PT J
AU Zeng, ZP
   Zhao, HL
   Wang, J
   Lv, PP
   Zhang, TH
   Xia, Q
AF Zeng, Zhipeng
   Zhao, Hailei
   Wang, Jie
   Lv, Pengpeng
   Zhang, Tianhou
   Xia, Qing
TI Nanostructured Fe3O4@C as anode material for lithium-ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Magnetite; Active carbon; Electrochemical properties; Anode materials;
   Lithium ion batteries
ID ELECTRODE MATERIALS; ELECTROCHEMICAL PERFORMANCE; ENERGY-CONVERSION;
   CARBON MATERIALS; STORAGE DEVICES; LI; NANOPARTICLES; CAPACITY;
   GRAPHENE; NANOCOMPOSITES
AB The active particle cracking and electrode pulverization of iron oxide anode material as a result of volume expansion during charge/discharge process cause poor reversibility and significant capacity fading in rechargeable lithium-ion batteries. Here, we demonstrate a facile solvothermal route to immobilize the Fe3O4 particles on the porous active carbon. The present method enables us to obtain nano-porous and mosaic structured Fe3O4@C spheres with an average size of ca. 100 nm. The porous active carbon plays an important role in the improvement of electrochemical properties of Fe3O4. It not only acts as a host for the deposition of Fe3O4 particles, but also provides void spaces for active Fe3O4 to buffer the volume expansion. The good contact between Fe3O4 and active carbon ensures the fast electron/Li-ion transport. As a result, the porous Fe3O4@C shows a high reversible specific capacity of similar to 1000 mAh g(-1), good cycle stability and excellent rate capability. Therefore, we believe that this composite is a potential candidate for anode material of high-energy lithium-ion battery. (C) 2013 Elsevier B.V. All rights reserved.
C1 [Zeng, Zhipeng; Zhao, Hailei; Wang, Jie; Lv, Pengpeng; Zhang, Tianhou; Xia, Qing] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
   [Zhao, Hailei; Zhang, Tianhou] Beijing Key Lab New Energy Mat & Technol, Beijing 100083, Peoples R China.
RP Zhao, HL (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
EM hlzhao@ustb.edu.cn
RI Zhao, Hailei/C-2524-2015
OI Zhao, Hailei/0000-0001-5564-3677
FU National Basic Research Program of China [2013CB934003]; National Nature
   Science Foundation of China [21273019]; Fundamental Research Funds for
   the Central Universities [FRF-MP-12-006B]
FX This work was financially supported by National Basic Research Program
   of China (2013CB934003), National Nature Science Foundation of China
   (21273019) and the Fundamental Research Funds for the Central
   Universities (FRF-MP-12-006B).
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NR 55
TC 31
Z9 31
U1 34
U2 216
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD FEB 15
PY 2014
VL 248
BP 15
EP 21
DI 10.1016/j.jpowsour.2013.09.063
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA 301RY
UT WOS:000330551000003
ER

PT J
AU Chen, SQ
   Bao, PT
   Huang, XD
   Sun, B
   Wang, GX
AF Chen, Shuangqiang
   Bao, Peite
   Huang, Xiaodan
   Sun, Bing
   Wang, Guoxiu
TI Hierarchical 3D mesoporous silicon@graphene nanoarchitectures for
   lithium ion batteries with superior performance
SO NANO RESEARCH
LA English
DT Article
DE silicon anode; graphene foam; chemical vapor deposition; lithium ion
   battery
ID ANODE MATERIALS; RECHARGEABLE BATTERIES; SECONDARY BATTERIES; NEGATIVE
   ELECTRODES; STORAGE; NANOTUBE; NANOPARTICLES; DEPOSITION; AEROGELS;
   NANOCOMPOSITES
AB Silicon has been recognized as the most promising anode material for high capacity lithium ion batteries. However, large volume variations during charge and discharge result in pulverization of Si electrodes and fast capacity loss on cycling. This drawback of Si electrodes can be overcome by combination with well-organized graphene foam. In this work, hierarchical three-dimensional carbon-coated mesoporous Si nanospheres@graphene foam (C@Si@GF) nanoarchitectures were successfully synthesized by a thermal bubble ejection assisted chemical-vapor-deposition and magnesiothermic reduction method. The morphology and structure of the as-prepared nanocomposites were characterized by field emission scanning electron microscopy, transmission electron microscopy and Raman spectroscopy. When employed as anode materials in lithium ion batteries, C@Si@GF nanocomposites exhibited superior electrochemical performance including a high specific capacity of 1,200 mAh/g at the current density of 1 A/g, excellent high rate capabilities and an outstanding cyclability. Post-mortem analyses identified that the morphology of 3D C@Si@GF electrodes after 200 cycles was well maintained. The synergistic effects arising from the combination of mesoporous Si nanospheres and graphene foam nanoarchitectures may address the intractable pulverization problem of Si electrode.
C1 [Chen, Shuangqiang; Huang, Xiaodan; Sun, Bing; Wang, Guoxiu] Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
   [Bao, Peite] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia.
RP Wang, GX (reprint author), Univ Technol Sydney, Sch Chem & Forens Sci, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia.
EM Guoxiu.wang@uts.edu.au
RI Sun, Bing/I-9339-2014
OI Sun, Bing/0000-0002-4365-486X
FU Australian Research Council (ARC) [DP1093855]; ARC [FT110100800];
   Chinese Scholarship Council (CSC) [2011689009]
FX This project is financially supported by the Australian Research Council
   (ARC) through the ARC Discovery project (No. DP1093855), ARC Future
   Fellowship project (No. FT110100800) and partially supported by the
   Chinese Scholarship Council (CSC, No. 2011689009).
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NR 56
TC 31
Z9 31
U1 44
U2 230
PU TSINGHUA UNIV PRESS
PI BEIJING
PA TSINGHUA UNIV, RM A703, XUEYAN BLDG, BEIJING, 10084, PEOPLES R CHINA
SN 1998-0124
EI 1998-0000
J9 NANO RES
JI Nano Res.
PD JAN
PY 2014
VL 7
IS 1
BP 85
EP 94
DI 10.1007/s12274-013-0374-y
PG 10
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 290YF
UT WOS:000329793800005
ER

PT J
AU Sun, PL
   Zhang, WX
   Hu, XL
   Yuan, LX
   Huang, YH
AF Sun, Panling
   Zhang, Wuxing
   Hu, Xianluo
   Yuan, Lixia
   Huang, Yunhui
TI Synthesis of hierarchical MoS2 and its electrochemical performance as an
   anode material for lithium-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HYDROTHERMAL SYNTHESIS; STORAGE; NANOPARTICLES; MICROSPHERES;
   NANOSHEETS; NANOTUBES; MECHANISM; GRAPHENE; NANOSTRUCTURES;
   INTERCALATION
AB A facile process is developed to synthesize MoS2 in basic solutions via a hydrothermal route by employing ammonium heptamolybdate and thiourea as starting materials and post-annealing in a N-2 atmosphere at 450 degrees C for 5 h. The morphologies of the MoS2 products can be tuned from porous flowers to dense spheres by addition of NaOH. Experimental results show that the MoS2 products have good crystallinity. A formation mechanism of the MoS2 is proposed in which the dense MoS2 spheres are evolved from the porous MoS2 flowers through growth along the < 00l > direction of the nanosheets. Based on the growth mechanism, the microstructure of MoS2 can be successfully controlled by adjustment of the S/Mo ratio or addition of a surfactant in the recipe. Electrochemical measurements demonstrate that the flower-like MoS2 shows better electrochemical performance than MoS2 spheres as anode materials for Li-ion batteries, which deliver a high reversible capacity of 900 mA h g(-1) at a current density of 100 mA g(-1), excellent cycling stability and rate capability.
C1 [Sun, Panling; Zhang, Wuxing; Hu, Xianluo; Yuan, Lixia; Huang, Yunhui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
RP Zhang, WX (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Peoples R China.
EM zhangwx@mail.hust.edu.cn; huangyh@mail.hust.edu.cn
RI Hu, Xianluo/E-6442-2010
OI Hu, Xianluo/0000-0002-5769-167X
FU Natural Science Foundation of China [51002057]; 863 program of the MOST
   [2011AA11290]; PCSIRT (Program for Changjiang Scholars and Innovative
   Research Team in University)
FX This work was supported by the Natural Science Foundation of China
   (Grant no. 51002057), the 863 program of the MOST (Grant no.
   2011AA11290), and the PCSIRT (Program for Changjiang Scholars and
   Innovative Research Team in University). The authors thank the
   Analytical and Testing Center of HUST for XRD tests, and the State Key
   Laboratory of Materials Processing and Die & Mould Technology of HUST
   for TEM, TG/DSC, FE-SEM and EDS measurements.
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NR 36
TC 31
Z9 31
U1 27
U2 195
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 10
BP 3498
EP 3504
DI 10.1039/c3ta13994h
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AA7AQ
UT WOS:000331249900030
ER

PT J
AU Tang, H
   Tu, JP
   Liu, XY
   Zhang, YJ
   Huang, S
   Li, WZ
   Wang, XL
   Gu, CD
AF Tang, Hong
   Tu, Jiang-ping
   Liu, Xia-yuan
   Zhang, Yi-jun
   Huang, Sen
   Li, Wen-zheng
   Wang, Xiu-li
   Gu, Chang-dong
TI Self-assembly of Si/honeycomb reduced graphene oxide composite film as a
   binder-free and flexible anode for Li-ion batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID REVERSIBLE LITHIUM STORAGE; CARBON-COATED SILICON; NEGATIVE ELECTRODE;
   SI NANOPARTICLES; HIGH-CAPACITY; METAL-OXIDE; PERFORMANCE; SHEETS;
   NANOCOMPOSITE; HYBRID
AB A silicon/honeycomb graphene composite film synthesized by the "breath figure" method is developed as a high-performance anode material for lithium ion batteries. The honeycomb graphene structure can effectively prevent the agglomeration of the silicon nanoparticles, increase the electrical conductivity and reduce the transfer resistance of Li+. The composite film presents a high specific capacity and good cycling stability (1118 mAh g(-1) at 50 mA g(-1) up to 50 cycles), as well as an enhanced rate capability. This approach to prepare such a honeycomb porous structure is a low-cost and facile route for silicon-based anode materials.
C1 [Tang, Hong; Tu, Jiang-ping; Liu, Xia-yuan; Zhang, Yi-jun; Huang, Sen; Li, Wen-zheng; Wang, Xiu-li; Gu, Chang-dong] Zhejiang Univ, Dept Mat Sci & Engn, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
RP Tu, JP (reprint author), Zhejiang Univ, Dept Mat Sci & Engn, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China.
EM tujp@zju.edu.cn
FU National Science and Technology Support Program [2012BAC08B08]; Program
   for Innovative Research Team in University of Ministry of Education of
   China [IRT13037]; Key Science and Technology Innovation Team of Zhejiang
   Province [2010R50013]
FX This work is supported by the National Science and Technology Support
   Program (2012BAC08B08), the Program for Innovative Research Team in
   University of Ministry of Education of China (IRT13037) and Key Science
   and Technology Innovation Team of Zhejiang Province (2010R50013).
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NR 61
TC 31
Z9 31
U1 25
U2 149
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 16
BP 5834
EP 5840
DI 10.1039/c3ta15395a
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AD8OF
UT WOS:000333524800036
ER

PT J
AU Wu, FX
   Magasinski, A
   Yushin, G
AF Wu, Feixiang
   Magasinski, Alexandre
   Yushin, Gleb
TI Nanoporous Li2S and MWCNT-linked Li2S powder cathodes for lithium-sulfur
   and lithium-ion battery chemistries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID OXIDE COATINGS; PERFORMANCE; COMPOSITES; PARTICLES; CAPACITY; GRAPHENE;
   BINDER; CELLS; ANODE; ELECTROLYTES
AB In order to achieve high capacity utilization and high rate performance of lithium sulfide (Li2S) cathode materials, it is critical to identify scalable methods for low-cost preparation of nanostructured Li2S or Li2S-carbon composites. Here, we report on the preparation and characterization of nanoporous Li2S and multiwalled (MW) carbon nanotube (CNT) - linked Li2S powders, prepared for the first time via a versatile solution-based method. The addition of MWCNTs enhances electrical conductivity and structural stability of the Li2S-based cathodes and reduces polarization of cells operating at high current densities. The nanostructured Li2S-based cathodes containing 20wt% MWCNT showed promising discharge capacities of up to similar to 1050mA h g(S)(-1) at a slow rate of C/20 and similar to 800 mA h g(S)(-1) at a C/2 rate. Quite remarkably, without any electrolyte additives (such as polysulfides or lithium nitrate) MWCNT-linked Li2S cathodes demonstrated up to similar to 90% capacity retention after 100 cycles in half cells (vs. Li foil) at a C/5 and C/10 rates.
C1 [Wu, Feixiang; Magasinski, Alexandre; Yushin, Gleb] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
   [Wu, Feixiang] Cent S Univ, Sch Met & Environm, Changsha 410083, Peoples R China.
RP Yushin, G (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.
EM yushin@gatech.edu
RI Yushin, Gleb/B-4529-2013
OI Yushin, Gleb/0000-0002-3274-9265
FU Army Research Office (ARO grant) [W911NF-12-1-0259]; China Scholarship
   Council [201206370083]; National Science Foundation [DMR 0922776]
FX This work was partially supported by the Army Research Office (ARO grant
   W911NF-12-1-0259). Wu fellowship was supported by China Scholarship
   Council (no. 201206370083). The TEM used in this work was purchased
   using support from the National Science Foundation (project DMR
   0922776).
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NR 35
TC 31
Z9 31
U1 24
U2 124
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 17
BP 6064
EP 6070
DI 10.1039/c3ta14161f
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AD9JH
UT WOS:000333580700012
ER

PT J
AU Yu, HL
   Zhu, CL
   Zhang, K
   Chen, YJ
   Li, CY
   Gao, P
   Yang, PP
   Ouyang, QY
AF Yu, Hailong
   Zhu, Chunling
   Zhang, Kai
   Chen, Yujin
   Li, Chunyan
   Gao, Peng
   Yang, Piaoping
   Ouyang, Qiuyun
TI Three-dimensional hierarchical MoS2 nanoflake array/carbon cloth as
   high-performance flexible lithium-ion battery anodes
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID ELECTROCHEMICAL PERFORMANCES; STORAGE PROPERTIES; EXFOLIATED MOS2;
   COMPOSITE; CATHODE; PHOTOLUMINESCENCE; ELECTRODES; NANOSHEETS; GRAPHENE;
   SURFACE
AB Flexible lithium-ion batteries are the key to powering a new generation of flexible electronics such as roll-up displays, smart electronics, and wearable devices. Here we report, for the first time, one-step hydrothermal synthesis of a three-dimensional (3D) hierarchical MoS2 nanoflake array/carbon cloth which shows potential for improving the performance of flexible lithium-ion batteries. Structural characterizations show that the 3D hierarchical MoS2 nanoflake array/carbon cloth has a similar ordered woven structure to the bare carbon cloth. Each carbon microfiber is covered with many highly ordered 3D MoS2 nanoflake arrays, and a typical MoS2 nanoflake, with expanded spacing of the (002) crystal plane, has a uniform width of about 400 nm and a thickness of less than 15 nm. The flexible 3D MoS2 nanoflake array/carbon cloth as a flexible lithium-ion battery anode has a high reversible capacity of 3.0-3.5 mA h cm(-2) at a current density of 0.15 mA cm(-2) and outstanding discharging/charging rate stability. Moreover, a fabricated full battery, with commercial LiCoO2 powder and the hierarchical architectures as electrodes, exhibits high flexibility and good electrochemical performance, and can light a commercial red LED even after 50 cycles of bending the full battery.
C1 [Yu, Hailong; Zhang, Kai; Chen, Yujin; Li, Chunyan; Ouyang, Qiuyun] Harbin Engn Univ, Minist Educ, Key Lab In Fiber Intregrated Opt, Harbin 150001, Heilongjiang, Peoples R China.
   [Yu, Hailong; Zhang, Kai; Chen, Yujin; Li, Chunyan; Ouyang, Qiuyun] Harbin Engn Univ, Coll Sci, Harbin 150001, Heilongjiang, Peoples R China.
   [Zhu, Chunling; Gao, Peng; Yang, Piaoping] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Heilongjiang, Peoples R China.
RP Chen, YJ (reprint author), Harbin Engn Univ, Minist Educ, Key Lab In Fiber Intregrated Opt, Harbin 150001, Heilongjiang, Peoples R China.
EM chenyujin@hrbeu.edu.cn; gaopeng@hrbeu.edu.cn; yangpiaoping@hrbeu.edu.cn
FU National Natural Science Foundation of China [51272050, 61205113,
   21171045, 21001035]; Program for New Century Excellent Talents in
   University [NECT-10-0049]; 111 project of Ministry Education of China
   [B13015]
FX We thank the National Natural Science Foundation of China (Grant nos.
   51272050, 61205113, 21171045 and 21001035), Program for New Century
   Excellent Talents in University (NECT-10-0049) for the financial support
   of this research, and also the 111 project (B13015) of Ministry
   Education of China to the Harbin Engineering University.
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NR 44
TC 31
Z9 32
U1 56
U2 201
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
EI 2050-7496
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2014
VL 2
IS 13
BP 4551
EP 4557
DI 10.1039/c3ta14744d
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA AC3ZR
UT WOS:000332460800010
ER

PT J
AU Yu, MP
   Wang, AJ
   Wang, YS
   Li, C
   Shi, GQ
AF Yu, Mingpeng
   Wang, Aiji
   Wang, Yinshu
   Li, Chun
   Shi, Gaoquan
TI An alumina stabilized ZnO-graphene anode for lithium ion batteries via
   atomic layer deposition
SO NANOSCALE
LA English
DT Article
ID ENHANCED ELECTROCHEMICAL PERFORMANCE; NEGATIVE ELECTRODES; STORAGE
   CAPABILITY; TIN OXIDES; NANOCOMPOSITES; NANOPARTICLES; COMPOSITES; LIFE
AB Atomic layer deposition (ALD) was applied to deposit ZnO on graphene aerogel, and this composite was used as an anode material for lithium ion batteries. This electrode material was further modified by an ultrathin Al2O3 layer via ALD to stabilize its electrochemical stability. These two metal oxides were uniformly immobilized on graphene frameworks, and the Al2O3 coating strongly improved the electrochemical performances of ZnO-graphene aerogel composite anodes. Particularly, the composite with 10 ALD cycles of Al2O3 coating (denoted as ZnO-G-10) exhibited a high initial discharge capacity of 1513 mA h g(-1) and maintained a reversible capacity of 490 mA h g(-1) after 100 cycles at a current density of 100 mA g(-1). Furthermore, the capacity retention rate increased from 70% to 90% in comparison with its uncoated counterpart after 100 cycles. The ZnO-G-10 anode also showed good rate-capability, delivering a discharge capacity of 415 mA h g(-1) at 1000 mA g(-1). The improved electrochemical performance is attributed to the formation of an artificial solid electrolyte interphase layer, stabilizing ZnO and the electrolyte by preventing the aggregation of Zn/ZnO nanograins and the side reaction that would cause the degradation of anodes.
C1 [Yu, Mingpeng; Li, Chun; Shi, Gaoquan] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
   [Wang, Aiji; Wang, Yinshu] Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China.
RP Shi, GQ (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China.
EM gshi@tsinghua.edu.cn
FU National Basic Research Program of China (973 Program) [2012CB933402,
   2013CB933001]; Natural Science Foundation of China [51161120361,
   91027028]; China Postdoctoral Science Foundation [2014M550708]
FX This work was supported by the National Basic Research Program of China
   (973 Program, 2012CB933402, 2013CB933001), Natural Science Foundation of
   China (51161120361, 91027028) and the China Postdoctoral Science
   Foundation (2014M550708).
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NR 38
TC 31
Z9 31
U1 25
U2 124
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 19
BP 11419
EP 11424
DI 10.1039/c4nr02576h
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AU2LR
UT WOS:000345450300043
PM 25148141
ER

PT J
AU Dong, YC
   Ma, RG
   Hu, MJ
   Cheng, H
   Yang, QD
   Li, YY
   Zapien, JA
AF Dong, Yucheng
   Ma, Ruguang
   Hu, Mingjun
   Cheng, Hua
   Yang, Qingdan
   Li, Yang Yang
   Zapien, Juan Antonio
TI Thermal evaporation-induced anhydrous synthesis of Fe3O4-graphene
   composite with enhanced rate performance and cyclic stability for
   lithium ion batteries
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID NEGATIVE ELECTRODE MATERIAL; ANODE MATERIAL; ELECTROCHEMICAL
   PERFORMANCE; REVERSIBLE CAPACITY; STORAGE CAPACITY; GRAPHENE; LI;
   NANOCOMPOSITES; OXIDE; NANOPARTICLES
AB We present a high-yield and low cost thermal evaporation-induced anhydrous strategy to prepare hybrid materials of Fe3O4 nanoparticles and graphene as an advanced anode for high-performance lithium ion batteries. The similar to 10-20 nm Fe3O4 nanoparticles are densely anchored on conducting graphene sheets and act as spacers to keep the adjacent sheets separated. The Fe3O4-graphene composite displays a superior battery performance with high retained capacity of 868 mA h g(-1) up to 100 cycles at a current density of 200 mA g(-1), and 539 mA h g(-1) up to 200 cycles when cycling at 1000 mA g(-1), high Coulombic efficiency (above 99% after 200 cycles), good rate capability, and excellent cyclic stability. The simple approach offers a promising route to prepare anode materials for practical fabrication of lithium ion batteries.
C1 [Dong, Yucheng; Yang, Qingdan; Li, Yang Yang; Zapien, Juan Antonio] City Univ Hong Kong, Ctr Super Diamond & Adv Films, Hong Kong, Hong Kong, Peoples R China.
   [Dong, Yucheng; Ma, Ruguang; Hu, Mingjun; Cheng, Hua; Yang, Qingdan; Zapien, Juan Antonio] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China.
RP Zapien, JA (reprint author), City Univ Hong Kong, Ctr Super Diamond & Adv Films, Hong Kong, Hong Kong, Peoples R China.
EM apjazs@cityu.edu.hk
RI Li, Yang Yang/J-9243-2012
FU Research Grants Council of the Hong Kong Special Administrative Region,
   China [CityU 103409]
FX The authors acknowledge support by a grant from the Research Grants
   Council of the Hong Kong Special Administrative Region, China (Project
   No. CityU 103409).
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NR 58
TC 31
Z9 31
U1 6
U2 108
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 1463-9076
J9 PHYS CHEM CHEM PHYS
JI Phys. Chem. Chem. Phys.
PY 2013
VL 15
IS 19
BP 7174
EP 7181
DI 10.1039/c3cp50588j
PG 8
WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
SC Chemistry; Physics
GA 131GK
UT WOS:000317980600023
PM 23558566
ER

PT J
AU Kim, HJ
   Wen, ZH
   Yu, KH
   Mao, O
   Chen, JH
AF Kim, Haejune
   Wen, Zhenhai
   Yu, Kehan
   Mao, Ou
   Chen, Junhong
TI Straightforward fabrication of a highly branched graphene nanosheet
   array for a Li-ion battery anode
SO JOURNAL OF MATERIALS CHEMISTRY
LA English
DT Article
ID CHEMICAL-VAPOR-DEPOSITION; CARBON NANOWALLS; LITHIUM STORAGE; REVERSIBLE
   CAPACITY; HIGH-PERFORMANCE; INSERTION; NANOSTRUCTURES; MODEL; GAS
AB A new graphene-based hybrid nanostructure is designed for anode materials in lithium-ion batteries. The highly branched graphene nanosheets (HBGNs) directly grown on a copper current collector exhibited promising electrochemical performance due to their unique morphology, high electrical conductivity, large interfacial surface area, and high porosity.
C1 [Kim, Haejune; Wen, Zhenhai; Yu, Kehan; Chen, Junhong] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA.
   [Mao, Ou] Global Technol & Innovat Power Solut Johnson Con, Milwaukee, WI 53209 USA.
RP Chen, JH (reprint author), Univ Wisconsin, Dept Mech Engn, 3200 N Cramer St, Milwaukee, WI 53211 USA.
EM jhchen@uwm.edu
RI wen, zhenhai/D-7165-2011; Yu, Kehan/H-3833-2011
OI wen, zhenhai/0000-0002-0397-4156; 
FU National Science Foundation [CMMI-0900509]; U.S. Department of Energy
   [DE-EE0003208]; Johnson Controls, Inc.; We Energies
FX The authors acknowledge financial support from the National Science
   Foundation (CMMI-0900509), the U.S. Department of Energy (DE-EE0003208),
   Johnson Controls, Inc., and We Energies. The SEM imaging was conducted
   at the UWM Bioscience Electron Microscope Facility, and TEM analyses
   were conducted at the UWM Physics HRTEM Laboratory.
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NR 34
TC 31
Z9 31
U1 4
U2 47
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 0959-9428
J9 J MATER CHEM
JI J. Mater. Chem.
PY 2012
VL 22
IS 31
BP 15514
EP 15518
DI 10.1039/c2jm33150k
PG 5
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 975AR
UT WOS:000306479600008
ER

PT J
AU Zhou, WW
   Tay, YY
   Jia, XT
   Wai, DYY
   Jiang, J
   Hng, HH
   Yu, T
AF Zhou, Weiwei
   Tay, Yee Yan
   Jia, Xingtao
   Wai, Denis Yu Yau
   Jiang, Jian
   Hng, Huey Hoon
   Yu, Ting
TI Controlled growth of SnO2@Fe2O3 double-sided nanocombs as anodes for
   lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID CORE-SHELL HETEROSTRUCTURES; NANOCRYSTAL HETEROSTRUCTURES; STRUCTURAL
   CHARACTERISTICS; PHOTOCATALYTIC ACTIVITY; NANOSTRUCTURES; PERFORMANCE;
   STORAGE; EFFICIENCY; CAPACITY; GRAPHENE
AB A novel heterostructure is developed by grafting 1D SnO2 nanorods onto both sides of pre-grown 2D F(e)2O(3) nanoflakes, forming a comb-like rather than tree-like branched nanostructure. The SnO2 nanorod branches are determined to grow along the [001] direction on the (+/-001) planes of Fe2O3 nanoflakes. The resulting SnO2@Fe2O3 nanocombs show stabilized cycling performance and improved volumetric energy density compared to pristine Fe2O3 nanoflakes presumably due to the integration of SnO2 branches as well as the 3D hierarchical structural features.
C1 [Zhou, Weiwei; Jia, Xingtao; Jiang, Jian; Yu, Ting] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore.
   [Tay, Yee Yan; Hng, Huey Hoon] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore.
   [Wai, Denis Yu Yau; Yu, Ting] Energy Res Inst NTU ERIAN, Singapore 637553, Singapore.
   [Yu, Ting] Natl Univ Singapore, Dept Phys, Fac Sci, Singapore 117542, Singapore.
RP Yu, T (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link, Singapore 637371, Singapore.
EM yuting@ntu.edu.sg
RI Hng, Huey Hoon/A-2246-2011; jiang, jian/F-9144-2011; 
OI Hng, Huey Hoon/0000-0002-8950-025X; jiang, jian/0000-0002-9175-4582; Yu,
   Ting/0000-0002-0113-2895; Yu, Denis/0000-0002-5883-7087
FU Singapore National Research Foundation under NRF RF [NRF-RF2010-07]; MOE
   [MOE 2009-T2-1-037]
FX This work is supported by the Singapore National Research Foundation
   under NRF RF award no. NRF-RF2010-07 and MOE Tier 2 MOE 2009-T2-1-037.
CR Xie H, 2010, J PHYS CHEM C, V114, P9706, DOI 10.1021/jp102525y
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NR 42
TC 31
Z9 31
U1 15
U2 137
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 15
BP 4459
EP 4463
DI 10.1039/c2nr31239e
PG 5
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 973AS
UT WOS:000306324000018
PM 22740439
ER

PT J
AU Wan, LJ
   Ren, ZY
   Wang, H
   Wang, G
   Tong, X
   Gao, SH
   Bai, JT
AF Wan, Lijuan
   Ren, Zhaoyu
   Wang, Hui
   Wang, Gang
   Tong, Xin
   Gao, Shuanghong
   Bai, Jintao
TI Graphene nanosheets based on controlled exfoliation process for enhanced
   lithium storage in lithium-ion battery
SO DIAMOND AND RELATED MATERIALS
LA English
DT Article
DE Graphite oxide; Graphene nanosheets; Electrochemical performances;
   Exfoliation process
ID MONOLAYER GRAPHENE; ELECTROCHEMICAL PERFORMANCE; ANODE MATERIAL; LI
   STORAGE; CARBON; GRAPHITE; CAPACITY; SHEETS; OXIDATION; OXIDE
AB A facile and rapid approach was used for the fabrication of chemically derived graphene nanosheets based on the reduction of graphite oxide (GO) in tube furnace assembly at different temperatures. The morphologies, microstructures, specific surface areas and other features of GO and graphene nanosheets were characterized. Structure characterization indicates that the platelet thickness of graphene nanosheets obtained at 300 C was 1.62 nm, which corresponds to an approximately 5 layers stacking of the monoatomic graphene nanosheets. Electrochemical performances of the as-prepared graphene nanosheets were performed, the result of which could prove the above observation that graphene nanosheets (5 layers) obtained at 300 C actually displayed the most remarkable electrochemical performances: the first discharge and charge capacities of graphene nanosheets were as high as 2137 mAh/g and 994 mAh/g, respectively, and after 100 cycles graphene nanosheets still possessed a high capacity of 478 mAh/g. (C) 2011 Elsevier B.V. All rights reserved.
C1 [Wan, Lijuan; Ren, Zhaoyu; Gao, Shuanghong; Bai, Jintao] NW Univ Xian, Natl Key Lab Photoelect Technol & Funct Mat, Culture Base, Xian 710069, Peoples R China.
   [Wan, Lijuan; Ren, Zhaoyu; Gao, Shuanghong; Bai, Jintao] NW Univ Xian, Applicat Sci & Technol Int Cooperat Base, Xian 710069, Peoples R China.
   [Wang, Hui; Wang, Gang; Tong, Xin] NW Univ Xian, Coll Chem & Mat Sci, Key Lab Synthet & Nat Funct Mol Chem, Minist Educ, Xian 710069, Peoples R China.
RP Ren, ZY (reprint author), NW Univ Xian, Natl Key Lab Photoelect Technol & Funct Mat, Culture Base, Xian 710069, Peoples R China.
EM rzy@nwu.edu.cn; huiwang@nwu.edu.cn
FU National Basic Research Program of China (973 Program) [2009CB626611];
   National Natural Science Foundation of China [21061130551, 20873099,
   10974152]; Ph. D. Programs Foundation of Ministry of Education of China
   [20096101110002]; NWU Doctorate Dissertation of Excellence Funds
   [09YYB04]; NWU Graduate Cross-discipline Funds [09YJC28]
FX The project was supported by the National Basic Research Program of
   China (973 Program) (No. 2009CB626611), the international cooperation
   research program of National Natural Science Foundation of China (No.
   21061130551), the Ph. D. Programs Foundation of Ministry of Education of
   China (No. 20096101110002), the National Natural Science Foundation of
   China (Nos. 20873099 and 10974152), NWU Doctorate Dissertation of
   Excellence Funds (09YYB04), and NWU Graduate Cross-discipline Funds
   (09YJC28).
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NR 27
TC 31
Z9 33
U1 3
U2 54
PU ELSEVIER SCIENCE SA
PI LAUSANNE
PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND
SN 0925-9635
J9 DIAM RELAT MATER
JI Diam. Relat. Mat.
PD MAY-JUN
PY 2011
VL 20
IS 5-6
BP 756
EP 761
DI 10.1016/j.diamond.2011.03.027
PG 6
WC Materials Science, Multidisciplinary
SC Materials Science
GA 779KE
UT WOS:000291775700022
ER

PT J
AU Meng, WJ
   Chen, W
   Zhao, L
   Huang, Y
   Zhu, MS
   Huang, Y
   Fu, YQ
   Geng, FX
   Yu, J
   Chen, XF
   Zhi, CY
AF Meng, Wenjun
   Chen, Wei
   Zhao, Lei
   Huang, Yang
   Zhu, Minshen
   Huang, Yan
   Fu, Yuqiao
   Geng, Fengxia
   Yu, Jie
   Chen, Xianfeng
   Zhi, Chunyi
TI Porous Fe3O4/carbon composite electrode material prepared from
   metal-organic framework template and effect of temperature on its
   capacitance
SO NANO ENERGY
LA English
DT Article
DE Metal organic framework; Fe3O4; Composite; Supercapacitor; Temperature
   effect
ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL CAPACITORS; ASYMMETRIC
   SUPERCAPACITORS; ANODE MATERIALS; PERFORMANCE; CARBON; GRAPHENE;
   HYBRIDS; STORAGE
AB In this paper, we report a porous Fe3O4/carbon composite supercapacitor electrode material possessing great temperature variation-resistive long-term cycle stability. The material is prepared via a facile one-step calcination of an iron-based metal organic framework (Fe-MOF) template and composed of porous Fe3O4 nanoparticles and carbon as a result of a well-controlled incomplete annealing process of the MOF template. With this material as an electrode, a specific capacitance of 139 F g(-1) at a discharging current density of 0.5 A g(-1) can be achieved. More attractively, the specific capacitance is significantly increased when the working temperature is elevated from 0 to 60 degrees C. Furthermore, even after 4000 cycles of charge-discharge at varied temperatures, 83.3% of the capacitance of the electrode material is retained, showing excellent temperature variation-resistive long-term cycle stability of the prepared composite electrode material. (C) 2014 Elsevier Ltd. All rights reserved.
C1 [Meng, Wenjun; Chen, Wei; Huang, Yang; Zhu, Minshen; Huang, Yan; Fu, Yuqiao; Chen, Xianfeng; Zhi, Chunyi] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Peoples R China.
   [Zhao, Lei; Yu, Jie] Univ Town, Shenzhen Grad Sch, Harbin Inst Technol, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China.
   [Geng, Fengxia] Soochow Univ, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China.
   [Chen, Xianfeng] City Univ Hong Kong, Ctr Super Diamond & Adv Films COSDAF, Dept Phys & Mat Sci, Hong Kong, Peoples R China.
   [Zhi, Chunyi] City Univ Hong Kong, Shenzhen Res Inst, Shenzhen, PR, Peoples R China.
RP Chen, XF (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, 83 Tat Chee Ave, Kowloon, Peoples R China.
EM xianfeng.chen@cityu.edu.hk; cy.zhi@cityu.edu.hk
OI ZHI, Chunyi/0000-0001-6766-5953
FU Early Career Scheme of the Research Grants Council of Hong Kong SAR,
   China [CityU 9041977]; Science Technology and Innovation Committee of
   Shenzhen Municipality [R-IND4901]; City University of Hong Kong
   [7200337]
FX This research was supported by the Early Career Scheme of the Research
   Grants Council of Hong Kong SAR, China, under Project numbers CityU
   9041977, the Science Technology and Innovation Committee of Shenzhen
   Municipality (Grant number R-IND4901), and a grant (7200337) from the
   City University of Hong Kong.
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NR 33
TC 30
Z9 30
U1 106
U2 466
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 2211-2855
EI 2211-3282
J9 NANO ENERGY
JI Nano Energy
PD SEP
PY 2014
VL 8
BP 133
EP 140
DI 10.1016/j.nanoen.2014.06.007
PG 8
WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
   Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AO0EK
UT WOS:000340981700017
ER

PT J
AU Li, L
   Zhou, GM
   Shan, XY
   Pei, SF
   Li, F
   Cheng, HM
AF Li, Lu
   Zhou, Guangmin
   Shan, Xu-Yi
   Pei, Songfeng
   Li, Feng
   Cheng, Hui-Ming
TI Co3O4 mesoporous nanostructures@graphene membrane as an integrated anode
   for long-life lithium-ion batteries
SO JOURNAL OF POWER SOURCES
LA English
DT Article
DE Mesoporous Co3O4; Controllable structures; Graphene membrane; Integrated
   anode; Lithium-ion batteries
ID HIGH-PERFORMANCE; REVERSIBLE CAPACITY; CURRENT COLLECTORS; STORAGE;
   COMPOSITE; NANOPARTICLES; LIGHTWEIGHT; ELECTRODES; NANOSHEETS; PARTICLES
AB One of the most attractive research areas in lithium-ion batteries (LIBs) is to design elaborate nano-structure of the electrode, which has been considered as keys to solve the problems such as the low energy density, slow lithium ion and electron transport, and the large volume change of electrode materials during cycling processes. Here, mesoporous CO3O4 with controllable structures was directly grown on a graphene membrane by hydrothermal reaction followed by annealing treatment, and used as an integrated anode in LIBs without using metallic current collector, binder and conductive additive. The light graphene membrane as current collector with high electrical conductivity and stability contributes to the high energy density of LIBs. A mesoporous structure with enough space is beneficial to lithium ion diffusion and strain buffer of CO3O4 during discharge/charge processes, rendering the electrodes high performance. The integrated electrode shows good rate capability and impressive cycling stability without capacity loss over 500 cycles under a high current density of 500 mA g(-1). (C) 2014 Elsevier B.V. All rights reserved.
C1 [Li, Lu; Zhou, Guangmin; Shan, Xu-Yi; Pei, Songfeng; Li, Feng; Cheng, Hui-Ming] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.
RP Li, F (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China.
EM fli@imr.ac.cn
RI Cheng, Hui-Ming/B-8682-2012; Pei, Songfeng/E-5598-2010
FU Key Research Program of Ministry of Science and Technology, China
   [2014CB932402, 2012AA030303]; National Science Foundation of China
   [51221264, 51172239, 51372253]; Chinese Academy of Sciences
   [XDA01020304]
FX This work was supported by the Key Research Program of Ministry of
   Science and Technology, China (Nos. 2014CB932402 and 2012AA030303), the
   National Science Foundation of China (Nos. 51221264, 51172239 and
   51372253), and the " Strategic Priority Research Program" of the Chinese
   Academy of Sciences (No. XDA01020304).
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NR 43
TC 30
Z9 30
U1 23
U2 289
PU ELSEVIER SCIENCE BV
PI AMSTERDAM
PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0378-7753
EI 1873-2755
J9 J POWER SOURCES
JI J. Power Sources
PD JUN 1
PY 2014
VL 255
BP 52
EP 58
DI 10.1016/j.jpowsour.2013.12.129
PG 7
WC Electrochemistry; Energy & Fuels
SC Electrochemistry; Energy & Fuels
GA AC3QN
UT WOS:000332436400008
ER

PT J
AU Li, WH
   Yang, ZZ
   Cheng, JX
   Zhong, XW
   Gu, L
   Yu, Y
AF Li, Weihan
   Yang, Zhenzhong
   Cheng, Jianxiu
   Zhong, Xiongwu
   Gu, Lin
   Yu, Yan
TI Germanium nanoparticles encapsulated in flexible carbon nanofibers as
   self-supported electrodes for high performance lithium-ion batteries
SO NANOSCALE
LA English
DT Article
ID HIGH-CAPACITY; ANODE MATERIAL; GE NANOWIRES; ELECTROCHEMICAL PROPERTIES;
   RATE CAPABILITY; STORAGE; GRAPHENE; SILICON; SINGLE; GROWTH
AB Germaniumis a promising high-capacity anode material for lithium ion batteries, but still suffers from poor cyclability due to its huge volume variation during the Li-Ge alloy/dealloy process. Here we rationally designed a flexible and self-supported electrode consisting of Ge nanoparticles encapsulated in carbon nanofibers (Ge-CNFs) by using a facile electrospinning technique as potential anodes for Li-ion batteries. The Ge-CNFs exhibit excellent electrochemical performance with a reversible specific capacity of similar to 1420 mA h g (1) after 100 cycles at 0.15 C with only 0.1% decay per cycle (the theoretical specific capacity of Ge is 1624 mA h g(-1)). When cycled at a high current of 1 C, they still deliver a reversible specific capacity of 829 mA h g(-1) g(-1) after 250 cycles. The strategy and design are simple, effective, and versatile. This type of flexible electrodes is a promising solution for the development of flexible lithium-ion batteries with high power and energy densities.
C1 [Li, Weihan; Cheng, Jianxiu; Zhong, Xiongwu; Yu, Yan] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China.
   [Yang, Zhenzhong; Gu, Lin] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China.
RP Yu, Y (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China.
EM yanyumse@ustc.edu.cn
RI Yu, Yan/C-7031-2012; Yang, Zhenzhong/O-2344-2014; Li, Weihan/D-7815-2016
OI Yang, Zhenzhong/0000-0002-7226-7973; Li, Weihan/0000-0001-5075-2719
FU National Natural Science Foundation of China [21171015, 21373195]; "1000
   plan" from the Chinese Government; program for New Century Excellent
   Talents in the University [NCET-12-0515]; Fundamental Research Funds for
   the Central Universities [WK2060140014]; sofja kovalevskaja award from
   the Alexander von Humboldt Foundation
FX This work was financially supported by the National Natural Science
   Foundation of China (no. 21171015 and no. 21373195), the "1000 plan"
   from the Chinese Government, the program for New Century Excellent
   Talents in the University (NCET-12-0515), the Fundamental Research Funds
   for the Central Universities (WK2060140014) and the sofja kovalevskaja
   award from the Alexander von Humboldt Foundation.
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NR 52
TC 30
Z9 30
U1 33
U2 145
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
EI 2040-3372
J9 NANOSCALE
JI Nanoscale
PY 2014
VL 6
IS 9
BP 4532
EP 4537
DI 10.1039/c4nr00140k
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA AF6WO
UT WOS:000334855500015
PM 24663690
ER

PT J
AU Ding, Y
   Li, GR
   Xiao, CW
   Gao, XP
AF Ding, Y.
   Li, G. R.
   Xiao, C. W.
   Gao, X. P.
TI Insight into effects of graphene in Li4Ti5O12/carbon composite with high
   rate capability as anode materials for lithium ion batteries
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Lithium-ion batteries; Anode; Li4Ti5O12; Graphene; High-rate capability
ID CARBON-COATED LI4TI5O12; SOLID-STATE REACTION; ELECTROCHEMICAL
   PERFORMANCE; GRAPHITE OXIDE; NANO-TUBES; NANOTUBES; TITANATE;
   NANOSHEETS; ELECTRODE; STORAGE
AB Li4Ti5O12/carbon composites have shown promising high rate capability as anode materials for lithium ion batteries. In this paper, unique effects of graphene in Li4Ti5O12/carbon composites on electrochemical performances are focused by means of comparing Li4Ti5O12/graphene with Li4Ti5O12/conductive carbon black (CCB) and Li4Ti5O12. The investigated anode materials are synthesized by a facile hydrothermal method. The amount of graphene or CCB in the Li4Ti5O12/carbon composites is about 3 wt% measured by thermogravimetric (TG) analysis. X-ray diffraction (XRD), scanning electron microscopy (SEM) and transmission electron microscopy (TEM) show that Li4Ti5O12/graphene consists of small sized Li4Ti5O12 nanocrystals supported on graphene nanosheets, while Li4Ti5O12/CCB comprises Li4Ti5O12 nanocrystal aggregates coated nearly by graphited carbon. The electrochemical performances of these samples as anode materials for lithium ion batteries are investigated by galvanostatic charge-discharge method. Li4Ti5O12/graphene provides a superior rate capability. At the high current density of 1600 mAg(-1), the reversible capacity after 200 cycles is still more than 120 mAh g(-1), which is about 40% higher than that of Li4Ti5O12/CCB. Cyclic voltammetry (CV) demonstrates that stronger pseudocapacitive effect occurs on Li4Ti5O12/graphene than on Li4Ti5O12/CCB. This derived from the structure features that graphene-supported small Li4Ti5O12 nanocrystals provide more surface active sites for the lithium ion insertion/extraction. The strong pseudocapacitive effect is responsible for the improvements of capacity and high-rate capability. Further, electrochemical impedance spectra (EIS) show that Li4Ti5O12/graphene electrode have lower charge transfer resistance and smaller diffusion impedance, indicating the obvious advantages in electrode kinetics over Li4Ti5O12 and Li4Ti5O12/CCB. The results clarify the positive effects of graphene in Li4Ti5O12/carbon composites as anode materials for lithium ion batteries. (c) 2013 Elsevier Ltd. All rights reserved.
C1 [Ding, Y.; Li, G. R.; Xiao, C. W.; Gao, X. P.] Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Tianjin 300071, Peoples R China.
RP Li, GR (reprint author), Nankai Univ, Inst New Energy Mat Chem, Tianjin Key Lab Met & Mol Based Mat Chem, Tianjin 300071, Peoples R China.
EM guoranli@nankai.edu.cn; xpgao@nankai.edu.cn
RI Li, Guoran/D-5091-2012
FU 973 Program [2009CB220100]
FX Financial support from the 973 Program (2009CB220100) is greatly
   appreciated.
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NR 44
TC 30
Z9 31
U1 21
U2 176
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JUL 15
PY 2013
VL 102
BP 282
EP 289
DI 10.1016/j.electacta.2013.04.002
PG 8
WC Electrochemistry
SC Electrochemistry
GA 178XS
UT WOS:000321481300035
ER

PT J
AU Cheng, JL
   Wang, B
   Xin, HLL
   Yang, GC
   Cai, HQ
   Nie, FD
   Huang, H
AF Cheng, Jianli
   Wang, Bin
   Xin, Huolin L.
   Yang, Guangcheng
   Cai, Huaqiang
   Nie, Fude
   Huang, Hui
TI Self-assembled V2O5 nanosheets/reduced graphene oxide hierarchical
   nanocomposite as a high-performance cathode material for lithium ion
   batteries
SO JOURNAL OF MATERIALS CHEMISTRY A
LA English
DT Article
ID HIGH-POWER; STORAGE PROPERTIES; CAPACITY; INTERCALATION; COMPOSITE;
   SUPERCAPACITORS; MICROSPHERES; CAPABILITY; ELECTRODES; NANOTUBES
AB A simple solvothermal method was used to prepare self-assembled V2O5 nanosheets/reduced graphene oxide (RGO) hierarchical nanocomposite. In this nanocomposite, the V2O5 nanosheets assembling on the RGO constitute a 3-D hierarchical nanostructure with high specific surface area and good electronic/ionic conducting path. When used as the cathode materials, the V2O5 nanosheets/RGO nanocomposites exhibit highly reversible capacity and good rate capability relative to the bulk material. The V2O5 nanosheets/RGO nanocomposite anode was able to charge/discharge at high current densities of 3000 mA g(-1) (10 C), 6000 mA g(-1) (20 C) and 15 A g(-1) (50 C), with discharge capacities of approximately 138, 112 and 76 mA h g(-1), respectively. Meanwhile, a discharge capacity of 102 mA h g(-1) can be delivered after 160 cycles at 2 C, showing a good cycling stability. The improved performance could be attributed to the enhanced electron transport and Li+ diffusion that results from the hierarchical nanostructure of V2O5 nanosheets/RGO nanocomposites.
C1 [Cheng, Jianli; Wang, Bin; Yang, Guangcheng; Cai, Huaqiang; Nie, Fude; Huang, Hui] China Acad Engn Phys, Inst Chem Mat, New Mat R&D Ctr, Mianyang 621900, Sichuan, Peoples R China.
   [Xin, Huolin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.
RP Wang, B (reprint author), China Acad Engn Phys, Inst Chem Mat, New Mat R&D Ctr, Mianyang 621900, Sichuan, Peoples R China.
EM edward.bwang@gmail.com; huanghui@caep.ac.cn
RI cheng, Jianli/K-1496-2014; Cheng, Jianli/K-4478-2014; Xin,
   Huolin/E-2747-2010
OI Xin, Huolin/0000-0002-6521-868X
FU Startup Foundation of China Academy of Engineering Physics, Institute of
   Chemical Materials [KJCX201301]
FX This work was supported by the Startup Foundation of China Academy of
   Engineering Physics, Institute of Chemical Materials (KJCX201301). This
   research made use of the TEM facility supported by Materials Sciences
   Division at Lawrence Berkeley National Laboratory. The authors thank Dr
   Chunjoong Kim and Mr Xiangyun Song for helpful analysis discussion.
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NR 42
TC 30
Z9 31
U1 17
U2 120
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2050-7488
J9 J MATER CHEM A
JI J. Mater. Chem. A
PY 2013
VL 1
IS 36
BP 10814
EP 10820
DI 10.1039/c3ta12066j
PG 7
WC Chemistry, Physical; Energy & Fuels; Materials Science,
   Multidisciplinary
SC Chemistry; Energy & Fuels; Materials Science
GA 203FJ
UT WOS:000323276200031
ER

PT J
AU Li, L
   Seng, KH
   Chen, ZX
   Liu, HK
   Nevirkovets, IP
   Guo, ZP
AF Li, Li
   Seng, Kuok Hau
   Chen, Zhixin
   Liu, Huakun
   Nevirkovets, Ivan P.
   Guo, Zaiping
TI Synthesis of Mn3O4-anchored graphene sheet nanocomposites via a facile,
   fast microwave hydrothermal method and their supercapacitive behavior
SO ELECTROCHIMICA ACTA
LA English
DT Article
DE Microwave hydrothermal; Graphene; Mn3O4; Nanocomposite; Supercapacitor
ID LITHIUM ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; ELECTRODE
   MATERIAL; MANGANESE OXIDES; HIGH-PERFORMANCE; CARBON NANOTUBE; ANODE
   MATERIALS; CAPACITORS; COMPOSITE; NANOPARTICLES
AB Well-crystallized Mn3O4-anchored reduced graphene oxide (rGO) nanocomposites have been successfully synthesized via a facile, effective, energy-saving, and scalable microwave hydrothermal technique for potential application as supercapacitor material. Integrating these nanostructures resulted in a strong synergistic effect between the two materials, consequently leading to a hybrid composite with higher specific capacitance compared to the bare Mn3O4 nanoparticles. The results from different sorts of characterization indicate that the Mn3O4 particles were deposited and anchored on graphene sheets. The capacitance value of the rGO(31.6%) Mn3O4 nanocomposite reached 153 F/g, much higher than that of the bare Mn3O4 (87 F/g) at a scan rate of 5 mV/s in the potential range from -0.1 V to 0.8 V. More importantly, a 200% increase in capacitance was observed for the nanocomposite with cycling at 10 mV/s due to electrochemical activation and the oxidization of Mn(II,III) to Mn(IV) during cycling, as verified by Xray photoelectron spectroscopy. There is no observable capacitance fading up to 1000 cycles. The facile synthesis method and good electrochemical properties indicate that the nanocomposite could be an electrode candidate for supercapacitors. (C) 2012 Elsevier Ltd. All rights reserved.
C1 [Li, Li; Seng, Kuok Hau; Liu, Huakun; Nevirkovets, Ivan P.; Guo, Zaiping] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2519, Australia.
   [Chen, Zhixin; Guo, Zaiping] Univ Wollongong, Sch Mech Mat & Mech Engn, Wollongong, NSW 2522, Australia.
RP Guo, ZP (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Squires Way, Wollongong, NSW 2519, Australia.
EM zguo@uow.edu.au
RI Liu, Hua/G-1349-2012
OI Liu, Hua/0000-0002-0253-647X
FU Australian Research Council (ARC) [DP1094261]
FX This work was funded by an Australian Research Council (ARC) Discovery
   Project (DP1094261). The authors also would like to thank Dr. Tania
   Silver at the University of Wollongong for critical reading of the
   manuscript, as well as Mr. Darren Attard and Mr. Alfred Chidembo for
   their great contributions.
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TC 30
Z9 32
U1 20
U2 196
PU PERGAMON-ELSEVIER SCIENCE LTD
PI OXFORD
PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0013-4686
J9 ELECTROCHIM ACTA
JI Electrochim. Acta
PD JAN 1
PY 2013
VL 87
BP 801
EP 808
DI 10.1016/j.electacta.2012.08.127
PG 8
WC Electrochemistry
SC Electrochemistry
GA 093DE
UT WOS:000315171100102
ER

PT J
AU Han, PX
   Yue, YH
   Zhang, LX
   Xu, HX
   Liu, ZH
   Zhang, KJ
   Zhang, CJ
   Dong, SM
   Ma, W
   Cui, GL
AF Han, Pengxian
   Yue, Yanhua
   Zhang, Lixue
   Xu, Hongxia
   Liu, Zhihong
   Zhang, Kejun
   Zhang, Chuanjian
   Dong, Shanmu
   Ma, Wen
   Cui, Guanglei
TI Nitrogen-doping of chemically reduced mesocarbon microbead oxide for the
   improved performance of lithium ion batteries
SO CARBON
LA English
DT Article
ID LI STORAGE PROPERTIES; ANODE MATERIAL; ELECTROCHEMICAL IMPEDANCE;
   CARBON; GRAPHITE; GRAPHENE; INSERTION; CHALLENGES; REDUCTION; COMPOSITE
AB Nitrogen was doped into chemically-reduced mesocarbon microbead oxide (CR-MCMBO) through simple annealing in ammonia at 800 degrees C, and the Li-ion storage properties of the prepared nitrogen-doped CR-MCMBO (NR-MCMBO) was studied. It was found that NR-MCMBO shows a highly reversible capacity of 762 mAh g(-1) at 20 mA g(-1) during the first charge process, which is much higher than that of the pristine MCMB (289 mAh g(-1)), and the specific capacity of NR-MCMBO still had a value of 535 mAh g(-1) after 200 cycles. When the current density reaches 1000 mA g(-1), the specific capacity of NR-MCMBO is 388 mAh g(-1). The high reversible capacity of NR-MCMBO is attributed to the high amount of pyridinic nitrogen and the large number of defects induced by oxidation and nitrogen-doping. Moreover, the open pores constituted by graphene-like nanoplatelets on the spherical NR-MCMBO surface facilitate the diffusion of Li ions. Crown Copyright (C) 2011 Published by Elsevier Ltd. All rights reserved.
C1 [Han, Pengxian; Yue, Yanhua; Zhang, Lixue; Xu, Hongxia; Liu, Zhihong; Zhang, Kejun; Zhang, Chuanjian; Dong, Shanmu; Ma, Wen; Cui, Guanglei] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
RP Cui, GL (reprint author), Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China.
EM cuigl@qibebt.ac.cn
RI Cui, Guanglei/D-4816-2011; Han, Pengxian/D-6159-2011; Zhang,
   Lixue/G-2721-2010
FU Chinese Academy of Sciences; National Key Basic Research Program of
   China [2011CB935700]; Shandong Province Funds for Distinguished Young
   Scientist [JQ200906]; National Natural Science Foundation of China
   [20971077]
FX We appreciate the support of "100 Talents" program of the Chinese
   Academy of Sciences, National Key Basic Research Program of China (Grant
   No. 2011CB935700), Shandong Province Funds for Distinguished Young
   Scientist (Grant No. JQ200906) and National Natural Science Foundation
   of China (Grant No. 20971077).
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PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0008-6223
EI 1873-3891
J9 CARBON
JI Carbon
PD MAR
PY 2012
VL 50
IS 3
BP 1355
EP 1362
DI 10.1016/j.carbon.2011.11.007
PG 8
WC Chemistry, Physical; Materials Science, Multidisciplinary
SC Chemistry; Materials Science
GA 895BR
UT WOS:000300471700072
ER

PT J
AU Chen, WF
   Zhu, ZY
   Li, SR
   Chen, CH
   Yan, LF
AF Chen, Wufeng
   Zhu, Zhiye
   Li, Sirong
   Chen, Chunhua
   Yan, Lifeng
TI Efficient preparation of highly hydrogenated graphene and its
   application as a high-performance anode material for lithium ion
   batteries
SO NANOSCALE
LA English
DT Article
ID ENERGY-STORAGE; REVERSIBLE HYDROGENATION; CARBONACEOUS MATERIALS;
   SHEETS; GRAPHANE; OXIDE; NANOSHEETS; REDUCTION; INSERTION; CAPACITY
AB A novel method has been developed to prepare hydrogenated graphene (HG) via a direct synchronized reduction and hydrogenation of graphene oxide (GO) in an aqueous suspension under Co-60 gamma ray irradiation at room temperature. GO can be reduced by the aqueous electrons (e(aq)(-)) while the hydrogenation takes place due to the hydrogen radicals formed in situ under irradiation. The maximum hydrogen content of the as-prepared highly hydrogenated graphene (HHG) is found to be 5.27 wt% with H/C = 0.76. The yield of the target product is on the gram scale. The as-prepared HHG also shows high performance as an anode material for lithium ion batteries.
C1 [Chen, Wufeng; Zhu, Zhiye; Yan, Lifeng] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
   [Chen, Wufeng; Zhu, Zhiye; Yan, Lifeng] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China.
   [Li, Sirong; Chen, Chunhua] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China.
RP Yan, LF (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China.
EM lfyan@ustc.edu.cn
RI Yan, Lifeng/D-5350-2009; Chen, Chunhua/F-5897-2010
FU National Natural Science Foundation of China [51073147, J1030412];
   National Basic Research Program of China [2010CB923302, 2011CB921403];
   Fundamental Research Funds for the Central Universities
FX This work is supported by the National Natural Science Foundation of
   China (No. 51073147 and No. J1030412), the National Basic Research
   Program of China (No. 2010CB923302 and 2011CB921403), and the
   Fundamental Research Funds for the Central Universities. WF Chen and ZY
   Zhu contributed equally to this work.
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NR 34
TC 30
Z9 31
U1 10
U2 66
PU ROYAL SOC CHEMISTRY
PI CAMBRIDGE
PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS,
   ENGLAND
SN 2040-3364
J9 NANOSCALE
JI Nanoscale
PY 2012
VL 4
IS 6
BP 2124
EP 2129
DI 10.1039/c2nr00034b
PG 6
WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
   Science, Multidisciplinary; Physics, Applied
SC Chemistry; Science & Technology - Other Topics; Materials Science;
   Physics
GA 901XC
UT WOS:000301000900034
PM 22334350
ER

EFEF